{"id":104796,"date":"2017-10-04T06:30:52","date_gmt":"2017-10-03T22:30:52","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=104796"},"modified":"2017-10-03T21:28:32","modified_gmt":"2017-10-03T13:28:32","slug":"%e6%b5%99%e6%b1%9f%e5%a4%a7%e5%ad%a6acs-nano%ef%bc%9a%e5%9f%ba%e4%ba%8e%e5%85%b7%e6%9c%89%e7%ad%89%e7%a6%bb%e6%bf%80%e5%85%83%e6%95%88%e5%ba%94%e7%9a%84%e6%8e%ba%e6%9d%82%e7%a1%85%e9%87%8f%e5%ad%90","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=104796","title":{"rendered":"\u6d59\u6c5f\u5927\u5b66ACS Nano\uff1a\u57fa\u4e8e\u5177\u6709\u7b49\u79bb\u6fc0\u5143\u6548\u5e94\u7684\u63ba\u6742\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u6742\u5316\u7ed3\u6784\u7684\u8d85\u5bbd\u5149\u8c31\u9ad8\u7075\u654f\u5149\u7535\u63a2\u6d4b\u5668"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u5f53\u524d\uff0c\u7269\u8054\u7f51\u6280\u672f\u548c\u519b\u4e8b\u79d1\u6280\u7684\u5feb\u901f\u53d1\u5c55\u6b63\u5728\u6709\u529b\u63a8\u52a8\u9ad8\u7075\u654f\u5ea6\u3001\u5bbd\u5149\u8c31\u5c24\u5176\u662f\u80fd\u62d3\u5c55\u81f3\u4e2d\u7ea2\u5916\u6ce2\u6bb5\u7684\u5149\u7535\u63a2\u6d4b\u5668\u7684\u7814\u7a76\u3002\u57fa\u4e8e\u77f3\u58a8\u70ef\u548c\u91cf\u5b50\u70b9\u7684\u4e8c\u7ef4\/\u96f6\u7ef4\u6742\u5316\u7ed3\u6784\u7684\u5149\u7535\u63a2\u6d4b\u5668\u5728\u8fd9\u65b9\u9762\u88ab\u5bc4\u4e88\u539a\u671b\u3002\u7136\u800c\u76ee\u524d\u57fa\u4e8e\u77f3\u58a8\u70ef\u548c\u91cf\u5b50\u70b9\uff08\u5982PbS\u548cPbSe\u91cf\u5b50\u70b9\uff09\u7684\u6742\u5316\u7ed3\u6784\u7684\u5149\u7535\u63a2\u6d4b\u5668\u53ea\u80fd\u5728\u7d2b\u5916\u5230\u8fd1\u7ea2\u5916\u6ce2\u6bb5\u5de5\u4f5c\uff0c\u65e0\u6cd5\u5b9e\u73b0\u5bf9\u4e2d\u7ea2\u5916\u5149\u7684\u6709\u6548\u63a2\u6d4b\u3002\u4e2d\u7ea2\u5916\u5149\u7684\u63a2\u6d4b\u4ecd\u7136\u4f9d\u8d56\u4e8e\u4f20\u7edf\u7684\u7a84\u7981\u5e26\u534a\u5bfc\u4f53\u6750\u6599\u5982HgTe\u7b49\u3002\u7136\u800c\u8fd9\u7c7b\u6750\u6599\u9762\u4e34\u7740\u7a33\u5b9a\u6027\u3001\u6bd2\u6027\u548c\u8d44\u6e90\u7a00\u7f3a\u7684\u95ee\u9898\uff0c\u5728\u5927\u89c4\u6a21\u7684\u5e94\u7528\u65b9\u9762\u9762\u4e34\u6311\u6218\u3002<\/p>\n

