{"id":103979,"date":"2017-10-08T06:30:08","date_gmt":"2017-10-07T22:30:08","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=103979"},"modified":"2017-10-07T16:50:44","modified_gmt":"2017-10-07T08:50:44","slug":"%e6%8a%95%e7%a8%bf%e5%be%85%e5%ae%9a%e8%b6%85%e8%96%84moox%e9%98%b4%e6%9e%81%e7%bc%93%e5%86%b2%e5%b1%82%e5%af%b9%e5%85%a8%e6%97%a0%e6%9c%bacspbibr2%e9%92%99%e9%92%9b%e7%9f%bf%e5%a4%aa%e9%98%b3","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=103979","title":{"rendered":"\u8d85\u8584MoOx\u9634\u6781\u7f13\u51b2\u5c42\u5bf9\u5168\u65e0\u673aCsPbIBr2\u9499\u949b\u77ff\u592a\u9633\u7535\u6c60\u6027\u80fd\u7684\u63d0\u5347"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u5728\u77ed\u77ed\u7684\u4e03\u5e74\u65f6\u95f4\u5185\uff0c\u57fa\u4e8e\u6709\u673a-\u65e0\u673a\u6742\u5316\u7684\u9499\u949b\u77ff\u592a\u9633\u7535\u6c60\u7684\u80fd\u91cf\u8f6c\u6362\u6548\u7387\u75313.8%\u63d0\u5347\u81f322.1%1-3<\/sup>\uff0c\u8868\u73b0\u51fa\u5de8\u5927\u7684\u5546\u4e1a\u6f5c\u529b\u3002\u4f46\u662f\uff0c\u6750\u6599\u53ca\u5668\u4ef6\u4e2d\u6709\u673a\u6750\u6599\u7684\u4f7f\u7528\uff0c\u5927\u5927\u964d\u4f4e\u4e86\u7535\u6c60\u5668\u4ef6\u7684\u70ed\u7a33\u5b9a\u6027\uff0c\u8fdb\u800c\u9650\u5236\u4e86\u5176\u8fdb\u4e00\u6b65\u7684\u53d1\u5c55\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

9\u670811\u53f7\uff0cNano Energy<\/strong>\u5728\u7ebf\u53d1\u8868\u4e86\u9898\u4e3a\u201cUltra-thin MoOx<\/sub>\u00a0as cathode buffer layer for the improvement of all-inorganic CsPbIBr2<\/sub>\u00a0perovskite solar cells<\/strong>\u201d\u7684\u7814\u7a76\u8bba\u6587\uff0c\u901a\u8baf\u4f5c\u8005\u4e3a\u66a8\u5357\u5927\u5b66\u65b0\u80fd\u6e90\u6280\u672f\u7814\u7a76\u9662\u7684\u8303\u5efa\u4e1c\u6559\u6388\u53ca\u9ea6\u8000\u534e\u6559\u6388\u3002<\/p>\n

\u3010\u672c\u6587\u4eae\u70b9\u3011<\/b><\/strong><\/p>\n

\u672c\u6587\u5f00\u53d1\u4e86\u4e00\u79cd\u901a\u8fc7\u201c\u7a33\u5b9a\u8fc7\u6e21\u76f8\u8584\u819c\u201d\u5236\u5907\u9ad8\u81f4\u5bc6\u3001\u9ad8\u6eb4\u542b\u91cf\u7684CsPbIBr2<\/sub>\u65e0\u673a\u9499\u949b\u77ff\u8584\u819c\uff0c\u5e76\u5236\u5907\u4e86\u7ed3\u6784\u4e3a(FTO\/NiOx<\/sub>\/CsPbIBr2<\/sub>\/MoOx<\/sub>\/Au)\u7684\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u7535\u6c60\u5668\u4ef6\u3002\u5728\u672c\u6587\u4e2d\uff0c\u8d85\u8584MoOx<\/sub>\u8584\u819c\u7ecf\u6c2e\u6c14\u73af\u5883\u4e2d\u9ad8\u6e29\u9000\u706b\u540e\u8868\u73b0\u51fa\u4f4e\u529f\u51fd\u7684n\u578b\u534a\u5bfc\u4f53\u6750\u6599\u7279\u6027\uff0c\u5c06\u5176\u4f5c\u4e3a\u9634\u6781\u7f13\u51b2\u5c42\u80fd\u591f\u6709\u6548\u7684\u964d\u4f4e\u8096\u7279\u57fa\u52bf\u5792\u3001\u63a5\u89e6\u7535\u963b\u548c\u754c\u9762\u7f3a\u9677\uff0c\u8fdb\u800c\u5668\u4ef6\u6548\u7387\u4e5f\u75311.3%\u63d0\u5347\u81f35.52%\u3002\u6b64\u5916\uff0c\u8be5\u7ed3\u6784\u7684\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u7535\u6c60\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u70ed\u7a33\u5b9a\u6027\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe1. <\/b>\u201c\u7a33\u5b9a\u8fc7\u6e21\u76f8\u8584\u819c\u201d\u5236\u5907CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819c<\/strong><\/p>\n

