{"id":166877,"date":"2019-02-14T06:30:09","date_gmt":"2019-02-13T22:30:09","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=166877"},"modified":"2019-02-13T22:11:28","modified_gmt":"2019-02-13T14:11:28","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91-jacs%ef%bc%9a%e5%90%88%e7%90%86%e8%ae%be%e8%ae%a1%e8%bf%91%e7%ba%a2%e5%a4%96%e8%81%9a%e9%9b%86%e8%af%b1%e5%af%bc%e5%8f%91%e5%b0%84%e6%b4%bb%e6%80%a7","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=166877","title":{"rendered":"JACS\uff1a\u5408\u7406\u8bbe\u8ba1\u8fd1\u7ea2\u5916\u805a\u96c6\u8bf1\u5bfc\u53d1\u5c04\u6d3b\u6027\u63a2\u9488\u7528\u4e8e\u5177\u6709\u8d85\u7075\u654f\u5ea6\u548c\u9ad8\u4fdd\u771f\u5ea6\u7684\u6dc0\u7c89\u6837\u86cb\u767d\u03b2\u6591\u5757\u7684\u539f\u4f4d\u6210\u50cf"},"content":{"rendered":"

\u3010\u7814\u7a76\u80cc\u666f\u3011<\/strong><\/p>\n

\u6dc0\u7c89\u6837\u86cb\u767d-\u03b2\uff08A\u03b2\uff09\u6591\u5757\u7684\u9ad8\u4fdd\u771f\u6210\u50cf\u5bf9\u65e9\u671f\u68c0\u6d4b\u963f\u5c14\u8328\u6d77\u9ed8\u75c7\u81f3\u5173\u91cd\u8981\u3002\u7136\u800c\uff0c\u4e8b\u5b9e\u8bc1\u660e\u901a\u8fc7\u5546\u4e1a\u4e0a\u53ef\u83b7\u5f97\u7684\u786b\u9ec4\u7d20\u884d\u751f\u7269\uff08ThT\u6216ThS\uff09\u5177\u6709\u660e\u663e\u7684\u805a\u96c6\u731d\u706d\u6548\u5e94\uff0c\u4f4e\u4fe1\u566a\u6bd4\uff08S \/ N\uff09\u548c\u5f31\u7684\u8840\u8111\u5c4f\u969c\uff08BBB\uff09\u7a7f\u900f\u529b\uff0c\u5728\u4f53\u5185\u68c0\u6d4bA\u03b2\u6591\u5757\u662f\u975e\u5e38\u53d7\u9650\u7684\u3002\u805a\u96c6\u8bf1\u5bfc\u53d1\u5c04\uff08AIE\uff09\u662f\u9274\u5b9a\u86cb\u767d\u8d28\u539f\u7ea4\u7ef4\u5f62\u6210\u7684\u4f18\u5148\u7b56\u7565\u3002\u8fd9\u79cd\u57fa\u4e8eAIE\u63a2\u9488\u7684\u8bbe\u8ba1\uff0c\u7279\u522b\u662f\u5c06\u6ce2\u957f\u5ef6\u4f38\u5230NIR\u533a\u57df\uff0c\u5bf9\u4e8e\u5f15\u5165\u53e6\u5916\u7684\u758f\u6c34\u6027\u03c0-\u5171\u8f6d\u6865\u57fa\u672c\u4e0a\u662f\u5fc5\u9700\u7684\u3002\u7136\u800c\uff0c\u5728\u63a2\u9488\u4e0eA\u03b2\u805a\u96c6\u4f53\u7ed3\u5408\u4e4b\u524d\u4e0d\u5e0c\u671b\u7684\u521d\u59cb\u805a\u96c6\u4e0d\u53ef\u907f\u514d\u5730\u5bfc\u81f4\u201c\u5047\u9633\u6027\u201dAIE\u4fe1\u53f7\u3002\u56e0\u6b64\uff0c\u8feb\u5207\u9700\u8981\u514b\u670d\u8f83\u957f\u6392\u653e\u7684\u4eb2\u8102\u6027\u8981\u6c42\u4e0e\u6c34\u4e0e\u86cb\u767d\u8d28\u539f\u7ea4\u7ef4\u5f62\u6210\u7684\u805a\u