{"id":187327,"date":"2019-10-12T06:30:28","date_gmt":"2019-10-11T22:30:28","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=187327"},"modified":"2019-10-11T20:13:04","modified_gmt":"2019-10-11T12:13:04","slug":"adv-mater-%ef%bc%9a%e6%97%a0%e9%93%85%e9%92%99%e7%a2%b3%e7%9f%bfmasnbr3%e5%ae%9e%e7%8e%b0%e9%a6%96%e4%b8%aa%e7%8b%ac%e7%ab%8b%e7%90%86%e6%83%b3%e5%bf%86%e5%ae%b9%e5%99%a8%e5%8f%8a%e5%9c%a8%e5%9b%9b","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=187327","title":{"rendered":"Adv. Mater.\uff1a\u65e0\u94c5\u9499\u78b3\u77ffMASnBr3\u5b9e\u73b0\u9996\u4e2a\u72ec\u7acb\u7406\u60f3\u5fc6\u5bb9\u5668\u53ca\u5728\u56db\u8fdb\u5236\u5b58\u50a8\u4e2d\u7684\u5e94\u7528"},"content":{"rendered":"

\"\"<\/p>\n

\u8bba\u6587DOI: 10.1002\/adma.201806424<\/p>\n

\u7b2c\u4e00\u4f5c\u8005\uff1a\u94b1\u6587\u864e; \u5171\u540c\u901a\u8baf\u4f5c\u8005\uff1a\u8d3a\u7ade\u8f89\u6559\u6388\u548c\u8def\u5efa\u7f8e\u6559\u6388\u3002<\/p>\n

1.\u7814\u7a76\u80cc\u666f<\/b><\/strong><\/h3>\n

\u5fc6\u963b\u5668\uff0c\u5168\u79f0\u8bb0\u5fc6\u7535\u963b\u5668(Memristor)\u3002\u5b83\u662f\u8868\u793a\u78c1\u901a\u4e0e\u7535\u8377\u5173\u7cfb\u7684\u7535\u8def\u5668\u4ef6\u3002\u5fc6\u963b\u5177\u6709\u7535\u963b\u7684\u91cf\u7eb2\uff0c\u4f46\u548c\u7535\u963b\u4e0d\u540c\u7684\u662f\uff0c\u5fc6\u963b\u7684\u963b\u503c\u662f\u7531\u6d41\u7ecf\u5b83\u7684\u7535\u8377\u786e\u5b9a\u3002\u901a\u8fc7\u6d4b\u5b9a\u5fc6\u963b\u7684\u963b\u503c\uff0c\u4fbf\u53ef\u77e5\u9053\u6d41\u7ecf\u5b83\u7684\u7535\u8377\u91cf\uff0c\u56e0\u6b64\u6709\u8bb0\u5fc6\u7535\u8377\u7684\u4f5c\u7528\u30021971\u5e74\uff0c\u8521\u5c11\u68e0\u63d0\u51fa\u5fc6\u963b\u5668\u30022008\u5e74\uff0c\u60e0\u666e\u516c\u53f8\u9996\u6b21\u5b9e\u9a8c\u4e0a\u5b9e\u73b0\u4e86\u5fc6\u963b\u5668\u4ef6\u3002\u5fc6\u963b\u5668\u7684\u51fa\u73b0\uff0c\u6709\u671b\u5b9e\u73b0\u975e\u6613\u5931\u6027\u968f\u673a\u5b58\u50a8\uff1b\u5b83\u5177\u6709\u96c6\u6210\u5ea6\u9ad8\uff0c\u529f\u8017\u4f4e\uff0c\u8bfb\u5199\u901f\u5ea6\u5feb\u7684\u7279\u70b9\uff0c\u56e0\u6b64\u8fc5\u901f\u6380\u8d77\u5fc6\u963b\u5668\u7814\u7a76\u70ed\u6f6e\u3002<\/p>\n

Fig.1<\/p>\n

\"\"<\/p>\n

(a) \u56db\u79cd\u57fa\u672c\u5143\u4ef6\u903b\u8f91\u5173\u7cfb(b)\u4ea4\u6d41\u73af\u5883\u4e2d\u7684\u5fc6\u963b\u5668(c)\u76f4\u6d41\u73af\u5883\u4e2d\u7684\u5fc6\u963b\u5668<\/p>\n

