{"id":205292,"date":"2020-07-22T06:08:28","date_gmt":"2020-07-21T22:08:28","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=205292"},"modified":"2020-07-22T10:38:42","modified_gmt":"2020-07-22T02:38:42","slug":"%e6%88%b4%e5%ae%8f%e6%9d%b0%e3%80%81%e7%8e%8b%e4%b8%ad%e6%9e%97%e3%80%81%e5%a4%8f%e5%b9%bc%e5%8d%97%e3%80%81%e6%ae%b5%e9%95%b6%e9%94%8b%e3%80%81%e4%b9%94%e4%b8%96%e7%92%8b%e3%80%81%e6%a5%bc%e9%9b%84","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=205292","title":{"rendered":"\u6234\u5b8f\u6770\u3001\u738b\u4e2d\u6797\u3001\u590f\u5e7c\u5357\u3001\u6bb5\u9576\u950b\u3001\u4e54\u4e16\u748b\u3001\u697c\u96c4\u6587\u3001\u80e1\u826f\u5175\u3001\u9648\u5fe0\u4f1f\u3001\u6bb7\u4e9a\u4e1c\u3001\u5f90\u5f3a\u3001\u6c6a\u56fd\u79c0\u7b49\u50ac\u5316\u65b0\u8fdb\u5c55"},"content":{"rendered":"

1<\/strong>\u3001<\/strong>JACS<\/strong>\uff1a\u94dc\u57fa\u50ac\u5316\u5242\u9ad8\u538b\u7535\u8fd8\u539f<\/strong>CO2<\/sub><\/strong>\u9ad8\u6548\u5236\u7532\u9178<\/strong><\/p>\n

\"\"<\/p>\n

\u7f8e\u56fd\u65af\u5766\u798f\u5927\u5b66\u7684\u6234\u5b8f\u6770\u9662\u58eb\u56e2\u961f<\/strong>\u8bbe\u8ba1\u4e86\u4e00\u79cd\u8d85\u7eaf\u94dc\u7b94\u7684\u65b9\u6ce2\u7535\u5316\u5b66\u6c27\u5316\u8fd8\u539f\u5faa\u73af\u5904\u7406\u65b9\u6cd5\uff0c\u5236\u5907\u4e86\u5bcc\u542b\uff08111\uff09\u53d6\u5411Cu2<\/sub>O\u7eb3\u7c73\u7c92\u5b50\u7684\u4e9a\u5fae\u7c73\u539a\u819c\uff0c\u7528\u4e8eCO2<\/sub>RR\uff0c CO2<\/sub>\u538b\u529b\u4e3a1-60 atm\u3002\u572845\u5927\u6c14\u538b\u4ee5\u4e0a\u7684KHCO3<\/sub>\u7535\u89e3\u6db2\u4e2d\uff0c\u6b63\u6781\u4e3aSW-Cu2<\/sub>O\/Cu\u7684CO2<\/sub>RR\u5360\u4e3b\u5bfc\u5730\u4f4d\uff0c\u4e3a\u9009\u62e9\u6027\u7532\u9178\u76d0\u751f\u4ea7\u63d0\u4f9b\u4e8698%\u7684\u6cd5\u62c9\u7b2c\u7535\u6d41\u6548\u7387\u3002SW-Cu2<\/sub>O\/Cu\u5728\u957f\u671f(\u223c20h) CO2<\/sub>RR\u671f\u95f4\u4fdd\u6301\u4e86\u8f83\u9ad8\u7684\u7532\u9178\u76d0\u9009\u62e9\u6027\u3002\u6574\u4e2a\u7535\u89e3\u69fd\u53ef\u4ee5\u9ad8\u6548\u8282\u80fd\u5730\u751f\u4ea7\u51fa\u5927\u91cf\u7684\u7532\u9178\u76d0(\u223c0.4 g\/cm2<\/sup>)\uff0c\u800c\u4e0d\u9700\u8981\u5bf9\u4ea7\u54c1\u8fdb\u884c\u5206\u79bb\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/pubs.acs.org\/doi\/10.1021\/jacs.0c00122<\/p>\n

2<\/strong>\u3001<\/strong>EES<\/strong>\uff1a\u53cc\u6469\u64e6\u7535\u7eb3\u7c73\u53d1\u7535\u673a\u9a71\u52a8\u7a7a\u6c14\u76f4\u63a5\u7535\u50ac\u5316\u5408\u6210\u6c28<\/strong><\/p>\n

