{"id":204540,"date":"2020-07-05T06:30:15","date_gmt":"2020-07-04T22:30:15","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=204540"},"modified":"2020-07-04T23:25:02","modified_gmt":"2020-07-04T15:25:02","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e7%89%b9%e6%8b%89%e5%8d%8e%e5%a4%a7%e5%ad%a6%e4%bb%98%e5%a0%83nano-letters-%e8%b6%85%e5%8f%96%e5%90%91%e7%a2%b3%e7%ba%a4%e7%bb%b4%e6%a1%86%e6%9e%b6","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=204540","title":{"rendered":"\u7279\u62c9\u534e\u5927\u5b66\u4ed8\u5803Nano Letters: \u8d85\u53d6\u5411\u78b3\u7ea4\u7ef4\u6846\u67b6\u52a9\u529b\u9ad8\u5bb9\u91cf\u8d85\u539a\u7535\u6781"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u4e3a\u4e86\u6ee1\u8db3\u5bf9\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u3001\u4f4e\u6210\u672c\u7684\u50a8\u80fd\u8bbe\u5907\u65e5\u76ca\u589e\u957f\u7684\u9700\u6c42\uff0c\u901a\u8fc7\u4f18\u5316\u7535\u6781\u7ed3\u6784\u6765\u63d0\u9ad8\u7535\u6781\u7684\u9ad8\u9762\u79ef\u5bb9\u91cf\u548c\u964d\u4f4e\u975e\u6d3b\u6027\u6750\u6599\u6210\u5206\u6bd4\uff08\u5982\u91d1\u5c5e\u96c6\u6d41\u4f53\u3001\u805a\u5408\u7269\u7c98\u7ed3\u5242\u548c\u5bfc\u7535\u57fa\u4f53\uff09\u662f\u4e00\u79cd\u6709\u524d\u9014\u7684\u65b9\u6cd5\u3002\u8be5\u65b9\u6cd5\u53ef\u4ee5\u6700\u5927\u9650\u5ea6\u5730\u5229\u7528\u9ad8\u5bb9\u91cf\u7535\u6781\u6750\u6599\u3002\u5728\u8fd9\u79cd\u60c5\u51b5\u4e0b\uff0c\u4f4e\u66f2\u6298\u548c\u9ad8\u4f20\u5bfc\u7684\u539a\u7535\u6781\u7ed3\u6784\u56e0\u5176\u7b80\u5355\u548c\u666e\u9002\u6027\u7684\u8bbe\u8ba1\u7406\u5ff5\u800c\u53d7\u5230\u8d8a\u6765\u8d8a\u591a\u7684\u5173\u6ce8\uff0c\u5e76\u4e14\u6b63\u5728\u8fc5\u901f\u7684\u5e94\u7528\u5230\u5404\u79cd\u7535\u6c60\u6280\u672f\u4e2d\u3002\u7136\u800c\uff0c\u901a\u8fc7\u589e\u52a0\u6d82\u5c42\u539a\u5ea6\u6765\u5236\u4f5c\u7535\u6781\u7684\u4f20\u7edf\u7684\u5236\u9020\u5de5\u827a\u5f80\u5f80\u5dee\u5f3a\u4eba\u610f\uff0c\u5236\u5907\u7684\u539a\u7535\u6781\u5b58\u5728Li+<\/sup>\u79bb\u5b50\u6216\u7535\u5b50\u4f20\u8f93\u6027\u80fd\u8fdf\u7f13\u548c\u529b\u5b66\u5f3a\u5ea6\u4e0d\u9ad8\u7b49\u95ee\u9898\u3002\u4e3a\u4e86\u89e3\u51b3\u8fd9\u4e9b\u95ee\u9898\uff0c\u6700\u8fd1\uff0c\u56fd\u5185\u5916\u79d1\u7814\u5de5\u4f5c\u8005\u62a5\u9053\u4e86\u4e00\u4e9b\u65b0\u578b\u5236\u9020\u65b9\u6cd5\u8bbe\u8ba1\u7684\u539a\u7535\u6781\u7ed3\u6784\uff0c\u8fd9\u4e9b\u7535\u6781\u7ed3\u6784\u663e\u793a\u51fa\u4e86\u4f4e\u66f2\u6298\u5ea6\uff0c\u9ad8\u9762\u79ef\u5bb9\u91cf\u548c\u826f\u597d\u7684\u500d\u7387\u6027\u80fd\u3002\u5176\u4e2d\u5305\u62ec\u5229\u7528\u78c1\u573a\u548c\u51b7\u51bb\u5e72\u71e5\u65b9\u6cd5\u521b\u9020\u7684\u7531\u4f4e\u66f2\u6298\u5ea6\u901a\u9053\u6784\u6210\u7684\u539a\u7535\u6781\u7ed3\u6784\uff0c\u4ee5\u53ca\u5f15\u5165\u4f4e\u66f2\u6298\u5ea6\u7684\u5bfc\u7535\u78b3\u6750\u6599\u6846\u67b6\u7684\u65b9\u6cd5\uff08\u5982\u78b3\u7eb3\u7c73\u7ba1\u3001\u78b3\u7eb3\u7c73\u7ea4\u7ef4\u3001\u77f3\u58a8\u70ef\u7eb3\u7c73\u7247\u3001\u78b3\u5316\u6728\u3001\u79bb\u5b50\u5bfc\u7535\u56fa\u4f53\u7535\u89e3\u8d28\u7b49\uff09\u521b\u9020\u7684\u5177\u6709\u8fde\u7eedLi+\u79bb\u5b50\u6216\u7535\u5b50\u4f20\u8f93\u8def\u5f84\u7684\u7535\u6781\u7ed3\u6784\u3002\u7136\u800c\uff0c\u8fd9\u4e9b\u65b9\u6cd5\u4e0d\u4ec5\u52a0\u5de5\u6210\u672c\u8f83\u9ad8\uff0c\u800c\u4e14\u4f7f\u7528\u7684\u6750\u6599\u5927\u591a\u4ef7\u683c\u6602\u8d35\uff0c\u4e0d\u80fd\u9002\u7528\u4e8e\u5927\u89c4\u6a21\u7684\u5b9e\u9645\u5e94\u7528\u3002\u6b64\u5916\uff0c\u901a\u8fc7\u78c1\u573a\u548c\u51b7\u51bb\u5e72\u71e5\u6cd5\u5236\u9020\u7684\u7535\u6781\u7ed3\u6784\u7684\u529b\u5b66\u6027\u80fd\u548c\u6839\u636e\u5bfc\u7535\u6846\u67b6\u4f53\u79ef\u548c\u8d28\u91cf\u8ba1\u7b97\u7684\u7535\u6781\u6bd4\u5bb9\u91cf\u4ecd\u4e0d\u6e05\u695a\u3002\u56e0\u6b64\uff0c\u8be5\u56e2\u961f\u8bd5\u56fe\u5f00\u53d1\u4e00\u79cd\u6210\u672c\u4f4e\u3001\u53ef\u6269\u5c55\u5236\u9020\u7684\u3001\u4e0e\u5927\u591a\u6570\u7535\u6781\u6750\u6599\u548c\u7535\u6c60\u5316\u5b66\u6027\u80fd\u6709\u826f\u597d\u7684\u517c\u5bb9\u6027\u7684\u5236\u5907\u65b9\u6cd5\uff0c\u4ece\u800c\u5236\u9020\u51fa\u5177\u6709\u9ad8\u5f3a\u5ea6\u3001\u4f4e\u5f2f\u66f2\u5ea6\u3001\u9ad8\u5bfc\u7535\u6027\u548c\u9ad8\u9762\u79ef\u5bb9\u91cf\u7684\u8d85\u539a\u7535\u6781\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u671f\uff0c\u7279\u62c9\u534e\u5927\u5b66<\/b><\/strong>\u4ed8<\/b><\/strong>\u5803<\/b><\/strong>\u6559\u6388<\/b><\/strong>\u56e2\u961f\u62a5\u544a\u4e86\u4e00\u79cd\u5168\u65b0\u7684\u8d85\u539a\u7535\u6781\u7ed3\u6784\uff08Fiber-aligned thick\u00a0(FAT)\u00a0\u7535\u6781\u7ed3\u6784\uff09\u8bbe\u8ba1\u6982\u5ff5\u3002\u8be5\u7535\u6781\u91c7\u7528\u8d2f\u7a7f\u539a\u5ea6\u65b9\u5411\u7ad6\u76f4\u6392\u5217\u7684IM7\u78b3\u7ea4\u7ef4\u4e3a\u6846\u67b6\u7ed3\u6784\uff0c\u5177\u6709\u7535\u6781\u6750\u6599\u8d1f\u8f7d\u9ad8\u3001\u66f2\u6298\u5ea6\u4f4e\u3001\u7535\u5bfc\u7387\u548c\u5bfc\u70ed\u7387\u9ad8\u3001\u538b\u7f29\u6027\u80fd\u597d\u7b49\u7279\u70b9\u3002FAT\u7535\u6781\u7684\u4f4e\u5f2f\u66f2\u5ea6\u8bbe\u8ba1\u4e0d\u4ec5\u80fd\u591f\u4f7f\u7535\u89e3\u6db2\u5feb\u901f\u6e17\u900f\u7535\u6781\u7ed3\u6784\uff0c\u800c\u4e14\u4e3a\u7535\u6781\u5185\u90e8Li\u79bb\u5b50\u6216\u7535\u5b50\u63d0\u4f9b\u4e86\u5feb\u901f\u4f20\u8f93\u8def\u5f84\u3002<\/p>\n

