{"id":186526,"date":"2019-09-29T06:06:22","date_gmt":"2019-09-28T22:06:22","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=186526"},"modified":"2019-09-28T21:06:46","modified_gmt":"2019-09-28T13:06:46","slug":"%e4%bb%8e%e8%bf%91%e6%9c%9fnature-science%e7%b3%bb%e5%88%97%e7%9c%8b%e6%96%b0%e6%8a%80%e6%9c%af%e5%8a%a9%e5%8a%9b%e7%94%b5%e5%8c%96%e5%ad%a6%e7%a0%94%e7%a9%b6","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=186526","title":{"rendered":"\u4ece\u8fd1\u671fNature & Science\u7cfb\u5217\u770b\u65b0\u6280\u672f\u52a9\u529b\u7535\u5316\u5b66\u7814\u7a76"},"content":{"rendered":"

\u8fd1\u5341\u5e74\u6765\uff0c\u7535\u5316\u5b66\u6280\u672f\u7a81\u98de\u731b\u8fdb\uff0c\u53d6\u5f97\u4e86\u663e\u8457\u7684\u6210\u679c\u3002\u7136\u800c\uff0c\u5f53\u524d\u7814\u7a76\u5f80\u5f80\u96c6\u4e2d\u4e8e\u7535\u6781\u50ac\u5316\u5242\u6750\u6599\u672c\u8eab\uff0c\u800c\u4e00\u4e2a\u5b8c\u6574\u7684\u7535\u5316\u5b66\u7cfb\u7edf\u662f\u7531\u591a\u4e2a\u90e8\u5206\u7ec4\u6210\u7684\u3002\u9664\u50ac\u5316\u5242\u6750\u6599\u672c\u8eab\u5916\uff0c\u7535\u89e3\u6db2\u3001\u4e09\u76f8\u754c\u9762\u3001\u7535\u89e3\u6c60\u8bbe\u8ba1\u7b49\u56e0\u7d20\u90fd\u53ef\u80fd\u5bf9\u7535\u50ac\u5316\u7cfb\u7edf\u7684\u6574\u4f53\u8868\u73b0\u4ea7\u751f\u5f71\u54cd\uff0c\u5728\u5df2\u6709\u50ac\u5316\u5242\u6027\u80fd\u7684\u57fa\u7840\u4e4b\u4e0a\uff0c\u4e00\u4e9b\u65b0\u6280\u672f\u7684\u5f15\u5165\u53ef\u663e\u8457\u63d0\u5347\u7535\u50ac\u5316\u7cfb\u7edf\u7684\u6574\u4f53\u8868\u73b0\u3002\u672c\u6587\u805a\u7126\u4e8e\u8fd1\u671fNature\u548cScience\u7cfb\u5217\u6742\u5fd7\u6700\u65b0\u6210\u679c\uff0c\u4ecb\u7ecd\u4e00\u4e9b\u65b0\u578b\u7684\u8f85\u52a9\u6280\u672f\u5728\u7535\u50ac\u5316\u7814\u7a76\u4e2d\u7684\u5e94\u7528\u3002<\/p>\n

1. Science: \u6d41\u52a8\u7535\u89e3\u6c60\u52a9\u529b\u5206\u5b50CO2<\/sub>\u7535\u8fd8\u539f\u50ac\u5316\u5242<\/h3>\n

CO2<\/sub>\u7535\u8fd8\u539f\u4f5c\u4e3a\u4e00\u9879\u91cd\u8981\u7684CO2<\/sub>\u518d\u751f\u624b\u6bb5\uff0c\u53ef\u7528\u4e8e\u56de\u6536CO2<\/sub>\u5e9f\u6c14\u751f\u4ea7\u591a\u79cd\u80fd\u6e90\u3001\u5316\u5de5\u539f\u6599\u3002\u73b0\u6709\u7684\u5f02\u76f8\u50ac\u5316\u5242\u5df2\u53ef\u5b9e\u73b0\u8f83\u5927\u8fd8\u539f\u7535\u6d41\uff08150 mA cm-2<\/sup>\uff09\uff0c\u4f46\u5728\u9ad8\u7535\u6d41\u4e0b\u4fdd\u6301\u9009\u62e9\u6027\u4f9d\u7136\u662f\u4e00\u4e2a\u5de8\u5927\u7684\u6311\u6218\uff1b\u800c\u5206\u5b50\u50ac\u5316\u5242\u5219\u53ef\u8fbe\u5230\u8f83\u9ad8\u7684\u9009\u62e9\u6027\u548c\u8f83\u4f4e\u7684\u8fc7\u7535\u4f4d\uff0c\u4f46\u5176\u7535\u6d41\u5bc6\u5ea6\u5f80\u5f80\u4e0d\u751a\u7406\u60f3\uff0c\u8fd8\u9762\u4e34\u81ea\u805a\u5408\u3001\u6eb6\u8131\u7b49\u539f\u56e0\u5bfc\u81f4\u7684\u5931\u6d3b\u3002\u6b64\u5916\uff0c\u76f8\u6bd4\u4e8e\u5b9e\u9a8c\u5ba4\u5e38\u7528\u7684\u6279\u5f0f\u7535\u89e3\u6c60\uff08\u5982H\u578b\u6c60\uff09\uff0c\u57fa\u4e8e\u819c\u7535\u6781\u7ec4\u7684\u6d41\u52a8\u578b\u7535\u89e3\u6c60\u5177\u6709\u66f4\u9ad8\u7684\u901a\u91cf\uff0c\u53ef\u5b9e\u73b0\u8fde\u7eed\u5316\u751f\u4ea7\uff0c\u66f4\u52a0\u9002\u7528\u4e8e\u5de5\u4e1a\u5316\u5927\u89c4\u6a21\u5e94\u7528\u3002\u8fd1\u65e5\uff0c\u52a0\u62ff\u5927\u4e0d\u5217\u98a0\u54e5\u4f26\u6bd4\u4e9a\u5927\u5b66Curtis P. Berlinguette<\/strong>\u4e0e\u6cd5\u56fd\u5df4\u9ece\u5927\u5b66Marc Robert<\/strong>\uff08\u5171\u540c\u901a\u8baf\uff09\u9886\u5bfc\u7684\u7814\u7a76\u5c0f\u7ec4\u4f7f\u7528\u81ea\u4e3b\u8bbe\u8ba1\u7684\u4e2d\u8bd5\u7ea7\u96f6\u95f4\u9694\u6d41\u5f0f\u7535\u89e3\u6c60\u8fdb\u884cCO2<\/sub>\u7535\u8fd8\u539f\u53cd\u5e94\uff0c\u5206\u522b\u4f7f\u7528\u78b3\u8d1f\u8f7d\u94b4\u535f\u5549\u548c\u6ce1\u6cab\u954d\u4f5c\u4e3a\u8d1f\u6781\/\u6b63\u6781\u50ac\u5316\u5242\uff0c\u5176\u4e2d\u94b4\u535f\u5549\uff08CoPc\uff09\u4e3a\u5206\u5b50CO2<\/sub>\u7535\u8fd8\u539f\u50ac\u5316\u5242\u3002\u8be5\u6d41\u5f0f\u7535\u89e3\u6c60\u53ef\u5728\u9ad8\u8fbe150 mA cm-2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u4fdd\u630195%\u4ee5\u4e0a\u7684CO\u6cd5\u62c9\u7b2c\u6548\u7387\uff0c\u5e76\u572850 mA cm-2<\/sup>\u7a33\u5b9a\u5de5\u4f5c\u8d85\u8fc7100 h\uff0c\u800c\u76f8\u6bd4\u4e4b\u4e0b\u94b4\u535f\u5549\u5728H\u578b\u7535\u89e3\u6c60\u4e2d\u53ea\u80fd\u4ee510 mA cm-2<\/sup>\u5de5\u4f5c\u4ec510 h\u5373\u5f00\u59cb\u5931\u6d3b\u3002<\/p>\n

