{"id":10311,"date":"2016-04-26T22:00:13","date_gmt":"2016-04-26T14:00:13","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=10311"},"modified":"2016-04-27T14:58:47","modified_gmt":"2016-04-27T06:58:47","slug":"%e7%be%8e%e5%9b%bd%e5%8c%96%e5%ad%a6%e4%bc%9a%ef%bc%88acs%ef%bc%89ncmnca%e9%94%82%e7%94%b5%e6%ad%a3%e6%9e%81%e6%9d%90%e6%96%99%e6%b1%87%e6%80%bb%e3%80%90%e6%96%b0%e8%83%bd%e6%ba%90160426%e6%9c%9f","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=10311","title":{"rendered":"\u7f8e\u56fd\u5316\u5b66\u4f1a\uff08ACS\uff09NCM&NCA\u4e09\u5143\u9502\u7535\u6b63\u6781\u6750\u6599\u6c47\u603b\u3010\u65b0\u80fd\u6e90160426\u671f\u3011"},"content":{"rendered":"

\u9502\u7535\u6c60\u4e09\u5143\u6b63\u6781\u6750\u6599NCM\u548cNCA\u5bb9\u91cf\u5927\u3001\u7535\u538b\u5e73\u53f0\u9ad8\u3001\u632f\u5b9e\u5bc6\u5ea6\u5927\u3001\u4f4e\u6e29\u6027\u80fd\u597d\uff0c\u56e0\u6b64\u5177\u6709\u5e7f\u9614\u7684\u5e94\u7528\u524d\u666f\u3002\u4f46\u662f\u4e09\u5143\u6750\u6599\u4e5f\u6709\u81ea\u8eab\u7684\u7f3a\u70b9\uff0c\u6bd4\u5982\u70ed\u7a33\u5b9a\u6027\u548c\u5b89\u5168\u6027\u5dee\u3002\u56e0\u6b64\uff0c\u4ece\u4e0d\u540c\u89d2\u5ea6\u51fa\u53d1\u6539\u5584\u4e09\u5143\u6750\u6599\u7684\u7f3a\u70b9\u5bf9\u4e8e\u63d0\u5347\u5176\u6027\u80fd\u663e\u5f97\u5c24\u4e3a\u91cd\u8981\u3002\u672c\u6587\u4e2d\u6211\u4eec\u6c47\u603b\u4e86\u8fd1\u671f\u7f8e\u56fd\u5316\u5b66\u4f1a\uff08ACS\uff09\u5728\u4e09\u5143\u6750\u6599\u65b9\u9762\u7684\u6700\u65b0\u8fdb\u5c55\u3002<\/p>\n

1. \u63ed\u79d8\u5bcc\u954d\u4e09\u5143\u6b63\u6781\u6750\u6599LiNi1-2x<\/sub>Cox<\/sub>Mnx<\/sub>O2<\/sub>\uff08NCM\uff09\u4e0d\u7a33\u5b9a\u6027\u539f\u56e0<\/p>\n

\"1-1\"<\/p>\n

\u8fc7\u53bb\u51e0\u5341\u5e74\u91cc\uff0c\u4e09\u5143\u5c42\u72b6\u6b63\u6781\u5bcc\u954d\u6750\u6599LiNi1-2x<\/sub>Cox<\/sub>Mnx<\/sub>O2<\/sub>\uff08x<0.2\uff09\u56e0\u4e3a\u5b83\u7684\u9ad8\u80fd\u91cf\u5bc6\u5ea6\uff08>200mAh\/g\uff09\uff0c\u5f15\u8d77\u4e86\u5e7f\u6cdb\u5173\u6ce8\u3002Ni\u3001Co\u3001Mn\u4e4b\u95f4\u4e0d\u540c\u7684\u914d\u6bd4\u4e5f\u5f71\u54cd\u4e86\u6750\u6599\u7684\u6027\u80fd\u3002\u5bcc\u954d\u7684NCM\u6709\u52a9\u4e8e\u63d0\u9ad8\u5bb9\u91cf\uff0c\u9530\u5219\u63d0\u9ad8\u4e86\u6750\u6599\u7684\u7a33\u5b9a\u6027\uff0c\u94b4\u80fd\u4f18\u5316\u6750\u6599\u7684\u500d\u7387\u6027\u80fd\u3002<\/p>\n

