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\u5f15\u8a00<\/b><\/strong><\/h3>\n

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\u56fd\u5185<\/b><\/strong><\/h3>\n

1. \u540c\u6d4e\u5927\u5b66-\u5f20\u4f1f\u8d24<\/b><\/strong><\/h4>\n

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\u6700\u65b0\u7684\u7814\u7a76\u9664\u78f7\u7684\u5de5\u4f5c\u88ab\u300aEnvironmental Science & Technology\u300b\u62a5\u9053\u3002\u805a\u82ef\u4e59\u70ef\u57fa\u7eb3\u7c73\u6c27\u5316\u94c1\u590d\u5408\u6750\u6599\u662f\u4e00\u79cd\u5177\u6709\u4ee3\u8868\u6027\u7684\u7eb3\u7c73\u6750\u6599\uff0c\u6210\u529f\u5730\u5e94\u7528\u4e8e\u7837\u3001\u78f7\u7684\u5927\u89c4\u6a21\u6c34\u51c0\u5316\u3002\u7136\u800c\uff0c\u5bf9\u4e8e\u6eb6\u6db2\u5316\u5b66(\u4f8b\u5982\u5171\u5b58\u7684Ca2+<\/sup>)\u5bf9\u7eb3\u7c73\u590d\u5408\u6750\u6599\u957f\u671f\u6027\u80fd\u7684\u5f71\u54cd\uff0c\u76ee\u524d\u8fd8\u77e5\u4e4b\u751a\u5c11\u3002\u5728\u672c\u7814\u7a76\u4e2d\uff0c\u6211\u4eec\u5728\u805a\u5408\u7269\u652f\u6301\u7684\u542b\u94c1\u7eb3\u7c73\u590d\u5408\u6750\u6599HFO@201\u4e0a\u8fdb\u884c\u4e8620\u6b21\u78f7\u9178\u76d0\u5438\u9644-\u89e3\u5438\u5faa\u73af\u3002\u51fa\u4e4e\u610f\u6599\u7684\u662f\uff0c\u5728\u6709\u9499\u79bb\u5b50\u5b58\u5728\u7684\u60c5\u51b5\u4e0b\uff0c\u78f7\u9178\u76d0\u7684\u53bb\u9664\u7387\u63d0\u9ad8\u4e86\uff0c\u8fd9\u4e0e\u5b83\u5bf9\u9897\u7c92\u72b6\u6c27\u5316\u94c1\u6355\u83b7\u78f7\u9178\u76d0\u7684\u4e0d\u5229\u5f71\u54cd\u622a\u7136\u4e0d\u540c\u3002\u8fdb\u4e00\u6b65\u7684\u673a\u7406\u7814\u7a76\u8868\u660e\uff0c\u4e3b\u8981\u662f\u901a\u8fc7HFO@201\u7f51\u7edc\u5b54\u9699\u5185\u7684Ca-P\u5171\u6c89\u6dc0\u6cd5\u4ee5\u5b9e\u73b0\u589e\u5f3a\u9664\u78f7\uff0c\u5e76\u53ef\u80fd\u5f62\u6210\u591a\u79cdFe -P – Ca-P\u7edc\u5408\u7269\u3002\u590d\u5408\u7269\u7684\u5f62\u6210\u663e\u8457\u589e\u52a0\u4e86P\u7684\u5438\u9644\u91cf\uff0c\u5728\u78f7\u9178\u76d0\u5438\u9644\u548c\u78b1\u6027\u518d\u751f\u8fc7\u7a0b\u4e2d\uff0c\u5c01\u95ed\u5b54\u9699\u4e2d\u79ef\u7d2f\u7684OH–<\/sup>\u4fc3\u4f7f\u5171\u6c89\u6dc0\u6cd5\u6709\u5229\u4e8e\u901a\u8fc7\u5185\u90e8\u975e\u6676\u6001\u78f7\u9178\u9499(ACP)\u548c\u7f9f\u57fa\u78f7\u7070\u77f3\u7684\u5f62\u6210\u6765\u53bb\u9664P\u3002TEM-EDS\u80fd\u8c31\u5206\u6790\u8868\u660e\uff0c\u8d1f\u8f7d\u7eb3\u7c73HFO\u8868\u9762\u4e0d\u53d1\u751f\u5171\u6c89\u6dc0\u7269\uff0c\u6781\u5927\u5730\u51cf\u8f7b\u4e86\u5171\u6c89\u6dc0\u7269\u5bf9\u7eb3\u7c73HFO\u8868\u9762P\u5438\u9644\u7684\u4e0d\u5229\u5f71\u54cd\u3002\u56fa\u5b9a\u5e8a\u67f1\u7814\u7a76\u8868\u660e\uff0cCa2+<\/sup>\u7684\u5b58\u5728\u4f7fHFO@201\u5bf9\u542b\u78f7\u6c61\u6c34\u7684\u6709\u6548\u5904\u7406\u4f53\u79ef\u63d0\u9ad8\u4e86\u7ea670%\u3002\u8be5\u7814\u7a76\u4e3a\u8fdb\u4e00\u6b65\u7814\u7a76\u6eb6\u6db2\u5316\u5b66\u5bf9\u7c7b\u4f3c\u7eb3\u7c73\u590d\u5408\u6750\u6599\u7684\u6c34\u5904\u7406\u6548\u679c\u63d0\u4f9b\u4e86\u65b0\u7684\u601d\u8def[<\/sup>4]<\/sup>\u3002<\/p>\n

