{"id":163207,"date":"2018-12-28T12:00:06","date_gmt":"2018-12-28T04:00:06","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=163207"},"modified":"2018-12-28T17:41:25","modified_gmt":"2018-12-28T09:41:25","slug":"%e9%83%ad%e9%91%ab%e6%9d%8e%e7%81%bf-joule-%e9%ab%98%e7%a8%b3%e5%ae%9a%e6%80%a7dion-jacobson-dj%e5%9e%8b%e4%ba%8c%e7%bb%b4%e9%92%99%e9%92%9b%e7%9f%bf%e5%a4%aa%e9%98%b3%e8%83%bd%e7%94%b5","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=163207","title":{"rendered":"\u90ed\u946b&\u674e\u707f Joule: \u9ad8\u7a33\u5b9a\u6027Dion-Jacobson (DJ)\u578b\u4e8c\u7ef4\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0 \u5728\u5316\u77f3\u71c3\u6599\u65e5\u8d8b\u67af\u7aed\u7684\u5f53\u4e0b\uff0c\u592a\u9633\u80fd\u5df2\u6210\u4e3a\u4eba\u7c7b\u4f7f\u7528\u80fd\u6e90\u7684\u91cd\u8981\u7ec4\u6210\u90e8\u5206\uff0c\u5e76\u5f97\u4ee5\u4e0d\u65ad\u53d1\u5c55\u3002\u592a\u9633\u80fd\u7684\u5229\u7528\u5305\u62ec\u591a\u79cd\u65b9\u5f0f\uff0c\u592a\u9633\u80fd\u5149\u4f0f\u53d1\u7535\u662f\u5176\u5229\u7528\u7684\u91cd\u8981\u9014\u5f84\u3002\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60(PSC)\u7531\u4e8e\u8f83\u9ad8\u7684\u5149\u7535\u8f6c\u6362\u6548\u7387(PCE)\u5f15\u8d77\u4e86\u5b66\u672f\u754c\u548c\u5de5\u4e1a\u754c\u7684\u5e7f\u6cdb\u5173\u6ce8\uff0c\u4f46\u662f\u4f20\u7edf\u7684\u4e09\u7ef4 (3D)\u9499\u949b\u77ff\u81ea\u8eab\u7ed3\u6784\u4e0d\u7a33\u5b9a\uff0c\u5bfc\u81f4\u5176\u5668\u4ef6\u7a33\u5b9a\u6027\u5dee\uff0c\u5236\u7ea6\u4e86PSC\u7684\u5176\u8fdb\u4e00\u6b65\u53d1\u5c55\u3002\u867d\u7136\u901a\u8fc7\u754c\u9762\u4fee\u9970\u548c\u63ba\u6742\u7b49\u65b9\u6cd5\u53ef\u4ee5\u4e00\u5b9a\u7a0b\u5ea6\u4e0a\u63d0\u9ad83D PSC\u7684\u7a33\u5b9a\u6027\uff0c\u4f46\u662f\u5e76\u4e0d\u80fd\u4ece\u6839\u672c\u4e0a\u89e3\u51b3\u8be5\u7c7b\u9499\u949b\u77ff\u6750\u6599\u81ea\u8eab\u7ed3\u6784\u7a33\u5b9a\u6027\u5dee\u7684\u95ee\u9898\u3002\u56e0\u6b64\uff0c\u63d0\u9ad8\u9499\u949b\u77ff\u6750\u6599\u672c\u8eab\u7684\u7ed3\u6784\u7a33\u5b9a\u6027\u662f\u4ece\u6839\u672c\u4e0a\u89e3\u51b3PSC\u7a33\u5b9a\u6027\u95ee\u9898\u7684\u5173\u952e\u3002<\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0 \u76ee\u524d\uff0c\u4e3a\u89e3\u51b3PSC\u7684\u7a33\u5b9a\u6027\u95ee\u9898\uff0c\u9664\u4e86\u754c\u9762\u5de5\u7a0b\u548c\u5668\u4ef6\u5c01\u88c5\u7b49\u65b9\u6cd5\u5916\uff0c\u4eba\u4eec\u4e5f\u5728\u63a2\u5bfb3D\u9499\u949b\u77ff\u7684\u66ff\u4ee3\u8005\u4ee5\u671f\u4ece\u672c\u8d28\u4e0a\u63d0\u9ad8\u5149\u6d3b\u6027\u6750\u6599\u7684\u7a33\u5b9a\u6027\u3002\u7814\u7a76\u8868\u660e\uff0cRuddlesden-Popper (RP) 2D\u5c42\u72b6\u9499\u949b\u77ff\u56e0\u542b\u6709\u5927\u5c3a\u5bf8\u4e14\u758f\u6c34\u7684\u6709\u673a\u9633\u79bb\u5b50\u53ef\u4ee5\u51cf\u5c0f\u6c34\u5206\u5b50\u6e17\u900f\u5230\u9499\u949b\u77ff\u6676\u683c\u4e2d\u7684\u53ef\u80fd\u6027\uff0c\u56e0\u6b64\u57fa\u4e8e2D PSC\u7684\u7a33\u5b9a\u6027\u4f18\u4e8e\u4f20\u7edf3D PSC\u3002\u7136\u800c\uff0c\u6b64\u7c7bRP\u578b2D\u9499\u949b\u77ff\u6750\u6599\u5c42\u95f4\u7684\u8303\u5fb7\u534e\u529b\u4f5c\u7528\u5f88\u5f31\uff0c\u4e0d\u8db3\u4ee5\u4fdd\u8bc1\u6750\u6599\u5177\u6709\u8db3\u591f\u7684\u7ed3\u6784\u7a33\u5b9a\u6027\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u6700\u8fd1\uff0c\u4e2d\u79d1\u9662\u5927\u8fde\u5316\u5b66\u7269\u7406\u7814\u7a76\u6240\u7684\u90ed\u946b\u7814\u7a76\u5458\u548c\u674e\u707f\u9662\u58eb\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u56e2\u961f\u62a5\u9053\u4e86\u901a\u8fc7\u5f15\u5165\u4e24\u7aef\u542b\u6709\u6c28\u57fa\u57fa\u56e2\u7684\u6709\u673a\u9633\u79bb\u5b50\uff0c\u53bb\u9664RP\u578b2D\u9499\u949b\u77ff\u5c42\u95f4\u7684\u8303\u5fb7\u534e\u76f8\u4e92\u4f5c\u7528\uff0c\u5f97\u5230Dion-Jacobson (DJ) \u578b2D\u5c42\u72b6\u9499\u949b\u77ff\u6750\u6599\u3002\u5229\u7528DJ\u578b2D\u9499\u949b\u77ff\u6750\u6599\u5236\u5907\u7684PSC\uff0c\u4e0d\u4ec5\u5149\u7535\u8f6c\u6362\u6548\u7387\u8fbe\u523013.3%\uff0c\u9ad8\u4e8e\u76f8\u540c\u6761\u4ef6\u4e0b\u5236\u5907\u7684RP\u578b2D PSC\u7684\u6548\u7387\uff0c\u800c\u4e14\u5176\u5668\u4ef6\u7a33\u5b9a\u6027\u4e5f\u663e\u8457\u63d0\u9ad8\u3002\u672a\u5c01\u88c5\u5668\u4ef6\u5728\u201c\u53cc85\u201d\uff0885\u2103\u548c85\uff05\u76f8\u5bf9\u6e7f\u5ea6\uff09\u548c\u4e00\u4e2a\u6807\u51c6\u592a\u9633\u5149\u6301\u7eed\u7167\u5c04\u6761\u4ef6\u4e0b\u8fdb\u884c\u7684\u8001\u5316\u6d4b\u8bd5\u8868\u660e\uff0cDJ\u578b2D PSC\u957f\u671f\u6d4b\u8bd5\u540e\u4ecd\u80fd\u4fdd\u630195%\u4ee5\u4e0a\u7684\u5149\u7535\u8f6c\u6362\u6548\u7387\uff0c\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u6e7f\u70ed\u7a33\u5b9a\u6027\u548c\u5149\u7167\u7a33\u5b9a\u6027\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cDion-Jacobson Phase 2D Layered Perovskites for Solar Cells with Ultrahigh Stability\u201d<\/strong>\u53d1\u8868\u5728\u56fd\u9645\u8457\u540d\u671f\u520aJoule<\/strong>\u4e0a\u3002<\/p>\n

