{"id":177206,"date":"2019-06-10T06:02:43","date_gmt":"2019-06-09T22:02:43","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=177206"},"modified":"2019-06-09T21:03:12","modified_gmt":"2019-06-09T13:03:12","slug":"nature-commun-%e9%80%89%e6%8b%a9%e6%80%a7%e5%90%b8%e5%85%89%e6%9d%90%e6%96%99%e8%be%85%e5%8a%a9%e7%9a%84%e9%95%8d%e5%8d%95%e5%8e%9f%e5%ad%90%e5%82%ac%e5%8c%96%e5%89%82%e7%94%a8%e4%ba%8e%e8%87%aa","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=177206","title":{"rendered":"Nature Commun.: \u9009\u62e9\u6027\u5438\u5149\u6750\u6599\u8f85\u52a9\u7684\u954d\u5355\u539f\u5b50\u50ac\u5316\u5242\u7528\u4e8e\u81ea\u7136\u73af\u5883\u592a\u9633\u5149\u9a71\u52a8\u7684CO2\u7532\u70f7\u5316"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u5316\u77f3\u71c3\u6599\u7684\u5feb\u901f\u6d88\u8017\u4f7f\u5f97\u4eba\u7c7b\u4e0d\u5f97\u4e0d\u9762\u4e34\u4e25\u91cd\u7684\u80fd\u6e90\u77ed\u7f3a\u53ca\u6e29\u5ba4\u6548\u5e94\u7b49\u8bf8\u591a\u95ee\u9898\u3002\u7532\u70f7\uff08CH4<\/sub>\uff09\u4f5c\u4e3a\u5929\u7136\u6c14\u7684\u4e3b\u8981\u6210\u5206\uff0c\u662f\u4e00\u79cd\u4f4e\u78b3\u6392\u653e\u7684\u6e05\u6d01\u80fd\u6e90\u3002\u901a\u8fc7\u7532\u70f7\u5316\u5c06CO2<\/sub>\u8f6c\u5316\u4e3a\u5408\u6210\u6c14\uff0c\u5bf9\u51cf\u5c11CO2<\/sub>\u6392\u653e\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002CO2<\/sub>\u7532\u70f7\u5316\u9700\u8981\u81f3\u5c11200 \u2103\u7684\u6e29\u5ea6\u624d\u80fd\u53cd\u5e94\uff0c\u9700\u8981\u4e8c\u6b21\u80fd\u6e90\u6d88\u8017\u3002\u5229\u7528\u5149\u70ed\u6548\u5e94\u7684\u592a\u9633\u80fd\u9a71\u52a8CO2<\/sub>\u7532\u70f7\u5316\uff0c\u4e0d\u9700\u8981\u4e8c\u6b21\u80fd\u6e90\u6295\u5165\u5c31\u80fd\u751f\u4ea7CH4<\/sub>\u3002\u7136\u800c\uff0c\u8fd9\u79cd\u65b9\u6cd5\u5fc5\u987b\u63d0\u4f9b\u5f3a\u5149\u8f90\u7167\uff08\u5927\u4e8e10 kW m-2<\/sup>\uff0c\u5373\u6807\u51c6\u592a\u9633\u5149\u5f3a\u5ea6\u7684\u5341\u500d\uff09\u5c06\u50ac\u5316\u5242\u52a0\u70ed\u81f3200 \u2103\u91cf\u7ea7\u4ee5\u9a71\u52a8CO2<\/sub>\u7532\u70f7\u5316\u3002\u5f3a\u5149\u8f90\u7167\u9700\u8981\u590d\u6742\u7684\u8bbe\u5907\u5e76\u589e\u52a0\u80fd\u91cf\u7684\u6d88\u8017\uff0c\u4ece\u800c\u9650\u5236\u4e86\u5149\u70ed\u50ac\u5316\u7684\u5de5\u4e1a\u5316\u5e94\u7528\u3002\u56e0\u6b64\uff0c\u91c7\u7528\u5f31\u592a\u9633\u5149\uff081 kW m-2<\/sup>\uff09\u6765\u5b9e\u73b0\u5149\u70edCO2<\/sub>\u7532\u70f7\u5316\u4ee5\u53ca\u5176\u4ed6\u5149\u70ed\u53cd\u5e94\u662f\u975e\u5e38\u5177\u6709\u6311\u6218\u6027\u7684\u3002\u91d1\u5c5e\u7eb3\u7c73\u7c92\u5b50\u3001\u78b3\u57fa\u6750\u6599\u7b49\u5177\u6709\u5168\u592a\u9633\u5149\u5149\u8c31\u5438\u6536\u80fd\u529b\u7684\u5149\u70ed\u50ac\u5316\u5242\u5f97\u5230\u4e86\u5e7f\u6cdb\u7684\u7814\u7a76\uff0c\u4f46\u7531\u4e8e\u5176\u5f3a\u70c8\u7684\u70ed\u8f90\u5c04\u963b\u788d\u4e86\u5149\u70ed\u6750\u6599\u7684\u70ed\u91cf\u50a8\u5b58\uff0c\u56e0\u6b64\u8fd9\u4e9b\u6750\u6599\u5728\u6807\u51c6\u592a\u9633\u5149\u8f90\u7167\u4e0b\u53ea\u80fd\u83b7\u5f9790 \u2103\u5de6\u53f3\u7684\u6e29\u5ea6\uff0c\u4e0d\u8db3\u4ee5\u63a8\u52a8\u4e8c\u6c27\u5316\u78b3\u7532\u70f7\u5316\u53cd\u5e94\u3002
