{"id":197304,"date":"2020-03-25T06:28:57","date_gmt":"2020-03-24T22:28:57","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=197304"},"modified":"2020-03-24T20:29:08","modified_gmt":"2020-03-24T12:29:08","slug":"%e7%94%b5%e5%ad%90%e7%a7%91%e5%a4%a7%e6%a8%8a%e8%81%aa-%e5%94%90%e6%ad%a6%e5%9b%a2%e9%98%9fadv-funct-mater-%ef%bc%9a%e6%96%b0%e5%9e%8b%e4%b8%8d%e6%ba%b6%e6%80%a7%e6%9c%89%e6%9c%ba%e6%ad%a3%e6%9e%81","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=197304","title":{"rendered":"\u7535\u5b50\u79d1\u5927\u6a0a\u806a\/\u5510\u6b66\u56e2\u961fAdv. Funct. Mater.\uff1a\u65b0\u578b\u4e0d\u6eb6\u6027\u6709\u673a\u6b63\u6781\u7528\u4e8e\u5148\u8fdb\u6709\u673a\u94be\u79bb\u5b50\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u94be\u79bb\u5b50\uff08K-ion\uff09\u7535\u6c60\uff08PIBs\uff09\u5177\u6709\u6210\u672c\u4f4e\u3001\u7535\u5316\u5b66\u6027\u80fd\u4e0e\u9502\u79bb\u5b50\u7535\u6c60\u76f8\u4f3c\u7b49\u7a81\u51fa\u4f18\u70b9\uff0c\u5f15\u8d77\u4e86\u4eba\u4eec\u5e7f\u6cdb\u7684\u7814\u7a76\u5174\u8da3\u3002\u8fd1\u5e74\u6765\uff0c\u6709\u673a\u6c27\u5316\u8fd8\u539f\u6d3b\u6027\u5316\u5408\u7269\u9010\u6e10\u6210\u4e3a\u6781\u5177\u53d1\u5c55\u524d\u666f\u7684\u7535\u6781\u6750\u6599\u3002\u4e0d\u540c\u7684\u7814\u7a76\u5c0f\u7ec4\u5df2\u7ecf\u8bc1\u660e\uff0c\u6709\u673a\u7535\u6781\u53ef\u4ee5\u6709\u6548\u5730\u5b58\u50a8\u5927\u534a\u5f84\u7684K\u79bb\u5b50\uff0c\u8fd9\u662f\u57fa\u4e8e\u6709\u673a\u56fa\u4f53\u7684\u5927\u7a7a\u9699\u7a7a\u95f4\uff0c\u8fd9\u4f7f\u5f97\u6709\u673a\u7535\u6781\u76f8\u5bf9\u4e8e\u57fa\u4e8e\u63d2\u5c42-\u8131\u5d4c\u673a\u5236\u7684\u65e0\u673a\u7535\u6781\u5177\u6709\u660e\u663e\u7684\u4f18\u52bf\u3002\u5f53\u524d\uff0c\u5f00\u53d1\u9ad8\u6548\u7684\u6709\u673a\u7535\u6781\u4ecd\u7136\u662fPIBs\u5546\u4e1a\u5316\u7684\u91cd\u4e2d\u4e4b\u91cd\uff0c\u56e0\u4e3a\u5df2\u62a5\u9053\u7684\u6709\u673a\u7535\u6781\u7684\u4e00\u4e9b\u5173\u952e\u53c2\u6570\uff08\u5982\u80fd\u91cf\u5bc6\u5ea6\u3001\u500d\u7387\u6027\u80fd\u548c\u5faa\u73af\u7a33\u5b9a\u6027\uff09\u79bb\u5b9e\u9645\u5e94\u7528\u8fd8\u5f88\u8fdc\u3002\u76ee\u524d\uff0c\u5728PIBs\u4e2d\u4f7f\u7528\u6709\u673a\u7535\u6781\u6709\u4e24\u4e2a\u660e\u663e\u7684\u5c40\u9650\u6027\uff1a\u5927\u591a\u6570\u5c0f\u5206\u5b50\u6709\u673a\u7535\u6781\u5728\u6db2\u4f53\u7535\u89e3\u8d28\u4e2d\u6eb6\u89e3\u95ee\u9898\u4e25\u91cd\uff08\u5faa\u73af\u7a33\u5b9a\u6027\u5dee\uff09\uff1b\u4e8c\u662f\u6709\u673a\u7535\u6781\u7535\u5bfc\u7387\u76f8\u5bf9\u8f83\u597d\uff08\u4f4e\u500d\u7387\u6027\u80fd\uff09\u3002\u53ef\u559c\u7684\u662f\uff0c\u4ece\u5206\u5b50\u5de5\u7a0b\u5b66\u7684\u89d2\u5ea6\u53ef\u4ee5\u5f88\u597d\u5730\u89e3\u51b3\u4e0a\u8ff0\u95ee\u9898\uff1a1\uff09\u8bbe\u8ba1\u65b0\u578b\u7684\u6709\u673a\u4f4e\u805a\u7269\u6216\u9ad8\u5206\u5b50\u91cf\u7684\u6742\u5316\u7269\u53ef\u4ee5\u89e3\u51b3\u6eb6\u89e3\u95ee\u9898\u3002\u6709\u673a\u4f4e\u805a\u7269\/\u6742\u5408\u7269\u5177\u6709\u786e\u5b9a\u7684\u5316\u5b66\u7ed3\u6784\uff0