\u8fd1\u65e5\uff0c\u5fb7\u514b\u8428\u65af\u5927\u5b66\u8fbe\u62c9\u65af\u5206\u6821\u4e00\u7814\u7a76\u56e2\u961f\u63a2\u7d22\u4e86\u8fc7\u6e21\u91d1\u5c5eNi\u3001Co\u3001Mn\u7684\u4e0d\u540c\u4ef7\u6001\u79bb\u5b50\u5bf9LiTMO2<\/sub>\uff08TM\u4e3a\u8fc7\u6e21\u91d1\u5c5e\u79bb\u5b50\uff09\u6750\u6599\u7a33\u5b9a\u6027\u7684\u5f71\u54cd\uff0c\u57fa\u4e8e\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\uff08DFT\uff09\u3001\u6676\u4f53\u7ed3\u6784\u5206\u6790\u3001\u76f8\u56fe\u3001TM\u2014TM\u952e\u5206\u6790\u7b49\u65b9\u6cd5\uff0c\u5f97\u51fa\u4e0a\u56fe\u7ed3\u8bba\uff0c\u5e76\u7814\u7a76\u4e86\u5728\u4e0d\u540c\u7684\u954d\u3001\u94b4\u3001\u9530\u539f\u5b50\u914d\u6bd4\u5bf9\u6750\u6599\u7a33\u5b9a\u6027\u5f71\u54cd\u3002\u8be5\u76f8\u56fe\u4e2d\u4e0d\u4ec5\u5305\u542b\u4e86TM\u2014TM\u952e\u5f3a\u5ea6\u987a\u5e8f\u7684\u4fe1\u606f\uff0c\u8fd8\u4e3a\u8bbe\u8ba1\u6700\u4f18\u7684NCM\u6b63\u6781\u6750\u6599\u63d0\u4f9b\u4e86\u6307\u5bfc\u610f\u4e49\u3002<\/p>\n

\u6587\u732e\u9898\u76ee\uff1aUnraveling the Origin of Instability in Ni-Rich LiNi1\u22122x<\/sub>Cox<\/sub>Mnx<\/sub>O2<\/sub> (NCM) Cathode Materials<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttp:\/\/pubs.acs.org\/doi\/pdfplus\/10.1021\/acs.jpcc.6b00369<\/a><\/p>\n

2. \u516b\u9762\u4f53Li(Ni1\/3<\/sub>Co1\/3<\/sub>Mn1\/3<\/sub>)O2<\/sub>\u5355\u6676\u5728\u7194\u878d\u76d0Na2<\/sub>SO4<\/sub>\u4e2d\u7684\u751f\u957f\u673a\u5236\u7814\u7a76<\/p>\n

\"2-1\"<\/p>\n

\u5f62\u72b6\u53ef\u63a7\u7684\u6676\u4f53\u5408\u6210\u5728\u6750\u6599\u5316\u5b66\u5c24\u4e3a\u91cd\u8981\uff0c\u8bb8\u591a\u79d1\u5b66\u5bb6\u901a\u8fc7\u6eb6\u80f6\u2014\u51dd\u80f6\u6cd5\u5f97\u5230\u7279\u5b9a\u5f62\u72b6\u7684\u4e9a\u5fae\u6676\u4f53\u9897\u7c92\uff0c\u7136\u800c\u5728\u9ad8\u6e29\u65f6\uff0c\u6676\u4f53\u7684\u805a\u96c6\u662f\u4e0d\u89c4\u5f8b\u7684\u3002<\/p>\n

\u65e5\u672c\u4fe1\u5dde\u5927\u5b66\u7684\u7814\u7a76\u56e2\u961f\u7814\u7a76\u4e86\u5bfc\u9502\u6750\u6599Li(Ni1\/3<\/sub>Co1\/3<\/sub>Mn1\/3<\/sub>)O2<\/sub>\u6676\u4f53\u5728\u7194\u878d\u76d0\u4e2d\u7684\u751f\u957f\u673a\u5236\uff0c\u8003\u8651\u4e86\u6eb6\u8d28\u6d53\u5ea6\u3001\u6e29\u5ea6\u548c\u4fdd\u6e29\u65f6\u95f4\u7b49\u7684\u5f71\u54cd\u56e0\u7d20\uff0c\u4f7f\u7528XRD\u3001SEM\u548c\u70ed\u91cd\u5206\u6790\u7b49\u65b9\u6cd5\u5206\u6790\u4e86\u6240\u5f97\u4ea7\u7269\u7684\u6676\u578b\u548c\u751f\u957f\u673a\u5236\u3002\u4ed6\u4eec\u53d1\u73b0\uff0cNa+<\/sup>\u5bf9\u6676\u4f53\u751f\u957f\u548c\u6676\u9762\u5b8c\u6574\u5177\u6709\u91cd\u8981\u4f5c\u7528\u3002<\/p>\n