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\u81ea\u7136\u754c\u4e2d\u7684\u7837\u4e3b\u8981\u4ee5\u4e09\u4ef7As(III)\u4e0e\u4e94\u4ef7As(V)\u4e24\u79cd\u5f62\u5f0f\u5b58\u5728\uff0c\u5176\u4e2dAs(III)\u7684\u6bd2\u6027\u66f4\u9ad8\uff0c\u7ea6\u4e3aAs(V)\u768460\u500d\u4ee5\u4e0a\uff0c\u4e14\u8fc1\u79fb\u6027\u66f4\u5f3a\u3001\u53bb\u9664\u96be\u5ea6\u66f4\u5927\u3002\u4e00\u822c\u60c5\u51b5\u4e0b\uff0cAs(III)\u4e3a\u5730\u4e0b\u6c34\u4e2d\u7837\u7684\u4f18\u52bf\u5f62\u6001\uff0c\u5e38\u7528\u7684\u79bb\u5b50\u4ea4\u6362\u3001\u6c89\u6dc0\u3001\u5438\u9644\u7b49\u5355\u5143\u6280\u672f\u5747\u96be\u4ee5\u5c06As(III)\u5904\u7406\u5230\u996e\u7528\u6c34\u5b89\u5168\u63a7\u5236\u6807\u51c6(\uff1c10 ppb)\u3002\u8fd1\u65e5\u7814\u5236\u6210\u529f\u4e00\u79cd\u6c27\u5316-\u5438\u9644\u529f\u80fd\u8026\u5408\u578b\u7eb3\u7c73\u590d\u5408\u6750\u6599HFO@PS-Cl\u3002\u8be5\u6750\u6599\u901a\u8fc7\u5728\u805a\u82ef\u4e59\u70ef\u8f7d\u4f53\u9aa8\u67b6\u4e0a\u5171\u4ef7\u952e\u8054\u6d3b\u6027\u6c2f\u5b9e\u73b0\u5bf9As(III)\u7684\u9ad8\u6548\u6c27\u5316\uff1b\u5e76\u901a\u8fc7\u5728\u8f7d\u4f53\u7eb3\u7c73\u5b54\u9053\u5185\u56fa\u5b9a\u6c27\u5316\u94c1\u7eb3\u7c73\u9897\u7c92\uff0c\u5b9e\u73b0\u5bf9\u6c27\u5316\u540eAs(V)\u7684\u4e13\u5c5e\u5438\u9644\u53bb\u9664\uff0c\u4ece\u800c\u5b9e\u73b0\u4e86\u6c34\u4e2dAs(III)\u7684\u9ad8\u6548\u5904\u7406\u3002HFO@PS-Cl\u53ef\u76f4\u63a5\u5c06\u6c34\u4e2dAs(III)\u7684\u542b\u91cf\u4ece1000 ppb\u964d\u81f310 ppb\u4ee5\u4e0b\uff0c\u5904\u7406\u5bb9\u91cf\u76f8\u6bd4\u73b0\u6709\u5546\u54c1\u5316\u9664\u7837\u7eb3\u7c73\u590d\u5408\u6750\u6599HFO@D201\u63d0\u53472\u500d (\u4ece\u5355\u6279\u6b21600\u5e8a\u4f53\u79ef\u63d0\u5347\u52301750 BV\u5de6\u53f3)\u3002\u6b64\u5916\uff0c\u4f7f\u7528\u540eHFO@PS-Cl\u7684\u6c27\u5316-\u5438\u9644\u80fd\u529b\u53ef\u5b9e\u73b0\u9ad8\u6548\u518d\u751f\uff0c\u5faa\u73af\u4f7f\u75287\u6b21\u4ee5\u4e0a\u5904\u7406\u6027\u80fd\u4ecd\u4fdd\u6301\u7a33\u5b9a\u3002\u8be5\u6750\u6599\u7ed3\u6784\u7a33\u5b9a\uff0c\u5bf9\u6c34\u4e2d\u5171\u5b58\u79bb\u5b50\u3001\u5929\u7136\u6709\u673a\u7269\u7b49\u6297\u5e72\u6270\u80fd\u529b\u5f3a\uff0c\u5177\u6709\u826f\u597d\u7684\u5b9e\u9645\u5e94\u7528\u524d\u666f\u3002\u8fd9\u4e00\u7814\u7a76\u5bf9\u53d1\u5c55\u5730\u4e0b\u6c34As(III)\u6df1\u5ea6\u5904\u7406\u65b0\u6280\u672f\u5177\u6709\u91cd\u8981\u610f\u4e49[<\/sup>5]<\/sup>\u3002<\/p>\n

