{"id":173545,"date":"2019-04-24T06:30:59","date_gmt":"2019-04-23T22:30:59","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=173545"},"modified":"2019-04-23T11:57:48","modified_gmt":"2019-04-23T03:57:48","slug":"%e6%b9%96%e5%8d%97%e5%a4%a7%e5%ad%a6%ef%bc%9a%e6%b0%a2%e9%94%ae%e5%b7%a5%e7%a8%8b-%e8%b0%83%e6%8e%a7%e6%b0%ae%e5%8c%96%e7%a2%b3%e5%bd%a2%e8%b2%8c%e5%92%8c%e5%82%ac%e5%8c%96%e6%80%a7","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=173545","title":{"rendered":"\u6e56\u5357\u5927\u5b66\uff1a\u6c22\u952e\u5de5\u7a0b\u2014\u2014\u8c03\u63a7\u6c2e\u5316\u78b3\u5f62\u8c8c\u548c\u50ac\u5316\u6027\u80fd\u7684\u65b0\u7b56\u7565"},"content":{"rendered":"

\u3010<\/b><\/strong>\u5f15\u8a00<\/b><\/strong>\u3011<\/b><\/strong><\/p>\n

\u5c42\u72b6\u6750\u6599\u7531\u4e8e\u5176\u4f18\u5f02\u7684\u5149\u7535\u5316\u5b66\u6027\u8d28\u5728\u5149\u50ac\u5316\u5206\u89e3\u6c34\u4ea7\u6c22\u7b49\u9886\u57df\u5f97\u5230\u5e7f\u6cdb\u5e94\u7528\u3002\u901a\u8fc7\u7269\u7406\u6216\u8005\u5316\u5b66\u624b\u6bb5\u53ef\u4ee5\u5c06\u7d27\u5bc6\u5806\u79ef\u7684\u591a\u5c42\u7ed3\u6784\u5265\u79bb\u6210\u51e0\u5c42\u751a\u81f3\u5355\u5c42\u7eb3\u7c73\u7247\u7ed3\u6784\uff0c\u8d4b\u4e88\u4e86\u8fd9\u4e9b\u6750\u6599\u4e0d\u540c\u4e8e\u5757\u4f53\u7ed3\u6784\u7684\u7269\u7406\u5316\u5b66\u7279\u6027\u3002\u4f5c\u4e3a\u4e00\u7c7b\u65e0\u91d1\u5c5e\u7684\u4e8c\u7ef4\u6750\u6599\uff0c\u77f3\u58a8\u76f8\u6c2e\u5316\u78b3 (CN)\u00a0\u7531\u4e8e\u5176\u5408\u9002\u7684\u80fd\u5e26\u7ed3\u6784\u3001\u9002\u5f53\u7684\u5e26\u9699 (\u301c2.7 eV)\u3001\u65e0\u6bd2\u3001\u5ec9\u4ef7\u7b49\u6027\u8d28\u6210\u4e3a\u4e86\u8fd1\u51e0\u5e74\u5149\u50ac\u5316\u4ea7\u6c22\u9886\u57df\u4e2d\u7684\u65b0\u5ba0\u3002\u4e0e\u5757\u4f53\u7ed3\u6784\u76f8\u6bd4\uff0c\u8d85\u8584CN\u7eb3\u7c73\u7247\u5177\u6709\u8f83\u5927\u7684\u6bd4\u8868\u9762\u79ef\u3001\u5145\u5206\u66b4\u9732\u7684\u6d3b\u6027\u4f4d\u70b9\u3001\u5feb\u901f\u7684\u7535\u8377\u4f20\u8f93\u901f\u5ea6\u4ee5\u53ca\u66f4\u5927\u7684\u53ef\u89c1\u5149\u54cd\u5e94\u8303\u56f4\uff0c\u56e0\u6b64\uff0c\u8d85\u8584CN\u7eb3\u7c73\u7247\u88ab\u770b\u4f5c\u662f\u4e00\u79cd\u7406\u60f3\u7684\u5149\u50ac\u5316\u5242\u5e94\u7528\u4e8e\u5206\u89e3\u6c34\u4ea7\u6c22\u3002\u5c3d\u7ba1\u76ee\u524d\u8d85\u8584CN\u00a0\u7eb3\u7c73\u7247\u5236\u5907\u6280\u672f\u5df2\u7ecf\u8d8b\u4e8e\u6210\u719f\uff0c\u4f46\u5176\u5236\u5907\u624b\u6bb5\u5f80\u5f80\u5c40\u9650\u4e8e\u6db2\u76f8\u8d85\u58f0\u5265\u79bb\u548c\u70ed\u6c27\u5316\u5265\u79bb\uff08\u7834\u574f\u5c42\u95f4\u8303\u5fb7\u74e6\u5c14\u65af\u529b\uff09\uff0c\u5982\u4f55\u901a\u8fc7\u8c03\u8282CN\u00a0\u9aa8\u67b6\u5185\u5316\u5b66\u952e\u5b9e\u73b0\u8d85\u8584\u7eb3\u7c73\u7247\u7684\u5236\u5907\u4ecd\u7136\u662f\u4e00\u4e2a\u5de8\u5927\u7684\u6311\u6218\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6e56\u5357\u5927\u5b66\u9ec4\u7ef4\u6e05\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u548c\u674e\u6ce2\u535a\u58eb\uff08\u7b2c\u4e00\u4f5c\u8005\uff09\uff0c\u4e0e\u8fbd\u5b81\u5927\u5b66\u8303\u6653\u661f\u6559\u6388\u5408\u4f5c<\/strong>\uff0c\u63d0\u51fa\u5229\u7528\u6c22\u952e\u5de5\u7a0b\u2014\u2014\u901a\u8fc7\u5c06\u975e\u91d1\u5c5e\u539f\u5b50B\/P\u63ba\u6742\u4e8eCN \u9aa8\u67b6\u5185\u7279\u5b9a\u4f4d\u7f6e\uff0c\u4ece\u800c\u9009\u62e9\u6027\u7834\u574fCN \u9aa8\u67b6\u5185\u90e8\u5206\u6c22\u952e\u2014\u2014\u5236\u5907\u4e86\u5177\u6709\u4f18\u5f02\u50ac\u5316\u6027\u80fd\u7684\u8d85\u8584CN\u7eb3\u7c73\u7247\u3002\u7814\u7a76\u4eba\u5458\u53d1\u73b0CN\u805a\u5408\u7269\u5185\u7684\u6c22\u952e\u548c\u8303\u5fb7\u74e6\u5c14\u65af\u529b\u5f71\u54cd\u4e86\u5176\u6700\u7ec8\u7684\u5fae\u89c2\u7ed3\u6784\u548c\u7269\u7406\u5316\u5b66\u529f\u80fd\uff1b\u4e0e\u5176\u4ed6\u4ec5\u4ec5\u53ea\u542b\u6709\u5171\u4ef7\u952e\u7684\u5c42\u72b6\u6750\u6599\u76f8\u6bd4\uff0c\u5728CN\u5c42\u5185\u5468\u671f\u6027\u8fde\u63a5\u5355\u5143\u5b58\u5728\u5927\u91cf\u7531NH\/NH2<\/sub>\u5f62\u6210\u7684\u6c22\u952e\uff0c\u800c\u6c22\u952e\u533a\u57df\u7684\u5de8\u5927\u52bf\u5792\u4e25\u91cd\u963b\u788d\u4e86\u7535\u5b50\u5728\u5c42\u4e4b\u95f4\u7684\u8fc1\u79fb\u3002\u56e0\u6b64\uff0c\u6c22\u952e\u5de5\u7a0b<\/b><\/strong>\uff08\u9009\u62e9\u6027\u8c03\u63a7\u6c22\u952e\uff09\u53ef\u4ee5\u4f5c\u4e3a\u4e00\u79cd\u9ad8\u6548\u7684\u7b56\u7565\u8c03\u63a7CN\u5fae\u89c2\u7ed3\u6784\u548c\u50ac\u5316\u6027\u80fd\u3002\u7814\u7a76\u4eba\u5458\u8bc1\u660e\u901a\u8fc7\u5143\u7d20\u63ba\u6742\u9009\u62e9\u6027\u7834\u574f\u6c22\u952e\u4f7f\u5f97CN\u540c\u65f6\u5177\u6709\u4e8c\u7ef4\u8d85\u8584\u7247\u72b6\u7ed3\u6784\u3001\u4f18\u5f02\u7684\u7535\u8377\u4f20\u8f93\u548c\u5206\u79bb\u6548\u7387\uff0c\u66f4\u591a\u7684\u6d3b\u6027\u8fb9\u7f18\u4f4d\u70b9\u3002\u7406\u8bba\u8ba1\u7b97\u548c\u5b9e\u9a8c\u7ed3\u679c\u5747\u8868\u660e\u9009\u62e9\u6027\u7834\u574f\u6c22\u952e\u53ef\u4ee5\u6709\u6548\u5730\u51cf\u5c0fCN\u7684\u5e26\u9699\uff0c\u589e\u5f3a\u53ef\u89c1\u5149\u54cd\u5e94\u8303\u56f4\u3002\u7531\u4e8e\u8fd9\u4e9b\u4f18\u5f02\u7684\u7279\u6027\uff0c\u5728\u6ce2\u957f\u5927\u4e8e400 nm\u7684\u53ef\u89c1\u5149\u7167\u5c04\u4e0b\uff0cB\/P-CNNs\u50ac\u5316\u5242\u7684\u4ea7\u6c22\u6548\u7387\u8fbe\u5230\u4e8610877.40 \u03bcmol h\u2212<\/sup>1 g\u22121<\/sup>, \u91cf\u5b50\u4ea7\u7387\u4e3a7.55%\uff0c\u8fdc\u9ad8\u4e8e\u5927\u591a\u6570\u62a5\u9053\u7684CN\u50ac\u5316\u5242\u3002\u8be5\u5de5\u4f5c\u63d0\u51fa\u7684\u6c22\u952e\u5de5\u7a0b<\/strong>\u7b56\u7565\uff0c\u4e5f\u53ef\u4ee5\u5b9e\u73b0\u5176\u4ed6\u542b\u6c22\u952e\u805a\u5408\u7269\u7684\u5fae\u89c2\u5f62\u8c8c\u8c03\u63a7\u53ca\u529f\u80fd\u8bbe\u8ba1\u3002\u76f8\u5173\u7ed3\u679c\u5df2\u5728\u77e5\u540d\u671f\u520aACS Applied Materials & Interfaces (DOI: 10.1021\/acsami.8b22366)\u4e0a\u53d1\u8868\uff0c\u9898\u4e3a\u201cDoping-Induced Hydrogen-Bond Engineering in Polymeric Carbon Nitride To Significantly Boost the Photocatalytic H2<\/sub>\u00a0Evolution\u00a0Performance\u201d<\/p>\n

