{"id":157751,"date":"2018-11-08T06:30:12","date_gmt":"2018-11-07T22:30:12","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=157751"},"modified":"2018-11-07T11:59:56","modified_gmt":"2018-11-07T03:59:56","slug":"%e6%be%b3%e5%a4%a7%e5%88%a9%e4%ba%9a%e6%96%b0%e5%8d%97%e5%a8%81%e5%b0%94%e5%a3%ab%e5%a4%a7%e5%ad%a6rose-amal%e6%95%99%e6%8e%88%e8%af%be%e9%a2%98%e7%bb%84j-photochem-photobiol-c-%e6%9c%80%e6%96%b0","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=157751","title":{"rendered":"\u6fb3\u5927\u5229\u4e9a\u65b0\u5357\u5a01\u5c14\u58eb\u5927\u5b66Rose Amal\u6559\u6388\u8bfe\u9898\u7ec4J. Photochem. Photobiol., C.\u6700\u65b0\u7efc\u8ff0\uff1a \u00a0\u6291\u5236Cu2O\u5149\u50ac\u5316\u548c\u5149\u7535\u50ac\u5316\u8150\u8680\u7684\u7814\u7a76\u8fdb\u5c55"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u81ea\u4ece1972\u5e74Fujishima\u548cHonda\u53d1\u8868\u4e86TiO2<\/sub>\u4f5c\u4e3a\u5149\u50ac\u5316\u5242\u7684\u91cd\u5927\u7a81\u7834\u4ee5\u6765\uff0c\u5149\u50ac\u5316\u5438\u5f15\u4e86\u5b66\u8005\u4eec\u7684\u6ce8\u610f\u5e76\u6295\u5165\u5927\u91cf\u7684\u7cbe\u529b\u63a2\u7d22\u9664\u4e8c\u6c27\u5316\u949b\u4ee5\u5916\u7684\u5149\u50ac\u5316\u5242\u3002\u5176\u4e2d\uff0c\u4f5c\u4e3a\u4e00\u79cd\u53ef\u89c1\u5149\u76f8\u5e94\u7684\u534a\u5bfc\u4f53\uff0cCu2<\/sub>O\u5728\u8fd1\u5e74\u6765\u88ab\u5e7f\u6cdb\u5e94\u7528\u4e8e\u5149\u50ac\u5316\u548c\u5149\u7535\u50ac\u5316\u4f53\u7cfb\u4e2d\u3002 \u7136\u800c\uff0cCu2<\/sub>O\u4e25\u91cd\u7684\u5149\u8150\u8680\u95ee\u9898\u9650\u5236\u4e86\u5b83\u7684\u5e7f\u6cdb\u5e94\u7528\u3002\u56e0\u6b64\uff0c\u5927\u91cf\u7814\u7a76\u6295\u5165\u5230\u63d0\u9ad8\u5176\u5149\u7a33\u5b9a\u6027\u4e2d\uff0c\u7279\u522b\u662f\u96c6\u4e2d\u4e8e\u5c06\u5149\u81f4\u8f7d\u6d41\u5b50\u4eceCu2<\/sub>O\u4e2d\u5feb\u901f\u8f6c\u79fb\u5230\u53cd\u5e94\u7269\u6216\u8005\u5171\u50ac\u5316\u5242\u4e2d\uff0c\u4ee5\u907f\u514d\u8f7d\u6d41\u5b50\u5728\u9897\u7c92\u4e2d\u7684\u5806\u79ef\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6fb3\u5927\u5229\u4e9a\u65b0\u5357\u5a01\u5c14\u58eb\u5927\u5b66Rose Amal \u6559\u6388<\/b><\/strong>\u7814\u7a76\u56e2\u961f\u5728J. Photochem. Photobiol., C.<\/i><\/b><\/em><\/strong>\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cRecent Advances in Suppressing the Photocorrosion of Cuprous Oxide for Photocatalytic and Photoelectrochemical Energy Conversion<\/b><\/strong>\u201d\u7684\u7efc\u8ff0\u6587\u7ae0\u3002\u672c\u6587\u4eceCu2<\/sub>O\u7684\u6750\u6599\u672c\u8d28\u5c5e\u6027\u53ca\u7535\u8377\u52a8\u529b\u5b66\u51fa\u53d1\uff0c\u603b\u7ed3\u4e86\u6291\u5236\u5176\u5149\u8150\u8680\u6027\u7684\u6700\u65b0\u7814\u7a76\u8fdb\u5c55\u3002\u4f5c\u8005\u6839\u636e\u4e0d\u540c\u7684\u6291\u5236\u624b\u6bb5\u8fdb\u884c\u5206\u7c7b\uff0c\u9610\u8ff0\u4e86\u5404\u79cd\u65b9\u6cd5\u7684\u673a\u7406\u53ca\u5e94\u7528\u3002\u6700\u540e\uff0c\u4f5c\u8005\u603b\u7ed3\u5e76\u5bf9\u672a\u6765\u8fdb\u4e00\u6b65\u63d0\u9ad8Cu2<\/sub>O\u5149\u7a33\u5b9a\u6027\u7684\u7814\u7a76\u63d0\u51fa\u4e86\u5c55\u671b\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u589e\u5f3aCu2<\/sub>O\u5149\u50ac\u5316\u7a33\u5b9a\u6027\u7684\u7814\u7a76\u8868\u660e\uff0c\u6700\u5e38\u89c1\u7684\u65b9\u6cd5\u5305\u62ec\uff1a1\uff09\u6676\u9762\u8c03\u63a7\uff08\u5f62\u8c8c\u63a7\u5236\uff09\uff0c2\uff09\u7c92\u5f84\u63a7\u5236\uff0c3\uff09\u53cd\u5e94\u6761\u4ef6\u7684\u8c03\u63a7\u548c4\uff09\u4e0e\u5176\u4ed6\u6750\u6599\u5f62\u6210\u5f02\u8d28\u7ed3\u3002 \uff08\u56fe1\uff09<\/p>\n

