{"id":156957,"date":"2018-11-05T06:30:33","date_gmt":"2018-11-04T22:30:33","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=156957"},"modified":"2018-11-04T21:58:57","modified_gmt":"2018-11-04T13:58:57","slug":"%e4%b8%8a%e6%b5%b7%e5%a4%a7%e5%ad%a6aem%e5%9f%ba%e4%ba%8emofs%e7%9a%84%e5%a4%9a%e7%9b%b8%e5%82%ac%e5%8c%96%e5%89%82%e8%83%bd%e9%87%8f%e7%9b%b8%e5%85%b3co2%e8%bd%ac%e5%8c%96%e7%9a%84%e6%96%b0","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=156957","title":{"rendered":"\u4e0a\u6d77\u5927\u5b66AEM:\u57fa\u4e8eMOFs\u7684\u591a\u76f8\u50ac\u5316\u5242:\u80fd\u91cf\u76f8\u5173CO2\u8f6c\u5316\u7684\u65b0\u673a\u9047"},"content":{"rendered":"<p>\u3010\u524d\u8a00\u3011<\/p>\n<p>\u73af\u5883\u548c\u80fd\u6e90\u76f8\u5173\u95ee\u9898\u5df2\u7ecf\u6210\u4e3a\u516c\u4f17\u5173\u6ce8\u7684\u4e3b\u8981\u95ee\u9898\u3002\u53e4\u5f80\u4eca\u6765\uff0c\u7164\u70ad\u3001\u77f3\u6cb9\u548c\u5929\u7136\u6c14\u7b49\u78b3\u5316\u77f3\u71c3\u6599\u7684\u8fc7\u5ea6\u5f00\u53d1\u548c\u8fc7\u5ea6\u4f7f\u7528\u63d0\u4f9b\u4e86\u8fd1200\u5e74\u7684\u80fd\u6e90\u4f9b\u5e94\u3002\u7136\u800c\uff0c\u8fc7\u5ea6\u4f7f\u7528\u8fd9\u4e9b\u5316\u77f3\u71c3\u6599\u4ee5\u53ca\u968f\u4e4b\u800c\u6765\u7684\u6e29\u5ba4\u6548\u5e94\/\u80fd\u6e90\u5371\u673a\u5df2\u7ecf\u6210\u4e3a\u4eba\u7c7b\u5fc5\u987b\u9762\u5bf9\u7684\u6700\u91cd\u8981\u7684\u95ee\u9898\u4e4b\u4e00\u3002\u5168\u7403\u89c2\u6d4b\u8868\u660e\uff0c\u6e29\u5ba4\u6c14\u4f53\u7684\u5927\u91cf\u6392\u653e\uff0c\u4e3b\u8981\u6765\u81ea\u5316\u77f3\u71c3\u6599\u7684\u6d88\u8017\uff0c\u5bfc\u81f4\u5168\u7403\u6c14\u5019\u53d8\u6696\u548c\u51b0\u5ddd\u6d88\u878d\u3002\u4e3a\u4e86\u51cf\u8f7b\u6e29\u5ba4\u6548\u5e94\uff0c\u79d1\u5b66\u5bb6\u547c\u5401\u5168\u4e16\u754c\u51cf\u5c11\u4f7f\u7528\u5e38\u89c4\u5316\u77f3\u71c3\u6599\u4ee5\u51cf\u5c11\u4e8c\u6c27\u5316\u78b3\u7684\u6392\u653e\uff0c\u5e76\u5927\u529b\u5bfb\u6c42\u73af\u4fdd\u66ff\u4ee3\u54c1\uff1b\u53e6\u4e00\u65b9\u9762\uff0c\u78b3\u4ea4\u6613\u548c\u78b3\u5c01\u5b58\u6280\u672f\u7684\u5efa\u7acb\u4e5f\u9700\u8981\u7a33\u6b65\u63a8\u8fdb\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u7814\u7a76\u4eba\u5458\u5c1d\u8bd5\u4e86\u5404\u79cd\u52aa\u529b\u6765\u6355\u83b7\u548c\u56fa\u5b9a\u4e8c\u6c27\u5316\u78b3\uff0c\u5305\u62ec\u751f\u7269\u8d28\u3001\u7269\u7406\u548c\u5316\u5b66\u65b9\u6cd5\u3002\u7136\u800c\uff0c\u76ee\u524d\u5927\u591a\u6570\u964d\u4f4eCO<sub>2<\/sub>\u6d53\u5ea6\u7684\u65b9\u6cd5\u90fd\u5f88\u8017\u65f6\uff0c\u751a\u81f3\u66f4\u5bb9\u6613\u8fbe\u5230\u5bb9\u91cf\u9650\u5236\u3002\u4e0d\u4ec5\u5982\u6b64\uff0c\u91c7\u7528\u4e00\u4e9b\u9694\u79bb\u65b9\u6cd5\uff0c\u5982\u6d77\u6d0b\u503e\u5012\uff0c\u53ef\u80fd\u4f1a\u5f15\u53d1\u53e6\u4e00\u573a\u73af\u5883\u707e\u96be\u3002<\/p>\n<p>MOFs\u5728CO<sub>2<\/sub>\u8fd8\u539f\u9886\u57df\u6709\u5f88\u5927\u7684\u5e94\u7528\u524d\u666f\uff0c\u5b83\u