{"id":149078,"date":"2018-08-13T06:30:30","date_gmt":"2018-08-12T22:30:30","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=149078"},"modified":"2018-08-13T23:17:52","modified_gmt":"2018-08-13T15:17:52","slug":"acs-nano-%e5%af%8c%e6%b0%a7%e7%a9%ba%e4%bd%8d%e6%b0%a7%e5%8c%96%e9%92%b4%e7%94%a8%e4%ba%8e%e6%9f%94%e6%80%a7%e9%98%b2%e6%b0%b4%e6%9d%82%e5%8c%96%e9%94%8c%e7%94%b5%e6%b1%a0","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=149078","title":{"rendered":"ACS Nano: \u5bcc\u6c27\u7a7a\u4f4d\u6c27\u5316\u94b4\u7528\u4e8e\u67d4\u6027\u9632\u6c34\u6742\u5316\u950c\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u968f\u7740\u79d1\u6280\u7684\u8fdb\u6b65\u548c\u4eba\u5de5\u667a\u80fd\u6280\u672f\u7684\u4e0d\u65ad\u53d1\u5c55\uff0c\u4fbf\u643a\u67d4\u6027\u548c\u53ef\u7a7f\u6234\u7535\u5b50\u4ea7\u54c1\u6210\u4e3a\u4e86\u672a\u6765\u7535\u5b50\u8bbe\u5907\u7684\u91cd\u8981\u53d1\u5c55\u8d8b\u52bf\u3002\u56e0\u6b64\uff0c\u5f00\u53d1\u9ad8\u6027\u80fd\u7684\u67d4\u6027\u50a8\u80fd\u5668\u4ef6\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002\u76f8\u6bd4\u4e8e\u4f20\u7edf\u7684\u9502\u79bb\u5b50\u7535\u6c60\uff0c\u65b0\u578b\u53ef\u5145\u7535\u950c\u57fa\u7535\u6c60\u7531\u4e8e\u5176\u672c\u8eab\u7684\u5b89\u5168\u6027\u3001\u50a8\u91cf\u4e30\u5bcc\u4ee5\u53caZn2+<\/sup>\/Zn\u8f83\u4f4e\u7684\u6c27\u5316\u8fd8\u539f\u7535\u4f4d\uff0c\u6210\u4e3a\u5f15\u4eba\u6ce8\u76ee\u7684\u5907\u9009\u89e3\u51b3\u65b9\u6848\u4e4b\u4e00\u3002\u5728\u950c\u57fa\u7535\u6c60\u4e2d\uff0c\u950c\u7a7a\u6c14\u7535\u6c60\u56e0\u5176\u8f83\u9ad8\u7684\u80fd\u91cf\u5bc6\u5ea6\u53d7\u5230\u4e86\u7814\u7a76\u8005\u7684\u5e7f\u6cdb\u5173\u6ce8\uff0c\u4f46\u662f\u5176\u8f83\u4f4e\u7684\u529f\u7387\u5bc6\u5ea6\uff0c\u8f83\u5dee\u7684\u9632\u6c34\u6027\u53ca\u67d4\u97e7\u6027\u9650\u5236\u4e86\u5176\u5728\u53ef\u7a7f\u6234\u7535\u5b50\u8bbe\u5907\u4e0a\u7684\u5e94\u7528\uff0c\u800c\u950c\u94b4\u7535\u6c60\u5219\u5177\u6709\u8f83\u9ad8\u7684\u529f\u7387\u5bc6\u5ea6\u548c\u8f83\u5f3a\u7684\u53ef\u5851\u6027\u3002\u56e0\u6b64\uff0c\u8bbe\u8ba1\u4e00\u79cd\u65e2\u5177\u6709\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u53c8\u5177\u6709\u9ad8\u529f\u7387\u5bc6\u5ea6\u7684\u65b0\u578b\u6df7\u5408\u50a8\u80fd\u5668\u4ef6\u5bf9\u4e8e\u53ef\u7a7f\u6234\u7535\u5b50\u8bbe\u5907\u7684\u5927\u89c4\u6a21\u5e94\u7528\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u9999\u6e2f\u57ce\u5e02\u5927\u5b66\u652f\u6625\u4e49\u6559\u6388<\/strong>\u8bfe\u9898\u7ec4\u5728ACS Nano<\/strong>\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cFlexible Waterproof Rechargeable Hybrid Zinc Batteries Initiated by Multifunctional Oxygen Vacancies-Rich Cobalt Oxide\u201d<\/strong>\u7684\u8bba\u6587\uff0c\u8be5\u5de5\u4f5c\u901a\u8fc7\u5728Ar\u6c14\u6c1b\u56f4\u4e0b\u4f7f\u7528\u7b49\u79bb\u5b50\u523b\u8680\u6280\u672f\u5408\u6210\u4e86\u4e00\u79cd\u542b\u6709\u4e30\u5bcc\u6c27\u7a7a\u4f4d\u7684\u94b4\u6c27\u5316\u7269\uff0c\u5e76\u4ee5\u6b64\u5236\u5907\u4e86\u4e00\u79cd\u65b0\u578b\u950c\u6c27\u5316\u94b4\u548c\u950c\u7a7a\u6c14\u6df7\u5408\u7535\u6c60\u3002Co3<\/sub>O4<\/sub>\u4f5c\u4e3a\u4e00\u79cd\u950c\u79bb\u5b50\u7535\u6c60\u6b63\u6781\u6750\u6599\uff0c\u5728\u5176\u8868\u9762\u4e2d\u5f15\u5165\u6c27\u7a7a\u4f4d\u53ef\u4ee5\u6709\u6548\u63d0\u9ad8\u5176OER\u548cORR\u7535\u50ac\u5316\u6027\u80fd\u8fdb\u800c\u63d0\u9ad8\u5176\u4f5c\u4e3a\u950c\u7a7a\u6c14\u7535\u6c60\u6b63\u6781\u6750\u6599\u7684\u7535\u5316\u5b66\u6027\u80fd\uff0c\u6545\u800c\u53ef\u4ee5\u4f5c\u4e3a\u540c\u65f6\u8fdb\u884c\u4e24\u79cd\u7535\u5316\u5b66\u53cd\u5e94\uff08OER\uff0cORR\u7535\u50ac\u5316\u548c\u6cd5\u62c9\u7b2cCo\u2212O \u2194 Co\u2212O\u2212OH\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\uff09\u7684\u8f7d\u4f53\u3002<\/p>\n

