{"id":207567,"date":"2020-08-16T06:43:04","date_gmt":"2020-08-15T22:43:04","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=207567"},"modified":"2020-08-15T20:43:25","modified_gmt":"2020-08-15T12:43:25","slug":"adv-energy-mater-%ef%bc%9a%e5%8a%9f%e7%8e%87%e8%bd%ac%e6%8d%a2%e6%95%88%e7%8e%87%e7%a0%b4%e7%ba%aa%e5%bd%95%ef%bc%81%e9%87%8d%e9%93%b8%e7%ad%96%e7%95%a5%e5%8a%a9%e5%8a%9b%e9%ab%98%e6%80%a7%e8%83%bd","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=207567","title":{"rendered":"Adv. Energy Mater.\uff1a\u529f\u7387\u8f6c\u6362\u6548\u7387\u7834\u7eaa\u5f55\uff01\u91cd\u94f8\u7b56\u7565\u52a9\u529b\u9ad8\u6027\u80fd\u5168\u65e0\u673a\u9499\u949b\u77ff\/\u6709\u673a\u96c6\u6210\u592a\u9633\u80fd\u7535\u6c60"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u5168\u65e0\u673a\u94ef-\u94c5\u6df7\u5408\u5364\u7d20\uff08CsPbX3<\/sub>, X=I, Br\uff09\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\uff08pero-SCs\uff09\u5177\u6709\u4f18\u5f02\u7684\u70ed\u7a33\u5b9a\u6027\u548c\u9ad8\u529f\u7387\u8f6c\u6362\u6548\u7387\uff08PCE\uff09\uff0c\u4f46\u662fI\u542b\u91cf\uff08I\/Br\u6bd4\uff09\u6781\u5927\u7684\u5f71\u54cd\u4e86\u5168\u65e0\u673a\u9499\u949b\u77ff\u7684\u6c34\/\u5149\u7a33\u5b9a\u6027\u548c\u6548\u7387\u3002\u5176\u4e2d\uff0cCsPbIBr2<\/sub>\u5177\u6709\u5e73\u8861\u7684\u5e26\u9699\u548c\u4f18\u5f02\u7a33\u5b9a\u6027\uff0c\u88ab\u8ba4\u4e3a\u662f\u5e94\u7528\u4e8e\u592a\u9633\u80fd\u7535\u6c60\u7684\u6700\u4f73\u9009\u62e9\u3002\u540c\u65f6\uff0cCsPbIBr2<\/sub>\u5177\u67092.1 eV\u7684\u7981\u5e26\u3001\u65e0\u9700\u9ad8\u6e29\u9000\u706b\u7b49\u4f18\u52bf\u3002\u56e0\u6b64\uff0c\u4e9f\u9700\u63a2\u7d22\u57fa\u4e8eCsPbIBr2<\/sub>\u7684\u9ad8\u6027\u80fdpero-SCs\u7684\u7814\u7a76\u9886\u57df\u3002\u4f46\u662f\uff0cpero-SCs\u8f83\u4f4e\u7684\u5f00\u8def\u7535\u538b\uff08V<\/em>oc<\/sub><1.2 V\uff09\u548c\u77ed\u8def\u7535\u6d41\u5bc6\u5ea6\uff08J<\/em>sc<\/sub><11 mA cm-2<\/sup>\uff09\uff0c\u5bfc\u81f4PCE\u8f83\u4f4e\uff08\uff1c9\uff05\uff09\u3002\u6709\u673a\u534a\u5bfc\u4f53\u6750\u6599\uff08OSMs\uff09\u5177\u6709\u53ef\u8c03\u80fd\u7ea7\/\u5e26\u9699\u3001\u4f4e\u56fa\u6709\u7f3a\u9677\u7b49\u4f18\u70b9\uff0c\u56e0\u6b64\uff0c\u5229\u7528OSMs\u6216\u8bb8\u53ef\u4ee5\u63d0\u9ad8\u5168\u65e0\u673aCsPbIBr2\u7684\u8d28\u91cf\u5e76\u6269\u5c55\u5176\u5438\u6536\u5149\u8c31\uff0c\u4ece\u800c\u63d0\u5347\u76f8\u5e94\u5668\u4ef6\u7684\u6548\u7387\u548c\u7a33\u5b9a\u6027\u3002\u6700\u8fd1\uff0c\u6839\u636e\u80fd\u7ea7\u5339\u914d\u548c\u4e92\u8865\u5438\u6536\u7684\u89c4\u5219\uff0c\u63d0\u51fa\u4e86\u5728\u9499\u949b\u77ff\u4e0a\u6c89\u79ef\u4f4e\u5e26\u9699\u6709\u673a\u672c\u4f53-\u5f02\u8d28\u7ed3\uff08BHJ\uff09\u5c42\u6765\u96c6\u6210\u4e24\u4e2a\u5149\u654f\u5c42\u7684\u6982\u5ff5\uff0c\u4ee5\u6269\u5c55pero-SCs\u7684\u5149\u54cd\u5e94\u3002\u4f46\u662f\uff0c\u5927\u591a\u6570\u96c6\u6210\u592a\u9633\u80fd\u7535\u6c60\uff08ISCs\uff09\u5177\u6709\u8f83\u5f31\u7684\u5149\u7535\u6d41\uff0c\u5e76\u4e14\u4f34\u6709\u586b\u5145\u56e0\u5b50\uff08FF\uff09\u4e25\u91cd\u6076\u5316\u3002\u56e0\u6b64\uff0c\u5fc5\u987b\u63a2\u7d22\u5728ISCs\u4e2d\u5b9e\u73b0\u9ad8\u5149\u7535\u6d41\u800c\u53c8\u4e0d\u964d\u4f4e\u5