\"\"<\/p>\n

\u7f8e\u56fd\u4f50\u6cbb\u4e9a\u7406\u5de5\u5b66\u9662\u3001\u4e2d\u56fd\u79d1\u5b66\u9662\u5317\u4eac\u7eb3\u7c73\u80fd\u6e90\u4e0e\u7cfb\u7edf\u7814\u7a76\u6240\u738b\u4e2d\u6797\u9662\u58eb\u548c\u5510\u4f1f\u7814\u7a76\u5458\u7b49\u4eba<\/strong>\u8bbe\u8ba1\u4e86\u4e00\u79cd\u7531\u9ad8\u8f93\u51fa\u53ccTENG\u88c5\u7f6e\u9a71\u52a8\u7684\u81ea\u4f9b\u7535\u7535\u50ac\u5316\u7cfb\u7edf\uff0c\u7528\u4e8e\u5408\u6210\u6c28\u3002\u901a\u8fc7\u7531TENG\u88c5\u7f6e\u5f15\u8d77\u7684\u7a7a\u6c14\u6392\u653e\uff0c\u6c2e\u6c14\u76f4\u63a5\u5229\u7528\u7a7a\u6c14\u4f5c\u4e3a\u8fdb\u4e00\u6b65\u5f62\u6210\u7535\u89e3\u8d28\u7684\u6e90\u800c\u56fa\u5b9a\u5728NOX<\/sub>\u4e2d\u3002\u540c\u65f6\uff0c\u5728\u53e6\u4e00\u4e2aTENG\u7684\u9a71\u52a8\u4e0b\uff0c\u4f7f\u7528\u4e8c\u6c27\u5316\u949b\u4f5c\u4e3a\u50ac\u5316\u5242\u8fdb\u884c\u7535\u50ac\u5316\u8fd8\u539f\u4ee5\u5728\u53cc\u5ba4\u7535\u50ac\u5316\u69fd\u4e2d\u5408\u6210\u6c28\u3002\u5728\u6d41\u901f\u4e3a3.5 m3<\/sup> min-1<\/sup>\u7684\u6a21\u62df\u5e9f\u6c14\u4e0b\uff0c\u81ea\u4f9b\u7535\u7535\u50ac\u5316\u7cfb\u7edf\u6bcf\u5c0f\u65f6\u7684\u6c28\u4ea7\u91cf\u4e3a2.4\u03bcgh-1<\/sup>\u3002\u4e0e\u4f20\u7edf\u7684\u5408\u6210\u65b9\u6cd5\u76f8\u6bd4\uff0c\u8be5\u7cfb\u7edf\u5177\u6709\u81ea\u4f9b\u7535\uff0c\u73af\u4fdd\uff0c\u6210\u672c\u4f4e\u5ec9\uff0c\u6613\u4e8e\u5236\u9020\uff0c\u53ef\u6269\u5c55\u7684\u4f18\u70b9\uff0c\u663e\u793a\u51fa\u5de8\u5927\u7684\u5408\u6210\u6c28\u6f5c\u529b\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/pubs.rsc.org\/en\/content\/articlepdf\/2020\/ee\/d0ee01102a<\/p>\n

3<\/strong>\u3001<\/strong>Nanoscale: Pt-Co<\/strong>\u516b\u9762\u4f53\u7eb3\u7c73\u6676\u4f53\uff1a\u4e00\u7c7b\u7528\u4e8e\u6c27\u8fd8\u539f\u7684\u9ad8\u6d3b\u6027\u548c\u6301\u4e45\u6027\u7684\u50ac\u5316\u5242<\/strong><\/p>\n

\"\"<\/p>\n

\u7f8e\u56fd\u4f50\u6cbb\u4e9a\u7406\u5de5\u5b66\u9662\u590f\u5e7c\u5357\u6559\u6388\u7b49\u4eba<\/strong>\u5f00\u53d1\u4e86\u4e00\u79cd\u4e00\u9505\u6cd5\u7b56\u7565\uff0c\u53ef\u7528\u4e8e\u5408\u6210Pt-Co\u516b\u9762\u4f53\u7eb3\u7c73\u6676\u4f53(TONs)\u3002\u7814\u7a76\u4eba\u5458\u53ef\u4ee5\u901a\u8fc7\u6539\u53d8Mn2<\/sub>(CO)10<\/sub>\u7684\u6dfb\u52a0\u91cf\u6765\u63a7\u5236\u5c3a\u5bf8\uff0c\u800c\u7eb3\u7c73\u6676\u4f53\u7684\u7ec4\u6210\u548c\u4ea7\u7387\u4e3b\u8981\u7531\u5f15\u5165\u53cd\u5e94\u6df7\u5408\u7269\u4e2d\u7684CHCl3<\/sub>\u7684\u4f53\u79ef\u51b3\u5b9a\u3002\u5728\u6db2\u4f53\u534a\u7535\u6c60\u6d4b\u8bd5\u4e2d\uff0c\u76f8\u5bf9\u4e8e\u5546\u4e1a\u5316TKK Pt3<\/sub>Co\/C\u7684\u6027\u80fd\uff0c\u6240\u83b7\u5f97\u7684Pt-Co TONs\u8868\u73b0\u51fa\u589e\u5f3a\u7684ORR\u6d3b\u6027\u3002\u5728\u76f8\u540c\u7684\u6d4b\u8bd5\u6761\u4ef6\u4e0b\uff0c\u50ac\u5316\u6d3b\u6027\u548c\u8010\u4e45\u6027\u5747\u8d85\u8fc7\u4e86\u5546\u4e1a\u5316\u7684TKK Pt3<\/sub>Co\/C\u3002\u7814\u7a76\u4eba\u5458\u5206\u6790\u8ba4\u4e3a\uff0c\u6027\u80fd\u7684\u63d0\u9ad8\u6e90\u81ea\u51cf\u5c0f\u7684\u7c92\u5f84\uff0c\u4ece\u800c\u6269\u5927\u4e86ECSA\uff0c\u4ee5\u53caPt-Co TON\u4e0a\u7ed3\u6784\u660e\u786e\u7684{111}\u9762\u3002\u53ef\u4ee5\u9884\u671f\uff0c\u8fd9\u79cd\u65b0\u578b\u7684Pt-Co\u50ac\u5316\u5242\u6709\u671b\u7528\u4e8e\u8d28\u5b50\u4ea4\u6362\u819c\u71c3\u6599\u7535\u6c60\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1039\/D0NR02904A<\/p>\n