\u6587\u732e\u9898\u76ee\uff1aGrowth Manner of Octahedral-Shaped Li(Ni1\/3<\/sub>Co1\/3<\/sub>Mn1\/3<\/sub>)O2<\/sub> Single Crystals in Molten Na2<\/sub>SO4<\/sub><\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttp:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acs.cgd.5b01723<\/a><\/p>\n

3\u3001\u901a\u8fc7Li\u2212Ni\u2212Co\u2212Mn\u56db\u5143\u76f8\u56fe\u7814\u7a76NCM\u6750\u6599\u7684\u5bb9\u91cf<\/p>\n

\"3-1\"<\/p>\n

\"3-2\"<\/p>\n

\u5728\u76ee\u524d\u5546\u4e1a\u5316\u5e94\u7528\u7684NCM\u6750\u6599\u6709LiNi1\/3<\/sub>Co1\/3<\/sub>Mn1\/3<\/sub>O2<\/sub>\uff08NCM111\uff09LiNi0.5<\/sub>Co0.2<\/sub>Mn0.3<\/sub>O2<\/sub>\uff08NCM523\uff09,\u4f46\u8fd9\u4e9b\u5c42\u72b6\u6750\u6599\u7684\u80fd\u91cf\u5bc6\u5ea6\u4ecd\u6709\u5f85\u63d0\u9ad8\uff0c\u8fd9\u5c31\u9700\u8981\u7814\u7a76\u4e0d\u540cNCM\u539f\u5b50\u914d\u6bd4\u60c5\u51b5\u4e0b\u76f8\u6001\u4e0e\u7ed3\u6784\u7684\u53d8\u5316\u3002<\/p>\n

\u5fb7\u514b\u8428\u65af\u5927\u5b66\u8fbe\u62c9\u65af\u5206\u6821\u4e00\u7814\u7a76\u56e2\u961f\u7814\u7a76\u4e86\u5f53Mn\/Co=1:1, Mn\/Ni=1:1, \u548c Co\/Ni = 1:1\u65f6\u7684NCM\u7684\u5316\u5408\u7269\uff0c\u7ed8\u5236\u4e86\u56db\u5143\u76f8\u56fe\uff0c\u5e76\u5bf9\u6240\u5f97\u6750\u6599\u8fdb\u884c\u8868\u5f81\u3002\u7ed3\u679c\u53ef\u5f97\u954d\u3001\u94b4\u3001\u9530\u8fc7\u6e21\u91d1\u5c5e\u79bb\u5b50\u5bf9\u6b63\u6781\u6750\u6599\u70ed\u529b\u5b66\u7a33\u5b9a\u6027\u548c\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u7684\u5f71\u54cd\uff1b\uff0c\u6839\u636e\u6240\u5f97\u7ed3\u679c\uff0c\u53ef\u8bbe\u8ba1\u4e0d\u540cNCM\u914d\u6bd4\u7684\u6750\u6599\uff0c\u5f97\u5230\u8f83\u9ad8\u7684\u7535\u5b50\u548c\u79bb\u5b50\u8fc1\u79fb\u7387\uff0c\u63d0\u9ad8\u6750\u6599\u7684\u6bd4\u5bb9\u91cf\u548c\u500d\u7387\u6027\u80fd\u3002<\/p>\n

\u6587\u732e\u9898\u76ee\uff1aTransition Metal Ordering Optimization for High-Reversible Capacity Positive Electrode Materials in the Li\u2212Ni\u2212Co\u2212Mn Pseudoquaternary System<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttp:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acs.jpcc.6b02240<\/a><\/p>\n

4.\u4e9a\u78f7\u9178\u76d0\u4f5c\u4e3a\u9502\u79bb\u5b50\u7535\u6c60\u7535\u89e3\u8d28\u6dfb\u52a0\u5242\u7684\u7814\u7a76<\/p>\n

