{"id":176633,"date":"2019-06-03T06:59:09","date_gmt":"2019-06-02T22:59:09","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=176633"},"modified":"2019-06-02T20:59:47","modified_gmt":"2019-06-02T12:59:47","slug":"%e4%b8%ad%e7%a7%91%e5%a4%a7%e5%8d%97%e6%b4%8b%e7%90%86%e5%b7%a5-adv-mater-mof%e8%a1%8d%e7%94%9f%e7%9a%84%e4%bb%8b%e5%ad%94%e7%ba%b3%e7%b1%b3%e9%85%b6%e4%ba%a7%e7%94%9f%e6%b0%a7%e6%b0%94%e7%94%a8","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=176633","title":{"rendered":"\u4e2d\u79d1\u5927&\u5357\u6d0b\u7406\u5de5 Adv. Mater.: MOF\u884d\u751f\u7684\u4ecb\u5b54\u7eb3\u7c73\u9176\u4ea7\u751f\u6c27\u6c14\u7528\u4e8e\u7f13\u89e3\u80bf\u7624\u7f3a\u6c27\uff0c\u663e\u8457\u7684\u589e\u5f3a\u5149\u52a8\u529b\u7597\u6cd5"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u5149\u52a8\u529b\u7597\u6cd5\uff08PDT\uff09\u662f\u4e00\u79cd\u6d89\u53ca\u5149\u654f\u5242\u548c\u5206\u5b50\u6c27\uff08O2<\/sub>\uff09\u7684\u4ea7\u751f\u6d3b\u6027\u6c27\u7684\u4e34\u5e8a\u6cbb\u7597\u6a21\u5f0f\uff0c\u73b0\u5df2\u88ab\u8bc1\u660e\u662f\u4e00\u79cd\u7279\u5f02\u6027\u7684\u5e7f\u8c31\u6cbb\u7597\u764c\u75c7\u6216\u5176\u4ed6\u75be\u75c5\u7684\u65b9\u6cd5\u3002PDT\u4e5f\u53ef\u4ee5\u8bf1\u5bfc\u80bf\u7624\u4e2d\u7684\u8840\u7ba1\u635f\u4f24\uff0c\u5e76\u6fc0\u6d3b\u514d\u75ab\u7cfb\u7edf\u7684\u53cd\u5e94\u3002\u5bf9\u6bd4\u5316\u7597\u3001\u653e\u7597\u548c\u624b\u672f\u7b49\u4f20\u7edf\u6cbb\u7597\u65b9\u6cd5\uff0c\u6709\u6c27\u6c14\u53c2\u4e0e\u7684PDT\u53ef\u663e\u7740\u63d0\u9ad8\u9009\u62e9\u6027\u5e76\u51cf\u5c11\u526f\u4f5c\u7528\uff0c\u540c\u65f6\u63d0\u9ad8PDT\u7684\u6cbb\u7597\u6548\u679c\u3002\u7136\u800c\uff0cPDT\u5f15\u8d77\u7684\u5fae\u8840\u7ba1\u584c\u9677\u5c06\u635f\u5bb3\u6c27\u6c14\u4f9b\u5e94\u5e76\u52a0\u91cd\u7f3a\u6c27\u72b6\u51b5\uff0c\u4ece\u800c\u964d\u4f4ePDT\u7684\u6cbb\u7597\u6548\u679c\u3002\u76ee\u524d\uff0c\u4e3b\u8981\u6709\u4e09\u79cd\u7b56\u7565\u6765\u514b\u670d\u7f3a\u6c27\u95ee\u9898\u5e76\u6539\u5584PDT\u7684\u6cbb\u7597\u3002\u5176\u4e2d\u4e00\u79cd\u901a\u7528\u65b9\u6cd5\u662f\u5c06PDT\u540c\u5176\u4ed6\u6cbb\u7597\u624b\u6bb5\u7ed3\u5408\u5b9e\u73b0\u534f\u540c\u6cbb\u7597\uff0c\u4f46\u662f\u8fd9\u9650\u5236\u4e86\u5b83\u4eec\u7684\u53ef\u6269\u5c55\u6027\u548c\u518d\u73b0\u6027\u3002\u53e6\u4e00\u79cd\u65b9\u6cd5\u662f\u5229\u7528\u667a\u80fd\u7eb3\u7c73\u6750\u6599\u5145\u5f53\u6c27\u6c14\u8f7d\u4f53\u5c06\u6c27\u6c14\u5206\u5b50\u76f4\u63a5\u8f93\u9001\u5230\u80bf\u7624\u90e8\u4f4d\u3002\u8fd8\u6709\u4e00\u79cd\u5c31\u662f\u57fa\u4e8e\u80bf\u7624\u5fae\u73af\u5883\u7684\u7279\u5f81\u6784\u5efa\u667a\u80fd\u7eb3\u7c73\u5e73\u53f0\uff0c\u5728\u5b9e\u4f53\u80bf\u7624\u5185\u539f\u4f4d\u751f\u6210\u6c27\u6c14\u3002\u4f46\u662f\u8fd9\u4e9b\u65b9\u6cd5\u90fd\u5404\u81ea\u5b58\u5728\u76f8\u5e94\u7684\u7f3a\u70b9\uff0c\u56e0\u6b64\u8feb\u5207\u9700\u8981\u6784\u5efa\u4e00\u79cd\u751f\u7269\u76f8\u5bb9\u6027\u6cbb\u7597\