4<\/strong>\u3001<\/strong>Nano Research: Pt3<\/sub>Ag<\/strong>\u5408\u91d1\u6ce2\u6d6a\u7eb3\u7c73\u7ebf\u4f5c\u4e3a\u4e59\u9187\u6c27\u5316\u53cd\u5e94\u7684\u9ad8\u6548\u7535\u50ac\u5316\u5242<\/strong><\/p>\n

\"\"<\/p>\n

\u7f8e\u56fd\u52a0\u5dde\u5927\u5b66\u6d1b\u6749\u77f6\u5206\u6821\u6bb5\u9576\u950b\u6559\u6388\u548c\u9ec4\u6631\u6559\u6388<\/strong>\u62a5\u544a\u4e86\u901a\u8fc7\u4e00\u79cd\u65b9\u4fbf\u7684\u6eb6\u5242\u70ed\u8fc7\u7a0b\u4e2d\u7684\u7c92\u5b50\u9644\u7740\u673a\u5236\u6765\u5408\u6210Pt3<\/sub>Ag\u6ce2\u6d6a\u72b6\u7eb3\u7c73\u7ebf\u3002\u900f\u5c04\u663e\u5fae\u955c\u7814\u7a76\u548c\u5143\u7d20\u5206\u6790\u663e\u793a\u51fa\u9ad8\u5ea6\u5448\u6ce2\u6d6a\u5f62\u7684\u7eb3\u7c73\u7ebf\u7ed3\u6784\uff0c\u5e73\u5747\u76f4\u5f84\u4e3a4.6\u00b11.0 nm\uff0c\u5e76\u4e14\u5f62\u6210\u4e86\u5747\u5300\u7684Pt3<\/sub>Ag\u5408\u91d1\u3002\u7535\u50ac\u5316\u7814\u7a76\u8868\u660e\uff0c\u5408\u91d1\u6ce2\u6d6a\u5f62\u7eb3\u7c73\u7ebf\u53ef\u4f5c\u4e3aEOR\u7684\u9ad8\u6548\u7535\u50ac\u5316\u5242\uff0c\u5177\u670928.0 mA\/cm2<\/sup>\u7684\u8d85\u9ad8\u6bd4\u6d3b\u5ea6\u548c6.1 A\/mg\u7684\u8d28\u91cf\u6d3b\u5ea6\uff0c\u8fdc\u8fdc\u8d85\u8fc7\u4e86\u5546\u7528Pt\/\u78b3\u6837\u54c1\uff081.10 A\/mg\uff09\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1007\/s12274-020-2754-4<\/p>\n

5<\/strong>\u3001<\/strong>Angew<\/strong>\uff1a\u901a\u8fc7\u7a33\u5b9a\u4e59\u6c27\u57fa\u4e2d\u95f4\u4f53\u5c06<\/strong>CO2<\/sub><\/strong>\u7535\u5316\u5b66\u8fd8\u539f\u4e3a\u4e59\u70f7<\/strong><\/p>\n

