{"id":201774,"date":"2020-05-16T06:07:41","date_gmt":"2020-05-15T22:07:41","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=201774"},"modified":"2020-05-15T20:07:59","modified_gmt":"2020-05-15T12:07:59","slug":"%e5%9b%bd%e5%ae%b6%e7%ba%b3%e7%b1%b3%e7%a7%91%e5%ad%a6%e4%b8%ad%e5%bf%83-adv-mater-%e6%8a%a5%e9%81%93%ef%bc%9a%e7%94%b5%e5%9c%ba%e8%b0%83%e6%8e%a7%e7%9a%84%e6%89%8b%e6%80%a7%e6%b6%b2%e6%99%b6","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=201774","title":{"rendered":"\u56fd\u5bb6\u7eb3\u7c73\u79d1\u5b66\u4e2d\u5fc3 Adv. Mater. \u62a5\u9053\uff1a\u7535\u573a\u8c03\u63a7\u7684\u624b\u6027\u6db2\u6676\u4e2d\u7684\u80fd\u91cf\u8f6c\u79fb\u7528\u4e8e\u589e\u5f3a\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u8fd1\u5e74\u6765\uff0c\u4e00\u79cd\u57fa\u4e8e\u53cd\u65af\u6258\u514b\u65af\uff08anti-Stokes\uff09\u4f4d\u79fb\u7684\u5706\u504f\u632f\u53d1\u5149\uff08CPL\uff09\u73b0\u8c61\uff0c\u5373\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\uff08UC-CPL\uff09\uff0c\u53d7\u5230\u4e86\u5e7f\u6cdb\u7684\u5173\u6ce8\u3002\u57fa\u4e8e\u4e0d\u540c\u53d1\u5149\u673a\u5236\u7684UC-CPL\u5df2\u7ecf\u88ab\u4e00\u4e00\u62a5\u9053\uff0c\u7136\u800c\u76ee\u524d\u6240\u5f97\u5230\u7684\u53d1\u5149\u4e0d\u5bf9\u79f0\u56e0\u5b50(glum<\/sub>)\u666e\u904d\u8f83\u4f4e\uff0c\u6240\u4ee5\u5bfb\u627e\u4e00\u79cd\u80fd\u591f\u63d0\u5347UC-CPL\u7684\u53d1\u5149\u4e0d\u5bf9\u79f0\u56e0\u5b50\uff0c\u5e76\u517c\u5177\u826f\u597d\u53d1\u5149\u6548\u7387\u7684\u65b9\u6cd5\uff0c\u5df2\u7ecf\u6210\u4e3a\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\u9886\u57df\u6700\u91cd\u8981\u7684\u95ee\u9898\u3002\u5728\u591a\u79cd\u624b\u6027\u6750\u6599\u4e2d\uff0c\u624b\u6027\u5411\u5217\u76f8\u6db2\u6676\uff08N*LC\uff09\u5df2\u7ecf\u88ab\u8bc1\u660e\u80fd\u591f\u5b9e\u73b0\u5177\u6709\u9ad8glum<\/sub>\u503c\u7684CPL\uff0c\u5e76\u4e14\u5728\u624b\u6027\u5149\u5b66\u6210\u50cf\u3001\u5149\u5b66\u5668\u4ef6\u3001\u6e29\u5ea6\u4f20\u611f\u5668\u7b49\u65b9\u9762\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u6027\u80fd\u3002\u4e00\u822c\u6765\u8bf4\uff0c\u5c06\u624b\u6027\u5206\u5b50\u63ba\u5165\u5230\u5411\u5217\u578b\u6db2\u6676\u4e2d\u5c31\u80fd\u591f\u83b7\u5f97N*LC\uff0c\u5e76\u4e14\u901a\u8fc7\u6539\u53d8\u63ba\u6742\u6bd4\u4f8b\u5c31\u80fd\u591f\u7075\u6d3b\u5730\u8c03\u8282N*LC\u7684\u5149\u5b50\u7981\u5e26\u3002\u901a\u8fc7\u4e0e\u53d1\u8272\u56e2\u7684\u53d1\u5149\u76f8\u91cd\u53e0\uff0c\u5149\u5b50\u7981\u5e26\u7ecf\u5e38\u88ab\u7528\u4e8e\u83b7\u5f97\u5177\u6709\u9ad8glum<\/sub>\u503c\u7684CPL\u3002\u7136\u800c\uff0c\u7531\u4e8eN*LC\u5177\u6709\u72ec\u7279\u7684\u5706\u4e8c\u8272\u6027\uff08\u5373\u9009\u62e9\u6027\u5730\u53cd\u5c04\u540c\u624b\u6027\u7684\u5706\u504f\u632f\u5149\uff09\uff0c\u56e0\u6b64\u901a\u8fc7\u8fd9\u79cd\u65b9\u5f0f\u83b7\u5f97\u7684CPL\u7684\u53d1\u5c04\u5f3a\u5ea6\u4f1a\u88ab\u4e25\u91cd\u6291\u5236\u3002\u56e0\u6b64\uff0c\u5bf9\u4e8e\u5177\u6709\u5706\u504f\u632f\u53d1\u5149\u6027\u80fd\u7684N*LC\u6765\u8bf4\uff0c\u5982\u4f55\u540c\u65f6\u517c\u5177\u9ad8glum<\/sub>\u