\u6b64\u65b0\u578b\u6df7\u5408\u950c\u57fa\u52a8\u529b\u7535\u6c60\u4e0d\u4ec5\u5177\u6709\u8f83\u9ad8\u7684\u529f\u7387\u5bc6\u5ea63200 W\u00b7kg\u22121<\/sup>, \u540c\u65f6\u5177\u6709\u8f83\u9ad8\u7684\u80fd\u91cf\u5bc6\u5ea61060 Wh\u00b7kg\u22121<\/sup>, \u5e76\u4e14\u7ecf\u8fc7440\u5c0f\u65f61500\u6b21\u5faa\u73af\u540e\u4ecd\u7136\u5177\u6709\u826f\u597d\u7684\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0c\u901a\u8fc7\u4f7f\u7528\u51dd\u80f6\u7535\u89e3\u8d28\u5c06\u5176\u7ec4\u88c5\u6210\u5168\u7535\u6c60\u540e\uff0c\u8be5\u56fa\u6001\u6df7\u5408\u7535\u6c60\u4e5f\u5c55\u793a\u51fa\u826f\u597d\u7684\u5b89\u5168\u6027\u3001\u4f18\u79c0\u7684\u9632\u6c34\u548c\u8010\u6d17\u80fd\u529b\uff0c\u5728\u6c34\u4e2d\u6d78\u6ce120\u5c0f\u65f6\u6216\u6d17\u6da41\u5c0f\u65f6\u540e\u4ecd\u53ef\u4fdd\u6301\u8fd190%\u4ee5\u4e0a\u7684\u7535\u5316\u5b66\u6027\u80fd\u3002\u9664\u6b64\u4e4b\u5916\uff0c\u5f53\u5176\u66b4\u9732\u5728\u7a7a\u6c14\u4e2d\u65f6\uff0c\u8be5\u65b0\u578b\u6df7\u5408\u950c\u57fa\u52a8\u529b\u7535\u6c60\u53ef\u4ee5\u81ea\u52a8\u6062\u590d\u8f93\u51fa\u7535\u91cf\u3002\u8be5\u5de5\u4f5c\u901a\u8fc7\u7b49\u79bb\u5b50\u4f53\u523b\u8680\u6280\u672f\u5bf9\u7535\u6781\u6750\u6599\u8fdb\u884c\u6539\u6027\uff0c\u5b9e\u73b0\u4e86\u5176\u5728\u6df7\u5408\u50a8\u80fd\u9886\u57df\u4e0a\u7684\u5e94\u7528\uff0c\u540c\u65f6\u5176\u6240\u7814\u5236\u7684\u67d4\u6027\u50a8\u80fd\u8bbe\u5907\u53ef\u4ee5\u7a33\u5b9a\u7684\u4e3a\u5546\u4e1a\u5316\u667a\u80fd\u624b\u8868\u63d0\u4f9b\u80fd\u91cf\uff0c\u5c55\u73b0\u51fa\u5de8\u5927\u7684\u5e94\u7528\u524d\u666f\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe1. \u5bcc\u6c27\u7a7a\u4f4dCo3<\/sub>O4\u2212x<\/sub>\u7eb3\u7c73\u68d2\u7ed3\u6784\u5408\u6210\u793a\u610f\u56fe\u53ca\u5fae\u89c2\u7ed3\u6784\u8868\u5f81<\/strong>
\n \"\"
\n (a) \u5bcc\u6c27\u7a7a\u4f4dCo3<\/sub>O4\u2212x<\/sub>\u7eb3\u7c73\u68d2\u7ed3\u6784\u5408\u6210\u793a\u610f\u56fe
\n (b) Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u68d2\u7684SEM\u7167\u7247
\n (c) Co3<\/sub>O4-x<\/sub>\u7eb3\u7c73\u68d2\u7684SEM\u7167\u7247
\n (d) Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u68d2Co 2p\u7684XPS\u56fe\u8c31
\n (e) Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u68d2O 1s \u7684XPS\u56fe\u8c31
\n (f) Co3<\/sub>O4-x<\/sub>\u7eb3\u7c73\u68d2Co 2p\u7684XPS\u56fe\u8c31
\n (g) Co3<\/sub>O4-x<\/sub>\u7eb3\u7c73\u68d2O 1s \u7684XPS\u56fe\u8c31<\/p>\n