53ef\u4ee5\u76f4\u63a5\u4f5c\u4e3a\u50ac\u5316\u5242\u6216\u7ec4\u5206\u5728\u6df7\u5408\u50ac\u5316\u4f53\u7cfb\u4e2d\u4fc3\u8fdbCO<sub>2<\/sub>\u8fd8\u539f\u3002MOFs\u7684\u5185\u90e8\u53ef\u4ee5\u8bbe\u8ba1\u6210\u5177\u6709\u5f00\u653e\u7684\u91d1\u5c5e\u4f4d\u70b9\u3001\u7279\u5b9a\u7684\u6742\u539f\u5b50\u3001\u529f\u80fd\u5316\u7684\u6709\u673a\u914d\u4f53\u3001\u5176\u4ed6\u6784\u5efa\u5355\u5143\u76f8\u4e92\u4f5c\u7528\u3001\u758f\u6c34\u6027\u3001\u7f3a\u9677\u3001\u5b54\u9699\u7387\u548c\u5d4c\u5165\u7684\u7eb3\u7c73\u7ea7\u91d1\u5c5e\u50ac\u5316\u5242\uff0c\u8fd9\u5bf9\u5f00\u53d1\u5177\u6709\u66f4\u597d\u7684CO<sub>2<\/sub>\u8fd8\u539f\u6027\u80fdMOFs\u81f3\u5173\u91cd\u8981\u3002\u7531\u4e8eMOFs\u7684\u7535\u5b50\u4f20\u5bfc\u6027\u5dee\uff0c\u4ee5\u53ca\u6240\u6709\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u5bf9\u53cd\u5e94\u7269\u4e0d\u53ef\u63a5\u8fd1\uff0cMOFs\u5728\u6c34\u4e2d\u548c\u7d2b\u5916\u5149\u7167\u5c04\u4e0b\u7684\u7a33\u5b9a\u6027\u9700\u8981\u8fdb\u4e00\u6b65\u63d0\u9ad8\u3002\u4e3a\u4e86\u53d6\u5f97\u66f4\u597d\u7684\u6210\u7ee9\uff0c\u6709\u5fc5\u8981\u4f7f\u7528MOF\u6765\u6784\u5efa\u66f4\u590d\u6742\u7684\u6750\u6599\uff0c\u4ee5\u5728\u4e00\u79cd\u6750\u6599\u4e2d\u540c\u65f6\u89e3\u51b3CO<sub>2<\/sub>\u5bb9\u91cf\u548c\u8fd8\u539f\u80fd\u529b\u95ee\u9898\u3002\u672a\u6765MOFs\u7528\u4e8e\u4e8c\u6c27\u5316\u78b3\u51cf\u6392\u7684\u6750\u6599\u5e94\u8be5\u662f\u7ecf\u6d4e\u73af\u4fdd\u7684\u3002\u4fc3\u8fdb\u50ac\u5316\u7684\u5173\u952e\u5305\u62ecMOFs\u4e2d\u7684\u7ed3\u6784\u7f3a\u9677\u3001\u91d1\u5c5e\u7c07\u7684\u5f00\u653e\u91d1\u5c5e\u4f4d\u70b9\u3001\u91d1\u5c5e\u7c07\u548c\u6709\u673a\u91d1\u5c5e\u63a5\u5934\u7684Lewis\u9178\u4f4d\u70b9\u4ee5\u53ca\u52a9\u50ac\u5316\u5242\u529f\u80fd\u5316\u7684MOFs\u3002<\/p>\n<p>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/p>\n<p>\u5177\u6709\u9ad8\u8868\u9762\u79ef\u548c\u53ef\u8c03\u5316\u5b66\u7ed3\u6784\u7684\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6(MOFs)\u5df2\u7ecf\u5f15\u8d77\u4e86\u7814\u7a76\u4eba\u5458\u6781\u5927\u7684\u5173\u6ce8\u3002\u6700\u8fd1\uff0c\u5229\u7528\u592a\u9633\u80fd\u8fdb\u884c\u4e8c\u6c27\u5316\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Energy Materials\u4e0a\u53d1\u8868\u7efc\u8ff0\u6587\u7ae0\uff0c\u9898\u4e3a\u201cMOFs-Based Heterogeneous Catalysts: New Opportunities for Energy-Related CO2 Conversion\u201d\u3002\u672c\u6587\u7efc\u8ff0\u4e86\u8fd1\u5e74\u6765MOFs\u57faCO<sub>2<\/sub>\u8f6c\u5316\u53cd\u5e94\u50ac\u5316\u5242\u7684\u7814\u7a76\u8fdb\u5c55\uff0c\u5305\u62ec\u5149\u50ac\u5316\u548c\u7535\u50ac\u5316\u3002\u7279\u522b\u8ba8\u8bba\u4e86\u57fa\u4e8eCO<sub>2<\/sub>\u8f6c\u5316\u7684MOFs\u7684\u5236\u5907\u548c\u673a\u7406\u3002\u8fd9\u4e9b\u4f8b\u5b50\u6709\u671b\u5728\u5236\u5907\u9ad8\u6d3b\u6027\u548c\u7a33\u5b9a\u7684\u57fa\u4e8eMOFs\u7684CO<sub>2<\/sub>\u8f6c\u5316\u6750\u6599\u4e2d\u63d0\u4f9b\u66f4\u6df1\u5165\u7684\u7406\u89e3\u3002<\/p>\n<p>\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/p>\n<p>\u56fe 1. MOFs\u5408\u6210\u65b9\u6cd5<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156958\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/1-22.jpg\" alt=\"\" width=\"600\" height=\"141\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/1-22.