3. \u54c8\u5c14\u6ee8\u5de5\u4e1a\u5927\u5b66-\u9a6c\u519b<\/b><\/strong><\/h4>\n

\u4eba\u7269\u7b80\u4ecb\uff1a<\/b><\/strong>\u4f5c\u4e3a\u300aEnvironmental Science & Technology\u300b\u7684\u5927\u6237\uff0c\u662f\u54c8\u5c14\u6ee8\u5de5\u4e1a\u5927\u5b66\u5e02\u653f\u73af\u5883\u5de5\u7a0b\u5b66\u9662\u526f\u9662\u957f\u3001\u6559\u6388\/\u535a\u58eb\u751f\u5bfc\u5e08,\u57ce\u5e02\u6c34\u8d44\u6e90\u5f00\u53d1\u5229 \u7528\uff08\u5317\u65b9\uff09\u56fd\u5bb6\u5de5\u7a0b\u7814\u7a76\u4e2d\u5fc3\u5e38\u52a1\u526f\u4e3b\u4efb\u3001\u57ce\u5e02\u6c34\u8d44\u6e90\u4e0e\u6c34\u73af\u5883\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u996e\u7528\u6c34\u5b89\u5168\u5b66\u672f\u5e26\u5934\u4eba\u3002\u6559\u80b2\u90e8\u201c\u957f\u6c5f\u5b66\u8005\u5956\u52b1\u8ba1\u5212\u7279\u8058\u6559\u6388\u201d\u3002<\/p>\n

