{"id":189588,"date":"2019-11-14T06:30:21","date_gmt":"2019-11-13T22:30:21","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=189588"},"modified":"2019-11-13T09:24:47","modified_gmt":"2019-11-13T01:24:47","slug":"%e3%80%90%e6%8a%95%e7%a8%bf%e3%80%91%e4%b8%ad%e5%8d%97%e5%a4%a7%e5%ad%a6acs-nano%e7%94%b5%e5%8c%96%e5%ad%a6%e5%8e%9f%e4%bd%8d%e7%94%9f%e6%88%90%e6%ad%a3%e6%9e%81%e7%95%8c%e9%9d%a2%e4%bf%9d%e6%8a%a4","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=189588","title":{"rendered":"\u4e2d\u5357\u5927\u5b66ACS Nano:\u7535\u5316\u5b66\u539f\u4f4d\u751f\u6210\u6b63\u6781\u754c\u9762\u4fdd\u62a4\u5c42\u52a9\u529b\u9ad8\u6027\u80fd\u6c34\u7cfb\u950c\u79bb\u5b50\u7535\u6c60"},"content":{"rendered":"

<\/b>\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e2d\u5357\u5927\u5b66\u5468\u6c5f<\/b><\/strong>\u3001<\/b><\/strong>\u6881\u53d4\u5168\u6559\u6388<\/b><\/strong>\u5728\u56fd\u9645\u81ea\u7136\u6307\u6570\u671f\u520aACS Nano\u4e0a\u53d1\u8868\u9898\u4e3a\u201cCathode Interfacial<\/b><\/strong>\u00a0Layer Formation <\/b><\/strong>via<\/i><\/b><\/em><\/strong>\u00a0<\/b><\/strong>In Situ<\/i><\/b><\/em><\/strong>\u00a0<\/b><\/strong>Electrochemically<\/b><\/strong>\u00a0Charging<\/b><\/strong>\u00a0<\/b><\/strong>in A<\/b><\/strong>queous Zinc-Ion <\/b><\/strong>B<\/b><\/strong>attery<\/b><\/strong>\u201d\u7684\u6700\u65b0\u7814\u7a76\u6210\u679c\u3002\u90ed\u73ca\u7855\u58eb\u4e3a\u8bba\u6587\u7b2c\u4e00\u4f5c\u8005\u3002\u8be5\u6587\u7ae0\u62a5\u5bfc\u4e86\u5728\u6c34\u7cfb\u950c\u79bb\u5b50\u7535\u6c60\u4e2d\uff0cCa2<\/sub>MnO4<\/sub>\u6b63\u6781\u8868\u9762\u53ef\u4ee5\u7535\u5316\u5b66\u539f\u4f4d\u751f\u6210\u4e00\u79cd\u5355\u4e00\u6210\u5206\u7684CaSO4<\/sub>\u20222H2<\/sub>O SEI\u819c\u3002DFT\u8ba1\u7b97\u786e\u8ba4\u4e86\u5b83\u7684\u7535\u5b50\u7edd\u7f18\u6027\u548c\u79bb\u5b50\u5bfc\u7535\u6027\uff0c\u8868\u660e\u5b83\u662f\u4e00\u79cd\u5408\u9002\u7684\u754c\u9762\u4fdd\u62a4\u819c\u3002\u6b63\u6781SEI\u819c\u7684\u5b58\u5728\u53ef\u4ee5\u6709\u6548\u5730\u6291\u5236\u6750\u6599\u7684\u6eb6\u89e3\uff0c\u4e0e\u6b64\u540c\u65f6\uff0c\u8fd9\u79cd\u539f\u4f4d\u751f\u6210\u7684\u4e2d\u95f4\u5c42\u6709\u5229\u4e8e\u964d\u4f4e\u963b\u6297\u3001\u6539\u5584\u754c\u9762\u3001\u964d\u4f4e\u6d3b\u5316\u80fd\uff0c\u4ece\u800c\u63d0\u9ad8\u7535\u6c60\u500d\u7387\u6027\u80fd\u548c\u5faa\u73af\u6027\u80fd\u3002\u6b63\u6781\u7684SEI\u4fdd\u62a4\u7b56\u7565\u53ef\u80fd\u4f1a\u5bf9\u53d1\u5c55\u9ad8\u7a33\u5b9a\u6027\u7684\u6c34\u7cfb\u950c\u79bb\u5b50\u7535\u6c60\u4ee5\u53ca\u5176\u4ed6\u6c34\u7cfb\u7535\u6c60\u63d0\u4f9b\u4e00\u4e2a\u65b0\u7684\u65b9\u5411\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

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\uff08a\uff09Ca2<\/sub>MnO4<\/sub>\u7684TEM\u56fe\uff1b<\/p>\n