\u8be5\u5de5\u4f5c\u4e2d\uff0c\u5b9e\u73b0\u9ad8\u7535\u6d41\u5bc6\u5ea6\u7684\u6838\u5fc3\u4e3a\u5176\u81ea\u4e3b\u8bbe\u8ba1\u7684\u96f6\u95f4\u9694\u6d41\u52a8\u7535\u89e3\u6c60\u3002\u9634\u6781\u50ac\u5316\u5242\u8d1f\u8f7d\u4e8e\u5e26\u6709\u81f4\u5bc6\u5fae\u5b54\u78b3\u5c42\u7684\u758f\u6c34\u78b3\u7eb8\u4e0a\uff0c\u5f62\u6210\u6c14\u4f53\u6269\u6563\u7535\u6781\uff08GDE\uff09\uff1b\u9633\u6781\u4f7f\u7528\u6ce1\u6cab\u954d\u4f5c\u4e3a\u6c14\u4f53\u6269\u6563\u5c42\u4ee5\u53caOER\u50ac\u5316\u5242\uff1b\u4e2d\u95f4\u4ee5\u9634\u79bb\u5b50\u4ea4\u6362\u819c\u76f8\u9694\u3002\u6b64\u5916\uff0c\u6d41\u5f0f\u7535\u89e3\u6c60\u53ef\u4f7f\u7528\u5faa\u73af\u76841M KOH\u6c34\u6eb6\u6db2\u4f5c\u4e3a\u7535\u89e3\u6db2\uff0c\u6291\u5236\u6790\u6c22\u526f\u53cd\u5e94\u3002\u76f8\u6bd4\u4e8e\u901a\u5e38\u7684\u6279\u5f0f\u53cd\u5e94\u6c60\uff0c\u8be5\u5de5\u4f5c\u4e2d\u7684\u6d41\u5f0f\u7535\u89e3\u6c60\u53ef\u5b9e\u73b0\u66f4\u9ad8\u7535\u6d41\u5bc6\u5ea6\uff0c\u4f5c\u8005\u5c06\u5176\u5f52\u56e0\u4e8e\uff1a\uff08i\uff09\u514b\u670d\u4f20\u7edfH\u578b\u6c60\u4e2d\u7684\u8d28\u91cf\u8f93\u8fd0\u95ee\u9898\uff1b\uff08ii\uff09\u4ee5\u6c14\u6001\u4e3a\u9634\u6781\u4f9b\u5e94CO2<\/sub>\uff0c\u907f\u514dCO2<\/sub>\u5728\u6c34\u6eb6\u6db2\u4e2d\u6709\u9650\u7684\u6eb6\u89e3\u5ea6\u548c\u6269\u6563\u7387\u3002\u9664\u672c\u6587\u5916\uff0c\u8fd1\u5e74\u6765\u4e5f\u6709\u6570\u7bc7\u5de5\u4f5c\u805a\u7126\u4e8e\u65b0\u578b\u7535\u89e3\u6c60\u5728\u6c34\u5206\u89e3\u3001CO2<\/sub>\u8fd8\u539f\u3001\u6c2e\u8fd8\u539f\u7b49\u7535\u5316\u5b66\u9886\u57df\u7684\u5e94\u7528\u3002\u968f\u7740\u7535\u5316\u5b66\u7814\u7a76\u9010\u6e10\u6210\u719f\u5e76\u4ece\u57fa\u7840\u79d1\u7814\u8f6c\u5411\u5e94\u7528\u7814\u7a76\uff0c\u4ee5\u819c\u7535\u6781\u7ec4\u578b\u6d41\u52a8\u7535\u89e3\u6c60\u4e3a\u4ee3\u8868\u7684\u4e2d\u8bd5\u7ea7\u7535\u89e3\u6c60\u5c06\u5728\u672a\u6765\u7684\u7814\u7a76\u4e2d\u626e\u6f14\u66f4\u52a0\u91cd\u8981\u7684\u89d2\u8272\u3002<\/p>\n

