{"id":201085,"date":"2020-05-05T06:27:03","date_gmt":"2020-05-04T22:27:03","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=201085"},"modified":"2020-05-04T22:27:16","modified_gmt":"2020-05-04T14:27:16","slug":"nano-energy%ef%bc%9a%e6%8b%93%e6%89%91%e8%ae%be%e8%ae%a1%e8%b6%85%e5%bc%bamxene%e5%9f%ba%e9%87%91%e5%b1%9e%e9%94%82%e8%b4%9f%e6%9e%81%e5%8f%8a%e5%85%b6%e7%94%a8%e4%ba%8e%e8%b6%85%e8%96%84%e3%80%81","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=201085","title":{"rendered":"Nano Energy\uff1a\u62d3\u6251\u8bbe\u8ba1\u8d85\u5f3aMXene\u57fa\u91d1\u5c5e\u9502\u8d1f\u6781\u53ca\u5176\u7528\u4e8e\u8d85\u8584\u3001\u5168\u67d4\u6027\u7684\u9502\u91d1\u5c5e\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u5177\u6709\u826f\u597d\u67d4\u6027\u3001\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u548c\u9ad8\u5b89\u5168\u6027\/\u53ef\u9760\u6027\u7684\u7535\u5316\u5b66\u50a8\u80fd\u7cfb\u7edf\uff0c\u662f\u5f00\u53d1\u53ef\u7a7f\u6234\u7535\u5b50\u8bbe\u5907\u3001\u667a\u80fd\u670d\u88c5\u548c\u5065\u5eb7\u76d1\u6d4b\u5668\u7684\u5173\u952e\u3002\u91d1\u5c5e\u9502\u8d1f\u6781\u56e0\u5176\u5177\u6709\u9ad8\u6bd4\u5bb9\u91cf\uff083860 mAh g-1<\/sup>\uff09\u548c\u4f4e\u7684\u8fd8\u539f\u7535\u4f4d\uff0c\u53ef\u4ee5\u5b9e\u73b0\u91d1\u5c5e\u9502\u7535\u6c60\uff08LMB\uff09\u9ad8\u7684\u80fd\u91cf\u5bc6\u5ea6\u3002\u6700\u8fd1\uff0c\u65b0\u578b\u7684\u4e8c\u7ef4\u8fc7\u6e21\u91d1\u5c5e\u78b3\u5316\u7269\u548c\u78b3\u6c2e\u5316\u7269\uff08Mn+1<\/sub>Xn<\/sub>Tx<\/sub>\uff1aM\u4e3a\u8fc7\u6e21\u91d1\u5c5e\uff1bX\u4e3aC\u6216N\uff1bn = 1\u30012\u62163\uff1bT\u4e3aO\u3001OH\u6216F\u7684\u672b\u7aef\u57fa\u56e2\uff1b\u8868\u793a\u4e3aMXenes\uff09\uff0c\u7531\u4e8e\u5176\u72ec\u7279\u7684\u8868\u9762\u7279\u6027\uff0c\u5728\u9ad8\u80fdLMB\u4e2d\u663e\u793a\u51fa\u6781\u5927\u7684\u5e94\u7528\u524d\u666f\u3002\u5176\u4e2d\uff0cTi3<\/sub>C2<\/sub>Tx<\/sub> MXenes\u6750\u6599\u7531\u4e8e\u5176\u4f18\u5f02\u7684\u5bfc\u7535\u6027\u3001\u5feb\u901f\u7684\u79bb\u5b50\u4f20\u8f93\u548c\u6613\u4e8e\u5408\u6210\u3001\u9ad8\u7684\u673a\u68b0\u67d4\u97e7\u6027\u3001\u8f83\u597d\u7684\u786b\u6c34\u6027\u548c\u4eb2\u9502\u6027\u7b49\u4f18\u70b9\uff0c\u88ab\u5f00\u53d1\u4e3a\u67d4\u6027\u50a8\u80fd\u5668\u4ef6\u4e2d\u7684\u91d1\u5c5e\u8d1f\u6781\u8f7d\u4f53\u3002\u53e6\u5916\uff0cMXene\u8868\u9762\u4e0a\u5bcc\u542b\u7684\u6781\u6027\u5b98\u80fd\u56e2\u53ef\u4ee5\u5e2e\u52a9\u7a33\u5b9aLi\/\u7535\u89e3\u8d28\u754c\u9762\uff0c\u5f15\u5bfc\u91d1\u5c5eLi\u7684\u5747\u5300\u6210\u6838\u548c\u751f\u957f\u3002\u5176\u4e2d\uff0c\u901a\u8fc7\u771f\u7a7a\u8f85\u52a9\u62bd\u6ee4\u5236\u5907\u7684MXene\u8584\u819c\u56e0\u5176\u5176\u8d28\u8f7b\u3001\u7535\u5bfc\u7387\u9ad8\u3001\u53ef\u673a\u68b0\u6027\u80fd\u597d\uff0c\u53ef\u4ee5\u4f5c\u4e3a\u91d1\u5c5e\u9502\u7684\u7406\u60f3\u8f7d\u4f53\u3002\u4f46\u662f\uff0cMXene\u7247\u5c42\u4e4b\u95f4\u4f5c\u7528\u529b\u8f83\u5f31\uff0c\u7247\u5c42\u4e4b\u95f4\u5bb9\u6613\u53d1\u751f\u6ed1\u79fb\uff0c\u8868\u73b0\u51fa\u76f8\u5bf9\u8f83\u4f4e\u7684\u62c9\u4f38\u5f3a\u5ea6\uff1b\u800c\u4e14\uff0c\u8fd9\u79cd\u5c42\u5c42\u53e0\u53e0\u7684\u7ed3\u6784\u4f1a\u9650\u5236\u9502\u7684\u5b58\u50a8\u548c\u5bfc\u81f4\u5782\u76f4\u65b9\u5411