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\"\"<\/p>\n

\u6700\u65b0\u5728\u300aEnvironmental Science & Technology\u300b\u53d1\u8868\u4e86\u539f\u4f4d\u6c2e\u63ba\u6742\u7684\u916e\u6d1b(HNC)\u7528\u4e8e\u81ed\u6c27\u7684\u50ac\u5316\uff1a\u63ed\u793a\u7f9f\u57fa\u81ea\u7531\u57fa\u6c27\u5316\u4e0e\u7535\u5b50\u4f20\u9012\u975e\u81ea\u7531\u57fa\u6c27\u5316\u7684\u534f\u540c\u673a\u7406\u3002O3<\/sub>\/NHC\u6027\u80fd\u4f18\u4e8e\u4f20\u7edf\u7684\u00b7OH\u50ac\u5316\u81ed\u6c27\u5316\u5de5\u827a\uff0c\u4e0eO3<\/sub>\u5355\u72ec\u76f8\u6bd4\uff0cO3<\/sub>\/NHC\u4e0d\u4ec5\u5b9e\u73b0\u4e86\u901f\u7387\u5e38\u6570\u768411\u500d\u589e\u5f3a\uff0c\u800c\u4e14\u5728\u8f83\u5bbd\u7684pH(4-9)\u548c\u6e29\u5ea6(15-35\u2103)\u8303\u56f4\u5185\u964d\u89e3KTP\uff0c\u5177\u6709\u8f83\u9ad8\u7684\u7a33\u5b9a\u6027\u3002NHC\u7684\u9ad8\u77f3\u58a8\u5316\u7a0b\u5ea6(ID\/IG = 0.78~0.88)\u548c\u4f4e\u4e0d\u9971\u548c\u6c27\u542b\u91cf(0.1~ 1.38%)\u7a81\u51fa\u4e86n\u6742\u539f\u5b50\u5bf9O3<\/sub>\/NHC\u4f53\u7cfb\u7684\u4e3b\u5bfc\u4f5c\u7528\u3002\u901a\u8fc7\u5173\u7cfb\u7814\u7a76(N\u6027\u8d28\u4e0e\u50ac\u5316\u6d3b\u6027\u7684\u5173\u7cfb)\u548cXPS\u8868\u5f81\uff0c\u8bc1\u5b9e\u4e86\u4e0d\u540cN\u79cd\u7684\u7279\u5f02\u6027\u4f5c\u7528\u3002\u77f3\u58a8\u7ed3\u6784\u4f53\u4e2d\u5f62\u6210\u7684\u77f3\u58a8\u6001N\u4f5c\u4e3a\u201c\u7535\u5b50\u8fc1\u79fb\u7387\u201d\u533a\u57df\uff0c\u901a\u8fc7\u975e\u81ea\u7531\u57fa\u53cd\u5e94\u8fc7\u7a0b\u5c06\u7535\u5b50\u4eceKTP\u5206\u5b50\u8f6c\u79fb\u5230O3<\/sub>\uff0c\u4fc3\u8fdbKTP\u964d\u89e3\u3002\u4f4d\u4e8e\u77f3\u58a8\u7ed3\u6784\u7f3a\u9677\u5904\u7684\u5421\u54af\u548c\u5421\u5576N\u4f5c\u4e3a\u201c\u81ea\u7531\u57fa\u751f\u6210\u201d\u533a\u57df\uff0c\u5c06O3<\/sub>\u5206\u89e3\u4e3a\u00b7OH\uff0c\u901a\u8fc7\u81ea\u7531\u57fa\u6c27\u5316\u8fc7\u7a0b\u964d\u89e3KTP\u3002\u8fd9\u4e00\u53d1\u73b0\u4e3a\u5728\u6709\u673a\u6c61\u67d3\u6c34\u7684\u50ac\u5316\u81ed\u6c27\u5316\u8fc7\u7a0b\u4e2d\uff0c\u51c6\u786e\u5730\u8bbe\u8ba1n\u63ba\u6742\u78b3\u8d28\u50ac\u5316\u5242\u63d0\u4f9b\u4e86\u4e00\u4e2a\u5168\u65b0\u7684\u89c6\u89d2[<\/sup>6]<\/sup>\u3002<\/p>\n

