{"id":154229,"date":"2018-09-23T06:25:38","date_gmt":"2018-09-22T22:25:38","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=154229"},"modified":"2018-09-22T20:25:59","modified_gmt":"2018-09-22T12:25:59","slug":"%e5%be%90%e7%ba%a2%e6%98%9f%e9%99%a2%e5%a3%ab%e5%bc%a0%e9%a1%ba%e5%b9%b3acs-nano%ef%bc%9a%e5%8f%91%e5%85%89plexciton%e5%88%a9%e7%94%a8%e4%b8%ad%e7%ad%89%e8%80%a6%e5%90%88%e5%bc%ba%e5%ba%a6%e5%8c%ba","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=154229","title":{"rendered":"\u5f90\u7ea2\u661f\u9662\u58eb&\u5f20\u987a\u5e73ACS Nano\uff1a\u53d1\u5149Plexciton:\u5229\u7528\u4e2d\u7b49\u8026\u5408\u5f3a\u5ea6\u533a\u57df\u7684\u7b49\u79bb\u6fc0\u5143-\u6fc0\u5b50\u76f8\u4e92\u4f5c\u7528"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6b66\u6c49\u5927\u5b66\u7684\u5f90\u7ea2\u661f\u9662\u58eb\u548c\u5f20\u987a\u5e73\u526f\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u62a5\u9053\u4e86\u5728\u7eb3\u7c73\u7acb\u65b9\u4f53\u2014\u91d1\u5c5e\u819c\u7cfb\u7edf (NCOM)\u4e2d\u4ea7\u751f\u7684\u9ad8\u5ea6\u5c40\u57df\u7684\u7b49\u79bb\u6fc0\u5143\u548c\u5355\u5c42WSe2<\/sub>\u4e2d\u7684\u4e2d\u6027\u6fc0\u5b50\u4e0e\u4e4b\u95f4\u7684\u8026\u5408\u3002\u8be5\u4f53\u7cfb\u7684\u6697\u573a\u6563\u5c04\u5149\u8c31\u4e2d\u51fa\u73b0\u4e86Rabi\u5288\u88c2\uff0c\u4e14\u5176\u8272\u6563\u66f2\u7ebf\u5448\u73b0\u51fa\u4e86anticrossing\u7684\u7279\u6027\uff0c\u8fd9\u8bf4\u660e\u7b49\u79bb\u6fc0\u5143\u548c\u6fc0\u5b50\u7684\u6df7\u5408\u6001plexciton\u5df2\u7ecf\u5f62\u6210\u4e86\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0c\u5728\u8fd9\u4e2a\u4f53\u7cfb\u4e2d\uff0cplexciton\u7684\u81ea\u53d1\u8f90\u5c04\u8367\u5149\u5f97\u5230\u4e86\u6781\u5927\u7684\u589e\u5f3a\uff0c\u76f8\u8f83\u4e8e\u6ca1\u6709\u7eb3\u7c73\u7acb\u65b9\u7684\u5730\u65b9\uff0c\u8367\u5149\u589e\u5f3a\u8fbe\u5230\u4e861700\u500d\uff0c\u5176\u4e2d\u8f90\u5c04\u589e\u5f3a\u8d21\u732e\u4e86410\u500d\u3002\u76f8\u5e94\u7684\u8ba1\u7b97\u8868\u660e