{"id":116149,"date":"2017-12-12T06:30:28","date_gmt":"2017-12-11T22:30:28","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=116149"},"modified":"2017-12-09T16:25:08","modified_gmt":"2017-12-09T08:25:08","slug":"nat-commun%ef%bc%9a%e9%ab%98%e5%ba%a6%e5%8f%af%e8%b0%83%e7%9a%84%e7%83%ad%e5%8a%9b%e5%ad%a6%e4%b8%8d%e7%a8%b3%e5%ae%9a%e7%9a%84%e9%87%91%e5%b1%9e-%e6%b0%a2%e4%bd%93%e7%b3%bb","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=116149","title":{"rendered":"Nat. commun\uff1a\u9ad8\u5ea6\u53ef\u8c03\u7684\u70ed\u529b\u5b66\u4e0d\u7a33\u5b9a\u7684\u91d1\u5c5e-\u6c22\u4f53\u7cfb"},"content":{"rendered":"<p><strong>\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n<p>\u8fd1\u5e74\u6765\u6e29\u5ba4\u6548\u5e94\u65e5\u76ca\u4e25\u91cd\uff0c\u5168\u7403\u53d8\u6696\u7684\u95ee\u9898\u5df2\u6210\u4e3a\u73b0\u4eca\u73af\u4fdd\u6700\u5927\u7684\u56f0\u6270\uff0c\u800c\u5316\u77f3\u71c3\u6599\u71c3\u70e7\u4ea7\u751f\u5927\u91cf\u7684CO2\u662f\u5168\u7403\u53d8\u6696\u4e3b\u8981\u7684\u539f\u56e0\uff0c\u56e0\u6b64\u65b0\u80fd\u6e90\u7684\u7814\u53d1\u548c\u63a8\u5e7f\u5f02\u5e38\u91cd\u8981\u3002\u6c22\u80fd\u4f5c\u4e3a\u4e00\u79cd\u73af\u4fdd\u7684\u518d\u751f\u80fd\u6e90\uff0c\u53cd\u5e94\u540e\u53ea\u751f\u6210\u6c34\uff0c\u540c\u65f6\u5176\u5206\u5e03\u5e7f\u6cdb\u3001\u65e0\u6c61\u67d3\u548c\u53ef\u50a8\u5b58\u7b49\u4e00\u7cfb\u5217\u4f18\u70b9\u53d7\u5230\u65e5\u76ca\u589e\u957f\u7684\u9752\u7750\uff0c\u5177\u6709\u5e7f\u6cdb\u7684\u5e94\u7528\u524d\u666f\u3002\u7a7a\u6c14\u4e2d\u6c22\u6c14\u7684\u542b\u91cf\u57284 %\uff5e74.5 % \u7684\u8303\u56f4\u5185\u65f6\uff0c\u6c14\u4f53\u9047\u660e\u706b\u6781\u6613\u53d1\u751f\u7206\u70b8\uff0c\u8fd9\u4e5f\u6210\u4e3a\u6c22\u6c14\u63a8\u5e7f\u7684\u5236\u7ea6\u6761\u4ef6\u3002\u56e0\u6b64\uff0c\u4e3a\u4e86\u4fdd\u8bc1\u4eba\u7684\u751f\u547d\u3001\u8d22\u4ea7\u548c\u8bbe\u5907\u7684\u5b89\u5168\uff0c\u4fc3\u8fdb\u6c22\u80fd\u5927\u89c4\u6a21\u63a8\u5e7f\u5e94\u7528\uff0c\u6709\u5fc5\u8981\u5f00\u5c55\u4f20\u611f\u5668\u7684\u76f8\u5173\u7814\u7a76\u3002\u00a0<\/p>\n<p><strong>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n<p>\u8fd1\u671f\uff0c<strong>\u8377\u5170\u4e4c\u5f97\u52d2\u652f\u5927\u5b66Peter