\u5c06CsPbIBr2<\/sub>\u524d\u9a71\u6db2\u65cb\u6d82\u4e8e\u4ee5NiOx<\/sub>\u4f5c\u4e3a\u7a7a\u7a74\u4f20\u8f93\u5c42\u7684\u57fa\u7247\u4e0a\uff0c\u968f\u540e\u5c06\u5176\u572830\u2103\u7684\u70ed\u53f0\u4e0a\u8fdb\u884c\u653e\u7f6e\uff0c\u968f\u7740\u65f6\u95f4\u7684\u63a8\u79fb\uff0c\u8584\u819c\u7684\u989c\u8272\u9010\u6e10\u7531\u65e0\u8272\u8f6c\u53d8\u4e3a\u6a59\u9ec4\u8272\uff08\u56fea1\uff09\uff0c\u5373\u751f\u6210\u201c\u7a33\u5b9a\u8fc7\u6e21\u76f8\u8584\u819c\u201d\u3002\u7ee7\u800c\u5c06\u70ed\u53f0\u6e29\u5ea6\u5347\u81f3160\u2103\uff0c\u70d8\u5e72\u6eb6\u5242\u5e76\u4fc3\u8fdb\u8584\u819c\u7684\u8fdb\u4e00\u6b65\u7ed3\u6676\uff08\u56fea2\uff09\u3002<\/p>\n

\"\"<\/p>\n

(a)\u201c\u7a33\u5b9a\u8fc7\u6e21\u76f8\u8584\u819c\u201d\u5236\u5907CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819c\u6d41\u7a0b\u793a\u610f\u56fe<\/p>\n

(b)\u201c\u7a33\u5b9a\u8fc7\u6e21\u76f8\u8584\u819c\u201d\u5236\u5907CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819c\u7ed3\u6676\u52a8\u529b\u5b66\u8fc7\u7a0b\u793a\u610f\u56fe<\/p>\n

(c)\u201c\u7a33\u5b9a\u8fc7\u6e21\u76f8\u8584\u819c\u201d\u5236\u5907CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819cXRD\u6f14\u53d8\u8fc7\u7a0b<\/p>\n

\u56fe2.<\/b><\/strong>\u00a0CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819c\u53ca\u65e0\u7535\u5b50\u4f20\u8f93\u5c42\u5668\u4ef6\u6027\u80fd\u8868\u5f81<\/strong><\/p>\n

\u5236\u5907\u7684CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819c\u5177\u6709\u5747\u5300\u3001\u81f4\u5bc6\u7b49\u7279\u70b9\uff0c\u5e76\u4e14\u65e0\u660e\u663e\u7684\u76f8\u5206\u79bb\u3002\u7531\u4e8e\u5b58\u5728\u8f83\u5f3a\u7684\u8096\u7279\u57fa\u52bf\u5792\uff0c\u65e0\u7535\u5b50\u4f20\u8f93\u5c42\u7535\u6c60\u5668\u4ef6\u8868\u73b0\u51fa\u8f83\u5dee\u7684\u5149\u4f0f\u6027\u80fd\u3002<\/p>\n