\u56fe2. \u5bcc\u6c27\u7a7a\u4f4dCo3O4\u2212x\u7eb3\u7c73\u68d2\u7535\u50ac\u5316\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

(a)Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u68d2\u548cCo3<\/sub>O4-x<\/sub> \u57280.1 M KOH\u4e2d\u7684CV\u66f2\u7ebf
\n (b)Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u68d2\u548cCo3<\/sub>O4-x<\/sub>\u7684ORR\u6027\u80fd
\n (c)RRDE\u6d4b\u8bd5
\n (d)Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u68d2\u548cCo3<\/sub>O4-x<\/sub>\u7684OER\u6027\u80fd
\n (e)Tafel\u66f2\u7ebf
\n (f)Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u68d2\u548cCo3<\/sub>O4-x<\/sub>\u7684\u6574\u4f53\u6781\u5316\u66f2\u7ebf<\/p>\n

\u56fe3. \u950c\u57fa\u6742\u5316\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong>
\n \"\"
\n (a)Zn\u2212Co3<\/sub>O4\u2212x<\/sub>\/Zn\u2212air \u6742\u5316\u7535\u6c60\u793a\u610f\u56fe
\n (b)\u6742\u5316\u950c\u7535\u6c60CV\u66f2\u7ebf
\n (c)\u5145\u653e\u7535\u66f2\u7ebf
\n (d)\u626b\u63cf\u7535\u6d41\u66f2\u7ebf
\n (e)\u5145\u653e\u7535\u529f\u7387\u5bc6\u5ea6\u66f2\u7ebf
\n (f)\u6301\u7eed\u653e\u7535\u66f2\u7ebf
\n (g)\u5faa\u73af\u6027\u6d4b\u8bd5
\n (h)\u4e0d\u540c\u65f6\u95f4\u5faa\u73af\u6027\u6d4b\u8bd5\u540e\u7684\u5145\u653e\u7535\u66f2\u7ebf<\/p>\n

\u56fe4. \u4e0d\u540c\u6d4b\u8bd5\u6761\u4ef6\u4e0b\u6742\u5316\u950c\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

(a)\u65e0\u6c27\u73af\u5883\u4e2d\u7684\u5145\u653e\u7535\u66f2\u7ebf
\n (b)\u6709\u6c27\u73af\u5883\u4e2d\u7684\u5145\u653e\u7535\u66f2\u7ebf
\n (c)\u5145\u653e\u7535\u5faa\u73af\u6d4b\u8bd5
\n (d)\u6052\u7535\u6d41\u5145\u7535\/\u653e\u7535\u5faa\u73af\u6d4b\u8bd5
\n (e)\u542b\u6c34\u73af\u5883\u4e2d\u7684\u7535\u538b\u66f2\u7ebf
\n (f)\u6301\u7eed\u6d78\u6ce1\u6d4b\u8bd5\u4e0b\u7684\u5f00\u8def\u7535\u538b
\n (g)\u6301\u7eed\u6c34\u6d17\u6d4b\u8bd5\u4e0b\u7684\u7535\u5316\u5b66\u6027\u80fd<\/p>\n

