{"id":147861,"date":"2018-07-28T14:00:29","date_gmt":"2018-07-28T06:00:29","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=147861"},"modified":"2018-07-26T22:45:17","modified_gmt":"2018-07-26T14:45:17","slug":"nano-energy-%e5%9f%ba%e4%ba%8e%e6%b0%a7%e7%a9%ba%e4%bd%8d%e5%92%8c%e6%99%b6%e9%9d%a2%e5%bc%82%e8%b4%a8%e7%bb%93%e7%9a%84%e5%a4%9a%e7%94%b5%e5%9c%ba%e8%b0%83%e6%8e%a7%e7%ad%96%e7%95%a5%e5%bc%ba","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=147861","title":{"rendered":"Nano Energy : \u57fa\u4e8e\u6c27\u7a7a\u4f4d\u548c\u6676\u9762\u5f02\u8d28\u7ed3\u7684\u591a\u7535\u573a\u8c03\u63a7\u7b56\u7565\u5f3a\u5316\u5149\u50ac\u5316\u53cd\u5e94\u7535\u8377\u5206\u79bb"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u76ee\u524d\uff0c\u5149\u751f\u8f7d\u6d41\u5b50\u5feb\u901f\u590d\u5408\u5bfc\u81f4\u7684\u8fc7\u4f4e\u50ac\u5316\u6548\u7387\u4e25\u91cd\u5236\u7ea6\u7740\u5149\u50ac\u5316\u6280\u672f\u7684\u5927\u89c4\u6a21\u5de5\u4e1a\u5e94\u7528\u3002\u6784\u5efa\u5185\u90e8\u7535\u573a\u662f\u6539\u5584\u534a\u5bfc\u4f53\u5149\u751f\u8f7d\u6d41\u5b50\u5206\u79bb\u6027\u80fd\u7684\u91cd\u8981\u9014\u5f84\uff0c\u800c\u6676\u9762\u8c03\u63a7\u7531\u4e8e\u5b58\u5728\u5149\u751f\u7535\u5b50\u548c\u7a7a\u7a74\u7684\u81ea\u53d1\u7a7a\u95f4\u5206\u79bb\uff0c\u53ef\u4ee5\u4e3a\u7535\u8377\u5206\u79bb\u63d0\u4f9b\u6f5c\u5728\u7684\u9a71\u52a8\u529b\u3002\u540c\u65f6\uff0c\u5149\u50ac\u5316\u5242\u7684\u754c\u9762\u7535\u5b50\u7ed3\u6784\u5bf9\u4e8e\u5f02\u8d28\u7ed3\u754c\u9762\u7535\u8377\u5206\u79bb\u8fc7\u7a0b\u5177\u6709\u91cd\u8981\u4f5c\u7528\uff0c\u6c27\u7a7a\u4f4d\u4f5c\u4e3a\u6c27\u5316\u7269\u534a\u5bfc\u4f53\u6700\u4e3a\u5e38\u89c1\u7684\u5e76\u663e\u8457\u5f71\u54cd\u8868\u9762\u5438\u9644\u6216\u53cd\u5e94\u81ea\u7531\u57fa\u7684\u5f62\u6210\u6240\u6d89\u53ca\u7684\u8fd9\u4e9b\u754c\u9762\u56e0\u7d20\u4e2d\u6700\u91cd\u8981\u7684\u662f\u6c27\u7a7a\u4f4d\u7ed3\u6784\u7f3a\u9677\uff0c\u5bf9\u50ac\u5316\u5242\u7684\u8868\u9762\u5438\u9644\u7279\u6027\u3001\u53cd\u5e94\u6d3b\u6027\u81ea\u7531\u57fa\u7684\u751f\u6210\u4ee5\u53ca\u754c\u9762\u7535\u8377\u8f6c\u79fb\u8def\u5f84\u7b49\u5177\u6709\u91cd\u8981\u5f71\u54cd\u3002\u7136\u800c\u5bf9\u4e8e\u4e0d\u540c\u66b4\u9732\u6676\u9762\uff0c\u6c27\u7a7a\u4f4d\u4e0e\u5f02\u8d28\u7ed3\u7535\u8377\u5206