\"\"<\/p>\n

\u4e0d\u65ad\u53d1\u6398\u4f20\u7edf\u6750\u6599\u5728\u73af\u5883\u4fee\u590d\u4e2d\u7684\u5404\u79cd\u53ef\u80fd\uff0c\u8fd1\u671f\u5728\u300aEnvironmental Science & Technology\u300b\u4e0a\u62a5\u9053\u4e86\u4e00\u79cd\u88ab\u4f4e\u4f30\u7684\u6c27\u5316\u5242\u9ad8\u94c1\u9178\u94be\u5728\u4e0d\u540c\u6761\u4ef6\u4e0b(\u6dfb\u52a0\uff0c\u4e0d\u6dfb\u52a0\u78f7\u9178\u76d0\uff0c\u6dfb\u52a0\u787c\u9178\u76d0)\u5bf9CBZ,BPS(\u53cc\u915aS),DCF\u548cCIP(\u73af\u4e19\u6c99\u661f)\u7684\u53bb\u9664\u6548\u679c\u3002\u9ad8\u94c1\u9178\u76d0(K2<\/sub>FeO4<\/sub>)\u662f\u4e00\u79cd\u5f3a\u6c27\u5316\u5242\uff0c\u5728Fe(VI) – Fe(V) – Fe(IV) –\u00a0Fe(III)\u7684\u7406\u8bba\u8f6c\u5316\u8fc7\u7a0b\u4e2d\uff0c\u9ad8\u94c1\u9178\u76d0\u76841mol\u53ef\u4ee5\u6355\u83b7\u9ad8\u8fbe3mol\u7684\u7535\u5b50\u3002\u4f46\u662f\uff0c\u7531\u4e8e\u4e2d\u95f4\u6001\u7684\u94c1\u7269\u79cd\u7684\u5feb\u901f\u81ea\u5206\u89e3\uff0c\u9ad8\u94c1\u9178\u76d0\u6c27\u5316\u80fd\u529b\u7684\u5229\u7528\u6548\u7387\u8f83\u4f4e\uff0c\u5bf9\u9ad8\u94c1\u9178\u76d0\u63a7\u5236\u6709\u673a\u6c61\u67d3\u7269\u7684\u6f5c\u529b\u4ea7\u751f\u4e86\u8d1f\u9762\u5f71\u54cd\u3002\u7814\u7a76\u4e2d\u53d1\u73b0\uff0c\u5bf9\u4e8e\u5361\u9a6c\u897f\u5e73(CBZ)\u3001\u53cc\u915aS (BPS)\u3001\u53cc\u6c2f\u82ac\u9178(DCF)\u3001\u73af\u4e19\u6c99\u661f(CIP)\u7684\u9ad8\u94c1\u9178\u76d0\u6c27\u5316\uff0c\u5728pH \u4e3a8.0\u65f6\uff0c\u78f7\u9178\u76d0\u7f13\u51b2\u6db2\u4e2d\u6d4b\u5b9a\u7684\u53cd\u5e94\u901f\u7387\u5e38\u6570\u6bd4\u787c\u9178\u7f13\u51b2\u6db2\u4e2d\u4f4e1.7 – 2.4\u500d\u3002\u9ad8\u94c1\u9178\u76d0\u4e0e2,2\u2019-\u5076\u6c2e\u4e8c\u6c2e(3\u4e59\u57fa\u82ef\u5e76\u567b\u5511\u5549-6-\u78fa\u9178\u76d0)(ABTS)\u5728pH 7.0\u4e0b\u53cd\u5e94\uff0c\u6d4b\u5b9a\u7684\u53cd\u5e94\u5316\u5b66\u8ba1\u91cf\u6570\u5206\u522b\u4e3a\u5728100 mM\u78f7\u9178\u76d0\u7f13\u51b2\u6db2\u4e2d1:1.04,10 mM\u78f7\u9178\u76d0\u7f13\u51b2\u6db2\u4e2d1:1.18, 10 mM\u787c\u9178\u76d0\u7f13\u51b2\u6db2\u4e2d1:1.93\u3002\u9ad8\u94c1\u9178\u76d0\u5728\u78f7\u9178\u76d0\u7f13\u51b2\u6db2\u4e2d\u7684\u6c27\u5316\u80fd\u529b\u4e0b\u964d\u3002\u5efa\u7acb\u94c1(VI)\u3001\u94c1(V)\u548c\u94c1(IV)\u4e09\u79cd\u5143\u7d20\u6c27\u5316ABTS\u7684\u52a8\u529b\u5b66\u6a21\u578b\uff0c\u5e76\u5728\u4e0d\u540c\u7684\u7f13\u51b2\u6761\u4ef6\u4e0b\u8f83\u597d\u5730\u62df\u5408\u4e86ABTS\u2022+\u7684\u751f\u6210\u52a8\u529b\u5b66\u3002\u7ed3\u679c\u8868\u660e\uff0c\u78f7\u9178\u76d0\u5bf9Fe(VI)\u548cFe(IV)\u7269\u79cd\u7684\u6c27\u5316\u80fd\u529b\u5f71\u54cd\u4e0d\u5927\uff0c\u4f46\u4f7fABTS\u4e0eFe(V)\u7269\u79cd\u7684\u6bd4\u901f\u7387\u5e38\u6570\u964d\u4f4e\u4e861 – 2\u4e2a\u6570\u91cf\u7ea7\uff0c\u5bfc\u81f4Fe(V)\u81ea\u5206\u89e3\u9014\u5f84\u76f8\u4e92\u7ade\u4e89\u3002\u78f7\u9178\u9634\u79bb\u5b50\u4e0eFe(V)\u7684\u7edc\u5408\u53ef\u80fd\u662f\u78f7\u9178\u7f13\u51b2\u6db2\u6291\u5236\u4f5c\u7528\u7684\u539f\u56e0\u4e4b\u4e00\u3002\u7531\u4e8e\u5728\u78f7\u9178\u76d0\u7f13\u51b2\u6db2\u4e2d\u8fdb\u884c\u4e86\u5927\u91cf\u9ad8\u94c1\u9178\u76d0\u6c27\u5316\u7684\u7814\u7a76\uff0c\u9ad8\u94c1\u9178\u76d0\u7684\u5b9e\u9645\u6c27\u5316\u80fd\u529b\u662f\u88ab\u4f4e\u4f30\u4e86\u7684[<\/sup>7]<\/sup>\u3002<\/p>\n

4. \u4e2d\u79d1\u9662\u751f\u6001\u4e2d\u5fc3-\u90dd\u90d1\u5e73<\/b><\/strong><\/h4>\n

