{"id":108623,"date":"2017-10-28T14:00:18","date_gmt":"2017-10-28T06:00:18","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=108623"},"modified":"2017-10-26T12:32:28","modified_gmt":"2017-10-26T04:32:28","slug":"adv-mater-%ef%bc%9a%e5%8f%af%e6%89%a9%e5%b1%95%e7%9a%84%e5%89%8d%e5%90%91%e6%95%a3%e5%b0%84%e4%bd%93%e7%9a%84%e5%87%a0%e4%bd%95%e8%ae%be%e8%ae%a1%ef%bc%8c%e7%94%a8%e4%ba%8e%e6%9c%80%e6%9c%89%e6%95%88","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=108623","title":{"rendered":"Adv. Mater.\uff1a\u53ef\u6269\u5c55\u7684\u524d\u5411\u6563\u5c04\u4f53\u7684\u51e0\u4f55\u8bbe\u8ba1\uff0c\u7528\u4e8e\u6700\u6709\u6548\u7684\u592a\u9633\u80fd\u53d8\u538b\u5668"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u592a\u9633\u80fd\u662f\u5730\u7403\u4e0a\u6700\u4e30\u5bcc\u7684\u80fd\u6e90\uff0c\u4e5f\u662f\u6240\u6709\u78b3\u6c22\u5316\u5408\u7269\u5316\u77f3\u71c3\u6599\u7684\u6700\u7ec8\u6765\u6e90\uff0c\u800c\u8fd9\u4e9b\u5316\u77f3\u71c3\u6599\u76ee\u524d\u662f\u4eba\u7c7b\u7ecf\u6d4e\u7684\u4e3b\u8981\u80fd\u6e90\u3002\u56e0\u6b64\uff0c\u5f53\u4ee3\u592a\u9633\u80fd\u4e5f\u53ef\u7528\u4e8e\u751f\u4ea7\u5176\u4ed6\u53ef\u518d\u751f\u80fd\u6e90\u3002\u7814\u7a76\u4eba\u5458\u4e00\u76f4\u5728\u52aa\u529b\u5f00\u53d1\u5404\u79cd\u592a\u9633\u80fd\u6536\u96c6\u6750\u6599\u3001\u8bbe\u5907\u548c\u6982\u5ff5\uff0c\u5305\u62ec\u5149\u7535\u3001\u592a\u9633\u80fd\u96c6\u6210\u7684\u5efa\u7b51\u8bbe\u8ba1\uff0c\u4ee5\u53ca\u7528\u4e8e\u5316\u5b66\u548c\u751f\u7269\u71c3\u6599\u751f\u4ea7\u7684\u4eba\u5de5\u5149\u5408\u7ec6\u80de\u3002\u5149\u751f\u7269\u53cd\u5e94\u5668\uff0c\u6216\u8005\u662f\u5c01\u95ed\u7684\uff0c\u7528\u4e8e\u79cd\u690d\u5bcc\u542b\u8102\u8d28\u7684\u85fb\u7c7b\u7684\u5de5\u7a0b\u7cfb\u7edf\uff0c\u5229\u7528\u592a\u9633\u80fd\u901a\u8fc7\u5149\u5408\u4f5c\u7528\u521b\u9020\u751f\u7269\u71c3\u6599\uff0c\u4e0d\u9700\u8981\u989d\u5916\u7684\u8bd5\u5242\uff0c\u5982\u7cd6\u6216\u8102\u8d28\u3002\u5c3d\u7ba1\u8bb8\u591a\u7814\u7a76\u4eba\u5458\u5c1d\u8bd5\u5c06\u751f\u7269\u53cd\u5e94\u5668\u5de5\u7a0b\u5316,\u4f46\u662f\u8fd9\u79cd\u6280\u672f\u7684\u4e3b\u8981\u969c\u788d\u4e4b\u4e00,\u4fbf\u662f\u5728\u5b9e\u8df5\u4e2d\u76f4\u63a5\u5229\u7528\u5165\u5c04\u592a\u9633\u80fd\u901a\u91cf\u7684\u4f4e\u6548\u7387:\u85fb\u7c7b\u8868\u9762\u7684\u7cfb\u7edf\u5fc5\u987b\u6709\u5c0f\u5438\u6536\u6a2a\u622a\u9762\u548c\u5229\u7528\u975e\u5149\u5316\u5b66\u673a\u5236\u6765\u7184\u706d\u5149\u8fdb\u800c\u907f\u514d\u5149\u7834\u574f,\u800c\u7ec6\u80de\u7684\u751f\u957f\u7cfb\u7edf\u5149\u9650\u5236\u66f4\u6df1\u3002\u5728\u7ed9\u5b9a\u7684\u4f4d\u7f6e\uff0c\u6f5c\u5728\u7684\u592a\u9633\u80fd\u8d44\u6e90\u8d8a\u591a\uff0c\u8fd9\u4e9b\u7cfb\u7edf\u4e2d\u6709\u6548\u8d44\u6e90\u5229\u7528\u7684\u57fa\u672c\u969c\u788d\u5c31\u8d8a\u4e25\u91cd\u3002<\/p>\n