\u79bb\u95f4\u7684\u5173\u7cfb\u4ecd\u7136\u662f\u4e00\u4e2a\u60ac\u800c\u672a\u51b3\u7684\u95ee\u9898\u3002\u56e0\u6b64\uff0c\u901a\u8fc7\u6676\u9762\u548c\u6c27\u7a7a\u4f4d\u8c03\u63a7\u7b56\u7565\u76f8\u7ed3\u5408\uff0c\u5bf9\u4e8e\u5b9e\u73b0\u5149(\u7535)\u50ac\u5316\u53cd\u5e94\u7684\u7535\u8377\u9ad8\u6548\u5206\u79bb\u5c24\u4e3a\u5173\u952e\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6e05\u534e\u5927\u5b66\u5b89\u6653\u5f3a\u526f\u7814\u7a76\u5458\u3001\u5317\u4eac\u822a\u5929\u822a\u7a7a\u5927\u5b66\u5218\u5229\u6c11\u6559\u6388\u3001\u82f1\u56fd\u4f26\u6566\u5927\u5b66\u5b66\u9662\u5510\u519b\u65fa\u6559\u6388\u7b49(\u5171\u540c\u901a\u8baf\u4f5c\u8005)<\/strong>\u4ee5ZnO\/BiVO4<\/sub>\u5206\u7ea7\u7eb3\u7c73\u7ed3\u6784\u4e3a\u4f8b\u6765\u8bc1\u660e\u591a\u7535\u573a\u8f85\u52a9\u7535\u8377\u5206\u79bb\u7684\u65b0\u6982\u5ff5\uff0c\u5e76\u5728Nano Energy<\/strong>\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cMulti-Electric Field Modulation for Photocatalytic Oxygen Evolution:Enhanced Charge Separation by Coupling Oxygen Vacancies with FacetedHeterostructures<\/strong>\u201d\u7684\u7814\u7a76\u8bba\u6587\u3002\u4f5c\u8005\u901a\u8fc7\u5b9e\u9a8c\u89c2\u5bdf\u548c\u7406\u8bba\u8ba1\u7b97\u8bc1\u5b9e\u4e86\u6676\u9762\u5de5\u7a0b\u548c\u7f3a\u9677\u8c03\u63a7\u5bf9\u4fc3\u8fdb\u5149\u50ac\u5316\u4f5c\u7528\u7684\u8d21\u732e\u3002\u590d\u5408\u6750\u6599\u96c6\u6210\u4e86\u5177\u6709\u5185\u5efa\u7535\u573a\u7684\u6676\u9762\u66b4\u9732BiVO4<\/sub>\u548c\u5404\u5411\u5f02\u6027ZnO\u7eb3\u7c73\u68d2\uff0c\u4ee5\u53ca\u5728\u754c\u9762\u5904\u53ef\u80fd\u7684Z\u578b\u7535\u8377\u4f20\u9012\u65b9\u5f0f\uff0c\u53ef\u89c1\u5149\u4e0b\u5149\u89e3\u6c34\u4ea7\u6c27\u901f\u7387\u8fbe\u52301.36 mmol\u00b7h-1<\/sup>\u00b7g-1<\/sup>\uff0c\u5e76\u4e14450nm\u5904\u8868\u89c2\u91cf\u5b50\u4ea7\u7387\u8f83BiVO4<\/sub>\u589e\u5f3a\u4e86\u4e00\u4e2a\u6570\u91cf\u7ea7\u3002\u8fd9\u9879\u5de5\u4f5c\u4e0d\u4ec5\u4e3a\u6676\u9762\u50ac\u5316\u5242\u7684\u754c\u9762\u7f3a\u9677\u8c03\u63a7\u63d0\u4f9b\u4e86\u57fa\u672c\u89c1\u89e3\uff0c\u800c\u4e14\u8fd8\u63d0\u4f9b\u4e86\u4e00\u79cd\u8bbe\u8ba1\u5177\u6709\u7f3a\u9677\u53ef\u63a7\u7684\u6676\u9762\u5f02\u8d28\u7ed3\u7b56\u7565\u4ee5\u663e\u8457\u589e\u5f3a\u7535\u8377\u5206\u79bb\u6548\u7387\u3002<\/p>\n