\uff0c\u8367\u5149\u589e\u5f3a\u4e00\u65b9\u9762\u6765\u81ea\u7eb3\u7c73\u95f4\u9699\u4e2d\u7b49\u79bb\u6fc0\u5143\u7684\u7a7a\u95f4\u5c40\u57df\u6027\uff0c\u53e6\u4e00\u65b9\u9762\u6765\u81ea\u5355\u5c42WSe2<\/sub>\u4e2d\u5f3a\u6fc0\u5b50\u6548\u5e94\u5bfc\u81f4\u6df7\u5408\u6001\u7684\u5c40\u57df\u6001\u5bc6\u5ea6\u5728WSe2<\/sub>\u533a\u57df\u5185\u5f97\u5230\u589e\u5f3a\uff0c\u5373\u5f3a\u6fc0\u5b50\u6548\u5e94\u5bfc\u81f4\u771f\u7a7a\u573a\u7684\u91cd\u65b0\u5206\u5e03\u3002\u800c\u8fd9\u4e24\u79cd\u673a\u5236\u7684\u5171\u540c\u4f5c\u7528\u662f\u4f53\u7cfb\u8fbe\u5230\u6700\u5927\u8367\u5149\u53d1\u5c04\u7684\u539f\u56e0\uff0c\u5145\u5206\u5229\u7528\u4e86\u590d\u5408\u4f53\u7cfb\u5904\u4e8e\u4e2d\u7b49\u8026\u5408\u5f3a\u5ea6\u533a\u57df\u7684\u4f18\u70b9\u3002\u6b64\u65f6\u7684\u8367\u5149\u589e\u5f3a\u4e0d\u518d\u662f\u4f20\u7edf\u7684Plasmon enhanced fluorescence\uff0c\u4e8c\u662f\u66f4\u4e3a\u5e7f\u4e49\u7684Plexciton enhanced fluorescence more than the traditional Purcell effect\u3002\u8fdb\u4e00\u6b65\u7684\u5b9e\u9a8c\u8bc1\u660e\uff0c\u6539\u53d8\u94f6\u7eb3\u7c73\u7acb\u65b9\u53ef\u4ee5\u5b9e\u73b0\u5bf9\u4e8eRabi\u5288\u88c2\u5927\u5c0f\u548c\u6a21\u5f0f\u4f53\u79ef\u5927\u5c0f\u7684\u8c03\u63a7\u3002\u603b\u7684\u6765\u8bf4\uff0c\u8fd9\u79cd\u9ad8\u5ea6\u7d27\u51d1\u7684\u7cfb\u7edf\u53ef\u4ee5\u4e3a\u6df1\u4e9a\u6ce2\u957f\u5c3a\u5ea6\u4e0b\u7684cQED\u5b9e\u9a8c\u63d0\u4f9b\u4e86\u5ba4\u6e29\u7684\u6d4b\u8bd5\u5e73\u53f0\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cLight-Emitting Plexciton: Exploiting Plasmon-Exciton Interaction in the Intermediate Coupling Regime\u201d<\/strong>\u53d1\u8868\u5728\u56fd\u9645\u8457\u540d\u671f\u520aACS Nano<\/strong>\u4e0a\u3002\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\u4e3a\u6b66\u6c49\u5927\u5b66\u9ad8\u7b49\u7814\u7a76\u9662\u7684\u535a\u58eb\u751f\u5b59\u5609\u4f1f\u548c\u80e1\u534e\u5929<\/strong>\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