\"\"<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe<\/b><\/strong>1.<\/b><\/strong>\u00a0\u6c22\u952e\u5de5\u7a0b<\/b><\/strong>\u5265\u79bbC<\/b><\/strong>N\uff1a\u5757\u4f53\u7ed3\u6784<\/b><\/strong>CN<\/b><\/strong>\u8f6c\u6362\u4e3a\u8d85\u8584<\/b><\/strong>B\/P-CNNs<\/b><\/strong>\u7ed3\u6784\u793a\u610f\u56fe\uff08\u6c22\u539f\u5b50\u3001\u787c\u539f\u5b50\u3001\u78b3\u539f\u5b50\u3001\u6c2e\u539f\u5b50\u548c\u78f7\u539f\u5b50\u5206\u522b\u7528\u9ec4\u8272\u3001\u7c89\u8272\u3001\u7eff\u8272\u3001\u84dd\u8272\u548c\u7ea2\u8272\u7684\u7403\u4f53\u8868\u793a\uff09<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u56fe2. B\/P-CNNs<\/b><\/strong>\u00a0\u5149\u50ac\u5316\u5242\u5236\u5907\u8fc7\u7a0b\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

\u8fd9\u79cd\u8d85\u8584\u787c\/\u78f7\u5171\u63ba\u6742\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247(B\/P-CNNs)\u4e3b\u8981\u5236\u5907\u8fc7\u7a0b\u5982\u4e0b\uff1a<\/p>\n

1.\u901a\u8fc7\u6c34\u70ed\u7f29\u5408\u53cd\u5e94\u5236\u5907\u524d\u9a71\u4f53\uff1a\u787c\u9178 (B\u6e90)\u548c\u4e09\u805a\u6c30\u80fa(C, N \u6e90)\u6df7\u5408\u6405\u62cc\u6eb6\u89e3\u540e\uff0c\u52a0\u5165\u9002\u91cf\u7684\u78f7\u9178\uff08P\u6e90\uff09\u76f4\u81f3\u5f62\u6210\u900f\u660e\u6eb6\u6db2\u3002\u5c06\u6df7\u5408\u6eb6\u6db2\u7f6e\u5165\u53cd\u5e94\u91dc\u4e2d\u5e76\u5728180\u2103\u7684\u6e29\u5ea6\u4e0b\u4fdd\u630110 h\u3002<\/p>\n