\u56fe1.<\/p>\n

\"\"<\/p>\n

A:\u94b4\u535f\u5549\u5206\u5b50\u50ac\u5316\u5242\u7ed3\u6784\uff1bB:\u96f6\u95f4\u9694\u6d41\u52a8\u5f0f\u53cd\u5e94\u6c60\u793a\u610f\u56fe\uff1bC:\u53cd\u5e94\u7535\u89e3\u6c60\u7167\u7247<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Molecular electrocatalysts can mediate fast, selective CO2<\/sub> reduction in a flow cell (Science, 2019, doi: 10.1126\/science.aax4608)<\/p>\n

2. Nat. Energy: \u56fa\u6001\u7535\u89e3\u8d28\u5b9e\u73b0CO2<\/sub>\u7535\u8fd8\u539f\u9ad8\u7eaf\u6db2\u6001\u4ea7\u7269\u8fde\u7eed\u751f\u4ea7<\/h3>\n

CO2<\/sub>\u7535\u8fd8\u539f\u901a\u5e38\u5728\u6db2\u6001\u6c34\u7cfb\u7535\u89e3\u6db2\u5982KHCO3<\/sub>\u6216KOH\u6eb6\u6db2\u4e2d\u8fdb\u884c\uff0c\u8fd9\u4e00\u8fc7\u7a0b\u4e2d\u4ea7\u751f\u7684\u6db2\u6001\u8fd8\u539f\u4ea7\u7269\u5982\u7532\u9187\u3001\u4e59\u9187\u3001\u7532\u9178\u7b49\u5c06\u4f1a\u76f4\u63a5\u6eb6\u4e8e\u7535\u89e3\u6db2\u4e2d\u5f62\u6210\u6df7\u5408\u6eb6\u6db2\uff0c\u9700\u8981\u590d\u6742\u7684\u540e\u7eed\u5206\u79bb\u63d0\u7eaf\u8fc7\u7a0b\u624d\u80fd\u5f97\u5230\u9ad8\u7eaf\u6db2\u6001\u4ea7\u54c1\uff0c\u8fd9\u671f\u95f4\u4ea7\u751f\u7684\u80fd\u8017\u4e25\u91cd\u62b5\u6d88\u4e86CO2<\/sub>\u7535\u8fd8\u539f\u672c\u8eab\u51cf\u5c11\u7684\u78b3\u6392\u653e\u3002\u5982\u679c\u5b9e\u73b0\u4f4e\u6210\u672c\u5236\u5907\u9ad8\u7eaf\u6db2\u6001\u4ea7\u7269\u662fCO2<\/sub>\u7535\u8fd8\u539f\u6280\u672f\u80fd\u5426\u8d70\u5411\u5546\u7528\u7684\u4e00\u4e2a\u5173\u952e\u56e0\u7d20\u3002\u8fd1\u671f\uff0c\u7f8e\u56fd\u8d56\u65af\u5927\u5b66Haotian Wang<\/strong>\u9886\u5bfc\u7814\u7a76\u5c0f\u7ec4\u5728Nature Energy\u53d1\u8868\u5de5\u4f5c\uff0c\u62a5\u9053\u4e86\u4e00\u79cd\u57fa\u4e8e\u56fa\u6001\u7535\u89e3\u8d28\u4e0e\u79bb\u5b50\u4ea4\u6362\u819c\u7684CO2<\/sub>\u7535\u89e3\u88c5\u7f6e\uff0c\u53ef\u5b9e\u73b0\u8fde\u7eed\u5316\u751f\u4ea7\u76f4\u63a5\u5236\u5907\u9ad8\u7eaf\u6db2\u6001\u8fd8\u539f\u4ea7\u7269\u3002\u4f7f\u7528\u9ad8HCOOH\u9009\u62e9\u6027\u7684Bi\u50ac\u5316\u5242\uff0c\u8be5\u7cfb\u7edf\u53ef\u5b9e\u73b0\u6d53\u5ea6\u9ad8\u8fbe12.1M\u7684HCOOH\u8fde\u7eed\u751f\u6210\uff0c\u6cd5\u62c9\u7b2c\u6548\u7387\u9ad8\u8fbe90%\u4ee5\u4e0a\uff1b\u6b64\u5916\uff0c\u8be5\u7cfb\u7edf\u5728100h\u7535\u89e3\u4e2d\u53ef\u6301\u7eed\u751f\u62100.1M HCOOH\u6eb6\u6db2\uff0c\u4e14\u51e0\u4e4e\u6ca1\u6709\u6027\u80fd\u8870\u51cf\u3002\u4f7f\u7528\u5546\u7528Cu2<\/sub>O\u50ac\u5316\u5242\u540c\u6837\u53ef\u5b9e\u73b0\u4e0d\u542b\u7535\u89e3\u8d28\u76d0\u7684\u9ad8\u7eafC2+<\/sup>\u6db2\u6001\u8fd8\u539f\u4ea7\u7269\u5982\u4e59\u9187\u3001\u4e59\u9178\u3001\u5f02\u4e19\u9187\u7b49\u6c34\u6eb6\u6db2\u7684\u751f\u4ea7\u3002<\/p>\n

\u56fe2. \u56fa\u4f53\u7535\u89e3\u8d28-\u79bb\u5b50\u4ea4\u6362\u819c\u578bCO2\u7535\u8fd8\u539f\u6d41\u52a8\u7535\u89e3\u6c60\u7ed3\u6784\u793a\u610f\u56fe<\/p>\n

