{"id":148805,"date":"2018-08-08T06:30:46","date_gmt":"2018-08-07T22:30:46","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=148805"},"modified":"2018-08-08T11:38:01","modified_gmt":"2018-08-08T03:38:01","slug":"%e9%99%88%e5%bf%a0%e4%bc%9fnano-energy-%ef%bc%9a%e4%bf%ae%e9%a5%b0%e7%9a%84%e7%a9%ba%e5%bf%83%e7%90%83%e5%bd%a2%e5%82%ac%e5%8c%96%e5%89%82%e5%a2%9e%e5%bc%ba%e6%b0%a7%e8%bf%98%e5%8e%9f%e5%8f%8d","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=148805","title":{"rendered":"\u9648\u5fe0\u4f1fNano Energy.\uff1a\u4fee\u9970\u7684\u7a7a\u5fc3\u7403\u5f62\u50ac\u5316\u5242\u589e\u5f3a\u6c27\u8fd8\u539f\u53cd\u5e94\u6d3b\u6027\u548c\u8010\u4e45\u6027"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u6742\u539f\u5b50\u63ba\u6742\u53ca\u8fc7\u5ea6\u91d1\u5c5e\u6742\u5316\u7684\u78b3\u6750\u6599\u53ef\u4ee5\u88ab\u8ba4\u4e3a\u662f\u4fc3\u8fdb\u6c27\u8fd8\u539f\u53cd\u5e94\uff08ORR\uff09\u7f13\u6162\u52a8\u529b\u5b66\u6700\u6709\u5e0c\u671b\u7684\u975e\u8d35\u91cd\u91d1\u5c5e\u5019\u9009\u7269\u3002\u7136\u800c\uff0c\u63d0\u9ad8\u6d3b\u6027\u540c\u65f6\u4fdd\u6301\u652f\u6491\u6750\u6599\u7684\u4f18\u52bf\u7ed3\u6784\u4e00\u76f4\u662f\u4e00\u4e2a\u6311\u6218\u3002\u5728\u8fc7\u53bb\u7684\u7814\u7a76\u4e2d\uff0c\u8bb8\u591a\u4e0d\u540c\u7684\u5355\u4f53\u548c\u805a\u5408\u7269\u5df2\u7ecf\u5355\u72ec\u7528\u4f5c\u6742\u539f\u5b50\u524d\u4f53\uff0c\u4f46\u6ca1\u6709\u4efb\u4f55\u5de5\u4f5c\u4e13\u95e8\u7814\u7a76\u5355\u4f53\u53ca\u5176\u805a\u5408\u7269\u4f5c\u4e3a\u6742\u539f\u5b50\u524d\u4f53\u7269\u4e4b\u95f4\u7684\u5dee\u5f02\u3002\u56e0\u6b64\uff0c\u8003\u8651\u5230\u5355\u4f53\u4e0e\u5176\u805a\u5408\u7269\u4e4b\u95f4\u7684\u7ec4\u5206\u76f8\u4f3c\u6027\u548c\u5206\u5b50\u5927\u5c0f\u7684\u5dee\u5f02\u6027\uff0c\u884d\u751f\u81ea\u5355\u4f53\u53ca\u5176\u805a\u5408\u7269\u7684\u4e24\u79cd\u7c7b\u578b\u50ac\u5316\u5242\u4e4b\u95f4\u7684\u5f02\u540c\u503c\u5f97\u6df1\u5165\u7814\u7a76\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5728\u52a0\u62ff\u5927\u6ed1\u94c1\u5362\u5927\u5b66\u9648\u5fe0\u4f1f<\/b><\/strong>\u6559\u6388<\/b><\/strong>\uff08\u901a\u8baf\u4f5c\u8005<\/b><\/strong>\uff0c\u7b2c\u4e00\u4f5c\u8005\u4e3a\u535a\u58eb\u751f\u5f90\u6500<\/b><\/strong>\uff09<\/b><\/strong>\u5e26\u9886\u4e0b\uff0c\u4e0e\u52a0\u62ff\u5927\u5df4\u62c9\u5fb7\u52a8\u529b\u7cfb\u7edf\u516c\u53f8<\/b><\/strong>\u5408\u4