503c\u548c\u9ad8\u53d1\u5149\u6548\u7387\u662f\u975e\u5e38\u5173\u952e\u7684\u95ee\u9898\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u57fa\u4e8e\u6b64\uff0c\u4e2d\u79d1\u9662\u56fd\u5bb6\u7eb3\u7c73\u79d1\u5b66\u4e2d\u5fc3\uff08NCNST\uff09\u7684\u6bb5\u9e4f\u98de\u7814\u7a76\u5458\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u56e2\u961f\u53d1\u73b0\u5c06\u4e0a\u8f6c\u6362\u7eb3\u7c73\u7c92\u5b50\uff08UCNPs\uff09\u548c\u9499\u949b\u77ff\u7eb3\u7c73\u6676\uff08CsPbBr3<\/sub>\uff09\u5206\u6563\u5230N*LC\u4e2d\uff0c\u901a\u8fc7\u7c92\u5b50\u95f4\u53d1\u751f\u7684\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b\uff0c\u80fd\u591f\u5b9e\u73b0glum<\/sub>\u6570\u503c\u9ad8\u8fbe1.1\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\uff08\u56fe\u4e00\uff09\u3002\u5728\u8fd9\u4e2a\u8fc7\u7a0b\u4e2d\uff0cCsPbBr3<\/sub>\u7684\u53d1\u5149\u6070\u597d\u4f4d\u4e8e\u5149\u5b50\u7981\u5e26\u7684\u4e2d\u5fc3\uff0c\u56e0\u6b64\u83b7\u5f97\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u5149\u5177\u6709\u6700\u9ad8\u7684glum<\/sub>\u503c\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0cUCNPs\u7684\u53d1\u5149\u7531\u4e8e\u5904\u5728\u5149\u5b50\u7981\u5e26\u7684\u8fb9\u7f18\u800c\u88ab\u663e\u8457\u589e\u5f3a\uff0c\u5e76\u4e14\u80fd\u591f\u901a\u8fc7\u8f90\u5c04\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b\u8fdb\u4e00\u6b65\u589e\u5f3aCsPbBr3<\/sub>\u7684\u53d1\u5149\u3002\u8fd9\u79cd\u8bbe\u8ba1\u6709\u6548\u5730\u514b\u670d\u4e86\u5149\u5b50\u7981\u5e26\u4e2d\u5fc3\u5bf9\u53d1\u5149\u7684\u6291\u5236\uff0c\u4f7f\u5f97CsPbBr3<\/sub>\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\u5728\u5177\u5907\u9ad8glum<\/sub>\u503c\u7684\u540c\u65f6\u8fd8\u5177\u6709\u8f83\u5f3a\u7684\u53d1\u5149\u5f3a\u5ea6\u3002\u6b64\u5916\uff0cCsPbBr3<\/sub>\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\u548c\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b\u90fd\u80fd\u591f\u901a\u8fc7\u7535\u573a\u548c\u5916\u529b\u8fdb\u884c\u8c03\u63a7\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cElectric-Field-Regulated Energy Transfer in Chiral Liquid Crystals for Enhancing Upconverted Circularly Polarized Luminescence through Steering the Photonic Bandgap\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aAdv. Mater.<\/strong>\u4e0a\uff0c\u7b2c\u4e00\u4f5c\u8005\u4e3a\u56fd\u5bb6\u7eb3\u7c73\u79d1\u5b66\u4e2d\u5fc3\u535a\u58eb\u7814\u7a76\u751f\u6768\u96ea\u5cf0<\/strong>\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001CsPbBr3<\/sub>\u548cUCNPs\u5728\u624b\u6027\u5411\u5217\u76f8\u6db2\u6676\u4e2d\u53d1\u751f\u8f90\u5c04\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"
\n \u56fe\u4e8c\u3001CsPbBr3<\/sub> \u7eb3\u7c73\u6676\u5728N*LC\u4e2d\u7684\u53d1\u5149<\/strong>
\n \"\"\uff08a\uff09\u5149\u5b50\u7981\u5e26\u5bf9CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u53d1\u5149\u5f71\u54cd\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09N*LC\u7684\u53cd\u5c04\u5149\u8c31\u548cCsPbBr3<\/sub>\u7eb3\u7c73\u6676\u7684\u53d1\u5c04\u5149\u8c31\uff1b<\/p>\n

