{"id":137147,"date":"2018-05-06T06:30:21","date_gmt":"2018-05-05T22:30:21","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=137147"},"modified":"2018-05-06T05:13:23","modified_gmt":"2018-05-05T21:13:23","slug":"energ-environ-sci-%ef%bc%9a%e7%83%ad%e6%95%8f%e5%bc%80%e5%85%b3%e5%9e%8b%e5%b9%b3%e9%9d%a2%e5%be%ae%e5%9e%8b%e8%b6%85%e7%ba%a7%e7%94%b5%e5%ae%b9%e5%99%a8%ef%bc%9a%e4%b8%80%e7%a7%8d%e5%af%8c%e6%9c%89","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=137147","title":{"rendered":"Energ. Environ. Sci.\uff1a\u70ed\u654f\u5f00\u5173\u578b\u5e73\u9762\u5fae\u578b\u8d85\u7ea7\u7535\u5bb9\u5668\uff1a\u4e00\u79cd\u5bcc\u6709\u6f5c\u529b\u7684\u7535\u5b50\u5668\u4ef6\u4fdd\u62a4\u65b9\u6848"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u8fd1\u5e74\u6765\uff0c\u73b0\u4ee3\u7535\u5b50\u5b66\u7684\u7814\u7a76\u91cd\u70b9\u96c6\u4e2d\u5728\u5b9e\u73b0\u7535\u5b50\u8bbe\u5907\u7684\u5c0f\u578b\u5316\u3001\u8f7b\u91cf\u5316\u3001\u9ad8\u6027\u80fd\u548c\u5b89\u5168\u6027\u7b49\u65b9\u9762\u3002\u9ad8\u6027\u80fd\u7535\u5b50\u8bbe\u5907\u603b\u662f\u9700\u8981\u5feb\u901f\u80fd\u91cf\u6d88\u8017\u548c\/\u6216\u9ad8\u529f\u7387\u80fd\u91cf\u8f93\u9001\u3002\u8fd9\u5c06\u5bfc\u81f4\u654f\u611f\u7535\u5b50\u5143\u4ef6\u7684\u81ea\u53d1\u70ed\u95ee\u9898\uff0c\u56e0\u6b64\u53ef\u80fd\u5bf9\u5176\u9020\u6210\u70ed\u635f\u4f24\u5e76\u5e26\u6765\u5b89\u5168\u9690\u60a3\uff0c\u540c\u65f6\u663e\u8457\u964d\u4f4e\u7535\u5b50\u5668\u4ef6\u7684\u5bff\u547d\u3002\u4f8b\u5982\uff0c\u624b\u673a\u6216\u7535\u8111\u7684\u5904\u7406\u5668\u548c\u7535\u8def\u677f\u7684\u64cd\u4f5c\u6e29\u5ea6\u5e94\u4e25\u683c\u63a7\u5236\u572880 \u2103\u4ee5\u4e0b\u3002\u4eba\u4eec\u8fc7\u53bb\u5e38\u5e38\u5229\u7528\u767e\u53f6\u7a97\u3001\u6563\u70ed\u7247\u548c\u51b7\u5374\u98ce\u6247\u7b49\u70ed\u63a7\u529f\u80fd\u6a21\u5757\u6765\u9632\u6b62\u7535\u5b50\u5668\u4ef6\u7684\u70ed\u5931\u63a7\u3002\u7136\u800c\uff0c\u7531\u4e8e\u7a7a\u95f4\u9650\u5236\u3001\u5de5\u827a\u590d\u6742\u548c\u6210\u672c\u6548\u7387\u7b49\u539f\u56e0\uff0c\u4ee5\u4e0a\u6a21\u5757\u5e76\u4e0d\u9002\u7528\u4e8e\u82af\u7247\u5f0f\u7535\u5b50\u5668\u4ef6\u3002\u5fae\u578b\u8d85\u7ea7\u7535\u5bb9\u5668(MSCs)\u662f\u4e00\u79cd\u53ef\u7528\u4e8e\u82af\u7247\u5f0f\u7535\u5b50\u5668\u4ef6\u7684\u5fae\u578b\u4f9b\u80fd\u8bbe\u5907\uff0c\u5176\u5177\u6709\u8d85\u9ad8\u529f\u7387\u5bc6\u5ea6\u3001\u5feb\u901f\u500d\u7387\u6027\u80fd\u548c\u8d85\u957f\u5faa\u73af\u5bff\u547d\u7b49\u4f18\u70b9\u3002\u7136\u800c\uff0c\u9ad8\u6027\u80fd\u7684\u5fae\u578b\u8d85\u7ea7\u7535\u5bb9\u5668\u901a\u5e38\u5bf9\u7269\u7406\u6216\u5316\u5b66\u523a\u6fc0\u4e0d\u654f\u611f\u3002\u56e0\u6b64\uff0c\u4e3a\u4e86\u5b9e\u73b0\u5fae\u578b\u7535\u5b50\u8bbe\u5907\u7684\u667a\u80fd\u70ed\u4fdd\u62a4\uff0c\u8bbe\u8ba1\u4e00\u79cd\u5177\u6709\u667a\u80fd\u70ed\u4fdd\u62a4\u529f\u80fd\u7684MSCs\u6709\u7740\u91cd\u8981\u7684\u5b9e\u9645\u610f\u4e49\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5fb7\u56fd\u5fb7\u7d2f\u65af\u987f\u5de5\u4e1a\u5927\u5b66<\/strong>\u7684\u51af\u65b0\u4eae\u4e0e\u5e84\u6653\u4e1c(\u5171\u540c\u901a\u8baf\u4f5c\u8005)<\/strong>\u5728\u5fae\u578b\u8d85\u7ea7\u7535\u5bb9\u5668\u9886\u57df\u53d6\u5f97\u65b0\u7684\u7814\u7a76\u8fdb\u5c55\uff0c\u5728\u56fd\u9645\u9876\u7ea7\u5b66\u672f\u671f\u520aEnergy & Environmental Science\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201dThermoswitchable on-chip microsupercapacitors One potential self-protection solution for electronic devices\u201d\u7684\u7814\u7a76\u8bba\u6587\u3002\u8be5\u5de5\u4f5c\u63d0\u51fa\u4e86\u4e00\u79cd\u53ef\u7528\u4e8e\u82af\u7247\u5f0f\u7535\u5b50\u5668\u4ef6\uff0c\u5177\u6709\u9ad8\u6e29\u4fdd\u62a4\u529f\u80fd\u7684\u70ed\u654f\u5f00\u5173\u5fae\u578b\u8d85\u7ea7\u7535\u5bb9\u5668(TS-MSC)\u3002\u5fae\u578b\u8d85\u7ea7\u7535\u5bb9\u5668\u4ee5\u4e00\u79cd\u6eb6\u89e3\u4e86\u9502\u76d0\u7684\u805a\u5408\u7269\u6eb6\u80f6\u4e3a\u7535\u89e3\u8d28\uff0c\u8be5\u7535\u89e3\u8d28\u5177\u5907\u72ec\u7279\u7684\u70ed\u529b\u5b66\u884c\u4e3a\u3002\u5f97\u76ca\u4e8e\u7535\u89e3\u8d28\u79bb\u5b50\u7535\u5bfc\u7387\u7684\u53ef\u9006\u53d8\u5316\uff0cTS-MSC\u5177\u5907\u8f83\u5bbd\u7684\u5de5\u4f5c\u6e29\u5ea6\u533a\u95f4\u548c\u4f18\u5f02\u7684\u52a0\u70ed\/\u51b7\u5374\u5faa\u73af\u7a33\u5b9a\u6027\u3002\u5f53\u6e29\u5ea6\u4e0a\u5347\u523080 \u2103\u65f6\u53ef\u4ee5\u5b9e\u73b0\u5b8c\u5168\u7684\u7535\u5bb9\u65ad\u5f00\uff0c\u5728\u51b7\u5374\u81f3\u5ba4\u6e29\u65f6\u53c8\u5b8c\u5168\u6062\u590d\u3002\u4e00\u822c\u60c5\u51b5\u4e0b\u8ba1\u7b97\u673aCPU\u7684\u4e34\u754c\u5de5\u4f5c\u6e29\u5ea6\u4e3a80 \u2103\uff0c\u56e0\u6b64\u82af\u7247\u5f0fTS-MSC\u9635\u5217\u4e3a\u8ba1\u7b97\u673aCPU\u7684\u70ed\u4fdd\u62a4\u63d0\u4f9b\u4e86\u65b0\u7684\u9014\u5f84\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\uff1a\u70ed\u654f\u5f00\u5173\u5fae\u578b\u8d85\u7ea7\u7535\u5bb9\u5668\u7684\u5236\u5907\u53ca\u673a\u7406<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u5728\u7845\u57fa\u677f\u548cPI\u8584\u819c\u4e0a\u5236\u5907TS-MSC\u7684\u8fc7\u7a0b\u793a\u610f\u56fe\uff0c\u5236\u5907\u8fc7\u7a0b\u5305\u62ec\u901a\u8fc7\u5149\u523b\u6cd5\u5236\u4f5c\u53c9\u6307\u72b6Au\u96c6\u6d41\u4f53\u3001\u7535\u6c89\u79ef\u5236\u5907\u6d3b\u6027\u6750\u6599(PEDOT)\u5c42\uff0c\u4ee5\u53ca\u6ef4\u6ce8\u6eb6\u89e3LiCl\u7684PNIPAAm\/MC\u6eb6\u6db2\u4f5c\u4e3a\u70ed\u654f\u7535\u89e3\u8d28\uff1b<\/p>\n

