{"id":197455,"date":"2020-03-13T06:28:01","date_gmt":"2020-03-12T22:28:01","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=197455"},"modified":"2020-03-12T21:38:49","modified_gmt":"2020-03-12T13:38:49","slug":"adv-funct-mater-%e9%80%9a%e8%bf%87%e6%bf%80%e5%ad%90%e7%9a%84%e8%b0%83%e6%8e%a7%e5%92%8c%e5%88%86%e9%85%8d%e8%8e%b7%e5%be%97%e8%b6%8520%e9%87%8f%e5%ad%90%e6%95%88%e7%8e%87%e7%9a%84%e7%99%bd","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=197455","title":{"rendered":"Adv. Funct. Mater. :\u901a\u8fc7\u6fc0\u5b50\u7684\u8c03\u63a7\u548c\u5206\u914d\u83b7\u5f97\u8d8520%\u91cf\u5b50\u6548\u7387\u7684\u767d\u5149\u6709\u673a\u53d1\u5149\u4e8c\u6781\u7ba1"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u767d\u5149\u6709\u673a\u53d1\u5149\u4e8c\u6781\u7ba1\uff08WOLEDs\uff09\u5177\u6709\u8f7b\u8d28\u3001\u67d4\u6027\u3001\u6210\u672c\u4f4e\u3001\u5de5\u827a\u7b80\u5355\u7b49\u4f18\u70b9\uff0c\u56e0\u6b64\u53d7\u5230\u5e7f\u6cdb\u7684\u7814\u7a76\u3002\u7814\u7a76\u8005\u5f80\u5f80\u901a\u8fc7\u6539\u53d8\u6750\u6599\u548c\u5668\u4ef6\u7ed3\u6784\u6765\u63d0\u5347WOLEDs\u5668\u4ef6\u7684\u6027\u80fd\u3002\u4e5f\u53ef\u4ee5\u901a\u8fc7\u8367\u5149\u6750\u6599\u7684\u7535\u81f4\u6fc0\u5b50\u884c\u4e3a\u6765\u6784\u5efa\u9ad8\u6548\u7387WOLEDs\u3002\u5c3d\u7ba1\u4f20\u7edf\u8367\u5149\u7c89\u6784\u6210\u7684WOLEDs\u5177\u6709\u8272\u7eaf\u5ea6\u9ad8\u3001\u6548\u7387\u4f4e\u3001\u4e0d\u542b\u7a00\u6709\u91d1\u5c5e\u7b49\u4f18\u70b9\uff0c\u4f46\u7531\u4e8e\u7f3a\u5c11\u5bf9\u4e09\u7ebf\u6001\u6fc0\u5b50\u7684\u5229\u7528\u800c\u4f7f\u5176\u53d1\u5149\u6548\u7387\u53d7\u5230\u7406\u8bba\u4e0a\u7684\u9650\u5236\u3002\u4ecb\u4e8e\u5355\u7ebf\u6001\u548c\u4e09\u7ebf\u6001\u6fc0\u5b50\u7684\u5bff\u547d\u53ca\u6269\u6563\u8ddd\u79bb\u4e0d\u540c\uff0c\u56e0\u6b64\u6709\u671b\u53ef\u4ee5\u5145\u5206\u5efa\u7acb\u591a\u4e2a\u5171\u632f\u80fd\u91cf\u8f6c\u79fb\u901a\u9053\u6765\u7a81\u7834\u4f20\u7edf\u91cf\u5b50\u6548\u7387\u7684\u9650\u5236\u3002<\/p>\n