\"\"<\/p>\n

\u8be5\u5de5\u4f5c\u7684\u91cd\u70b9\u5728\u4e8e\u5f00\u53d1\u4e86\u57fa\u4e8e\u56fa\u6001\u7535\u89e3\u8d28\u7684\u6d41\u52a8\u578bCO2\u7535\u89e3\u6c60\uff0c\u5176\u4e2d\uff0c\u9634\u6781\u3001\u9633\u6781\u50ac\u5316\u5242\u5747\u8d1f\u8f7d\u4e8e\u6c14\u4f53\u6269\u6563\u5c42\uff08GDL\uff09\u4e0a\uff0c\u5e76\u5206\u522b\u901a\u8fc7\u9634\u79bb\u5b50\u4ea4\u6362\u819c\uff08AEM\uff09\u3001\u9633\u79bb\u5b50\u4ea4\u6362\u819c\uff08CEM\uff09\u4e0e\u56fa\u6001\u7535\u89e3\u8d28\u5c42\uff08SSE\uff09\u63a5\u89e6\u3002\u56fa\u6001\u7535\u89e3\u8d28\u4e3a\u591a\u5b54\u79bb\u5b50\u5bfc\u4f53\u9ad8\u5206\u5b50\uff0c\u4f46\u5176\u4ed6\u56fa\u4f53\u7535\u89e3\u8d28\u5982\u65e0\u673a\u591a\u9178\u76d0\uff0c\u9676\u74f7\uff0c\u9ad8\u5206\u5b50\/\u9676\u74f7\u590d\u5408\u7269\uff0c\u51dd\u80f6\u7b49\u90fd\u53ef\u7528\u4e8e\u6b64\u5904\u3002\u6839\u636e\u56fa\u4f53\u7535\u89e3\u8d28\u79cd\u7c7b\u4e0d\u540c\uff0c\u6db2\u6001\u4ea7\u7269\u5c06\u5728SSE\u4e8e\u4e24\u4fa7\u79bb\u5b50\u4ea4\u6362\u819c\u754c\u9762\u751f\u6210\uff0c\u8f7d\u6c14\u6d41\u6216\u6c34\u6d41\u901a\u8fc7\u56fa\u4f53\u7535\u89e3\u8d28\u5c42\uff0c\u5c06\u6240\u5f97\u4ea7\u7269\u4ee5\u6269\u6563\u5f62\u5f0f\u5206\u79bb\uff0c\u5f97\u5230\u4e0d\u540c\u6d53\u5ea6\u7684\u6db2\u6001\u4ea7\u7269\u6eb6\u6db2\u6216\u84b8\u6c7d\uff0c\u6b64\u5916\u901a\u8fc7\u8c03\u6574\u8f7d\u4f53\u6d41\u901f\uff0c\u53ef\u5f97\u5230\u4e0d\u540c\u6d53\u5ea6\u7684\u4e0d\u542b\u7535\u89e3\u8d28\u76d0\u7684\u7eaf\u6db2\u6001\u4ea7\u7269\u6c34\u6eb6\u6db2\u3002\u8be5\u5de5\u4f5c\u4e3aCO2\u7535\u8fd8\u539f\u4e2d\u957f\u671f\u5b58\u5728\u7684\u6db2\u6001\u4ea7\u7269\u5206\u79bb\u4e0e\u63d0\u7eaf\u95ee\u9898\u63d0\u4f9b\u4e86\u4e00\u79cd\u53ef\u9760\u7684\u89e3\u51b3\u601d\u8def\uff0c\u4e14\u6709\u671b\u5c06\u8be5\u7406\u5ff5\u63a8\u5e7f\u81f3\u5176\u4ed6\u4ea7\u751f\u6db2\u6001\u4ea7\u7269\u7684\u7535\u5316\u5b66\/\u5149\u7535\u5316\u5b66\u53cd\u5e94\u4f53\u7cfb\u4e2d\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Continuous production of pure liquid fuel solutions via electrocatalytic CO2<\/sub> reduction using solid-electrolyte devices (Nature Energy, 2019, doi: 10.1038\/s41560-019-0451-x)<\/p>\n