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\n \uff08a\uff09 NCOM\u7cfb\u7edf\u7684\u793a\u610f\u56fe\uff0c\u5305\u62ec\u5728\u8d85\u5149\u6ed1\u91d1\u819c\u57fa\u5e95\u4e0a\u7684\u94f6\u7eb3\u7c73\u7acb\u65b9\u4f53\uff0c\u6c27\u5316\u94dd\u3001\u5355\u5c42WSe2<\/sub>\u548c\u94f6\u7eb3\u7c73\u7acb\u65b9\u8868\u9762\u7684PVP\u5c06\u94f6\u7eb3\u7c73\u7acb\u65b9\u548c\u91d1\u819c\u9694\u5f00\uff1b<\/p>\n

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\n \uff08a\uff09 \u7531P-\uff08\u7ea2\u8272\uff09\u548cS-\uff08\u9ed1\u8272\uff09\u504f\u632f\u5149\u6fc0\u53d1\u7684\u5f52\u4e00\u5316\u6697\u573a\u6563\u5c04\u5149\u8c31\uff0c\u5b83\u4eec\u4e4b\u95f4\u7684\u5dee\uff08\u84dd\u8272\uff09\u5f97\u5230\u4e86800 nm\u5904\u7684\u5cf0\uff1b<\/p>\n

\uff08b\uff09 \u8ba1\u7b97\u5f97\u5230\u7684\u7531P\u504f\u632f\u5e73\u9762\u6ce2\uff08PW\uff0c\u7ea2\u7ebf\uff09\u6fc0\u53d1\u7684\u5f52\u4e00\u5316\u6563\u5c04\u5149\u8c31\u548c\u6cbfz\u65b9\u5411\u7531\u5076\u6781\u5b50\u6fc0\u53d1\u7684\u5f52\u4e00\u5316\u5438\u6536\u5149\u8c31\uff08\u84dd\u7ebf\uff09\u3002<\/p>\n

\u56fe\u4e09\u3001WSe2<\/sub>\u4e2d\u7684X0<\/sup>\u6fc0\u5b50\u4e0eNCOM\u4e2d\u7684\u7b49\u79bb\u6fc0\u5143\u78c1\u6a21\u5f0f\u4e4b\u95f4\u7684\u8026\u5408<\/strong><\/p>\n

\"\"\uff08a\uff09 \u5355\u5c42WSe2<\/sub>\u9694\u79bb\u7684NCOM\u7684\u6697\u573a\u6563\u5c04\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09 \u5728\uff08a\uff09\u4e2d\u6807\u51fa\u7684\u5355\u4e2a\u94f6\u7eb3\u7c73\u7acb\u65b9\u4f53\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09 NCOM\u548c\u5355\u5c42WSe2<\/sub>\u8026\u5408\u7684\u6697\u573a\u6563\u5c04\u5149\u8c31\uff0c\u6c27\u5316\u94dd\u6c89\u79ef\u7684\u8303\u56f4\u4e3a10 nm\u81f332 nm\uff1b<\/p>\n

\uff08d\uff09 \u4e0aplexciton\u5206\u652f\uff08UPB\uff09\u548c\u4e0bplexciton\u5206\u652f\uff08LPB\uff09\u7684\u8272\u6563\u66f2\u7ebf\uff1b<\/p>\n

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\n \"\"
\n \uff08a\uff09 \u5355\u5c42WSe2<\/sub>\u9694\u79bb\u7684NCOM\u7684PL\u6210\u50cf\uff1b<\/p>\n

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\uff08c\uff09 PL\u589e\u5f3a\u4e0e\u7b49\u79bb\u6fc0\u5143\u5171\u632f\u5cf0\u4f4d\u7684\u5173\u7cfb\u3002<\/p>\n

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\n \"\"\uff08a\uff09 \u6ca1\u6709WSe2<\/sub>\u5c42\u65f6\u7684NCOM\u5728x\u6216y\u65b9\u5411\u4e0a\u7684LDOS\u5206\u91cf\uff0c\u6ce2\u957f\u5728746.4 nm\uff1b<\/p>\n

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\uff08d\uff09 \u80fd\u91cf\u5728WSe2<\/sub>\u548c\u5176\u4ed6\u90e8\u5206\u4e2d\u7684\u767e\u5206\u6bd4\u4e0e\u7ea6\u5316\u632f\u5b50\u5f3a\u5ea6f<\/em>\u7684\u5173\u7cfb\u3002<\/p>\n

\u56fe\u516d\u3001\u590d\u5408\u4f53\u7cfb\u7684\u6027\u8d28\u968f\u7acb\u65b9\u4f53\u5c3a\u5bf8\u53d8\u5316\u7684\u89c4\u5f8b\"\"<\/strong>
\n \uff08a\uff09 \u4ece\u6697\u573a\u6563\u5c04\u5149\u8c31\u4e2d\u62df\u5408\u7684Rabi\u5288\u88c2\u5927\u5c0f\u4e0e9\u4e2a\u4e0d\u540c\u5927\u5c0f\u7684\u94f6\u7eb3\u7c73\u7acb\u65b9\u4f53\u7684\u5c3a\u5bf8\u7684\u5173\u7cfb\uff1b<\/p>\n