\u4eba\u7269\u7b80\u4ecb\uff1a<\/b><\/strong>\u73af\u5883\u6750\u6599\u754c\u4e0d\u5f97\u4e0d\u63d0\u7684\u90dd\u90d1\u5e73\uff0c\u4e2d\u56fd\u79d1\u5b66\u9662\u751f\u6001\u73af\u5883\u7814\u7a76\u4e2d\u5fc3\u7814\u7a76\u5458\u3001\u535a\u58eb\u751f\u5bfc\u5e08\u3001\u73af\u5883\u7eb3\u7c73\u6750\u6599\u4e0e\u6280\u672f\u7814\u7a76\u5ba4\u4e3b\u4efb\u3002\u4e2d\u79d1\u9662\u5927\u5b66\u5c97\u4f4d\u6559\u6388\u3001\u6325\u53d1\u6027\u6709\u673a\u7269\u6c61\u67d3\u63a7\u5236\u6750\u6599\u4e0e\u6280\u672f\u56fd\u5bb6\u5de5\u7a0b\u5b9e\u9a8c\u5ba4\u4e3b\u4efb\u3002\u56fd\u5bb6\u6770\u51fa\u9752\u5e74\u79d1\u5b66\u57fa\u91d1\u83b7\u5f97\u8005\u3001\u5165\u9009\u65b0\u4e16\u7eaa\u5343\u767e\u4e07\u4eba\u624d\u5de5\u7a0b\u56fd\u5bb6\u7ea7\u3002\u4e3b\u8981\u4ece\u4e8b\u6709\u5173\u5de5\u4e1a\u6c61\u67d3\u51cf\u6392\u63a7\u5236\u3001\u50ac\u5316\u79d1\u5b66\u3001\u7eb3\u7c73\u6750\u6599\u3001\u73af\u5883\u79d1\u5b66\u4e0e\u5de5\u7a0b\u3001\u73af\u5883\u653f\u7b56\u65b9\u9762\u7684\u7814\u7a76\u548c\u5f00\u53d1\u7684\u5de5\u4f5c\u3002\u5728\u5de5\u4e1a\u6c61\u67d3\u7269(\u6325\u53d1\u6027\u6709\u673a\u6c61\u67d3\u7269\u3001\u9178\u6027\u6c14\u4f53\u3001\u6e29\u5ba4\u6c14\u4f53\u7b49)\u6392\u653e\u3001\u8f6c\u5316\u53cd\u5e94\u673a\u7406\u3001\u6c61\u67d3\u63a7\u5236\u6750\u6599\u3001\u51cf\u6392\u63a7\u5236\u6280\u672f\u7b49\u65b9\u9762\u53d6\u5f97\u4e00\u4e9b\u91cd\u8981\u7684\u7814\u7a76\u6210\u679c\uff0c\u5f62\u6210\u4e86\u591a\u9879\u6c61\u67d3\u63a7\u5236\u6750\u6599\u4e0e\u51cf\u6392\u6280\u672f,\u5e76\u8fdb\u884c\u4e86\u5b9e\u9645\u5de5\u7a0b\u5e94\u7528\u3002<\/p>\n

