{"id":199014,"date":"2020-04-07T06:54:33","date_gmt":"2020-04-06T22:54:33","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=199014"},"modified":"2020-04-06T19:55:09","modified_gmt":"2020-04-06T11:55:09","slug":"%e5%90%89%e6%9e%97%e5%a4%a7%e5%ad%a6%e6%9d%a8%e6%9f%8fadv-mater-%ef%bc%9a%e5%85%b7%e6%9c%89%e8%b6%85%e7%aa%84%e5%8d%8a%e5%b3%b0%e5%ae%bd%e7%9a%84%e6%b7%b1%e7%ba%a2%e7%a2%b3%e5%8c%96%e8%81%9a%e5%90%88","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=199014","title":{"rendered":"\u5409\u6797\u5927\u5b66\u6768\u67cfAdv. Mater.\uff1a\u5177\u6709\u8d85\u7a84\u534a\u5cf0\u5bbd\u7684\u6df1\u7ea2\u78b3\u5316\u805a\u5408\u7269\u70b9"},"content":{"rendered":"

\u3010\u7814\u7a76\u80cc\u666f\u3011<\/strong><\/p>\n

\u78b3\u70b9\u51ed\u501f\u5176\u4e30\u5bcc\u4e14\u4f4e\u5ec9\u7684\u78b3\u6e90\uff0c\u826f\u597d\u7684\u751f\u7269\u76f8\u5bb9\u6027\uff0c\u8f83\u9ad8\u7684\u8367\u5149\u91cf\u5b50\u6548\u7387\u53ca\u8f83\u4f4e\u7684\u751f\u7269\u6bd2\u6027\u7b49\u4f18\u52bf\u800c\u5907\u53d7\u5173\u6ce8\uff0c\u5728\u8bf8\u591a\u9886\u57df\u6709\u7740\u91cd\u8981\u7684\u5546\u4e1a\u5e94\u7528\u524d\u666f\uff0c\u5c24\u5176\u662f\u5728\u751f\u7269\u6210\u50cf\u65b9\u9762\u3002\u800c\u7a84\u7684\u534a\u5cf0\u5bbd\u53d1\u5c04\u5bf9\u4e8e\u589e\u5f3a\u6210\u50cf\u5bf9\u6bd4\u5ea6\u3001\u51cf\u5c0f\u80cc\u666f\u566a\u58f0\uff0c\u63d0\u9ad8\u663e\u793a\u5668\u4ef6\u7684\u8272\u7eaf\u5ea6\uff0c\u751a\u81f3\u7528\u4f5c\u6fc0\u5149\u53d1\u5c04\u6750\u6599\u7b49\u65b9\u9762\u610f\u4e49\u91cd\u5927\u3002\u6b64\u5916\uff0c\u5236\u5907\u53d1\u5c04\u6ce2\u957f\u5927\u4e8e660 nm \uff08\u6df1\u7ea2\u8272\u8367\u5149\u7a97\u53e3\uff09\u7684\u9ad8\u6027\u80fd\u78b3\u70b9\u4e5f\u6709\u5229\u4e8e\u6df1\u5c42\u7ec4\u7ec7\u6210\u50cf\uff0c\u4f46\u540c\u65f6\u83b7\u5f97\u534a\u5cf0\u5bbd\u7a84\u3001\u91cf\u5b50\u6548\u7387\u9ad8\u3001\u751f\u7269\u76f8\u5bb9\u6027\u597d\u7684\u6df1\u7ea2\u5149\/\u8fd1\u7ea2\u5916\u5149\u78b3\u70b9\u4ecd\u662f\u4e00\u4e2a\u91cd\u5927\u6311\u6218\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5409\u6797\u5927\u5b66\u8d85\u5206\u5b50\u7ed3\u6784\u4e0e\u6750\u6599\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u6768\u67cf\u7814\u7a76\u7ec4<\/strong>\u62a5\u9053\u5408\u6210\u4e86\u4e00\u79cd\u534a\u5cf0\u5bbd\u7ea6\u4e3a20 