c\u4e0e\u6709\u673a\u805a\u5408\u7269\u76f8\u6bd4\u66f4\u5bb9\u6613\u7eaf\u5316\uff1b2\uff09\u6269\u5927\u82b3\u65cf\u03c0\u5171\u8f6d\u53ef\u663e\u7740\u63d0\u9ad8\u6709\u673a\u6750\u6599\u7684\u7535\u5b50\u7535\u5bfc\u7387\uff0c\u5e7f\u6cdb\u7528\u4e8e\u6709\u673a\u53d1\u5149\u4e8c\u6781\u7ba1\uff08OLED\uff09\u548c\u6709\u673a\u592a\u9633\u80fd\u7535\u6c60\uff08OSC\uff09\u3002\u8003\u8651\u5230\u975e\u5e38\u4e30\u5bcc\u7684\u6709\u673a\u7ed3\u6784\u7684\u53ef\u8bbe\u8ba1\u6027\uff0c\u5fc5\u987b\u6709\u8bb8\u591a\u9ad8\u6027\u80fd\u7684\u6709\u673a\u7535\u6781\u7b49\u5f85\u5f00\u53d1\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u7535\u5b50\u79d1\u6280\u5927\u5b66\u6a0a\u806a<\/b><\/strong>\/\u5510\u6b66<\/b><\/strong>\u56e2\u961f<\/b><\/strong>\u4e3a\u6709\u673a\u94be\u79bb\u5b50\u7535\u6c60\uff08OPIB\uff09\u8bbe\u8ba1\u4e86\u4e00\u79cd\u65b0\u578b\u7684\u4e0d\u6eb6\u6027\u5c0f\u5206\u5b50\u6709\u673a\u6b63\u6781[N,N’-\u53cc(2-\u84bd\u918c)]-\u82dd-3,4,9,10-\u56db\u7fa7\u57fa\u4e8c\u9170\u4e9a\u80fa\uff08PTCDI-DAQ\uff0c200 mAh g-1<\/sup>\uff09\u3002\u5728\u4e8c\u7532\u6c27\u57fa\u4e59\u70f7\uff08DME\uff09\u4f7f\u75281 m KPF6<\/sub>\u7684\u534a\u7535\u6c60\uff081-3.8 V vs K+<\/sup>\/K\uff09\u4e2d\uff0cPTCDI-DAQ\u63d0\u4f9b\u4e86216 mAh g-1<\/sup>\u7684\u9ad8\u5ea6\u7a33\u5b9a\u7684\u6bd4\u5bb9\u91cf\uff0c\u5e76\u572820 A g-1<\/sup>\uff08100 C\uff09\u7684\u8d85\u9ad8\u7535\u6d41\u5bc6\u5ea6\u65f6\u4ecd\u4fdd\u6301133 mAh g-1<\/sup>\u7684\u6bd4\u5bb9\u91cf\u3002\u4f7f\u7528\u8fd8\u539f\u7684\u5bf9\u82ef\u4e8c\u7532\u9178\u94be\uff08K4<\/sub>TP\uff09\u4f5c\u4e3a\u6709\u673a\u8d1f\u6781\uff0c\u5728DME\u4e2d\u4f7f\u7528\u7535\u89e3\u8d28\u4e3a1 m KPF6<\/sub>\u7684\u6240\u5f97K4<\/sub>TP || PTCDI-DAQ OPIBs\u53ef\u5b9e\u73b0\u6700\u5927295 Wh kg-1<\/sup>\u6b63\u6781<\/sub>\uff08213 mAh g-1<\/sup>\u6b63\u6781\u00d71.38 V\uff09\u7684\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u3002 \u57280.2-3.2 V\u5de5\u4f5c\u7535\u538b\u4e0b\u62e5\u670913800 W Kg-1<\/sup>\u6b63\u6781<\/sub>\uff0894 mAh g-1<\/sup>\u00d71.38 V@10 A g-1<\/sup>\uff09\u7684\u529f\u7387\u5bc6\u5ea6\u3002\u540c\u65f6\uff0cK4<\/sub>TP || PTCDI-DAQ OPIBs\u5177\u6709\u8d85\u957f\u7684\u4f7f\u7528\u5bff\u547d\uff0c10000\u6b21\u5faa\u73af\u540e\uff0c\u5176\u7a33\u5b9a\u653e\u7535\u5bb9\u91cf\u4e3a62 mAh g-1<\/sup>\u6b63\u6781<\/sub>\uff0c3\u4e07\u6b21\u5faa\u73af\u540e\u7a33\u5b9a\u653e\u7535\u5bb9\u91cf\u4e3a40 mAh g-1<\/sup>\u6b63\u6781<\/sub>\uff083 A g-1<\/sup>\uff09\u3002PTCDI-DAQ\u7684\u7efc\u5408\u6027\u80fd\u8fbe\u5230\u76ee\u524d\u4e16\u754c\u6700\u597d\u6c34\u5e73\u3002\u8be5\u6210\u679c\u4ee5\u9898\u4e3a\u201c<\/b><\/strong>Novel Insoluble Organic Cathodes for Advanced Organic K-Ion Batteries<\/b><\/strong>\u201d<\/b><\/strong>\u53d1\u8868\u5728\u4e86Adv. Funct. Mater.<\/b><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe1 <\/b><\/strong>PTCDI-DAQ<\/b><\/strong>\u7684\u7ed3\u6784\u8868\u5f81<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