3. Nat. Energy: \u78c1\u573a\u8f85\u52a9\u589e\u5f3a\u7535\u89e3\u6c34<\/h3>\n

\u6c27\u6790\u51fa\u53cd\u5e94\uff08OER\uff09\u4f5c\u4e3a\u7535\u89e3\u6c34\u4ea7\u6c22\u3001CO2<\/sub>\u7535\u8fd8\u539f\u3001N2<\/sub>\u7535\u8fd8\u539f\u7b49\u8fd8\u539f\u53cd\u5e94\u6700\u5e38\u89c1\u7684\u6b63\u6781\u53cd\u5e94\uff0c\u56e0\u5176\u53cd\u5e94\u52a8\u529b\u5b66\u7f13\u6162\uff0c\u8fc7\u7535\u52bf\u9ad8\uff0c\u6210\u4e3a\u7535\u89e3\u8fc7\u7a0b\u4e2d\u4e3b\u8981\u7684\u8017\u7535\u6765\u6e90\u3002\u8fd1\u51e0\u5341\u5e74\u7684\u7814\u7a76\u5927\u5e45\u63d0\u5347\u4e86OER\u50ac\u5316\u5242\u7684\u6d3b\u6027\uff0c\u4f46\u76ee\u524d\u7814\u7a76\u4e5f\u9010\u6e10\u8fdb\u5165\u74f6\u9888\uff0c\u50ac\u5316\u5242\u8fc7\u7535\u4f4d\u96be\u4ee5\u8fdb\u4e00\u6b65\u5927\u5e45\u63d0\u5347\uff0c\u800c\u5f53\u524d\u6280\u672f\u4f9d\u7136\u96be\u4ee5\u6ee1\u8db3\u5de5\u4e1a\u5316\u9700\u6c42\u30022018\u5e74\uff0c\u6cd5\u56fdMarian Chatenet\u200a<\/strong>\u7b49\u4eba\u9996\u6b21\u63d0\u51fa\u4f7f\u7528\u9ad8\u9891\u4ea4\u53d8\u78c1\u573a\u901a\u8fc7\u78c1\u70ed\u6548\u5e94\u5bf9OER\u50ac\u5316\u5242\u8fdb\u884c\u539f\u4f4d\u52a0\u70ed\uff0c\u5b9e\u73b0\u4e86\u50ac\u5316\u6027\u80fd\u7684\u5927\u5e45\u63d0\u5347\u3002Ni\u5305\u88f9FeC\u7eb3\u7c73\u9897\u7c92\u50ac\u5316\u5242\u5728\u9ad8\u9891\u4ea4\u53d8\u78c1\u573a\u4f5c\u7528\u4e0b\uff0c\u8fbe\u523020mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u6240\u9700\u7684\u8fc7\u7535\u4f4d\u663e\u8457\u4e0b\u964d\uff0c\u5bf9\u4e8eOER\u548cHER\u5206\u522b\u4e0b\u964d\u7ea6200mV\u548c100mV\uff0c\u76f8\u5f53\u4e8e\u53cd\u5e94\u6e29\u5ea6\u63d0\u9ad8\u4e86200\u2103\uff0c\u800c\u5b9e\u9645\u7684\u53cd\u5e94\u6e29\u5ea6\u63d0\u9ad8\u4e0d\u8db35\u2103\u3002\u5176\u4e2d\uff0c\u78c1\u6027FeC\u6838\u5fc3\u5177\u6709\u4f18\u5f02\u7684\u78c1\u70ed\u6027\u80fd\uff0c\u5728300kHz\u9ad8\u9891\u4ea4\u53d8\u78c1\u573a\u4e2d\u5feb\u901f\u52a0\u70ed\uff0c\u800c\u5916\u5c42Ni\u5305\u8986\u5c42\u5219\u4f5c\u4e3a\u50ac\u5316\u6d3b\u6027\u7ec4\u5206\u50ac\u5316\u6c34\u5206\u89e3\u53cd\u5e94\u3002\u8be5\u5de5\u4f5c\u9996\u6b21\u8868\u660e\u4e86\u78c1\u70ed\u6548\u5e94\u5728\u7535\u50ac\u5316\u7814\u7a76\u4e2d\u7684\u5de8\u5927\u6f5c\u529b\u3002<\/p>\n

\u8fd1\u671f\uff0c\u897f\u73ed\u7259\u5df4\u585e\u7f57\u90a3\u79d1\u6280\u5b66\u9662Jos\u00e9 Ram\u00f3n Gal\u00e1n-Mascar\u00f3s<\/strong>\u8bfe\u9898\u7ec4\u62a5\u9053\u4e86\u5355\u7eaf\u7684\u78c1\u573a\u6548\u5e94\uff08\u800c\u975e\u6b64\u524d\u7684\u78c1\u70ed\u6548\u5e94\uff09\u5bf9\u4e8e\u78c1\u6027OER\u50ac\u5316\u5242\u6027\u80fd\u7684\u63d0\u5347\uff0c\u8be5\u5de5\u4f5c\u4e2d\u78c1\u573a\u65e0\u9700\u901a\u8fc7\u7ebf\u5708\u7531\u5916\u63a5\u7535\u6e90\u989d\u5916\u751f\u6210\uff0c\u4ec5\u901a\u8fc7\u5c06\u7535\u6781\u7f6e\u4e8e\u4e24\u5757\u5546\u7528\u9495\u6c38\u78c1\u94c1\u4e4b\u95f4\u751f\u6210\u3002\u5728~450 mT\u5916\u52a0\u78c1\u573a\u4e0b\uff0c\u7b80\u5355\u7684\u6ce1\u6cab\u954d\u7535\u6781\u4ee5\u53caNi\u7b94\u8d1f\u8f7d\u591a\u79cd\u91d1\u5c5e\u50ac\u5316\u5242\u5747\u8868\u73b0\u51fa\u8fc7\u7535\u4f4d\u964d\u4f4e\u3001\u7535\u6d41\u63d0\u5347\u4ee5\u53caTafel\u659c\u7387\u4e0b\u964d\uff0c\u800c\u65e0\u9700\u7ecf\u8fc7\u4efb\u4f55\u7535\u89e3\u6c60\u6539\u9020\u3002\u78c1\u573a\u5f15\u53d1\u7684\u81ea\u65cb\u6781\u5316\u5f71\u54cd\u4e86\u53cd\u5e94\u5386\u7a0b\uff0c\u8bc1\u636e\u4e4b\u4e00\u5c31\u662f\u78c1\u751f\u7535\u6d41\u5f3a\u5ea6\u660e\u663e\u53d7pH\u53d8\u5316\u5f71\u54cd\uff0c\u5728pH14\u5904\u8fbe\u5230\u6700\u5927\uff0c\u8868\u660e\u5f3a\u78b1\u6027\u6761\u4ef6\u4e0b\u7684OER\u51b3\u901f\u6b65\u4e3a\u81ea\u65cb\u9650\u5236\u7684\u3002\u5bf9\u591a\u79cd\u4e0d\u540c\u78c1\u6027\u7684\u50ac\u5316\u5242\u6750\u6599\u8fdb\u884c\u78c1\u573a\u4f5c\u7528\u4e0b\u7535\u50ac\u5316\u6d4b\u8bd5\uff0c\u7ed3\u679c\u8868\u660e\uff0c\u975e\u78c1\u6027\u7684IrO2<\/sub>\u5728\u78c1\u573a\u4e0b\u7684\u589e\u5f3a\u53ef\u4ee5\u5ffd\u7565\uff0c\u800c\u5f3a\u78c1\u6027\u7684NiZnFe4<\/sub>Ox\u5728\u78c1\u573a\u4e0b\u4e8e1.65V\u5904\u7535\u6d41\u4ece24 mA cm-2<\/sup>\u5927\u5e45\u63d0\u5347\u81f340 mA cm-2<\/sup>\u3002\u591a\u79cd\u5bf9\u6bd4\u5b9e\u9a8c\u5747\u8868\u660e\uff0c\u8be5\u78c1\u573a\u6548\u5e94\u5e76\u975e\u78c1\u573a\u8bf1\u5bfc\u4ea7\u751f\u7684\u4f20\u8d28\u589e\u5f3a\u3001\u6e29\u5ea6\u63d0\u5347\u7b49\u4e8c\u6b21\u4f5c\u7528\uff0c\u800c\u662f\u76f4\u63a5\u6765\u6e90\u4e8e\u78c1\u573a\u6539\u53d8\u4e86\u53cd\u5e94\u5386\u7a0b\u672c\u8eab\u3002<\/p>\n