\u3010\u6210\u679c\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6d59\u6c5f\u5927\u5b66\u7845\u6750\u6599\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u548c\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662\u7531\u6768\u5fb7\u4ec1\u6559\u6388\u9886\u8854\u7684\u7845\u6750\u6599\u7814\u7a76\u56e2\u961f\u7684\u76ae\u5b5d\u4e1c\u6559\u6388\u7814\u7a76\u7ec4\u4e0e\u6d59\u6c5f\u5927\u5b66\u4fe1\u606f\u4e0e\u7535\u5b50\u5de5\u7a0b\u5b66\u9662\u7684\u5f90\u6768\u6559\u6388\u7814\u7a76\u7ec4\u4ee5\u53ca\u4e2d\u56fd\u79d1\u5b66\u9662\u4e0a\u6d77\u6280\u672f\u7269\u7406\u7814\u7a76\u6240\u7684\u80e1\u4f1f\u8fbe\u7814\u7a76\u5458\u7814\u7a76\u7ec4\u5408\u4f5c\u5728ACS Nano\u671f\u520a\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cPlasmonic Silicon Quantum Dots Enabled High-Sensitivity Ultrabroadband Photodetection of Graphene-Based Hybrid Phototransistors\u201d\u7684\u8bba\u6587\uff0c\u502a\u6715\u4f0a\u535a\u58eb\u548c\u9a6c\u73b2\u73b2\u4e3a\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\u3002\u8be5\u8bba\u6587\u62a5\u9053\u4e86\u4e00\u79cd\u57fa\u4e8e\u63ba\u6742\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u6742\u5316\u7ed3\u6784\u7684\u6676\u4f53\u7ba1\u578b\u5149\u7535\u63a2\u6d4b\u5668\uff0c\u5229\u7528\u63ba\u6742\u7845\u91cf\u5b50\u70b9\u5728\u4e2d\u7ea2\u5916\u5149\u6ce2\u6bb5\u7684\u5c40\u57df\u8868\u9762\u7b49\u79bb\u6fc0\u5143\u5171\u632f\u6548\u5e94\uff08LSPR\uff09\u548c\u7d2b\u5916\u5230\u8fd1\u7ea2\u5916\u5149\u6ce2\u6bb5\u7684\u7535\u5b50\u8dc3\u8fc1\u5149\u5b66\u5438\u6536\u7279\u6027\uff0c\u5b9e\u73b0\u4e86\u4ece\u7d2b\u5916\u5149\uff08375nm\uff09\u5230\u4e2d\u7ea2\u5916\u5149\uff084\u03bcm\uff09\u7684\u8d85\u5bbd\u5149\u8c31\u63a2\u6d4b\u3002\u5668\u4ef6\u5728\u7d2b\u5916\u5230\u8fd1\u7ea2\u5916\u5149\u6ce2\u6bb5\u7684\u54cd\u5e94\u5ea6\u53ef\u8fbe109<\/sup> A\/W\uff0c\u6bd4\u63a2\u6d4b\u7387\u53ef\u8fbe1013<\/sup> Jones\uff1b\u5728\u4e2d\u7ea2\u5916\u5149\u6ce2\u6bb5\u54cd\u5e94\u5ea6\u53ef\u8fbe45 A\/W\uff0c\u6bd4\u63a2\u6d4b\u7387\u53ef\u8fbe105<\/sup> Jones\uff0c\u5176\u6027\u80fd\u5728\u5177\u6709\u540c\u7c7b\u578b\u7ed3\u6784\u7684\u5668\u4ef6\u4e2d\u5904\u4e8e\u56fd\u9645\u5148\u8fdb\u6c34\u5e73\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong>1. <\/strong>\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u6742\u5316\u7ed3\u6784\u7684\u5149\u7535\u63a2\u6d4b\u5668\u7684\u7ed3\u6784\u548c\u5de5\u4f5c\u539f\u7406\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

(a)\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u6742\u7ed3\u6784\u7684\u6676\u4f53\u7ba1\u578b\u5149\u7535\u63a2\u6d4b\u5668\u793a\u610f\u56fe\u3002<\/p>\n