\u5982\u679c\u80fd\u5c06\u540c\u6837\u6709\u6548\u7684\u9633\u5149\u7167\u5c04\u5230\u5149\u751f\u7269\u53cd\u5e94\u5668\u7cfb\u7edf\u4e2d\u7684\u6240\u6709\u7535\u6c60\u4e2d\uff0c\u540c\u65f6\u5229\u7528\u73af\u5883\u4e2d\u6240\u6709\u7684\u592a\u9633\u8f90\u5c04\u6765\u8fdb\u884c\u5149\u5316\u5b66\uff0c\u90a3\u8be5\u600e\u4e48\u529e\u5462?\u8fd9\u6837\u7684\u7b56\u7565\u76f8\u5f53\u4e8e\u4e00\u4e2a\u592a\u9633\u80fd\u53d8\u538b\u5668\uff0c\u7c7b\u4f3c\u4e8e\u7535\u7f51\u914d\u7535\u7cfb\u7edf\u4e2d\u7684\u7535\u78c1\u53d8\u538b\u5668\u3002\u5728\u4e4b\u524d\u7684\u5c1d\u8bd5\u4e2d\uff0c\u901a\u8fc7\u201c\u5149\u7a00\u91ca\u201d\u6765\u5b9e\u73b0\u7c7b\u4f3c\u7684\u201c\u5b9a\u91cf\u201d\u65b9\u6cd5\uff0c\u7814\u7a76\u4eba\u5458\u8bbe\u8ba1\u4e86\u5f15\u5bfc\u5149\u7ebf\u6df1\u5165\u5230\u6587\u5316\u80cc\u666f\u7684\u6ce2\u5bfc\uff0c\u5e76\u4f7f\u7528\u5355\u8272\u5149\u6765\u51cf\u5c11\u5149\u6291\u5236\uff0c\u63d0\u9ad8\u85fb\u7684\u5149\u5408\u4f5c\u7528\u6548\u7387\u3002\u8fd9\u4e9b\u5c1d\u8bd5\u51cf\u5c11\u4e86\u5230\u8fbe\u6bcf\u4e2a\u7535\u6c60\u7684\u5149\u91cf\uff0c\u907f\u514d\u4e86\u5149\u635f\u5bb3\uff0c\u4f46\u662f\u603b\u7684\u6765\u8bf4\uff0c\u5ffd\u89c6\u4e86\u592a\u9633\u80fd\u4f5c\u4e3a\u4e00\u4e2a\u6574\u4f53\u7684\u6709\u6548\u5229\u7528\u3002\u53e6\u4e00\u79cd\u8f83\u65e9\u7684\u5173\u4e8e\u5149\u7a00\u91ca\u7684\u6750\u6599\u7b56\u7565\u6d89\u53ca\u5230\u4e3a\u5747\u5300\u7684\u8868\u9762\u6563\u5c04\u7684\u5411\u524d\u6563\u5c04\u548c\/\u6216\u975e\u5747\u5300\u7684\u5fae\u7ed3\u6784\u3002\u8fd9\u4e9b\u5c1d\u8bd5\u5305\u62ec\u7b49\u79bb\u5b50\u4f53\u7eb3\u7c73\u7c92\u5b50(NPs)\uff0c\u6838\u58f3\u7eb3\u7c73\u7c92\u5b50\uff0c\u4ee5\u53ca\u692d\u5706\u72b6\u7684\u4ecb\u7535\u7eb3\u7c73\u7c92\u5b50\u3002\u7136\u800c\uff0c\u8fd9\u4e9b\u65b9\u6cd5\u9700\u8981\u81ea\u4e0a\u800c\u4e0b\u7684\u5236\u5907\uff0c\u5728\u7eb3\u7c73\u5c3a\u5ea6\u4e0a\u7cbe\u786e\u63a7\u5236\u7c92\u5b50\u7684\u5c3a\u5bf8\u548c\u5f62\u72b6\uff0c\u5e76\u4f7f\u7528\u9ad8\u6298\u5c04\u7387\u6750\u6599\u3002\u4f46\u662f\uff0c\u56e0\u4e3a\u4ef7\u683c\u6602\u8d35\uff0c\u4e0d\u80fd\u7528\u4e8e\u751f\u4ea7\u548c\u5b9e\u73b0\u751f\u7269\u71c3\u6599\u53cd\u5e94\u5806\u3002\u6b64\u5916\uff0c\u4eba\u4eec\u5bf9\u5176\u6ce2\u957f\u7684\u9009\u62e9\u6027\u3001\u5149\u5b66\u635f\u8017\u6216\u6df1\u5ea6\u4fe1\u9053\u7684\u4eae\u5ea6\u7684\u4e00\u81f4\u6027\u77e5\u4e4b\u751a\u5c11\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5bbe\u5915\u6cd5\u5c3c\u4e9a\u5927\u5b66\u7684\u6768\u6f8d\u6559\u6388<\/strong>\uff0cAlison