\uff08c\uff09CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u5728N*LC\u4e2d\u7684\u5706\u504f\u632f\u53d1\u5149\u5149\u8c31\uff1b<\/p>\n

\uff08d\uff09N*LC\u4e2d\u7684CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u4f4d\u4e8e\u4e0d\u540c\u7535\u573a\u4e0b\u7684\u5706\u504f\u632f\u53d1\u5149\u5149\u8c31\uff1b<\/p>\n

\uff08e\uff09N*LC\u5728\u4e0d\u540c\u7535\u573a\u4e0b\u7684\u53cd\u5c04\u5149\u8c31\u3002<\/p>\n

\u56fe\u4e09\u3001CsPbBr3<\/sub> \u7eb3\u7c73\u6676\u5728\u6db2\u6676\u4e2d\u7684\u4e0a\u8f6c\u6362\u53d1\u5149\u6027\u80fd<\/strong>
\n \"\"\uff08a\uff09CsPbBr3<\/sub>\/UCNPs\u5728\u6db2\u6676\u4e2d\u7684\u4e0a\u8f6c\u6362\u53d1\u5c04\u5149\u8c31\uff1b<\/p>\n

\uff08b\uff09CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u4e0a\u8f6c\u6362\u53d1\u5149\u7684\u53cc\u5bf9\u6570\u70b9\u56fe\uff1b<\/p>\n

\uff08c\uff09\u6db2\u6676\u4e2d\u7684UCNPs\u5728\u6709\u3001\u65e0CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u6761\u4ef6\u4e0b\u7684\u5f52\u4e00\u5316\u4e0a\u8f6c\u6362\u53d1\u5c04\u5149\u8c31\uff1b<\/p>\n

\uff08d\uff09CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u5728N*LC\u4e2d\u65f6\u95f4\u5206\u8fa8\u7684\u4e0a\u8f6c\u6362\u53d1\u5c04\u5149\u8c31\uff1b<\/p>\n

\uff08e\uff09CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u548cUCNPs\u5728\u4e0d\u540c\u6bd4\u4f8b\u4e0b\u7684\u5bff\u547d\u53d8\u5316\uff1b<\/p>\n

\uff08f\uff09CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u548cUCNPs\u5728\u624b\u6027\u548c\u975e\u624b\u6027\u5411\u5217\u76f8\u6db2\u6676\u4e2d\u7684\u4e0a\u8f6c\u6362\u53d1\u5c04\u5149\u8c31\u3002<\/p>\n

\u56fe\u56db\u3001CsPbBr3<\/sub> \u7eb3\u7c73\u6676\u5728N*LC\u4e2d\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\u6027\u80fd<\/strong>
\n \"\"\uff08a\uff09CsPbBr3<\/sub>\u548cUCNPs\u5728N*LC\u4e2d\u53d1\u751f\u8f90\u5c04\u80fd\u91cf\u8f6c\u79fb\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09CsPbBr3<\/sub>\u548cUCNPs\u5728N*LC\u4e2d\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\u5149\u8c31\uff1b<\/p>\n