(b)\u5668\u4ef6\u7684\u5de5\u4f5c\u539f\u7406\u793a\u610f\u56fe\u3002\u5728\u4e2d\u7ea2\u5916\u5149\uff08MIR\uff09\u6ce2\u6bb5\uff0c\u63ba\u6742\u7845\u91cf\u5b50\u70b9\u7684LSPR\u6548\u5e94\u80fd\u591f\u5728\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u4e4b\u524d\u4ea7\u751f\u589e\u5f3a\u7684\u5c40\u57df\u7535\u573a\uff0c\u8be5\u5c40\u57df\u7535\u573a\u80fd\u591f\u663e\u8457\u589e\u52a0\u77f3\u58a8\u70ef\u5728\u4e2d\u7ea2\u5916\u5149\u6ce2\u6bb5\u7684\u5149\u5b66\u5438\u6536\uff0c\u5f62\u6210\u5149\u7535\u54cd\u5e94\uff1b\u5728\u7d2b\u5916\u5230\u8fd1\u7ea2\u5916\u5149\uff08UV-NIR\uff09\u6ce2\u6bb5\uff0c\u7845\u91cf\u5b50\u70b9\u5e26\u8fb9\u6216\u5e26\u5c3e\u6001\u4e0a\u7684\u7535\u5b50\u5438\u6536\u5149\u5b50\u4ea7\u751f\u8dc3\u8fc1\uff0c\u5f62\u6210\u7535\u5b50-\u7a7a\u7a74\u5bf9\uff0c\u5176\u4e2d\u7535\u5b50\u88ab\u7845\u91cf\u5b50\u70b9\u7684\u7f3a\u9677\u6001\u6240\u4fd8\u83b7\uff0c\u7a7a\u7a74\u5728\u5185\u5efa\u7535\u573a\u7684\u4f5c\u7528\u4e0b\u8f6c\u79fb\u5230\u77f3\u58a8\u70ef\u4e2d\uff0c\u4ea7\u751f\u589e\u5927\u7684\u5149\u7535\u6d41\u3002<\/p>\n

\u56fe<\/strong>2. <\/strong>\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u4e4b\u95f4\u7684\u5c40\u57df\u7535\u573a\u589e\u5f3a\u53ca\u5149\u81f4\u6805\u8c03\u63a7\uff08<\/strong>photogating<\/strong>\uff09\u6548\u5e94<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

(a)\u901a\u8fc7FDTD\u6a21\u62df\u7684\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u4e4b\u95f4\u7684\u7535\u573a\u5f3a\u5ea6\u968f\u5165\u5c04\u5149\u6ce2\u957f\u7684\u53d8\u5316\u3002\u5728\u5165\u5c04\u5149\u4e3a3\u03bcm\u65f6\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u4e4b\u95f4\u7684\u5c40\u57df\u7535\u573a\u8fbe\u5230\u6700\u5927\uff0c\u548c\u7845\u91cf\u5b50\u70b9\u7684LSPR\u5cf0\u4f4d\u76f8\u4e00\u81f4\u3002<\/p>\n