\u4ee5\u4e0a\u4e24\u7bc7\u5de5\u4f5c\u8868\u660e\u4e86\u78c1\u6548\u5e94\u8fd9\u4e00\u76ee\u524d\u7814\u7a76\u8f83\u5c11\u7684\u4f5c\u7528\u5728\u7535\u50ac\u5316\u9886\u57df\u5177\u6709\u5de8\u5927\u7684\u5e94\u7528\u6f5c\u529b\u3002\u65e0\u8bba\u662f\u901a\u8fc7\u78c1\u70ed\u5b9e\u73b0\u50ac\u5316\u5242\u9897\u7c92\u7684\u5feb\u901f\u9ad8\u6548\u539f\u4f4d\u52a0\u70ed\uff0c\u8fd8\u662f\u901a\u8fc7\u6052\u5b9a\u78c1\u573a\u76f4\u63a5\u6539\u53d8\u50ac\u5316\u53cd\u5e94\u5386\u7a0b\uff0c\u76ee\u524d\u62a5\u9053\u4f9d\u7136\u5341\u5206\u6709\u9650\uff0c\u4e14\u5176\u4e2d\u673a\u7406\u5c1a\u4e0d\u5341\u5206\u660e\u786e\u3002\u6b64\u5916\uff0c\u76ee\u524d\u5bf9\u78c1\u6548\u5e94\u589e\u5f3a\u50ac\u5316\u6d3b\u6027\u7684\u7814\u7a76\u4ec5\u9650\u4e8e\u7535\u89e3\u6c34\uff0c\u800c\u5728\u7535\u5316\u5b66\u9886\u57df\u7684\u5176\u4ed6\u7814\u7a76\u5982CO2<\/sub>\u8fd8\u539f\uff0cN2<\/sub>\u8fd8\u539f\u7b49\u4e2d\u5c1a\u65e0\u5e94\u7528\u3002<\/p>\n

\u56fe3\u00a0\u9ad8\u9891\u4ea4\u53d8\u78c1\u573a\u52a0\u70ed\u91d1\u5c5e\u7eb3\u7c73\u9897\u7c92\u589e\u5f3a\u7535\u89e3\u6c34\u7684\u88c5\u7f6e\u793a\u610f\u56fe<\/p>\n

\"\"<\/p>\n

a. \u56fa\u5b9a\u53cd\u5e94\u6c60\uff1bb. \u6d41\u52a8\u53cd\u5e94\u6c60\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Improved water electrolysis using magnetic heating of FeC\u2013Ni core\u2013shell nanoparticles (Nature Energy, 2018, doi: 10.1038\/s41560-018-0132-1); Direct magnetic enhancement of electrocatalytic water oxidation in alkaline media (Nature Energy, 2019, doi: 10.1038\/s41560-019-0404-4)<\/p>\n

4. Nat. Energy: \u9633\u6781\u8026\u5408\uff0cCO2<\/sub>\u4e0e\u7518\u6cb9\u5171\u7535\u89e3\u964d\u4f4e\u53cd\u5e94\u7535\u538b<\/h3>\n