M. Sweeney\u6559\u6388<\/strong>\u7b49\u4eba\u5728Advanced Materials<\/strong>\u4e0a\u53d1\u6587\uff0c\u9898\u4e3a\uff1a\u201cGeometric Design of Scalable Forward Scatterers for Optimally Efficient Solar Transformers\u201d<\/strong>\u3002\u7814\u7a76\u4eba\u5458\u4ecb\u7ecd\u4e86\u7535\u6c60\u7cfb\u7edf\u4e2d\u7a81\u51fa\u7684\u524d\u5411\u6563\u5c04\u884c\u4e3a\u7684\u8bbe\u8ba1\u3001\u5408\u6210\u548c\u7279\u5f81\u63cf\u8ff0\uff0c\u63d0\u51fa\u4e86\u4e00\u79cd\u5229\u7528\u592a\u9633\u80fd\u6700\u5927\u9650\u5ea6\u5730\u5229\u7528\u7535\u6c60\u7684\u6700\u5927\u91cf\u5b50\u6548\u7387\u7684\u51e0\u4f55\u89e3\u51b3\u65b9\u6848\u3002\u5408\u6210\u7684\u7535\u6c60\u662f\u7531\u5d4c\u5165\u5728\u51dd\u80f6\u4e2d\u7684\u5fae\u7403\u4e2d\u7684\u4e8c\u6c27\u5316\u7845\u7eb3\u7c73\u9897\u7c92\u7ec4\u6210\uff0c\u5b83\u4eec\u90fd\u662f\u4f4e\u6298\u5c04\u7387\u6750\u6599\u548c\u5ec9\u4ef7\u7684\u6750\u6599\u3002\u5b83\u4eec\u663e\u793a\u4e86\u6ce2\u957f\u7684\u9009\u62e9\u6027\uff0c\u51e0\u4e4e\u6ca1\u6709\u635f\u5931(\u53cd\u5411\u6563\u5c04\u5f3a\u5ea6\u51cf\u5c0f\u5230\u5c0f\u4e8e0.01%\u7684\u6b63\u5411\u6563\u5c04\u5f3a\u5ea6)\uff0c\u5e76\u7f29\u5c0f\u4e86\u7c7b\u4f3c\u4e8e\u5927\u8d1d\u58f3\u5316\u77f3\u7684\u7a84\u7684\u524d\u6563\u5c04\u9525\u3002\u6b64\u5916\uff0c\u901a\u8fc7\u6bd4\u8f83\u5b9e\u9a8c\u548c\u7406\u8bba\u8ba1\u7b97\uff0c\u53ef\u4ee5\u786e\u5b9a\u6563\u5c04\u5c3a\u5bf8\u7684\u4e0d\u5747\u5300\u6027\u662f\u8bbe\u8ba1\u7684\u4e00\u4e2a\u201c\u7279\u6027\u800c\u975e\u7f3a\u9677\u201d\uff0c\u4ece\u800c\u53ef\u4ee5\u5728\u4e00\u4e2a\u5fae\u7c73\u5c3a\u5ea6\u7684\u6a21\u578b\u4e2d\u5b9e\u73b0\u5bf9\u592a\u9633\u901a\u91cf\u7684\u6709\u6548\u7684\u518d\u5206\u914d\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe1. \u5de8\u86e4\u7ec6\u80de\u7684\u6563\u5c04\u884c\u4e3a\uff0c\u5e76\u8bbe\u8ba1\u4e86\u5408\u6210\u7684\u8679\u5f69\u819c\u7684\u6982\u8ff0<\/strong><\/p>\n