(b)\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u6742\u5316\u7ed3\u6784\u7684\u6676\u4f53\u7ba1\u578b\u5149\u63a2\u6d4b\u5668\u5728\u4e2d\u7ea2\u5916\u5149\u6ce2\u6bb5\uff083 \u03bcm\uff09\u548c\u53ef\u89c1\u5149\u6ce2\u6bb5\uff08532 nm\uff09\u7684\u8f6c\u79fb\u7279\u6027\u66f2\u7ebf\u3002\u5728\u4e2d\u7ea2\u5916\u5149\u6ce2\u6bb5\uff0c\u77f3\u58a8\u70ef\u7684\u8d39\u7c73\u80fd\u7ea7\u4e0d\u968f\u5149\u7167\u53d1\u751f\u53d8\u5316\uff0c\u8868\u660e\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u4e4b\u95f4\u6ca1\u6709\u53d1\u751f\u7535\u8377\u8f6c\u79fb\uff1b\u5728\u7d2b\u5916\u5230\u53ef\u89c1\u5149\u6ce2\u6bb5\uff0c\u5149\u7167\u4ee5\u540e\u77f3\u58a8\u70ef\u7684\u8d39\u7c73\u80fd\u7ea7\u5411\u4e0a\u79fb\u52a8\uff0c\u8868\u660e\u7a7a\u7a74\u4ece\u7845\u91cf\u5b50\u70b9\u6ce8\u5165\u5230\u77f3\u58a8\u70ef\u4e2d\u3002<\/p>\n

(c)\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u63a5\u89e6\u65f6\u4ee5\u53ca\u5728\u7d2b\u5916\u5230\u8fd1\u7ea2\u5916\u5149\uff08UV-NIR\uff09\u7167\u5c04\u65f6\u7684\u80fd\u7ea7\u548c\u7535\u5b50\u6216\u7a7a\u7a74\u8f6c\u79fb\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe<\/strong>3. <\/strong>\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u6742\u5316\u7ed3\u6784\u7684\u5149\u63a2\u6d4b\u5668\u6027\u80fd\u548c\u5df2\u53d1\u8868\u5de5\u4f5c\u7684\u6bd4\u8f83<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

(a) \u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u6742\u5316\u7ed3\u6784\u7684\u5149\u63a2\u6d4b\u5668\u7684\u54cd\u5e94\u5ea6\u968f\u6ce2\u957f\u7684\u53d8\u5316\u3002\u7ea2\u8272\u661f\u53f7\u4e3a\u672c\u5de5\u4f5c\u7684\u7ed3\u679c\u3002<\/p>\n

(b) \u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u6742\u5316\u7ed3\u6784\u7684\u5149\u63a2\u6d4b\u5668\u7684\u6bd4\u63a2\u6d4b\u7387\u968f\u6ce2\u957f\u7684\u53d8\u5316\u3002\u7ea2\u8272\u661f\u53f7\u4e3a\u672c\u5de5\u4f5c\u7684\u7ed3\u679c\u3002<\/p>\n