\u8be5\u5de5\u4f5c\u4ee5\u6807\u9898\u4e3a\u00a0\u201cLow Tortuous, Highly Conductive, and High-Areal-Capacity Battery Electrodes Enabled by Through-thickness Aligned Carbon Fiber Framework<\/b><\/strong>\u201d <\/b><\/strong>\u53d1\u8868\u5728\u56fd\u9645\u77e5\u540d\u671f\u520a\u300aNano Letters<\/i><\/b><\/em><\/strong>\u300b\u4e0a\uff0c\u7b2c\u4e00\u4f5c\u8005\u4e3a\u53f2\u5b9d\u4f1a<\/b><\/strong>\uff08\u4e1c\u534e\u5927\u5b66\u8054\u5408\u57f9\u517b\u535a\u58eb\uff09<\/b><\/strong>\u548c\u5546\u5143\u5143<\/b><\/strong>\uff08\u9752\u5c9b\u79d1\u6280\u5927\u5b66<\/b><\/strong>\u8054\u5408\u57f9\u517b\u535a\u58eb<\/b><\/strong>\uff09<\/b><\/strong>\uff0c\u901a\u8baf\u4f5c\u8005\u4e3a\u4ed8<\/b><\/strong>\u5803<\/b><\/strong>\u6559\u6388<\/b><\/strong>\u3002<\/b><\/strong><\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