\"\" \u7814\u7a76\u4eae\u70b9\uff1a<\/strong><\/p>\n

1\u3001\u5f00\u53d1\u4e86\u4e00\u79cd\u65e0\u5c42\u95f4\u8303\u5fb7\u534e\u76f8\u4e92\u4f5c\u7528\u7684Dion-Jacobson (DJ)\u578b2D\u9499\u949b\u77ff\u6750\u6599\uff1b<\/strong><\/p>\n

2\u3001DJ\u578b2D\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60(PSC)\u7684\u5149\u7535\u8f6c\u6362\u6548\u7387(PCE)\u4e3a13.3\uff05\uff1b<\/strong><\/p>\n

3\u3001\u672a\u5c01\u88c5\u5668\u4ef6\u53ef\u7ecf\u53d7\u4e25\u82db\u6761\u4ef6\u7684\u7a33\u5b9a\u6027\u6d4b\u8bd5\uff1b<\/strong><\/p>\n

4\u3001\u4e8c\u80fa\u9633\u79bb\u5b50\u4e24\u7aef\u4e0e\u9499\u949b\u77ff\u5c42\u5f62\u6210\u6c22\u952e\u4f5c\u7528\uff0c\u63d0\u9ad8\u4e86\u4e8c\u7ef4\u5c42\u72b6\u7ed3\u6784\u7684\u7a33\u5b9a\u6027\u3002<\/strong><\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001RP\u548cDJ\u578b2D\u5c42\u72b6\u9499\u949b\u77ff\u6750\u6599\u7ed3\u6784\u793a\u610f\u56fe\"\"<\/strong><\/p>\n

\u56fe\u4e8c\u3001(PDA) (MA)n-1<\/sub>PbnI3n+1<\/sub>\u8584\u819c\u7684\u8868\u5f81<\/strong>
\n \"\"\uff08A\uff09\u7d2b\u5916\u53ef\u89c1\u5438\u6536\u5149\u8c31\uff08\u63d2\u56fe\uff1a\u819c\u989c\u8272\u968f\u5c42\u6570\uff08n\u503c\uff09\u589e\u52a0\u7684\u53d8\u5316\u8d8b\u52bf\uff09\uff1b<\/p>\n

\uff08B\uff09\u4e0d\u540c\u5c42\u6570\uff08n\u503c\uff09DJ\u578b2D\u9499\u949b\u77ff\u7684XRD\u56fe\uff08\u63d2\u56fe\uff1a 14.2\u00b0\u548c28.4\u00b0\u5904\u884d\u5c04\u5cf0\u7684\u4f4d\u79fb\u53d8\u5316\uff09\uff1b<\/p>\n

\uff08C\uff09\u5404\u79cd\u70ed\u6d82\u6e29\u5ea6\u4e0bn = 4\u7684XRD\u56fe\uff1b<\/p>\n

\uff08D\uff09\u6676\u4f53\u5c3a\u5bf8\u548c\u534a\u5cf0\u5bbd\uff08FWHM\uff09\u968f\u70ed\u6d82\u6e29\u5ea6\u589e\u52a0\u7684\u53d8\u5316\uff0c\u6570\u636e\u53d6\u81ea14.2\u00b0\u7684\u884d\u5c04\u5cf0\u3002<\/p>\n

\u56fe\u4e09\u3001\u5404\u79cd\u70ed\u6d82\u6e29\u5ea6\u4e0b(PDA)(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u8584\u819c\u7684\u4e8c\u7ef4 GI-XRD\u56fe<\/strong>
\n \"\"\uff08A\uff09\u5ba4\u6e29\u3001\uff08B\uff09110 \u2103\u3001\uff08C\uff09130 \u2103\u3001\uff08D\uff09150 \u2103\u3001\uff08E\uff09170 \u2103\u548c\uff08F\uff09190 \u2103\u3002<\/p>\n

\u56fe\u56db\u3001(PDA)(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u57fa\u5668\u4ef6\u7684\u5149\u4f0f\u6027\u80fd<\/strong>
\n \"\"\uff08A\uff09\u5668\u4ef6\u7ed3\u6784\uff1b<\/p>\n

\uff08B\uff09\u80fd\u7ea7\u56fe\uff1b<\/p>\n

\uff08C\uff09\u57fa\u4e8e(PDA)(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u7684\u7535\u6c60\u7684\u6a2a\u622a\u9762SEM\u56fe\uff1b<\/p>\n

