{"id":184027,"date":"2019-08-26T06:30:16","date_gmt":"2019-08-25T22:30:16","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=184027"},"modified":"2019-10-18T18:29:54","modified_gmt":"2019-10-18T10:29:54","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e9%a6%99%e6%b8%af%e5%9f%8e%e5%a4%a7%e6%94%af%e6%98%a5%e4%b9%89%e5%9b%a2%e9%98%9facs-nano%ef%bc%9a%e9%ab%98%e7%ba%a7%ce%b4-mno2%e6%ad%a3%e6%9e%81%e5%92%8c","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=184027","title":{"rendered":"\u9999\u6e2f\u57ce\u5927\u652f\u6625\u4e49\u56e2\u961fACS Nano\uff1a\u9ad8\u7ea7\u03b4-MnO2\u6b63\u6781\u548c\u81ea\u4fee\u590dZn-\u03b4-MnO2\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

ZIBs\u7684\u5404\u79cd\u7c7b\u578b\u7684\u6b63\u6781\u6750\u6599\u4e2d\uff0c\u9492\u57fa\u6750\u6599\u548cMnO2<\/sub>\u7eb3\u7c73\u6750\u6599\u56e0\u5176\u6613\u4e8e\u5236\u9020\u3001\u9ad8\u7406\u8bba\u5bb9\u91cf\u548c\u4f4e\u6210\u672c\u800c\u8131\u9896\u800c\u51fa\u3002\u7279\u522b\u662f\uff0c\u8f83\u9ad8\u7684\u653e\u7535\u7535\u538b\u548c\u8f83\u4f4e\u7684\u6bd2\u6027\u6709\u52a9\u4e8eMnO2<\/sub>\u5728ZIBs\u4e2d\u7684\u5e7f\u6cdb\u7814\u7a76\u3002\u867d\u7136\u6709\u591a\u79cd\u6676\u578b\u7684MnO2<\/sub>\u88ab\u62a5\u9053\u53ef\u7528\u4e8eZIBs\uff0c\u5c24\u5176\u662f\u62e5\u67092\u00d72\u96a7\u9053\u7ed3\u6784\u7684\u03b1-MnO2<\/sub>\uff0c\u7531\u4e8e\u5176\u4f18\u5f02\u7684\u6027\u80fd\u800c\u6210\u4e3a\u7814\u7a76\u6e29\u548cZn-MnO2<\/sub>\u7535\u6c60\u7684\u70ed\u95e8\u8bdd\u9898\u3002\u7136\u800c\uff0c\u4e0e\u8be5\u96a7\u9053\u7ed3\u6784\u76f8\u6bd4\uff0c\u03b4-MnO2<\/sub>\u7406\u8bba\u4e0a\u66f4\u9002\u5408\u4e8eZn2+<\/sup>\u7684\u50a8\u5b58\u548c\u91ca\u653e\uff0c\u8fd9\u662f\u7531\u4e8e\u5176\u6709\u66f4\u5bbd\u655e\u7684\u5c42\u72b6\u901a\u9053\u3002\u4e0d\u5e78\u5730\u662f\uff0c\u5230\u76ee\u524d\u4e3a\u6b62\uff0c\u6240\u62a5\u9053\u7684Zn\/\/\u03b4-MnO2<\/sub>\u8fd8\u6ca1\u6709\u5c55\u73b0\u51fa\u4f18\u5f02\u7684\u7535\u5316\u5b66\u6027\u80fd\u3002\u800c\u4e3b\u8981\u95ee\u9898\u8868\u73b0\u4e3a\u5feb\u901f\u7684\u5bb9\u91cf\u8870\u51cf\u548c\u4f4e\u500d\u7387\u6027\u3002\u7814\u7a76\u8868\u660e\u5176\u6839\u672c\u539f\u56e0\u5b58\u5728\u4e8e\uff0c\u03b4-MnO2<\/sub>\u7684\u5c42\u72b6\u7ed3\u6784\u4f1a\u8f6c\u53d8\u6210\u5176\u4ed6\u6676\u578b\uff0c\u8fd9\u79cd\u8f6c\u53d8\u5f15\u8d77\u4e86\u8f83\u5927\u7684\u4f53\u79ef\u53d8\u5316\u548c\u7ed3\u6784\u5012\u584c\uff0c\u8fd9\u662f\u5faa\u73af\u7a33\u5b9a\u6027\u5dee\u7684\u5173\u952e\u539f\u56e0\u3002\u6b64\u5916\uff0c\u4f4e\u5bfc\u79bb\u5b50\u7387\u4e5f\u5bfc\u81f4\u4e86\u03b4-MnO2<\/sub>\u7684\u500d\u7387\u6027\u5dee\u3002\u56e0\u6b64\uff0c\u5982\u4f55\u4f7f\u5c42\u72b6\u7ed3\u6784\u03b4-MnO2<\/sub>\u8868\u73b0\u51fa\u9ad8\u6027\u80fd\u662f\u503c\u5f97\u671f\u5f85\u