u7cfb\u7edf\u65e2\u80fd\u5b9e\u73b0\u9ad8\u6548\u50ac\u5316O2<\/sub>\u7684\u4ea7\u751f\uff0c\u53c8\u80fd\u5b9e\u73b0\u53ef\u6301\u7eed\u7684O2<\/sub>\u4f9b\u7ed9\uff0c\u4ea7\u751f\u66f4\u591a\u7ec6\u80de\u6bd2\u60271<\/sup>O2<\/sub>\u4ee5\u589e\u5f3aPDT\u6548\u679c\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5357\u6d0b\u7406\u5de5\u5927\u5b66\u8d75\u5f66\u5229\u6559\u6388\u8bfe\u9898\u7ec4\u548c\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u9648\u4e7e\u65fa\u6559\u6388\u3001\u4ee5\u53ca\u90ed\u632f\u526f\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u5171\u540c\u62a5\u9053\u4e86\u4e00\u79cd\u4ece\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6\uff08MOFs\uff09\u4e2d\u63d0\u53d6\u7684\u591a\u529f\u80fd\u4ecb\u5b54\u7eb3\u7c73\u9176\uff08NE\uff09\uff0c\u7528\u4e8e\u539f\u4f4d\u751f\u6210\u5185\u6e90\u6027O2<\/sub>\uff0c\u63d0\u9ad8PDT\u6cbb\u7597\u6548\u7387\u3002\u4ecb\u5b54\u6c27\u5316\u9176NE\u662f\u5728\u9530\u57faMOFs\u8868\u9762\u6d82\u8986\u4ecb\u5b54\u4e8c\u6c27\u5316\u7845\uff0c\u63a5\u7740\u5728\u5e38\u6e29\u4e0b\u8fdb\u884c\u7b80\u5355\u7684\u9000\u706b\u5904\u7406\u800c\u5236\u6210\u3002\u5728\u53bb\u9664\u4ecb\u5b54\u4e8c\u6c27\u5316\u7845\u5916\u58f3\u540e\uff0c\u7528\u805a\u591a\u5df4\u80fa\u548c\u805a\u4e59\u4e8c\u9187\u5bf9\u5176\u8fdb\u884c\u540e\u5904\u7406\uff0c\u63d0\u9ad8NE\u7684\u751f\u7269\u76f8\u5bb9\u6027\uff0c\u5e76\u8d1f\u8f7d\u4e86\u5e38\u7528\u7684\u5149\u654f\u5242Ce6\u3002\u901a\u8fc7\u50ac\u5316\u91cfNE\u4e0e\u5185\u6e90\u6027H2<\/sub>O2<\/sub>\u7684\u50ac\u5316\u53cd\u5e94\u751f\u6210O2<\/sub>\u540e\uff0c\u7f13\u89e3\u4e86\u80bf\u7624\u5fae\u73af\u5883\u7f3a\u6c27\u60c5\u51b5\u3002\u6b64\u5916\uff0cCe6\u8d1f\u8f7d\u7684NE\u53ef\u4f5c\u4e3a\u4ea7\u751f\u6c27\u6c14\u7684\u4f9b\u4f53\uff0c\u7528\u4e8e\u589e\u52a0\u5c40\u90e8O2<\/sub>\u6d53\u5ea6\uff0c\u663e\u8457\u63d0\u9ad8\u4f53\u5185\u5916\u6297\u80bf\u7624PDT\u6cbb\u7597\u6548\u679c\u3002\u8be5\u7814\u7a76\u63d0\u51fa\u4e86\u4e00\u4e2a\u6709\u6548\u7684\u751f\u7269\u533b\u5b66\u5e94\u7528\u7684MOF\u884d\u751f\u7684\u4ecb\u5b54NE\u4f5c\u4e3a\u591a\u529f\u80fd\u8bca\u7597\u5242\u7528\u4e8e\u764c\u75c7\u8bca\u65ad\u548c\u6cbb\u7597\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cA Mesoporous Nanoenzyme Derived from Metal\u2013Organic Frameworks with Endogenous Oxygen Generation to Alleviate Tumor Hypoxia for Signifcantly Enhanced Photodynamic Therapy\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aAdv. Mater.<\/strong>\u4e0a\u3002
\n \"\"
\n \u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001MCOPP-NE\u7684\u5408\u6210\u53ca\u5176\u7ed3\u6784\u548c\u6027\u8d28\u7684\u8868\u5f81<\/strong>
\n \"\"\uff08a\uff09\u5236\u5907MCOPP-NE\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09MCOPP-NE\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09\u4f5c\u4e3aMn\u6d53\u5ea6\u51fd\u6570\u76841\/T2<\/sub><\/em>\u7684\u56fe\uff1b<\/p>\n