\uff08c\uff09CsPbBr3<\/sub>\u5728\u4e0d\u540c\u7535\u573a\u4e0b\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\u5149\u8c31\uff1b<\/p>\n

\uff08d\uff09\u7535\u573a\u548c\u5916\u529b\u8c03\u63a7\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\u5f00\u5173\u3002<\/p>\n

\u56fe\u4e94\u3001\u7535\u573a\u548c\u5916\u529b\u8c03\u63a7\u7684\u8f90\u5c04\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b<\/strong>
\n \"\"\uff08a\uff090 V\u65f6\uff0cCsPbBr3<\/sub>\u7eb3\u7c73\u6676\u548cUCNPs\u5728\u624b\u6027\u6db2\u6676\u4e2d\u53d1\u751f\u80fd\u91cf\u8f6c\u79fb\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff090 V\u65f6\uff0c\u504f\u5149\u663e\u5fae\u955c\u7167\u7247\u53ca\u6837\u54c1\u53d1\u5149\u7167\u7247\uff1b<\/p>\n

\uff08c\uff090 V\u65f6\uff0c\u4e0a\u8f6c\u6362\u53d1\u5149\u5149\u8c31\uff1b<\/p>\n

\uff08d\uff09100 V\u65f6\uff0cCsPbBr3<\/sub>\u7eb3\u7c73\u6676\u548cUCNPs\u5728\u624b\u6027\u5411\u5217\u76f8\u6db2\u6676\u4e2d\u53d1\u751f\u80fd\u91cf\u8f6c\u79fb\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08e\uff09100 V\u65f6\uff0c\u504f\u5149\u663e\u5fae\u955c\u7167\u7247\u53ca\u6837\u54c1\u53d1\u5149\u7167\u7247\uff1b<\/p>\n

\uff08f\uff09100 V\u65f6\uff0c\u4e0a\u8f6c\u6362\u53d1\u5149\u5149\u8c31\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u8be5\u56e2\u961f\u901a\u8fc7\u5c06CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u548cUCNPs\u63ba\u5165\u5230\u624b\u6027\u5411\u5217\u76f8\u6db2\u6676\u4e2d\uff0c\u9996\u6b21\u5b9e\u73b0\u4e86\u57fa\u4e8e\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b\u7684UC-CPL\u3002\u901a\u8fc7\u8c03\u8282\u624b\u6027\u5411\u5217\u76f8\u6db2\u6676\u7684\u5149\u5b50\u7981\u5e26\uff0c\u83b7\u5f97\u4e86\u6700\u5927glum<\/sub>\u503c\u4e3a1.1\u7684CsPbBr3<\/sub>\u7eb3\u7c73\u6676\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\uff1b\u540c\u65f6\uff0c\u901a\u8fc7\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b\u514b\u670d\u4e86\u5149\u5b50\u7981\u5e26\u5bf9\u53d1\u5149\u7684\u6291\u5236\u3002\u6b64\u5916\uff0cCsPbBr3<\/sub>\u7eb3\u7c73\u6676\u7684\u4e0a\u8f6c\u6362\u5706\u504f\u632f\u53d1\u5149\u548c\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b\u88ab\u8bc1\u5b9e\u90fd\u80fd\u591f\u901a\u8fc7\u7535\u573a\u548c\u5916\u529b\u8fdb\u884c\u8c03\u63a7\u3002\u603b\u4e4b\uff0c\u8be5\u5de5\u4f5c\u4e0d\u4ec5\u63d0\u4f9b\u4e86\u4e00\u79cd\u83b7\u5f97UC-CPL\u7684\u65b0\u7b56\u7565\uff0c\u800c\u4e14\u9996\u6b21\u5c55\u793a\u4e86\u901a\u8fc7\u8c03\u8282\u5149\u5b50\u7981\u5e26\u5b9e\u73b0\u5177\u6709\u9ad8glum<\/sub>\u503c\u7684UC-CPL\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aElectric-Field-Regulated Energy Transfer in Chiral Liquid Crystals for Enhancing Upconverted Circularly Polarized Luminescence through Steering the Photonic Bandgap<\/a><\/strong>.\uff08Adv. Mater.<\/em>, 2020<\/strong>, DOI: 10.1002\/adma.202000820\uff09<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

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