\uff08b\uff09Ca2<\/sub>MnO4<\/sub>\u7684SAED\u56fe\uff1b<\/p>\n

\uff08c\uff09Ca2<\/sub>MnO4<\/sub>\u7684HRTEM\u56fe\uff1b<\/p>\n

\uff08d\uff09Ca2<\/sub>MnO4<\/sub>\u7684HRTEM\u56fe\uff1b<\/p>\n

\uff08e\uff09Ca2<\/sub>MnO4<\/sub>\u7684mapping\u56fe\uff1b<\/p>\n

\uff08f\uff09Ca2<\/sub>MnO4<\/sub>\u7684\u7ebf\u6027EDS\u56fe\uff1b<\/p>\n

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\"\"<\/b><\/strong><\/p>\n

\uff08a\uff09Ca2<\/sub>MnO4<\/sub>\u9996\u4e24\u5708\u7684ex situ<\/i><\/em>\u00a0XRD\u56fe\uff1b<\/p>\n

\uff08b\uff09Ca2<\/sub>MnO4<\/sub>\u5b8c\u5168\u5145\u7535\u72b6\u6001\u4e0b\u7684SAED\u56fe\uff1b<\/p>\n

\uff08c\uff09Ca2<\/sub>MnO4<\/sub>\u5b8c\u5168\u5145\u7535\u72b6\u6001\u4e0b\u7684mapping\u56fe\uff1b<\/p>\n

\uff08d\uff09Ca2<\/sub>MnO4<\/sub>\u5b8c\u5168\u5145\u7535\u72b6\u6001\u4e0b\u7684\u5143\u7d20\u6210\u5206\u5206\u6790\u56fe\uff1b<\/p>\n

\uff08e\uff09Ca2<\/sub>MnO4<\/sub>\u5b8c\u5168\u5145\u7535\u72b6\u6001\u4e0b\u7684\u7ebf\u6027EDS\u56fe\uff1b<\/p>\n

\uff08f\uff09CaSO4<\/sub>\u20222H2<\/sub>O\u7684\u5f62\u6210\u673a\u7406\u793a\u610f\u56fe\uff1b<\/p>\n

\u56fe<\/b><\/strong>\u4e09<\/b><\/strong>\u3001<\/b><\/strong>DFT\u8ba1\u7b97<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

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\uff08d\uff09CaSO4<\/sub>\u20222H2<\/sub>O\u5d4c\u950c\u7684\u6a21\u578b\u56fe\uff1b<\/p>\n

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\uff08f\uff09\u950c\u79bb\u5b50\u8fc1\u79fb\u80fd\uff1b<\/p>\n

\u56fe<\/b><\/strong>\u56db<\/b><\/strong>\u3001<\/b><\/strong>\u7535\u5316\u5b66<\/b><\/strong>\u6027\u80fd<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

\uff08a\uff090.1 mV s-1<\/sup>\u626b\u901f\u4e0b\u7684CV\u66f2\u7ebf\u56fe\uff1b<\/p>\n

\uff08b\uff09100 mA g-1<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684GCD\u66f2\u7ebf\u56fe\uff1b<\/p>\n

\uff08c\uff09\u500d\u7387\u6027\u80fd\u56fe\uff1b<\/p>\n

\uff08d\uff091000 mA g-1<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u957f\u5faa\u73af\u6027\u80fd\u56fe\uff1b<\/p>\n

\u56fe<\/b><\/strong>\u4e94<\/b><\/strong>\u3001<\/b><\/strong>\u53cd\u5e94\u673a\u7406<\/b><\/strong>\u5206\u6790<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

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\uff08b\uff09\u4e0d\u540c\u626b\u901f\u4e0b\u7684\u8d5d\u7535\u5bb9\u8d21\u732e\u56fe\uff1b<\/p>\n

\uff08c\uff09Ca2<\/sub>MnO4<\/sub>\u548c\u03b1<\/i><\/em>-MnO2<\/sub>\u7684\u7b2c\u4e8c\u5708\u6269\u6563\u7cfb\u6570\u5bf9\u6bd4\u56fe\uff1b<\/p>\n

\uff08d\uff09\u03b1<\/i><\/em>-MnO2<\/sub>\u5728100 mA g-1<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u653e\u7535\u66f2\u7ebf\u56fe\uff1b<\/p>\n

\uff08e\uff09Ca2<\/sub>MnO4<\/sub>\u5728100 mA g-1<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u653e\u7535\u66f2\u7ebf\u56fe\uff1b<\/p>\n

\u56fe<\/b><\/strong>\u516d<\/b><\/strong>\u3001<\/b><\/strong>\u53cd\u5e94\u673a\u7406<\/b><\/strong>\u5206\u6790<\/b><\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

\uff08a\uff09Ca2<\/sub>MnO4<\/sub>\u5728\u4e0d\u540c\u7535\u89e3\u6db2\u4e0b\u7684\u5faa\u73af\u6027\u80fd\u5bf9\u6bd4\u56fe\uff1b<\/p>\n