\u3010\u7814\u7a76\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u82cf\u5dde\u5927\u5b66\u848b\u4f50\u6743\u6559\u6388\u7b49\u4eba\u5728Adv. Funct. Mater.\u4e0a\u53d1\u8868\u4e86\u4e00\u7bc7\u901a\u8fc7\u6fc0\u5b50\u7684\u8c03\u63a7\u548c\u5206\u914d\u83b7\u5f97\u9ad8\u6548\u7eaf\u8367\u5149\u767d\u5149\u6709\u673a\u53d1\u5149\u4e8c\u6781\u7ba1\u7684\u6587\u7ae0\uff0c\u9898\u76ee\u4e3a\u201cAll-Fluorescence White Organic Light-Emitting Diodes Exceeding 20% EQEs by Rational Manipulation of Singlet and Triplet Excitons\u201d\u3002\u65e9\u57281995\u5e74\uff0c\u65e5\u672c\u5c71\u5f62\u5927\u5b66\u7684Kido\u6559\u6388\u7b49\u4eba\u62a5\u9053\u4e86\u7b2c\u4e00\u4e2a\u57fa\u4e8e\u8367\u5149\u7684OLED\u767d\u5149\u5668\u4ef6\uff08Science 1995, 267, 1332.\uff09\uff0c\u4f46\u662f\u8367\u5149\u5668\u4ef6\u672c\u8eab\u7684\u4f4e\u6548\u7387\u5236\u7ea6\u4e86\u5176\u8fdb\u4e00\u6b65\u53d1\u5c55\uff0c\u968f\u7740\u6709\u673a\u78f7\u5149\u53d1\u5149\u548c\u70ed\u6fc0\u6d3b\u5ef6\u8fdf\u8367\u5149\u6750\u6599\uff08TADF\uff09\u7684\u5d1b\u8d77\uff0c\u8367\u5149\u767d\u5149\u5668\u4ef6\u7684\u7814\u7a76\u9010\u6e10\u6de1\u51fa\u4e86\u821e\u53f0\u4e2d\u5fc3\u3002\u8fd1\u5e74\u6765\uff0c\u7814\u7a76\u4eba\u5458\u53d1\u73b0TADF\u6750\u6599\u9664\u4e86\u81ea\u8eab\u53d1\u5149\u4e4b\u5916\uff0c\u8fd8\u53ef\u4ee5\u4f5c\u4e3a\u654f\u5316\u6750\u6599\u6fc0\u6d3b\u4f20\u7edf\u7684\u8367\u5149\u6750\u6599\u6765\u53d6\u5f97\u9ad8\u6548\u5668\u4ef6\u3002\u8fd9\u4e2a\u7b56\u7565\u5728\u5929\u84dd\u5149\u3001\u7eff\u5149\u548c\u7ea2\u5149\u5668\u4ef6\u4e2d\u53d6\u5f97\u4e86\u6210\u529f\uff0c\u4f3c\u4e4e\u9ad8\u6548\u8367\u5149\u767d\u5149\u53ef\u4ee5\u7528\u8fd9\u79cd\u65b9\u6848\u642d\u914d\u201c\u84dd+\u9ec4\u201d\u7684\u989c\u8272\u8c03\u914d\u6765\u5b9e\u73b0\uff0c\u4f46\u5b9e\u9645\u96be\u5ea6\u5728\u4e8e\u654f\u5316\u7684\u7eaf\u84dd\u5149\u6216\u8005\u6df1\u84dd\u5149\u90fd\u975e\u5e38\u96be\u5f97\uff0c\u5bf9\u4e3b\u4f53\u3001TADF\u654f\u5316\u5242\u90fd\u63d0\u51fa\u82db\u523b\u7684\u6750\u6599\u8981\u6c42\u6c42\u3002\u8be5\u6587\u7684\u4f5c\u8005\u63d0\u51fa\u4e86\u4e00\u4e2a\u66f4\u4e3a\u7b80\u4fbf\u7684\u66ff\u4ee3\u65b9\u6848\uff0c\u5373\u84dd\u5149\u90e8\u5206\u91c7\u7528\u4f20\u7edf\u7684\u8367\u5149\u6750\u6599\uff0c\u800c\u4e0d\u662f\u88ab\u654f\u5316\u7684\u84dd\u8272\u8367\u5149\uff0c\u867d\u7136\u5176\u6548\u7387\u504f\u4f4e\uff0c\u4f46\u662f\u7ed3\u5408\u5408\u7406\u7684\u6fc0\u5b50\u5206\u914d\uff0c\u5373\u5c0625%\u7684\u5355\u7ebf\u6001\u9650\u5236\u5728\u84dd\u5149\u8367\u5149\u5c42\uff0c\u800c\u5229\u7528\u4e09\u7ebf\u6001\u6fc0\u5b50\u8fc1\u79fb\u8ddd\u79bb\u957f\u7684\u7279\u70b9\u6765\u6700\u7ec8\u5728\u90bb\u8fd1\u5c42\u8f6c\u6362\u4e3a\u9ad8\u6548\u654f\u5316\u9ec4\u8272\u8367\u5149\uff0c\u4e5f\u5c31\u662f\u8bf4\u901a\u8fc7\u5408\u7406\u5730\u5206\u914d\u5355\u7ebf\u6001\u548c\u4e09\u7ebf\u6001\u6fc0\u5b50\u5230\u76f8\u5e94\u7684\u590d\u5408\u901a\u9053\u4e2d\u3002\u6700\u7ec8\uff0c\u5355\u7ebf\u6001\u6fc0\u5b50\u88ab\u84dd\u8272\u8367\u5149\u56e2\u6355\u83b7\uff0c\u6269\u6563\u7684\u4e09\u7ebf\u6001\u6fc0\u5b50\u88ab\u7eff\u5149\u70ed\u6fc0\u6d3b\u5ef6\u8fdf\u8367\u5149\u6750\u6599\u6355\u83b7\u5e76\u5b9e\u73b0\u4e0a\u8f6c\u6362\u8fc7\u7a0b\uff0c\u6700\u7ec8\u4ece\u9ec4\u8272\u8367\u5149\u6750\u6599\u53d1\u5c04\u3002\u4e3a\u6b64\uff0c\u7533\u8bf7\u4eba\u8fd8\u8bbe\u8ba1\u4e86\u4e00\u4e2a\u5168\u65b0\u7684\u87ba\u73af\u4e3b\u4f53\u6750\u6599SF4-TPE\u3002\u8be5\u6750\u6599\u7684\u5355\u7ebf\u6001\u80fd\u7ea7\uff083.28 eV\uff09\u548c\u4e09\u7ebf\u6001\u80fd\u7ea7\uff082.71 eV\uff09\u5206\u522b\u5339\u914d\u84dd\u8272\u8367\u5149\u5ba2\u4f53\u4e0eTADF\u654f\u5316\u5206\u5b50\uff0c\u540e\u8005\u53ef\u8fdb\u4e00\u6b65\u6fc0\u6d3b\u9ec4\u8272\u8367\u5149\u5206\u5b50\u3002SF4-TPE\u529f\u80fd\u5c42\u7684\u539a\u5ea6\u53ef\u8c03\u8282\u6fc0\u5b50\u751f\u6210\u548c\u590d\u5408\u754c\u9762\uff0c\u4ece\u800c\u5b9e\u73b0\u5355\u7ebf\u6001\u548c\u4e09\u7ebf\u6001\u6fc0\u5b50\u7684\u6709\u6548\u5206\u79bb\u3001\u4f20\u9012\u4e0e\u5171\u632f\u3002\u5728\u6b64\u5168\u65b0\u673a\u5236\u4e0b\uff0c\u57fa\u4e8e\u8367\u5149\u5206\u5b50\u53d1\u5149\u7684\u767d\u5149\u5668\u4ef6\u7684\u6548\u7387\u8fbe\u523024.5%\u4e0e65.4\u6d41\u660e\u6bcf\u74e6\uff0c\u5e76\u540c\u65f6\u5b9e\u73b0\u4e86\u7a33\u5b9a\u7684\u5149\u8272\u4e0e\u5e73\u7a33\u7684\u6548\u7387\u6eda\u964d\u3002\u8be5\u8bba\u6587\u7684\u7b2c\u4e00\u4f5c\u8005\u662f\u82cf\u5dde\u5927\u5b66\u7855\u58eb\u751f\u6c64\u6d35\uff0c\u73b0\u4e3a\u65e5\u672c\u4e5d\u5dde\u5927\u5b66\u535a\u58eb\u751f\uff0c\u901a\u8baf\u4f5c\u8005\u4e3a\u848b\u4f50\u6743\u6559\u6388\u3002<\/p>\n