f5c\uff0c\u5236\u5907\u4e86\u9ad8\u8868\u9762\u79ef\u7684\u4e2d\u7a7a\u7403\u5f62\u78b3\u4f5c\u4e3a\u652f\u6491\u6750\u6599\uff0c\u5e76\u4f7f\u7528\u6c28\u57fa\u82ef\u786b\u915a\uff08ATI\uff09\u548c\u805a\u6c28\u57fa\u82ef\u786b\u915a\uff08PATI\uff09\u4f5c\u4e3a\u6742\u539f\u5b50\u524d\u9a71\u4f53\u6765\u5408\u6210\u6c2e\u786b\u5171\u63ba\u6742\u50ac\u5316\u5242\uff0c\u5373HCS-A\u548cHCS-PA\u3002\u8fd9\u4e24\u79cd\u50ac\u5316\u5242\u5177\u6709\u5316\u5b66\u4e0a\u76f8\u4f3c\u7684\u8868\u9762\u7ec4\u6210\uff0c\u6bcf\u79cd\u5143\u7d20\u7684\u5316\u5b66\u72b6\u6001\u4e00\u81f4\u3002\u7136\u800c\uff0c\u53ea\u6709HCS-A\u80fd\u591f\u5927\u7a0b\u5ea6\u7ee7\u627f\u78b3\u8f7d\u4f53\u7684\u5f62\u6001\u5b66\u4f18\u52bf\u548c\u9ad8\u8868\u9762\u79ef\u3002\u5728\u52a8\u529b\u5b66\u548c\u4f20\u8d28\u8fc7\u7a0b\u65b9\u9762\uff0c\u9178\u78b1\u4ecb\u8d28\u4e2dHCS-A\u6bd4HCS-PA\u90fd\u8868\u73b0\u51fa\u66f4\u597d\u7684ORR\u6d3b\u6027\u548c\u66f4\u9ad8\u7684\u56db\u7535\u5b50\u9009\u62e9\u6027\u3002\u9664\u4e86\u51fa\u8272\u7684ORR\u6d3b\u6027\u5916\uff0cHCS-A\u8fd8\u8868\u73b0\u51fa\u4f18\u826f\u7684\u8010\u4e45\u6027\uff0c\u5728\u78b1\u6027\u4ecb\u8d28\u4e2d2\u4e07\u6b21\u5faa\u73af\u540e\u6d3b\u6027\u51e0\u4e4e\u4fdd\u6301\u4e0d\u53d8\u3002PEM\u71c3\u6599\u7535\u6c60\u6d4b\u8bd5HCS-A\u4f5c\u4e3a\u9634\u6781\u50ac\u5316\u5242\u8fbe\u5230\u5cf0\u503c\u529f\u7387\u5bc6\u5ea6500 mW\u00a0cm\u22122<\/sup>\u3002\u5728\u950c\u7a7a\u6c14\u7535\u6c60\u6d4b\u8bd5\u4e2d\uff0cHCS-A\u5728\u7a7a\u6c14\u73af\u5883\u4e2d\u653e\u7535\u5cf0\u503c\u529f\u7387\u5bc6\u5ea6\u8fbe\u5230195 mW\u00a0cm\u22122<\/sup>\u3002\u8fd9\u9879\u5de5\u4f5c\u4e0d\u4ec5\u663e\u793a\u4e86HCS-A\u7684\u826f\u597d\u6027\u80fd\uff0c\u800c\u4e14\u66f4\u91cd\u8981\u7684\u662f\u4e3a\u9009\u62e9\u80fd\u591f\u4fdd\u6301\u826f\u597d\u7ed3\u6784\u7684\u6742\u539f\u5b50\u524d\u4f53\u63d0\u4f9b\u4e86\u65b0\u7684\u89c6\u89d2\u3002\u76f8\u5173\u6210\u679c\u4ee5\u9898\u4e3a\u201cEmbellished hollow spherical catalyst boosting activity and durability for oxygen reduction reaction<\/b><\/strong>\u201d\u53d1\u8868\u5728Nano Energy<\/b><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe1.<\/b><\/strong>\u00a0<\/b><\/strong>HCS-PA\u548cHCS-A<\/b><\/strong>\u5408\u6210<\/b><\/strong>\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a\uff09\u6d3b\u5316HCS\u7684\u5408\u6210\u65b9\u6cd5\u3002<\/p>\n