96c6\u884c\u4e3a\u4e4b\u95f4\u7684\u56f0\u5883\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u534e\u4e1c\u7406\u5de5\u5927\u5b66\u6731\u4e3a\u5b8f\u548c\u90ed\u5fd7\u524d\u6559\u6388\u8bfe\u9898\u7ec4<\/strong>\u7b49\u91c7\u7528\u7406\u6027\u7684\u201cstep-by-step\u201d\u5206\u5b50\u8bbe\u8ba1\u7b56\u7565\u6765\u89e3\u51b3\u5546\u4e1a\u67d3\u6599ThT\u7684\u56fa\u6709\u7f3a\u9677\uff0c\u901a\u8fc7\u5f15\u5165\u4eb2\u8102\u6027\u03c0-\u5171\u8f6d\u567b\u5429\u6865\u6269\u5c55\u5230NIR\u8fd1\u7ea2\u5916\u6ce2\u957f\u8303\u56f4\uff0c\u5e76\u4f7f\u5176\u6ee1\u8db3BBB\u7a7f\u900f\u6027\u6240\u9700\u7684\u4eb2\u8102\u6027\u9700\u6c42\uff0c\u8fdb\u4e00\u6b65\u901a\u8fc7\u6539\u53d8\u4eb2\u6c34\u6027\u78fa\u9178\u76d0\u57fa\u56e2\u7684\u53d6\u4ee3\u4f4d\u7f6e\uff0c\u4fdd\u8bc1\u7279\u5b9a\u7684\u4eb2\u6c34\u6027\u4f7f\u5206\u5b50\u5728\u7ed3\u5408A\u03b2\u6c89\u79ef\u4e4b\u524d\u5904\u4e8e\u5206\u6563\u6001\uff0c\u4ee5\u4fdd\u8bc1AIE\u63a2\u9488\u5728\u672a\u7ed3\u5408A\u03b2\u6591\u5757\u524d\u8367\u5149\u7ef4\u6301\u8367\u5149\u5173\u95edoff\u72b6\u6001\uff0c\u5c55\u793a\u4e86\u8fd1\u7ea2\u5916(NIR)\u805a\u96c6\u8bf1\u5bfc\u53d1\u5c04(AIE)-A\u03b2\u6591\u5757\u6d3b\u6027\u63a2\u9488\u7684\u5408\u7406\u8bbe\u8ba1\u7b56\u7565\u3002\u8fd1\u7ea2\u5916\u63a2\u9488QM-FN-SO3\u5df2\u7ecf\u5f88\u597d\u5730\u89e3\u51b3\u4e86AIE\u5728\u8f83\u957f\u53d1\u5c04\u7684\u4eb2\u8102\u6027\u8981\u6c42\u548c\u4ece\u6c34\u5230\u86cb\u767d\u8d28\u539f\u7ea4\u7ef4\u5f62\u6210\u7684\u805a\u96c6\u884c\u4e3a\u4e4b\u95f4\u7684\u95ee\u9898\uff0c\u4ece\u800c\u5728\u4f53\u5185\u68c0\u6d4b\u5177\u6709\u663e\u8457\u7ed3\u5408\u4eb2\u548c\u529b\u7684A\u03b2\u6591\u5757\u7684\u9ad8\u4fdd\u771f\u53cd\u9988\u65b9\u9762\u53d6\u5f97\u4e86\u7a81\u7834\uff0c\u53ef\u4ee5\u4f5c\u4e3a\u5546\u4e1a\u63a2\u9488ThT\u6216ThS\u7684\u6709\u6548\u66ff\u4ee3\u54c1\u3002\u8be5\u7814\u7a76\u6210\u679c\u4eca\u65e5\u4ee5\u9898\u4e3a\u201cRational Design of Near-Infrared Aggregation-Induced-EmissionActive Probes: In Situ Mapping of Amyloid\u2011\u03b2 Plaques with Ultrasensitivity and High-Fidelity<\/strong>\u201d\u53d1\u8868\u5728\u77e5\u540d\u671f\u520aJACS<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\uff1a\u5408\u7406\u8bbe\u8ba1\u8fdc\u7ea2\u5916AIE\u6fc0\u6d3b\u7684\u8367\u5149\u63a2\u9488\u7528\u4e8e\u68c0\u6d4bA\u03b2\u6c89\u79ef<\/strong><\/p>\n