a\uff09PTCDI-DAQ\u7684\u4e00\u6b65\u5408\u6210\u8def\u7ebf\uff1b<\/p>\n

b\uff09PTCDI-DAQ\u5728D2<\/sub>SO4<\/sub>\u4e2d\u76841<\/sup>H NMR\u5149\u8c31\uff1b\u00a0<\/p>\n

c\uff09\u5206\u522b\u4e3aAQNH2<\/sub>\u3001PTCDA\u3001PTCDI\u548cPTCDI-DAQ\u7684FT-IR\u5149\u8c31\uff1b\u00a0<\/p>\n

d\uff094\u79cd\u6709\u673a\u5316\u5408\u7269\u7684FT-IR\u5149\u8c31\u7684\u653e\u5927\u90e8\u5206\u3002<\/p>\n

\u56fe2 <\/b><\/strong>PTCDI-DAQ<\/b><\/strong>\u7684\u6c27\u5316\u8fd8\u539f\u673a\u5236<\/b><\/strong>\"\"<\/p>\n

a\uff09\u534a\u7535\u6c60\u4e2dPTCDI-DAQ\u7684\u591a\u91cdCV\u66f2\u7ebf\uff08\u626b\u63cf\u901f\u7387\u4e3a0.1 mV s-1<\/sup>\uff0c\u7535\u538b\u4e3a1-3.8 V vs K+<\/sup>\/K\uff09\uff1b<\/p>\n

b\uff09\u534a\u7535\u6c60\u4e2dPTCDI-DAQ\u7684\u5f02\u4f4dFT-IR\u5149\u8c31\uff1b<\/p>\n

c\uff09OPIBs\u4e2dPTCDI-DAQ\u7684\u6c27\u5316\u8fd8\u539f\u673a\u5236\u3002<\/p>\n