\uff08b\uff09 NCOM\u4f53\u7cfb\u7684\u6a21\u5f0f\u4f53\u79ef\u4e0e\u94f6\u7eb3\u7c73\u7acb\u65b9\u8fb9\u957f\u7684\u5173\u7cfb\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb<\/strong><\/p>\n

\n \u5f90\u7ea2\u661f\u9662\u58eb\uff1a<\/strong> \u6c5f\u82cf\u704c\u4e91\u53bf\u4eba\uff0c\u73b0\u4efb\u6b66\u6c49\u5927\u5b66\u7269\u7406\u79d1\u5b66\u4e0e\u6280\u672f\u5b66\u9662\u9662\u957f\uff0c\u6b66\u6c49\u5927\u5b66\u9ad8\u7b49\u7814\u7a76\u9662\u526f\u9662\u957f\u30021992\u5e74\u6bd5\u4e1a\u4e8e\u5317\u4eac\u5927\u5b66\u6280\u672f\u7269\u7406\u7cfb\uff0c\u83b7\u5b66\u58eb\u5b66\u4f4d\uff1b2002\u5e74\u6bd5\u4e1a\u4e8e\u745e\u5178\u67e5\u5c14\u83ab\u65af\u7406\u5de5\u5927\u5b66\u5e94\u7528\u7269\u7406\u7cfb\uff0c\u83b7\u535a\u58eb\u5b66\u4f4d\u30022002\u5e74\u81f32004\u5e74\u4efb\u745e\u5178\u9686\u5fb7\u5927\u5b66\u56fa\u4f53\u7269\u7406\u7cfb\u52a9\u7406\u6559\u6388\u30022005\u5e74\u5165\u9009\u4e2d\u79d1\u9662\u767e\u4eba\u8ba1\u5212\uff0c\u4efb\u7269\u7406\u7814\u7a76\u6240\u7814\u7a76\u5458\uff1b2006\u5e74\u81f32008\u5e74\u4efb\u4e2d\u79d1\u9662\u7269\u7406\u7814\u7a76\u6240\u8868\u9762\u7269\u7406\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u526f\u4e3b\u4efb\uff1b2009\u5e74\u81f32014\u5e74\u4efb\u4e2d\u79d1\u9662\u7269\u7406\u7814\u7a76\u6240\u7eb3\u7c73\u7269\u7406\u4e0e\u5668\u4ef6\u5b9e\u9a8c\u5ba4\u4e3b\u4efb\u30022012\u5e746\u6708\u4efb\u6b66\u6c49\u5927\u5b66\u7eb3\u7c73\u79d1\u5b66\u4e0e\u6280\u672f\u7814\u7a76\u4e2d\u5fc3\u4e3b\u4efb\uff1b2014\u5e74\u4efb\u6b66\u6c49\u5927\u5b66\u7269\u7406\u79d1\u5b66\u4e0e\u6280\u672f\u5b66\u9662\u6559\u6388\u3001\u526f\u9662\u957f\uff0c\u6b66\u6c49\u5927\u5b66\u9ad8\u7b49\u7814\u7a76\u9662\u526f\u9662\u957f\uff1b2016\u5e74\u4efb\u6b66\u6c49\u5927\u5b66\u7269\u7406\u79d1\u5b66\u4e0e\u6280\u672f\u5b66\u9662\u9662\u957f\u30022006\u5e74\u83b7\u56fd\u5bb6\u6770\u51fa\u9752\u5e74\u79d1\u5b66\u57fa\u91d1\u8d44\u52a9\uff0c2008\u5e74\u548c2014\u5e74\u5206\u522b\u4efb\u56fd\u5bb6\u91cd\u5927\u79d1\u5b66\u7814\u7a76\u8ba1\u5212