\"\"<\/p>\n

(A) \u57fa\u4e8e\u5e38\u5f00\u6a21\u5f0f\u7684\u5546\u7528\u63a2\u9488ThT\uff1b
\n (B-C) \u201c\u9010\u6b65\u6cd5\u201d\u8bbe\u8ba1\u7684\u89e3\u51b3\u5546\u7528ThT\u56fa\u6709\u7f3a\u9677\u5e76\u521b\u5efa\u8d85\u654f\u611f\u7684NIR\u63a2\u9488\u3002<\/p>\n

\u56fe\u4e8c\uff1aQM-FN-SO3\u663e\u8457\u7684\u5149\u7269\u7406\u7279\u6027<\/strong><\/p>\n

\"\"<\/p>\n

(A)\u4e0d\u540c\u6eb6\u5242\u73af\u5883\u6761\u4ef6\u4e0b\u7684\u53d1\u5c04\u5149\u8c31\uff1b
\n (B)I\/I0\u7684\u53d8\u5316\uff1b
\n (C)\u9010\u6b65\u6ef4\u52a0A\u03b242\u805a\u96c6\u4f53\u65f6QM-FN-SO3\u7684\u8367\u5149\u5149\u8c31\uff1b
\n (D) QM-FN-SO3\u63a2\u9488\u4e0e\u65b0\u9c9c\u8001\u9f20\u8840\u6e05\u5b75\u80b220h\u5728720nm\u5904\u8367\u5149\u53d8\u5316\uff1b
\n (E)ICG\u3001ThT\u3001QM-FN-SO3\u4e09\u79cd\u63a2\u9488\u6301\u7eed\u5149\u7167\u7684\u7684\u7d2b\u5916\u5438\u6536\u53d8\u5316\uff1b
\n (F) \u5728A\u03b242\u805a\u96c6\u4f53\u54cd\u5e94\u5e73\u8861\u540e\uff0cI \/ I0\u968f\u4e0d\u540c\u6d53\u5ea6QM-FN-SO3\u3001QM-FN\u3001ThT\u3001DCM-N\u7684\u53d8\u5316\u56fe\u3002<\/p>\n

\u56fe\u4e09\uff1a\u5728\u6eb6\u6db2\u548c\u8111\u5207\u7247\u4e2d\u9ad8\u4fdd\u771fA\u03b2\u9a71\u52a8\u7684\u5373\u65f6NIR\u6548\u5e94<\/strong><\/p>\n