\uff08D\uff09\u4f7f\u7528(PDA)(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u4f5c\u4e3a\u6d3b\u6027\u5c42\u7684\u5668\u4ef6\u5728\u4e00\u4e2a\u6807\u51c6\u592a\u9633\u5149\u7167\u6761\u4ef6\u4e0b\u7684J-V\u66f2\u7ebf\uff1b\uff08\u63d2\u56fe\uff1a\u5728\u6700\u5927\u529f\u7387\u70b9\uff08Vmp<\/sub> = 0.72 V\uff09\u4e0b\u6d4b\u91cf\u7684\u7a33\u5b9a\u5149\u7535\u6d41\uff09<\/p>\n

\uff08E\uff09\u70ed\u6d82\u6e29\u5ea6\u5bf9PCE\u548cJsc<\/sub>\u7684\u5f71\u54cd\uff1b<\/p>\n

\uff08F\uff0950\u4e2a(PDA)(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u57fa\u5668\u4ef6\u7684\u6548\u7387\u5206\u5e03\u76f4\u65b9\u56fe\uff1b<\/p>\n

\uff08G\uff09EQE\u548c\u79ef\u5206Jsc<\/sub>\u968f\u6ce2\u957f\u7684\u53d8\u5316\u3002<\/strong><\/p>\n

\u56fe\u4e94\u3001TRPL\u548cEIS\u6570\u636e<\/strong>
\n \"\"\uff08A\uff09(PDA)(MA)3<\/sub> Pb4<\/sub>I13<\/sub>\u548c(PA)2<\/sub>(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u5728FTO\/TiO2<\/sub>\u57fa\u5e95\u4e0a\u7684TRPL\u5149\u8c31\uff1b<\/p>\n

\uff08B\uff09\u5206\u522b\u4f7f\u7528(PDA)(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u548c(PA)2<\/sub>(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u4f5c\u4e3a\u6d3b\u6027\u5c42\u7684\u5668\u4ef6\u7684\u5948\u594e\u65af\u7279\u56fe\uff0c\u6697\u6001\u3001\u5f00\u8def\u6761\u4ef6\u4e0b\u6d4b\u5f97\uff08\u63d2\u56fe\uff1a\u7b49\u6548\u7535\u8def\uff09\u3002<\/p>\n

\u56fe\u516d\u3001MAPbI3<\/sub>\u3001(PA)2<\/sub>(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u548c(PDA)(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u57fa\u5668\u4ef6\u7684\u7a33\u5b9a\u6027\u6d4b\u8bd5<\/strong><\/p>\n

\"\"\uff08A\uff09\u5ba4\u6e29\u7a7a\u6c14\u4e2d\uff1b<\/p>\n

\uff08B\uff09\u6e7f\u70ed\u6761\u4ef6\u4e0b\uff0885 \u2103\u548c40\uff05-70\uff05\u76f8\u5bf9\u6e7f\u5ea6\uff09\uff1b<\/p>\n

\uff08C\uff09\u6e7f\u70ed\u6761\u4ef6\u4e0b\uff0885 \u2103\u548c85\uff05\u76f8\u5bf9\u6e7f\u5ea6\uff09\uff1b<\/p>\n

\uff08D\uff09\u4e00\u4e2a\u6807\u51c6\u592a\u9633\u5149\u6301\u7eed\u5149\u7167\u6761\u4ef6\u4e0b\u3002<\/p>\n

\u56fe\u4e03\u3001\u8584\u819c\u7a33\u5b9a\u6027\u6d4b\u8bd5\u7684XRD\u56fe<\/strong>
\n \"\"\uff08A\uff09\u5ba4\u6e29\u7a7a\u6c14\u4e2d\u7684MAPbI3<\/sub>\u8584\u819c (\u76f8\u5bf9\u6e7f\u5ea6\u4e3a40\uff05-70%)\uff1b<\/p>\n

\uff08B\uff09\u5ba4\u6e29\u7a7a\u6c14\u4e2d\u7684(PA)2<\/sub>(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u8584\u819c\uff1b<\/p>\n

\uff08C\uff09\u5ba4\u6e29\u7a7a\u6c14\u4e2d\u7684(PDA)(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u8584\u819c\uff1b<\/p>\n

\uff08D\uff09\u7a7a\u6c14\u6c1b\u56f4\u300185 \u2103\u52a0\u70ed\u6761\u4ef6\u4e0b\u7684MAPbI3<\/sub>\u8584\u819c\uff1b<\/p>\n

\uff08E\uff09\u7a7a\u6c14\u6c1b\u56f4\u300185 \u2103\u52a0\u70ed\u6761\u4ef6\u4e0b\u7684(PA)2<\/sub>(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u8584\u819c\uff1b<\/p>\n