\u9879\u76ee\u9996\u5e2d\u79d1\u5b66\u5bb6\uff0c2010\u5e74\u83b7\u4e2d\u56fd\u9752\u5e74\u79d1\u6280\u5956\uff0c2013\u5e74\u83b7\u4e2d\u56fd\u7269\u7406\u5b66\u4f1a\u9976\u6bd3\u6cf0\u7269\u7406\u5956\uff0c\u540c\u5e74\u83b7\u5f97\u56fd\u52a1\u9662\u653f\u5e9c\u7279\u6b8a\u6d25\u8d34\uff0c2014\u5e74\u4efb\u957f\u6c5f\u5b66\u8005\u5956\u52b1\u8ba1\u5212\u7279\u8058\u6559\u6388\uff0c2016\u5e74\u5165\u9009\u4e07\u4eba\u8ba1\u5212\u79d1\u6280\u521b\u65b0\u9886\u519b\u4eba\u624d\u30022017\u5e7411\u6708\u5f53\u9009\u4e2d\u56fd\u79d1\u5b66\u9662\u9662\u58eb\u3002\u957f\u671f\u4ece\u4e8b\u7b49\u79bb\u6fc0\u5143\u5149\u5b50\u5b66\u3001\u7eb3\u7c73\u5149\u5b66\u3001\u5355\u5206\u5b50\u5149\u8c31\u548c\u7eb3\u7c73\u5149\u82af\u7247\u7b49\u524d\u6cbf\u9886\u57df\u7684\u7814\u7a76\uff0c\u505a\u51fa\u4e86\u5f00\u521b\u6027\u548c\u7cfb\u7edf\u6027\u7684\u5de5\u4f5c\u3002\u5728\u56fd\u9645\u8457\u540d\u79d1\u5b66\u6742\u5fd7\u53d1\u8868\u8bba\u6587180\u4f59\u7bc7\uff0c\u88abSCI\u6742\u5fd7\u5f15\u752812000\u4f59\u6b21\uff0c\u5355\u7bc7\u5f15\u7528\u8d85\u8fc7100\u6b21\u768433\u7bc7\uff0ch\u56e0\u5b5054\u3002\u5176\u4e2d\u5173\u4e8e\u5355\u5206\u5b50\u8868\u9762\u589e\u5f3a\u62c9\u66fc\u5149\u8c31\u7684\u7814\u7a76\u6709\u4e24\u7bc7\u8bba\u6587\u5206\u522b\u88ab\u5f15\u75281660\u4f59\u6b21\uff08Physical Review Letters 1999, 83, 4357\uff09\u548c1190\u4f59\u6b21\uff08Physical Review E 2000, 62, 4318\uff0c\u88ab\u9009\u4e3a\u8be5\u6742\u5fd7\u521b\u520a\u4ee5\u6765\u7684\u91cc\u7a0b\u7891\u8bba\u6587\uff09\u3002\u4ed6\u5df2\u4f5c\u56fd\u9645\u4f1a\u8bae\u9080\u8bf7\u62a5\u544a60\u4f59\u6b21\uff1b\u4f5c\u4e3a\u4f1a\u8bae\u4e3b\u5e2d\u7ec4\u7ec7\u4e86\u5341\u4f59\u6b21\u8457\u540d\u56fd\u9645\u5b66\u672f\u4f1a\u8bae\uff1b\u66fe\u4efbNanoscale\u3001Optics Express\u526f\u4e3b\u7f16\uff1b2014-2017\u5e74\u8fde\u7eed\u5165\u9009Elsevier\u53d1\u5e03\u7684\u4e2d\u56fd\u9ad8\u88ab\u5f15\u5b66\u8005\u699c\uff1b\u53d7\u9080\u51fa\u7248\u4e13\u8457Nanophotonics: Manipulating Light with Plasmons\u3002<\/p>\n