FAT<\/strong>\u7535\u6781\u5236\u5907\u8fc7\u7a0b\u662f\uff1a\u5c06\u8d1f\u8f7d<\/strong>LiFePO4<\/sub><\/strong>\uff08<\/strong>LFP<\/strong>\uff09\u7eb3\u7c73\u9897\u7c92\u7684\u9ad8\u5ea6\u53d6\u5411\u7684\u78b3\u7ea4\u7ef4\u819c\u7ed3\u6784\uff08\u539a\u5ea6\u4e3a<\/strong>100um<\/strong>\uff09\u5377\u66f2\u6210\u5706\u7b52\u72b6\uff0c\u5e76\u5207\u5272\u6210\u539a\u5ea6\u4e3a<\/strong>1mm<\/strong>\u7684\u7535\u6781\u7ed3\u6784\u3002\u7531\u4e8e\u78b3\u7ea4\u7ef4\u5728\u7535\u6781\u7ed3\u6784\u4e2d\u7ad6\u76f4\u6392\u5217\uff0c\u56e0\u6b64\uff0c<\/strong>\u5c55\u73b0\u4e86\u9ad8\u7684\u6297\u538b\u5f3a\u5ea6\uff08<\/strong>2.8 MPa<\/strong>\uff09\u548c\u6a21\u91cf\uff08<\/strong>36.8 MPa<\/strong>\uff09\uff0c\u5206\u522b\u6bd4\u4f20\u7edf\u539a\u7535\u6781\u63d0\u9ad8\u4e86<\/strong>3.6<\/strong>\u548c<\/strong>4.6<\/strong>\u500d\u3002<\/strong><\/p>\n