\"4-1\"<\/p>\n

\"4-2\"<\/p>\n

\u5728NCM523\u4e3a\u6b63\u6781\u6750\u6599\u7684\u7535\u6c60\u4e2d\uff0c\u5931\u6548\u7684\u539f\u56e0\u4e00\u822c\u6709\u5faa\u73af\u65f6\u5c16\u6676\u77f3\u7ed3\u6784\u7684\u53d8\u5316\uff0c\u7535\u89e3\u8d28\u819c\u7684\u6c89\u79ef\u53d8\u539a\uff0c\u4f20\u7edf\u78b3\u9178\u76d0\u7535\u89e3\u8d28\u5728\u9ad8\u7535\u538b\u65f6\u7684\u5206\u89e3\u7b49\u3002\u800c\u89e3\u51b3\u8fd9\u4e9b\u95ee\u9898\u7684\u65b9\u6cd5\u6709\u6dfb\u52a0\u9634\u6781\u8868\u9762\u6d82\u5c42\u7c92\u5b50\uff0c\u5408\u6210\u8010\u9ad8\u538b\u7684\u7a33\u5b9a\u7535\u89e3\u8d28\uff0c\u5bfb\u627e\u5408\u9002\u7684\u7535\u89e3\u8d28\u6dfb\u52a0\u5242\u7b49\u3002<\/p>\n

\u963f\u8d21\u56fd\u5bb6\u5b9e\u9a8c\u5ba4\u7814\u7a76\u4e86\u5728NCM523\/\u77f3\u58a8\u7535\u6c60\u4e2d\uff0c\u4e09\u4e59\u57fa\u4e9a\u78f7\u9178(TEP)\u548c\u4e09(2,2,2\u2014\u4e09\u6c1f\u4e59\u57fa)\u4e9a\u78f7\u9178(TTFP)\u4f5c\u4e3a\u7535\u89e3\u8d28\u6dfb\u52a0\u5242\u7684\u5f71\u54cd\u3002TEP\u548cTTFP\u90fd\u6709\u6bd4\u6eb6\u5242\u66f4\u4f4e\u7684\u6c27\u5316\u7535\u52bf\uff0c\u5f53\u7535\u89e3\u8d28\u542b\u67091wt%\u7684TTFP\u65f6\uff0c\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd\u5f97\u5230\u4e86\u6539\u5584\u3002\u8fd9\u79cd\u53d8\u5316\u53ef\u5f52\u56e0\u4e8eTTFP\u5728\u7535\u6c60\u9996\u6b21\u5faa\u73af\u7684\u9009\u62e9\u6027\u5206\u89e3\uff0c\u5bfc\u81f4\u4e86\u9634\u6781\u7684\u6539\u6027\u4fee\u9970\u3002\u8fd9\u79cd\u6539\u6027\u53ef\u4ee5\u6291\u5236\u7535\u89e3\u8d28\u7684\u6c27\u5316\u5206\u89e3\uff0c\u5728\u7535\u6781\u8868\u9762\u5f62\u6210\u4fdd\u62a4\u819c\u3002\u5f53\u7535\u89e3\u8d28\u4e2d\u542b\u67091wt%\u7684TEP\u65f6\uff0c\u6dfb\u52a0\u5242\u7684\u5206\u89e3\u5728\u7535\u6781\u8868\u9762\u5f62\u6210\u81f4\u5bc6\u5c42\uff0c\u5e76\u4fdd\u62a4\u7535\u89e3\u8d28\uff0c\u963b\u6b62\u5176\u8fdb\u4e00\u6b65\u5206\u89e3\uff0c\u4f46\u540c\u65f6\u4e5f\u963b\u788d\u4e86\u9502\u79bb\u5b50\u7684\u8fd0\u8f93\uff0c\u589e\u52a0\u4e86\u754c\u9762\u963b\u6297\u3002<\/p>\n

\u6587\u732e\u9898\u76ee\uff1aMechanistic Insight in the Function of Phosphite Additives for Protection<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttp:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acsami.6b01544<\/a><\/p>\n

5.\u9502\u79bb\u5b50\u4e0d\u540c\u6b63\u6781\u6750\u6599\u7684\u70ed\u7a33\u5b9a\u6027\u548c\u6d3b\u6027\u7684\u7814\u7a76<\/p>\n