\u56fe3<\/b><\/strong>\u00a0\u4e0d\u540c\u7535\u89e3\u8d28\u4e2d<\/b><\/strong>PTCDI-DAQ\u7684\u5145\u653e\u7535\u66f2\u7ebf<\/b><\/strong>\"\"<\/p>\n

a\uff09DME\u4e2d1 M\u00a0KPF6<\/sub>\u7535\u89e3\u8d28\u4e2dPTCDI-DAQ\u7684\u5145\u653e\u7535\u66f2\u7ebf\uff1b<\/p>\n

b\uff09DME\u4e2d1 M\u00a0KPF6<\/sub>\u00a0+\u00a00.05 M\u00a0LiTFSI\u7535\u89e3\u8d28\u4e2dPTCDI-DAQ\u7684\u5145\u653e\u7535\u66f2\u7ebf\u3002<\/p>\n

\u56fe4 <\/b><\/strong>\u4e0d\u540c\u7535\u89e3\u8d28\u7684K||Cu\u7535\u6c60\u7684\u7535\u538b\u66f2\u7ebf<\/b><\/strong>\"\"<\/p>\n

a\uff09DME\u4e2d1 M\u00a0KPF6<\/sub>\u7684K||Cu\u7535\u6c60\u7684\u7535\u538b\u66f2\u7ebf\uff1b<\/p>\n

b\uff09DME\u4e2d\u76841 M\u00a0KPF6<\/sub>\u00a0+\u00a00.05 M\u00a0LiTFSI\u7684K||Cu\u7535\u6c60\u7684\u7535\u538b\u66f2\u7ebf\u3002<\/p>\n

c\uff09\u5206\u522b\u4f7f\u7528DME\u4e2d\u76841 M\u00a0KPF6<\/sub>\u548cDME\u4e2d\u76841 M\u00a0KPF6<\/sub>\u00a0+\u00a00.05 M\u00a0LiTFSI\u57281 mA cm-2<\/sup>\u65f6\uff0cK||K\u5bf9\u79f0\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd\u3002<\/p>\n

\u56fe<\/b><\/strong>5 <\/b><\/strong>PTCDI-DAQ<\/b><\/strong>\u7684\u5faa\u73af\u66f2\u7ebf<\/b><\/strong>\"\"<\/p>\n

a\uff09\u5e26\u6709LiTFSI\u7684PTCDI-DAQ\u5728100 mA g\u22121<\/sup>\u5904\u7684\u5faa\u73af\u66f2\u7ebf\uff1b<\/p>\n

b\uff09PTCDI-DAQ\u7684\u500d\u7387\u6027\u80fd\uff1b<\/p>\n

c\uff09PTCDI-DAQ\u57283 A g-1<\/sup>\u4e0b\u7684\u957f\u5faa\u73af\u66f2\u7ebf\uff1b<\/p>\n

d\uff09\u8fc4\u4eca\u4e3a\u6b62\u62a5\u544a\u7684K\u79bb\u5b50\u534a\u7535\u6c60\u4e2d\u9009\u5b9a\u6b63\u6781\u7684\u500d\u7387\u6027\u80fd\u6c47\u603b\u3002<\/p>\n

\u56fe<\/b><\/strong>6<\/b><\/strong>\u00a0<\/b><\/strong>PTCDI-DAQ\u5728\u4e0d\u540c\u626b\u63cf\u901f\u7387\u4e0b\u7684CV\u66f2\u7ebf<\/b><\/strong>\"\"<\/p>\n

a\uff09GITT\u66f2\u7ebf\u548cb\uff09PTCDI-DAQ\u7684\u5b9e\u73b0K+<\/sup>\u6269\u6563\u7cfb\u6570\uff08D\uff09\uff1b<\/p>\n

c\uff09PTCDI-DAQ\u57280.1~10 mV s-1<\/sup>\u7684\u4e0d\u540c\u626b\u63cf\u901f\u7387\u4e0b\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

d\uff09\u5cf0\u503c\u7535\u6d41\uff08i\uff09\u4e0e\u4e0d\u540c\u626b\u63cf\u901f\u7387\u4e4b\u95f4\u7684\u5bf9\u6570\uff08log\uff09\u5173\u7cfb\u7684\u7ebf\u6027\u62df\u5408\u7ed3\u679c\u3002<\/p>\n