b\uff09HCS-PA\u7684\u5408\u6210\u65b9\u6cd5\u3002<\/p>\n

c\uff09HCS-A\u7684\u5408\u6210\u65b9\u6cd5\u3002<\/p>\n

\u56fe2.<\/b><\/strong>\u00a0<\/b><\/strong>HCS\uff0cHCS-PA<\/b><\/strong>\u548c<\/b><\/strong>HCS-A<\/b><\/strong>\u7684\u5f62\u8c8c\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a-b\uff09\u5206\u522b\u4e3aHCS\u7684SEN\u56fe\u548cTEM\u56fe\u3002\u6bd4\u4f8b\u5c3a\uff1aa\uff09200nm\uff0cb\uff09100nm\u3002<\/p>\n

c-d\uff09\u5206\u522b\u4e3aHCS-PA\u7684SEN\u56fe\u548cTEM\u56fe\u3002\u6bd4\u4f8b\u5c3a\uff1ac\uff09200nm\uff0cd\uff09300nm\u3002<\/p>\n

e-f\uff09\u5206\u522b\u4e3aHCS-A\u7684SEN\u56fe\u548cTEM\u56fe\u3002\u6bd4\u4f8b\u5c3a\uff1ae\uff09300nm\uff0cf\uff09100nm\u3002<\/p>\n

\u56fe3.<\/b><\/strong>\u00a0<\/b><\/strong>HCS-PA\u548cHCS-A\u7684\u5143\u7d20\u5206\u6790<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a\uff09N\uff0cS\u548cFe\u542b\u91cf\u3002<\/p>\n

b-d\uff09\u5206\u522b\u4e3aN 1s\uff0cS 2p\u548cFe 2p\u7684\u00a0XPS\u5149\u8c31\u3002<\/p>\n

e\uff09HCS-A\u7684STEM\u6697\u573a\u56fe\u50cf\u3002<\/p>\n

f-h\uff09HCS-A\u7684C\uff0cS\u548cFe\u539f\u5b50\u7684\u76f8\u5e94EDX\u5143\u7d20\u5206\u5e03\u56fe\uff0c\u6bd4\u4f8b\u5c3a\uff1a50nm\u3002<\/p>\n

\u56fe<\/b><\/strong>4<\/b><\/strong>.<\/b><\/strong>\u00a0<\/b><\/strong>HCS-A\uff0cHCS-PA<\/b><\/strong>\uff0cHCS-mf\u548cPt<\/b><\/strong>\/<\/b><\/strong>C\u7684\u7535\u5316\u5b66\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a-b\uff09\u5206\u522b\u57285 MH2<\/sub>SO4<\/sub>\u548c0.1 M KOH\u7684RDE\u6781\u5316\u66f2\u7ebf\u56fe\u3002a\uff09\u548cb\uff09\u63d2\u56fe\u5206\u522b\u4e3aHCS-A\u548cHCS-PA\u5728\u52a8\u529b\u5b66\u533a\u57df\u7684LSV\u66f2\u7ebf\uff0c\u901a\u8fc7BET\u8868\u9762\u79ef\u5f52\u4e00\u5316\uff0c\u65cb\u8f6c\u901f\u5ea6\uff1a900rpm\uff0c\u626b\u63cf\u901f\u7387\uff1a5mV cm -2<\/sup>\u3002<\/p>\n

c-d\uff09\u5206\u522b\u57280.5 M\u00a0H2<\/sub>SO4<\/sub>\u548c0.1M KOH\u4e2d\u8ba1\u7b97HCS-A\u548cHCS-PA\u7684\u7535\u5b50\u8f6c\u79fb\u6570\u548c\u8fc7\u6c27\u5316\u7269\u4ea7\u7387\u3002<\/p>\n

e-f\uff09\u5206\u522b\u57280.5 M\u00a0H2<\/sub>SO4<\/sub>\u548c0.1M KOH\u4e2d\u8ba1\u7b97HCS-A\u548cHCS-PA\u7684Tafel\u56fe\u3002<\/p>\n

\u56fe<\/b><\/strong>5<\/b><\/strong>. <\/b><\/strong>HCS-A\u7684\u5faa\u73af\u8010\u4e45\u6027<\/b><\/strong>\u6d4b\u8bd5<\/b><\/strong><\/p>\n

\"\"a-b\uff09\u5206\u522b\u57285 MH2<\/sub>SO4<\/sub>\u548c0.1 M KOH\u4e2d\u6d4b\u8bd5HCS-A\u7684\u5faa\u73af\u8010\u4e45\u6027\u7684LSV\u66f2\u7ebf\u3002<\/p>\n

c-d\uff09\u5206\u522b\u57280.5 M\u00a0H2<\/sub>SO4<\/sub>\u548c0.1 M KOH\u4e2d\u6d4b\u8bd5ADT\u540e\u7684HCS-A\u7684TEM\u56fe\u50cf\u3002\u6bd4\u4f8b\u5c3a\uff1a100nm\u3002<\/p>\n