\u7531\u53ef\u518d\u751f\u80fd\u6e90\u9a71\u52a8\u7684CO2<\/sub>\u7535\u8fd8\u539f\u53cd\u5e94\u53ef\u7528\u4e8e\u5c06\u5316\u77f3\u71c3\u6599\u71c3\u70e7\u4ea7\u751f\u7684CO2<\/sub>\u8f6c\u53d8\u4e3a\u6709\u7528\u7684\u5316\u5de5\u539f\u6599\u6216\u71c3\u6599\u5b9e\u73b0\u5faa\u73af\u518d\u5229\u7528\u3002\u76ee\u524d\u8f83\u4e3a\u901a\u7528\u7684CO2<\/sub>\u7535\u89e3\u6c60\u5c06\u9634\u6781\u7684CO2<\/sub>\u7535\u8fd8\u539f\u4e0e\u9633\u6781\u7684OER\u53cd\u5e94\u8026\u5408\u6784\u6210\u5168\u7535\u89e3\u6c60\uff0c\u5728\u8fd9\u4e00\u8fc7\u7a0b\u4e2d\u7531\u4e8eOER\u53cd\u5e94\u672c\u8eab\u9644\u52a0\u4ef7\u503c\u4e0d\u5927\uff0c\u4e14\u7535\u538b\u6781\u9ad8\uff081.23V\uff09\uff0c\u53cd\u5e94\u52a8\u529b\u5b66\u6162\uff0c\u8fc7\u7535\u52bf\u5927\uff0c\u5bfc\u81f4\u8d85\u8fc790%\u7684\u8017\u7535\u7528\u4e8e\u9a71\u52a8OER\u53cd\u5e94\uff0c\u9020\u6210\u4e25\u91cd\u7684\u7535\u80fd\u6d6a\u8d39\u3002\u9633\u6781\u8026\u5408\u4f5c\u4e3a\u4e00\u79cd\u5168\u65b0\u7684\u7535\u89e3\u6c60\u8bbe\u8ba1\u7406\u5ff5\uff0c\u8fd1\u5e74\u6765\u53d7\u5230\u4e86\u8d8a\u53d1\u5e7f\u6cdb\u7684\u5173\u6ce8\uff0c\u5176\u57fa\u672c\u5b97\u65e8\u4e3a\u901a\u8fc7\u8026\u5408\u9ad8\u9644\u52a0\u4ef7\u503c\u7684\u9633\u6781\u53cd\u5e94\u4e0e\u9634\u6781\u53cd\u5e94\uff0c\u4ece\u800c\u66ff\u4ee3OER\uff0c\u964d\u4f4e\u69fd\u7535\u538b\uff0c\u8282\u7ea6\u53cd\u5e94\u8017\u7535\uff0c\u63d0\u9ad8\u7ecf\u6d4e\u6548\u76ca\u3002\u8fd1\u671f\uff0c\u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66\u9999\u69df\u5206\u6821\u7684Paul J. A. Kenis<\/strong>\u5c0f\u7ec4\u63d0\u51fa\u5c06\u7518\u6cb9\u7535\u6c27\u5316\u4e0eCO2<\/sub>\u7535\u8fd8\u539f\u76f8\u7ed3\u5408\uff0c\u53ef\u5c06\u53cd\u5e94\u69fd\u7535\u538b\u964d\u4f4e\u7ea60.85V\uff0c\u8282\u7ea653%\u7684\u53cd\u5e94\u8017\u7535\u91cf\uff0c\u4ece\u800c\u964d\u4f4e\u5b9e\u9645\u64cd\u4f5c\u4e2d\u7684\u6210\u672c\u53ca\u78b3\u8db3\u8ff9\uff0c\u5e76\u83b7\u5f97\u9ad8\u9644\u52a0\u503c\u768412\u7535\u5b50\u8fd8\u539f\u4ea7\u7269\u5982\u4e59\u70ef\u3001\u4e59\u9187\u3002\u7518\u6cb9\u4f5c\u4e3a\u4e00\u79cd\u4f4e\u6210\u672c\u7684\u5de5\u4e1a\u751f\u7269\u67f4\u6cb9\u548c\u7682\u78b1\u5de5\u4e1a\u526f\u4ea7\u7269\uff0c\u53ef\u5927\u91cf\u5ec9\u4ef7\u83b7\u5f97\uff0c\u4e14\u5176\u7535\u6c27\u5316\u4ea7\u7269\u672c\u8eab\u4e5f\u5177\u6709\u7ecf\u6d4e\u4ef7\u503c\uff0c\u5982\u7518\u6cb9\u919b\u3001\u7532\u9178\u3001\u4e73\u9178\u7b49\u3002\u7ecf\u8fc7\u8be6\u7ec6\u5bf9\u6bd4\u6765\u6e90\u3001\u6210\u672c\u548c\u89c4\u6a21\uff0c\u7518\u6cb9\u4f5c\u4e3a\u9633\u6781\u66ff\u4ee3\u7269\u76f8\u6bd4\u4e8e\u5176\u4ed6\u66ff\u4ee3\u7269\u5982\u4e59\u9187\u3001\u5f02\u4e19\u9187\u3001\u82ef\u7532\u9187\u7b49\u5177\u6709\u663e\u8457\u4f18\u52bf\uff0c\u53ef\u6ee1\u8db3\u9ad8\u901a\u91cf\u5927\u89c4\u6a21\u5de5\u4e1a\u5316\u5e94\u7528\u9700\u6c42\u3002<\/p>\n

\u5728\u9488\u5bf9\u5355\u4e00\u7535\u6781\u53cd\u5e94\u7684\u7535\u5316\u5b66\u7814\u7a76\u4e2d\u901a\u5e38\u88ab\u5ffd\u89c6\u7684\u4e00\u4e2a\u56e0\u7d20\u662f\uff0c\u5728\u5b9e\u9645\u751f\u4ea7\u4e2d\u7535\u89e3\u69fd\u662f\u4f5c\u4e3a\u4e00\u4e2a\u53cc\u7535\u6781\u53cd\u5e94\u8fdb\u884c\u7684\u3002\u5bf9\u4e8e\u6c34\u4e2d\u8fdb\u884c\u7684\u9633\u6781\u53cd\u5e94\u6765\u8bf4\uff0c\u5bf9\u5e94\u7684\u9634\u6781\u53cd\u5e94\u603b\u662fHER\uff0c\u6240\u4ea7\u751f\u7684\u6c22\u6c14\u672c\u8eab\u5373\u53ef\u7528\u4f5c\u80fd\u6e90\uff1b\u7136\u800c\u5bf9\u4e8e\u9634\u6781\u53cd\u5e94\u4e3a\u4e3b\u7684\u4f53\u7cfb\uff0c\u5982\u7535\u89e3\u6c34\u4ea7\u6c22\uff0cCO2<\/sub>\u7535\u8fd8\u539f\uff0cN2<\/sub>\u7535\u8fd8\u539f\u7b49\u4f53\u7cfb\uff0c\u5bf9\u5e94\u9633\u6781\u53cd\u5e94\u901a\u5e38\u4e3aOER\uff0c\u800c\u4ea7\u751fO2<\/sub>\u7684\u5de5\u4e1a\u548c\u7ecf\u6d4e\u6548\u76ca\u8f83\u4f4e\uff0c\u4e14\u53cd\u5e94\u7535\u4f4d\u9ad8\uff0c\u8017\u7535\u591a\u3002\u9664\u8be5\u5de5\u4f5c\u63d0\u51fa\u7684\u7518\u6cb9\u7535\u6c27\u5316\u5916\uff0c\u8fd1\u5e74\u6765\u4e5f\u6709\u4e00\u7cfb\u5217\u5de5\u4f5c\u805a\u7126\u4e8e\u5bfb\u627eOER\u7684\u66ff\u4ee3\u53cd\u5e94\uff0c\u5176\u4e2d\u4ee5\u751f\u7269\u8d28\u6c27\u5316\u4e3a\u4e3b\uff0c\u5982\u7f9f\u7532\u57fa\u7ce0\u919b\uff08HMF\uff09\u6c27\u5316\u4e3a\u544b\u5583\u4e8c\u7532\u9178\uff08FDCA\uff09\uff0c\u4e59\u9187\u6c27\u5316\uff0c\u5c3f\u7d20\u6c27\u5316\uff0c\u6c28\u6c27\u5316\uff0c\u82ef\u7532\u9187\u6c27\u5316\u7b49\u3002\u8fd9\u7c7b\u53cd\u5e94\u5728\u964d\u4f4e\u53cd\u5e94\u69fd\u7535\u538b\u7684\u540c\u65f6\u53ef\u4ea7\u751f\u989d\u5916\u7684\u7ecf\u6d4e\u4e0e\u73af\u5883\u6548\u76ca\uff0c\u5982\u544b\u5583\u4e8c\u7532\u9178\u53ef\u4f5c\u4e3a\u5355\u4f53\u5408\u6210\u751f\u7269\u8d28PEF\u5851\u6599\uff0c\u4ece\u800c\u66ff\u4ee3\u77f3\u5316\u884d\u751f\u7684PET\u5851\u6599\uff0c\u800c\u5c3f\u7d20\u3001\u6c28\u7684\u6c27\u5316\u5219\u53ef\u7528\u4e8e\u5904\u7406\u5bcc\u6c2e\u5e9f\u6c34\uff0c\u964d\u4f4e\u6c61\u6c34\u5904\u7406\u6210\u672c\u3002\u5728\u672a\u6765\u7684\u7814\u7a76\u4e2d\uff0c\u9664\u50ac\u5316\u5242\u672c\u8eab\u5916\uff0c\u6574\u4e2a\u53cd\u5e94\u4f53\u7cfb\u7684\u7efc\u5408\u7ecf\u6d4e\/\u73af\u5883\u6548\u76ca\u4e5f\u662f\u9700\u8981\u8ba1\u5165\u8003\u91cf\u7684\u91cd\u8981\u56e0\u7d20\u3002<\/p>\n