\u4e0a\u8f83\u4f4e\u7684\u79bb\u5b50\u6269\u6563\u901f\u7387\uff0c\u8fdb\u800c\u5bfc\u81f4\u8f83\u4f4e\u7684\u9502\u9762\u5bb9\u91cf\u548c\u5dee\u7684\u9ad8\u500d\u7387\u6027\u80fd\u3002\u672c\u6587\u63d0\u51fa\u4e86\u91c7\u7528\u65cb\u84b8\u6280\u672f\uff0c\u8bf1\u5bfc\u7ea4\u7ef4\u7d20\u7eb3\u7c73\u7ea4\u7ef4\uff08CNF\uff09\u548cTi3<\/sub>C2<\/sub>Tx<\/sub> MXene\u81ea\u7ec4\u88c5\uff0c\u5236\u5907\u5177\u6709\u4e92\u9501\u62d3\u6251\u7ed3\u6784\u3001\u81ea\u652f\u6491\u3001\u8d85\u8f7b\u3001\u8d85\u8584\u548c\u8d85\u67d4\u6027MXene\u819c\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u534e\u4e2d\u519c\u4e1a\u5927\u5b66\u53f6\u6b22\u526f\u6559\u6388<\/strong>\u3001\u66f9\u83f2\u83f2\u6559\u6388<\/strong>\uff0c\u6fb3\u5927\u5229\u4e9a\u4f0d\u4f26\u8d21\u5927\u5b66\u90ed\u518d\u840d\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u4eba\u62a5\u9053\u4e86\u4e00\u79cd\u4e92\u9501\u7684\u62d3\u6251\u7ed3\u6784\u8bbe\u8ba1\uff0c\u501f\u52a9\u65cb\u84b8\u6280\u672f\uff0c\u5f15\u5165\u7684\u5fae\u91cf\u7eb3\u7c73\u7ea4\u7ef4\u7d20\uff08CNF\uff09\u53ef\u4ee5\u548c\u90e8\u5206MXene\u7eb3\u7c73\u7247\u81ea\u7ec4\u88c5\u6210\u7eb3\u7c73\u5fae\u7403\u3002\u8be5\u7eb3\u7c73\u5fae\u7403\u8fdb\u4e00\u6b65\u4e0e\u5bcc\u4f59\u7684MXene\u7247\u76f8\u4e92\u4ea4\u53e0\u5f62\u6210\u4e92\u9501\u7684\u62d3\u6251\u7ed3\u6784\u3002\u8fd9\u79cd\u4e92\u9501\u62d3\u6251\u5fae\u89c2\u7ed3\u6784\uff0c\u6781\u5927\u5730\u63d0\u9ad8\u4e86MXene@CNF\u8584\u819c\u7684\u673a\u68b0\u5f3a\u5ea6\u548c\u67d4\u97e7\u6027\u3002\u66f4\u4e3a\u91cd\u8981\u7684\u662f\uff0cMXene\u5177\u6709\u4e30\u5bcc\u7684Li\u6210\u6838\u4f4d\u70b9\uff0c\u8868\u73b0\u51fa\u5f3a\u7684\u4eb2Li\u7279\u6027\u3002\u4f5c\u8005\u5b9e\u73b0\u4e86\u67d4\u6027\u3001\u8d85\u8584\uff08\u7ea625 \u03bcm\uff09\uff0c\u81ea\u652f\u6491\u7684MXene@CNF\/Li\u590d\u5408\u8d1f\u6781\uff0c\u8be5\u590d\u5408\u8d1f\u6781\u8868\u73b0\u51fa\u65e0\u679d\u6676\u751f\u957f\u884c\u4e3a\uff0c\u7ec4\u88c5\u7684\u5bf9\u79f0\u7535\u6c60\u57280.5 mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0c\u80fd\u7a33\u5b9a\u5faa\u73af\u8d85\u8fc71300\u5c0f\u65f6\u3002\u6240\u5236\u5907\u7684\u590d\u5408\u9502\u8d1f\u6781\u4e0e\u67d4\u6027\u7684\u81ea\u652f\u6491LiFePO4<\/sub>\/\u7ea4\u7ef4\u7d20\u7eb3\u7c73\u7ea4\u7ef4\uff08LFP@CNF\uff09\u6b63\u6781\u76f8\u5339\u914d\uff0c\u53ef\u6784\u5efa\u5177\u6709\u9ad8\u6bd4\u5bb9\u91cf\u548c\u9ad8\u7a33\u5b9a\u6027\u7684\u67d4\u6027LMB\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<\/strong>Topological design of ultrastrong MXene paper hosted Li enables ultrathin and fully flexible lithium metal batteries<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nano Energy<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong> 1 MXene@CNF<\/strong>\u819c\u4e0a\u9540\u9502\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong> 2 Ti3<\/sub>C2<\/sub>Tx<\/sub> MXene<\/strong>\u819c\u7684\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09Ti3<\/sub>C2<\/sub>Tx<\/sub> MXene\u6837\u54c1\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09Ti3<\/sub>C2<\/sub>Tx<\/sub> MXene\u7684HRTEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09MXene\u57fa\u9762\u7684HRTEM\u56fe\u50cf\uff1b<\/p>\n