Ngene\u7814\u7a76\u5458\u7b49\u4eba\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7814\u5236\u4e86\u4e00\u79cd\u80fd\u901a\u8fc7\u989c\u8272\u6539\u53d8\u6765\u68c0\u6d4b\u6c22\u6c14\u6d53\u5ea6\u7684\u4f20\u611f\u5668\u3002\u8be5\u7814\u7a76\u901a\u8fc7\u5411\u9487\u4e2d\u52a0\u5165\u5c11\u91cf\u7684\u9506\u5bfc\u81f4\u9487\u6676\u683c\u7684\u6536\u7f29\uff0c\u4f7f\u5f97YH<sub>2<\/sub>\u2194YH<sub>3<\/sub>\u7684\u5e73\u8861\u6c22\u6c14\u6d53\u5ea6\u53ef\u4ee5\u5728\u4e94\u4e2a\u6570\u91cf\u7ea7\u7684\u8303\u56f4\u5185\u88ab\u6709\u6548\u5730\u88ab\u8c03\u63a7\uff0c\u800c\u6210\u529f\u5236\u5907\u4e86\u4e00\u4e2a\u53ef\u4ee5\u4ea7\u751f\u8089\u773c\u53ef\u8fa9\u7684\u989c\u8272\u53d8\u5316\u6765\u68c0\u6d4b\u6c22\u6c14\u7684\u6c22\u6c14\u4f20\u611f\u5668\uff0c\u5b83\u80fd\u6709\u6548\u5730\u68c0\u6d4b\u56db\u4e2a\u6570\u91cf\u7ea7\u7684\u6c22\u6c14\u6d53\u5ea6\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<strong>Metal-hydrogen systems with an exceptionally large and tunable thermodynamic destabilization<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u4e86N<strong>ature Communications<\/strong>\u4e0a\u3002<\/p>\n<p><strong>\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n<p><strong>\u56fe1. Zr\u5bf9Y\u6c22\u5316\u538b\u529b\u7684\u5f71\u54cd\u00a0<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-116235\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/1-28.jpg\" alt=\"\" width=\"740\" height=\"583\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/1-28.jpg 740w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/1-28-300x236.jpg 300w\" sizes=\"(max-width: 740px) 100vw, 740px\" \/><\/p>\n<p>\uff08a\uff09\u572870\u00d75 cm\u7684\u77f3\u82f1\u886c\u5e95\u4e0a\u5236\u5907\u6210\u6954\u5f62\u51e0\u4f55\u768435~83 nm\u7684Y-Zr\u68af\u5ea6\u8584\u819c\uff0c\u518d\u8986\u67095 nm\u7684Ti\u548c30 nm\u7684Pd\u9876\u5c42\u7684\u793a\u610f\u56fe\uff1b<\/p>\n<p>\uff08b\uff09\u5728\u7b2c\u4e00\u4e2a\u6c22\u6c14\u5438\u6536\u5faa\u73af\uff0825\u00b0C\u65f60-40 mbar 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at.\uff05\uff1b<\/p>\n<p>\uff08c\uff09\u572825\u2103\u4ece\u4e8c\u6c22\u5316\u7269\u72b6\u6001\u5f00\u59cb\u7684\u7b2c\u516d\u6c22\u5438\u6536\u5faa\u73af\u671f\u95f4\u7684PTI\uff1b<\/p>\n<p>\uff08d\uff09\u5bf9\u4e8e\u9009\u5b9a\u7684Zr\u6d53\u5ea6\uff08Y<sub>96.6<\/sub>Zr<sub>3.4<\/sub>-Y<sub>85.5<\/sub>Zr<sub>14.5<\/sub>\uff09220\u2103\u4e0b\u7684\u89e3\u5438\u7b49\u6e29\u7ebf\uff08PTIs\uff09\u3002\u6bcf\u4e2a\u7b49\u6e29\u7ebf\u4ee3\u8868Zr\u4ece3.5\uff05\u5f00\u59cb\u6bcf\u6b21\u589e\u52a0\u542b\u91cf0.38 at.