Figure 1: Summary of the main approaches for photostability enhancement of Cu<\/b><\/strong>2<\/b><\/sub><\/strong>O photocatalyst. <\/b><\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

    \n
  1. <\/b>\u6676\u9762\u5de5\u7a0b<\/b><\/strong><\/li>\n<\/ol>\n

    Cu2<\/sub>O\u6700\u5e38\u89c1\u7684\u5f62\u8c8c\u662f\u5404\u5411\u540c\u6027\u7684\u7acb\u65b9\u4f53\uff0c\u516b\u9762\u4f53\u548c\u5341\u4e8c\u9762\u4f53 \uff08\u4ec5\u4e00\u4e2a\u66b4\u9732\u6676\u9762\uff09\u3002\u5927\u591a\u6570\u7814\u7a76\u8868\u660eCu2<\/sub>O\uff08111\uff09\u5177\u6709\u66f4\u597d\u7684\u7a33\u5b9a\u6027\uff0c\u8fd9\u8d77\u56e0\u4e8e\uff08110\uff09\u6676\u9762\u7684\u4ef7\u5e26\u4f4d\u7f6e\u66f4\u6b63\uff0c\u4ece\u800c\u53ef\u4ee5\u4fc3\u8fdb\u5149\u751f\u7a7a\u7a74\u8f6c\u79fb\u81f3Cu2<\/sub>O\u7684\uff08100\uff09\u548c\uff08110\uff09\u6676\u9762\uff08\u5982\u56fe2a\u6240\u793a\uff09\u3002\u57fa\u4e8e\u5404\u5411\u540c\u6027\u6676\u9762\u7684Cu2<\/sub>O\uff0c\u516b\u9762\u4f53Cu2<\/sub>O\u6781\u597d\u7684\u7a33\u5b9a\u6027\u53ef\u4ee5\u5f52\u56e0\u4e8e\uff1a\uff081\uff09\u5728\u672b\u68a2\/\u8fb9\u754c\u5f62\u6210\u7684\u865a\u6784\u6676\u9762\uff1b\uff082\uff09\u8f83\u4f4e\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd\uff0c\u8fd9\u4f7f\u5176\u5177\u6709\u70ed\u529b\u5b66\u53ca\u5316\u5b66\u7a33\u5b9a\u6027\uff08\u56fe2b\uff09\u3002<\/p>\n