2.\u70ed\u7f29\u805a\u53cd\u5e94\u751f\u6210B\/P-CNNs:\u5c06\u6c34\u70ed\u53cd\u5e94\u540e\u7684\u524d\u9a71\u4f53\u7f6e\u5165\u9676\u74f7\u5769\u57da\u5185\u5e76\u5728550\u2103\u7684\u6e29\u5ea6\u4e0b\u4fdd\u63012 h\uff0c\u5f85\u6837\u54c1\u51b7\u5374\u81f3\u5ba4\u6e29\uff0c\u6700\u7ec8\u5f97\u5230\u8d85\u8584\u787c\/\u78f7\u5171\u63ba\u6742\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247(B\/P-CNNs)\u3002<\/p>\n

\u56fe3<\/b><\/strong>. <\/b><\/strong>CN\u4ee5\u53ca\u63ba\u6742B<\/b><\/strong>,P\u5143\u7d20\u50ac\u5316\u5242<\/b><\/strong>\u5fae\u89c2\u7ed3\u6784\u6f14\u53d8\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a) CN\u6837\u54c1\u7684SEM\u56fe\u50cf(\u5757\u4f53\u7ed3\u6784)\uff1b<\/p>\n

b,) P-CN\u6837\u54c1\u7684SEM\u56fe\u50cf(\u7247\u72b6\u7ed3\u6784)\uff1b<\/p>\n

c,) B-CN\u6837\u54c1\u7684SEM\u56fe\u50cf(\u7247\u72b6\u7ed3\u6784)\uff1b<\/p>\n

d,) B\/P-CNNs\u6837\u54c1\u7684SEM\u56fe\u50cf(\u8d85\u8584\u7247\u72b6\u7ed3\u6784)\uff1b<\/p>\n

e, f) B\/P-CNNs\u6837\u54c1\u7684AFM\u56fe\u50cf\u4ee5\u53ca\u539a\u5ea6\u5206\u5e03\u56fe\uff1b<\/p>\n

g, h) B\/P-CNNs\u6837\u54c1\u7684TEM\u56fe\u50cf\u3002<\/p>\n

\u56fe<\/b><\/strong>4. <\/b><\/strong>CN<\/b><\/strong>\u4ee5\u53ca\u63ba\u6742<\/b><\/strong>B, P<\/b><\/strong>\u5143\u7d20<\/b><\/strong>\u50ac\u5316\u5242\u5143\u7d20\u6210\u5206\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a, b,) CN, P-CN, B-CN\u4ee5\u53caB\/P-CNNs\u50ac\u5316\u5242\u7684XRD\u548cFT-IR\u8868\u5f81\u56fe\u8c31\uff1b<\/p>\n

c,) B\/P-CNNs\u50ac\u5316\u5242\u7684\u7ed3\u5408\u80fd\u56fe\u8c31\uff1b<\/p>\n

d, e) B\/P-CNNs\u50ac\u5316\u5242\u7684B\u00a01s \u548cP\u00a02p \u56fe\u8c31\uff1b<\/p>\n

f) B\/P-CNNs\u50ac\u5316\u5242\u7684C1s(\u5de6) \u548cN 1s (\u53f3) \u56fe\u8c31\u3002<\/p>\n

\u56fe<\/b><\/strong>5. <\/b><\/strong>CN<\/b><\/strong>\u4ee5\u53ca\u63ba\u6742<\/b><\/strong>B, P<\/b><\/strong>\u5143\u7d20\u50ac\u5316\u5242<\/b><\/strong>\u5149\u5b66\u53ca\u80fd\u5e26\u6027\u8d28\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a, ) CN\u53ca\u63ba\u6742B\uff0cP\u5143\u7d20\u50ac\u5316\u5242\u7684\u5438\u6536\u5149\u8c31\u8868\u5f81\uff1b<\/p>\n

b,) CN\u53ca\u63ba\u6742B\uff0cP\u5143\u7d20\u50ac\u5316\u5242\u7684PL\u5149\u8c31\u8868\u5f81\uff1b<\/p>\n

c) CN\u53caB\/P-CNNs\u50ac\u5316\u5242\u7684\u80fd\u5e26\u7ed3\u6784\uff1b<\/p>\n

d) CN\u53ca\u63ba\u6742B\uff0cP\u5143\u7d20\u50ac\u5316\u5242\u7684\u65f6\u95f4\u5206\u8fa8\u5149\u8c31\u8868\u5f81\u3002<\/p>\n

