{"id":201647,"date":"2020-05-13T06:08:23","date_gmt":"2020-05-12T22:08:23","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=201647"},"modified":"2020-05-13T00:08:30","modified_gmt":"2020-05-12T16:08:30","slug":"%e5%8d%97%e5%bc%80%e5%a4%a7%e5%ad%a6%e9%ab%98%e5%ad%a6%e5%b9%b3adv-sci-%ef%bc%9a%e5%9f%ba%e4%ba%8e%e9%87%8d%e8%b4%a8%e5%92%8c%e5%85%b7%e6%9c%89%e5%82%ac%e5%8c%96%e6%b4%bb%e6%80%a7%e9%87%91%e5%b1%9e","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=201647","title":{"rendered":"\u5357\u5f00\u5927\u5b66\u9ad8\u5b66\u5e73Adv. Sci.\uff1a\u57fa\u4e8e\u91cd\u8d28\u548c\u5177\u6709\u50ac\u5316\u6d3b\u6027\u91d1\u5c5e\u6c27\u5316\u7269\u57fa\u8d28\u6750\u6599\u6784\u7b51\u9502\u786b\u7535\u6c60\u7528\u9ad8\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\u786b\u6b63\u6781"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u662f\u4e8c\u6b21\u7535\u6c60\u53d1\u5c55\u7684\u9a71\u52a8\u529b\u3002\u9502\u786b\u7535\u6c60\u7684\u7406\u8bba\u8d28\u91cf\u548c\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\u9ad8\u8fbe2600 Wh kg-1<\/sup>\u548c2800 Wh L-1<\/sup>\u3002\u4f46\u76ee\u524d\u9502\u786b\u7535\u6c60\u7684\u5b9e\u9645\u8d28\u91cf\u80fd\u91cf\u548c\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\u5bc6\u5ea6\u4ec5\u8fbe\u5230609 Wh kg-1<\/sup>\u548c581 Wh L-1<\/sup>\uff0c\u8fd9\u4e3b\u8981\u7531\u4e8e\u786b\u57fa\u8d28\u901a\u5e38\u91c7\u7528\u8f7b\u8d28\u7684\u78b3\u7eb3\u7c73\u6750\u6599\uff0c\u5bfc\u81f4\u6b63\u6781\u4e2d\u786b\u4f53\u79ef\u6bd4\u5bb9\u91cf\u8f83\u4f4e\u3002\u76ee\u524d\uff0c\u63d0\u9ad8S\u6b63\u6781\u5bc6\u5ea6\u7684\u65b9\u6cd5\u6709\uff1a\u9ad8\u786b\u8d1f\u8f7d\u91cf\u3001\u81f4\u5bc6\u77f3\u58a8\u70ef\u57fa\u8d28\u3001\u7d27\u51d1\u7684\u7535\u6781\u7ed3\u6784\u6216\u8005\u91c7\u7528Mo6<\/sub>S8<\/sub>\u548cFeS\u4f5c\u4e3a\u6d3b\u6027\u6750\u6599\u3002\u7136\u800c\uff0c\u76ee\u524d\u65b9\u6cd5\u5c1a\u65e0\u6cd5\u517c\u987e\u9502\u786b\u7535\u6c60\u7684\u9ad8\u8d28\u91cf\/\u4f53\u79ef\u6bd4\u5bb9\u91cf\u548c\u9ad8\u5faa\u73af\u7a33\u5b9a\u6027\u7684\u591a\u91cd\u8981\u6c42\u3002\u56e0\u6b64\uff0c\u63a2\u7d22\u4e00\u79cd\u901a\u7528\u7684\u7b56\u7565\u6765\u6784\u5efa\u81f4\u5bc6S\u6b63\u6781\u5bf9\u4e8e\u6ee1\u8db3Li-S\u7684\u5b9e\u9645\u5e94\u7528\u5c06\u975e\u5e38\u91cd\u8981\u3002\u672c\u6587\u63d0\u51fa\u4e86\u4e09\u201c\u9ad8\u201d\u539f\u5219\u6765\u5236\u5907\u81f4\u5bc6\u578bS\u6b63\u6781\uff0c\u4ee5\u5b9e\u73b0\u9ad8\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\uff1a\uff081\uff09\u786b\u57fa\u590d\u5408\u6750\u6599\u4e2d\u8d85\u8fc780 wt\uff05\u7684\u201c\u9ad8\u201d\u786b\u542b\u91cf\uff1b\uff082\uff09\u786b\u6b63\u6781\u4e2d\u8d85\u8fc74 mg