7684\u3002\u5728\u5668\u4ef6\u65b9\u9762\uff0c\u57fa\u4e8e\u6c34\u7cfb\u7535\u89e3\u8d28\u7684ZIBs\u4f5c\u4e3a\u4e00\u79cd\u5177\u6709\u7edd\u5bf9\u5b89\u5168\u6027\u7684\u53ef\u7a7f\u6234\u50a8\u80fd\u5668\u4ef6\u5177\u6709\u591a\u79cd\u4f18\u52bf\u3002\u8d4b\u4e88\u5668\u4ef6\u4ee5\u81ea\u4fee\u590d\u7279\u6027\u662f\u63d0\u9ad8\u5176\u8010\u4e45\u6027\u7684\u6709\u6548\u9014\u5f84\uff0c\u4f46\u7531\u4e8e\u5176\u591a\u7ec4\u5206\u7ed3\u6784\uff0c\u5bf9\u7535\u6c60\u6765\u8bf4\u4ecd\u662f\u4e00\u4e2a\u6311\u6218\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5728\u9999\u6e2f\u57ce\u5e02\u5927\u5b66\u652f\u6625\u4e49\u6559\u6388<\/b><\/strong>\u548c\u9996\u90fd\u5e08\u8303\u5927\u5b66\u6881\u5efa\u6ce2\u526f\u7814\u7a76\u5458\u56e2\u961f\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/b><\/strong>\u5e26\u9886\u4e0b\uff0c\u4f7f\u7528\u9884\u5d4c\u5165\u65b9\u6cd5\u4e88Na+<\/sup>\u548c\u6c34\u5206\u5b50\u5d4c\u5165\u548c\u7a33\u5b9a\u5c42\u72b6\u7ed3\u6784\u5e76\u6fc0\u6d3b\u03b4-MnO2<\/sub>\u7684\u5185\u5728\u9ad8\u6027\u80fd\uff0c\u63a5\u8fd1\u7406\u8bba\u503c\u3002\u4ee5Na+<\/sup>\u548c\u6c34\u4e3a\u652f\u67f1\uff0c\u4e2d\u95f4\u5c42\u95f4\u9699\u4e3a0.72nm\u3002\u5f53\u7528\u4f5cZIBs\u7684\u4e3b\u4f53\u65f6\uff0c\u663e\u793a\u51fa\u975e\u51e1\u7684Zn2+<\/sup>\u5b58\u50a8\u6027\u80fd\uff0c\u89e3\u51b3\u4e86\u5148\u524dZn\/\/\u03b4-MnO2<\/sub>\u5de5\u4f5c\u7684\u74f6\u9888\u3002\u5b9e\u73b010,000\u6b21\u7684\u8d85\u957f\u7a33\u5b9a\u5faa\u73af\u5bff\u547d\uff0c\u4fdd\u7559\u7387\u4e3a98\uff05\u3002\u5373\u4f7f\u5728\u9ad8\u8fbe20 C\u7684\u7535\u6d41\u500d\u7387\u4e0b\uff0c\u4e5f\u4f1a\u91ca\u653e\u51fa106 mAh g-1<\/sup>\u7684\u5927\u5bb9\u91cf\u3002\u57fa\u4e8e\u8be5Zn\/\/\u03b4-MnO2<\/sub>\u7535\u6c60\u7684\u4f18\u8d8a\u6027\u80fd\u548cZIBs\u7684\u9ad8\u5b89\u5168\u6027\uff0c\u91c7\u7528\u5177\u6709\u81ea\u4fee\u590d\u80fd\u529b\u7684\u78b3\u9178\u805a\u6c28\u916f\uff08CPU\uff09\u4f5c\u4e3a\u7535\u6781\u7684\u57fa\u5e95\uff0c\u8bbe\u8ba1\u5e76\u5b9e\u73b0\u4e86\u9ad8\u6027\u80fd\u7684\u81ea\u4fee\u590dZn-MnO2<\/sub>\u7535\u6c60\u3002\u7ecf\u8fc7\u6570\u6b21\u5207\u5272\u548c\u6108\u5408\u540e\uff0c\u572810C\u7684\u6761\u4ef6\u4e0b\uff0c\u5145\u653e\u7535\u5bb9\u91cf\u4fdd\u6301\u826f\u597d\u3002\u76f8\u5173\u6210\u679c\u4ee5\u9898\u4e3a\u201c<\/b><\/strong>A Superior \u03b4-MnO<\/b><\/strong>2<\/b><\/sub><\/strong>\u00a0Cathode and a Self-Healing Zn-\u03b4-MnO<\/b><\/strong>2<\/b><\/sub><\/strong>\u00a0Battery<\/b><\/strong>\u201d<\/b><\/strong>\u53d1\u8868\u5728\u4e86ACS Nano<\/b><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe1<\/b><\/strong>\u00a0<\/b><\/strong>\u51e0\u79cd\u6c27\u5316\u9530\u6676\u4f53\u7ed3\u6784\u7684\u591a\u9762\u4f53<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