\n \u53e6\u4e00\u65b9\u9762\uff0c\u948c\uff08Ru\uff09\u50ac\u5316\u5242\u5df2\u88ab\u8bc1\u5b9e\u662f\u5149\u70edCO2<\/sub>\u7532\u70f7\u5316\u7684\u6700\u4f73\u50ac\u5316\u5242\uff0c\u4f46\u948c\u4f5c\u4e3a\u7a00\u6709\u91d1\u5c5e\u4ef7\u683c\u6602\u8d35\uff0c\u56e0\u6b64\u6025\u9700\u5f00\u53d1\u51fa\u5ec9\u4ef7\u91d1\u5c5e\u50ac\u5316\u5242\u6765\u66ff\u4ee3\u6602\u8d35\u7684\u948c\u50ac\u5316\u5242\u3002\u8fd1\u5e74\u6765\u8d1f\u8f7d\u578b\u5355\u539f\u5b50\u50ac\u5316\u5242\u5728\u50ac\u5316\u52a0\u6c22\u3001\u6c27\u5316\u3001\u6c34\u7164\u6c14\u53d8\u6362\u7b49\u591a\u79cd\u53cd\u5e94\u4e2d\u5747\u8868\u73b0\u51fa\u8f83\u9ad8\u7684\u6d3b\u6027\u3002\u7136\u800c\uff0c\u8fc4\u4eca\u4e3a\u6b62\uff0c\u5173\u4e8e\u5355\u539f\u5b50\u50ac\u5316\u5242\u7528\u4e8e\u5149\u70edCO2<\/sub>\u7532\u70f7\u5316\u7684\u7814\u7a76\u62a5\u9053\u4e0d\u591a\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u6700\u8fd1\uff0c\u6cb3\u5317\u5927\u5b66\u674e\u4e9a\u5149\u56e2\u961f<\/strong>\uff08\u7b2c\u4e00\u4f5c\u8005\u3001\u901a\u8baf\u4f5c\u8005\uff09\u4e0e\u6d59\u6c5f\u5e08\u8303\u5927\u5b66\u80e1\u52c7\u7814\u7a76\u5458<\/strong>\u3001\u65e5\u672c\u56fd\u5bb6\u6750\u6599\u7814\u7a76\u6240\uff08NIMS\uff09\u53f6\u91d1\u82b1\u7814\u7a76\u5458<\/strong>\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u5408\u4f5c\uff0c\u5728\u5149\u70ed\u50ac\u5316\u9886\u57df\u53d6\u5f97\u91cd\u8981\u8fdb\u5c55\u3002\u4f5c\u8005\u5728\u5149\u70ed\u7cfb\u7edf\u4e2d\u6dfb\u52a0\u80fd\u591f\u5438\u6536\u6574\u4e2a\u592a\u9633\u5149\u8c31\u5e76\u4ea7\u751f\u6781\u5c11\u70ed\u8f90\u5c04\u7684\u9009\u62e9\u6027\u5438\u5149\u6750\u6599\uff0c\u53ef\u4ee5\u5728\u6807\u51c6\u592a\u9633\u5149\uff081 kW m-2<\/sup>\uff09\u8f90\u7167\u4e0b\u5c06\u50ac\u5316\u5242\u52a0\u70ed\u5230288 \u2103\uff0c\u6210\u529f\u5b9e\u73b0\u6807\u51c6\u592a\u9633\u5149\u9a71\u52a8\u7684\u5149\u70edCO2<\/sub>\u7532\u70f7\u5316\u3002\u6b64\u5916\uff0c\u4ed6\u4eec\u8fd8\u5236\u5907\u4e86Ni\u5355\u539f\u5b50\u4fee\u9970\u7684\u4e8c\u7ef4\u975e\u6676\u6001Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\uff08SA Ni\/Y2<\/sub>O3<\/sub>\uff09\u3002\u4e0e\u5176\u4ed6\u954d\u57fa\u50ac\u5316\u5242\u76f8\u6bd4\uff0cSA Ni\/Y2<\/sub>O3<\/sub>\u5177\u6709\u8f83\u4f4e\u7684\u521d\u59cb\u53cd\u5e94\u6e29\u5ea6\u548c\u8f83\u9ad8\u7684CO2<\/sub>\u7532\u70f7\u5316\u6d3b\u6027\u3002\u4f5c\u8005\u7ed3\u5408\u9009\u62e9\u6027\u5438\u5149\u6750\u6599\u548cSA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\uff0c\u5728\u5ba4\u5916\u592a\u9633\u5149\u8f90\u5c04\u4e0b\u5b9e\u73b0\u9ad8\u6548CO2<\/sub>\u7532\u70f7\u5316\uff0c\u5176\u8f6c\u5316\u6548\u7387\u4e3a80%\uff0c\u7532\u70f7\u4ea7\u7387\u4e3a7.5 l m\u22122<\/sup> h\u22121<\/sup>\u3002\u8fd9\u9879\u5de5\u4f5c\u5bf9\u4e8e\u81ea\u7136\u592a\u9633\u5149\u9a71\u52a8CO2<\/sub>\u8f6c\u5316\u4e3a\u7532\u70f7\u7684\u7814\u7a76\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201cSelective light absorber-assisted single nickel atom catalysts for ambient sunlight-driven CO2<\/sub> methanation<\/strong>\u201d\u53d1\u8868\u4e8eNature Communications<\/strong>\u671f\u520a\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u4f20\u7edf\u7684\u548c\u9009\u62e9\u6027\u5438\u5149\u6750\u6599\u8f85\u52a9\u7684\u5149\u70ed\u7cfb\u7edf<\/strong>
\n \"\"\uff08a\uff09Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7c89\u672b\u7167\u7247\uff1b<\/p>\n