\"\"<\/p>\n

(A-B)QM-FN-SO3\u7684\u8d85\u9ad8S\/N\u6bd4\u7387\u7ec4\u5408\u80cc\u666f\u6700\u5c0f\u5316\u548c\u5bf9A\u03b242\u805a\u96c6\u4f53\u7684\u4fdd\u771f\u5ea6\u4fe1\u53f7\u653e\u5927\uff1b
\n (C)QM-FN-SO3\uff080-1\u03bcM\uff09\u6709\u6548\u5730\u4eceThT\/A\u03b242\u805a\u96c6\u590d\u5408\u7269\u4e2d\u7f6e\u6362ThT\u7a81\u51fa\u663e\u8457\u7684\u4eb2\u548c\u529b\uff1b
\n (D)\u5bf9A\u03b242\u805a\u96c6\u4f53\u9ad8\u6548\u7684\u9009\u62e9\u6027\uff1b
\n (E-J)\u5206\u522b\u4f7f\u7528ThS\u548cQM-FN-SO3\u5bf9\u6765\u81ea\u91ce\u751f\u578b\u5c0f\u9f20\u548c\u963f\u5c14\u8328\u6d77\u9ed8\u6c0f\u75c5\uff08AD\uff09-\u6a21\u578b\u5c0f\u9f20\u7684\u6d77\u9a6c\u533a\u57df\u4e2d\u7684\u8111\u5207\u7247\u8fdb\u884c\u7ec4\u7ec7\u5b66\u67d3\u8272\u6210\u50cf\uff1b
\n (K) \u8111\u5207\u7247\u7ebf\u6027\u76ee\u6807\u533a\u57df\uff08ROI\uff09\u7684\u5f3a\u5ea6\u5206\u5e03\uff1b
\n (L) DCM-N\uff0cQM-FN\u548cQM-FN-SO3\u7684S\/N\u6bd4\uff1b
\n (M-U)\u6765\u81eaAPP\/PS1\u5c0f\u9f20\u7684\u76f8\u90bb\u8111\u5207\u7247\u5206\u522b\u5728\u6d77\u9a6c\u533a\u57df\uff0c\u76ae\u8d28\u533a\u57df\u548c\u76ae\u8d28\u533a\u57df\u653e\u5927\u540e\uff0840x\uff09\u7528DCM-N\uff0cQM-FN\u548cQM-FNSO3\u67d3\u8272\uff1b
\n (V-W)\u5206\u522b\u5728\u9759\u8109\u5185\u6ce8\u5c04\u63a2\u9488QM-FN-SO3\u548cThT\uff082mg kg-1\uff095\u5206\u949f\u540e\u4ece\u91ce\u751f\u578b\u5c0f\u9f20\u7684\u8111\u7ec4\u7ec7\u4e2d\u63d0\u53d6\u7684\u9ad8\u5206\u8fa8\u7387\u8d28\u8c31\u3002<\/p>\n

\u56fe\u56db\uff1aAD\u6a21\u578b\u5c0f\u9f20\u6d3b\u4f53\u5185A\u03b2\u6a21\u5757\u6210\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