\u6700\u8fd1\uff0c\u8be5\u8bfe\u9898\u7ec4\u9488\u5bf9\u6709\u673a\u767d\u5149\u4e2d\u7684\u6750\u6599\u4e0e\u5668\u4ef6\u7684\u7ed3\u5408\u63d0\u51fa\u4e86\u4e00\u4e9b\u65b0\u7684\u7b56\u7565\uff0c\u6bd4\u5982\u63d0\u51fa\u6fc0\u5b50\u590d\u5408\u7269\u4e3b\u4f53\u4e2d\u53ef\u91c7\u7528\u68af\u5ea6\u5171\u6df7\u7684\u7b56\u7565\uff0c\u800c\u4e0d\u662f\u4f20\u7edf\u56fa\u5b9a\u76841\uff1a1\u6bd4\u4f8b\uff0c\u5e76\u4ee5\u6b64\u5b9e\u73b0\u4e861000\u5c3c\u7279\u4eae\u5ea6\u4e0b\u8d85\u8fc770\u6d41\u660e\u6bcf\u74e6\u7684\u9ad8\u6548\u767d\u8272\u78f7\u5149\u5668\u4ef6\uff08ACS Appl. Mater. Interfaces 2018, 10, 29840\uff09\uff0c\u4e0e\u663e\u8272\u6307\u6570\u8d85\u8fc780\u7684\u9ad8\u6548\u9ad8\u8d28\u91cf\u767d\u5149\uff08Adv. Funct. Mater. 2019, 29, 1807541\uff09\u3002\u6b64\u5916\uff0c\u848b\u4f50\u6743\u6559\u6388\u8fd8\u53d1\u5c55\u4e86\u975e\u5e38\u89c4\u7684\u7eaf\u78b3\u6c22\u7ec4\u5206\u7684\u4e3b\u4f53\u6750\u6599\uff08Adv. Mater. 2015, 27, 4213\uff1bAngew. Chem. Int. Ed. 2019, 58, 3848\uff09\uff0c\u672c\u6587\u4e2d\u62a5\u9053\u7684SF4-TPE\u4e5f\u662f\u6b64\u7c7b\u7eaf\u78b3\u6c22\u6750\u6599\u7684\u65b0\u5e94\u7528\u3002<\/p>\n