    Figure 2: Photocorrosion of cubic, octahedral and rhombic dodecahedral Cu<\/b><\/strong>2<\/b><\/sub><\/strong>O under illumination. [1,2]<\/b><\/strong><\/p>\n

    \u00a0\"\"<\/b><\/strong><\/p>\n

      \n
    1. <\/b>\u7c92\u5f84\u63a7\u5236<\/b><\/strong><\/li>\n<\/ol>\n

      Cu2<\/sub>O\u9897\u7c92\u5c3a\u5bf8\u4e5f\u4f1a\u5f71\u54cd\u5b83\u7684\u7ed3\u6784\u7a33\u5b9a\u6027\uff0c\u56e0\u4e3a\u7eb3\u7c73\u9897\u7c92\u5177\u6709\u8f83\u9ad8\u8868\u9762\u80fd\u4ece\u800c\u4fc3\u8fdb\u9897\u7c92\u7684\u56e2\u805a\u3002\u6b64\u5916\uff0c\u7531\u4e8e\u7ed3\u6676\u5ea6\u7684\u964d\u4f4e\u548c\u80fd\u5e26\u5f2f\u66f2\u7684\u51cf\u5f31\uff0c\u7eb3\u7c73\u7ed3\u6784\u8fd8\u53ef\u80fd\u5bf9\u7535\u5b50\u8f6c\u79fb\u6548\u7387\u4ea7\u751f\u4e0d\u5229\u7684\u5f71\u54cd\uff08\u56fe3\uff09\u3002<\/p>\n

      Figure 3: Cu<\/b><\/strong>2<\/b><\/sub><\/strong>O particles with different sizes and their corresponding XRD patterns before and after illumination. [3]<\/b><\/strong><\/p>\n

      \"\"<\/p>\n

        \n
      1. <\/b>\u53cd\u5e94\u6761\u4ef6\u7684\u8c03\u63a7<\/b><\/strong><\/li>\n<\/ol>\n

        \u6211\u4eec\u6700\u8fd1\u7684\u5de5\u4f5c\u8bc1\u5b9e\uff0c\u4f7f\u7528\u5408\u9002\u7684\u53cd\u5e94\u6eb6\u5242\u4e0d\u4ec5\u53ef\u4ee5\u6291\u5236\u5149\u81f4\u8150\u8680\u7684\u53d1\u751f\uff0c\u800c\u4e14\u8fd8\u53ef\u4ee5\u589e\u5f3a\u5149\u53cd\u5e94\u6d3b\u6027\u3002\u5728\u5149\u50ac\u5316\u4ea7\u6c22\u53cd\u5e94\u4f53\u7cfb\u4e2d\u52a0\u5165\u7a7a\u7a74\u590d\u5408\u5242\u4fc3\u8fdb\u4e86\u7a7a\u7a74\u6d88\u8017\uff0c\u4ece\u800c\u9632\u6b62\u4e86\u7a7a\u7a74\u53c2\u4e0e\u7684\u81ea\u6c27\u5316\u53cd\u5e94\uff08\u56fe4\uff09\u3002<\/p>\n

        Figure 4: Characterisation of Cu<\/b><\/strong>2<\/b><\/sub><\/strong>O after illumination with and without scavengers. [4]<\/b><\/strong><\/p>\n

        \"\"<\/p>\n

          \n
        1. <\/b>\u5f02\u8d28\u7ed3\u7684\u5f62\u6210 (\u5176\u4ed6\u534a\u5bfc\u4f53\uff0c\u78b3\u6750\u6599\u548c\u91d1\u5c5e)<\/b><\/strong><\/li>\n<\/ol>\n