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/1-22-300x71.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>MIL-53(Fe)\u5408\u6210(a)\u5728424K\u7535\u5b50\u52a0\u70ed18\u5c0f\u65f6, (b) z\u5728424K\u5fae\u6ce230min\uff0c(c)\u752860%\u7684\u529f\u7387\u8d85\u58f015min\u3002<\/p>\n<p>\u56fe2. CO<sub>2<\/sub>\u8fd8\u539f\u673a\u7406<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156959\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/2-22.jpg\" alt=\"\" width=\"600\" height=\"396\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/2-22.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/2-22-300x198.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>latimer &#8211; Frost\u56fe\uff0c\u7528\u4e8e\u5728pH 7\u4e0b\u5728\u5747\u5300\u6c34\u6eb6\u6db2\u4e2d\u591a\u7535\u5b50\u3001\u591a\u8d28\u5b50CO<sub>2<\/sub>\u8fd8\u539f\uff1b<\/p>\n<p>\u56fe3.\u57fa\u4e8eMOFs\u7684\u91d1\u5c5e\u591a\u76f8\u50ac\u5316\u5242\u6750\u6599<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156960\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/3-23.jpg\" alt=\"\" width=\"600\" height=\"252\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/3-23.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/3-23-300x126.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>&nbsp;<\/p>\n<p>(a) Pt\/NH<sub>2<\/sub>-MIL-125(Ti) \u548c(b) Au\/NH<sub>2<\/sub>-MIL-125(Ti)\u7684ESR\u8c31\uff1b<\/p>\n<p>\u56fe4. UiO-66\/CNNS\u7684\u5408\u6210\u4e0e\u6027\u80fd<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156961\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/4-21.jpg\" alt=\"\" width=\"600\" height=\"251\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/4-21.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/4-21-300x126.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a) UiO-66\/CNNS\u5236\u5907\u793a\u610f\u56fe\uff1b<\/p>\n<p>(b) UiO-66\/CNNS\u7684TEM\u548cHRTEM\u56fe\uff1b<\/p>\n<p>(c,d) UiO-66\/CNNS\u548cUiO-66\/\u5757\u4f53CN\u7684PL\u56fe\uff1b<\/p>\n<p>(e) \u4e09\u79cd\u50ac\u5316\u5242\u50ac\u5316\u4ea7CO\uff1b<\/p>\n<p>(f) UiO-66\/CNNS \u5149\u50ac\u5316CO2\u8fd8\u539f\u673a\u7406\uff1b<\/p>\n<p>\u56fe5. UiO-66-NH<sub>2<\/sub>\u5149\u54cd\u5e94<\/p>\n<p>&nbsp;<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156967\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/6-9.jpg\" alt=\"\" width=\"600\" height=\"189\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/6-9.