\u56fe<\/b><\/strong>6<\/b><\/strong>. <\/b><\/strong>HCS-A\u7684<\/b><\/strong>\u8ba1\u65f6\u7535\u6d41\u54cd\u5e94<\/b><\/strong>\u6d4b\u8bd5<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a\uff09\u57280.5 M\u00a0H2<\/sub>SO4<\/sub>\u4e2d\u57280.6V vs. RHE\u65f6\u6d4b\u8bd5\u52a0\u51653M\u7532\u9187\u7684HCS-A\u50ac\u5316\u5242\u548c\u5546\u4e1aTKK 46.6wt\uff05Pt\/C\u50ac\u5316\u5242\u7684\u8ba1\u65f6\u7535\u6d41\u54cd\u5e94\u3002<\/p>\n

b\uff09\u57280.1M KOH\u4e2d\u57280.6V vs. RHE\u65f6\u6d4b\u8bd5\u52a0\u51653M\u7532\u9187\u7684HCS-A\u50ac\u5316\u5242\u548c\u5546\u4e1aTKK 46.6wt\uff05Pt\/C\u50ac\u5316\u5242\u7684\u8ba1\u65f6\u7535\u6d41\u54cd\u5e94\u3002<\/p>\n

\u56fe<\/b><\/strong>7<\/b><\/strong>. <\/b><\/strong>\u71c3\u6599\u7535\u6c60\u548c\u950c\u7a7a\u6c14\u7535\u6c60<\/b><\/strong>\u7684\u7535\u5316\u5b66\u6027\u80fd<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a\uff0cd\uff09\u5206\u522b\u4e3a\u81ea\u5236\u7684\u71c3\u6599\u7535\u6c60\u548c\u81ea\u5236\u950c\u7a7a\u6c14\u7535\u6c60\u3002<\/p>\n

b\uff0ce\uff09\u5206\u522b\u4e3a\u71c3\u6599\u7535\u6c60\u548c\u950c\u7a7a\u6c14\u7535\u6c60\u7684\u5de5\u4f5c\u793a\u610f\u56fe\u3002<\/p>\n

c\uff0cf\uff09\u5206\u522b\u4e3a\u7528HCS-A\u9634\u6781\u5236\u5907\u7684\u71c3\u6599\u7535\u6c60\u548c\u950c\u7a7a\u6c14\u7535\u6c60\u7684\u7535\u6c60\u7535\u538b\u548c\u529f\u7387\u5bc6\u5ea6\u3002<\/p>\n

\u3010\u5c0f\u7ed3<\/b><\/strong>\u3011<\/p>\n

\u672c\u6587\u8bbe\u8ba1\u4e86\u4e00\u79cd\u8d85\u9ad8\u8868\u9762\u79ef\u7684\u7a7a\u5fc3\u78b3\u7403(HCS)\u3002\u4ee5HCS\u4e3a\u78b3\u8f7d\u4f53\uff0c\u5206\u522b\u7528\u6c28\u57fa\u82ef\u786b\u915a\uff08ATI\uff09\u548c\u805a\u6c28\u57fa\u82ef\u786b\u915a\uff08PATI\uff09\u4f5c\u4e3a\u63ba\u6742\u5242\u5236\u5907\u4e86\u4e24\u79cd\u4e0d\u540c\u7c7b\u578b\u7684\u6742\u539f\u5b50\u63ba\u6742\u50ac\u5316\u5242HCS-A\u548cHCS-PA\u3002\u7ed3\u679c\u8868\u660e\uff0c\u4f5c\u4e3a\u6742\u539f\u5b50\u63ba\u6742\u524d\u4f53\u7684\u5355\u4f53\u548c\u805a\u5408\u7269\u5747\u80fd\u63d0\u9ad8ORR\u6d3b\u6027\u3002\u7136\u800c\uff0c\u6c28\u57fa\u82ef\u786b\u915a\u53ef\u4ee5\u4fdd\u6301\u8d85\u9ad8\u8868\u9762\u79ef\u7403\u5f62\u652f\u6491\u6750\u6599\u7684\u521d\u5f62,\u4ece\u800c\u83b7\u5f97\u4f18\u52bf\u5f62\u6001\u548c\u9ad8\u8868\u9762\u79ef\u3002HCS-A\u5728\u9178\u6027\u548c\u78b1\u6027\u4ecb\u8d28\u4e2d\u5747\u8868\u73b0\u51fa\u663e\u8457\u7684ORR\u6d3b\u6027\u3002\u6b64\u5916\uff0cHCS-A\u88ab\u8bc1\u660e\u4f18\u5f02\u7684\u7532\u9187\u8010\u53d7\u6027\u4ee5\u53ca\u5728\u71c3\u6599\u7535\u6c60\u548c\u950c\u7a7a\u6c14\u7535\u6c60\u4e2d\u51fa\u8272\u7684\u529f\u7387\u5bc6\u5ea6\u3002\u6b64\u9879\u7814\u7a76\u4e0d\u4ec5\u62a5\u9053\u4e86\u4e00\u79cd\u9ad8\u6d3b\u6027\u50ac\u5316\u5242\uff0c\u66f4\u91cd\u8981\u7684\u662f\u9a8c\u8bc1\u4e86\u4e00\u79cd\u4ece\u652f\u6491\u6750\u6599\u4e2d\u4fdd\u6301\u7ed3\u6784\u4f18\u52bf\u7684\u7b56\u7565\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5<\/b><\/strong>\uff1a<\/b><\/strong>Embellished hollow spherical catalyst boosting activity and durability for oxygen reduction reaction<\/u><\/a>\uff08Nano Energy,2018,DOI\uff1a10.1016\/j.nanoen.2018.07.031\uff09<\/p>\n