\uff08d\uff09\u5728PBS\u4e2d\u7528MCOPP-NE\u5904\u7406\u540e\u4ea7\u751fO2<\/sub>\uff1b<\/p>\n

\uff08e\uff09\u6709\u548c\u65e0MCOPP-NE\u7684H2<\/sub>O2<\/sub>\u964d\u89e3\uff1b<\/p>\n

\uff08f\uff09\u5728MCOPP-NE\u5b58\u5728\u4e0bH2<\/sub>O2<\/sub>-Ti(SO4<\/sub>)2<\/sub>\u6eb6\u6db2\u7684\u76f8\u5e94\u5438\u6536\u5149\u8c31\uff1b<\/p>\n

\uff08g\uff09\u91cd\u590d\u52a0\u5165H2<\/sub>O2<\/sub>\uff0cMCOPP-NE\u7684\u91cd\u590d\u50ac\u5316\u80fd\u529b\uff1b<\/p>\n

\uff08h\uff09\u5728671 nm\u6fc0\u5149\u7167\u5c0410 s\u540e\uff0c\u5728\u4e0d\u540c\u6761\u4ef6\u4e0b\u88abTEMP\u6355\u83b7\u76841<\/sup>O2<\/sub>\u7684ESR\u5149\u8c31\uff1b<\/p>\n

\uff08i\uff09\u5728671 nm\u6fc0\u5149\u7167\u5c04\u4e4b\u524d\u548c\u4e4b\u540e\uff0c\u5728\u5404\u79cd\u6761\u4ef6\u4e0b\u7531DPBF\u6d4b\u5b9a\u76841<\/sup>O2<\/sub>\u4ea7\u751f\u6548\u7387\u3002<\/p>\n

\u56fe\u4e8c\u3001MCOPP-NE\u7684\u4f53\u5916\u6cbb\u7597<\/strong>
\n \"\"\uff08a\uff09\u7528\u4e0d\u540c\u6d53\u5ea6\u7684MCOPP-NE\u5bf94T1\u7ec6\u80de\u7684\u6bd2\u6027\uff1b<\/p>\n

\uff08b, c\uff09\u5728671 nm\u6fc0\u5149\u7167\u5c04\u4e4b\u524d\u548c\u4e4b\u540e\u5728\u6b63\u5e38\u6c27\u6c14\uff08b\uff09\u548c\u4f4e\u6c27\u6c14\uff08c\uff09\u73af\u5883\u4e2d\u4e0d\u540c\u6761\u4ef6\u4e0b\u5bf94T1\u7ec6\u80de\u7684\u6bd2\u6027\uff1b<\/p>\n