\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u56fe1 <\/strong>\u5206\u5b50\u7ed3\u6784\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

a) \u7eaf\u78b3\u6c22\u4e3b\u4f53\u6750\u6599 SF4-TPE\uff1b<\/p>\n

b) TADF\u654f\u5316\u6750\u6599PXZ-TRZ\uff1b<\/p>\n

c) \u9ec4\u5149\u8367\u5149\u53d1\u5149\u6750\u6599TBRb\uff1b<\/p>\n

d) \u84dd\u5149\u8367\u5149\u53d1\u5149\u6750\u65994P-NPD\uff1b<\/p>\n

e-f) SF4-TPE\u7684HOMO\u53caLUMO\u8f68\u9053\u5206\u5e03\u56fe\u3002<\/p>\n

\u56fe2<\/strong><\/p>\n

\"\"<\/p>\n

a) SF4-TPE\u3001PXZ-TRZ\u548cTBRb\u7684\u5438\u6536\u5149\u8c31\u3001\u8367\u5149\u548c\u78f7\u5149\u5149\u8c31\uff1b<\/p>\n

b) SF4-TPE\u7684\u77ac\u6001\u8367\u5149\u5149\u8c31:SF4-TPE: TBRb\u63ba\u6742\u8584\u819c, SF4-TPE: PXZ-TRZ: TBRb\u63ba\u6742\u8584\u819c\uff1b<\/p>\n

c) PXZ-TRZ\u654f\u5316\u9ec4\u8272\u8367\u5149\u6750\u6599TBRb\u7684\u5668\u4ef6\u7ed3\u6784\u548c\u76f8\u5e94\u6750\u6599\u7684\u80fd\u7ea7\u56fe\u3002<\/p>\n