a<\/b><\/strong>\uff09<\/b><\/strong>\u03b1-MnO<\/b><\/strong>2<\/b><\/sub><\/strong>; b\uff09<\/b><\/strong>\u03b2-MnO<\/b><\/strong>2<\/b><\/sub><\/strong>; c<\/b><\/strong>\uff09<\/b><\/strong>\u03b3-MnO<\/b><\/strong>2<\/b><\/sub><\/strong>; d<\/b><\/strong>\uff09<\/b><\/strong>\u03b4-MnO<\/b><\/strong>2<\/b><\/sub><\/strong>\u3002<\/b><\/strong><\/p>\n

\u56fe2<\/b><\/strong>\u00a0<\/b><\/strong>\u03b4-MnO<\/b><\/strong>2<\/b><\/sub><\/strong>\u6b63<\/b><\/strong>\u6781\u7684<\/b><\/strong>\u7269\u7406<\/b><\/strong>\u6027\u80fd<\/b><\/strong>\u8868\u5f81<\/b><\/strong>\"\"<\/p>\n

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\u56fe3<\/b><\/strong>\u00a0\u03b4-NMOH<\/b><\/strong>\u6b63<\/b><\/strong>\u6781\u7684\u7535\u5316\u5b66\u6027\u80fd<\/b><\/strong>\u8868\u5f81<\/b><\/strong>\"\"<\/p>\n

\uff08a\uff09\u99966\u5708CV\u56fe\uff081mV\/s\uff09\u3002<\/p>\n

\uff08b\uff09\u500d\u7387\u80fd\u529b\uff081-20 C\uff09\u3002<\/p>\n

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\uff08d\uff09Zn-\u03b4-NMOH\u7535\u6c60\u7684Ragone\u56fe\u3002<\/p>\n

\uff08e\uff09Zn-\u03b4-NMOH\u7535\u6c60\u5728\u4e0d\u540c\u500d\u7387\uff088-12 C\uff09\u4e0b\u7684\u957f\u671f\u5faa\u73af\u7a33\u5b9a\u6027\u3002<\/p>\n

\uff08f\uff09Zn-\u03b4-NMOH\u7535\u6c60\u548cZn-\u03b4-NMOH-500\u7535\u6c60\u572820 C\u4e0b\u7684\u957f\u671f\u5faa\u73af\u7a33\u5b9a\u6027\uff0c\u63d2\u56fe\u663e\u793a\u572850\u4e2a\u5faa\u73af\u5185\u7684\u6d3b\u5316\u8fc7\u7a0b\u3002<\/p>\n