\u56fe1 FAT\u7535\u6781\u7684\u8bbe\u8ba1\u548c\u5236\u5907<\/b><\/strong>\"\"<\/p>\n

\u8bbe\u8ba1\u7684FAT\u539a\u7535\u6781\u7ed3\u6784\u7684LFP\u538b\u5b9e\u5bc6\u5ea6\u4e3a1.26g\/cm3<\/sup>, \u5177\u6709\u9ad8\u7684LFP\u8d1f\u8f7d\u5e76\u4e14\u7535\u6781\u7ed3\u6784\u7d27\u5bc6\u3002FAT\u7535\u6781\u7684\u901a\u8fc7\u539a\u5ea6\u65b9\u5411\uff080.35 ohm\u00a0\u20131\u00a0<\/sup>cm\u00a0\u20131<\/sup>\uff0c1.12\u00b10.19 W\/m\u00b7K\uff09\u8868\u73b0\u51fa\u6bd4\u5e73\u9762\u65b9\u5411\uff080.005\u00a0ohm\u00a0\u20131<\/sup>\u00a0cm\u00a0\u20131<\/sup>\uff0c0.45\u00b10.08 W\/m\u00b7K\uff09\u00a0\u9ad870\u500d\u7684\u7535\u5bfc\u7387\u548c2.5\u500d\u7684\u70ed\u5bfc\u7387\uff0c\u7535\u6781\u7ed3\u6784\u5c55\u73b0\u4e86\u7a81\u51fa\u7684\u7535\u5b66\u548c\u70ed\u5b66\u5404\u5411\u5f02\u6027\u3002\u540c\u65f6\uff0c\u7ad6\u76f4\u6392\u5217\u7684\u78b3\u7ea4\u7ef4\u6846\u67b6\u7ed3\u6784\u4e5f\u4fc3\u8fdb\u4e86\u7535\u89e3\u6db2\u7684\u5feb\u901f\u6e17\u900f\u3002<\/p>\n

\u56fe2 FAT<\/b><\/strong>\u7535\u6781\u7ed3\u6784<\/b><\/strong>\u5fae\u89c2\u5f62\u8c8c<\/b><\/strong>\"\"<\/p>\n

3D\u91cd\u5efaX\u5c04\u7ebf\u03bc-CT\u56fe\u50cf\u548cSEM\u56fe\u50cf\u5c55\u793a\u4e86\u7535\u6781\u7ed3\u6784\u5168\u8c8c\u3002\u78b3\u7ea4\u7ef4\u7ad6\u76f4\u6392\u5217\u8d2f\u7a7f\u7535\u6781\u7ed3\u6784\uff0cLFP\u7eb3\u7c73\u9897\u7c92\u5747\u5300\u5206\u5e03\u4e8e\u7535\u6781\u5185\u90e8\u3002<\/p>\n

\u56fe3 FAT\u7535\u6781\u7684\u70ed\u6027\u80fd\u6d4b\u91cf<\/b><\/strong>\"\"<\/p>\n

FAT\u7535\u6781\u57280.5\u30012\u548c5 mA\/cm2\u65f6\u5206\u522b\u63d0\u4f9b\u4e86155\u3001150\u548c123 mAh\/g\u7684\u9ad8\u6bd4\u5bb9\u91cf\u3002\u76f8\u6bd4\u4e4b\u4e0b\uff0c\u4f20\u7edf\u65b9\u6cd5\u5236\u5907\u7684\u539a\u7535\u6781\u57280.5\u30012\u548c5 mA\/cm2\u65f6\u5177\u6709\u8f83\u4f4e\u7684\u6bd4\u5bb9\u91cf\u5206\u522b\u4e3a102\u300165\u548c25 mAh\/g\u3002<\/p>\n

\u56fe4 FAT\u7535\u6781\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong>\"\"<\/p>\n