\u56fe<\/b><\/strong>7<\/b><\/strong>\u00a0<\/b><\/strong>PTCDI-DAQ\u57fa\u6b63\u6781\u548cK<\/b><\/strong>4<\/b><\/sub><\/strong>TP\u8d1f\u6781\u7684OPIBs\u7684\u7ed3\u6784<\/b><\/strong>\"\"<\/p>\n

a\uff09PTCDI-DAQ\u57fa\u6b63\u6781\u548cK4<\/sub>TP\u8d1f\u6781\u7684OPIBs\u7684\u7ed3\u6784\uff1b<\/p>\n

b\uff09OPIBs\u70b9\u4eae\u4e86\u7ea2\u8272LED\u3002<\/p>\n

\u56fe<\/b><\/strong>8<\/b><\/strong>\u00a0<\/b><\/strong>K<\/b><\/strong>4<\/b><\/sub><\/strong>TP||PTCDI-DAQ<\/b><\/strong>\u5168<\/b><\/strong>\u7535\u6c60<\/b><\/strong>\u7684\u7535\u5316\u5b66\u8868\u5f81<\/b><\/strong>\"\"<\/p>\n

a\uff09K4<\/sub>TP || PTCDI-DAQ\u5168\u7535\u6c60\u57280.2-3.2 V\u7535\u538b\u8303\u56f4\u5185\u7684\u5145\u653e\u7535\u66f2\u7ebf\uff1b<\/p>\n

b\uff09\u5168\u7535\u6c60\u7684300\u4e2a\u5faa\u73af\u66f2\u7ebf\uff1b<\/p>\n

c\uff09\u5168\u7535\u6c60\u7684\u500d\u7387\u6027\u80fd\uff1b<\/p>\n

d\uff09\u8fd9\u9879\u5de5\u4f5c\u4e0e\u5176\u4ed6K\u79bb\u5b50\u5168\u7535\u6c60\u7684\u80fd\u91cf\u5bc6\u5ea6\u548c\u529f\u7387\u5bc6\u5ea6\u7684\u6bd4\u8f83\uff1b<\/p>\n

e\uff093 A g-1<\/sup>\u65f6\u5168\u7535\u6c60\u7684\u957f\u5faa\u73af\u66f2\u7ebf\u3002<\/p>\n

\u3010\u5c0f\u7ed3<\/b><\/strong>\u3011<\/p>\n

\u62a5\u9053\u4e86\u4e00\u79cd\u65b0\u578b\u7684\u4e0d\u6eb6\u6027\u5c0f\u5206\u5b50\u6709\u673a\u6b63\u6781PTCDI-DAQ\uff0c\u5176\u6bd4\u5bb9\u91cf\u4e3a200 mAh g\u22121<\/sup>\u3002PTCDI-DAQ\u5728\u534a\u7535\u6c60\u548c\u5168\u7535\u6c60\u4e2d\u5747\u8868\u73b0\u51fa\u4ee4\u4eba\u5370\u8c61\u6df1\u523b\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u3001\u9ad8\u901f\u7387\u6027\u80fd\u548c\u957f\u5bff\u547d\u3002\u4f8b\u5982\uff0c\u6240\u5f97\u5230\u7684\u5168\u7535\u6c60\u53ef\u4ee5\u63d0\u4f9b295 Wh kg-1<\/sup>\u6b63<\/sub>\u6781<\/sub>\u7684\u9ad8\u80fd\u91cf\u5bc6\u5ea6\uff0c\u9ad8\u529f\u7387\u5bc6\u5ea6\u768413\u202f800 Wkg-1<\/sup>\u6b63<\/sub>\u6781<\/sub>\u548c\u8d85\u8fc730 000\u4e2a\u5faa\u73af\u7684\u8d85\u957f\u5bff\u547d\u3002\u603b\u4e4b\uff0c\u8fd9\u9879\u5de5\u4f5c\u4e3a\u9ad8\u6027\u80fd\u6709\u673a\u7535\u6781\u7684\u5206\u5b50\u8bbe\u8ba1\u6253\u5f00\u4e86\u5927\u95e8\uff0c\u540c\u65f6\u4e5f\u4e3a\u6709\u673a\u94be\u79bb\u5b50\u7535\u6c60\u7684\u53d1\u5c55\u8fc8\u51fa\u4e86\u91cd\u8981\u7684\u4e00\u6b65\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>Novel Insoluble Organic Cathodes for Advanced Organic K-Ion Batteries<\/u><\/a>\uff08Adv. Funct. Mater.\uff0c 2020\uff0cDOI:10.1002\/adfm.202000675\uff09<\/p>\n

\u672c\u6587\u7531\u6728\u6587\u97ec<\/b><\/strong>\u7ffb\u8bd1\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

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