{"id":173302,"date":"2019-04-30T06:30:19","date_gmt":"2019-04-29T22:30:19","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=173302"},"modified":"2019-04-29T18:58:14","modified_gmt":"2019-04-29T10:58:14","slug":"%e3%80%90%e5%9b%bd%e5%a4%96%e6%97%a0%e6%b3%95%e6%a0%a1%e7%a8%bf%e3%80%91manuel-tsotsalas%e5%8d%a1%e5%b0%94%e6%96%af%e9%b2%81%e5%8e%84%e7%90%86%e5%b7%a5%e5%ad%a6%e9%99%a2acc-chem-res-%ef%bc%9a","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=173302","title":{"rendered":"Manuel Tsotsalas\u5361\u5c14\u65af\u9c81\u5384\u7406\u5de5\u5b66\u9662Acc. Chem. Res.\uff1a\u91d1\u5c5e-\u6709\u673a\u9aa8\u67b6\u6a21\u677f\u7684\u751f\u7269\u6750\u6599\uff1a\u5408\u6210\u3001\u529f\u80fd\u5316\u548c\u5e94\u7528"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u591a\u5b54\u7ed3\u6676\u9aa8\u67b6\u4e0e\u8f6f\u805a\u5408\u7269\u7ed3\u5408\u7684\u65b0\u578b\u751f\u7269\u6750\u6599\u6709\u5f88\u5927\u5e94\u7528\u6f5c\u529b\uff0c\u4f46\u662f\u8fd9\u9879\u5de5\u4f5c\u975e\u5e38\u5177\u6709\u6311\u6218\u6027\u3002\u6839\u636e\u751f\u7269\u529f\u80fd\u8fdb\u884c\u5b9a\u5236\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6\uff08MOF\uff09\u6a21\u677f\u805a\u5408\u7269\uff08MTP\uff09\u4f5c\u4e3a\u6a21\u5757\u5316\u6750\u6599\uff0c\u7ed3\u5408\u4e86MOF\u7684\u4f18\u70b9\uff08\u7cbe\u786e\u63a7\u5236\u7684\u7ed3\u6784\u3001\u6846\u67b6\u62d3\u6251\u4e2d\u7684\u5de8\u5927\u591a\u6837\u6027\u548c\u9ad8\u5b54\u9699\u7387\uff09\u548c\u805a\u5408\u7269\u7684\u5185\u5728\u884c\u4e3a\uff08\u8d28\u5730\u67d4\u8f6f\u3001\u67d4\u97e7\u6027\u3001\u751f\u7269\u76f8\u5bb9\u6027\u548c\u751f\u7406\u6761\u4ef6\u4e0b\u7684\u7a33\u5b9a\u6027\u63d0\u9ad8\uff09\u3002\u901a\u8fc7\u6b63\u4ea4\u5171\u4ef7\u4ea4\u8054\u8f6c\u5316\u8868\u9762\u951a\u5b9a\u7684MOF\uff08Surmof\uff09\uff0c\u4ea7\u751f\u8868\u9762\u951a\u5b9a\u7684\u805a\u5408\u7269\u51dd\u80f6\uff08Surgel\uff09\uff0c\u5f00\u8f9f\u4e86\u83b7\u5f97\u8f6f\u7eb3\u7c73\u591a\u5b54\u6750\u6599\u7684\u65b0\u65b9\u6cd5\u3002\u672c\u6587\u603b\u7ed3\u4e86\u91d1\u5c5e-\u6709\u673a\u9aa8\u67b6\u6a21\u677f\u5316\u751f\u7269\u6750\u6599\u7684\u5408\u6210\u3001\u529f\u80fd\u5316\u548c\u5e94\u7528\u7684\u6700\u65b0\u8fdb\u5c55\uff1b\u5206\u6790\u4e86\u9650\u5236Surgel\u53d1\u5c55\u7684\u56e0\u7d20\uff1b\u6307\u660e\u4e86Surgel\u672a\u6765\u53d1\u5c55\u7684\u65b9\u5411\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5fb7\u56fd\u5361\u5c14\u65af\u9c81\u5384\u7406\u5de5\u5b66\u9662<\/strong>\u7684Manuel Tsotsalas<\/strong>\uff08\u901a\u8baf\uff09<\/strong>\u4f5c\u8005\u7b49\u4eba\uff0c\u91cd\u70b9\u4ecb\u7ecd\u5c06Surmof\u8f6c\u5316\u4e3a\u751f\u7269\u529f\u80fd\u5b9a\u5236\u7684\u6301\u4e45\u6a21\u5757\u5316\u7eb3\u7c73\u591a\u5b54\u6750\u6599\u7684\u7814\u7a76\u8fdb\u5c55\u3002\u4f7f\u7528\u7ec6\u80de\u57f9\u517b\u7814\u7a76Surgel\u6750\u6599\u7684\u5404\u4e2a\u65b9\u9762\uff0c\u4f8b\u5982\uff1a\u751f\u7269\u6d3b\u6027\u5206\u5b50\u9012\u9001\u5230Surgel\u8868\u9762\u4e0a\u7684\u7c98\u9644\u7ec6\u80de\u7684\u80fd\u529b\uff0c\u5e94\u7528\u4e8e\u836f\u7269\u9012\u9001\u7cfb\u7edf\uff1b\u8868\u9762\u4fee\u9970\u8c03\u8282\u7ec6\u80de\u7c98\u9644\u7684\u80fd\u529b\uff0c\u4ee5\u53ca\u535f\u5549\u5f00\u53d1Surgel\u8584\u819c\u7684\u6297\u83cc\u6027\u80fd\u3002\u7136\u540e\uff0c\u6279\u5224\u6027\u5730\u5206\u6790\u5f53\u524d\u65b9\u5411\u7684\u6311\u6218\u548c\u5c40\u9650\uff1b\u8ba8\u8bba\u4e86\u672a\u6765\u7684\u7814\u7a76\u65b9\u5411\uff1b\u603b\u7ed3\u4e86MOF\u6a21\u677f\u5316\u751f\u7269\u76f8\u5bb9\u6027\u6750\u6599\u7684\u65b0\u65b9\u6cd5\uff0c\u5f3a\u8c03\u9700\u8981\u4f53\u7cfb\u4e2d\u54cd\u5e94\u548c\u9002\u5e94\u6027\u529f\u80fd\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<\/strong>Metal\u2212organic framework-templated biomaterials: Recent progress in synthesis, functionalization, and applications<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Accounts Of Chemical Research<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong> 1 <\/strong>\u8bbe\u8ba1<\/strong>Surmof<\/strong>\u6a21\u677f\u5206\u5c42\u7ed3\u6784\u751f\u7269\u6750\u6599<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong> 2 <\/strong>\u81ea\u7ec4\u88c5\u5355\u5c42\uff08<\/strong>SAM<\/strong>\uff09\u4e0a\u7684\u6db2\u76f8\u5916\u5ef6\u9010\u5c42<\/strong>Surmof<\/strong>\u5408\u6210\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\u00a0\"\"<\/strong><\/p>\n

