{"id":205897,"date":"2020-08-01T06:35:25","date_gmt":"2020-07-31T22:35:25","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=205897"},"modified":"2020-07-31T20:35:48","modified_gmt":"2020-07-31T12:35:48","slug":"%e9%a6%99%e6%b8%af%e5%9f%8e%e5%b8%82%e5%a4%a7%e5%ad%a6chun-sing-lee%e4%b8%8e%e7%8e%8b%e7%ab%8b%e4%bb%a3%e5%9b%a2%e9%98%9f%e8%81%94%e5%90%88%e6%b2%b3%e5%8d%97%e5%a4%a7%e5%ad%a6%e9%bb%84%e6%b0%b8","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=205897","title":{"rendered":"\u9999\u6e2f\u57ce\u5e02\u5927\u5b66Chun-Sing Lee\u4e0e\u738b\u7acb\u4ee3\u56e2\u961f\u8054\u5408\u6cb3\u5357\u5927\u5b66\u9ec4\u6c38\u4f1fAdv. Mater.\uff1aNIR-II\u751f\u7269\u7a97\u4e2d\u5171\u8f6d\u5c0f\u5206\u5b50\u5bf9\u8d85\u5f3a\u5149\u70ed\u7406\u8bba\u7684\u5408\u7406\u8bbe\u8ba1"},"content":{"rendered":"

\u3010\u5f15\u8a00<\/strong>\u3011<\/p>\n

\u8fd1\u51e0\u5341\u5e74\u6765\uff0c\u5149\u70ed\u7597\u6cd5\uff08PTT\uff09\u5229\u7528\u5149\u5438\u6536\u5242\u5438\u6536\u5149\u80fd\u5236\u9020\u5c40\u90e8\u70ed\u91cf\u6765\u6d88\u878d\u764c\u75c7\u7684\u65b0\u578b\u7597\u6cd5\uff0c\u4e14\u5728\u8fc7\u53bb\u5341\u5e74\u53d6\u5f97\u4e86\u5de8\u5927\u8fdb\u6b65\u3002\u5bf9\u4e8ePTT\u5e94\u7528\uff0c\u4e5f\u5df2\u7ecf\u63a2\u7d22\u4e86\u4e0d\u540c\u7684PTT\u8bd5\u5242\uff0c\u5305\u62ec\u91d1\u7eb3\u7c73\u7ed3\u6784\uff0c2D\u78b3\u6750\u6599\uff0c\u8fc7\u6e21\u91d1\u5c5e\u4e8c\u5364\u5316\u7269\uff08TMDC\uff09\uff0c2D\u78b3\u5316\u7269\u548c\u6c2e\u5316\u7269\uff08MXenes\uff09\u4ee5\u53ca\u5171\u8f6d\u805a\u5408\u7269\u3002 \u5728\u8fc7\u53bb\u7684\u51e0\u5e74\u4e2d\uff0c\u79d1\u5b66\u5bb6\u4eec\u805a\u7126\u5de8\u5927\u7684\u52aa\u529b\u6765\u5f00\u53d1\u5177\u6709\u826f\u597d\u7684\u8fd1\u7ea2\u5916\uff08NIR\uff09\u54cd\u5e94\u7684PTT\u5242\uff0c\u4ee5\u5b9e\u73b0\u66f4\u6df1\u7684\u7ec4\u7ec7\u6e17\u900f\u5e76\u6700\u5c0f\u5316\u5bf9\u5065\u5eb7\u7ec4\u7ec7\u7684\u635f\u5bb3\u3002\u5c24\u5176\u662fNIR-II\uff081000-1700 nm\uff09\u6d3b\u6027\u7684PTT\u5242\u5f15\u8d77\u4e86\u4eba\u4eec\u7684\u5e7f\u6cdb\u5173\u6ce8\uff0c\u8fd9\u662f\u56e0\u4e3aNIR-II\u4e0eNIR-I\uff08700-1000 nm\uff09\u76f8\u6bd4\u5177\u6709\u66f4\u6df1\u7684\u7a7f\u900f\u529b\u548c\u66f4\u9ad8\u7684\u5141\u8bb8\u66b4\u9732\u91cf\u3002\u5c3d\u7ba1\u5728\u8fc7\u53bb\u51e0\u5e74\u4e2d\u5df2\u7ecf\u53d6\u5f97\u4e86\u5927\u91cf\u7684\u6210\u529f\uff0c\u76ee\u524d\u62a5\u9053\u7684NIR-II PTT\u8bd5\u5242\u4ecd\u7136\u505c\u7559\u5728\u8f83\u4f4e\u7684\u5149\u70ed\u8f6c\u5316\u6548\u7387\uff08PCE\uff09\uff0c\u4e14\u4ecd\u8fdc\u4f4e\u4e8e\u6210\u719f\u7684NIR-I PTT\u8bd5\u5242\u3002<\/p>\n