\u8fd1\u671f\u7814\u7a76\u6210\u679c\uff1a<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u6700\u65b0\u53d1\u8868\u4e8e\u300aApplied Catalysis B: Environmental\u300b\u5149\u50ac\u5316\u52a0\u901fAs(III)\u7684\u91ca\u653e\u548c\u6c27\u5316\u3002\u5728\u73af\u5883\u4e2d\uff0c\u542b\u7837\u7684\u6c61\u6ce5\u7684\u6392\u653e\u548c\u6c89\u79ef\u91cf\u8f83\u5927\uff0c\u7279\u522b\u662f\u5728\u9178\u6027\u91c7\u77ff\u548c\u77ff\u77f3\u51b6\u70bc\u5e9f\u6c34\u7684\u5904\u7406\u8fc7\u7a0b\u4e2d\u3002\u7531\u4e8e\u7837\u79bb\u5b50\u7684\u6f5c\u5728\u91ca\u653e\uff0c\u6c61\u6ce5\u5bf9\u73af\u5883\u6784\u6210\u4e86\u91cd\u5927\u5a01\u80c1\u3002\u6c61\u6ce5\u5728\u592a\u9633\u5149\u7167\u5c04\u4e0b\uff0c\u4e0d\u4ec5As(III)\u7684\u91ca\u653e\u901f\u7387\u663e\u8457\u52a0\u5feb\uff0cAs(III)\u6c27\u5316\u4e3aAs(V)\u7684\u901f\u7387\u4e5f\u663e\u8457\u52a0\u5feb\uff0c\u8fd9\u5c06\u8fdb\u4e00\u6b65\u589e\u52a0\u6c61\u6ce5\u6392\u653e\u7684\u73af\u5883\u98ce\u9669\u3002\u672c\u6587\u7814\u7a76\u4e86\u53ef\u89c1\u5149\u5bf9\u67d0\u51b6\u70bc\u5382\u786b\u5316\u7837\u6c61\u6ce5\u6eb6\u89e3\u6c27\u5316\u7684\u5f71\u54cd\u3002\u7ed3\u679c\u8868\u660e\uff0c\u5728\u53ef\u89c1\u5149\u7167\u5c04\u4e0b\uff0cAs(III)\u79bb\u5b50\u7684\u91ca\u653e\u548cAs(III)\u5411As(V)\u7684\u6c27\u5316\u5747\u660e\u663e\u52a0\u5feb\u3002\u7535\u5b50\u987a\u78c1\u5171\u632f(EPR)\u548c\u81ea\u7531\u57fa\u731d\u706d\u5b9e\u9a8c\u8868\u660e\uff0cASS\u5728\u53ef\u89c1\u5149\u4e0b\u4f5c\u4e3a\u534a\u5bfc\u4f53\u5149\u50ac\u5316\u5242\u4ea7\u751f\u6c22\u6c27\u6839\u548c\u8d85\u6c27\u5316\u7269\u81ea\u7531\u57fa\u3002\u5728pH\u503c\u4e3a7\u548c11\u65f6\uff0c\u6c61\u6ce5\u7684\u6eb6\u89e3\u548c\u6c27\u5316\u90fd\u76f4\u63a5\u53d7\u5230.<\/b><\/sup><\/strong>O2<\/sub>\u00af\u7684\u52a0\u901f\u3002\u5728pH = 3\u65f6\uff0c\u6c61\u6ce5\u7684\u6eb6\u89e3\u7531.<\/b><\/sup><\/strong>O2<\/sub>\u00af\u548c.<\/b><\/sup><\/strong>OH\u5171\u540c\u4fc3\u8fdb\uff0c\u800cAs(III)\u7684\u6c27\u5316\u4e3b\u8981\u7531.<\/b><\/sup><\/strong>OH\u63a7\u5236\u3002\u6b64\u5916\uff0c\u56fa\u76f8\u8f6c\u5316\u4e3a\u786b(S8)\u6709\u5229\u4e8e\u6c61\u6ce5\u7684\u805a\u96c6\u548c\u6c89\u6dc0\u3002\u79bb\u5b50\u8272\u8c31\u6cd5\u548c\u4f4e\u6e29EPR\u6cd5\u5206\u522b\u6d4b\u5b9a\u4e86\u4e2d\u95f4\u786b\u79cd\u548c\u542b\u786b\u81ea\u7531\u57fa\u7684\u751f\u6210\u5bf9\u8f6c\u5316\u7684\u5f71\u54cd\u3002\u63d0\u51fa\u4e86\u4e00\u79cd\u57fa\u4e8e\u5149\u50ac\u5316\u6c27\u5316\u7684\u6a21\u578b\u6765\u652f\u6301As(III)\u5728\u53ef\u89c1\u5149\u6761\u4ef6\u4e0b\u7684\u91ca\u653e\u548c\u6c27\u5316\u884c\u4e3a[<\/sup>8]<\/sup>\u3002<\/p>\n

\"\"<\/p>\n

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\u56fd\u5916<\/b><\/strong><\/h3>\n

1. \u8036\u9c81\u5927\u5b66-<\/b><\/strong>Menachem Elimelech<\/span><\/h4>\n

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2. \u65af\u5766\u798f\u5927\u5b66-\u5d14\u5c79<\/b><\/strong><\/h4>\n

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\"\"<\/p>\n

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\u53c2\u8003\u6587\u732e<\/h3>\n

[1] Wei Teng, Nan Bai, Yang Liu, Yupu Liu, Jianwei Fan, Wei xian Zhang, Sci. Technol. 2018, 52, 230-236. \u00a0<\/p>\n

[2] Lan Ling, Xiao-Yue Huang, Wei Xian Zhang, Adv. Mater. 2018, 30, 1705703.<\/p>\n