(b) \u52a0\u70ed\u51b7\u5374\u65f6\u70ed\u54cd\u5e94\u6027\u7535\u89e3\u8d28\u7684\u53ef\u9006\u6eb6\u80f6-\u51dd\u80f6\u8f6c\u53d8\u4ee5\u53ca\u53c9\u6307\u72b6\u7535\u6781\u4e4b\u95f4\u7684\u79bb\u5b50\u4f20\u8f93\u793a\u610f\u56fe\u3002\u00a0<\/strong><\/p>\n

\u56fe\u4e8c\uff1a<\/strong>\u7535\u89e3\u8d28\u7684\u70ed\u54cd\u5e94\u884c\u4e3a\u4e0e\u7535\u6781\u7684\u5fae\u89c2\u5f62\u8c8c<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0c\u52a0\u70ed\/\u51b7\u5374\u65f6PNIPAAm\/MC\u4f53\u7cfb\u7684\u53ef\u9006\u6eb6\u80f6-\u51dd\u80f6\u8f6c\u53d8\uff1b<\/p>\n

(b) \u5f53\u5165\u5c04\u5149\u6ce2\u957f\u4e3a600 nm\u65f6\uff0cPNIPAAm\/MC\u6eb6\u6db2\u7684\u900f\u5149\u7387-\u6e29\u5ea6\u53d8\u5316\u66f2\u7ebf\uff1b<\/p>\n

(c) \u57fa\u4e8ePEDOT\u7535\u6781\u6750\u6599\u7684MSC\u5149\u5b66\u663e\u5fae\u56fe\u50cf\uff0c\u6697\u533a\u5bf9\u5e94\u7535\u5316\u5b66\u805a\u5408PEDOT\uff0c\u4eae\u533a\u5bf9\u5e94\u7845\u57fa\u5e95\uff1b<\/p>\n

(d) \u7845\u57fa\u677f\u652f\u6491Au\u7535\u6781\u4e0ePEDOT\u819c\u7684\u9876\u89c6\u56feSEM\u56fe\u50cf\uff1b<\/p>\n

(e) \u7845\u57fa\u677f\u652f\u6491Au\u7535\u6781\u4e0ePEDOT\u819c\u7684\u6a2a\u622a\u9762SEM\u56fe\u50cf\uff1b<\/p>\n

(f) \u57fa\u4e8ePEDOT\u7535\u6781\u6750\u6599\u7684\u7684MSCs\u7684\u622a\u9762\u9ad8\u5ea6\u5206\u6790\u3002<\/p>\n

\u56fe\u4e09\uff1a<\/strong>\u5728<\/strong>30-80 <\/strong>\u2103\u6e29\u5ea6\u533a\u95f4\u5185<\/strong>\uff0c<\/strong>TS-MSC<\/strong>\u4e0e<\/strong>C-MSC<\/strong>\u7684\u7535\u5316\u5b66\u884c\u4e3a\u5bf9\u6bd4<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0cTS-MSCs\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

(b) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0cTS-MSCs\u7684GCD\u66f2\u7ebf\uff1b<\/p>\n

(c) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0c\u70ed\u54cd\u5e94PNIPAAm\/MC\/LiCl\u7535\u89e3\u8d28\u7684\u79bb\u5b50\u7535\u5bfc\u7387\u53d8\u5316\u66f2\u7ebf\uff1b<\/p>\n

(d)-(e) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0cTS-MSC\u7684\u5948\u594e\u65af\u7279\u56fe\uff1b<\/p>\n