\uff08d\uff09\u6298\u53e0MXene@CNF\u819c\u7684\u5149\u5b66\u56fe\u50cf\uff1b<\/p>\n

\uff08e\uff0cf\uff09MXene@CNF\u819c\u7684\u622a\u9762SEM\u56fe\u50cfe)\u548c\u653e\u5927\u7684SEM\u56fe\u50cff)\uff1b<\/p>\n

\uff08g\uff09MXene@CNF\u819c\u7684\u5e73\u9762SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08h\uff09MXene@CNF\u590d\u5408\u5fae\u7403\u7684TEM\u56fe\u50cf\u53ca\u5176Na i\uff09\uff0cC j\uff09\uff0cF k\uff09\u548cTi l\uff09\u7684EDX\u5143\u7d20\u56fe\u3002<\/p>\n

\u56fe<\/strong> 3 MXene<\/strong>\u5fae\u7403\u7684\u5f62\u6210\u673a\u7406\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong> 4 <\/strong>\u5728<\/strong>MXene<\/strong>\u819c\u4e0a\u7684<\/strong>Li<\/strong>\u6c89\u79ef\u6d4b\u8bd5<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09Ti3<\/sub>C2<\/sub>\u548cTi3<\/sub>C2<\/sub>F2<\/sub>\u4e0eLi\u539f\u5b50\u4e4b\u95f4\u7684\u7ed3\u5408\u80fd\uff1b<\/p>\n