\"\"<\/p>\n

\u6fb3\u5927\u5229\u4e9a\u963f\u5fb7\u83b1\u5fb7\u5927\u5b66\u4e54\u4e16\u748b\u6559\u6388\u56e2\u961f<\/strong>\u4f7f\u7528\u67d0\u4e9b\u6a21\u578b\u5316\u5408\u7269\u884d\u751f\u7684\u94dc\u7535\u50ac\u5316\u5242\uff0c\u5373\u7898\u5316\u7269\u884d\u751f\u7684\u94dc\uff08ID-Cu\uff09\u548c\u6c27\u5316\u7269\u884d\u751f\u7684\u94dc\uff08OD-Cu\uff09\u6ce1\u6cab\uff0c\u7814\u7a76\u4e86CO2<\/sub>\u8f6c\u5316\u4e3a\u4e59\u70f7\u7684\u9014\u5f84\u3002\u4e0eOD-Cu\u76f8\u6bd4\uff0cID-Cu\u8868\u73b0\u51fa\u660e\u663e\u66f4\u9ad8\u7684\u4e59\u70f7\u9009\u62e9\u6027\u548c\u66f4\u6709\u5229\u7684\u52a8\u529b\u5b66\u3002XAS\u548c\u62c9\u66fc\u7814\u7a76\u8868\u660e\uff0c\u6d89\u53ca\u4e0e\u6c27\u7ed3\u5408\u7684\u4e59\u6c27\u57fa\uff08* OCH2<\/sub>CH3<\/sub>\uff09\u4e2d\u95f4\u4f53\uff0c\u7ecf\u8fc7\u9009\u62e9\u6027\u6b65\u9aa4\u53ef\u4ea7\u751f\u4e59\u70f7\u6216\u4e59\u9187\u3002\u7531\u4e8e\u94dc\u6676\u683c\u4e2d\u5b58\u5728\u5fae\u91cf\u7684\u7898\uff0c\u8be5\u4e2d\u95f4\u4f53\u4f3c\u4e4e\u5728ID-Cu\u4e0a\u5177\u6709\u66f4\u597d\u7684\u7a33\u5b9a\u6027\u3002\u56e0\u6b64\uff0c\u8be5\u7814\u7a76\u63d0\u4f9b\u4e86\u4e00\u79cd\u5408\u7406\u7684\u7b56\u7565\u6765\u8bbe\u8ba1\u5bf9\u9664\u4e59\u70ef\u548c\u4e59\u9187\u4ee5\u5916\u7684\u4ea7\u54c1\u5177\u6709\u9009\u62e9\u6027\u7684\u94dc\u57fa\u50ac\u5316\u5242\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/anie.202004846<\/p>\n

6<\/strong>\u3001<\/strong>AM<\/strong>\uff1a\u7a3b\u58f3\u76f4\u63a5\u8f6c\u5316\u4e3a\u7eb3\u7c73\u7ed3\u6784\u7684<\/strong>SiC\/C<\/strong>\u7528\u4e8e<\/strong>CO2 <\/sub>RR<\/strong><\/p>\n

\"\"<\/p>\n

\u5357\u6d0b\u7406\u5de5\u5927\u5b66\u697c\u96c4\u6587\u6559\u6388\u548c\u6b66\u6c49\u5927\u5b66\u8096\u5dcd\u6559\u6388<\/strong>\u5c55\u793a\u4e86\u4e00\u79cd\u7528\u4e8e\u690d\u7269\u751f\u7269\u8d28\u589e\u503c\u5229\u7528\u7684\u4e00\u6b65\u7194\u878d\u76d0\u8f85\u52a9\u7535\u5316\u5b66\u5408\u6210\u7b56\u7565\u3002\u901a\u8fc7\u4f7f\u7528CaCl2<\/sub>-NaCl\u7194\u878d\u76d0\u4f5c\u4e3a\u7535\u89e3\u8d28\uff0c\u56fa\u4f53\u7a3b\u58f3\u76f4\u63a5\u8f6c\u5316\u4e3aSiC-\u7eb3\u7c73\u7ebf\/C\uff08SiC-NW\/C\uff09\u590d\u5408\u6750\u6599\u3002\u8fd9\u79cd\u7eb3\u7c73\u7ed3\u6784\u7684\u590d\u5408\u6750\u6599\u5728\u4e0d\u4f7f\u7528\u4efb\u4f55\u52a9\u50ac\u5316\u5242\u6216\u727a\u7272\u5242\u7684\u60c5\u51b5\u4e0b\uff0c\u5bf9CO2<\/sub>\u5149\u8fd8\u539f\u4e3aCO\u7684\u6d3b\u6027\u5927\u5927\u589e\u5f3a\u3002\u7194\u878d\u76d0\u7cfb\u7edf\u5177\u6709\u81ea\u6eb6\u80fd\u529b\uff0c\u53ef\u6eb6\u89e3\u6709\u5bb3\u5143\u7d20\uff0c\u56e0\u6b64\u65e0\u9700\u4efb\u4f55\u7cbe\u5236\u6b65\u9aa4\u5373\u53ef\u786e\u4fdd\u751f\u7269\u8d28\u5229\u7528\u7684\u667a\u80fd\u8fc7\u7a0b\u3002\u8be5\u8fc7\u7a0b\u8fd8\u53ef\u80fd\u5728\u751f\u7269\u8d28\u7684\u751f\u4ea7\u5229\u7528\u4e2d\u5b9e\u73b0\u53ef\u6301\u7eed\u7684\u78b3\u5faa\u73af\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/adma.202001560<\/a><\/p>\n

7<\/strong>\u3001<\/strong>AEM<\/strong>\uff1a\u5206\u5c42\u591a\u5143\u7d20\u7eb3\u7c73\u9897\u7c92\u4f5c\u4e3a\u53cc\u529f\u80fd\u50ac\u5316\u5242\uff0c\u7528\u4e8e<\/strong>OER<\/strong>\u548c<\/strong>ORR<\/strong><\/p>\n