(f) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0cC-MSC\u7684\u5948\u594e\u65af\u7279\u56fe\u3002<\/p>\n

\u56fe\u56db\uff1a<\/strong>TS-MSCs<\/strong>\u7684\u70ed\u54cd\u5e94\u884c\u4e3a<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0cTS-MSCs\u7684GCD\u66f2\u7ebf\uff1b<\/p>\n

(b) \u5f53\u7535\u6d41\u5bc6\u5ea6\u4e3a20 \u03bcA\u00b7cm-2<\/sup>\u65f6\uff0c30-80 \u2103\u4e0bTS-MSCs\u7684\u9762\u7535\u5bb9\u4e0e\u5faa\u73af\u6b21\u6570\u7684\u5173\u7cfb\uff1b<\/p>\n

(c) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0cTS-MSCs\u7684\u963b\u6297\u76f8\u4f4d\u89d2\u4e0e\u9891\u7387\u7684\u5173\u7cfb\uff1b<\/p>\n

(d) 50\u6b21\u52a0\u70ed-\u51b7\u5374\u5faa\u73af\u4e2d\uff0cTS-MSCs\u7684\u53ef\u9006\u9762\u7535\u5bb9\u884c\u4e3a\uff1b<\/p>\n

(e) \u4e32\u8054\/\u5e76\u8054\u4e24\u4e2a\u6216\u56db\u4e2aTS-MSCs\u5355\u5143\u7684\u7535\u8def\u56fe\uff1b<\/p>\n

(f) \u5f53\u7535\u6d41\u5bc6\u5ea6\u4e3a60 \u03bcA\u2219cm-2<\/sup>\u65f6\uff0c\u4e32\u8054\u56db\u4e2aTS-MSCs\u5355\u5143\u7684\u5668\u4ef6\u7684GCD\u66f2\u7ebf\uff1b<\/p>\n

(g) \u5ba4\u6e29\u6761\u4ef6\u4e0b\uff0c\u5f53\u626b\u63cf\u901f\u7387\u4e3a200 mV\u2219s-1<\/sup>\u65f6\uff0c\u4e32\u8054\/\u5e76\u8054\u4e24\u4e2a\u6216\u56db\u4e2aTS-MSCs\u5355\u5143\u7684\u5668\u4ef6\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

(h) \u5ba4\u6e29\u6761\u4ef6\u4e0b\uff0c\u5f53\u7535\u6d41\u5bc6\u5ea6\u4e3a40 \u03bcA\u00b7cm-2<\/sup>\u65f6\uff0c\u4e32\u8054\/\u5e76\u8054\u4e24\u4e2a\u6216\u56db\u4e2aTS-MSCs\u5355\u5143\u7684GCD\u66f2\u7ebf\u3002<\/p>\n

\u56fe\u4e94\uff1a\u8fde\u63a5\u5728\u8ba1\u7b97\u673aCPU\u9762\u677f\u4e0a\u7684TS-MSC\u9635\u5217\u7684\u70ed\u54cd\u5e94\u884c\u4e3a<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u4e32\u8054\u56db\u4e2aTS-MSCs\u5355\u5143\u7684\u6570\u7801\u7167\u7247\u548c\u7535\u8def\u56fe\uff0c\u767d\u8272\u865a\u7ebf\u5708\u51fa\u90e8\u5206\u8868\u793aTS-MSC\u5355\u5143\uff0c\u5176\u4ed6\u5355\u5143\u4e3aC-MSC\u5355\u5143\uff0c\u7ea2\u8272\u548c\u7eff\u8272\u7b26\u53f7\u5206\u522b\u4ee3\u8868\u5668\u4ef6\u5904\u4e8e\u5f00\u542f\u548c\u5173\u95ed\u72b6\u6001\uff1b<\/p>\n

(b) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0c\u5f53\u626b\u63cf\u901f\u7387\u4e3a500 mV\u00b7s-1<\/sup>\u65f6\uff0c\u4e32\u8054\u56db\u4e2aTS-MSCs\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

(c) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0c\u5f53\u7535\u6d41\u5bc6\u5ea6\u4e3a500 mV\u00b7s-1<\/sup>\u65f6\uff0c\u4e32\u8054\u56db\u4e2aTS-MSCs\u7684GCD\u66f2\u7ebf\uff1b<\/p>\n