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/6-9-300x95.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a) Cd<sub>0.2<\/sub>Zn<sub>0.8<\/sub>S@UiO-66-NH<sub>2<\/sub>\u5149\u751f\u7535\u5b50\u548c\u7a7a\u7a74\u7684\u4f20\u8f93\u793a\u610f\u56fe\uff1b<\/p>\n<p>(b) Cd<sub>0.2<\/sub>Zn<sub>0.8<\/sub>S@UiO-66-NH<sub>2<\/sub>\u7684PL \u56fe\uff1b<\/p>\n<p>(c) Cd<sub>0.2<\/sub>Zn<sub>0.8<\/sub>S@UiO-66-NH<sub>2<\/sub>\u5149\u7535\u6d41\u56fe\uff1b<\/p>\n<p>\u56fe6. Au&amp;Pt@ZIF\u5236\u5907\u4e0e\u6027\u80fd<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156968\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/7-5.jpg\" alt=\"\" width=\"600\" height=\"389\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/7-5.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/7-5-300x195.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a) Au&amp;Pt@ZIF\u5149\u7167\u5c04\u4e0b\u7684\u5f62\u6210\u548c\u6e29\u5ea6\u53d8\u5316\u7684\u793a\u610f\u56fe\uff1b<\/p>\n<p>(b) Au&amp;Pt@ZIF\u7684TEM\u56fe\uff1b<\/p>\n<p>(c)\u5728100\u00b0C\u548c150\u00b0C\u4e0b\uff0c\u6709\/\u65e0\u5149\u71673h\uff0c\u94c2\u7eb3\u7c73\u7acb\u65b9\u4f53\u3001Pt@ZIF\u3001Au&amp;Pt@ZIF\u548cPt@ZIF+Au\u7684\u4ea7\u7269\u4ea7\u7387\u6bd4\u8f83\uff1b<\/p>\n<p>\u56fe7.\u91c7\u7528\u4e0d\u540c\u50ac\u5316\u5242\u5c06CO2\u5149\u50ac\u5316\u8f6c\u5316\u4e3aCO\u7684\u901f\u7387<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156969\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/8-5.jpg\" alt=\"\" width=\"600\" height=\"291\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/8-5.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/8-5-300x146.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a) MAF-X27-Cl, (b) MAF-X27-OH, (c) MOF-74-Co, (d) Co-ZIF-9, (e) MAF-X27l-Cl, (f) MAF-X27l-OH.<\/p>\n<p>\u56fe8. MOFs\u5f62\u8c8c\u8bbe\u8ba1<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156971\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/9-5.jpg\" alt=\"\" width=\"600\" height=\"333\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/9-5.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/9-5-300x167.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a) CO<sub>2<\/sub>\u5438\u9644\u66f2\u7ebf(273 K), (b) SEM\u56fe\uff0c (c) TEM\u56fe\uff0c (d)\u5408\u6210\u65b9\u6848\uff1b<\/p>\n<p>\u56fe9. \u5185\u90e8\u5316\u5b66\u7ed3\u6784\u7684\u53d8\u5316<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156975\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/12-3.jpg\" alt=\"\" width=\"600\" height=\"611\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/12-3.