cm-2<\/sup> \u7684\u201c\u9ad8\u201d\u786b\u8f7d\u91cf\uff1b\uff083\uff09\u5177\u6709\u826f\u597d\u7535\u50ac\u5316\u6d3b\u6027\u7684\u201c\u9ad8\u201d\u5bc6\u5ea6\u57fa\u8d28\u6750\u6599\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5357\u5f00\u5927\u5b66<\/strong>\u7684\u9ad8\u5b66\u5e73\u7814\u7a76\u5458\uff08\u901a\u8baf\uff09<\/strong>\u4f5c\u8005\u7b49\u4eba\uff0c\u63d0\u51fa\u901a\u8fc7\u4e00\u79cd\u4ee5\u9ad8\u5bc6\u5ea6\u786b\u57fa\u8d28\u6750\u6599\u6765\u5b9e\u73b0\u81f4\u5bc6\u578b\u786b\u6b63\u6781\u7684\u5236\u5907\u3002\u57fa\u4e8e\u8be5\u7b56\u7565\uff0c\u5f15\u5165\u4e86\u7406\u8bba\u5bc6\u5ea6\u9ad8\u8fbe6.5 g cm-3<\/sup>\u7684\u9567\u9536\u9530\u6c27\u5316\u7269\uff08La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\uff09\u4f5c\u4e3a\u786b\u8d1f\u8f7d\u57fa\u8d28\u6750\u6599\u3002\u540c\u65f6\uff0cLa0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u672c\u8eab\u53ef\u4ee5\u4f5c\u4e3a\u5145\u653e\u7535\u8fc7\u7a0b\u4e2d\u52a0\u901f\u591a\u786b\u5316\u9502\u7684\u6269\u6563\u3001\u5438\u9644\u548c\u6c27\u5316\u8fd8\u539f\u52a8\u529b\u5b66\u7684\u6709\u6548\u7535\u50ac\u5316\u5242\u3002\u7814\u7a76\u8868\u660e\uff0c\u8fd9\u79cdS\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u6b63\u6781\u5448\u73b0\u51fa\u9ad8\u7684\u8d28\u91cf\/\u4f53\u79ef\u6bd4\u5bb9\u91cf\u548c\u51fa\u8272\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u3002\u6b64\u5916\uff0c\u57fa\u4e8e\u66f4\u9ad8\u632f\u5b9e\u5bc6\u5ea6\uff081.69 g cm-3<\/sup>\uff09\u7684\u81f4\u5bc6\u5316\u6548\u679c\uff0c\u5b9e\u73b0\u4e862727 Wh L-1<\/sup>\uff09\u6b63\u6781\u7684\u8d85\u9ad8\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\uff0c\u8fd9\u4e0e\u5bcc\u954d\u6c27\u5316\u7269\u5d4c\u5165\u6b63\u6781\u6750\u6599\uff081800-2160 WhL-1<\/sup>\uff09\u76f8\u6bd4\u5177\u6709\u4e00\u5b9a\u7684\u7ade\u4e89\u4f18\u52bf\u3002\u8be5\u7814\u7a76\u4e3a\u6784\u5efa\u5177\u6709\u91cd\u8d28\/\u50ac\u5316\u6d3b\u6027\u7684\u9ad8\u5bb9\u91cf\u786b\u6b63\u6781\u5f00\u8f9f\u4e86\u4e00\u6761\u9014\u5f84\uff0c\u6539\u5584\u4e86\u9502\u786b\u7535\u6c60\u7684\u5b9e\u7528\u6027\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<\/strong>High Volumetric Energy Density Sulfur Cathode with Heavy and Catalytic Metal Oxide Host for Lithium\u2013Sulfur Battery<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Advanced Science<\/strong>\u4e0a\u3002\u7b2c\u4e00\u4f5c\u8005\u4e3a\u5357\u5f00\u5927\u5b66\u535a\u58eb\u751f\u5218\u4e9a\u6d9b<\/strong>\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u00a0<\/strong>1 Li-S<\/strong>\u7535\u6c60\u7684\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\u65b9\u6848<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u4e0d\u540cS\u6b63\u6781\u7684\u9884\u8ba1\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\u4e0e\u786b\u9762\u8f7d\u91cf\u7684\u5173\u7cfb\uff1b<\/p>\n