\u56fe5 FAT\u7535\u6781\u4e0e\u5176\u4ed6\u62a5\u9053\u7684\u539a\u7535\u6781\u7684\u6bd4\u8f83<\/strong>\"\"<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u8be5\u56e2\u961f\u5f00\u53d1\u4e86\u4e00\u79cd\u65b0\u7684\u8d85\u539aFAT\u7535\u6781\u8bbe\u8ba1\u6982\u5ff5\uff0c\uff0c\u8be5\u65b9\u6cd5\u57fa\u4e8e\u6c34\u6027LFP\u6d46\u6599\u548c\u9ad8\u5ea6\u5bf9\u9f50\u7684\u78b3\u7ea4\u7ef4\u819c\uff0c\u901a\u8fc7\u5377\u66f2\u548c\u5207\u5272\u6765\u751f\u4ea7\u7ea4\u7ef4\u6846\u67b6\u7684\u7535\u6781\u7ed3\u6784\u3002\u8be5\u7535\u6781\u5177\u6709\u4f4e\u5f2f\u66f2\u5ea6\u3001\u9ad8\u7a7f\u900f\u539a\u5ea6\u3001\u9ad8\u6297\u538b\u5f3a\u5ea6\u7b49\u4e00\u7cfb\u5217\u72ec\u7279\u7279\u6027\u3002\u5728\u8be5\u7ed3\u6784\u4e2d\u78b3\u7ea4\u7ef4\u7ad6\u76f4\u6392\u5217\u8d2f\u7a7f\u6574\u4e2a\u7535\u6781\uff0c\u5176\u4e2d\u6d3b\u6027\u6750\u6599\uff08\u5982LFP\u7eb3\u7c73\u9897\u7c92\uff09\u5d4c\u5165\u5728\u76f8\u90bb\u7684\u78b3\u7ea4\u7ef4\u4e4b\u95f4\uff0c\u4ece\u800c\u4ea7\u751f\u4e00\u4e2a\u4f4e\u66f2\u6298\u7684\u5b54\u9699\u7ed3\u6784\u3002\u78b3\u7ea4\u7ef4\u4e4b\u95f4\u7684\u5b54\u9699\u901a\u8fc7\u7535\u6781\u539a\u5ea6\u5f62\u6210\u901a\u9053\uff0c\u5141\u8bb8\u79bb\u5b50\u5728\u6d78\u6e0d\u6db2\u4f53\u7535\u89e3\u8d28\u4e2d\u5feb\u901f\u4f20\u8f93\u3002FAT\u7535\u6781\u5177\u67090.35 ohm-1<\/sup>\u00a0cm-1<\/sup>\u7684\u9ad8\u901a\u5b54\u7535\u5bfc\u7387\uff0c1.12\u00b10.019 W\/m\u00b7K\u7684\u70ed\u5bfc\u7387\u548c2.8 MPa\u7684\u6297\u538b\u5f3a\u5ea6\u3002\u5728\u8fd9\u9879\u5de5\u4f5c\u4e2d\u5f00\u53d1\u7684FAT\u7535\u6781\u7684\u539a\u5ea6\u7ea6\u4e3a1 mm\uff0c\u6709\u6548\u8d1f\u8f7d\u4e3a128 mg\/cm2<\/sup>\uff0c\u57280.5 mA\/cm2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u53ef\u63d0\u4f9b155 mAh\/g\u7684\u9ad8\u5bb9\u91cf\u3002\u4e0e\u5176\u4ed6\u62a5\u9053\u7684\u539a\u7535\u6781\u76f8\u6bd4\uff0cFAT\u7535\u6781\u8fd8\u663e\u793a\u51fa\u826f\u597d\u7684\u500d\u7387\u6027\u80fd\u3002\u8fd9\u79cd\u7535\u6781\u7ed3\u6784\u8bbe\u8ba1\u4e5f\u53ef\u4ee5\u517c\u5bb9\u591a\u79cd\u7535\u6c60\u6750\u6599\u548c\u5316\u5b66\u7269\u8d28\uff08\u5982Li-S\u3001Li-air\uff09\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Low Tortuous, Highly Conductive, and High-Areal-Capacity Battery Electrodes Enabled by Through-thickness Aligned Carbon Fiber Framework<\/a>\uff08Nano Letters\uff0c 2020\uff0cDOI:10.1021\/acs.nanolett.0c02053\uff09<\/p>\n

\u672c\u6587\u7531\u6728\u6587\u97ec\u7ffb\u8bd1\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002
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