\"\"<\/p>\n

(a)\u00a0CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819c\u8868\u9762SEM\u56fe<\/p>\n

(b)\u00a0CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819c\u8868\u9762EDS-Mapping\u56fe<\/p>\n

(c)\u00a0FTO\/NiOx<\/sub>\/CsPbIBr2<\/sub>\/Au\u65e0\u7535\u5b50\u4f20\u8f93\u5c42\u5668\u4ef6I-V\u6d4b\u8bd5\u66f2\u7ebf<\/p>\n

(d)\u00a0CsPbIBr2<\/sub>\/Au\u8096\u7279\u57fa\u52bf\u5792\u793a\u610f\u56fe<\/p>\n

\u56fe3.<\/b><\/strong>\u00a0FTO\/NiOx<\/sub>\/CsPbIBr2<\/sub>\/MoOx<\/sub>\/Au\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u7535\u6c60\u5668\u4ef6\u80fd\u5e26\u6392\u5217<\/strong><\/p>\n

CsPbIBr2<\/sub>\u5728\u5668\u4ef6\u5185\u57fa\u672c\u4e3a\u8d2f\u7a7f\u819c\uff0c\u8868\u73b0\u51fa\u826f\u597d\u7684\u7ed3\u6676\u6027\u80fd\uff1b\u4f4e\u529f\u51fdMoOx<\/sub>\u4e0eCsPbIBr2<\/sub>\u9499\u949b\u77ff\u6750\u6599\u5f62\u6210\u826f\u597d\u7684\u80fd\u5e26\u9635\u5217\uff0c\u6709\u5229\u4e8e\u7535\u5b50\u7684\u8403\u53d6\u3002<\/p>\n

\"\"<\/p>\n

(a)\u00a0FTO\/NiOx<\/sub>\/CsPbIBr2<\/sub>\/MoOx<\/sub>\/Au\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u7535\u6c60\u5668\u4ef6\u622a\u9762SEM\u56fe<\/p>\n

(b,c)\u00a0CsPbIBr2<\/sub>\u53caMoOx<\/sub>\u7684UPS\u6d4b\u8bd5\u7684\u7ed3\u5408\u80fd\u66f2\u7ebf<\/p>\n

(d)\u00a0FTO\/NiOx<\/sub>\/CsPbIBr2<\/sub>\/MoOx<\/sub>\/Au\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u7535\u6c60\u5668\u4ef6\u80fd\u5e26\u6392\u5217<\/p>\n

(e,f)\u00a0MoOx<\/sub>\u5bf9\u4e8eCsPbIBr2<\/sub>\u8584\u819c\u7684\u7535\u5b50\u8403\u53d6\u4f5c\u7528<\/p>\n

\u56fe4. <\/b>MoOx<\/sub>\u9634\u6781\u7f13\u51b2\u5c42\u964d\u4f4e\u8584\u819c\u63a5\u89e6\u7535\u963b\u4f5c\u7528<\/strong><\/p>\n

MoOx<\/sub>\u8986\u76d6\u5728CsPbIBr2<\/sub>\u8584\u819c\u8868\u9762\uff0c\u964d\u4f4e\u4e86\u8584\u819c\u7684\u7c97\u7cd9\u5ea6\uff0c\u5e76\u4e14\u660e\u663e\u7684\u6539\u5584\u4e86\u8584\u819c\u8868\u9762\u7684\u6d78\u6da6\u6027\uff0c\u4ece\u800c\u6709\u5229\u4e8e\u66f4\u597d\u7684\u7535\u6781\u63a5\u89e6\u3002<\/p>\n

\"\"<\/p>\n

(a)\u00a0CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819c\u8868\u9762AFM\u56fe<\/p>\n

(b)\u00a0CsPbIBr2<\/sub>\/MoOx<\/sub>\u8584\u819c\u8868\u9762AFM\u56fe<\/p>\n

(c)\u00a0CsPbIBr2<\/sub>\u9499\u949b\u77ff\u8584\u819c\u8868\u9762\u6c34\u63a5\u89e6\u89d2\u6d4b\u8bd5<\/p>\n