nm\uff08\u76ee\u524d\u62a5\u9053\u7684\u6700\u5c0f\u503c\uff09\u3001\u53d1\u5c04\u6ce2\u957f\u5728673 nm\u3001\u6bd2\u6027\u4f4e\u3001\u751f\u7269\u76f8\u5bb9\u6027\u597d\u7684\u6df1\u7ea2\u5149\u78b3\u5316\u805a\u5408\u7269\u70b9 \uff08Carbonized Polymer Dots, CPDs\uff09\u3002\u5728\u4e8c\u7532\u57fa\u4e9a\u781c\uff08DMSO\uff09\u6eb6\u6db2\u4e2d\uff0c413 nm\u548c660 nm\u6fc0\u53d1\u5149\u6fc0\u53d1\u4e0b\uff0c\u8be5\u6df1\u7ea2\u5149CPDs\u7684\u91cf\u5b50\u6548\u7387\u5206\u522b\u9ad8\u8fbe59%\u548c31%\uff0c\u662f\u76ee\u524d\u5df2\u62a5\u9053\u7684\u7ea2\u5149\/\u8fd1\u7ea2\u5916\u5149\u78b3\u70b9\u7684\u6700\u9ad8\u91cf\u5b50\u6548\u7387\u3002\u5b9e\u9a8c\u8868\u660e\uff0c\u8367\u5149\u57fa\u5143\u5355\u4e00\uff0c\u80fd\u7ea7\u7ed3\u6784\u7b80\u5355\u4ee5\u53caN\u6742\u73af\u548c\u82b3\u9999\u73af\u6784\u6210\u7684\u5171\u8f6d\u7ed3\u6784\u7684\u5b8c\u6574\u6027\u662f\u6df1\u7ea2\u5149CPDs\u4e3b\u8981\u7684\u8367\u5149\u673a\u7406\u3002\u6b64\u5916\uff0c\u8be5\u5de5\u4f5c\u9996\u6b21\u6df1\u5165\u63a2\u8ba8\u4e86CPDs\u7684\u6838\u58f3\u7ed3\u6784\u53ca\u805a\u5408\u7269\u7279\u6027\uff0c\u5206\u6790\u4e86CPDs\u5728\u4f53\u5185\u7684\u80be\u810f\u53ca\u809d\u80c6\u4ee3\u8c22\u9014\u5f84\uff0c\u5e76\u5c06\u5176\u7528\u4e8e\u5355\u5149\u5b50\u548c\u53cc\u5149\u5b50\u751f\u7269\u6210\u50cf\u3002\u8be5\u6587\u7ae0\u8fd1\u65e5\u4ee5\u9898\u4e3a\u201cDeep Red Emissive Carbonized Polymer Dots with Unprecedented Narrow Full Width at Half Maximum<\/strong>\u201d\u53d1\u8868\u5728\u77e5\u540d\u671f\u520aAdv. Mater.<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u78b3\u5316\u805a\u5408\u7269\u70b9\uff08<\/strong>CPDs<\/strong>\uff09\u7684\u5408\u6210\u53ca\u5149\u5b66\u6027\u8d28<\/strong><\/p>\n

\"\"<\/p>\n

a\uff09\u5236\u5907\u793a\u610f\u56fe\u3002<\/p>\n

b\uff09\u5438\u6536\u5149\u8c31\u3002<\/p>\n

c\uff09\u8367\u5149\uff08PL\uff09\u5149\u8c31\u3002<\/p>\n

d\uff09\u4e0d\u540c\u6fc0\u53d1\u5149\u4e0b\u7684\u5149\u5b66\u7167\u7247\u3002<\/p>\n

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f\uff09CPDs\u7684\u79ef\u5206\u8367\u5149\u5f3a\u5ea6\u4e0e\u6fc0\u5149\u529f\u7387\u5e73\u65b9\u4e4b\u95f4\u7684\u5173\u7cfb\u3002<\/p>\n

