{"id":155789,"date":"2018-10-09T06:30:34","date_gmt":"2018-10-08T22:30:34","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=155789"},"modified":"2018-10-09T20:12:16","modified_gmt":"2018-10-09T12:12:16","slug":"%e5%86%85%e8%92%99%e5%8f%a4%e5%a4%a7%e5%ad%a6%e7%8e%8b%e5%8b%a4adv-energy-materials%e5%b0%81%e9%9d%a2-%e7%a6%bb%e5%ad%90%e6%b6%b2%e4%bd%93%e8%b0%83%e6%8e%a7cofe2o4%e5%b0%96%e6%99%b6%e7%9f%b3","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=155789","title":{"rendered":"\u5185\u8499\u53e4\u5927\u5b66\u738b\u52e4Adv. Energy Materials\u5c01\u9762.:\u79bb\u5b50\u6db2\u4f53\u8c03\u63a7CoFe2O4\u5c16\u6676\u77f3\u6c27\u7a7a\u4f4d\u52a0\u901fOER\u52a8\u529b\u5b66"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u968f\u7740\u5316\u77f3\u71c3\u6599\u7684\u65e5\u76ca\u67af\u7aed\uff0c\u5168\u7403\u6027\u73af\u5883\u95ee\u9898\u53d8\u5f97\u6108\u53d1\u4e25\u5cfb\uff0c\u6025\u9700\u5f00\u53d1\u4e00\u79cd\u65b0\u578b\u73af\u5883\u53cb\u597d\u4e14\u53ef\u518d\u751f\u7684\u80fd\u91cf\u8f7d\u4f53\u3002\u7eff\u8272\u3001\u53ef\u6301\u7eed\u7684\u6c22\u80fd\u88ab\u8ba4\u4e3a\u662f\u4e00\u79cd\u7406\u60f3\u7684\u5316\u77f3\u80fd\u6e90\u66ff\u4ee3\u54c1\uff0c\u800c\u7535\u89e3\u6c34\u63d0\u4f9b\u4e86\u4e00\u79cd\u5927\u89c4\u6a21\u5236\u53d6\u9ad8\u7eaf\u6c22\u7684\u597d\u65b9\u6cd5\u3002\u53d7\u9650\u4e8e\u56db\u7535\u5b50\u4f20\u8f93\u7684\u7f13\u6162\u52a8\u529b\u5b66\uff0c\u9633\u6781\u7684\u6c34\u6c27\u5316\u534a\u53cd\u5e94\u76ee\u524d\u4ecd\u662f\u7535\u89e3\u6c34\u7684\u74f6\u9888\uff0c\u9700\u8981\u9ad8\u6548\u7684\u50ac\u5316\u5242\u6765\u52a0\u901f\u8be5\u7c7b\u53cd\u5e94\u7684\u52a8\u529b\u5b66\uff0c\u4ece\u800c\u8fbe\u5230\u5728\u6781\u5c0f\u7684\u8fc7\u7535\u4f4d\u4e0b\u83b7\u5f97\u9ad8\u50ac\u5316\u7535\u6d41\u5bc6\u5ea6\u3002\u76ee\u524dRuO2<\/sub>\u7b49\u91d1\u5c5e\u6c27\u5316\u7269\u8868\u73b0\u51fa\u6700\u9ad8\u7684\u6c34\u6c27\u5316\u50ac\u5316\u6d3b\u6027\uff0c\u4f46\u662f\u5176\u50a8\u91cf\u4f4e\u3001\u4ef7\u683c\u6602\u8d35\uff0c\u6781\u5927\u5730\u9650\u5236\u4e86\u5176\u5927\u89c4\u6a21\u5546\u4e1a\u5316\u5e94\u7528\uff0c\u56e0\u6b64\u5f00\u53d1\u4ef7\u683c\u4f4e\u5ec9\u3001\u9ad8\u6548\u3001\u8010\u7528\u7684\u975e\u8d35\u91d1\u5c5e\u7535\u50ac\u5316\u5242\u6765\u52a0\u901f\u50ac\u5316\u52a8\u529b\u5b66\u53d8\u5f97\u81f3\u5173\u91cd\u8981\u3002\u7814\u7a76\u8868\u660e\uff0c\u5c16\u6676\u77f3\u94c1\u6c27\u4f53\u7531\u4e8e\u5176\u591a\u91cd\u7ec4\u6210\u3001\u5f62\u8c8c\u3001\u7279\u6b8a\u7684\u51e0\u4f55\u7535\u5b50\u7ed3\u6784\u548c\u8868\u9762\u5316\u5b66\u7f3a\u9677\u7b49\u7279\u5f81\uff0c\u5728\u7535\u5316\u5b66\u50ac\u5316\u9886\u57df\u53d1\u6325\u4e86\u91cd\u8981\u7684\u4f5c\u7528\u3002\u672c\u6587\u9996\u6b21\u91c7\u7528\u79bb\u5b50\u6db2\u4f53\u4f5c\u4e3a\u63ba\u6742\u5242\uff0c\u5728\u5c16\u6676\u77f3\u578b\u94c1\u6c27\u4f53\u5185\u90e8\u6784\u7b51\u5927\u91cf\u6c27\u7a7a\u4f4d\uff0c\u540c\u65f6\u6742\u539f\u5b50\u7684\u8868\u9762\u63ba\u6742\u53ef\u4ee5\u7a33\u5b9a\u8868\u9762\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\uff0c\u5bf9\u5176\u7535\u5b50\u7ed3\u6784\u3001OER\u7535\u50ac\u5316\u6027\u80fd\u53ca\u8868\u9762\u6d3b\u6027\u4f4d\u70b9\u7b49\u8fdb\u884c\u4e86\u6df1\u5165\u7814\u7a76\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5185\u8499\u53e4\u5927\u5b66\u5316\u5b66\u5316\u5de5\u5b66\u9662\u738b\u52e4\u6559\u6388\u8bfe\u9898\u7ec4\u4e0e\u4e2d\u56fd\u79d1\u5b66\u9662\u5316\u5b66\u7814\u7a76\u6240\u4f55\u5cf0\u52a9\u7406\u7814\u7a76\u5458\u3001\u5409\u6797\u5927\u5b66\u65e0\u673a\u5408\u6210\u4e0e\u5236\u5907\u5316\u5b66\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u9ec4\u79d1\u79d1\u6559\u6388\u3001\u82cf\u5dde\u5927\u5b66\u6750\u6599\u4e0e\u5316\u5b66\u5316\u5de5\u5b66\u90e8\u674e\u8000\u6587\u6559\u6388\u5408\u4f5c\uff0c\u5728\u300aAdvanced Energy Materials\u300b\u53d1\u8868\u6709\u5173\u5c16\u6676\u77f3\u8868\u9762\u6c27\u7f3a\u9677\u8c03\u63a7\u7684\u7814\u7a76\u8bba\u6587\u201cA Facile Strategy to Construct Amorphous Spinel-based Electrocatalysts with Massive Oxygen Vacancies Using Ionic Liquid-Dopant\u201d\u00a0(\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/onlinelibrary.wiley.com\/doi\/epdf\/10.1002\/aenm.201800980)\u3002\u5185\u8499\u53e4\u5927\u5b66\u662f\u8be5\u8bba\u6587\u7b2c\u4e00\u4f5c\u8005\u5355\u4f4d\u548c\u7b2c\u4e00\u901a\u8baf\u4f5c\u8005\u5355\u4f4d\uff0c2016\u7ea7\u7855\u58eb\u7814\u7a76\u751f\u5b59\u9759\u662f\u8be5\u8bba\u6587\u7684\u7b2c\u4e00\u4f5c\u8005\uff0c\u738b\u52e4\u6559\u6388\u4e3a\u7b2c\u4e00\u901a\u8baf\u4f5c\u8005\uff0c\u4f55\u5cf0\u52a9\u7406\u7814\u7a76\u5458\u4e3a\u5171\u540c\u901a\u8baf\u4f5c\u8005\u3002<\/p>\n