(d)\u00a0CsPbIBr2<\/sub>\/MoOx<\/sub>\u8584\u819c\u8868\u9762\u6c34\u63a5\u89e6\u89d2\u6d4b\u8bd5<\/p>\n

(e) \u6697\u7535\u6d41\u6d4b\u8bd5<\/p>\n

\u56fe5. \u4e0d\u540cMoOx<\/sub>\u539a\u5ea6\u4e0b\u5668\u4ef6\u8f7d\u6d41\u5b50\u4f20\u8f93\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\u8fc7\u8584\u7684MoOx<\/sub>\u7f13\u51b2\u5c42\u4e0d\u80fd\u6709\u6548\u7684\u964d\u4f4e\u8096\u7279\u57fa\u52bf\u5792\uff0c\u8fc7\u539a\u7684MoOx<\/sub>\u7f13\u51b2\u5c42\u6709\u53ef\u80fd\u5bfc\u81f4\u7535\u5b50\u4f20\u8f93\u7535\u963b\u589e\u52a0\u3002<\/p>\n

\"\"<\/p>\n

(a)\u00a0\u65e0\u9634\u6781\u7f13\u51b2\u5c42MoOx<\/sub>\u65f6<\/p>\n

(b)\u00a0\u5408\u9002\u539a\u5ea6\u7684\u9634\u6781\u7f13\u51b2\u5c42MoOx<\/sub><\/p>\n

(c) \u8fc7\u539a\u7684\u9634\u6781\u7f13\u51b2\u5c42MoOx<\/sub>\u65f6<\/p>\n

\u56fe6.\u00a0\u4e0d\u540cMoOx<\/sub>\u539a\u5ea6\u4e0b\u5668\u4ef6\u6027\u80fd\u6d4b\u8bd5<\/strong><\/p>\n

\u5f53MoOx<\/sub>\u9634\u6781\u7f13\u51b2\u5c42\u7684\u539a\u5ea6\u4e3a4nm\u65f6\uff0c\u8fbe\u52305.52%\u6700\u9ad8\u7684\u80fd\u91cf\u8f6c\u6362\u6548\u7387\u3002<\/p>\n

\"\"<\/p>\n

(a)\u00a0\u4e0d\u540cMoOx<\/sub>\u539a\u5ea6\u4e0b\u5668\u4ef6\u6027\u80fd\u7edf\u8ba1<\/p>\n

(b)\u00a0\u6dfb\u52a0\u9634\u6781\u7f13\u51b2\u5c42MoOx<\/sub>\u524d\u540eEQE\u5bf9\u6bd4<\/p>\n

(c) \u6700\u9ad8\u5668\u4ef6I-V\u6d4b\u8bd5\u66f2\u7ebf<\/p>\n

(d) \u5bf9\u5e94\u7684\u7a33\u5b9a\u6548\u7387\u8f93\u51fa<\/p>\n

\u56fe7.<\/b><\/strong>\u00a0FTO\/NiOx<\/sub>\/CsPbIBr2<\/sub>\/MoOx<\/sub>\/Au\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u7535\u6c60\u5668\u4ef6\u70ed\u7a33\u5b9a\u6027\u6d4b\u8bd5<\/strong><\/p>\n

FTO\/NiOx<\/sub>\/CsPbIBr2<\/sub>\/MoOx<\/sub>\/Au\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u7535\u6c60\u5668\u4ef6\u5728160\u2103\u4e0b\uff0c\u6c2e\u6c14\u73af\u5883\u4e2d\u53ca\u7a7a\u6c14\u4e2d\u8868\u73b0\u51fa\u826f\u597d\u7684\u70ed\u7a33\u5b9a\u6027\u3002\u5728\u5ba4\u6e29\u4e0b\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u4fdd\u5b58\u7a33\u5b9a\u6027\u3002<\/p>\n