\u5230\u76ee\u524d\u4e3a\u6b62\uff0c\u6240\u6709\u62a5\u9053\u7684NIR-II PTT\u8bd5\u5242\u90fd\u662f\u65e0\u673a\u6750\u6599\u6216\u805a\u5408\u6750\u6599\u3002\u5230\u76ee\u524d\u4e3a\u6b62\uff0c\u5c1a\u65e0\u5173\u4e8e\u5177\u6709NIR-II\u53cd\u5e94\u7684\u5c0f\u5206\u5b50PTT\u836f\u7269\u7684\u62a5\u9053\u3002\u4e0e\u65e0\u673a\u548c\u805a\u5408\u7269\u6750\u6599\u76f8\u6bd4\uff0c\u5c0f\u5206\u5b50\u6750\u6599\u901a\u5e38\u5177\u6709\u66f4\u597d\u7684\u751f\u7269\u76f8\u5bb9\u6027\uff0c\u5c24\u5176\u662f\u8f83\u9ad8\u7684\u8eab\u4f53\u6e05\u9664\u7387\u3002\u5728\u8fc7\u53bb\u7684\u51e0\u5e74\u4e2d\uff0c\u5df2\u91c7\u7528\u4e86\u5404\u79cd\u4e0d\u540c\u7684\u7b56\u7565\uff0c\u4f8b\u5982\u5f15\u5165\u5206\u5b50\u5185\u7535\u8377\u8f6c\u79fb\uff08ICT\uff09\u548c\u5177\u6709\u8fd0\u52a8\u7075\u6d3b\u6027\u7684\u5206\u5b50\u7247\u6bb5\uff0c\u6765\u589e\u5f3aNIR\u5149\u70ed\u8f6c\u6362\u3002\u7136\u800c\uff0c\u8fd9\u4e9b\u65b9\u6cd5\u7684\u6548\u679c\u4ec5\u9650\u4e8e\u8c03\u8282NIR-1\u7a97\u53e3\u4e2d\u7684\u5149\u6536\u96c6\u3002\u56e0\u6b64\uff0c\u975e\u5e38\u9700\u8981\u5f00\u53d1\u65b0\u7684\u65b9\u6cd5\u6765\u5c06\u8fd9\u4e9b\u5c0f\u5206\u5b50PTT\u8bd5\u5242\u7684\u53cd\u5e94\u8f6c\u53d8\u4e3aNIR-II\u65b9\u6848\u3002\u5728\u8fc7\u53bb\u7684\u51e0\u5341\u5e74\u4e2d\uff0c\u5177\u6709\u7535\u5b50\u79bb\u57df\u548c\u5149\u6355\u83b7\u6027\u80fd\u7684\u5171\u8f6d\u5c0f\u5206\u5b50\u5df2\u7ecf\u5e7f\u6cdb\u5e94\u7528\u4e8e\u6709\u673a\u53d1\u5149\u4e8c\u6781\u7ba1\uff08OLED\uff09\uff0c\u6709\u673a\u5149\u4f0f\uff08OPV\uff09\u548c\u6709\u673a\u573a\u6548\u5e94\u6676\u4f53\u7ba1\uff08OFET\uff09\u3002\u6700\u8fd1\u7684\u8fdb\u5c55\u8868\u660e\u4e86\u5b83\u4eec\u5728\u5149\u6536\u96c6\u548c\u653e\u5927\u80fd\u529b\u65b9\u9762\u7684\u4f18\u52bf\uff0c\u5e76\u4fc3\u8fdb\u4e86\u5305\u62ec\u5149\u5b66\u751f\u7269\u4f20\u611f\u5668\uff0c\u751f\u7269\u6210\u50cf\u548c\u5149\u7597\u5728\u5185\u7684\u5927\u91cf\u751f\u7269\u533b\u5b66\u5e94\u7528\u3002\u5f53\u524d\u7684\u5f00\u91c7\u4e3b\u8981\u96c6\u4e2d\u5728\u53ef\u89c1\u533a\u57df\uff0c\u8fd9\u963b\u788d\u4e86\u5b83\u4eec\u5728\u6df1\u5c42\u7ec4\u7ec7\u4e2d\u7684\u5e94\u7528\u3002\u8fd1\u7ea2\u5916\u5171\u8f6d\u5c0f\u5206\u5b50\u7684\u53d1\u5c55\u5f15\u8d77\u4e86\u8d8a\u6765\u8d8a\u591a\u7684\u5173\u6ce8\uff0c\u7279\u522b\u662f\u5149\u70ed\u5206\u5b50\u3002\u7136\u800c\uff0c\u5728NIR-II\u7a97\u53e3\u4e2d\u6d89\u53ca\u5171\u8f6d\u5206\u5b50\u7684PTT\u7684\u62a5\u9053\u5f88\u5c11\uff0c\u7279\u522b\u662f\uff0c\u63a2\u7d22PTT\u5206\u5b50\u7684\u7ed3\u6784-\u529f\u80fd\u5173\u7cfb\u4ecd\u7136\u662f\u4e00\u4e2a\u6311\u6218\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb<\/strong>\u3011<\/p>\n