Fig.2\u5fc6\u5bb9\u5668\u53ca\u5176\u7279\u5f81<\/p>\n

\"\"<\/p>\n

(a)\u7535\u8377-\u7535\u538b\u66f2\u7ebf\u5728\u5468\u671f\u626b\u63cf\u65f6\u51fa\u73b00\u70b9\u675f\u8170\u7684\u201d8\u201d\u5b57\u56de\u73af\u3002\uff08b\uff09\u201c8\u201d\u5b57\u56de\u73af\u548c\u9891\u7387\u6709\u5173\u3002\uff08c\uff09\u7535\u5bb9-\u7535\u538b\u5468\u671f\u626b\u63cf\u65f6\u51fa\u73b0\u56de\u6ede\u66f2\u7ebf\u3002<\/p>\n

2009\u5e74\uff0cVentra\u00a0M.D.\u3001\u8521\u5c11\u68e0\u7b49\u5728\u5fc6\u963b\u5668\uff08Memristor\u5bf9\u5e94\u4e8e\u7535\u963b\uff09\u7684\u57fa\u7840\u4e0a\uff0c\u8fdb\u4e00\u6b65\u62d3\u5c55\u4e86\u8bb0\u5fc6\u5143\u4ef6\u7684\u6982\u5ff5\uff0c\u63d0\u51fa\u4e86\u5fc6\u5bb9\u5668\uff08Memcapacitor\u5bf9\u5e94\u4e8e\u7535\u5bb9\uff09\u3002\u5fc6\u5bb9\u5668\u6307\u7535\u91cf\u548c\u7535\u538b\u5b58\u5728\u975e\u7ebf\u6027\u6027\u8d28\u7684\u65b0\u5668\u4ef6\u3002\u90a3\u4e48\u5fc6\u5bb9\u5668\u76f8\u5bf9\u4e8e\u5fc6\u963b\u5668\u7a76\u7adf\u6709\u4ec0\u4e48\u4e0d\u540c\uff1f\u5176\u5b58\u50a8\u6027\u80fd\u4e0e\u5fc6\u963b\u5668\u76f8\u6bd4\u662f\u5426\u6027\u80fd\u66f4\u52a0\u4f18\u5f02\uff1f\u5fc6\u5bb9\u5668\u5e94\u7528\u9886\u57df\u8303\u56f4\u53c8\u5c06\u662f\u4ec0\u4e48\uff1f\u7b49\u7b49\u5404\u7c7b\u95ee\u9898\uff0c\u7531\u4e8e\u4e00\u76f4\u4ee5\u6765\u6ca1\u6709\u5b9e\u9a8c\u7684\u7684\u5fc6\u5bb9\u5668\uff0c\u8fd9\u4e9b\u95ee\u9898\u8fdf\u8fdf\u6ca1\u80fd\u56de\u7b54\uff0c\u5fc6\u5bb9\u5668\u7814\u7a76\u4e00\u76f4\u505c\u6ede\u4e0d\u524d\u3002<\/p>\n

2.\u6210\u679c\u7b80\u4ecb<\/b><\/strong><\/h3>\n

\u8fd1\u671f\uff0c\u8def\u5efa\u7f8e\u8bfe\u9898\u7ec4<\/b><\/strong>\u53d1\u73b0\u6709\u673a\u65e0\u673a\u6742\u5316\u9499\u949b\u77ff\u5177\u6709\u5fc6\u5bb9\u884c\u4e3a\uff08\u8fd9\u91cc\u4ee5MASnBr3<\/sub>\u4e3a\u4f8b\uff09\uff0c\u5e76\u5bf9\u8fd9\u79cd\u5fc6\u5bb9\u884c\u4e3a\u52a0\u4e8e\u5e94\u7528\u4e0e\u6807\u51c6\u5316\uff1b\u9996\u6b21\u5728\u4e16\u754c\u4e0a\u5f97\u5230\u4e86\u53ef\u4ee5\u5b9e\u9645\u4f7f\u7528\u7684\u7406\u60f3\u5fc6\u5bb9\u5668\uff0c\u5e76\u5b9e\u73b0\u4e86\u7a33\u5b9a\u7684\u56db\u8fdb\u5236\u5b58\u50a8\u3002\u540c\u65f6\u53d1\u73b0\uff0c\u4e0e\u5fc6\u963b\u5668\u5b58\u50a8\u76f8\u6bd4\uff0c\u5fc6\u5bb9\u5668\u5b58\u50a8\u6027\u80fd\u66f4\u4e3a\u7a33\u5b9a\uff08\u5982\u70ed\u7a33\u5b9a\u6027\uff09\uff0c\u8fd9\u53ef\u80fd\u4e0e\u5fc6\u963b\u5668\u4e0d\u540c\u673a\u7406\u7684\u4f5c\u7528\u7ed3\u679c\u3002\u8fd9\u5bf9\u4ee5\u540e\u7684\u7814\u7a76\uff08\u5305\u62ec\u5fc6\u963b\u5668\u3001\u5fc6\u5bb9\u5668\u7684\u6750\u6599\u4e0e\u5b9e\u9645\u5e94\u7528\uff09\u5177\u6709\u957f\u8fdc\u7684\u6307\u5f15\u610f\u4e49\u3002\u8be5\u6210\u679c\u8fd1\u65e5\u4ee5\u201cIndependent Memcapacitive Switching Triggered by Bromide Ion Migration for Quaternary Information Storage<\/b><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u671f\u520aAdvanced Materials\u6742\u5fd7\u4e0a\u3002<\/p>\n