\u8be5\u5de5\u4f5c\u8bbe\u8ba1\u5408\u6210\u4e86\u4e00\u79cdMoS2<\/sub>\u56e2\u7c07\u539f\u4f4d\u951a\u5b9a\u7684\u3001\u8868\u9762\u6742\u539f\u5b50\u63ba\u6742\u7684MoS2<\/sub>-NPF\/CoFe2<\/sub>O4<\/sub>\uff08MNC\uff09\u5f02\u8d28\u7ed3\u7eb3\u7c73\u50ac\u5316\u6750\u6599\u3002\u79bb\u5b50\u6db2\u4f53\u63ba\u6742\u5242\u53ef\u4ee5\u8c03\u63a7\u5c16\u6676\u77f3CoFe2<\/sub>O4<\/sub>\u50ac\u5316\u6750\u6599\u7684\u6c27\u7a7a\u4f4d\uff0c\u6539\u53d8\u5176\u7535\u5b50\u7ed3\u6784\uff1bMoS2<\/sub>\u56e2\u7c07\u7684\u539f\u4f4d\u751f\u957f\uff0c\u4e00\u65b9\u9762\u53ef\u4ee5\u56fa\u5b9a\u50ac\u5316\u6750\u6599\u8868\u9762\u7684\u6742\u539f\u5b50\uff0c\u53e6\u4e00\u65b9\u9762\u53ef\u4ee5\u5728\u5176\u8868\u9762\u751f\u6210\u66f4\u591a\u7684Fe-N\u3001Co-N\u7b49\u591a\u6d3b\u6027\u4f4d\u70b9\u3002\u7814\u7a76\u7ed3\u679c\u8868\u660e\uff0c\u6c27\u7a7a\u4f4d\u7684\u5927\u91cf\u5b58\u5728\u3001\u5927\u7684\u6bd4\u8868\u9762\u79ef\u4ee5\u53ca\u5404\u7ec4\u5206\u95f4\u7684\u534f\u540c\u8bf1\u5bfc\u6548\u5e94\u5bf9\u63d0\u5347\u7535\u50ac\u5316\u6790\u6c27\u53cd\u5e94\u6027\u80fd\u8d77\u5230\u81f3\u5173\u91cd\u8981\u7684\u4f5c\u7528\u3002\u6b64\u5916\uff0c\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u7ed3\u679c\u8868\u660e\uff0c\u8868\u9762\u6742\u539f\u5b50\u7684\u63ba\u6742\u548cMoS2<\/sub>\u56e2\u7c07\u7684\u539f\u4f4d\u751f\u957f\uff0c\u53ef\u4ee5\u964d\u4f4e\u591a\u7535\u5b50\u53cd\u5e94\u4e2d\u95f4\u8fc7\u7a0b\u5409\u5e03\u65af\u81ea\u7531\u80fd\u3002<\/p>\n