\"5-1\"<\/p>\n

\"5-2\"<\/p>\n

\u76ee\u524d\uff0c\u666e\u904d\u5546\u4e1a\u5316\u7684\u9502\u79bb\u5b50\u7535\u6c60\u6750\u6599\u6709LiMO2<\/sub>\uff08M=Mn,Co,Ni\uff09\u548cLiMPO4<\/sub>\uff08M=Fe,Mn,Co,Ni\uff09\u7136\u800c\uff0c\u5145\u7535\u72b6\u6001\u65f6\uff0cMnPO4<\/sub>\u5728\u4f4e\u4e8e400\u2103\u65f6\u5c31\u53d1\u751f\u5206\u89e3\u5e76\u91ca\u653e\u51fa\u5927\u91cf\u6c27\u6c14\uff0c\u9020\u6210\u7535\u6c60\u7684\u4e0d\u5b89\u5168\u6027\u3002VOPO4<\/sub>\u80fd\u4e0e\u4e24\u4e2aLi+<\/sup>\u53ef\u9006\u5730\u5d4c\u5165\u8131\u51fa\u53cd\u5e94\uff0c\u6709\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u548c\u826f\u597d\u7684\u70ed\u7a33\u5b9a\u6027\uff0c\u6210\u4e3a\u53e6\u4e00\u6709\u524d\u666f\u7684\u6b63\u6781\u6750\u6599\u3002\u7136\u800c\uff0cVOPO4<\/sub>\u6709\u53ef\u80fd\u4e0e\u6709\u673a\u7535\u89e3\u6db2\u53d1\u751f\u53cd\u5e94\u3002\u56e0\u4e3a\uff0c\u7535\u89e3\u6db2\u4e2d\u5f80\u5f80\u6709\u57fa\u4e8eV\/P\/O\u7684\u50ac\u5316\u5242\u3002<\/p>\n

\u5728\u8fd9\u7bc7\u7814\u7a76\u62a5\u5bfc\u4e2d\uff0c\u5bbe\u6c49\u59c6\u987f\u5927\u5b66\u7814\u7a76\u4eba\u5458\u7740\u91cd\u7814\u7a76\u4e86\u7535\u6781\u6750\u6599\u4e0e\u7535\u89e3\u6db2\u4e4b\u95f4\u7684\u5173\u7cfb\u548cLiVOPO4<\/sub> \u548cLi2<\/sub>VOPO4<\/sub>\u7684\u70ed\u7a33\u5b9a\u6027\u3002\u7535\u6781\u6750\u6599\u6709\u4e09\u7c7b\uff0c\u5c42\u72b6\u6c27\u5316\u7269LiNi0.8<\/sub>Co0.15<\/sub>Al0.05<\/sub>O2<\/sub> (NCA)\uff1b\u6a44\u6984\u77f3\u578b\u78f7\u9178\u76d0 LiFePO4 <\/sub>(LFP) \uff0c\u5bcc\u9530\u6750\u6599LiMn0.8<\/sub>Fe0.2<\/sub>PO4<\/sub>(LMFP)\u548c\u591a\u7535\u5b50\u9492\u6c27\u57fa\u78f7\u9178\u76d0VOPO4<\/sub>\u3001LiVOPO4<\/sub>\u548c Li2<\/sub>VOPO4<\/sub>\uff0c\u7535\u89e3\u6db2\u4e3a1 M LiPF6<\/sub>(EC\/DMC=1:1)\u3002\u70ed\u7a33\u5b9a\u6027\u987a\u5e8f\u8868\u4e3aNCA < VOPO4 < MFP < FP\u3002\u7ed3\u679c\u8868\u660e\uff0c\u4e0d\u540c\u4e8eMFP\uff0cVOPO4<\/sub>\u53d7\u70ed\u65f6\u4e0d\u4ea7\u751f\u6c27\u6c14\uff0c\u56e0\u6b64\u9ad8\u6e29\u65f6\u8f83\u4e0d\u4f1a\u6709\u70ed\u5931\u63a7\u7684\u73b0\u8c61\uff0c\u56e0\u6b64\u66f4\u5b89\u5168\uff1b\u867d\u7136\u4e0e\u7535\u89e3\u6db2\u63a5\u89e6\u8f83\u4e3a\u7a33\u5b9a\uff0c\u4f46\u662f\u5728\u5bc6\u5c01\u9ad8\u538b\u5b9e\u9a8c\u4e2d\uff0c200\u2014300\u2103\u6761\u4ef6\u4e0b\uff0cVOPO4<\/sub>\u5b58\u5728\u8fd9\u6837\u4e00\u4e2a\u8f6c\u53d8\uff1aVOPO4<\/sub> \u2192 HVOPO4 <\/sub>\u2192 H2<\/sub>VOPO4<\/sub>\u3002<\/p>\n

\u6587\u732e\u9898\u76ee\uff1aThermal Stability and Reactivity of Cathode Materials for Li-Ion Batteries<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttp:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acsami.5b12081<\/a><\/p>\n

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