\u3010\u76f8\u5173\u5de5\u4f5c\u3011<\/strong><\/p>\n

\u524d\u671f\u7684\u7814\u7a76\u8868\u660e\uff0c\u5229\u7528\u672a\u63ba\u6742\u7684\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u5f62\u6210\u6742\u5316\u7ed3\u6784\u5e76\u5c06\u5176\u4e0e\u4f53\u7845\u5f62\u6210\u8096\u7279\u57fa\u7ed3\uff0c\u5c31\u80fd\u5236\u5907\u51fa\u7684\u9ad8\u901f\u7684\u5149\u7535\u63a2\u6d4b\u5668\uff08Adv. Mater. 28, 4912-4919 (2016). DOI: 10.1002\/adma.201506140\/full<\/a>\uff09\u3002\u8fdb\u4e00\u6b65\u7684\u7814\u7a76\u53d1\u73b0\uff0c\u628a\u63ba\u6742\u7845\u91cf\u5b50\u70b9\u7f6e\u4e8e\u77f3\u58a8\u70ef\u548c\u4f53\u7845\u4e4b\u95f4\u53ef\u4ee5\u5f62\u6210\u5177\u6709\u7ea7\u8054\u7ed3\u6784\u7684\u8096\u7279\u57fa\u5149\u7535\u63a2\u6d4b\u5668\uff0c\u5176\u9ad8\u6027\u80fd\u7684\u5149\u54cd\u5e94\u5728\u6ce2\u957f\u957f\u81f3\u7ea62 \u03bcm\u7684\u8fd1\u7ea2\u5916\u6ce2\u6bb5\u4e5f\u80fd\u89c2\u5bdf\u5230\uff0c\u5668\u4ef6\u7684\u6700\u5927\u54cd\u5e94\u5ea6\u53ef\u8fbe0.6 A\/W\uff0c\u54cd\u5e94\u65f6\u95f4\u4e3a10-6<\/sup> s\uff0c\u6bd4\u63a2\u6d4b\u7387\u53ef\u8fbe1011<\/sup> Jones\uff0c\u5728\u540c\u7c7b\u578b\u5668\u4ef6\u4e2d\u8fbe\u5230\u56fd\u9645\u5148\u8fdb\u6c34\u5e73\u3002\u8be5\u7814\u7a76\u6210\u679c\u201cGraphen\/silicon-quantum-dot\/silicon Schottky-PN cascade heterojuction for short-wavelength infrared photodetection\u201d\u6700\u8fd1\u88ab\u7535\u6c14\u548c\u7535\u5b50\u5de5\u7a0b\u5e08\u534f\u4f1a\uff08IEEE\uff09\u7684\u77e5\u540d\u56fd\u9645\u4f1a\u8baeInternational Electron Devices Meeting \uff08IEDM\uff092017\u6240\u6536\u5f55\uff0c\u675c\u601d\u8d85\u535a\u58eb\u3001\u502a\u6715\u4f0a\u535a\u58eb\u548c\u5218\u96ea\u6885\u4e3a\u6587\u7ae0\u7684\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u8be5\u9879\u76ee\u5236\u5907\u4e86\u4e00\u79cd\u57fa\u4e8e\u63ba\u6742\u7845\u91cf\u5b50\u70b9\u548c\u77f3\u58a8\u70ef\u6742\u5316\u7ed3\u6784\u7684\u6676\u4f53\u7ba1\u578b\u5149\u7535\u63a2\u6d4b\u5668\uff0c\u5229\u7528\u63ba\u6742\u5f15\u5165\u7684\u7845\u91cf\u5b50\u70b9\u5149\u5b66\u5438\u6536\u7279\u6027\u548c\u77f3\u58a8\u70ef\u7684\u9ad8\u8fc1\u79fb\u7387\u7279\u6027\u5b9e\u73b0\u4e86\u4ece\u7d2b\u5916\u5149\uff08375nm\uff09\u5230\u4e2d\u7ea2\u5916\u5149\uff084\u03bcm\uff09\u7684\u8d85\u5bbd\u5149\u8c31\u63a2\u6d4b\u3002\u8fd9\u4e00\u6210\u679c\u5c55\u793a\u4e86\u7845\u91cf\u5b50\u70b9\u5728\u5149\u7535\u5668\u4ef6\u4e2d\u7684\u5e94\u7528\u6709\u671b\u901a\u8fc7\u4e0e\u4e8c\u7ef4\u6750\u6599\u5982\u77f3\u58a8\u70ef\u5f62\u6210\u6742\u5316\u7ed3\u6784\u800c\u53d6\u5f97\u7a81\u7834\uff0c\u4e5f\u4e3a\u5176\u4ed6\u5177\u6709\u7b49\u79bb\u6fc0\u5143\u6548\u5e94\u7684\u91cf\u5b50\u70b9\u5728\u5149\u7535\u5668\u4ef6\u4e2d\u7684\u5e94\u7528\u63d0\u4f9b\u4e86\u501f\u9274\u3002<\/p>\n

\u6587\u732e\u8fde\u63a5<\/strong>\uff1aPlasmonic Silicon Quantum Dots Enabled High-Sensitivity Ultrabroadband Photodetection of Graphene-Based Hybrid Phototransistors <\/a>(ACS Nano, 2017, DOI: 10.1021\/acsnano.7b03569)<\/p>\n

\u672c\u6587\u7531\u6d59\u6c5f\u5927\u5b66\u502a\u6715\u4f0a\u535a\u58eb\u6295\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

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