\u56fe<\/strong> 3\u00a0<\/strong>\u5185\u90e8\u8868\u9762\uff08\u5c0f\u5206\u5b50\u5728\u5b54\u4e2d\u6269\u6563\uff09\u548c\u5916\u8868\u9762\uff08\u8f83\u5927\u5206\u5b50\u9644\u7740\u5728\u5916\u8868\u9762\u4e0a\uff09\u7684<\/strong>MOF<\/strong>\u540e\u5408\u6210\u529f\u80fd\u5316\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong> 4 <\/strong>\u6709\u673a\u914d\u4f53\u7684\u7ed3\u6784\u5355\u5143\u6216\u5206\u5b50\u5f0f<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u53e0\u6c2e\u5316\u7269\u6216\u7094\u70c3\u6807\u8bb0\u4f5c\u4e3a\u7ed3\u6784\u5355\u5143\u7684\u4ee3\u8868\u6027\u7684\u6709\u673a\u914d\u4f53\uff1b<\/p>\n

\uff08b\uff09\u4e8c\u7ea7\u4ea4\u8054\u5242\uff08CL\uff09\u7684\u786b\u9187\u6216\u7094\u70c3\u6807\u8bb0\u7684\u5206\u5b50\u3002<\/p>\n

\u56fe<\/strong> 5 Surmof-Surgel<\/strong>\u53ca\u6b63\u4ea4\u5408\u6210\u805a\u5408\u65b9\u6cd5<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09Surmof-Surgel\u5408\u6210\u805a\u5408\u65b9\u6cd5\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u6b63\u4ea4\u529f\u80fd\u4f4d\u70b9\u3002\u4f8b\u5982\uff1a\u63a5\u5934\u9aa8\u67b6\u5185\u7684\u53e0\u6c2e\u5316\u7269\u548c\u70f7\u6c27\u57fa\uff0c\u4e0eCL\u5206\u5b50\u76f8\u4e92\u4f5c\u7528\uff0c\u70b9\u51fb\u53cd\u5e94\u673a\u5236\u5171\u4ef7\u4e92\u8fdeMOF\u7ed3\u6784\u3002<\/p>\n