\"\"<\/p>\n

a) \u5de8\u86e4\u56fe\u7247\uff1b \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 b) \u5de8\u86e4\u7ec6\u80de\u5fae\u89c2\u56fe\uff1b<\/p>\n

c) \u5de8\u86e4\u7ec6\u80de\u5c55\u73b0\u4e3a\u7eb3\u7c73\u7247\u7684TEM\u56fe\uff1b<\/p>\n

d) \u4e00\u4e2a\u5355\u4e00\u7684\u7ec6\u80de\u7684\u6563\u5c04\u884c\u4e3a\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

e) \u5728\u51dd\u80f6\u4e2d\u5d4c\u5165\u4e8c\u6c27\u5316\u7845\u5408\u6210\u9897\u7c92\u7684\u5408\u6210\u7684\u8679\u5f69\u80f6\u7247\uff1b<\/p>\n

f) \u5408\u6210\u7684\u8679\u5f69\u819c\u7684\u6563\u5c04\u884c\u4e3a\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\u56fe2. \u7ec6\u80de\u5408\u6210<\/strong><\/p>\n

\"\"<\/p>\n

a) \u5236\u4f5c\u5408\u6210\u7684\u7ec6\u80de\u8584\u819c\u7684\u8fc7\u7a0b\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

b,c)\u6765\u81ea250nm\u5927\u5c0f\u7684\u7845\u7eb3\u7c73\u7c92\u5b50\u7684\u590d\u5408\u7c92\u5b50\u7684SEM\u56fe\uff1b<\/p>\n

\u56fe3. \u4e0e\u5de8\u86e4\u7ec6\u80de\u7cfb\u7edf\u76f8\u5f53\u7684\u5408\u6210\u7684\u7535\u6c60\u7cfb\u7edf\u7684\u51e0\u4f55\u8bbe\u8ba1\u7684\u8ba1\u7b97\u548c\u5efa\u6a21<\/strong><\/p>\n

\"\"<\/p>\n

a) \u963b\u5c3c\u66f2\u7ebf\uff1b<\/p>\n

b) \u4e0d\u5bf9\u79f0\u56e0\u5b50 (g<\/em>) \u5bf9\u4e8e\u5355\u4e2a\u7684\u7b80\u5355\u5fae\u7403\u4f53\uff0c\u5b83\u662f\u4e00\u4e2a\u5927\u5c0f\u53c2\u6570(\u03c7)\u7684\u51fd\u6570\uff0c\u5b83\u6709\u4e0d\u540c\u7684\u6298\u5c04\u7387\u5bf9n\u7403\u4f53\/n\u4ecb\u8d28\uff1b<\/p>\n

c) \u4e00\u79cd\u5408\u6210\u7684200nm\u7eb3\u7c73\u7c92\u5b50\u7684\u76f8\u4f4d\u51fd\u6570\u7684DDA\u8ba1\u7b97\uff1b<\/p>\n

d) \u56fe(c)\u5728\u03b8 = 0\u00b0\u201410\u00b0\u8303\u56f4\u7684\u7ebf\u5f62\u56fe\uff0c\u7167\u5c04\u6ce2\u957f\u4e3a\u03bb = 509 nm\uff1b<\/p>\n

\u56fe4. \u7531\u5408\u6210\u7684\u8679\u819c\u8584\u819c\u548c\u7845\u7eb3\u7c73\u7c92\u5b50\u80f6\u7247\u8fdb\u884c\u7684\u524d\u5411\u6563\u5c04\u548c\u540e\u5411\u6563\u5c04\u7684\u89d2\u5ea6\u5206\u5e03\uff0c\u5e76\u5c06\u5b83\u4eec\u4e0eDDA-\u8ba1\u7b97\u7ed3\u679c\u8fdb\u884c\u6bd4\u8f83<\/strong><\/p>\n