\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u56fe1 \u00a0ZnO\u548cBiVO4<\/sub>\u4e0d\u540c\u6676\u9762\u590d\u5408\u7684\u539f\u5b50\u7ed3\u6784\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

a) ZnO\u8d1f\u8f7d\u5728BiVO4<\/sub>{110}\u6676\u9762\u539f\u5b50\u7ed3\u6784\u793a\u610f\u56fe\uff0c\u5176\u4e2d\u9ec4\u8272\u5706\u5708\u4ee3\u8868\u6c27\u7a7a\u4f4d\u4f4d\u70b9(\u4e0b\u540c)\uff1b<\/p>\n

b)ZnO\u8d1f\u8f7d\u5728BiVO4<\/sub>{010}\u6676\u9762\u539f\u5b50\u7ed3\u6784\u793a\u610f\u56fe\u539f\u5b50\u7ed3\u6784\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe2 \u00a0\u5bf9\u5149\u751f\u7535\u5b50\u548c\u7a7a\u7a74\u7684\u81ea\u53d1\u7a7a\u95f4\u5206\u79bb\u8bc1\u5b9e<\/strong><\/p>\n

\"\"<\/p>\n

a)\u5149\u6c89\u79efAg\u5728BiVO4<\/sub>\u8868\u9762\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

b) \u5149\u6c89\u79efCo3<\/sub>O4<\/sub>\u5728BiVO4<\/sub>\u8868\u9762\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

c) \u5149\u6c89\u79efAg\u5728ZnO\u7eb3\u7c73\u68d2\u8868\u9762\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

d) \u5149\u6c89\u79efCo3<\/sub>O4<\/sub>\u5728ZnO\u7eb3\u7c73\u68d2\u8868\u9762\u7684SEM\u56fe\u50cf\u3002<\/p>\n

\u56fe3 \u00a0ZnO\u7eb3\u7c73\u68d2\u9635\u5217\u8d1f\u8f7d\u5728BiVO4<\/sub>\u8868\u9762\u7684\u5236\u5907\u8fc7\u7a0b\u548c\u5f62\u8c8c<\/strong><\/p>\n

\"\"<\/p>\n

a) ZnO\u7eb3\u7c73\u68d2\u8d1f\u8f7d\u5728BiVO4<\/sub>\u8868\u9762\u5236\u5907\u8fc7\u7a0b\u793a\u610f\u56fe\uff1b<\/p>\n

b-e) \u5bf9\u5e94a\u56fe\u4e2d\u7ed3\u6784i-iv\u7684SEM\u56fe\u50cf\u3002<\/p>\n

\u56fe4 \u00a0ZnO\/BiVO4<\/sub>\u5f02\u8d28\u7ed3\u7684\u80fd\u5e26\u7ed3\u6784\u548c\u5bf9\u7f3a\u9677\u8c03\u63a7<\/strong><\/p>\n

\"\"<\/p>\n

a) BiVO4<\/sub>\u548cZnO\u7684Mott-Schottky\u66f2\u7ebf\uff1b<\/p>\n

b) BiVO4<\/sub>\u548cZnO\u7684\u7d2b\u5916\u5149\u7535\u5b50\u8c31\uff0c\u5185\u63d2\u56fe\u4e3a\u5176\u80fd\u5e26\u7ed3\u6784\uff1b<\/p>\n

c) BiVO4<\/sub>\u548cZnO\/BiVO4<\/sub>\u4e2dXPS V 2p\u5149\u8c31\u7684\u53d8\u5316\uff1b<\/p>\n

d)BiVO4<\/sub>\u3001ZnO\/BiVO4<\/sub>\u548cVo<\/sub>-ZnO\/BiVO4<\/sub>ESR\u8c31\u4e2d\u7f3a\u9677\u7684\u53d8\u5316\u8fc7\u7a0b\u3002<\/p>\n

\u56fe5 \u00a0Vo<\/sub>-ZnO\/BiVO4<\/sub>\u7684\u7406\u8bba\u8ba1\u7b97<\/strong><\/p>\n

\"\"<\/p>\n

a-f)\u6709\u6c27\u7a7a\u4f4d\u7684ZnO\/BiVO4\u5f02\u8d28\u7ed3\u6001\u5bc6\u5ea6\u8ba1\u7b97\u548c\u7f3a\u9677\u80fd\u6001\u7684\u5206\u5e03\u3002<\/p>\n