\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u56fe1 \u5f02\u8d28\u7ed3\u7eb3\u7c73\u50ac\u5316\u6750\u6599\u5408\u6210\u793a\u610f\u56fe\u53ca\u7ed3\u6784\u6f14\u53d8\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

    \n
  1. a) \u50ac\u5316\u5242\u5408\u6210\u793a\u610f\u56fe, b-c)XRD\u56fe, d)\u5438\u8131\u9644\u7b49\u6e29\u7ebf\u53ca\u5b54\u9699\u5927\u5c0f\u5206\u5e03\u3002<\/li>\n<\/ol>\n

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    \"\"<\/p>\n

      \n
    1. a) CoFe2<\/sub>O4<\/sub>, b) NPF\/CoFe2<\/sub>O4<\/sub>, c) MoS2<\/sub>\/CoFe2<\/sub>O4<\/sub>\u7684SEM\u56fe\uff1bd-e) MoS2<\/sub>\/CoFe2<\/sub>O4<\/sub>\u7684TEM\u56fef) MoS2<\/sub>\/CoFe2<\/sub>O4<\/sub>\u7684HAADF-STEM\u53ca\u5143\u7d20\u9762\u626b\u56fe\u3002<\/li>\n<\/ol>\n

      \u56fe3 \u5f02\u8d28\u7ed3\u7eb3\u7c73\u50ac\u5316\u6750\u6599\u7535\u50ac\u5316\u6027\u80fd<\/b><\/strong><\/p>\n