\uff08b\uff09Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684\u5f52\u4e00\u5316UV-Vis-IR\u5438\u6536\u5149\u8c31\uff1b<\/p>\n

\uff08c\uff09Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u5728200 \u2103\u4e0b\u7684\u592a\u9633\u80fd\u5438\u6536\u548c\u70ed\u8f90\u5c04\u56fe\uff1b<\/p>\n

\uff08d\uff09\u9009\u62e9\u6027\u5149\u5438\u6536\u6750\u6599\u7684\u6a2a\u622a\u9762SEM\u56fe\uff1b<\/p>\n

\uff08e\uff09\u9009\u62e9\u6027\u5149\u5438\u6536\u6750\u6599\u7684\u5f52\u4e00\u5316UV-Vis-IR\u5438\u6536\u5149\u8c31\uff1b<\/p>\n

\uff08g\uff09\u5229\u7528\u9009\u62e9\u6027\u5149\u5438\u6536\u6750\u6599\u548c\u50ac\u5316\u5242\u8fdb\u884c\u5149\u70ed\u50ac\u5316CO2<\/sub>\u7532\u70f7\u5316\u7684\u5149\u70ed\u7cfb\u7edf\u539f\u7406\u56fe\uff1b<\/p>\n

\uff08h~i\uff09\u5728\u4e0d\u540c\u5f3a\u5ea6\u7684\u9633\u5149\u7167\u5c04\u4e0b\uff0c\u5177\u6709\u548c\u4e0d\u5177\u6709\u9009\u62e9\u6027\u5149\u5438\u6536\u8f85\u52a9\u5149\u70ed\u7cfb\u7edf\u7684Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684\u5149\u50ac\u5316\u6e29\u5ea6\u548cCO2<\/sub>\u7532\u70f7\u5316\u8f6c\u5316\u7387\u3002<\/p>\n

\u56fe\u4e8c\u3001SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684\u5236\u5907\u53ca\u8868\u5f81<\/strong>
\n \"\"\uff08a\uff09Ni\u5355\u539f\u5b50\u4fee\u9970\u7684\u4e8c\u7ef4\u975e\u6676\u6001Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\uff08SA Ni\/Y2<\/sub>O3<\/sub>\uff09\u7684\u5236\u5907\u5de5\u827a\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684XRD\u8c31\uff1b<\/p>\n

\uff08c\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684N2<\/sub>\u5438\u9644\u7b49\u6e29\u7ebf\uff1b<\/p>\n

\uff08d\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684SEM\u56fe\uff1b<\/p>\n

\uff08e\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684TEM\u56fe\uff1b<\/p>\n

\uff08f\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684HRTEM\u56fe\u3002\u63d2\u56fe\u662f\u5bf9\u5e94\u7684\u7535\u5b50\u884d\u5c04\u56fe\u6837\uff1b<\/p>\n

\uff08g\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684STEM\u56fe\uff0c\u4ee5\u53caNi\u3001Y\u548cO\u7684EDS\u6620\u5c04\u56fe\u3002<\/p>\n

\u56fe\u4e09\u3001SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u4e2d\u954d\u7684\u8868\u5f81<\/strong>
\n \"\"\uff08a\uff09\u7403\u5dee\u6821\u6b63\u7684SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247TEM\u56fe\uff1b<\/p>\n

\uff08b\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u3001NiO\u548cNi\u7b94\u7684Ni k\u8fb9\u7684EXAFS\u8c31\u56fe\uff1b<\/p>\n

\uff08c\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u3001NiO\u548cNi\u7b94\u7684Ni k\u8fb9\u8fdb\u884c\u5085\u91cc\u53f6\u53d8\u6362\uff08FT\uff09EXAFS\u8c31\u56fe\uff1b<\/p>\n

\uff08d\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684\u7ed3\u6784\u6a21\u578b\u53ca\u76f8\u5e94\u7684FT-EXAFS\u62df\u5408\u66f2\u7ebf\u3002<\/p>\n

\u56fe\u56db\u3001CO2<\/sub>\u52a0\u6c22\u70ed\u50ac\u5316\u5b9e\u9a8c<\/strong>
\n \"\"\uff08a\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\uff08SA Ni\/Y2<\/sub>O3<\/sub>\uff09\u548cNi\u7eb3\u7c73\u9897\u7c92\/ Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\uff08Ni\/Y2<\/sub>O3<\/sub>\uff09\u7684CO2<\/sub>\u7532\u70f7\u5316\u6027\u80fd\u56fe\uff1b<\/p>\n

\uff08b\uff09SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684CO2<\/sub>\u7532\u70f7\u5316\u6027\u80fd\uff1aCH4<\/sub>\u548cCO\u7684\u4ea7\u7387\u968f\u6e29\u5ea6\u7684\u53d8\u5316\uff1b<\/p>\n

\uff08c\uff09240\u2103\u4e0b\uff0cSA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684CO2<\/sub>\u6c22\u5316\u53cd\u5e94\u7a33\u5b9a\u6027\uff1b<\/p>\n

\uff08d\uff09\u7a33\u5b9a\u6027\u6d4b\u8bd5\u540e\u7684SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684TEM\u7403\u5dee\u6821\u6b63\u56fe\u3002<\/p>\n

\u56fe\u4e94\u3001\u9009\u62e9\u6027\u5438\u5149\u6750\u6599\u8f85\u52a9SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684CO2<\/sub>\u7532\u70f7\u5316\u6027\u80fd\u7684\u7814\u7a76<\/strong>
\n \"\"\uff08a\uff09\u6807\u51c6\u592a\u9633\u5149\u8f90\u5c04\u4e0b\uff0c\u7ea2\u5916\u76f8\u673a\u83b7\u5f97\u7684\u6d82\u8986\u6709SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684\u9009\u62e9\u6027\u5438\u5149\u6750\u6599\u8f85\u52a9\u53cd\u5e94\u5668\u7684\u7a7a\u95f4\u6e29\u5ea6\u56fe\uff1b<\/p>\n

\uff08b\uff09\u4e0d\u540c\u5f3a\u5ea6\u6a21\u62df\u592a\u9633\u5149\u8f90\u5c04\u4e0b\uff0c\u9009\u62e9\u6027\u5438\u5149\u6750\u6599\u8f85\u52a9\u7684SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684\u6e29\u5ea6\u53caCO2<\/sub>\u8f6c\u5316\u7387\uff1b<\/p>\n

\uff08c\uff092018\u5e746\u670830\u65e58\u65f6\u81f318\u65f6\uff0c\u6cb3\u5317\u7701\u4fdd\u5b9a\u5e02\u5ba4\u5916\u592a\u9633\u5149\u901a\u91cf\u968f\u65f6\u95f4\u7684\u53d8\u5316\uff1b<\/p>\n

\uff08d\uff092018\u5e746\u670830\u65e58\u65f6\u81f318\u65f6\u5ba4\u5916\u592a\u9633\u5149\u8f90\u7167\u4e0b\uff0c\u9009\u62e9\u6027\u5438\u5149\u6750\u6599\u8f85\u52a9\u7684SA Ni\/Y2<\/sub>O3<\/sub>\u7eb3\u7c73\u7247\u7684\u5149\u70edCO2<\/sub>\u8f6c\u6362\u7387\u3002<\/p>\n

\n \u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aSelective light absorber-assisted single nickel atom catalysts for ambient sunlight-driven CO2 methanation<\/a>\uff08Nat. Commun.,<\/em> 2019,<\/strong> 10(1): 2359.\uff09<\/p>\n

\u672c\u6587\u7531\u6211\u4ea6\u662f\u884c\u4eba\u7f16\u8bd1<\/p>\n

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