\u56fe6 \u00a0\u5149\u50ac\u5316\u6d3b\u6027\u6d4b\u8bd5<\/strong><\/p>\n

\"\"<\/p>\n

a) \u5728\u53ef\u89c1\u5149(\u03bb>420 nm)\u7167\u5c04\u4e0b BiVO4<\/sub>\u548c\u5176\u590d\u5408\u7ed3\u6784\u7684\u5149\u89e3\u6c34\u4ea7\u6c27\u6d3b\u6027\u6d4b\u8bd5\uff1b<\/p>\n

b) BiVO4<\/sub>\u548cVo-ZnO\/BiVO4<\/sub>\u4e0d\u540c\u6ce2\u957f\u7684AQY\uff1b<\/p>\n

c)\u53cc\u7535\u573a\u8f85\u52a9ZnO\/BiVO4<\/sub>\u5f02\u8d28\u7ed3\u7535\u8377\u5206\u79bb\u7684\u673a\u7406\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe7 \u00a0\u6676\u9762\u4f9d\u8d56\u7684\u591a\u7535\u573a\u6548\u5e94\u8bc1\u5b9e<\/strong><\/p>\n

\"\"<\/p>\n

a) ZnO\u7eb3\u7c73\u68d2\u8d1f\u8f7d\u5728BiVO4<\/sub>\u7eb3\u7c73\u7247\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

b) BiVO4<\/sub>\u7eb3\u7c73\u7247\u548c\u5176\u590d\u5408\u7ed3\u6784\u5728\u5168\u5149\u8c31\u548c\u53ef\u89c1\u5149\u7167\u5c04\u4e0b\u7684\u5149\u89e3\u6c34\u4ea7\u6c27\u6d3b\u6027\u6d4b\u8bd5\uff1b<\/p>\n

c) ZnO\u7eb3\u7c73\u68d2\u8d1f\u8f7d\u5728\u5546\u4e1a\u5316BiVO4<\/sub>(C-ZnO\/BiVO4<\/sub>)\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

d) \u5546\u4e1a\u5316BiVO4<\/sub>\u548c\u5176\u590d\u5408\u7ed3\u6784\u5728\u53ef\u89c1\u5149\u7167\u5c04\u4e0b\u7684\u5149\u89e3\u6c34\u4ea7\u6c27\u6d3b\u6027\u6d4b\u8bd5\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u6784\u7b51\u4e86ZnO\/BiVO4<\/sub>\u5206\u7ea7\u7eb3\u7c73\u7ed3\u6784\u4ee5\u8bc1\u660e\u591a\u7535\u573a\u8c03\u63a7\u7684\u7b56\u7565\u80fd\u591f\u5b9e\u73b0\u7535\u8377\u7684\u9ad8\u6548\u5206\u79bb\u3002\u5b9e\u9a8c\u89c2\u5bdf\u548c\u7406\u8bba\u8ba1\u7b97\u5145\u5206\u8868\u660e\uff0c\u5f02\u8d28\u754c\u9762\u7f3a\u9677\u7684\u5f62\u6210\u548c\u7535\u8377\u4f20\u8f93\u8def\u5f84\u5747\u5177\u6709\u6676\u9762\u4f9d\u8d56\u6027\uff0c\u901a\u8fc7\u6676\u9762\u5de5\u7a0b\u4e0e\u754c\u9762\u7f3a\u9677\u8c03\u63a7\u76f8\u7ed3\u5408\uff0c\u50ac\u5316\u5242\u5728\u6709\u673a\u6c61\u67d3\u7269\u964d\u89e3\u548c\u6c34\u5206\u89e3\u53cd\u5e94\u4e2d\u5448\u73b0\u51fa\u9ad8\u6d3b\u6027\uff0c\u4f8b\u5982\u5149\u89e3\u6c34\u4ea7\u6c27\u901f\u7387\u53ef\u8fbe\u523068 \u03bcmol\u00b7h-1<\/sup>\uff0c450 nm\u5904AQY\u76f8\u6bd4\u4e8e\u6676\u9762BiVO4<\/sub>\u5149\u50ac\u5316\u5242\u63d0\u9ad8\u4e86\u4e00\u4e2a\u6570\u91cf\u7ea7\u4ee5\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aMulti-Electric Field Modulation for Photocatalytic Oxygen Evolution: Enhanced Charge Separation by Coupling Oxygen Vacancies with Faceted Heterostructures<\/a> <\/strong>(Nano Energy<\/strong>,2018, DOI: 10.1016\/j.nanoen.2018.07.018)<\/p>\n