      \"\"<\/p>\n

        \n
      1. a) \u50ac\u5316\u5242\u57280 M KOH\u4e2d\u7684OER\u6027\u80fd; b-c) Tafel\u659c\u7387\u53ca\u5176\u67f1\u72b6\u56fe; d) Nyquist\u56fe; e) \u53cc\u5c42\u7535\u5bb9\u503c; f) \u7a33\u5b9a\u6027I-t\u66f2\u7ebf\u3002<\/li>\n<\/ol>\n

        \u56fe4 OER\u50ac\u5316\u8fc7\u7a0b\u5409\u5e03\u65af\u81ea\u7531\u80fd\u8ba1\u7b97<\/b><\/strong><\/p>\n

        \"\"<\/p>\n

        \u50ac\u5316\u5242\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd\u8ba1\u7b97<\/p>\n

        \u56fe5 OER\u50ac\u5316\u53cd\u5e94\u673a\u7406<\/b><\/strong><\/p>\n

        \"\"<\/p>\n

         <\/p>\n

        \u56fe6. \u8bba\u6587\u5c01\u9762\uff08<\/b><\/strong>Adv<\/b><\/strong>. <\/b><\/strong>Energy Materials<\/b><\/strong>, 2018, 8, 1800980\uff09<\/b><\/strong><\/p>\n

        \"\"<\/p>\n

        \u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

        \u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u91c7\u7528\u6eb6\u5242\u70ed\u6cd5\uff0c\u4ee5\u79bb\u5b50\u6db2\u4f53\u4f5c\u4e3a\u63ba\u6742\u5242\uff0c\u5c06\u6c27\u7a7a\u4f4d\u3001\u6742\u539f\u5b50\u6210\u529f\u5f15\u5165\u5230CoFe2<\/sub>O4<\/sub>\u4e2d\uff0c\u4f7f\u5176\u7531\u9762\u5fc3\u7acb\u65b9\u7ed3\u6784\uff08fcc\uff09\u8f6c\u53d8\u4e3a\u975e\u6676\u7ed3\u6784\uff1b\u540c\u65f6\u5728\u5176\u8868\u9762\u539f\u4f4d\u751f\u957f\u8d85\u5c0f\u5c3a\u5bf8MoS2<\/sub>\u7eb3\u7c73\u56e2\u7c07\uff0c\u4ee5\u589e\u52a0\u5176\u6bd4\u8868\u9762\u79ef\u548c\u8868\u9762\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u3002\u8be5\u7814\u7a76\u5236\u5907\u7684\u5bcc\u6c27\u6c27\u7a7a\u4f4d\u7684\u5f02\u8d28\u7ed3\u7eb3\u7c73\u50ac\u5316\u6750\u6599\u5177\u6709\u8d85\u4f4e\u7684\u8fc7\u7535\u4f4d\uff08250 mV\uff09\u548cTafel\u659c\u7387\uff0841 mV dec-1<\/sup>\uff09\uff0c\u8fd9\u662f\u76ee\u524d\u6587\u732e\u62a5\u9053\u7684\u5c16\u6676\u77f3\u578b\u94c1\u6c27\u4f53\u6700\u4f18\u7684\u7535\u50ac\u5316OER\u6027\u80fd\u3002\u5176\u4f18\u5f02\u7684OER\u50ac\u5316\u6027\u80fd\u53ef\u5f52\u56e0\u4e8e\u5927\u91cf\u7684\u6c27\u7a7a\u4f4d\u3001\u975e\u6676\u7ed3\u6784\u3001\u5927\u6bd4\u8868\u9762\u79ef (148.9 m2<\/sup>\u00a0g-1<\/sup>)\uff0c\u4ee5\u53ca\u8868\u9762\u5927\u91cf\u7684\u7535\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\uff08N-Fe\u3001N- Co\u548cP-O\u7b49\uff09\u4e4b\u95f4\u7684\u534f\u540c\u8026\u5408\u4f5c\u7528\u3002DFT\u8ba1\u7b97\u7ed3\u679c\u8868\u660e\uff0c\u6742\u539f\u5b50\u548cMoS2<\/sub>\u7684\u5b58\u5728\u53ef\u4ee5\u8c03\u8282OER\u8fc7\u7a0b\u4e2d\u7684\u7535\u5b50\u7ed3\u6784\uff0c\u964d\u4f4e\u4e2d\u95f4\u8fc7\u7a0b\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd\uff0c\u8fd9\u5bf9\u589e\u5f3aOER\u6027\u80fd\u662f\u975e\u5e38\u6709\u5229\u7684\u3002\u672c\u8bbe\u8ba1\u4e0d\u4ec5\u63d0\u4f9b\u4e86\u4e00\u79cd\u5229\u7528\u79bb\u5b50\u6db2\u4f53\u63ba\u6742\u5242\u6784\u7b51\u5177\u6709\u5927\u91cf\u6c27\u7a7a\u4f4d\u3001\u975e\u6676\u7ed3\u6784\u50ac\u5316\u5242\u7684\u7b80\u5355\u7b56\u7565\uff0c\u800c\u4e14\u5bf9\u78b1\u6027\u6eb6\u6db2\u4e2d\u7684OER\u50ac\u5316\u673a\u7406\u4e5f\u8fdb\u884c\u4e86\u6df1\u5165\u7814\u7a76\u3002<\/p>\n