\u00a0\u00a0\u00a0\u00a0\u00a0\u00a0\u00a0 <\/strong>\u5728\u8fd9\u4e2a\u5de5\u4f5c\u4e2d\uff0c\u901a\u8fc7\u53d6\u4ee3\u5355\u4e2a\u539f\u5b50\u7684\u5206\u5b50\u624b\u672f\u7cbe\u786e\u5730\u8c03\u8282\u4e86\u4ece\u7b2c\u4e00NIR\u7a97\u53e3\u5230NIR-II\u7a97\u53e3\u7684\u03c0\u5171\u8f6d\u5c0f\u5206\u5b50\u7684\u5149\u5438\u6536\u3002\u5229\u7528\u8fd9\u79cd\u6280\u672f\uff0c\u9996\u6b21\u5c55\u793a\u4e86\u5438\u6536\u5cf0\u8d85\u8fc71000 nm\u7684\u5171\u8f6d\u4f4e\u805a\u7269\uff08IR-SS\uff09\uff0c\u5176\u7eb3\u7c73\u9897\u7c92\u57281064 nm\u6fc0\u53d1\u4e0b\u5b9e\u73b0\u4e86\u521b\u7eaa\u5f55\u768477\uff05\u7684\u9ad8\u5149\u70ed\u8f6c\u6362\u6548\u7387\u3002 \u7eb3\u7c73\u7c92\u5b50\u5728\u4f53\u5916\u548c\u4f53\u5185\u663e\u793a\u51fa\u826f\u597d\u7684\u5149\u58f0\u54cd\u5e94\uff0c\u5149\u70ed\u6cbb\u7597\u529f\u6548\u548c\u751f\u7269\u76f8\u5bb9\u6027\u3002\u8fd9\u9879\u5de5\u4f5c\u5236\u5b9a\u4e86\u63d0\u9ad8\u764c\u75c7\u6cbb\u7597\u5b66\u5728NIR-II\u7a97\u53e3\u4e2d\u7684\u5149\u6536\u96c6\u6548\u7387\u7684\u7b56\u7565\uff0c\u4e3a\u63a8\u8fdbNIR-II\u5149\u70ed\u5242\u7684\u8bbe\u8ba1\u548c\u5e94\u7528\u8fc8\u51fa\u4e86\u91cd\u8981\u7684\u4e00\u6b65\u3002\u8be5\u6210\u679c\u4ee5\u9898\u4e3a\u201cRational Design of Conjugated Small Molecules for Superior Photothermal Theranostics in the NIR-II Biowindow\u201d<\/strong>\u53d1\u8868\u5728Adv. Mater.<\/strong>\u4e0a<\/strong>\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