[3] Huawei Xu,Hui Xu,\u00a0Zehan Chen,\u00a0Xianqiang Ran,\u00a0Jianwei Fan,\u00a0Wei Luo,\u00a0Zhenfeng Bian,\u00a0Wei xian Zhang, Jianping,\u00a0ACS Applied Materials & Interfaces,\u00a02019,\u00a011,\u00a04,\u00a03861-3868.<\/p>\n

[4] Hongbo Lua, Xueming Liu, Feng Liu, Zhengping Hao\uff0cJing Zhang, Zhang Lin, Yvonne Barnett\uff0cGang Pan\uff0c Cata. B: Environ, 2109, 250, 1\u20139.<\/p>\n

[5] FenglianZhang,XinZhang,\u00a0GuoxiaJiang,<\/sub>\u00a0NaLi,<\/sub>\u00a0ZhengpingHao,<\/sub>\u00a0SiqiuQu, Chem. Eng. J. 2018, 348, 831\u2013839.<\/p>\n

[6] Zhiqiang Sun, Lei Zhao, Caihong Liu,Yufei Zhen,\u00a0Jun Ma, \u00a0DOI .org\/10.1021\/acs.est.9b02745.<\/p>\n

[7] Zhuang Song Huang, Lu Wang, Yu Lei Liu, Jin Jiang, Mang Xue, Cheng-Biao Xu, Yu-Fei Zhen, Yi-Cheng Wang,Jun Ma\uff0c Sci. Technol, 2018, 52, 13897\u221213907.<\/p>\n

[8] Xiaolin Zhang, Mengfei Wu, Hao Dong, Hongchao Li, Bingcai Pan, Environ. Sci. Technol. 2017, 51, 6326\u22126334.<\/p>\n

[9] Yanyang Zhang, Xinwei She, Xiang Gao, Chao Shan, Bingcai Pan, Sci. Technol.2019, 531, 365-372.<\/p>\n

[10] Tong Wu, Chong Liu, Biao Kong, Jie Sun, Yongji Gong, Kai Liu, Jin Xie, Allen Pei, Yi Cui,ACS Cent. Sci. 2019, 5, 719\u2212726<\/p>\n

[11] Jinwei Xu, Chong Liu, Po-Chun Hsu, Jie Zhao, Tong Wu, Jing Tang, Kai Liu, Yi Cui, (2019) 10:2440 | https:\/\/doi.org\/10.1038\/s41467-019-10472-x.<\/p>\n

[12] Camrynn L. Fauseya, Ines Zuckerb , Evyatar Shaulsky, Julie B. Zimmermana, Menachem Elimelech, Eng. J., 2019, 375, 122040.<\/p>\n

\u672c\u6587\u7531Jane<\/strong>\u4f9b\u7a3f\u3002<\/p>\n

\u5f80\u671f\u56de\u987e\uff1a<\/strong><\/p>\n

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\u5927\u725b\u901f\u89c8\uff1a\u65af\u5766\u798f\u5973\u795e\u548c\u4eba\u5de5\u7535\u5b50\u76ae\u80a4<\/a><\/p>\n

\u5927\u725b\u901f\u89c8\uff1a\u795e\u5947\u7684\u6728\u5934\u2014\u2014\u770b\u201c\u6728\u5934\u4e13\u5bb6\u201d\u5982\u4f55\u73a9\u8f6c\u6728\u5934\uff01<\/a><\/p>\n

Brainy is the new sexy\u2014-\u9177\u70ab\u7684\u6559\u6388\u4e54\u4e16\u748b<\/a><\/p>\n

\u4f60\u4e0d\u77e5\u9053\u7684\u90a3\u4e9b\u4e8b\uff1a\u79d1\u7814\u5927\u4f6c\u884c\u4e3a\u4e00\u89c8<\/a><\/div>\n

\u5dfe\u5e3c\u4e0d\u8ba9\u987b\u7709\u2014\u2014\u8bb0\u6750\u6599\u9886\u57df\u7684\u79d1\u7814\u5973\u795e<\/a><\/p>\n

\u5168\u7403\u751f\u7269\u6750\u6599\u7b2c\u4e00\u95e8\u6d3e \u2014\u2014 Robert Langer \u548c\u4ed6\u7684\u5b66\u751f\u4eec<\/a><\/p>\n

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\u76d8\u70b9\u56fd\u5185\u751f\u72693D\u6253\u5370\u9886\u57df\u7684\u5341\u4f4d\u5927\u725b<\/a><\/p>\n

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