\uff08b\uff09S\u6b63\u6781\u5bc6\u5ea6\u4e0e\u57fa\u8d28\u5bc6\u5ea6\u7684\u5173\u7cfb\u56fe\u3002<\/p>\n

\u56fe\u00a0<\/strong>2 La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub><\/strong>\u7eb3\u7c73\u7ea4\u7ef4\u548c<\/strong>S\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub><\/strong>\u590d\u5408\u6750\u6599\u7684\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u7eb3\u7c73\u7ea4\u7ef4\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u7eb3\u7c73\u7ea4\u7ef4\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u7eb3\u7c73\u7ea4\u7ef4\u7684HRTEM\u56fe\u50cf\u548c\uff08\u63d2\u56fe\uff09SAED\u56fe\uff1b<\/p>\n

\uff08d\uff09La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u7eb3\u7c73\u7ea4\u7ef4\u7684XRD\u56fe\u8c31\uff1b<\/p>\n

\uff08e\uff09La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u7eb3\u7c73\u7ea4\u7ef4\u7684N2<\/sub>\u5438\u9644\u7b49\u6e29\u7ebf\u548c\u5b54\u5206\u5e03\uff1b<\/p>\n

\uff08f\uff09\u5728Ar\u6c14\u6c1b\u4e2d\uff0cS\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u590d\u5408\u6750\u6599\u7684\u70ed\u91cd\uff08TG\uff09\u66f2\u7ebf\u3002<\/p>\n

\u56fe\u00a0<\/strong>3 S\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub><\/strong>\u6b63\u6781\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff0cb\uff09\u57281.3 \u00b5g cm-2<\/sup>\u7684\u786b\u8d1f\u8f7d\u548c5 \u00b5L mg-1<\/sup>\u7535\u89e3\u6db2\u4e2d\uff0cS\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u548cS\/A-CNT\u6b63\u6781\u7684\u5145\u653e\u7535\u66f2\u7ebf\u548cb\uff09\u5faa\u73af\u66f2\u7ebf\uff1b<\/p>\n

\uff08c\uff09\u5728\u4e0d\u540c\u786b\u542b\u91cf\u4e0b\uff0c\u57287 \u00b5L mg-1<\/sup>\u7535\u89e3\u8d28\u4e2dS\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u6b63\u6781\u7684\u8d28\u91cf\u548c\u9762\u5bb9\u91cf\u7684\u5145\u653e\u7535\u66f2\u7ebf;<\/p>\n

\uff08d\uff09\u57287 \u00b5L mg-1<\/sup>\u7535\u89e3\u8d28\u4e2d\uff0cS\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u6b63\u6781\u7684\u5bb9\u91cf\u5faa\u73af\u66f2\u7ebf\u3002<\/p>\n

\u56fe\u00a0<\/strong>4 <\/strong>S\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub><\/strong>\u548c<\/strong>S\/A-CNT<\/strong>\u6b63\u6781\u7684\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\u8868\u5f81\u53ca\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09S\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u548cS\/A-CNT\u6b63\u6781\u7684\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6<\/p>\n

\uff08a\uff0cb\uff09S\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u6b63\u6781\u8868\u9762\u548cb\uff09\u6a2a\u622a\u9762\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff0cd\uff09\u538b\u5b9eS\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u6b63\u6781\u7684\u8868\u9762\u548cd\uff09\u6a2a\u622a\u9762\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08e\uff0cf\uff09S\/A-CNT\u6b63\u6781\u7684\u8868\u9762\u548cf\uff09\u6a2a\u622a\u9762\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08g\uff0ch\uff09\u538b\u5b9eS\/A-CNT\u6b63\u6781\u7684\u8868\u9762\u548ch\uff09\u6a2a\u622a\u9762\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08i\uff0cj\uff09\u57280.2 MPa\u538b\u5b9e\u524d\u540e\uff0cS\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u548cS\/A-CNT\u6b63\u6781\u7684\u5bc6\u5ea6\u548cJ\uff09\u4f53\u79ef\u80fd\u5bc6\u5ea6\uff1b<\/p>\n

\uff08k\uff09\u57280.2MPa\u52a0\u538b\u540e\uff0cLa0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u6b63\u6781\u7684\u5faa\u73af\u7a33\u5b9a\u6027\uff1b<\/p>\n

\uff08l\uff09\u4e0e\u6587\u732e\u4e2d\u786b\u6b63\u6781\u7684\u5bb9\u91cf\u5bf9\u6bd4\u56fe\u3002<\/p>\n

\u56fe\u00a0<\/strong>5 LiPS<\/strong>\u5728<\/strong>La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub><\/strong>\u4e0a\u7684\u50ac\u5316\u8f6c\u5316\u673a\u7406<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a-c\uff09\u57280.1mVs-1<\/sup>\u4e0b\uff0ca\uff09S\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u548cb\uff09S\/A-CNT\u6b63\u6781\u7684CV\u66f2\u7ebf\u53cac\uff09ip<\/sub>\/v1\/2<\/sup>\u7684\u659c\u7387\uff1b<\/p>\n

\uff08d\uff09LiPS\u5728La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u4e2d\u5149\u5b66\u56fe\u50cf\u4ee5\u53ca\u4e0a\u6e05\u6db2\u7684UV-vis\u5149\u8c31\uff1b<\/p>\n

\uff08e\uff09La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u548cLi2<\/sub>S4<\/sub>\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u7684Mn2p\u7684XPS\u8c31\u56fe\uff1b<\/p>\n

\uff08f\uff09La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u548cLi2<\/sub>S4<\/sub>\/La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u7684O1s\u7684XPS\u8c31\u56fe\uff1b<\/p>\n

\uff08g\uff0ch\uff09La0.8<\/sub>Sr0.2<\/sub>MnO3<\/sub>\u548cA-CNT\u7535\u6781\u7684g\uff09\u8fd8\u539f\u8fc7\u7a0b\u548ch\uff09\u6c27\u5316\u8fc7\u7a0b\u4e2d\u7684Tafel\u659c\u7387\u56fe\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a<\/strong>High Volumetric Energy Density Sulfur Cathode with Heavy and Catalytic Metal Oxide Host for Lithium\u2013Sulfur Battery<\/strong><\/a>\uff08Advanced Science, 2020, DOI: 10.1002\/advs.201903693\uff09.<\/p>\n

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