\"\"<\/p>\n

(a)\u00a0\u6c2e\u6c14\u73af\u5883\u5185\uff0c160\u2103\u52a0\u70ed60min<\/p>\n

(b)\u00a0\u5927\u6c14\u73af\u5883\u5185\uff0c160\u2103\u52a0\u70ed90min<\/p>\n

(c) \u6c2e\u6c14\u73af\u5883\u5185\uff0c\u4fdd\u5b58150\u5929<\/p>\n

(d) \u5927\u6c14\u73af\u5883\u5185\uff0c\u4fdd\u5b5820\u5929<\/p>\n

\u5c55\u671b\uff1a<\/b><\/strong>\u8be5\u5de5\u4f5c\u63d0\u4f9b\u4e86\u4e00\u79cd\u5236\u5907\u9ad8\u6eb4\u542b\u91cf\u7684\u65e0\u673a\u9499\u949b\u77ff\u8584\u819c\u65b0\u65b9\u6cd5\u3002\u7814\u7a76\u8868\u660e\uff0c\u8d85\u8584\u4f4e\u529f\u51fd\u6570n\u578b\u534a\u5bfc\u4f53\u8584\u819cMoOx<\/sub>\u53ef\u7528\u4f5c\u9634\u6781\u7f13\u51b2\u5c42\u6750\u6599\uff0c\u5e76\u80fd\u591f\u6709\u6548\u7684\u964d\u4f4e\u8096\u7279\u57fa\u52bf\u5792\u9ad8\u5ea6\u3002\u6240\u5236\u5907\u7684\u5168\u65e0\u673a\u7535\u6c60\u5668\u4ef6\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u70ed\u7a33\u5b9a\u6027\uff0c\u53ef\u6ee1\u8db3\u7535\u6c60\u5668\u4ef6\u5728\u9ad8\u6e29\u4e0b\u4f7f\u7528\u7684\u9700\u6c42\u3002\u76ee\u524d\uff0c\u8be5\u7c7b\u7535\u6c60\u5668\u4ef6\u6548\u7387\u53d7\u9650\u7684\u4e3b\u8981\u539f\u56e0\u5728\u4e8e\u7a7a\u7a74\u4f20\u8f93\u6750\u6599\u4e0e\u9499\u949b\u77ff\u4e4b\u95f4\u7684\u4ef7\u5e26\u9876\u80fd\u7ea7\u5dee\u8f83\u5927\uff0c\u5bfc\u81f4\u5668\u4ef6Voc<\/sub>\u53d7\u9650\u3002\u56e0\u6b64\uff0c\u672a\u6765\u5f00\u5c55\u7684\u5de5\u4f5c\u5c06\u96c6\u4e2d\u5728\u5bfb\u627e\u80fd\u5e26\u66f4\u4e3a\u5339\u914d\u7684\u7a7a\u7a74\u4f20\u8f93\u6750\u6599\uff0c\u6216\u8005\u5bf9\u73b0\u6709\u7684\u7a7a\u7a74\u4f20\u8f93\u6750\u6599NiOx<\/sub>\u8fdb\u884c\u9633\u6781\u4fee\u9970\uff0c\u4ee5\u671f\u53d6\u5f97\u66f4\u9ad8\u7684\u5668\u4ef6Voc<\/sub>\u3002<\/p>\n

\u53c2\u8003\u6587\u732e\uff1a<\/strong><\/p>\n

[1]\u00a0A. Kojima, K. Teshima, Y. Shirai, T. Miyasaka, J. Am. Chem. Soc. 131 (2009) 6050\u20136051.<\/p>\n

[2]\u00a0M. Liu, M.B. Johnston, H.J. Snaith, Nature 501 (2013) 395\u2212398.<\/p>\n

[3] W.S. Yang, B.-W. Park, E.H. Jung, N.J. Jeon, Y.C. Kim, D.U. Lee, S.S. Shin, J. Seo, E.K. Kim, J.H. Noh, Science 356 (2017) 1376\u20131379.<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aUltra-thin MoOx<\/sub>\u00a0as cathode buffer layer for the improvement of all-inorganic CsPbIBr2<\/sub>\u00a0perovskite solar cells<\/a>\uff08Nano Energy,2017,DOI:10.1016\/j.nanoen.2017.08.048\uff09<\/p>\n

\u6750\u6599\u4eba\u7f16\u8f91\u6574\u7406\u3002<\/p>\n

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