\u56fe<\/strong> 6 MOF<\/strong>\u8f6c\u5316\u4e3a\u805a\u5408\u7269\u51dd\u80f6\uff1a<\/strong>AzoMOF<\/strong>\uff08<\/strong>AzM<\/strong>\uff09\u4ea4\u8054<\/strong>MOF<\/strong>\uff08<\/strong>CLM<\/strong>\uff09\u8f6c\u5316\u4e3a<\/strong>MOF<\/strong>\u6a21\u677f\u5316\u805a\u5408\u7269\uff08<\/strong>MTP<\/strong>\uff09<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong> 7 <\/strong>\u5206\u5b50\u7eba\u7ec7\u54c1\u7684\u5f62\u6210\u7b56\u7565<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong> 8 <\/strong>\u5149\u8bf1\u5bfc\u7684\u786b\u9187<\/strong>–<\/strong>\u7094\u70b9\u51fb\u6cd5\u5c06\u542b<\/strong>RGD<\/strong>\u7684\u5be1\u80bd\u63a5\u679d\u5230<\/strong>Surgel<\/strong><\/p>\n

\"\"<\/p>\n

\uff08\u5de6\uff09Surgel\u6846\u67b6\u7684\u65b9\u6848\uff1b<\/p>\n

\uff08\u53f3\uff09\u786b\u9187-\u7094\u70b9\u51fb\u8868\u9762\u6539\u6027\u7684Surgel\u3002<\/p>\n

\u56fe<\/strong> 9 Surmof<\/strong>\u7684\u94fe\u63a5\u548c\u8367\u5149\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u516d\u8fb9\u5f62\u56fe\u6848\u7684\u5149\u63a9\u6a21\u5c40\u90e8\u9650\u5236rhodamine-SH\u4e0eZn2<\/sub>(BA-BDC)2<\/sub>\uff08dabco\uff09Surmof\u7684\u8fde\u63a5\u4f53\u7684\u8fde\u63a5\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09Surmof\u7684\u8367\u5149\u663e\u5fae\u955c\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09Surgel\u8584\u819c\u7684\u8367\u5149\u663e\u5fae\u955c\u56fe\u50cf\uff1b<\/p>\n

\uff08d\uff09\u6cbf\u5782\u76f4\u4e8e\u7ebf\u7684\u8367\u5149\u5f3a\u5ea6\u8ff9\u7ebf\u3002<\/p>\n

\u56fe 10 \u9010\u5c42\u5f02\u8d28\u5916\u5ef6\u6cd5\uff0c\u5728\u78c1\u82af\u9897\u7c92\uff08MagMOF\uff09\u5468\u56f4MOF\u751f\u957f\u8bbe\u8ba1\u53ca\u6027\u80fd\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09Cu\u7684MOF\u751f\u957f\uff08BA-TPDC\uff09\uff1b<\/p>\n

\uff08b\uff09\u70b9\u51fb\u53cd\u5e94\u52a0\u8f7d\u84dd\u8272\u67d3\u6599\u5206\u5b50\uff1b<\/p>\n

\uff08c\uff09Cu\uff08TPDC\uff09\u7684MOF\u589e\u957f\uff1b<\/p>\n

\uff08d\uff09Cu\uff08BA-TPDC\uff09\u7684MOF\u589e\u957f\uff1b<\/p>\n

\uff08e\uff09\u70b9\u51fb\u53cd\u5e94\u52a0\u8f7d\u7ea2\u8272\u67d3\u6599\u5206\u5b50\uff1b<\/p>\n

\uff08f-g\uff09\u4e0d\u540c\u6ee4\u5149\u5668\u7684\u67d3\u6599\u5b98\u80fd\u5316\u7684\u591a\u58f3MOF\u6d82\u8986\u7eb3\u7c73\u9897\u7c92\u7684\u5171\u805a\u7126\u663e\u5fae\u955c\u56fe\u50cf\uff1a\u84dd\u8272\u901a\u9053\u3001\u3001\u7ea2\u8272\u901a\u9053\u548c\u7ea2\u8272\u548c\u84dd\u8272\u901a\u9053\u7684\u53e0\u52a0\u3002<\/p>\n