3.\u56fe\u6587\u5bfc\u8bfb<\/b><\/strong><\/h3>\n

\u56fe\u4e00\u3001MASnBr<\/b><\/strong>3<\/b><\/sub><\/strong>\u7684\u5fc6\u5bb9\u5668\u5236\u5907<\/b><\/strong><\/p>\n

\"\"<\/p>\n

Figure 1.<\/b><\/strong>\u00a0MASnBr3<\/sub>\u8584\u819c\u8868\u9762\u5f62\u8c8c\u4e0e\u5236\u5907\u6210\u7684\u5668\u4ef6(a) \u626b\u63cf\u7535\u5b50\u663e\u5fae\u955c\u62cd\u6444\u7684MASnBr3<\/sub>\u00a0MASnBr3<\/sub>\u8584\u819c\u8868\u9762\u5f62\u8c8c. (b) MASnBr3<\/sub>\u8584\u819cX\u5c04\u7ebf\u884d\u5c04\u8c31.\u00a0(c)\u5b58\u50a8\u5668\u4ef6\u7ed3\u6784ITO\/MASnBr3<\/sub>\/Au . (d) \u5b58\u50a8\u5668\u4ef6ITO\/MASnBr3<\/sub>\/Au \u622a\u9762.<\/p>\n

\u4e24\u6b65\u6cd5\u5728ITO\u73bb\u7483\u4e0a\u5236\u5907MASnBr3<\/sub>\u81f4\u5bc6\u8584\u819c\uff0c\u5e76\u5728\u8868\u9762\u901a\u8fc7\u78c1\u63a7\u6e85\u5c04\u4eea\u5668\u6e85\u5c04\u91d1\u7535\u6781,\u5236\u5907\u6210MASnBr3<\/sub>\u57fa\u7684\u5fc6\u5bb9\u5668\u4ef6\u3002<\/p>\n

\u56fe\u4e8c\u3001\u4ee5MASnBr<\/b><\/strong>3<\/b><\/sub><\/strong>\u4e3a\u4f8b\u7684\u4e8c\u8fdb\u5236\u5fc6\u5bb9\u5668<\/b><\/strong><\/p>\n

\"\"<\/p>\n

Figure <\/b><\/strong>2<\/b><\/strong>.<\/b><\/strong>\u00a0ITO\/MASnBr3<\/sub>\/Au\u5b58\u50a8\u5668\u4ef6\u7684\u5fc6\u5bb9\u6027\u80fd. (a)\u5fc6\u5bb9\u56681\u00a0MHz\u65f6\u7ecf\u5178\u56de\u6ede\u66f2\u7ebf.(b)\u4e0d\u540c\u6d4b\u8bd5\u9891\u7387\u4e0b\u7535\u5bb9-\u7535\u538b\u56de\u6ede\u66f2\u7ebf.(c)\u5fc6\u5bb9\u56681\u00a0MHz\u65f6\u8fde\u7eed\u8fd0\u884c130\u6b21.(d)\u8fde\u7eed\u8fd0\u884c130\u6b21,0V\u8bfb\u53d6\u65f6ON\u6001OFF\u6001\u7535\u5bb9\u5206\u5e03\u8303\u56f4.(e)\u7535\u5bb9-\u7535\u538b\u56de\u6ede\u66f2\u7ebf\u4e0e\u6e29\u5ea6\u7684\u5173\u7cfb.(f)\u7535\u5bb9-\u7535\u538b\u56de\u6ede\u66f2\u7ebf\u4e0e\u5149\u654f\u7684\u5173\u7cfb.<\/p>\n