\"\"<\/p>\n

\u7f8e\u56fd\u9a6c\u91cc\u5170\u5927\u5b66\u80e1\u826f\u5175\u6559\u6388\uff0c\u674e\u817e\u6559\u6388<\/strong>\u63d0\u51fa\u4e86\u4e00\u79cd\u7b80\u4fbf\u7684\u65b9\u6cd5\uff0c\u7528\u4e8e\u5408\u6210\u5206\u7ea7\u7684\u591a\u5143\u7d20\u53cc\u529f\u80fd\u50ac\u5316\u5242\uff0c\u4ee5\u8fdb\u884c\u6709\u6548\u7684\u6c27\u6c14\u91ca\u653e\u548c\u8fd8\u539f\u53cd\u5e94\u3002\u901a\u8fc7\u4e00\u6b65\u5408\u6210\uff0c\u5c06\u8d85\u5c0f\u7684IrPt\u5408\u91d1\u7eb3\u7c73\u9897\u7c92\u56fa\u5b9a\u5728\u5c16\u6676\u77f3\u578bFeCoNiOx<\/sub>\u6df7\u5408\u7eb3\u7c73\u9897\u7c92\u4e0a\uff0c\u4ee5\u751f\u4ea7\u72ec\u7279\u7684\u5206\u7ea7\u50ac\u5316\u5242\u3002\u5177\u6709\u591a\u79cd\u6d3b\u6027\u5143\u7d20\uff0c\u6df7\u5408\u5316\u5b66\u72b6\u6001\u548c\u9ad8\u7535\u6d3b\u6027\u8868\u9762\u79ef\u7684\u7eb3\u7c73\u50ac\u5316\u5242\u5177\u6709\u534f\u540c\u548c\u5e73\u8861\u7684\u5438\u9644\/\u89e3\u5438\u7279\u6027\uff0c\u4f7f\u5176\u6210\u4e3a\u9ad8\u6548\u7684\u53cc\u529f\u80fd\u50ac\u5316\u5242\u3002\u5728\u76f8\u540c\u7684\u8d85\u7535\u52bf\u4e0b\uff0c\u805a\u5143\u7d20\u7eb3\u7c73\u50ac\u5316\u5242\u7684\u8d28\u91cf\u6d3b\u5ea6\uff08\u6807\u51c6\u5316\u4e3aIr\u6216Pt\uff09\u5728OER\u4e2d\u662fIr\u768428\u500d\uff0c\u5728ORR\u4e2d\u662fPt\u76847\u500d\u3002\u9ad8\u6e29\u5904\u7406\u8fd8\u53ef\u4ee5\u5728\u5206\u5c42\u7eb3\u7c73\u9897\u7c92\u4e2d\u5b9e\u73b0Pt-\u91d1\u5c5e\u952e\u5408\uff0c\u4ece\u800c\u4e3a\u6301\u4e45\u7684\u7535\u50ac\u5316\u63d0\u4f9b\u4e86\u7a33\u5b9a\u7684\u7ed3\u6784\u3002\u8fd9\u79cd\u9ad8\u6548\u4e14\u8010\u7528\u7684\u53cc\u529f\u80fd\u6c27\u7535\u50ac\u5316\u5242\u53ef\u4ee5\u5927\u5927\u63d0\u9ad8\u91d1\u5c5e-\u7a7a\u6c14\u7535\u6c60\u7684\u80fd\u6e90\u6548\u7387\uff0c\u5e76\u6709\u53ef\u80fd\u5728\u6c34\u7535\u89e3\uff0c\u71c3\u6599\u7535\u6c60\u7b49\u9886\u57df\u4e2d\u4f7f\u7528\u3002\u8fd9\u79cd\u5206\u5c42\u7684\u591a\u5143\u7d20\u7eb3\u7c73\u9897\u7c92\u8bbe\u8ba1\u4e3a\u53d1\u73b0\u5177\u6709\u957f\u5bff\u547d\u548c\u6210\u672c\u6548\u76ca\u7684\u591a\u529f\u80fd\u50ac\u5316\u5176\u5b83\u591a\u5143\u7d20\u7eb3\u7c73\u6750\u6599\u6253\u5f00\u4e86\u4e00\u6247\u95e8\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/aenm.202001119<\/p>\n

8<\/strong>\u3001<\/strong>AEM<\/strong>\uff1a\u77f3\u58a8\u70ef\u91cf\u5b50\u70b9\u57fa\u5148\u8fdb\u7535\u6781\u6750\u6599\u7684\u8bbe\u8ba1\u3001\u5408\u6210\u53ca\u5176\u5728\u7535\u5316\u5b66\u50a8\u80fd\u548c\u7535\u50ac\u5316\u4e2d\u7684\u5e94\u7528<\/strong><\/p>\n