          \u5408\u7406\u7684\u4e0e\u5176\u4ed6\u6750\u6599\u7ec4\u5408\u4e3a\u590d\u5408\u6750\u6599\u53ef\u4ee5\u52a0\u5feb\u7535\u5b50\u8f6c\u79fb\uff1b\u56e0\u6b64\uff0c\u51cf\u5c11\u4e86\u5149\u751f\u7535\u8377\u5728\u9897\u7c92\u5185\u7684\u7d2f\u79ef\u3002\u5728\u5149\u50ac\u5316\uff08\u7c89\u672b\uff09\u4f53\u7edf\u4e2d\u91c7\u7528\u7684\u7b56\u7565\u4e0e\u7528\u4e8e\u5149\u7535\u50ac\u5316\uff08\u8584\u819c\uff09Cu2<\/sub>O\u7684\u65b9\u6cd5\u7565\u6709\u4e0d\u540c\u3002\u7c89\u672b\u72b6Cu2<\/sub>O\u901a\u5e38\u4f7f\u7528\u91d1\u5c5e\/\u534a\u5bfc\u4f53\/\u78b3\u6750\u6599\u6765\u4fee\u9970\u4ee5\u4fc3\u8fdb\u5176\u7535\u5b50\u8f6c\u79fb\uff0c\u800c\u5728\u5149\u7535\u5316\u5b66\u4f53\u7cfb\u4e2d\uff0c\u5176\u4ed6\u6750\u6599\u901a\u5e38\u8986\u76d6\u5728\u8584\u819cCu2<\/sub>O\u8868\u9762\u4e0a\u5f62\u6210\u4fdd\u62a4\u5c42\u3002<\/p>\n

          4.1 \u534a\u5bfc\u4f53<\/b><\/strong><\/p>\n

          \u5728\u4e4b\u524d\u7684\u5de5\u4f5c\u4e2d\uff0c\u672c\u8bfe\u9898\u7ec4\u5df2\u7ecf\u4f7f\u7528\u4e86Cu2<\/sub>O\u8584\u819c\u8868\u9762\u949d\u5316\u7684\u6982\u5ff5\u3002\u6211\u4eec\u9996\u6b21\u63d0\u51fa\u4e86\u901a\u8fc7\u70ed\u5904\u7406\u5728Cu2<\/sub>O\u8584\u819c\u4e0a\u5f15\u5165CuO\u7eb3\u7c73\u7ebf\uff0c\u4ee5\u7a33\u5b9aCu2<\/sub>O\u819c\uff08\u56fe5a\uff09\u3002\u6b64\u5916\uff0c Cu2<\/sub>O\u5c42\u548cCuO\u5916\u5c42\u4e4b\u95f4\u5939\u6742TiO2<\/sub>\u5c42\u7684\u4e09\u660e\u6cbb\u7ed3\u6784\u4e5f\u8fdb\u4e00\u6b65\u8bf1\u5bfc\u4e86\u66f4\u597d\u7684PEC\u6027\u80fd\u548c\u589e\u5f3a\u7684Cu2<\/sub>O-CuO\u5149\u7535\u6781\u7a33\u5b9a\u6027\uff08\u56fe5b-d\uff09\u3002<\/p>\n

          Figure 5: Incorporation of CuO nanowires and TiO<\/b><\/strong>2<\/b><\/sub><\/strong>\u00a0thin layer on Cu<\/b><\/strong>2<\/b><\/sub><\/strong>O thin film.<\/b><\/strong><\/p>\n