(A-D)\u91ce\u751f\u578b\u5408AD\u6a21\u578b\u5c0f\u9f20\u6ce8\u5c04QM-FN-SO3\u540e0\u5206\u949f\u548c20\u5206\u949f\u8111\u90e8\u6d3b\u4f53\u6210\u50cf\uff1b
\n (E-G) AD\u6a21\u578b\u5c0f\u9f20\u8111\u90e8\u5207\u7247\uff0840\u00d7\uff09\u6210\u50cf\uff0c\u7528\u6297\u4f532454\u67d3\u8272\u786e\u8ba4\u4ee5\u53ca\u5171\u805a\u6210\u50cf\u56fe\u50cf\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u603b\u4e4b\uff0c\u8be5\u5de5\u4f5c\u91cd\u70b9\u662f\u5982\u4f55\u5f00\u53d1\u8fd1\u7ea2\u5916 AIE\u6fc0\u6d3b\u7684\u63a2\u9488QM-FN-SO3\u4ee5\u907f\u514d\u5546\u4e1a\u63a2\u9488ThT\u548cThS\u7684\u56fa\u6709\u7f3a\u9677\uff0c\u4ee5\u6ee1\u8db3\u4f53\u5185\u68c0\u6d4bA\u03b2\u6591\u5757\u7684\u9ad8\u4fdd\u771f\u8981\u6c42\u3002\u5728\u201c\u9010\u6b65\u201d\u5408\u7406\u8bbe\u8ba1\u7b56\u7565\u4e2d\uff0c\u4f5c\u8005\u901a\u8fc7\u5f15\u5165\u4e86\u4eb2\u8102\u6027\u03c0-\u5171\u8f6d\u567b\u5429\u6865\uff0c\u7136\u540e\u5c06ACQ\u8367\u5149\u56e2\u66ff\u6362\u4e3aAIE\u7684\u55b9\u5549\u8148\u6bcd\u4f53\uff0c\u6700\u540e\u8c03\u6574\u78fa\u9178\u57fa\u56e2\u7684\u53d6\u4ee3\u4f4d\u7f6e\u3002\u56e0\u6b64\uff0c\u63a2\u9488QM-FNSO3\u540c\u65f6\u6d88\u9664\u4e86\u6765\u81eaThT\u7684\u81ea\u731d\u706d\u4fe1\u53f7\u548c\u6765\u81ea\u521d\u59cb\u805a\u96c6AIE\u63a2\u9488\u7684\u201c\u5047\u9633\u6027\u201d\u4fe1\u53f7\uff0c\u7136\u540e\u7ed3\u5408A\u03b2\u566c\u6591\u3002\u4f53\u5916\u548c\u4f53\u5185\u7684\u6d3b\u4f53\u52a8\u7269\u5b9e\u9a8c\u4e3aA\u03b2\u6591\u5757\u7684\u51c6\u786e\u53cd\u9988\u63d0\u4f9b\u4e86\u7684\u786e\u51ff\u8bc1\u636e\u3002\u4f5c\u8005\u9996\u6b21\u89e3\u51b3\u4e86\u03c0-\u5171\u8f6d\u7ed3\u6784\u5bf9\u8fd1\u7ea2\u5916\u53d1\u5c04\u548c\u805a\u96c6\u884c\u4e3a\u8981\u6c42\u4e4b\u95f4\u7684AIE\u56f0\u5883\uff0c\u901a\u8fc7\u7cbe\u786e\u8c03\u63a7\u5206\u5b50\u7684\u805a\u96c6\u72b6\u6001\uff0c\u5b9e\u73b0\u5bf9AD-\u6a21\u578b\u5c0f\u9f20\u5927\u8111\u4e2dA\u03b2\u6591\u5757\u7684\u51c6\u786e\u7ed3\u5408\u548c\u8fd1\u7ea2\u5916\u8367\u5149\u6807\u8bb0\uff0c\u5728A\u03b2\u6591\u5757\u7684\u9ad8\u4fdd\u771f\u68c0\u6d4b\u65b9\u9762\u53d6\u5f97\u4e86\u7a81\u7834\u3002\u63a2\u9488QM-FN-SO3\u5177\u6709\u8d85\u9ad8S\/N\u6bd4\u7684\u663e\u7740\u7279\u5f81\uff0c\u4e0eBBB\u6e17\u900f\u6027\u7684\u663e\u7740\u7ed3\u5408\u4eb2\u548c\u529b\u548c\u9ad8\u6027\u80fdNIR\u53d1\u5c04\u3002\u8be5\u7814\u7a76\u4e3aNIR AIE\u6d3b\u6027\u63a2\u9488\u7684\u8bbe\u8ba1\u63d0\u4f9b\u4e86\u4e00\u79cd\u6709\u524d\u666f\u7684\u7b56\u7565\uff0c\u53ef\u4f5c\u4e3a\u5546\u4e1a\u63a2\u9488\u5e02\u552e\u67d3\u6599ThT\/S\u7684\u6709\u6548\u66ff\u4ee3\u54c1\u8fdb\u884c\u66f4\u9ad8\u4fdd\u771f\u5ea6\u7684\u7ec4\u7ec7\u5b66\u67d3\u8272\uff0c\u4e3a\u4f53\u5185\u86cb\u767d\u8d28\u539f\u7ea4\u7ef4\u5f62\u6210\u7684\u53ef\u89c6\u5316\u94fa\u5e73\u4e86\u65b0\u7684\u9014\u5f84\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aRational Design of Near-Infrared Aggregation-Induced-EmissionActive Probes: In Situ Mapping of Amyloid\u2011\u03b2 Plaques with Ultrasensitivity and High-Fidelity<\/a> (JACS<\/em>, 2018<\/strong>, DOI: 10.1021\/jacs.8b12820)<\/p>\n

\u3010\u4f5c\u8005\u7b80\u4ecb\u3011<\/b><\/p>\n

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