\uff08b-d\uff0cf-h\uff09\u57280.5 mA cm-2<\/sup>\u4e0b\uff0c\u5728MXene@CNF\u819c\u4e0a\u6c89\u79ef\u91d1\u5c5eLi\u9762\u5bb9\u91cf\u5206\u522b\u4e3a0.5\uff0c1\uff0c2 mAh cm-2<\/sup>\u7684\u8868\u9762b-d\uff09\u548c\u622a\u9762f-h\uff09SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08e\uff0ci\uff09\u57280.5 mA cm-2<\/sup>\u4e0b\uff0c\u5265\u79bb\u9762\u5bb9\u91cf\u4e3a2 mAh cm-2<\/sup>\u7684MXene@CNF\u819c\u7684\u8868\u9762\u548c\u6a2a\u622aSEM\u56fe\u50cf\uff1b<\/p>\n

\uff08j-l\uff09MXene@CNF\/Li\u8d1f\u6781(2 mAh cm-2<\/sup>)\uff0cToF-SIMS\u63a2\u6d4b\u7684Li–<\/sup> j\uff09\uff0c O–<\/sup> k\uff09\u548cF–<\/sup> l\uff09\u7684\u5143\u7d20\u5206\u5e03\u56fe\u50cf\u3002<\/p>\n

\u56fe<\/strong> 5 MXene@CNF<\/strong>\u548c<\/strong>Cu<\/strong>\u7b94\u4e0a<\/strong>Li<\/strong>\u7684\u6c89\u79ef<\/strong>\/<\/strong>\u6790\u51fa\u884c\u4e3a<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u57280.5 mA cm-2<\/sup>\u548c2 mA h cm-2<\/sup>\u4e0b\uff0cMXene@CNF\u548cCu\u7b94\u4e0a\u7684Li\u7684\u6052\u7535\u6d41\u5145\u653e\u7535\u7535\u538b\u66f2\u7ebf\uff1b<\/p>\n

\uff08b\uff09MXene@CNF\u548cCu\u7b94\u4e0aLi\u7684\u76f8\u5e94\u6c89\u79ef\/\u6790\u51fa\u6548\u7387\uff1b<\/p>\n

\uff08c\uff09MXene@CNF\/Li\u548cCu\/Li\u5bf9\u79f0\u7535\u6c60\u4e2d\u7684\u6052\u7535\u6d41\u5145\u653e\u7535\u7535\u538b\u7279\u6027\uff1b<\/p>\n

\uff08d\uff0ce\uff09\u56fec\u4e2d\u653e\u5927300-400 h\u548c1000-1100 h\u5904\u7684\u5c40\u90e8\u7535\u538b\u66f2\u7ebf\u3002<\/p>\n

\u56fe<\/strong> 6 MXene@CNF\/Li||LFP<\/strong>\u548c<\/strong>Cu\/Li||LFP<\/strong>\u5168\u7535\u6c60\u7684\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff0cb\uff09\u57280.2 C\u65f6\uff0cMXene@CNF\/Li||LFP\u548cCu\/Li||LFP\u5168\u7535\u6c60\u7684\u5145\u653e\u7535\u7535\u538b\u66f2\u7ebfa\uff09\u548c\u5faa\u73af\u6027\u80fd\u56feb\uff09\uff1b<\/p>\n

\uff08c\uff09\u57280.1-2 C\u4e0b\uff0cMXene@CNF\/Li||LFP\u548cCu\/Li||LFP\u7684\u500d\u7387\u6027\u80fd\uff1b<\/p>\n