%\u3002<\/p>\n<p><strong>\u56fe2. \u4e0eZr\u63ba\u6742\u76f8\u5173\u7684YH<sub>x<\/sub>\u7684\u6676\u683c\u884c\u4e3a\u00a0<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-116185\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/2-21.jpg\" alt=\"\" width=\"700\" height=\"458\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/2-21.jpg 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/2-21-300x196.jpg 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/p>\n<p>\uff08a\uff09Y-Zr\u8584\u819c\u7684XRD\u56fe\uff0c\u5b83\u663e\u793a\u4e86\u5236\u5907\u6001hcp-Y\uff08002\uff09\u3001\u5b8c\u5168\u6c22\u5316\u6001hcp-YH<sub>3<\/sub>\uff08002\uff09\u548c\u8131\u6c22\u6001YH<sub>2<\/sub>\uff08111\uff09\u4e2d\u7684\u884d\u5c04\u5cf0\u3002\u5cf0\u7684\u4f4d\u7f6e\u4e0eZr\u7684\u6d53\u5ea6\u5bc6\u5207\u76f8\u5173\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\u5373\u4f7f\u6301\u7eed\u901a24h\u768410 bar H<sub>2<\/sub>\uff0cY<sub>86<\/sub>Zr<sub>14<\/sub>\u6837\u54c1\u4e5f\u4e0d\u80fd\u5b8c\u5168\u6c22\u5316\u4e3aYH<sub>3<\/sub>\uff1b<\/p>\n<p>\uff08b\uff09\u4f5c\u4e3aZr\u6d53\u5ea6\u51fd\u6570\u7684YH<sub>x<\/sub>\u7684d-\u95f4\u8ddd\u7684\u6539\u53d8\uff0c\u5206\u522b\u5bf9\u5e94\u5b8c\u5168\u5236\u5907\u6001\u3001\u5b8c\u5168\u6c22\u5316\u6001\uff08YH<sub>3<\/sub>\uff09\u548c\u8131\u6c22\u6001\uff08YH<sub>2<\/sub>\uff09\uff1b<\/p>\n<p>\uff08c\uff09YH<sub>2<\/sub>\u6469\u5c14\u4f53\u79ef\u7684\u76f8\u5bf9\u53d8\u5316\u503c\uff08\u0394V\/ V\uff09\u548cYH<sub>2<\/sub>\u2194YH<sub>3<\/sub>\u76f8\u53d8\u65f6\u7684\u5e73\u53f0\u538b\u529b\u4e4b\u95f4\u7684\u5173\u7cfb\uff0c\u4e0e\u672a\u538b\u7f29\u6001\uff08P<sub>f<\/sub>\uff09\u548c\u538b\u7f29\u6001\uff08P<sub>C<\/sub>\uff09YH<sub>2<\/sub>\u76f8\u6bd4\u8f83\u3002<\/p>\n<p><strong>\u56fe3. \u7528XAS\u8fdb\u884c\u5c40\u90e8\u7ed3\u6784\u5206\u6790\u00a0<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-116372 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/41467_2017_2043_Fig3_HTML.jpg\" alt=\"\" width=\"600\" height=\"1450\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/41467_2017_2043_Fig3_HTML.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/41467_2017_2043_Fig3_HTML-124x300.jpg 124w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/41467_2017_2043_Fig3_HTML-424x1024.jpg 424w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\uff08a\uff09\u6c89\u79ef\u6001\uff0c\uff08c\uff09\u5b8c\u5168\u6c22\u5316\u6001\u548c\uff08e\uff09\u8131\u6c22\u6001\u8584\u819c\u7684XANES\u5149\u8c31\uff1b<\/p>\n<p>\uff08b\uff09\u6c89\u79ef\u6001\uff0c\uff08d\uff09\u5b8c\u5168\u6c22\u5316\u6001\u548c\uff08f\uff09\u8131\u6c22\u6001Zr\u548cY-Zr\u8584\u819c\u7684EXAFS\u5149\u8c31\u76f8\u4f4d\u672a\u6821\u6b63\u7684FT\u3002<\/p>\n<p>\n <strong>\u56fe4. \u5728\u6c22\u5316\u7684Zr\u548cYZr\u8584\u819c\u4e0a\u8fdb\u884cXANES\u6a21\u62df\u00a0<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-116187\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/4-19.jpg\" alt=\"\" width=\"700\" height=\"555\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/4-19.jpg 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/4-19-300x238.jpg 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/p>\n<p>\uff08a\uff09ZrH<sub>x<\/sub>\u819c\uff1b<\/p>\n<p>\uff08b\uff09\uff08c\uff09YZrH<sub>x<\/sub>\u8584\u819c\u3002<\/p>\n<p><strong>\u56fe5. \u572870\u00d75mm\u7684Y<sub>97<\/sub>Zr<sub>3<\/sub>-Y<sub>90<\/sub>Zr<sub>10<\/sub>\u68af\u5ea6\u8584\u819c\u4e0aYH<sub>3<\/sub>\u5f62\u6210\u7684\u8089\u773c\u53ef\u89c1\u7684\u989c\u8272\u53d8\u5316<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-116188\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/5-17.jpg\" alt=\"\" width=\"700\" height=\"488\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/5-17.jpg 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/12\/5-17-300x209.jpg 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/p>\n<p>\u00a0\u56fe\u7247\u4ee3\u8868\u5728\u4e0d\u540cH<sub>2<\/sub>\u538b\u529b\u4e0b\u7684\u8584\u819c\u6c22\u5316\u7684\u4e0d\u540c\u9636\u6bb5\u3002\u989c\u8272\u524d\u6cbf\u7684\u4f4d\u7f6e\uff08\u7bad\u5934\u6240\u793a\uff09\u53d6\u51b3\u4e8e\u6c22\u6c14\u538b\u529b\u548cZr\u6d53\u5ea6\u3002\u4e3a\u589e\u5f3a\u8be5\u819c\u7684\u5149\u5b66\u5bf9\u6bd4\u5ea6\uff0c\u8be5\u6837\u54c1\u6e85\u5c04\u7684Pd\u5c42\u7684\u539a\u5ea6\u4e3a50nm\u3002<\/p>\n<p><strong>\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n<p>\u8be5\u7814\u7a76\u53d1\u73b0\u4e86\u4e00\u4e2a\u65b0\u578b\u7684\u91d1\u5c5e-\u6c22\u4f53\u7cfb\uff0c\u8be5\u4f53\u7cfb\u7531\u7eb3\u7c73\u5c3a\u5ea6\u7684\u7269\u7406\u7ea6\u675f\u800c\u5177\u6709\u975e\u5e38\u5927\u4e14\u53ef\u8c03\u8282\u70ed\u529b\u5b66\u4e0d\u7a33\u5b9a\u6027\u3002\u5728\u7ed3\u6784\u76f8\u5e72\u7684\uff08Y-Zr\uff09H<sub>x<\/sub>\u8584\u819c\u4e2d\uff0cZr\u7eb3\u7c73\u56e2\u7c07\u5728\u9487\u4e0a\u5f15\u8d77\u5f39\u6027\u5e94\u53d8\uff0c\u5bfc\u81f4\u4e09\u6c22\u5316\u7269\uff08YH<sub>3<\/sub>\uff09\u76f8\u53d8\u5f97\u4e0d\u7a33\u5b9a\u3002\u901a\u8fc7\u4ece0\u523013 at.