\u3010\u4f5c\u8005\u7b80\u4ecb<\/b><\/strong>\u3011<\/p>\n

\u9648\u5fe0\u4f1f<\/b><\/strong>\uff1a\u52a0\u62ff\u5927\u6ed1\u94c1\u5362\u5927\u5b66(University of Waterloo)\u5316\u5b66\u5de5\u7a0b\u7cfb\u6559\u6388\uff0c\u6ed1\u94c1\u5362\u5927\u5b66\u7535\u5316\u5b66\u80fd\u6e90\u4e2d\u5fc3\u4e3b\u4efb\uff0c\u52a0\u62ff\u5927\u56fd\u5bb6\u9996\u5e2d\u79d1\u5b66\u5bb6(CRC-Tier 1), \u56fd\u9645\u7535\u5316\u5b66\u80fd\u6e90\u79d1\u5b66\u9662\uff08IAOEES\uff09\u526f\u4e3b\u5e2d\uff0c\u52a0\u62ff\u5927\u5de5\u7a0b\u9662\u9662\u58eb\u3002\u9648\u5fe0\u4f1f\u9662\u58eb\u5e26\u9886\u4e00\u652f\u7ea670\u4eba\u7684\u7814\u7a76\u56e2\u961f\u5e38\u5e74\u81f4\u529b\u4e8e\u71c3\u6599\u7535\u6c60\uff0c\u91d1\u5c5e\u7a7a\u6c14\u7535\u6c60\uff0c\u9502\u79bb\u5b50\u7535\u6c60\uff0c\u9502\u786b\u7535\u6c60\uff0c\u9502\u7845\u7535\u6c60\uff0c\u6db2\u6d41\u7535\u6c60\u7b49\u50a8\u80fd\u5668\u4ef6\u7684\u7814\u53d1\u548c\u4ea7\u4e1a\u5316\u3002\u8fd1\u5e74\u6765\u5728Nature Energy, Nature Nanotechnology, Nature Communication, Angewandte Chemie International Edition, Advanced Materials, Energy & Environmental Science, Journal of the American Chemical Society, ACS Nano \u7b49\u56fd\u9645\u77e5\u540d\u671f\u520a\u53d1\u8868\u8bba\u6587230\u4f59\u7bc7\u3002\u76ee\u524d\u4e3a\u6b62\uff0c\u6587\u7ae0\u5df2\u5f15\u7528\u6b21\u6570\u8fd1 14000\u6b21, H-index \u6307\u6570\u4e3a58\uff0c\u5e76\u62c5\u4efbACS applied & Material Interfaces (ACS-AMI) \u526f\u4e3b\u7f16\u3002<\/p>\n

\u8bfe\u9898\u7ec4\u4e3b\u9875\uff1ahttp:\/\/chemeng.uwaterloo.ca\/zchen\/<\/u><\/a><\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u5b66\u672f\u7ec4\u6728\u6587\u97ec<\/b><\/strong>\u7ffb\u8bd1\uff0cTongwen<\/b><\/strong>\u4fee\u6b63\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8<\/u><\/a>\u3002\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

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