\u8bfe\u9898\u7ec4\u7f51\u7ad9\uff1ahttp:\/\/np.whu.edu.cn<\/a><\/strong><\/p>\n

\u5f20\u987a\u5e73\u526f\u6559\u6388<\/strong>\uff1a\u6b66\u6c49\u5927\u5b66\u7269\u7406\u4e0e\u79d1\u5b66\u6280\u672f\u5b66\u9662\u526f\u6559\u6388\uff0c\u6b66\u6c49\u5927\u5b66\u73de\u73c8\u9752\u5e74\u5b66\u8005\uff082016\uff09\u30022008\u5e74\u6bd5\u4e1a\u4e8e\u4e2d\u5c71\u5927\u5b66\u7269\u7406\u79d1\u5b66\u4e0e\u5de5\u7a0b\u6280\u672f\u5b66\u9662\uff0c\u83b7\u5b66\u58eb\u5b66\u4f4d\uff1b2012\u5e7412\u6708\u6bd5\u4e1a\u4e8e\u4e2d\u56fd\u79d1\u5b66\u9662\u7269\u7406\u7814\u7a76\u6240\uff0c\u83b7\u535a\u58eb\u5b66\u4f4d\u3002\u7814\u7a76\u5174\u8da3\u5305\u62ec\u7b49\u79bb\u6fc0\u5143\u5149\u5b50\u5b66\u3001\u5fae\u7eb3\u5c3a\u5ea6\u4e0a\u5149\u4e0e\u7269\u8d28\u76f8\u4e92\u4f5c\u7528\u3001\u6709\u6e90\u4e0e\u65e0\u6e90\u7eb3\u7c73\u5149\u7535\u5668\u4ef6\u3001\u589e\u5f3a\u5149\u8c31\u7b49\u9886\u57df\u3002\u5728\u4f4e\u7ef4\u91d1\u5c5e\u7eb3\u7c73\u7ed3\u6784\u7684\u8868\u9762\u7b49\u79bb\u6fc0\u5143\u3001\u4e9a\u6ce2\u957f\u5149\u5b66\u6ce2\u5bfc\u7b49\u65b9\u9762\u53d6\u5f97\u4e00\u4e9b\u91cd\u8981\u539f\u521b\u6027\u5de5\u4f5c\u3002\u4e3b\u6301\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u59d4\u9762\u4e0a\u9879\u76ee1\u9879\u3001\u9752\u5e74\u9879\u76ee1\u9879\u3001\u4e2d\u56fd\u535a\u58eb\u540e\u57fa\u91d12\u9879\uff0c\u53c2\u4e0e973\u9879\u76ee1\u9879\u3001\u56fd\u5bb6\u91cd\u70b9\u7814\u53d1\u8ba1\u5212\u9879\u76ee1\u9879\u3002\u4ee5\u7b2c\u4e00\u6216\u901a\u8baf\u4f5c\u8005\u5728Phys. Rev. Lett.\u3001Nat. Commun.\u3001Nano Lett.(4\u7bc7)\u3001Light: Sci.& Appl.\u3001ACS Nano(2\u7bc7)\u7b49\u671f\u520a\u5171\u53d1\u8868\u8bba\u658710\u4f59\u7bc7\uff0cSCI\u88ab\u5f151800\u4f59\u6b21\uff08\u5355\u7bc7\u6700\u9ad8\u88ab\u5f15300\u4f59\u6b21\uff09\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aLight-Emitting Plexciton: Exploiting Plasmon-Exciton Interaction in the Intermediate Coupling Regime<\/a><\/strong>\uff08ACS Nano, 2018<\/strong>, DOI:10.1021\/acsnano.8b05880\uff09<\/p>\n

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