          \"\"<\/p>\n

          4.2 \u78b3\u6750\u6599<\/b><\/strong><\/p>\n

          \u53e6\u4e00\u4e2a\u88ab\u5e7f\u6cdb\u7814\u7a76\u7684\u6291\u5236Cu2<\/sub>O\u5149\u8150\u8680\u7684\u65b9\u6cd5\u662f\u4e0e\u78b3\u6750\u6599\uff08\u5305\u62ecgraphene\uff0creduced graphene oxide (rGO)\uff0cC3<\/sub>N4<\/sub>\u4ee5\u53ca\u78b3\u91cf\u5b50\u70b9\uff09\u7684\u590d\u5408\u3002\u4f8b\u5982\uff0crGO\u590d\u5408\u7684Cu2<\/sub>O\u4ee5\u53ca\u78b3\u91cf\u5b50\u70b9\u4fee\u9970\u7684Cu2<\/sub>O\u88ab\u53d1\u73b0\u5bf9\u4e8e\u7a33\u5b9a\u5149\u50ac\u5316\u5242\u53ca\u63d0\u9ad8\u5176\u6d3b\u6027\u5177\u6709\u79ef\u6781\u7684\u4f5c\u7528\uff08\u56fe6\uff09\u3002<\/p>\n

          Figure 6: (a) Cu<\/b><\/strong>2<\/b><\/sub><\/strong>O-rGO and (b)-(c) CQDs\/Cu<\/b><\/strong>2<\/b><\/sub><\/strong>O [6,7]<\/b><\/strong><\/p>\n

          \"\"<\/p>\n

          4.3 \u91d1\u5c5e<\/b><\/strong><\/p>\n

          Au\/Cu2<\/sub>O, Ag\/Cu2<\/sub>O \u53ca Cu\/Cu2<\/sub>O\u662f\u6bd4\u8f83\u5e38\u89c1\u7684\u51e0\u79cd\u91d1\u5c5e\u8d1f\u8f7d\u4e8eCu2<\/sub>O\u6750\u6599\u3002\u9664\u4e86\u8868\u9762\u6c89\u79ef\uff0c\u6838\u58f3\u7ed3\u6784\u7684\u91d1\u5c5e-Cu2<\/sub>O\u4e5f\u5f15\u8d77\u4e86\u660e\u663e\u7684\u5173\u6ce8\u3002Au-Cu2<\/sub>O\u6838\u58f3\u7ed3\u6784\u88ab\u8bc1\u5b9e\u80fd\u591f\u63d0\u9ad8\u7535\u8377\u5206\u79bb\u6548\u7387\uff0c\u540c\u65f6\u80fd\u591f\u63d0\u9ad8Cu2<\/sub>O\u7684\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\uff08\u56fe7\uff09\u3002<\/p>\n

          Figure 7: Au-Cu<\/b><\/strong>2<\/b><\/sub><\/strong>O core shell structures. [8]<\/b><\/strong><\/p>\n

          \"\"<\/p>\n

          \u3010\u603b\u7ed3\u3011<\/b><\/strong><\/p>\n

          \u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u7cfb\u7edf\u5730\u603b\u7ed3\u4e86\u8fd1\u5e74\u6765\u5728\u6291\u5236Cu2<\/sub>O\u5149\u8150\u8680\u4e0a\u6240\u53d6\u5f97\u7684\u6210\u5c31\u3002\u63d0\u9ad8\u5176\u5149\u7a33\u5b9a\u6027\u7684\u624b\u6bb5\u5305\u62ec\u4e86\u6676\u9762\u63a7\u5236\uff0c\u7c92\u5f84\u8c03\u8282\uff0c\u53cd\u5e94\u6761\u4ef6\u8c03\u63a7\u4ee5\u53ca\u4e0e\u5176\u4ed6\u6750\u6599\u590d\u5408\u3002\u5927\u90e8\u5206\u65b9\u6cd5\u7684\u7406\u8bba\u57fa\u7840\u90fd\u662f\u907f\u514dCu2<\/sub>O\u5149\u751f\u8f7d\u6d41\u5b50\u5728\u9897\u7c92\u5185\u7684\u5806\u79ef\uff0c\u56e0\u4e3a\u5149\u751f\u7535\u5b50\u6216\u8005\u7a7a\u7a74\u7684\u7d2f\u79ef\u4f1a\u5bfc\u81f4\u5176\u81ea\u8fd8\u539f\u6216\u81ea\u6c27\u5316\u53cd\u5e94\u7684\u53d1\u751f\u3002\u56e0\u6b64\uff0c\u63d0\u9ad8Cu2<\/sub>O\u7684\u7535\u8377\u53cd\u5e94\u52a8\u529b\u5b66\uff08\u5373\u6709\u6548\u7684\u8f6c\u79fb\u7535\u5b50\u6216\u7a7a\u7a74\uff09\u4e0d\u4ec5\u53ef\u4ee5\u6539\u5584\u5176\u5149\u7a33\u5b9a\u6027\uff0c\u4e5f\u80fd\u591f\u663e\u8457\u63d0\u9ad8Cu2<\/sub>O\u7684\u53cd\u5e94\u6d3b\u6027\u3002\u6700\u540e\uff0c\u4f5c\u8005\u63d0\u51fa\u4e86\u89e3\u5149\u8150\u8680\u7684\u673a\u7406\u5bf9\u4e8e\u8fdb\u4e00\u6b65\u63d0\u9ad8Cu2<\/sub>O\u7a33\u5b9a\u6027\u7684\u91cd\u8981\u6027\u3002<\/p>\n