\uff08b\uff09Ca2<\/sub>MnO4<\/sub>\u548c\u03b1<\/i><\/em>-MnO2<\/sub>\u5728\u4e0d\u540c\u7535\u89e3\u6db2\u4e0b\u7684\u9530\u6eb6\u89e3\u5bf9\u6bd4\u56fe\uff1b<\/p>\n

\uff08c\uff09\u03b1<\/i><\/em>-MnO2<\/sub>\u7684Nyquist\u66f2\u7ebf\u548c\u7b49\u6548\u7535\u8def\u56fe\uff1b<\/p>\n

\uff08d\uff09Ca2<\/sub>MnO4<\/sub>\u5728\u5b8c\u5168\u5145\u7535\u72b6\u6001\u4e0b\u7684Nyquist\u66f2\u7ebf\u548c\u7b49\u6548\u7535\u8def\u56fe\uff1b<\/p>\n

\uff08e\uff09\u03b1<\/i><\/em>-MnO2<\/sub>\u5728\u4e0d\u540c\u6e29\u5ea6\u4e0b\u7684Nyquist\u66f2\u7ebf\u56fe\uff1b<\/p>\n

\uff08f\uff09Ca2<\/sub>MnO4<\/sub>\u5728\u5b8c\u5168\u5145\u7535\u72b6\u6001\u4e0b\u4e0d\u540c\u6e29\u5ea6\u7684Nyquist\u66f2\u7ebf\u56fe\uff1b<\/p>\n

\uff08g\uff09Ca2<\/sub>MnO4<\/sub>\u548c\u03b1<\/i><\/em>-MnO2<\/sub>\u7684E<\/i><\/em>a1<\/i><\/sub><\/em>\u5bf9\u6bd4\u56fe\uff1b<\/p>\n

\uff08h\uff09Ca2<\/sub>MnO4<\/sub>\u548c\u03b1<\/i><\/em>-MnO2<\/sub>\u7684E<\/i><\/em>a2<\/i><\/sub><\/em>&E<\/i><\/em>a3<\/i><\/sub><\/em>\u5bf9\u6bd4\u56fe\uff1b<\/p>\n

\uff08i\uff09Ca2<\/sub>MnO4<\/sub>\u548c\u03b1<\/i><\/em>-MnO2<\/sub>\u7684\u6d3b\u5316\u80fd\u5bf9\u6bd4\u56fe\uff1b<\/p>\n

\uff08j\uff09Ca2<\/sub>MnO4<\/sub>\u548c\u03b1<\/i><\/em>-MnO2<\/sub>\u7684\u53cd\u5e94\u673a\u7406\u5bf9\u6bd4\u56fe\uff1b<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

\u6211\u4eec\u9996\u6b21\u628aCa2<\/sub>MnO4<\/sub>\u7528\u4e8e\u6c34\u7cfb\u950c\u79bb\u5b50\u7535\u6c60\u6b63\u6781\u6750\u6599\uff0c\u5e76\u4e14\u53d1\u73b0\u901a\u8fc7\u7535\u5316\u5b66\u539f\u4f4d\u5145\u7535\u65b9\u6cd5\u53ef\u4ee5\u751f\u6210CaSO4<\/sub>\u20222H2<\/sub>O\u754c\u9762\u4fdd\u62a4\u819c\u3002CaSO4<\/sub>\u20222H2<\/sub>O \u754c\u9762\u4fdd\u62a4\u819c\u6709\u5229\u4e8e\u6291\u5236\u4e3b\u4f53\u6750\u6599Ca2<\/sub>MnO4<\/sub>\u7684\u9530\u6eb6\u89e3\u3001\u51cf\u5c11\u963b\u6297\u3001\u6539\u5584\u754c\u9762\u3001\u964d\u4f4e\u6d3b\u5316\u80fd\uff0c\u4ece\u800c\u63d0\u9ad8\u7535\u6c60\u7684\u7a33\u5b9a\u6027\uff0c\u5ef6\u957f\u7535\u6c60\u5bff\u547d\u3002\u57281000 mA g-1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0c\u5faa\u73af1000\u5708\uff0c\u6ca1\u6709\u660e\u663e\u7684\u6ce2\u52a8\u3002\u539f\u4f4d\u751f\u6210SEI\u754c\u9762\u819c\u4fdd\u62a4\u6b63\u6781\u7684\u65b9\u6cd5\u53ef\u80fd\u6709\u52a9\u4e8e\u4fc3\u8fdb\u6c34\u7cfb\u7535\u6c60\u7684\u53d1\u5c55\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5: Cathode Interfacial Layer Formation <\/b><\/strong>via<\/i><\/b><\/em><\/strong>\u00a0<\/b><\/strong>in Situ<\/i><\/b><\/em><\/strong>\u00a0Electrochemically Charging in Aqueous Zinc-Ion Battery <\/b><\/strong>(ACS Nano, 2019, \u00a0https:\/\/doi.org\/10.1021\/acsnano.9b07042)<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u6574\u7406\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

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