\uff08d\uff09\u5e38\u6c27\u6c14\u548c\u4f4e\u6c27\u6c14\u6761\u4ef6\u4e0b\u7528PBS\u3001\u6e38\u79bbCe6\u548cMCOPP-Ce6\u5904\u7406\u540e\u7684\u7ec6\u80de\u7684\u6d3b\/\u6b7b\u67d3\uff1b<\/p>\n

\uff08e\uff09\u7531O2<\/sub>\u6307\u793a\u5242\u67d3\u8272\u76844T1\u7ec6\u80de\u7684CLSM\u56fe\u50cf\uff1b<\/p>\n

\uff08f\uff09\u7528MCOPP-NE\u5904\u7406\u540e\uff0c4T1\u7ec6\u80de\u4e2dHIF-1\u03b1\u8868\u8fbe\u7684Western\u5370\u8ff9\uff1b<\/p>\n

\uff08g\uff09\u5728\u6b63\u5e38\u6c27\u6c14\u548c\u7f3a\u6c27\u6c14\u6761\u4ef6\u4e0b\u4e0eMCOPP-NE\u5b75\u80b2\u7684\u7ec6\u80de\u4e2dHIF-1\u03b1\uff08\u7eff\u8272\uff09\u548cF-\u808c\u52a8\u86cb\u767d\uff08\u7ea2\u8272\uff09\u7684CLSM\u56fe\u50cf\u3002<\/p>\n

\u56fe\u4e09\u3001\u4f53\u5185\u6210\u50cf\u548c\u6cbb\u7597<\/strong>
\n \"\"\uff08a\uff09\u5728\u4e0d\u540c\u65f6\u95f4\u6bb5\u5bf9\u8377\u7624\u5c0f\u9f20\u8fdb\u884cT2<\/sub><\/em>*<\/sup>\u52a0\u6743MR\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09\u5728\u4e0d\u540c\u65f6\u95f4\u901a\u8fc7\u9759\u8109\u5185\u6ce8\u5c04MCOPP-Ce6\u5bf9\u8377\u7624\u5c0f\u9f20\u8fdb\u884c\u8367\u5149\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09\u7f3a\u6c27\u67d3\u8272\u540e\uff0c\u80bf\u7624\u5207\u7247\u7684\u4ee3\u8868\u6027\u514d\u75ab\u8367\u5149\u56fe\u50cf\uff1b<\/p>\n

\uff08d\uff09\u76f8\u5bf9\u5e94\u7684\u80bf\u7624\u5207\u7247\u7f3a\u6c27\u9633\u6027\u533a\u57df\u548c\u8840\u7ba1\u5bc6\u5ea6\uff1b<\/p>\n

\uff08e\uff09\u5404\u79cd\u5904\u7406\uff08\u540e\u5c0f\u9f20\u7684\u76f8\u5bf9\u80bf\u7624\u4f53\u79ef\uff0c\u5373I\uff08\u5bf9\u7167\uff09\u3001II\uff08\u6fc0\u5149\uff09\u3001III\uff08Ce6\uff09\u3001IV\uff08MCOPP Ce6\uff09\u3001V\uff08Ce6+\u6fc0\u5149\uff09\u548cVI\uff08MCOPP-Ce6+\u6fc0\u5149\uff09\uff1b<\/p>\n

\uff08f\uff09\u5904\u7406\u540e\uff0c\u5c0f\u9f20\u7684\u6444\u5f71\u56fe\u50cf\uff1b<\/p>\n

\uff08g\uff09\u6cbb\u7597\u540e\uff0c\u80bf\u7624\u7684\u5e73\u5747\u91cd\u91cf\uff1b<\/p>\n

\uff08h\uff09\u7528\u82cf\u6728\u7cbe\u548c\u66d9\u7ea2\u67d3\u8272\u7684\u80bf\u7624\u7ec4\u7ec7\u7684\u7ec4\u7ec7\u5b66\u5206\u6790\u3002<\/p>\n

\u56fe\u56db\u3001\u4f53\u5185\u6bd2\u6027\u8bc4\u4f30<\/strong>
\n \"\"\uff08a\uff09\u5728\u6574\u4e2a\u6cbb\u7597\u8fc7\u7a0b\u4e2d\u6307\u793a\u7684\u4e0d\u540c\u6cbb\u7597\u540e\u5c0f\u9f20\u7684\u5e73\u5747\u4f53\u91cd\uff1b<\/p>\n