\u56fe4. \u4f7f\u7528Ag\u7eb3\u7c73\u9897\u7c92\u8d1f\u8f7d\u7684GDL\u9634\u6781\u50ac\u5316CO2<\/sub>\u7535\u8fd8\u539f\u4e0e\u4e0d\u540c\u9633\u6781\u53cd\u5e94\u5076\u8054\u65f6\u7535\u89e3\u6c60\u7535\u538b\u4e0eCO\u5206\u7535\u6d41\u7684\u5173\u7cfb<\/p>\n

\"\"<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Co-electrolysis of CO2<\/sub> and glycerol as a pathway to carbon chemicals with improved technoeconomics due to low electricity consumption (Nature Energy, 2019, doi: 10.1038\/s41560-019-0374-6)<\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u7535\u5316\u5b66\u7cfb\u7edf\u662f\u7531\u591a\u90e8\u5206\u6784\u6210\u7684\u590d\u6742\u4f53\u7cfb\uff0c\u4ec5\u9760\u50ac\u5316\u5242\u672c\u8eab\u7684\u8bbe\u8ba1\u4e0e\u6539\u6027\u5f88\u96be\u5f97\u5230\u5168\u9762\u7684\u6027\u80fd\u63d0\u5347\u3002\u5728\u50ac\u5316\u5242\u6027\u80fd\u9762\u4e34\u95e8\u69db\u7684\u60c5\u51b5\u4e0b\uff0c\u5f15\u5165\u989d\u5916\u7684\u8f85\u52a9\u624b\u6bb5\u6216\u7cfb\u7edf\u53c2\u6570\u4f18\u5316\u53ef\u8fdb\u4e00\u6b65\u6709\u6548\u63d0\u9ad8\u50ac\u5316\u6d3b\u6027\uff0c\u5bf9\u672a\u6765\u7814\u7a76\u5177\u6709\u91cd\u8981\u53c2\u8003\u4ef7\u503c\u3002\u5176\u4e2d\uff0c\u7535\u89e3\u8d28\u3001\u7535\u89e3\u6c60\u8bbe\u8ba1\u5bf9\u4e8e\u5168\u7535\u89e3\u6c60\u7cfb\u7edf\u7684\u6027\u80fd\u5177\u6709\u5173\u952e\u6027\u7684\u5f71\u54cd\uff0c\u800c\u591a\u79cd\u8f85\u52a9\u624b\u6bb5\u5982\u78c1\u573a\u3001\u5fae\u6ce2\u3001\u8d85\u58f0\u7b49\u90fd\u53ef\u80fd\u5728\u73b0\u6709\u50ac\u5316\u5242\u57fa\u7840\u4e0a\u8fdb\u4e00\u6b65\u63d0\u5347\u50ac\u5316\u6027\u80fd\u3002\u6b64\u5916\uff0c\u968f\u7740\u7535\u5316\u5b66\u7814\u7a76\u9010\u6e10\u5411\u5b9e\u7528\u5316\u63a8\u8fdb\uff0c\u50ac\u5316\u5242\u4ee5\u53ca\u6574\u4e2a\u50ac\u5316\u4f53\u7cfb\u7684\u7ecf\u6d4e\u6027\u548c\u5b9e\u7528\u6027\u4e5f\u662f\u4e0d\u5f97\u4e0d\u8003\u91cf\u7684\u91cd\u8981\u56e0\u7d20\u3002\u7535\u5316\u5b66\u9886\u57df\u672a\u6765\u7684\u8d8b\u52bf\u5fc5\u5c06\u662f\u591a\u79cd\u5148\u8fdb\u6280\u672f\u7684\u590d\u5408\uff0c\u800c\u5355\u7eaf\u5bf9\u50ac\u5316\u5242\u672c\u8eab\u8fdb\u884c\u63d0\u5347\u5df2\u4e0d\u8db3\u4ee5\u6ee1\u8db3\u5e94\u7528\u548c\u79d1\u7814\u7684\u9700\u6c42\u3002<\/p>\n

\u672c\u6587\u7531Lane<\/strong>\u4f9b\u7a3f\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

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