\u56fe<\/b><\/strong>6. <\/b><\/strong>CN<\/b><\/strong>\u4ee5\u53ca\u63ba\u6742<\/b><\/strong>B, P<\/b><\/strong>\u5143\u7d20\u50ac\u5316\u5242<\/b><\/strong>DFT<\/b><\/strong>\u8ba1\u7b97<\/b><\/strong><\/p>\n

\"\"<\/p>\n

HOMO\u7684\u80fd\u5e26\u7ed3\u6784\u548c\u7535\u5b50\u5bc6\u5ea6\u5206\u5e03(\u7eff\u8272)\u548cLUMO(\u7c89\u8272)DFT\u8ba1\u7b97<\/p>\n

a)CN;<\/p>\n

b-f)\u00a0B\/P-CNNs\u3002<\/p>\n

\u56fe<\/b><\/strong>7. <\/b><\/strong>CN<\/b><\/strong>\u53ca\u63ba\u6742<\/b><\/strong>B, P<\/b><\/strong>\u5143\u7d20\u50ac\u5316\u5242<\/b><\/strong>\u7535\u5316\u5b66<\/b><\/strong>\u548c\u5149\u50ac\u5316\u4ea7\u6c22\u6027\u80fd\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a, b,) CN, P-CN, B-CN\u4ee5\u53caB\/P-CNNs\u50ac\u5316\u5242\u7684\u963b\u6297\u53ca\u5149\u7535\u6d41\u8868\u5f81\u56fe\u8c31\uff1b<\/p>\n

c,) CN \u53caB\/P-CNNs\u50ac\u5316\u5242\u5728\u53ef\u89c1\u5149\u4e0b\u4ea7\u6c22\u6027\u80fd\u5bf9\u6bd4\u00a0(\u03bb>400 nm)\uff1b<\/p>\n

d) B\/P-CNNs\u50ac\u5316\u5242\u7684\u4ea7\u6c22\u5faa\u73af\u56fe\u8c31\u3002<\/p>\n

\u56fe<\/b><\/strong>8. <\/b><\/strong>CN<\/b><\/strong>\u53ca\u63ba\u6742<\/b><\/strong>B, P<\/b><\/strong>\u5143\u7d20\u50ac\u5316\u5242\u5149\u50ac\u5316<\/b><\/strong>\u964d\u89e3<\/b><\/strong>\u6709\u673a\u67d3\u6599\u6027\u80fd\u8868\u5f81<\/b><\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

CN, P-CN, B-CN\u4ee5\u53caB\/P-CNNs\u50ac\u5316\u5242\u53ef\u89c1\u5149 (300 W \u5364\u7d20\u706f)\u00a0\u4e0b\u964d\u89e3\u6709\u673a\u67d3\u6599\u6027\u80fd\u8868\u5f81 a, b) \u7532\u57fa\u84dd\uff1b<\/p>\n

c, d) \u7532\u57fa\u6a59\uff1b<\/p>\n

e, f) \u82ef\u915a\u3002<\/p>\n

\u56fe<\/b><\/strong>9<\/b><\/strong>.<\/b><\/strong>\u00a0B\/P-CNNs<\/b><\/strong>\u50ac\u5316\u5242\u5149\u50ac\u5316\u5236\u6c22\u4ee5\u53ca\u6709\u673a\u67d3\u6599\u964d\u89e3\u673a\u7406<\/b><\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

\u3010<\/b><\/strong>\u5c0f\u7ed3<\/b><\/strong>\u3011<\/b><\/strong><\/p>\n

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\u6587\u7ae0\u94fe\u63a5\uff1a<\/b><\/strong>Doping-Induced Hydrogen-Bond Engineering in Polymeric Carbon Nitride To Significantly Boost the Photocatalytic H2<\/sub>\u00a0Evolution\u00a0Performance\u00a0(ACS Applied Materials & Interfaces<\/a>,\u00a0https:\/\/pubs.acs.org.ccindex.cn\/doi\/abs\/10.1021\/acsami.8b22366)<\/p>\n

\u672c\u6587\u7531\u4f5c\u8005\u4f9b\u7a3f<\/strong>\uff0c\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u7f16\u8f91\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaorenVIP.<\/p>\n","protected":false},"excerpt":{"rendered":"

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