\u56fe3<\/strong>\u4f20\u7edf\u8367\u5149\u548cPXZ-TRZ<\/strong>\u654f\u5316\u9ec4\u8272\u8367\u5149OLED<\/strong>\u7684\u5668\u4ef6\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

a)\u7535\u6d41\u5bc6\u5ea6-\u7535\u538b-\u4eae\u5ea6(J-V-L)\u66f2\u7ebf\uff1b<\/p>\n

b)\u5916\u90e8\u91cf\u5b50\u6548\u7387(EQE)-\u4eae\u5ea6\u66f2\u7ebf\uff1b<\/p>\n

c)\u529f\u7387\u6548\u7387-\u4eae\u5ea6\u66f2\u7ebf\uff1b<\/p>\n

d)\u9ec4\u8272\u8367\u5149OLED\u7684\u7535\u81f4\u53d1\u5149\u5149\u8c31\uff0c\u63d2\u56fe\u662fY4\u7684\u9ec4\u8272\u53d1\u5149\u56fe\u3002<\/p>\n

\u56fe4<\/strong><\/p>\n

\u00a0\u00a0\u00a0\u00a0\"\"<\/p>\n

a\uff09\u5168\u8367\u5149WOLEDs\u7684\u5668\u4ef6\u7ed3\u6784\u548c\u80fd\u7ea7\u56fe\uff1b<\/p>\n

b\uff09\u53d1\u5149\u5c42\u4e2d\u7684\u5355\u7ebf\u6001\u548c\u4e09\u7ebf\u6001\u6fc0\u5b50\u8f6c\u79fb\u8fc7\u7a0b\u548c\u673a\u7406\uff1b<\/p>\n

c\uff09SF4-TPE\u30014P-NPD\u7684\u5438\u6536\u3001\u8367\u5149\u548c\u78f7\u5149\u5149\u8c31\uff1b<\/p>\n

d\uff094P-NPD\u3001PXZ-TRZ\u548cTBRb\u5438\u6536\u3001\u8367\u5149\u548c\u78f7\u5149\u5149\u8c31\u3002<\/p>\n

\u56fe5 WOLEDs<\/strong>\u7684\u5668\u4ef6\u6027\u80fd<\/strong><\/p>\n

\u00a0\"\"<\/strong><\/p>\n

a\uff09\u7535\u6d41\u5bc6\u5ea6-\u7535\u538b-\u4eae\u5ea6\uff08J\u2013V\u2013L\uff09\u66f2\u7ebf\uff1b<\/p>\n

b\uff09\u5916\u91cf\u5b50\u6548\u7387\uff08EQE\uff09-\u4eae\u5ea6\u66f2\u7ebf\uff1b<\/p>\n

c\uff09\u529f\u7387\u6548\u7387-\u4eae\u5ea6\u66f2\u7ebf\uff1b<\/p>\n

d\uff09\u5168\u8367\u5149\u7684\u7535\u81f4\u53d1\u5149\u5149\u8c31,\u63d2\u56fe\u662fW4\u7684\u767d\u8272\u53d1\u5149\u56fe\u3002<\/p>\n

\u56fe6<\/strong>\u4e0d\u540c\u4eae\u5ea6\u4e0b\u7684EL<\/strong>\u5149\u8c31<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe7 WOLED<\/strong>\u7684EL<\/strong>\u5149\u8c31\u53d8\u5316<\/strong><\/p>\n

\"\"<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a<\/strong>All-Fluorescence White Organic Light-Emitting Diodes Exceeding 20% EQEs by Rational Manipulation of Singlet and Triplet Excitons<\/a>, 2020, Adv. Funct. Mater., doi: 10.1002\/adfm.201910633.<\/p>\n","protected":false},"excerpt":{"rendered":"

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