\"\"<\/p>\n

\u52a0\u62ff\u5927\u6ed1\u94c1\u5362\u5927\u5b66\u9648\u5fe0\u4f1f\u9662\u58eb\uff0c\u4f59\u7231\u840d\u6559\u6388\u548c\u5409\u6797\u5e08\u8303\u5927\u5b66\u51af\u660e\u6559\u6388<\/strong>\u7efc\u8ff0\u4e86GQD\u548c\u57fa\u4e8eGQD\u7684\u6750\u6599\u5728\u5f00\u53d1\u9ad8\u6027\u80fd\u7535\u5316\u5b66\u80fd\u91cf\u5b58\u50a8\u548c\u50ac\u5316\u7cfb\u7edf\u4e2d\u7684\u91cd\u8981\u6027\u548c\u5de8\u5927\u6f5c\u529b\u3002\u4ed4\u7ec6\u7814\u7a76\u672c\u7efc\u8ff0\u4e2d\u8ba8\u8bba\u7684\u57fa\u4e8eGQD\u7684\u6750\u6599\u5728\u8fd9\u4e9b\u4e0e\u80fd\u6e90\u76f8\u5173\u7684\u9886\u57df\u4e2d\u7684\u5e94\u7528\uff0c\u53d1\u73b0\u4ecd\u7136\u6709\u8bb8\u591a\u5de5\u4f5c\u8981\u505a\uff0c\u8bb8\u591a\u7814\u7a76\u9886\u57df\u9700\u8981\u8fdb\u4e00\u6b65\u53d1\u5c55\u3002\u7279\u522b\u5730\uff0c\u968f\u7740\u5148\u8fdb\u6280\u672f\u548c\u8868\u5f81\u7684\u53d1\u5c55\uff0c\u7814\u7a76\u4eba\u5458\u5c06\u4f1a\u53d1\u73b0GQD\u7684\u65b0\u9896\u7269\u7406\u5316\u5b66\u6027\u8d28\uff0c\u4ece\u800c\u8d4b\u4e88GQD\u4f18\u5f02\u7684\u6027\u80fd\uff0c\u5e76\u5c06\u5176\u5e94\u7528\u6269\u5c55\u5230\u5176\u5b83\u6709\u524d\u9014\u7684\u7814\u7a76\u9886\u57df\u3002\u56e0\u6b64\uff0c\u7814\u7a76\u4eba\u5458\u4ecd\u6709\u5f88\u5927\u7684\u7a7a\u95f4\u53ef\u4ee5\u7ee7\u7eed\u521b\u65b0\uff0c\u5e76\u5728\u80fd\u91cf\u5b58\u50a8\u548c\u50ac\u5316\u9886\u57df\u627e\u5230\u66f4\u591a\u7684\u6f5c\u5728\u5e94\u7528\u3002\u603b\u800c\u8a00\u4e4b\uff0c\u7814\u7a76\u4eba\u5458\u5e0c\u671b\u8fd9\u4e00\u91cd\u8981\u7684\u603b\u7ed3\u548c\u8fdb\u5c55\u80fd\u591f\u4e3a\u4e0e\u9ad8\u6027\u80fd\u7535\u5316\u5b66\u50a8\u80fd\u548c\u7535\u50ac\u5316\u88c5\u7f6e\u7684\u521b\u65b0\u548c\u5efa\u8bbe\u6709\u5173\u7684\u7814\u7a76\u63d0\u4f9b\u4e00\u4e9b\u5efa\u8bbe\u6027\u7684\u5efa\u8bae\u548c\u65b0\u89c1\u89e3\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/aenm.202001275<\/p>\n

9<\/strong>\u3001<\/strong>Chem. Rev.<\/strong>\uff1a\u5305\u8986\u91d1\u5c5e\u7eb3\u7c73\u9897\u7c92\u5728\u50ac\u5316\u4e2d\u7684\u5e94\u7528<\/strong><\/p>\n