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/12-3-295x300.jpg 295w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a)\u56fa\u4f53\u4e2dTi(\u5b9e\u5fc3\u56fe\u6807)\u548cZr(\u7a7a\u5fc3\u56fe\u6807)\u91cf\u4e0e\u76f8\u5e94\u6eb6\u6db2\u548c\u56fa\u4f53\u7684\u989c\u8272\uff1b<\/p>\n<p>(b) XPS\u56fe\u7684Ti 2p\uff1b<\/p>\n<p>(c) NH<sub>2<\/sub>-UiO-66(Zr)\u548cTi-\u63ba\u6742 NH<sub>2<\/sub>-UiO-66(Zr)\u7684UV\u5149\u8c31\uff1b<\/p>\n<p>(d,e) NH<sub>2<\/sub>-UiO-66(Zr)\u548cTi-\u63ba\u6742 NH<sub>2<\/sub>-UiO-66(Zr)\u7684\u5e26\u7ed3\u6784\uff1b<\/p>\n<p>(f,g) \u4e0d\u540c\u6837\u54c1\u7684ESR\u56fe\uff1b<\/p>\n<p>(h) NH<sub>2<\/sub>-Uio-66(Zr\/Ti)\u5149\u50ac\u5316\u673a\u7406\uff1b<\/p>\n<p>\u56fe10. MOFs\u884d\u751f\u50ac\u5316\u5242<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156982\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/18-1.jpg\" alt=\"\" width=\"600\" height=\"561\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/18-1.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/18-1-300x281.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a,b) GNP\/ NH<sub>2<\/sub>-MIL-125(Ti)\u548cGNP\/TiO<sub>2<\/sub>\u7684\u4eae\u573aTEM\u56fe\uff1b<\/p>\n<p>(c)\u4e0d\u540c\u6837\u54c1CH<sub>4<\/sub>\u7684\u4ea7\u91cf\uff1b<\/p>\n<ol>\n<li>d) \u70ed\u89e3\u4ea7\u7269XRD\u56fe\uff1b<\/li>\n<\/ol>\n<p>\u56fe11. ZnO@Co<sub>3<\/sub>O<sub>4<\/sub>\u5236\u5907<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156983\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/19.jpg\" alt=\"\" width=\"600\" height=\"527\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/19.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/19-300x264.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a) ZIF-8-\u884d\u751f\u7684ZnO \u548cZIF-8@ZIF-67-\u884d\u751f\u7684ZnO@Co<sub>3<\/sub>O<sub>4<\/sub>\u7684\u5236\u5907\u793a\u610f\u56fe\uff1b<\/p>\n<p>(b,c) ZIF-8 \u548cZIF-8@ZIF-67\u7684SEM\u56fe\uff1b<\/p>\n<p>(d) ZnO@Co<sub>3<\/sub>O<sub>4<\/sub>\u7684TEM\u56fe\uff1b<\/p>\n<p>(e,f) XRD\u56fe\uff1b<\/p>\n<p>(g,h) ZnO\u548cZnO@Co<sub>3<\/sub>O<sub>4<\/sub>\u7684XPS\u56fe\u7684C1s\uff1b<\/p>\n<p>\u56fe12. CO<sub>2<\/sub>\u7535\u50ac\u5316\u8fd8\u539f<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156987\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/22.jpg\" alt=\"\" width=\"600\" height=\"671\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/22.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/22-268x300.jpg 268w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a)\u91d1\u5c5e\u94dc\u7535\u50ac\u5316\u8fd8\u539f\u4e8c\u6c27\u5316\u78b3\uff1b<\/p>\n<p>(b)Cu-MOF\u7535\u50ac\u5316\u8fd8\u539f\u4e8c\u6c27\u5316\u78b3\uff1b<\/p>\n<p>\u56fe13. \u53cd\u5e94\u8def\u5f84<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-156988\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/23.jpg\" alt=\"\" width=\"600\" height=\"216\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/23.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2018\/10\/23-300x108.