\uff08b, c\uff09\u672a\u6cbb\u7597\u7684\u5c0f\u9f20\uff08\u5bf9\u7167\uff09\u548c\u6ce8\u5c04MCOPP-Ce6\u7684\u5c0f\u9f20\u57287\u548c15 d\u7684AST\u3001ALT\u3001BUN\u7b49\u809d\u80be\u529f\u80fd\u6307\u6807\u6570\u636e\u3002<\/p>\n

\uff08d-I\uff09\u672a\u5904\u7406\u7684\u5c0f\u9f20\uff08\u5bf9\u7167\uff09\u548c\u5728\u7b2c7 d\u548c\u7b2c15 d\u7528MCOPP-Ce6\u5904\u7406\u7684\u5c0f\u9f20\u7684\u8840\u5e38\u89c4\u6570\u636e\uff1b<\/p>\n

\uff08m\uff09\u672a\u5904\u7406\u5c0f\u9f20\uff08\u5bf9\u7167\uff09\u548c\u7528MCOPP-Ce6+\u6fc0\u5149\u5904\u7406\u7684\u5c0f\u9f20\u7684\u4e3b\u8981\u5668\u5b98\uff08\u5fc3\u810f\u3001\u809d\u810f\u3001\u813e\u810f\u3001\u80ba\u810f\u3001\u80be\u810f\u548c\u80a0\uff09\u7684\u7ec4\u7ec7\u5b66\u5206\u6790\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u91c7\u7528\u4e00\u6b65\u6cd5\u9000\u706b\u7b56\u7565\u548c\u751f\u7269\u76f8\u5bb9\u6027\u7684PDA\u548cPEG\u4fee\u9970\uff0c\u6210\u529f\u5730\u5408\u6210\u4e86\u4ee5MOFs\u4e3a\u524d\u9a71\u4f53\u7684\u591a\u529f\u80fd\u4ecb\u5b54MCOPP\u9176\u3002\u5229\u7528\u4f53\u5916\u548c\u4f53\u5185\u5b9e\u9a8c\uff0c\u7ed3\u679c\u8868\u660e\u5185\u6e90\u6027H2<\/sub>O2<\/sub>\u4e0eMCOPP-NE\u7684\u50ac\u5316\u53cd\u5e94\u53ef\u4ee5\u6709\u6548\u5730\u7f13\u89e3\u7f3a\u6c27\u6761\u4ef6\u3002\u4ecb\u5b54MCOPP-NE\u5bf9Ce6\u5149\u654f\u5242\u5177\u6709\u5f88\u9ad8\u7684\u8d1f\u8f7d\u80fd\u529b\uff0c\u5236\u5907\u7684MCOPP-Ce6\u5e73\u53f0\u53ef\u663e\u8457\u63d0\u9ad8PDT\u5bf9\u4f4e\u6c27\u80bf\u7624\u7684\u6cbb\u7597\u6548\u679c\u3002\u5728\u80bf\u7624\u90e8\u4f4d\u9009\u62e9\u6027\u5730\u79ef\u7d2fMCOPP-Ce6\u4ee5\u6301\u7eed\u50ac\u5316H2<\/sub>O2<\/sub>\u8f6c\u5316\u4e3aO2<\/sub>\uff0c\u79d1\u7814\u540c\u65f6\u7f13\u89e3\u80bf\u7624\u7f3a\u6c27\u548c\u63d0\u9ad8PDT\u6cbb\u7597\u6548\u679c\u3002\u56e0\u6b64\uff0c\u751f\u7269\u76f8\u5bb9\u6027MCOPP-NE\u5177\u6709\u5de8\u5927\u6f5c\u529b\u4f5c\u4e3a\u4e00\u79cd\u5148\u8fdb\u7684\u764c\u75c7\u6cbb\u7597\u7cfb\u7edf\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aA Mesoporous Nanoenzyme Derived from Metal-OrganicFrameworks with Endogenous Oxygen Generation to Alleviate Tumor Hypoxia for Signifcantly Enhanced Photodynamic Therapy<\/a><\/strong>\uff08Adv. Mater., 2019<\/strong>, DOI:10.1002\/adma.201901893\uff09<\/p>\n

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