\u5bf9MASnBr3<\/sub>\u5668\u4ef6\u7684\u7535\u6027\u80fd\u8fdb\u884c\u6d4b\u8bd5\uff0c\u53d1\u73b0\u7535\u5bb9-\u7535\u538b\u66f2\u7ebf\u51fa\u73b0\u56de\u6ede\u66f2\u7ebf\uff0c\u4e25\u683c\u7b26\u5408\u8521\u5c11\u68e0\u7b49\u4eba\u5b9a\u4e49\u7684\u72ec\u7acb\u7684\u5fc6\u5bb9\u5668\u6027\u80fd\u3002\u4e14\u5b58\u50a8\u6027\u80fd\u51fa\u4f17\uff0c\u5e76\u4e14\u5bf9\u5916\u754c\u7684\u5149\u3001\u70ed\u523a\u6fc0\u4e0d\u654f\u611f\u3002<\/p>\n

\u56fe\u4e09\u3001\u4ee5MASnBr<\/b><\/strong>3<\/b><\/sub><\/strong>\u4e3a\u4f8b\u7684\u591a\u8fdb\u5236\u5b58\u50a8\u5fc6\u5bb9\u5668<\/b><\/strong><\/p>\n

\"\"<\/p>\n

Figure 3.<\/b><\/strong>\u00a0\u00a0ITO\/MASnBr3<\/sub>\/Au\u5b58\u50a8\u5668\u4ef6\u56db\u8fdb\u5236\u5b58\u50a8.(a)\u5178\u578b\u7684\u591a\u8fdb\u5236C-V\u8fdf\u6ede\u56de\u7ebf-Vmax<\/sub>\u00e00\u00e0Vmax<\/sub>\u00e00\u00e0-Vmax<\/sub>,\u8fd9\u91ccVmax<\/sub>\u00a0\u4ece\u00a01.1V,\u00a01.7V\u589e\u52a05 V. (b)\u57281MHz\u65f60V\u8bfb\u53d6\u65f6,\u56db\u79cd\u7535\u5bb9\u6001\u7684\u4fdd\u6301\u6027\u80fd.(c) \u8109\u51b2\u8bfb\u53d6\u56db\u79cd\u7535\u5bb9\u5b58\u50a8\u6001\uff08\u5176\u4e2d\u8109\u51b2\u8bbe\u7f6e\u7535\u538b\u4e3a1.1V\u3001\u00a01.7 V\u3001\u00a05 V\uff1b\u8bfb\u53d6\u7535\u538b\u4e3a0\u00a0V\uff1b\u7535\u5bb9\u5b58\u50a8\u6001\u8109\u51b2\u64e6\u9664\u7535\u538b\u4e3a-5 V\uff1b\u8109\u51b2\u5bbd\u5ea6\u4e3a30 ms\uff09(d) \u540c\u4e00\u6279\u6b2132\u4e2a\u5b58\u50a8\u5668\u4ef6\u56db\u79cd\u7535\u5bb9\u5b58\u50a8\u6001\u7684\u5206\u5e03.<\/p>\n

MASnBr3<\/sub>\u5668\u4ef6\u7684\u5177\u6709\u591a\u8fdb\u5236\u5fc6\u5bb9\u5b58\u50a8\u6027\u80fd\uff0c\u53ef\u901a\u8fc7\u7535\u538b\u5199\u81f34\u4e2a\u4e0d\u540c\u7684\u7535\u5bb9\u6001\uff08\u6700\u5927\u53ef\u4ee510\u8fdb\u5236\uff09\u3002\u65ad\u7535\u4e4b\u540e\uff0c\u4e0d\u4f46\u5b58\u50a8\u6027\u80fd\u7a33\u5b9a\uff0c\u800c\u4e14\u5176\u5668\u4ef6\u53ef\u4ee5\u76f4\u63a5\u4f7f\u7528\u8109\u51b2\u8bfb\u5199\uff0c\u5177\u6709\u826f\u597d\u7684\u6279\u6b21\u5747\u5300\u6027\u3002<\/p>\n

\u56fe\u56db\u3001\u5fc6\u5bb9\u5668\u7684\u5b58\u50a8\u673a\u7406<\/b><\/strong><\/p>\n

\"\"<\/p>\n

Figure 4. <\/b><\/strong>\u7535\u5bb9\u5668\u5f00\u5173\u5b58\u50a8\u673a\u7406.(a)(b)\u5fc6\u5bb9\u5668\u5207\u7247\u5728ON\u6001\u4e0eOFF\u6001\u65f6\u7684\u900f\u5c04\u7535\u955c\u56fe\u4e0e\u5143\u7d20\u7ebf\u6027\u5206\u5e03\u56fe.(c)\u5b58\u50a8\u5668\u4ef6\u91d1\u7535\u6781\u4e0a\u7684Br 3d\u7684x\u5c04\u7ebf\u5149\u7535\u5b50\u80fd\u8c31,\u6b64\u4e2dAu\u7535\u6781\u4ece\u5668\u4ef6\u4e0a\u5265\u79bb.<\/p>\n