\"\"<\/p>\n

\u52a0\u5dde\u5927\u5b66\u6cb3\u6ee8\u5206\u6821\u6bb7\u4e9a\u4e1c\u6559\u6388<\/strong>\u5bf9\u5305\u8986\u91d1\u5c5e\u7eb3\u7c73\u9897\u7c92\u7684\u5408\u6210\u548c\u50ac\u5316\u6027\u80fd\u7684\u6700\u65b0\u8fdb\u5c55\u7684\u5168\u9762\u603b\u7ed3\u3002\u8fd9\u7bc7\u7efc\u8ff0\u9996\u5148\u4ecb\u7ecd\u4e86\u7528\u4e8e\u5408\u6210\u5177\u6709\u4e0d\u540c\u7ed3\u6784\u7684\u91d1\u5c5e\u7eb3\u7c73\u9897\u7c92\u7684\u5408\u6210\u7b56\u7565\uff0c\u5305\u62ec\u5728\u65e0\u673a\u6c27\u5316\u7269\u548c\u78b3\uff0c\u591a\u5b54\u6750\u6599\uff08\u6cb8\u77f3\uff0c\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6\u548c\u5171\u4ef7\u6709\u673a\u9aa8\u67b6\uff09\u4ee5\u53ca\u6709\u673a\u80f6\u56ca\uff08\u6811\u679d\u72b6\u5927\u5206\u5b50\u548c\u6709\u673a\u7b3c\u5b50\uff09\u3002\u7136\u540e\u8ba8\u8bba\u4e86\u5305\u8986\u7684\u91d1\u5c5e\u7eb3\u7c73\u9897\u7c92\u7684\u4f18\u52bf\uff0c\u4f8b\u5982\u589e\u5f3a\u7684\u7a33\u5b9a\u6027\u548c\u53ef\u56de\u6536\u6027\uff0c\u6539\u8fdb\u7684\u9009\u62e9\u6027\uff0c\u5f3a\u5927\u7684\u91d1\u5c5e-\u8f7d\u4f53\u76f8\u4e92\u4f5c\u7528\u4ee5\u53ca\u5b9e\u73b0\u4e32\u8054\u50ac\u5316\u7684\u80fd\u529b\uff0c\u968f\u540e\u4ecb\u7ecd\u4e86\u5305\u8986\u7684\u91d1\u5c5e\u7eb3\u7c73\u9897\u7c92\u5728\u70ed\u50ac\u5316\uff0c\u5149\u50ac\u5316\u548c\u7535\u50ac\u5316\u7b49\u7684\u5e94\u7528\u3002\u5728\u8fd9\u7bc7\u8bc4\u8bba\u7684\u7ed3\u5c3e\uff0c\u7814\u7a76\u4eba\u5458\u8ba8\u8bba\u4e86\u4e0e\u5c01\u88c5\u7684\u91d1\u5c5e\u7eb3\u7c73\u9897\u7c92\u76f8\u5173\u7684\u4e00\u4e9b\u6311\u6218\uff0c\u5e76\u63d0\u4f9b\u4e86\u5bf9\u8be5\u9886\u57df\u672a\u6765\u53d1\u5c55\u7684\u770b\u6cd5\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/dx.doi.org\/10.1021\/acs.chemrev.0c00237<\/p>\n

10<\/strong>\u3001<\/strong>Angew.:<\/strong>\u5236\u5907\u7528\u4e8e\u9ad8\u6548\u6790\u6c27\u53cd\u5e94\u7684\u53cc\u539f\u5b50\u94c1\u50ac\u5316\u5242\uff1a\u4e00\u79cd\u6742\u539f\u5b50\u8c03\u8282\u5242\u65b9\u6cd5<\/strong><\/p>\n

\"\"<\/p>\n

\u65e5\u672c\u4ea7\u4e1a\u6280\u672f\u7efc\u5408\u7814\u7a76\u6240\u5f90\u5f3a\u6559\u6388<\/strong>\u7b49\u4eba\u8bbe\u8ba1\u5e76\u6784\u5efa\u4e86\u72ec\u7279\u7684MOF\uff0c\u5176\u7ed3\u6784\u4e0a\u5177\u6709\u4e30\u5bcc\u7684\u6709\u5e8f\u82b3\u9999\u73af\u9635\u5217\uff0c\u53ef\u4ee5\u901a\u8fc7\u70ed\u5904\u7406\u8f6c\u53d8\u4e3a\u63ba\u6c2e\u78b3\u5c42\u3002\u91cd\u8981\u7684\u662f\uff0c\u57fa\u4e8e\u8fd9\u79cd\u5e73\u53f0\u6750\u6599\uff0c\u5df2\u5f00\u53d1\u51fa\u4e00\u79cd\u6742\u539f\u5b50\u8c03\u5236\u5668\u65b9\u6cd5\u6765\u63ed\u793a\u6240\u652f\u6301\u7684\u91d1\u5c5e\u56e2\u7c07\u5f62\u5f0f\u4e0e\u91d1\u5c5e\u539f\u5b50\u7684\u79cd\u7c7b\u548c\u6570\u91cf\u4e4b\u95f4\u7684\u660e\u786e\u76f8\u5173\u6027\u3002\u501f\u52a9\u5f3a\u5927\u7684XAFS\u5206\u6790\u548cTEM\u6210\u50cf\u4ee5\u53ca\u7406\u8bba\u8ba1\u7b97\uff0c\u7814\u7a76\u4eba\u5458\u786e\u5b9a\u4e86\u8d1f\u8f7d\u7684\u53cc\u539f\u5b50\u94c1\u7a33\u5b9a\u5728\u78b3\u5c42\u5185\u7684\u6700\u4f73\u91d1\u5c5e\u6c2e\u90e8\u5206\u4e2d\uff0c\u8bc1\u660e\u4e86\u8d1f\u8f7d\u7684\u94c1\u4e8c\u805a\u4f53\uff08\u7528\u4f5c\u91d1\u5c5e\u914d\u5408\u4f4d\u70b9\uff09\u53ef\u6709\u6548\u5730\u50ac\u5316\u6790\u6c27\u53cd\u5e94\u3002\u8fd9\u9879\u5de5\u4f5c\u63d0\u51fa\u7684\u6982\u5ff5\u3001\u65b9\u6cd5\u548c\u7ed3\u679c\u5c06\u4e3a\u672a\u6765\u9ad8\u6d3b\u6027USMC\u50ac\u5316\u8bbe\u8ba1\u63d0\u4f9b\u6709\u4ef7\u503c\u7684\u7b56\u7565\u6307\u5bfc\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1002\/anie.202007221<\/p>\n