\u56fe<\/strong> 11 MagGel<\/strong>\u80f6\u56ca\u7684\u5236\u5907\u53ca\u5176\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08\u4e0a\uff09\u5206\u5c42\u7ed3\u6784\u7684\u58f3\u4e0a\u58f3MOF\u9897\u7c92\u53ca\u5176\u8f6c\u5316\u4e3aMagGel\u80f6\u56ca\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08\u4e0b\uff09\u901a\u8fc7\u53d1\u5c04\u5149\u8c31\u8bc1\u5b9e\uff0cpH\u5f15\u53d1\u7684\u6eb6\u80c0\u548c\u4eceMagGel\u80f6\u56ca\u4e2d\u91ca\u653e\u67d3\u6599\u7684\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe<\/strong> 12\u00a0<\/strong>\u5728<\/strong>Surgel<\/strong>\u57fa\u4f53\u4e0a\uff0c<\/strong>P. putida <\/em><\/strong>pJN::gfp<\/strong>\u7ec6\u83cc\u57f9\u517b<\/strong>24 h<\/strong>\u65f6\u540e\u7684\u793a\u610f\u56fe\u548c\u8367\u5149\u663e\u5fae\u955c\u56fe\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong> 13 <\/strong>\u535f\u5549<\/strong>Surmof<\/strong>\u5230<\/strong>Surgel<\/strong>\u7684\u7ed3\u6784\u548c\u6027\u80fd\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\uff08\u4e0a\uff09\u535f\u5549Surmof\u5230Surgel\u8f6c\u6362\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08\u4e0b\uff09\u535f\u5549\u5bf9\u5927\u80a0\u6746\u83cc\u7684\u6297\u83cc\u6f5c\u529b\u7684\u8584\u819c\u7684\u8367\u5149\u663e\u5fae\u955c\u56fe\u50cf\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\uff081\uff09\u9650\u5236\u3001\u529f\u80fd\u5316\u548c\u5e94\u7528\u7684\u56e0\u7d20<\/p>\n

Surgel\u65b9\u6cd5\u5177\u6709\u9ad8\u5ea6\u7075\u6d3b\u6027\uff0c\u80fd\u591f\u7528\u751f\u7269\u6d3b\u6027\u5206\u5b50\u52a0\u8f7d\u548c\u8868\u9762\u529f\u80fd\u5316\u5206\u5c42\u7ed3\u6784\u7684\u819c\uff0c\u6bcf\u4e2a\u9650\u5b9a\u7684\u4f4d\u7f6e\u5305\u542b\u591a\u4e2a\u6d3b\u6027\u7ec4\u5206\u3002\u5c3d\u7ba1Surgel\u751f\u7269\u6750\u6599\u53d6\u5f97\u4e86\u8fdb\u5c55\uff0c\u4f46\u5b83\u4eec\u4ecd\u7136\u5904\u4e8e\u8d77\u6b65\u9636\u6bb5\uff0c\u4ecd\u9650\u5236\u5176\u5728\u751f\u7269\u73af\u5883\u548c\u529f\u80fd\u5316\u4e2d\u7684\u5b9e\u9645\u6f5c\u529b\u7684\u67d0\u4e9b\u6311\u6218\u3002\u9700\u89e3\u51b3\u5f53\u524d\u7684\u5c40\u9650\u6027\uff1a\uff081\uff09\u9ad8\u901a\u91cf\u7b5b\u9009\u65b9\u6cd5\u5bf9MOF\u6a21\u677f\u6750\u6599\u7684\u7ed3\u6784-\u6d3b\u6027\/\u6bd2\u6027\u5173\u7cfb\u8fdb\u884c\u7cfb\u7edf\u7814\u7a76\uff1b\uff082\uff09Surgel\u6750\u6599\u5728\u7eb3\u7c73\u5668\u4ef6\u4e2d\u5b9e\u73b0\u6700\u4f73\u7684\u7269\u7406\u3001\u5316\u5b66\u548c\u67d0\u4e9b\u673a\u68b0\u6027\u80fd\u7684\u5de5\u4e1a\u751f\u4ea7\u65b9\u6cd5\uff1b\uff083\uff09\u5408\u6210\u5206\u5b50\u7ec4\u5206\u3001\u751f\u7269\u6d3b\u6027\u5316\u5408\u7269\u3001\u7eb3\u7c73\u548c\u5fae\u89c2\u7ed3\u6784\u592a\u5c0f\uff0c\u8ba1\u7b97\u65b9\u6cd5\u6765\u660e\u786e\u7ec4\u5206\u548c\u7ed3\u6784\u3002<\/p>\n

\uff082\uff09\u672a\u6765\u7684\u7814\u7a76\u65b9\u5411<\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Metal\u2212organic framework-templated biomaterials: Recent progress in synthesis, functionalization, and applications<\/strong><\/a>\uff08Accounts Of Chemical Research, 2019, DOI: 10.1021\/acs.accounts.9b00039\uff09\u3002<\/p>\n

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