(d) \u5fc6\u5bb9\u5668\u5b58\u50a8\u5668\u4ef6\u5728ON\u6001\u4e0eOFF\u6001\u65f6\u4e0e\u6e29\u5ea6\u3001\u9891\u7387\u7684\u5173\u7cfb\u00a0(e) \u5fc6\u5bb9\u5668\u7684\u5b58\u50a8\u673a\u7406\u56fe\u00a0(f) \u4f7f\u7528\u00a0p-i-n \u7ed3\u6a21\u578b\u5bf9C-V\u8fdb\u884c\u62df\u5408.<\/p>\n

\u539f\u4f4dXPS\u548c\u62c9\u66fc\u5149\u8c31\uff0cTEM\u548cSEM\u6210\u50cf\u8868\u660e\uff0c\u9499\u78b3\u77ff\u6750\u6599\u5728\u5916\u52a0\u7535\u573a\u73af\u5883\u4e0b\uff0c\u7531\u4e8e\u79bb\u5b50\u8fc1\u79fb\uff0c\u5f62\u6210\u4e86\u81ea\u63ba\u6742\uff0c\u5f62\u6210\u4e86p-i-n\u7ed3\uff0cp-i-n\u7ed3\u7535\u5bb9\u7684\u53d8\u5316\u5bf9\u5e94\u7535\u5bb9\u7684\u53d8\u6362\uff0c\u5f62\u6210\u5fc6\u5bb9\u5668\u884c\u4e3a\u3002<\/p>\n

4.\u603b\u7ed3\u4e0e\u5c55\u671b<\/b><\/strong><\/h3>\n

\u672c\u6587\u4e2d\u5668\u4ef6\u5c3d\u7ba1\u4e5f\u51fa\u73b0\u5fc6\u963b\u884c\u4e3a\uff0c\u5176\u673a\u7406\u548c\u5fc6\u5bb9\u5668\u673a\u7406\u662f\u5b8c\u5168\u4e0d\u540c\u7684\u3002\u5fc6\u963b\u662f\u7531\u4e8e\u5728\u7535\u573a\u4e0b\u5f62\u6210\u4e86\u5bfc\u7535\u7ec6\u4e1d;\u800c\u5fc6\u5bb9\u5c5e\u4e8ep-i-n\u7ed3\u7535\u5bb9,\u53ea\u9700\u8981\u7535\u8377\u5728\u5668\u4ef6\u7684\u4e24\u6781\u8fdb\u884c\u79ef\u7d2f\u5373\u53ef\u3002\u6b63\u662f\u56e0\u4e3a\u5fc6\u5bb9\u673a\u7406\u4e0e\u5fc6\u963b\u673a\u7406\u7684\u4e0d\u540c\uff0c\u5176\u70ed\u7a33\u5b9a\u6027\u8981\u6bd4\u5fc6\u963b\u5668\u6765\u7684\u7a33\u5b9a\u3002<\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f7f\u7528\u9499\u78b3\u77ff\u6750\u6599\uff08MASnBr3<\/sub>\u4e3a\u4f8b)\uff0c\u5b9e\u9a8c\u4e0a\u5b9e\u73b0\u4e86\u9996\u4e2a\u72ec\u7acb\u7684\u7406\u60f3\u5fc6\u5bb9\u5668\uff0c\u5e76\u5e94\u7528\u4e8e\u591a\u8fdb\u5236\u5b58\u50a8\uff0c\u5e76\u5efa\u7acb\u4e86\u5fc6\u5bb9\u5668\u7684\u7406\u8bba\u6a21\u578b\uff0c\u8fd9\u5c06\u4e3a\u4ee5\u540e\u7684\u5fc6\u5bb9\u5668\u66f4\u591a\u7684\u7406\u8bba\u7814\u7a76\u4e0e\u5b9e\u9645\u5e94\u7528\u63d0\u4f9b\u542f\u53d1\u3002<\/b><\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

Independent Memcapacitive Switching Triggered by Bromide Ion Migration for Quaternary Information Storage\u00a0https:\/\/doi.org\/10.1002\/adma.201806424<\/b><\/strong><\/a>. <\/b><\/strong><\/p>\n

\u672c\u6587\u7531\u82cf\u5dde\u5927\u5b66<\/b><\/strong>\u8def\u5efa\u7f8e<\/b><\/strong>\u8bfe\u9898\u7ec4<\/b><\/strong>\u4f9b\u7a3f\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaorenVIP.<\/p>\n","protected":false},"excerpt":{"rendered":"

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