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a)Zn-MOF\/CP\u5728\u79bb\u5b50\u6db2\u4f53\u4e2d\u5c06CO<sub>2<\/sub>\u7535\u50ac\u5316\u8f6c\u5316\u4e3aCH4\u53ef\u80fd\u7684\u7535\u5316\u5b66\u8fd8\u539f\u8def\u5f84\u4ee5\u53ca(b)Re-SURMOF\u53ef\u80fd\u7684\u7535\u8377\u4f20\u8f93\u8def\u5f84;<\/p>\n<p>\u3010\u603b\u7ed3\u3011<\/p>\n<p>\u5177\u6709\u8fd8\u539fCO<sub>2<\/sub>\u5e76\u540c\u65f6\u7ed3\u5408\u5bfc\u7535\u6027\u3001\u78c1\u6027\u3001\u8367\u5149\u529f\u80fd\u7684\u6750\u6599\u4ecd\u7136\u662f\u4e00\u4e2a\u91cd\u5927\u6311\u6218\u3002\u672a\u6765\u591a\u529f\u80fd\u6027\u7684MOF\u57fa\u6750\u6599\u7684\u4ea7\u751f\u53ef\u4ee5\u4e3a\u529f\u80fd\u6027MOF\u57fa\u6750\u6599\u63d0\u4f9b\u65b0\u7684\u9014\u5f84\uff0c\u540c\u65f6\u4e5f\u4e3aMOF\u5f00\u8f9f\u4e00\u4e2a\u65b0\u7684\u9886\u57df\u63d0\u4f9b\u4e86\u673a\u4f1a\uff0c\u800c\u4e14\u4e5f\u4e3a\u5de5\u4e1a\u5e94\u7528\u63d0\u4f9b\u4e86\u673a\u4f1a\u3002<\/p>\n<p>\u6587\u732e\u94fe\u63a5\uff1a<a href=\"https:\/\/onlinelibrary.wiley.com\/doi\/abs\/10.1002\/aenm.201801587\" target=\"_blank\" rel=\"noopener\">MOFs-Based Heterogeneous Catalysts: New Opportunities for Energy-Related CO<sub>2<\/sub> Conversion<\/a>, (Advanced Energy Materials, 2018, DOI: 10.1002\/aenm.201801587)<\/p>\n<p>\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u8ba1\u7b97\u7ec4<strong><b>Z,Chen<\/b><\/strong>\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n<p>\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1\uff1atougao@cailiaoren.com\u3002<\/p>\n<p>\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaokefu<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u3010\u524d\u8a00\u3011 \u73af\u5883\u548c\u80fd\u6e90\u76f8\u5173\u95ee\u9898\u5df2\u7ecf\u6210\u4e3a\u516c\u4f17\u5173\u6ce8\u7684\u4e3b\u8981\u95ee\u9898\u3002\u53e4\u5f80\u4eca\u6765\uff0c\u7164\u70ad\u3001\u77f3\u6cb9\u548c\u5929\u7136\u6c14\u7b49\u78b3\u5316\u77f3\u71c3\u6599\u7684\u8fc7\u5ea6\u5f00\u53d1\u548c\u8fc7\u5ea6\u4f7f\u7528\u63d0\u4f9b\u4e86\u8fd1200\u5e74\u7684\u80fd\u6e90\u4f9b\u5e94\u3002\u7136\u800c\uff0c\u8fc7\u5ea6\u4f7f\u7528\u8fd9&#8230;<\/p>\n","protected":false},"author":3029,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[533],"tags":[],"class_list":["post-156957","post","type-post","status-publish","format-standard","hentry","category-zongshu"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/156957"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/3029"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=156957"}],"version-history":[{"count":7,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/156957\/revisions"}],"predecessor-version":[{"id":158170,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/156957\/revisions\/158170"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=156957"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=156957"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=156957"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}