Scheme 1.NIR-II<\/strong>\u7eb3\u7c73\u70ed\u589e\u5f3a\u5171\u8f6d\u5c0f\u5206\u5b50\u5206\u5b50\u624b\u672f\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

Figure 1.<\/strong>\u5206\u5b50\u7684\u7ed3\u6784\u4e0e\u8868\u5f81<\/strong>\"\"<\/strong><\/p>\n

a\uff09\u7ea2\u5916\u5206\u5b50\u7684\u7ed3\u6784<\/p>\n

b\uff09\u56db\u6c22\u544b\u5583\u4e2d\u4e09\u4e2a\u5206\u5b50\u7684\u5f52\u4e00\u5316\u5438\u6536\u5149\u8c31<\/p>\n

c\uff09\u8ba1\u7b97\u7684HOMO\u548cLUMO\u80fd\u7ea7<\/p>\n

Figure <\/strong>2.NP<\/strong>\u7684\u5236\u5907\u4e0e\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

a\uff09NP\u7684\u5236\u5907\u8fc7\u7a0b\u793a\u610f\u56fe<\/p>\n

b\uff09NP\u7684TEM\u56fe\u50cf<\/p>\n

c\uff09NPs\u5206\u6563\u4f53\u7684DLS\u8c31<\/p>\n

d\uff09\u4e09\u79cdNPs\u6c34\u6eb6\u6db2\u7684\u5f52\u4e00\u5316\u5438\u6536\u5149\u8c31<\/p>\n

e\uff09\u4e09\u79cdNP\u5206\u6563\u4f53\u57281064 nm\u8f90\u716710\u5206\u949f\u540e\u7684\u5149\u70ed\u52a0\u70ed\u66f2\u7ebf\uff0c\u7136\u540e\u51b7\u5374\u81f3\u5ba4\u6e29<\/p>\n

f\uff09\u4e09\u79cdNPs\u5206\u6563\u4f53\u7684\u7ea2\u5916\u6210\u50cf\u4e0e\u8f90\u5c04\u65f6\u95f4\u7684\u5173\u7cfb<\/p>\n

g\uff09\u57281064 nm\u6fc0\u5149\u7167\u5c0410\u5206\u949f\u540e\uff0cIR-SS NP\u7684\u5149\u70ed\u6027\u80fd\u4e0e\u6d53\u5ea6\u7684\u5173\u7cfb<\/p>\n

h\uff09\u57285\u4e2a\u5f00\/\u5173\u5faa\u73af\u4e2d\uff0c\u57281 W\/cm2<\/sup>\u76841064 nm\u6fc0\u5149\u8f90\u7167\u4e0b\uff0cIR-SS NP\u7684\u5149\u70ed\u7a33\u5b9a\u6027<\/p>\n

i\uff09\u901a\u8fc7\u7ebf\u6027\u5206\u6790\u51b7\u5374\u5230\u5ba4\u6e29\uff0cIR-SS NP\u7684\u5149\u70ed\u6027\u80fd<\/p>\n

j\uff09NIR-II\u7a97\u53e3\u4e2d\u62a5\u544a\u7684PTT\u5242\u7684PCE\u6bd4\u8f83<\/p>\n