\uff08d\uff09\u67d4\u6027MXene@CNF\/Li||LFP@CNF\u5168\u7535\u6c60\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08e\uff0cf\uff09MXene@CNF\/Li||LFP@CNF\u5168\u7535\u6c60\u7684\u5145\u653e\u7535\u7535\u538b\u66f2\u7ebfe\uff09\uff0c\u4ee5\u53ca0.2 C\u4e0b\u7684\u5faa\u73af\u6027\u80fdf\uff09\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u672c\u6587\u62a5\u9053\u4e86\u4e00\u79cd\u57fa\u4e8e\u4e92\u9501\u62d3\u6251\u8bbe\u8ba1\u601d\u60f3\u5236\u5907\u7684\u8d85\u8584\uff08~25 \u03bcm\uff09\u3001\u67d4\u6027\u3001\u81ea\u652f\u6491Ti3<\/sub>C2<\/sub>Tx<\/sub> MXene@CNF\u8584\u819c\u3002MXene\u7247\u5c42\u4e0eMXene@CNF\u5fae\u7403\u95f4\u4e92\u9501\u7684\u5fae\u89c2\u7ed3\u6784\uff0c\u6709\u52a9\u4e8e\u964d\u4f4e\u7247\u5c42\u7684\u5c42\u6ed1\u52a8\uff0c\u63d0\u9ad8MXene\u819c\u7684\u673a\u68b0\u5f3a\u5ea6\u548c\u67d4\u97e7\u6027\uff0c\u6269\u5927\u5c42\u95f4\u8ddd\uff0c\u9632\u6b62MXene\u7684\u91cd\u65b0\u5806\u79ef\uff0c\u52a0\u5feb\u4e86\u53cd\u5e94\u52a8\u529b\u5b66\uff0c\u786e\u4fdd\u9502\u8d1f\u6781\u8f83\u9ad8\u7684\u9762\u5bb9\u91cf\u548c\u4f18\u5f02\u7684\u500d\u7387\u6027\u80fd\u3002MXene\u8868\u9762\u5bcc\u542b\u7684\u4eb2\u9502\u5b98\u80fd\u56e2\u4e0eLi\u8868\u73b0\u51fa\u8f83\u5f3a\u7684\u76f8\u4e92\u4f5c\u7528\uff0c\u53ef\u4ee5\u8bf1\u5bfcLi\u91d1\u5c5e\u7684\u5747\u5300\u6210\u6838\u548c\u65e0\u679d\u6676\u751f\u957f\u3002\u7531\u6b64\u6784\u5efa\u7684Li\u8d1f\u6781\uff0c\u57281 mA cm-2<\/sup>\u4e0b\uff0c\u5faa\u73af250\u5708\uff0c\u663e\u793a\u51fa\u7a33\u5b9a\u7684\u5e93\u4ed1\u6548\u7387\uff0c0.5 mA cm-2<\/sup>\u4e0b\uff0c\u7a33\u5b9a\u5faa\u73af1300 h\u3002\u57fa\u4e8e\u8be5\u67d4\u6027MXene@CNF\/Li\u590d\u5408\u8d1f\u6781\u548c\u67d4\u6027\u81ea\u652f\u6491LFP@CNF\u6b63\u6781\u7ec4\u88c5\u7684\u67d4\u6027\u5168\u7535\u6c60\uff0c\u663e\u793a\u51fa\u826f\u597d\u7684\u957f\u5faa\u73af\u7a33\u5b9a\u6027\uff0c\u5faa\u73af\u7ea6100\u5708\uff0c\u5bb9\u91cf\u4fdd\u6301\u7387\u8fbe95.25%\u3002\u8fd9\u9879\u5de5\u4f5c\u4e0d\u4ec5\u4e3a\u8d85\u8584\u3001\u67d4\u6027\u548c\u81ea\u652f\u6491\u7279\u6027\u7684\u529f\u80fd\u5316MXene\u8584\u819c\u63d0\u4f9b\u4e86\u4e00\u79cd\u7b80\u4fbf\u7684\u3001\u5927\u89c4\u6a21\u7684\u5236\u5907\u65b9\u6cd5\uff0c\u4e5f\u5c06\u5176\u5b9e\u9645\u5e94\u7528\u6269\u5c55\u5230\u4e86\u67d4\u6027\u50a8\u80fd\u5668\u4ef6\u9886\u57df\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>\u201cTopological design of ultrastrong MXene paper hosted Li enables ultrathin and fully flexible lithium metal batteries<\/strong>\u201d<\/a>\uff08Nano Energy, 2020, DOI: 10.1016\/j.nanoen.2020.104817\uff09\u3002<\/p>\n

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