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\u56fe<\/b><\/strong>4 Zn-\u03b4-NMOH<\/b><\/strong>\u7535\u6c60\u7684<\/b><\/strong>\u7535\u5316\u5b66\u6027\u80fd<\/b><\/strong>\u8868\u5f81<\/b><\/strong>\"\"<\/p>\n

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\uff08b\uff09CV\u66f2\u7ebf\u4e2d\u4e09\u4e2a\u5cf0\u7684Log\uff08i\uff09vs log\uff08v\uff09\u66f2\u7ebf\u3002<\/p>\n

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\u56fe<\/b><\/strong>5<\/b><\/strong>\u00a0CPU\u7684\u81ea\u4fee\u590d<\/b><\/strong>\u6d4b\u8bd5<\/b><\/strong>\"\"<\/p>\n

\uff08a\uff09\u6f14\u793aCPU\u7684\u81ea\u4fee\u590d\u8fc7\u7a0b\uff1a\u539f\u59cbCPU\uff0c\u526a\u5207\u540e\u548c\u81ea\u4fee\u590d\u540e\u3002<\/p>\n

\uff08b\uff09CPU\u7684\u81ea\u4fee\u590d\u673a\u5236\u7684\u793a\u610f\u56fe\u3002<\/p>\n

\uff08c\uff09CPU-Zn-PAM-\u03b4-NMOH-CPU\u88c5\u7f6e\u7684\u5207\u5272\u548c\u81ea\u4fee\u590d\u8fc7\u7a0b\u4ee5\u53ca\u7ec4\u88c5\u7ed3\u6784\u7684\u56fe\u793a\u3002<\/p>\n

\uff08e\uff09\u5728\u5207\u5272\u4e4b\u524d\u548c\u81ea\u4fee\u590d\u4e4b\u540e\uff0c\u8bc1\u660eCPU\u8d1f\u8f7d\u7684\u8d1f\u6781\u548c\u6b63\u6781\u7684\u7535\u963b\u4ee5\u53ca\u65b0\u7684CPU-Zn-PAM-\u03b4-NMOH-CPU\u88c5\u7f6e\u7684\u5f00\u8def\u7535\u538b\u3002\u4e07\u7528\u8868\u4e0a\u663e\u793a\u7684\u7535\u963b\u4ee5\u03a9\u4e3a\u5355\u4f4d\uff0c\u7535\u538b\u4ee5V\u4e3a\u5355\u4f4d\u3002<\/p>\n

\uff08e\uff09\u5728\u81ea\u4fee\u590d\u524d\u540e\uff0c\u81ea\u4fee\u590d\u7684Zn-\u03b4-NMOH\u7535\u6c60\u7684\u5b9e\u9a8c\u548c\u62df\u5408EIS\u66f2\u7ebf\uff0c\u63d2\u56fe\u663e\u793a\u76f8\u5e94\u7684\u62df\u5408\u7535\u8def\u3002<\/p>\n

\uff08f\uff09\u5145\u7535\u540e\u4e0d\u540c\u81ea\u4fee\u590d\u6b21\u6570\u540e\u5f00\u8def\u7535\u538b\u53d8\u5316\u3002<\/p>\n

\uff08g\uff09\u572810 C\u65f6\uff0c\u7535\u6c60\u5bb9\u91cf\u7684\u53d8\u5316\u4e0e\u81ea\u4fee\u590d\u6b21\u6570\u7684\u5173\u7cfb\u3002<\/p>\n

\uff08h\uff09\u5728\u81ea\u4fee\u590d\u524d\u548c\u81ea\u4fee\u590d4\u6b21\u540e\u6240\u5bf9\u5e94\u7684\u653e\/\u5145\u7535\u66f2\u7ebf\u6bd4\u8f83\u3002<\/p>\n

\uff08i\uff09\u5728\u81ea\u4fee\u590d\u524d\u548c\u81ea\u4fee\u590d4 \u6b21\u540e\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\u5bf9\u6bd4\u3002<\/p>\n

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