\uff08F\uff09\u7a7a\u6c14\u6c1b\u56f4\u300185 \u2103\u52a0\u70ed\u6761\u4ef6\u4e0b\u7684(PDA)(MA)3<\/sub>Pb4<\/sub>I13<\/sub>\u8584\u819c\u3002<\/p>\n

\u3010\u603b\u7ed3\u3011<\/strong><\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0 \u00a0\u4e8c\u7ef4\u9499\u949b\u77ff\u5df2\u6210\u4e3a\u89e3\u51b3\u4f20\u7edf\u4e09\u7ef4\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7a33\u5b9a\u6027\u95ee\u9898\u7684\u6709\u6548\u65b9\u6848\u3002\u7136\u800c\uff0c\u6587\u732e\u62a5\u9053\u7684RP\u578b\u4e8c\u7ef4\u9499\u949b\u77ff\u867d\u7136\u7531\u4e8e\u542b\u6709\u758f\u6c34\u9633\u79bb\u5b50\uff08BA+<\/sup>\u3001PEA+<\/sup>\u7b49\uff09\u53ca\u5c42\u95f4\u8303\u5fb7\u534e\u76f8\u4e92\u4f5c\u7528\uff0c\u4f7fRP\u578b\u4e8c\u7ef4\u9499\u949b\u77ffPSC\u7684\u7a33\u5b9a\u6027\u9ad8\u4e8e\u4f20\u7edf\u4e09\u7ef4PSC\uff0c\u4f46\u8303\u5fb7\u534e\u5f31\u76f8\u4e92\u4f5c\u7528\u4e0d\u8db3\u4ee5\u4fdd\u8bc1\u6750\u6599\u7684\u7ed3\u6784\u7a33\u5b9a\u6027\uff0c\u5728\u9ad8\u6e29\u9ad8\u6e7f\u7684\u82db\u523b\u6d4b\u8bd5\u6761\u4ef6\u4e0b\uff0c\u5176\u5668\u4ef6\u6548\u7387\u4ecd\u4f1a\u660e\u663e\u8870\u51cf\u3002<\/p>\n

\u00a0 \u00a0 \u00a0 \u00a0\u672c\u6587\u62a5\u5bfc\u7684Dion-Jacobson\uff08DJ\uff09\u578b\u4e8c\u7ef4\u9499\u949b\u77ff\u65e0\u5c42\u95f4\u8303\u5fb7\u534e\u76f8\u4e92\u4f5c\u7528\uff0c\u4e24\u7aef\u6c22\u952e\u4f5c\u7528\u4f7f\u5f97\u7834\u574f\u5176\u4e8c\u7ef4\u5c42\u72b6\u7ed3\u6784\u9700\u8981\u66f4\u591a\u7684\u5916\u90e8\u80fd\u91cf\uff0c\u663e\u8457\u63d0\u9ad8\u4e86\u6750\u6599\u7684\u7ed3\u6784\u7a33\u5b9a\u6027\uff0c\u57fa\u4e8e\u6b64\u7684\u5668\u4ef6\u5728\u4e25\u82db\u7684\u6d4b\u8bd5\u6761\u4ef6\u4e0b\u8868\u73b0\u51fa\u4f18\u5f02\u7a33\u5b9a\u6027\u3002\u8be5\u5de5\u4f5c\u4ece\u6539\u5584\u9499\u949b\u77ff\u6750\u6599\u7ed3\u6784\u7a33\u5b9a\u6027\u89d2\u5ea6\u51fa\u53d1\uff0c\u4e3a\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7a33\u5b9a\u6027\u7814\u7a76\u63d0\u4f9b\u4e86\u65b0\u89c6\u89d2\uff0c\u6709\u5229\u4e8e\u63a8\u52a8\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u8fdb\u4e00\u6b65\u53d1\u5c55\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aDion-Jacobson Phase 2D Layered Perovskites for Solar Cells with Ultrahigh Stability<\/a><\/strong>\uff08Joule, 2018<\/strong>, DOI: 10.1016\/j.joule.2018.11.026. \uff09<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7eb3\u7c73\u7ec4\u5c0f\u80d6\u7eb8\u7f16\u8bd1\uff0c\u6750\u6599\u4eba\u6574\u7406\u3002<\/strong><\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaokefu.<\/p>\n","protected":false},"excerpt":{"rendered":"

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