Figure <\/strong>3.<\/strong>\u7ec6\u80de\u5b9e\u9a8c<\/strong><\/p>\n

\"\"<\/p>\n

a,b\uff09\u5728\u6709\u6216\u6ca1\u67091064 nm\u6fc0\u5149\u7167\u5c04\u7684\u60c5\u51b5\u4e0b\uff0c\u7528\u4e0d\u540c\u6d53\u5ea6\u7684IR-SS NP\u5b75\u80b2\u540e\uff0cA549\u7ec6\u80de\uff08a\uff09\u548c4T1\u7ec6\u80de\uff08b\uff09\u7684\u7ec6\u80de\u6d3b\u529b<\/p>\n

c\uff09\u5404\u79cd\u5904\u7406\u540eA549\u7ec6\u80de\u7684\u6d3b\/\u6b7b\u56fe\u50cf<\/p>\n

Figure <\/strong>4.<\/strong>\u52a8\u7269\u5b9e\u9a8c<\/strong><\/p>\n

\"\"<\/p>\n

a\uff091064 nm\u8f90\u7167\u4e0b\u4e0d\u540c\u6d53\u5ea6\u7684IR-SS NP\u7684\u6c34\u5206\u6563\u4f53\u7684\u4f53\u5916PA\u56fe\u50cf<\/p>\n

b\uff09PA\u4fe1\u53f7\u4e0e\u7eb3\u7c73\u9897\u7c92\u6d53\u5ea6\u6210\u6bd4\u4f8b\u5173\u7cfb<\/p>\n

c\uff09\u5728\u6ce2\u957f\u4e3a10 mJ\/cm2<\/sup>\u7684\u4e0d\u540c\u6ce2\u957f\u7684\u6fc0\u5149\u7167\u5c04\u4e0b\uff0c\u5145\u6ee1IR-SS NP\u7684\u6bdb\u7ec6\u7ba1\u7684PA\u56fe\u50cf<\/p>\n

d\uff09\uff08c\uff09\u4e2d\u7684PA\u5f3a\u5ea6\u6700\u5927\u503c\u4e0e\u6fc0\u53d1\u6ce2\u957f\u7684\u5173\u7cfb<\/p>\n

e\uff09\u529f\u7387\u653e\u5927\u5668\u4eea\u5668\u7684\u7167\u7247<\/p>\n

f\uff09\u5728808 nm\uff08\u4e0a\u4e00\u884c\uff09\u62161064 nm\u4ee5\u4e0b\u4e0d\u540c\u539a\u5ea6\u4e0b\u53e0\u52a0\u4e00\u5757\u5d4c\u6709IR-TT\u548cIR-SS NPs\u7684\u6bdb\u7ec6\u7ba1\u7684\u9e21\u80f8\u7ec4\u7ec7\u7684\u8d85\u58f0\u56fe\u50cf\uff08\u9ed1\u767d\uff09\u548cPA\u4fe1\u53f7\uff08\u7ea2\u8272\uff09 nm\uff08\u4e0b\u6392\uff09\u6fc0\u53d1\uff0c\u80fd\u91cf\u5bc6\u5ea6\u4e3a10 mJ\/cm2<\/sup><\/p>\n

g\uff09\u6765\u81ea\uff08f\uff09\u7684\u76f8\u5e94PA\u5f3a\u5ea6\u4e0e\u7ec4\u7ec7\u6df1\u5ea6\u7684\u5173\u7cfb<\/p>\n

h\uff09\u5728\u5c3e\u9759\u8109\u6ce8\u5c04IR-SS NP\u540e\u4e0d\u540c\u65f6\u95f4\u7684\u80bf\u7624PA\u56fe\u50cf<\/p>\n

i\uff09\uff08h\uff09\u4e2d\u7684PA\u5f3a\u5ea6\u7ed8\u5236\u4e3a\u6ce8\u5c04\u540e\u65f6\u95f4\u7684\u51fd\u6570<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5<\/strong>\uff1aRational Design of Conjugated Small Molecules for Superior Photothermal Theranostics in the NIR-II Biowindow. Adv. Mater., <\/em>2020<\/strong>, DOI: 10.1002\/adma.202001146<\/p>\n

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