(d) \u5e76\u8054\u56db\u4e2aTS-MSCs\u7684\u6570\u7801\u7167\u7247\u548c\u7535\u8def\u56fe\uff1b<\/p>\n

(e) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0c\u5f53\u626b\u63cf\u901f\u7387\u4e3a500 mV\u00b7s-1<\/sup>\u65f6\uff0c\u5e76\u8054\u56db\u4e2aTS-MSCs\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

(f) \u572830-80 \u2103\u6e29\u5ea6\u533a\u95f4\u5185\uff0c\u5f53\u626b\u63cf\u901f\u7387\u4e3a500 mV\u00b7s-1<\/sup>\u65f6\uff0c\u5e76\u8054\u56db\u4e2aTS-MSCs\u7684GCD\u66f2\u7ebf\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u57fa\u4e8eLiCl\/PNIPAAm\/MC\u7535\u89e3\u8d28\u5728\u52a0\u70ed-\u51b7\u5374\u8fc7\u7a0b\u4e2d\u7684\u6eb6\u80f6-\u51dd\u80f6\u8f6c\u53d8\u884c\u4e3a\uff0c\u8be5\u5de5\u4f5c\u8bbe\u8ba1\u4e86\u4e00\u79cd\u5177\u6709\u53ef\u9006\u70ed\u54cd\u5e94\u4fdd\u62a4\u529f\u80fd\u7684\u70ed\u654f\u5f00\u5173\u5fae\u578b\u8d85\u7ea7\u7535\u5bb9\u5668(TS-MSCs)\u3002\u5728\u9ad8\u6e29\u6761\u4ef6\u4e0b\uff0c\u7535\u89e3\u8d28\u7684\u70ed\u8bf1\u5bfc\u51dd\u80f6\u5316\u6291\u5236\u4e86\u9502\u79bb\u5b50\u7684\u8fc1\u79fb\uff0c\u800c\u5728\u51b7\u5374\u72b6\u6001\u4e0b\u9502\u79bb\u5b50\u7684\u81ea\u7531\u8fc1\u79fb\u53c8\u5f97\u4ee5\u6062\u590d\u3002\u7531\u4e8e\u79bb\u5b50\u7535\u5bfc\u7387\u7684\u53ef\u9006\u53d8\u5316\uff0cTS-MSCs\u5177\u6709\u8f83\u5bbd\u7684\u5de5\u4f5c\u6e29\u5ea6\u8303\u56f4(30-80 \u2103)\u548c\u4f18\u5f02\u7684\u51b7\u70ed\u5faa\u73af\u7a33\u5b9a\u6027\u3002\u901a\u8fc7\u5bf9TS-MSCs\u9635\u5217\u7684\u96c6\u6210\uff0c\u4f7f\u5f97\u5668\u4ef6\u5177\u5907\u4e86\u9ad8\u6548\u7684\u70ed\u54cd\u5e94\u5f00\u5173\u80fd\u529b\uff0c\u4ece\u800c\u53ef\u4ee5\u5b9e\u73b0\u5bf9\u6e29\u5ea6\u654f\u611f\u5143\u4ef6\u7684\u5b9e\u65f6\u4fdd\u62a4\u3002\u8be5\u5de5\u4f5c\u4e3a\u70ed\u54cd\u5e94\u5fae\u578b\u529f\u80fd\u5668\u4ef6\u7684\u8bbe\u8ba1\u63d0\u4f9b\u4e86\u65b0\u7684\u601d\u8def\uff0c\u4e5f\u4e3a\u89e3\u51b3\u4fbf\u643a\u5f0f\u82af\u7247\u5f0f\u7535\u5b50\u8bbe\u5907\u7684\u5b89\u5168\u95ee\u9898\u63d0\u4f9b\u4e86\u4e00\u79cd\u53ef\u884c\u7684\u89e3\u51b3\u65b9\u6848\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aThermoswitchable on-chip microsupercapacitors: One potential self-protection solution for electronic devices\u00a0<\/a>(Energ. Environ. Sci.\uff0c2018\uff0cDOI: 10.1039\/C8EE00365C)<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u674e\u5609\u6b23\u7f16\u8bd1\uff0c\u5f20\u6770\u5ba1\u6838\uff0c\u70b9\u6211\u52a0\u5165\u6750\u6599\u4eba\u7f16\u8f91\u90e8<\/a>\u3002<\/p>\n

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 <\/p>\n","protected":false},"excerpt":{"rendered":"

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