        \u3010\u901a\u8baf\u4f5c\u8005<\/b><\/strong>\u7b80\u4ecb<\/b><\/strong>\u3011<\/b><\/strong>\uff1a\u738b\u52e4\uff0c\u5185\u8499\u53e4\u5927\u5b66\u6559\u6388\uff0c\u535a\u58eb\u751f\u5bfc\u5e08\uff0c2010\u5e74\u6bd5\u4e1a\u4e8e\u5409\u6797\u5927\u5b66\u5316\u5b66\u5b66\u9662\uff0c\u83b7\u7406\u5b66\u535a\u58eb\u5b66\u4f4d\u3002\u73b0\u4e3a\u4e2d\u56fd\u5316\u5de5\u5b66\u4f1a\u5316\u5de5\u65b0\u6750\u6599\u59d4\u5458\u4f1a\u59d4\u5458\uff0c\u4e2d\u56fd\u5316\u5b66\u4f1a\u4f1a\u5458\uff0c\u4e2d\u56fd\u5316\u5de5\u5b66\u4f1a\u4f1a\u5458\u3002\u83b72016\u5e74\u5ea6\u5185\u8499\u53e4\u81ea\u7136\u79d1\u5b66\u4e00\u7b49\u5956\uff0c2017\u5e74\u5185\u8499\u53e4\u6770\u51fa\u9752\u5e74\u57f9\u80b2\u57fa\u91d1\u8d44\u52a9\uff0c\u5165\u9009\u5185\u8499\u53e4\u81ea\u6cbb\u533a\u201c\u8349\u539f\u82f1\u624d\u201d\u5de5\u7a0b\u9752\u5e74\u521b\u65b0\u4eba\u624d\u4e00\u5c42\u6b21\uff0c\u5165\u9009\u5185\u8499\u53e4\u81ea\u6cbb\u533a\u201c\u65b0\u4e16\u7eaa321\u4eba\u624d\u5de5\u7a0b\u201d\u3002\u5728\u56fd\u9645\u8457\u540d\u5b66\u672f\u671f\u520aAdv. Energy Mater\u7b49\u53d1\u8868\u5b66\u672f\u8bba\u658750\u4f59\u7bc7\uff0c\u5176\u4e2d\u5c01\u9762\u548c\u70ed\u70b9\u8bba\u65876\u7bc7\uff0cESI\u9ad8\u88ab\u5f15\u8bba\u65872\u7bc7\u3002<\/p>\n

        \u6587\u732e\u94fe\u63a5\uff1aA Facile Strategy to Construct Amorphous Spinel-based Electrocatalysts with Massive Oxygen Vacancies Using Ionic Liquid-Dopant\u00a0(Adv. Energy Mater., 2018, 8, 1800980, DOI: 10.1002\/aenm.201800980)<\/p>\n

         <\/p>\n

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