\u56fe\u4e8c\u3001<\/strong>CPDs<\/strong>\u7684\u5f62\u8c8c\u53ca\u805a\u5408\u7269\u7279\u6027<\/strong><\/p>\n

\"\"<\/p>\n

a\uff09\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u56fe\u3002<\/p>\n

b\uff09\u539f\u5b50\u529b\u663e\u5fae\u955c\u56fe\u3002<\/p>\n

c\uff09\u70ed\u91cd\u5206\u6790\uff08\u7ea2\u8272\u66f2\u7ebf\uff09\u548c\u5fae\u5206\u70ed\u91cd\u5206\u6790\uff08\u84dd\u8272\u66f2\u7ebf\uff09\u56fe\u3002<\/p>\n

d\uff09\u5dee\u793a\u626b\u63cf\u91cf\u70ed\u5206\u6790\u3002<\/p>\n

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f\uff09\u6e29\u5ea6\u5bf9CPDs\u7c98\u5ea6\u7684\u5f71\u54cd\u3002<\/p>\n

\u56fe\u4e09\u3001<\/strong>CPDs<\/strong>\u7684\u8367\u5149\u673a\u7406<\/strong><\/p>\n

\"\"<\/p>\n

CPDs\u5728670 nm\uff08a\uff09\u548c720 nm\uff08b\uff09\u5904\u7684PL\u8870\u51cf\u66f2\u7ebf\u3002<\/p>\n

c\uff09CPDs\u7684\u77ac\u6001\u5438\u6536\uff08TA\uff09\u5149\u8c31\u76843D\u4f2a\u5f69\u8272\u56fe\u3002<\/p>\n

d\uff09\u4e0d\u540c\u65f6\u95f4\u5ef6\u8fdf\u4e0b\u7684TA\u5149\u8c31\u3002<\/p>\n

e\uff09\u4e0d\u540c\u7279\u5f81\u6ce2\u957f\u7684\u52a8\u529b\u5b66\u8870\u51cf\u66f2\u7ebf\uff0c\u5b9e\u7ebf\u4e3a\u62df\u5408\u66f2\u7ebf\u3002<\/p>\n

f\uff09\u5168\u5c40\u62df\u5408\u7ed3\u679c\u5206\u6790\u3002<\/p>\n

\u56fe\u56db\u3001<\/strong>CPDs<\/strong>\u7684\u8367\u5149\u673a\u7406<\/strong><\/p>\n

\"\"<\/p>\n

a\uff09c-CPDs\u7684\u8367\u5149\u5149\u8c31\u3002<\/p>\n

b\uff09CPDs\uff08\u7ea2\u8272\u66f2\u7ebf\uff09\u548cc-CPDs\uff08\u9ed1\u8272\u66f2\u7ebf\uff09\u7684\u5438\u6536\u5149\u8c31\u3002<\/p>\n

c\uff09CPDs\uff08\u7ea2\u8272\u66f2\u7ebf\uff09\u548cc-CPDs\uff08\u9ed1\u8272\u66f2\u7ebf\uff09\u7684\u5085\u7acb\u53f6\u53d8\u6362\u7ea2\u5916\u5149\u8c31\u3002<\/p>\n

CPDs\u7684\u9ad8\u5206\u8fa8\u7387d\uff09C1s X\u5c04\u7ebf\u5149\u7535\u5b50\u80fd\u8c31\uff08XPS\uff09\uff0ce\uff09N1s XPS\u548cf\uff09O1s\u5149\u8c31\u3002<\/p>\n

c-CPD\u7684\u9ad8\u5206\u8fa8\u7387g\uff09C1s XPS\uff0ch\uff09N1s XPS\u548ci\uff09O1s\u5149\u8c31\u3002<\/p>\n

\u56fe\u4e94\u3001<\/strong>CPDs<\/strong>\u7684\u5355\u5149\u5b50\u548c\u53cc\u5149\u5b50\u751f\u7269\u6210\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