\uff05\u6539\u53d8Zr\u6d53\u5ea6\uff0c\u5728\u5ba4\u6e29\u4e0b\u53ef\u4ee5\u7cbe\u786e\u5730\u4ece10<sup>-1<\/sup>\u523010<sup>4<\/sup> mbar\uff08\u4e94\u4e2a\u6570\u91cf\u7ea7\uff09\u8fde\u7eed\u8c03\u6574YH<sub><sup>3<\/sup><\/sub>\u5f62\u6210\u7684\u5e73\u8861\u538b\u529b\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u8be5\u7cfb\u7edf\u5728\u5faa\u73af\u65f6\u76f8\u5f53\u7a33\u5b9a\uff0c\u751a\u81f3\u8868\u73b0\u51fa\u53ef\u8c03\u8282\u7684\u5e73\u8861\u8131\u6c22\u538b\u529b\uff0c\u800c\u8fd9\u6b63\u662f\u70ed\u529b\u5b66\u4e0d\u7a33\u5b9a\u6027\u7684\u8868\u73b0\u3002\u8be5\u7814\u7a76\u8868\u660e\uff0c\u5373\u4f7f\u6dfb\u52a0\u4e0d\u56fa\u6eb6\u7684\u63ba\u6742\u5242\uff0c\u4e5f\u4f1a\u5bf9\u91d1\u5c5e\u5438\u9644\u6c22\u7684\u6027\u80fd\u4ea7\u751f\u663e\u8457\u7684\u5f71\u54cd\u3002\u5f53\u7136\uff0c\u5728\u5757\u4f53\u6750\u6599\u4e2d\u662f\u5426\u53ef\u4ee5\u83b7\u5f97\u7c7b\u4f3c\u7684\u7ed3\u8bba\u8fd8\u6709\u5f85\u7814\u7a76\u3002\u7136\u800c\uff0cAsano\u7b49\u4eba\u7684\u5b9e\u9a8c\u8868\u660e\uff0c\u5728MgTH<sub>x<\/sub>\u8584\u819c\u4e2d\u89c2\u5bdf\u5230\u7684\u7c7b\u4f3c\u76f8\u5e72\u6027\u5728\u7403\u78e8\u7684\u5927\u5757\u6837\u54c1\u4e2d\u53ef\u4ee5\u518d\u73b0\u3002\u8be5\u7814\u7a76\u4e3a\u5408\u7406\u8c03\u6574\u91d1\u5c5e\u6c22\u7cfb\u7edf\u7684\u6027\u80fd\u4ee5\u8fbe\u5230\u5e94\u7528\u6240\u9700\u5f00\u8f9f\u4e86\u4e00\u6761\u65b0\u9014\u5f84\u3002\u8be5\u7814\u7a76\u7684\u53d1\u73b0\u4e5f\u9002\u7528\u4e8e\u6676\u683c\u8fde\u8d2f\u7684\u56fa\u4f53\u57fa\u4f53\uff0c\u56e0\u6709\u95f4\u9699\u539f\u5b50\u4f7f\u5f97\u4f53\u79ef\u663e\u8457\u6539\u53d8\u800c\u5bfc\u81f4\u7684\u5404\u79cd\u53cd\u5e94\u3002<\/p>\n<p><strong>\u6587\u732e\u94fe\u63a5\uff1a<\/strong><a href=\"https:\/\/www.nature.com\/articles\/s41467-017-02043-9\" target=\"_blank\" rel=\"noopener\">Metal-hydrogen systems with an exceptionally large and tunable thermodynamic destabilization<\/a>\u00a0 (Nature Communications\uff0c 2017\uff0cDOI: 10.1038\/s41467-017-02043-9)<\/p>\n<p>\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u91d1\u5c5e\u6750\u6599\u5b66\u672f\u7ec4Nancy\u6574\u7406\u7f16\u8bd1\uff0c<a href=\"http:\/\/www.cailiaoniu.com\/25127.html\" target=\"_blank\" rel=\"noopener\">\u70b9\u6211\u52a0\u5165\u6750\u6599\u4eba\u7f16\u8f91\u90e8<\/a>\u3002<\/p>\n<p><strong>\u6750\u6599\u6d4b\u8bd5\uff0c\u6570\u636e\u5206\u6790\uff0c\u4e0a<a href=\"http:\/\/www.ceshigu.com\/\" target=\"_blank\" rel=\"noopener\">\u6d4b\u8bd5\u8c37<\/a>\uff01<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u3010\u5f15\u8a00\u3011 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