\u56fe5. \u950c\u57fa\u6742\u5316\u7535\u6c60\u7684\u5e94\u7528\u5c55\u793a\u548c\u5b89\u5168\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

(a)Zn\u2212Co3<\/sub>O4\u2212x<\/sub>\/Zn\u2212air \u6742\u5316\u7535\u6c60\u6052\u7535\u6d41\u5145\u7535\/\u653e\u7535\u66f2\u7ebf
\n (b)\u6742\u5316\u7535\u6c60\u4e3aLED\u4f9b\u7535
\n (c)\u6742\u5316\u7535\u6c60\u7535\u91cf\u8017\u5c3d
\n (d)\u6742\u5316\u7535\u6c60\u6062\u590d\u4f9b\u7535
\n (e-g) \u6742\u5316\u7535\u6c60\u7684\u67d4\u6027\u6d4b\u8bd5<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u8be5\u7814\u7a76\u901a\u8fc7\u5728\u5177\u6709\u81ea\u652f\u6491Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u68d2\u7ed3\u6784\u4e0a\u521b\u9020\u4e30\u5bcc\u7684\u6c27\u7a7a\u4f4d\uff0c\u4f7f\u94b4\u6c27\u5316\u7269(Co3<\/sub>O4\u2212x<\/sub>)\u53ef\u4ee5\u6210\u529f\u7684\u6267\u884c\u591a\u4e2a\u7535\u5316\u5b66\u53cd\u5e94\uff0c\u5305\u62ecORR\/ OER\u7535\u50ac\u5316\u53cd\u5e94\u548c\u6cd5\u62c9\u7b2cCo\u2212O \u2194 Co\u2212O\u2212OH\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u3002\u7814\u7a76\u8005\u5229\u7528\u6b64\u7279\u6b8a\u6027\u8d28\u6240\u5236\u5907\u7684\u950c\u57fa\u6742\u5316\u7535\u6c60\u5177\u6709\u9ad8\u529f\u7387\u5bc6\u5ea63200 W\u00b7kg\u22121<\/sup>\u548c\u9ad8\u80fd\u91cf\u5bc6\u5ea61060 Wh\u00b7kg\u22121<\/sup>,\u4ee5\u53ca\u5728\u4e0d\u540c\u6d4b\u8bd5\u6761\u4ef6\u4e0b\u5c55\u73b0\u51fa\u4f18\u79c0\u7684\u5145\u653e\u7535\u7a33\u5b9a\u6027\u3002\u57fa\u4e8e\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u7684\u56fa\u6001\u6df7\u5408\u7535\u6c60
\n \u66f4\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u9632\u6c34\u6027\uff0c\u67d4\u97e7\u6027\u548c\u826f\u597d\u7684\u73af\u5883\u9002\u5e94\u80fd\u529b\u3002\u6b64\u5916\uff0c\u5b83\u53ef\u4ee5\u5728\u7a7a\u6c14\u4e2d\u81ea\u52a8\u6062\u590d\u8f93\u51fa\u7535\u529b\uff0c\u5f88\u6709\u6f5c\u529b\u6210\u4e3a\u4e0b\u4e00\u4ee3\u50a8\u80fd\u5668\u4ef6\u5e76\u5927\u89c4\u6a21\u5e94\u7528\u4e8e\u67d4\u6027\u53ef\u7a7f\u6234\u7535\u5b50\u8bbe\u5907\u53ca\u5176\u4ed6\u6280\u672f\u9886\u57df\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a Flexible Waterproof Rechargeable Hybrid Zinc Batteries Initiated by Multifunctional Oxygen Vacancies-Rich Cobalt Oxide (DOI: 10.1021\/acsnano.8b04317)<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/pubs.acs.org\/doi\/10.1021\/acsnano.8b04317<\/a><\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u65b0\u80fd\u6e90\u5c0f\u7ec4\u6a59\u590f\u7f16\u8bd1\u6574\u7406\uff0c\u53c2\u4e0e\u65b0\u80fd\u6e90\u8bdd\u9898\u8ba8\u8bba\u8bf7\u52a0\u5165\u201c\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u6750\u6599\u4ea4\u6d41\u7fa4 422065953\u201d\u3002<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaokefu\uff0c\u6211\u4eec\u4f1a\u9080\u8bf7\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/strong><\/p>\n

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