          \u6587\u7ae0\u94fe\u63a5\uff1aDOI: https:\/\/doi.org\/10.1016\/j.jphotochemrev.2018.10.001<\/a><\/p>\n

          \u8bfe\u9898\u7ec4\u7b80\u4ecb<\/b><\/strong><\/p>\n

          Rose Amal\u6559\u6388\u8bfe\u9898\u7ec4\uff08Particles and Catalysis Research Group\uff09\u4f9d\u6258\u4e8e\u6fb3\u5927\u5229\u4e9a\u65b0\u5357\u5a01\u5c14\u58eb\u5927\u5b66\u5316\u5b66\u5de5\u7a0b\u5b66\u9662\uff0c\u4e3b\u8981\u4ece\u4e8b\u50ac\u5316\u6750\u6599\u5728\u80fd\u6e90\u8f6c\u6362\u53ca\u5b58\u50a8\uff0c\u73af\u5883\u5e94\u7528\u7b49\u65b9\u9762\u7684\u7814\u7a76\u3002\u66f4\u591a\u5185\u5bb9\uff0c\u6b22\u8fce\u8bbf\u95ee\u8bfe\u9898\u7ec4\u7f51\u9875\uff1ahttp:\/\/www.pcrg.unsw.edu.au\/<\/u><\/a>\u00a0<\/p>\n

          \u53c2\u8003\u6587\u732e<\/b><\/strong><\/p>\n

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          4. Y. Toe, Z. Zheng, H. Wu, J. Scott, R. Amal, Y.H. Ng, Photocorrosion of cuprous oxide in hydrogen production: Rationalising self\u2010oxidation or self\u2010reduction, Angew. Chem., 57 (2018), 13613-13617.<\/li>\n
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          6. D. Tran, S.K. Batabyal, S.S. Pramana, J. Barber, L.H. Wong, S.C.J. Loo, A cuprous oxide-reduced graphene oxide (Cu2<\/sub>O-rGO) composite photocatalyst for hydrogen generation: Employing rGO as an electron acceptor to enhance the photocatalytic activity and stability of Cu2<\/sub>O, Nanoscale, 4 (2012) 3875-3878.<\/li>\n
          7. Li, R. Liu, Y. Liu, H. Huang, H. Yu, H. Ming, S. Lian, S.-T. Lee, Z. Kang, Carbon quantum dots\/Cu2<\/sub>O composites with protruding nanostructures and their highly efficient (near) infrared photocatalytic behavior, J. Mater. Chem., 22 (2012) 17470-17475.<\/li>\n
          8. Ma, X. Zhu, X. Shusheng, G. He, L. Yao, N. Hu, Y. Su, J. Feng, Y. Zhang, Z. Yang, Gold nanobipyramid@cuprous oxide jujube-like nanostructures for plasmon-enhanced photocatalytic performance, Appl. Catal., B, 234 (2018), 26-36.<\/li>\n<\/ol>\n

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