\"\"
\n a) \u5b9e\u9a8c\u7279\u5f81\u7684\u76f8\u4f4d\u51fd\u6570(T)\u56fa\u5b9a\u6ce2\u957f\u4e3a509nm\uff0c\u5176\u89d2\u5ea6\u4e3a\u03b8=0\u00b0\u201350\u00b0\u548c\u03b8=110\u00b0\u2013165\u00b0\u3002\u5bf9\u4e8e\u534a\u5f84\u56fe\uff0c\u901a\u8fc7\u6d4b\u91cf\u6570\u636e\u5916\u63a8(\u4e0d\u53ef\u6d4b\u91cf\u7684\u6570\u636e\u70b9\u53d6\u800c\u4ee3\u4e4b\u7684\u662f\u76f4\u7ebf)\u56e0\u4e3a\u5f3a\u5ea6\u76f8\u6bd4\uff0c\u8fd9\u4e2a\u8303\u56f4\u662f\u5f88\u4f4e\u5f3a\u5ea6\u7684\u5cf0\u503c\u3002\u5149\u5f3a\u5ea6\u7684\u89d2\u8303\u56f4\u88ab\u9650\u5236\u5728\u5b9e\u9a8c\u6d4b\u91cf\u51e0\u4f55(50\u00b0-110\u00b0\u548c165\u00b0-180\u00b0)\u8303\u56f4\u6765\u88ab\u5916\u63a8\u5f97\u5230\uff1b<\/p>\n

b) \u88ab\u79ef\u51fd\u6570\u5728\u7a84\u7684\u524d\u89d2\u900f\u5c04\u5149\u5f3a\u5ea6(\u03b8 = 0\u00b0\u201310\u00b0)\uff1b<\/p>\n

\u56fe5. \u6d4b\u91cf\u5185\u90e8\u8584\u819c\u8f90\u5c04\u6d4b\u91cf\u6570\u636e<\/strong><\/p>\n

\"\"<\/p>\n

a) \u5782\u76f4\u63a2\u6d4b\u5668\u4f4d\u7f6e\u5bf9\u7c92\u5b50\u6563\u5c04\u4e8b\u4ef6\u7684\u5f71\u54cd\u7a0b\u5ea6\u7684\u56fe\u89e3\u8bf4\u660e\uff0c\u6709\u52a9\u4e8e\u63a2\u6d4b\u7531\u63a2\u6d4b\u5668\u63a2\u6d4b\u5230\u7684\u6807\u91cf\u8f90\u7167\u5ea6\uff1b.<\/p>\n

\u6807\u91cf\u8f90\u5c04\u5f3a\u5ea6\u662f\u819c\u8868\u9762\u6807\u91cf\u8f90\u7167\u5ea6\u7684\u4e00\u4e2a\u767e\u5206\u6bd4\u3002b) \u5bf9\u4e8e\u542b\u7845\u7684\u4e8c\u6c27\u5316\u7845\u7eb3\u7c73\u7c92\u5b50\uff1b c) \u5305\u542b\u590d\u5408\u7c92\u5b50\u7684\u8584\u819c\uff1b<\/p>\n

\u3010\u603b\u7ed3\u3011<\/strong><\/p>\n

\u7814\u7a76\u4eba\u5458\u63d0\u51fa\u4e86\u4e00\u79cd\u57fa\u4e8e\u7406\u8bba\u7684\u5de5\u7a0b\u65b9\u6cd5\u548c\u5149\u5b66\u5143\u4ef6\u7684\u5b9e\u9a8c\u5b9e\u73b0\uff0c\u53ef\u4ee5\u6709\u6548\u5730\u63a7\u5236\u548c\u5206\u914d\u901a\u91cf\u8f93\u5165\u88c5\u7f6e\uff0c\u4ee5\u5b9e\u73b0\u592a\u9633\u80fd\u5149\u8f6c\u6362\u3002\u91cd\u8981\u7684\u662f,\u7814\u7a76\u4eba\u5458\u7684\u8ba1\u7b97\u548c\u5b9e\u9a8c\u8868\u660e\uff0c\u5411\u524d\u6563\u5c04\u7684\u5f62\u72b6\u548c\u5927\u5c0f\u8303\u56f4\u5411\u524d\u6563\u5c04\u5173\u952e\u884c\u4e3a\u4ee5\u53ca\u7c92\u5ea6\u5747\u5300\u6027\u5e76\u4e0d\u91cd\u8981,\u8fd9\u4f7f\u5f97\u7814\u7a76\u4eba\u5458\u53ef\u4ee5\u4f7f\u7528\u4e00\u4e2a\u7b80\u5355\u7684\u6da1\u6d41\u65b9\u6cd5\u5927\u89c4\u6a21\u751f\u4ea7\u63a5\u8fd1\u7cbe\u786e\u6a21\u62df\u7684\u5de8\u578b\u86e4\u7ec6\u80de\u7684\u5149\u5b66\u529f\u80fd\u590d\u5408\u5fae\u7c92\u5b50\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Geometric Design of Scalable Forward Scatterers for Optimally Efficient Solar Transformers<\/a> (Advanced Materials, 2017, DOI: 10.1002\/adma.201702922)<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u524d\u7ebfZ. Chen\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

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