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\u3010\u7ed3\u8bba\u5c55\u671b\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u4ee5\u7ea2\u8c46\u6749\u6811\u53f6\u4e3a\u524d\u9a71\u4f53\uff0c\u901a\u8fc7\u6eb6\u5242\u70ed\u5408\u6210\u65b9\u6cd5\uff0c\u67f1\u5c42\u6790\u63d0\u7eaf\u6280\u672f\u5236\u5907\u4e86\u534a\u5cf0\u5bbd\u7ea6\u4e3a20 nm\u7684\u6df1\u7ea2\u5149CPDs\u3002\u5728413 nm\u548c660 nm\u6fc0\u53d1\u5149\u6fc0\u53d1\u4e0b\uff0cCPDs\u7684\u91cf\u5b50\u6548\u7387\u5206\u522b\u9ad8\u8fbe59%\u548c31%\u3002\u5b9e\u9a8c\u53d1\u73b0\uff0cCPDs\u7684\u7ed3\u6784\u4e0d\u540c\u4e8e\u5df2\u62a5\u9053\u7684\u78b3\u91cf\u5b50\u70b9\u6750\u6599\u3002\u5176\u5177\u6709\u6838\u58f3\u7ed3\u6784\uff0c\u4e3b\u8981\u542b\u6709\u7f9f\u57fa\uff0c\u6c28\u57fa\uff0c\u82b3\u9999\u73af\uff0cN\u6742\u5316\u73af\uff0c\u919a\u952e\u7b49\u5316\u5b66\u952e\u3002CPDs\u6700\u5916\u5c42\u662f\u78b3\u5316\u7a0b\u5ea6\u8f83\u4f4e\u7684\u805a\u5408\u7269\u94fe\uff1b\u800c\u78b3\u6838\u4e3b\u8981\u662f\u7531\u805a\u5408\u7269\u94fe\u7684\u4ea4\u8054\u3001\u78b3\u5316\u5f62\u6210\u7684\u3002\u8fdb\u4e00\u6b65\u7814\u7a76\u8868\u660e\uff0c\u8367\u5149\u57fa\u5143\u5355\u4e00\uff0c\u80fd\u7ea7\u7ed3\u6784\u7b80\u5355\u4ee5\u53caN\u6742\u73af\u548c\u82b3\u9999\u73af\u6784\u6210\u7684\u5171\u8f6d\u7ed3\u6784\u7684\u5b8c\u6574\u6027\u662f\u6df1\u7ea2\u5149CPDs\u4e3b\u8981\u7684\u8367\u5149\u673a\u7406\u3002\u6b64\u5916\uff0cCPDs\u5728\u6df1\u7ea2\u5149\u533a\u57df\u8868\u73b0\u51fa\u8f83\u5f3a\u7684\u5438\u6536\u548c\u53d1\u5c04\uff0c\u5177\u6709\u4f4e\u6bd2\u6027\u548c\u826f\u597d\u7684\u751f\u7269\u76f8\u5bb9\u6027\uff0c\u4e14\u5b98\u80fd\u56e2\u4e30\u5bcc\u6613\u4e8e\u4fee\u9970\uff0c\u5355\u5149\u5b50\u548c\u53cc\u5149\u5b50\u751f\u7269\u6210\u50cf\u6548\u679c\u4f73\u3002\u8be5\u5de5\u4f5c\u4e0d\u4ec5\u4f7f\u7814\u7a76\u8005\u4eec\u4e86\u89e3\u4e86\u78b3\u70b9\u6750\u6599\u7684\u805a\u5408\u7269\u7279\u6027\uff0c\u800c\u4e14\u4e3a\u751f\u7269\u533b\u5b66\u53ca\u5149\u7535\u5668\u4ef6\u9886\u57df\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u7684\u6df1\u7ea2\u5149\u7eb3\u7c73\u6750\u6599\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aDeep Red Emissive Carbonized Polymer Dots with Unprecedented Narrow Full Width at Half Maximum <\/a>(Adv. Mater.<\/em>, 2020<\/strong>, DOI: 10.1002\/adma.201906641)<\/p>\n

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