\u3010\u8bfe\u9898\u7ec4\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u534a\u5bfc\u4f53\u5f02\u8d28\u7ed3\u6784\u662f\u63d0\u9ad8\u5149\u50ac\u5316\u5242\u50ac\u5316\u6d3b\u6027\u7684\u6709\u6548\u9014\u5f84\uff0c\u7136\u800c\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u754c\u9762\u884c\u4e3a\u53d7\u5230\u7ec4\u6210\u534a\u5bfc\u4f53\u80fd\u5e26\u7ed3\u6784\u3001\u754c\u9762\u80fd\u7ea7\u5339\u914d\u3001\u754c\u9762\u7f3a\u9677\u7b49\u590d\u6742\u56e0\u7d20\u7684\u5f71\u54cd\uff0c\u7279\u522b\u662f\u5982\u4f55\u901a\u8fc7\u754c\u9762\u7f3a\u9677\u8c03\u63a7\u5b9e\u73b0\u7535\u5b50\u548c\u7a7a\u7a74\u7684\u9ad8\u6548\u5206\u79bb\u4ecd\u662f\u672c\u9886\u57df\u7814\u7a76\u7684\u96be\u70b9\u95ee\u9898\u4e4b\u4e00\u3002\u8fd1\u5e74\u6765\uff0c\u4ee5\u4e0a\u8bfe\u9898\u7ec4\u901a\u8fc7\u6301\u7eed\u6027\u5408\u4f5c\u7814\u7a76\uff0c\u57fa\u4e8e\u6c27\u5316\u949b\u3001\u9492\u9178\u94cb\u7684\u6c27\u5316\u7269\u534a\u5bfc\u4f53\u5f02\u8d28\u7ed3\uff0c\u9488\u5bf9\u754c\u9762\u6c27\u7a7a\u4f4d\u7f3a\u9677\u4e0e\u5149(\u7535)\u50ac\u5316\u6548\u7387\u95f4\u7684\u5185\u5728\u5173\u7cfb\u8fdb\u884c\u4e86\u6df1\u5165\u7814\u7a76\uff0c\u901a\u8fc7\u7406\u8bba\u6a21\u62df\u548c\u6d4b\u8bd5\u8868\u5f81\u63ed\u793a\u4e86\u6c27\u7a7a\u4f4d\u7a7a\u95f4\u5206\u5e03\u53ca\u7f3a\u9677\u91cd\u6784\u7b49\u8fc7\u7a0b\u5bf9\u754c\u9762\u7535\u8377\u5206\u79bb\u6548\u7387\u7684\u91cd\u8981\u5f71\u54cd\uff0c\u76f8\u5173\u7ed3\u679c\u5148\u540e\u53d1\u8868\u5728Adv. Energy Mater.\u3001Nano Energy\u3001J. Mater. Chem. A\u7b49\u91cd\u8981\u671f\u520a\uff0c\u4e3a\u57fa\u4e8e\u7f3a\u9677\u8c03\u63a7\u8bbe\u8ba1\u9ad8\u6027\u80fd\u5f02\u8d28\u7ed3\u63d0\u4f9b\u4e86\u91cd\u8981\u4f9d\u636e\u3002<\/p>\n

1. Xiaoqiang An, Tong Li, Bo Wen, Junwang Tang, Ziyu Hu, Li-Min Liu*, Jiuhui Qu, C. P. Huang, and Huijuan Liu*, New insights into defect-mediated heterostructures for photoelectrochemical water splitting<\/strong><\/a>, Adv. Energy Mater.<\/strong>, 2016, 1502268.<\/p>\n

2. Xiaoqiang An, Le Zhang, Bo Wen, Zhenao Gu, Li-Min Liu*, Jiuhui Qu, Huijuan Liu*, Boosting photoelectrochemical activities of heterostructured photoanodes through interfacial modulation of oxygen vacancies<\/a><\/strong>, Nano Energy<\/strong> 2017, 35, 290\u2013298.<\/p>\n

3. Xiaoqiang An, Chengzhi Hu, Huijuan Liu, Jiuhui Qu, Oxygen vacancy mediated construction of anatase\/brookite heterophase junctions for high-efficiency photocatalytic hydrogen evolution<\/a><\/strong>, J. Mater. Chem. A<\/strong>, 2017, 5, 24989-24994.<\/p>\n

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