11<\/strong>\u3001<\/strong>Nano Lett.<\/strong>\uff1a<\/strong> \u78b3\u5316\u949b\u7a33\u5b9a\u7684\u5206\u5b50\u8584\u6c2e\u5316\u7269\u8584\u5c42\u4f5c\u4e3a\u7ea4\u7ef4\u72b6\u53ef\u5145\u7535\u950c\u7a7a\u6c14\u7535\u6c60\u7684\u9ad8\u6548\u53cc\u529f\u80fd\u7535\u50ac\u5316\u5242<\/strong><\/p>\n

\"\"<\/p>\n

\u6fb3\u5927\u5229\u4e9a\u6089\u5c3c\u79d1\u6280\u5927\u5b66\u6c6a\u56fd\u79c0\u6559\u6388\u548c\u82cf\u5dde\u5927\u5b66\u803f\u51e4\u971e\u6559\u6388\u7b49\u4eba<\/strong>\u6210\u529f\u5730\u83b7\u5f97\u4e86\u4e00\u79cd\u975e\u8d35\u91d1\u5c5e\u7684\u4e09\u91d1\u5c5e\u6c2e\u5316\u7269\u7535\u50ac\u5316\u5242\uff0c\u8be5\u50ac\u5316\u5242\u65e2\u5177\u6709\u51fa\u8272\u7684OER\u8868\u73b0\uff0c\u53c8\u5177\u6709\u4f18\u5f02\u7684ORR\u7535\u50ac\u5316\u6d3b\u6027\u3002\u4f7f\u7528\u8bbe\u8ba1\u7684\u7535\u50ac\u5316\u5242\u4f5c\u4e3a\u7a7a\u6c14\u6b63\u6781\u548c\u51dd\u80f6\u805a\u5408\u7269\u7535\u89e3\u8d28\u7684\u67d4\u6027\u7ea4\u7ef4\u72b6\u950c\u7a7a\u6c14\u7535\u6c60\u53ef\u4ee5\u8f93\u51fa\u521b\u7eaa\u5f55\u7684627 Wh kgzn-1<\/sup>\u7684\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u3002\u5373\u4f7f\u5728\u4e25\u91cd\u7684\u673a\u68b0\u53d8\u5f62\u4e0b\uff0c\u8be5\u7535\u6c60\u4e5f\u80fd\u591f\u7a33\u5b9a\u5730\u4e3a\u5305\u62ecLED\u706f\uff0c\u7535\u81f4\u53d1\u5149\u9762\u677f\u7b49\u5728\u5185\u7684\u5404\u79cd\u7535\u5b50\u8bbe\u5907\u4f9b\u7535\u3002\u8fd9\u9879\u5de5\u4f5c\u7684\u6210\u529f\u7a81\u51fa\u4e86\u50ac\u5316\u5242\u7ed3\u6784\u7684\u91cd\u8981\u6027\uff0c\u5e76\u4e3a\u63a2\u7d22\u6750\u6599\u56fa\u6709\u7684\u50ac\u5316\u53cd\u5e94\u6027\u5f00\u8f9f\u4e86\u65b0\u7684\u7a97\u53e3\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1ahttps:\/\/pubs.acs.org\/doi\/pdf\/10.1021\/acs.nanolett.0c00717<\/p>\n

\u672c\u6587\u7531eric<\/span>\u4f9b\u7a3f\u3002<\/p>\n

\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n

\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaorenVIP\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"

1\u3001JACS\uff1a\u94dc\u57fa\u50ac\u5316\u5242\u9ad8\u538b\u7535\u8fd8\u539fCO2\u9ad8\u6548\u5236\u7532\u9178 \u7f8e\u56fd\u65af\u5766\u798f\u5927\u5b66\u7684\u6234\u5b8f\u6770\u9662\u58eb\u56e2\u961f\u8bbe\u8ba1\u4e86\u4e00\u79cd\u8d85\u7eaf\u94dc\u7b94\u7684\u65b9\u6ce2\u7535\u5316\u5b66\u6c27\u5316\u8fd8\u539f\u5faa\u73af\u5904\u7406\u65b9\u6cd5\uff0c\u5236\u5907\u4e86\u5bcc\u542b\uff08111\uff09\u53d6\u5411C…<\/p>\n","protected":false},"author":11454,"featured_media":205304,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[1187],"tags":[],"class_list":["post-205292","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-zhuanlan"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/205292"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/11454"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=205292"}],"version-history":[{"count":4,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/205292\/revisions"}],"predecessor-version":[{"id":205934,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/205292\/revisions\/205934"}],"wp:featuredmedia":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/media\/205304"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=205292"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=205292"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=205292"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}