668\u4ef6\u6027\u80fd\u7684\u6709\u6548\u7b56\u7565\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u82cf\u5dde\u5927\u5b66\u7684\u674e\u8000\u6587\u6559\u6388\u3001\u4e2d\u79d1\u9662\u5316\u5b66\u7814\u7a76\u6240\u7684\u6731\u6653\u5f20\u7814\u7a76\u5458\u548c\u56fd\u5bb6\u7eb3\u7c73\u79d1\u5b66\u4e2d\u5fc3\u7684\u5468\u4e8c\u519b\u7814\u7a76\u5458\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u8054\u5408\u62a5\u9053\u4e86\u4e00\u79cd\u91cd\u94f8\u7b56\u7565\uff0c\u4ee5\u4f18\u5316\u4f4e\u5e26\u9699\u6709\u673a\u672c\u4f53-\u5f02\u8d28\u7ed3\uff08BHJ\uff09\u8584\u819c\u7684\u7a7a\u95f4\u5206\u5e03\u7ec4\u4ef6\uff0c\u5e76\u4e0e\u5168\u65e0\u673a\u9499\u949b\u77ff\u76f8\u7ed3\u5408\u4ee5\u6784\u9020\u9499\u949b\u77ff\/BHJ ISCs\u3002\u6839\u636e\u4e92\u8865\u5438\u6536\u548c\u80fd\u7ea7\u5339\u914d\u7684\u89c4\u5219\uff0c\u901a\u8fc7\u5c06\u91cd\u94f8\u6709\u673aBHJ\u4e0eCsPbIBr2<\/sub>\u7ed3\u5408\u8d77\u6765\uff0c\u6210\u529f\u5b9e\u73b0\u4e86\u9ad8\u6027\u80fdISCs\u3002\u5176\u4e2d\uff0cCsPbIBr2<\/sub>\u5177\u6709\u51fa\u8272\u7684\u70ed\u7a33\u5b9a\u6027\uff0c\u53ef\u4ee5\u9632\u6b62\u9499\u949b\u77ff\u5728BHJ\u8584\u819c\u6c89\u79ef\u8fc7\u7a0b\u4e2d\u964d\u89e3\u3002\u91cd\u94f8\u7684BHJ\u8584\u819c\u4e0d\u4ec5\u53ef\u4ee5\u5b9e\u73b0\u9876\u90e8\u5bcc\u96c6\u4f9b\u4f53\u7ec4\u5206\uff0c\u800c\u4e14\u53ef\u4ee5\u5fae\u8c03\u7ec4\u5206\u7684\u5206\u5b50\u65b9\u5411\u3002\u5177\u6709\u91cd\u94f8BHJ\u8584\u819c\u7684ISCs\u53ef\u4ee5\u6709\u6548\u6291\u5236\u754c\u9762\u7535\u8377\u8f7d\u6d41\u5b50\u590d\u5408\uff0c\u589e\u5f3a\u9499\u949b\u77ff\u4e0eBHJ\u8584\u819c\u4e4b\u95f4\u7684\u53cc\u6781\u6027\u7535\u8377\u4f20\u8f93\u884c\u4e3a\u3002\u5b9e\u9a8c\u7ed3\u679c\u53d1\u73b0\uff0c\u9ad8\u5149\u54cd\u5e94\u4ece600 nm\u6269\u5c55\u5230730 nm\uff0c\u6700\u5927\u5916\u90e8\u91cf\u5b50\u6548\u7387\uff08EQE\uff09\u503c\u4e3a40\uff05\uff0c\u540c\u4e8b\u5728\u4e0d\u727a\u7272\u5176\u5b83\u5149\u4f0f\u6027\u80fd\u4e0b\u53c8\u8d21\u732e\u4e8620\uff05\u7684J<\/em>sc<\/sub>\u3002\u603b\u4e4b\uff0c\u57fa\u4e8eCsPbIBr2<\/sub>\u7684pero-SCs\u7684PCE\u8fbe\u5230\u4e86\u521b\u7eaa\u5f55\u768411.08\uff05\uff0c\u5e76\u5177\u6709\u4f18\u5f02\u7684\u957f\u671f\u70ed\uff0885 o<\/sup>C\uff09\u7a33\u5b9a\u6027\u548c\u7d2b\u5916\u5149\uff08100 mW cm-2<\/sup>\uff09\u7a33\u5b9a\u6027\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cSpatial Distribution Recast for Organic Bulk Heterojunctions for High-Performance All-Inorganic Perovskite\/Organic Integrated Solar Cells\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aAdv. Energy Mater.<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001BHJ\u8584\u819c\u7684\u5e94\u7528\u548c\u6027\u80fd<\/strong>
\n \"\"\uff08a\uff09\u5de6\uff1a\u5168\u65e0\u673a\u9499\u949b\u77ff\/\u6709\u673aBHJ ISC\u7684\u88c5\u7f6e\u7ed3\u6784\uff1b\u53f3\uff1aCsPbIBr2<\/sub>\u7684\u6676\u4f53\u7ed3\u6784\u548cOSMs\u7684\u5206\u5b50\u7ed3\u6784\uff1b<\/p>\n

\uff08b\uff09CsPbIBr2<\/sub>\u3001BHJ-1\u548cBHJ-2\u8584\u819c\u7684\u5f52\u4e00\u5316\u5438\u6536\u5149\u8c31\u548cAM 1.5G\u5149\u8c31\uff1b<\/p>\n

\uff08c-d\uff09\u5728AM 1.5G 100 mW cm-2<\/sup>\u7167\u660e\u4e0b\uff0c\u5177\u6709\u4e0d\u540cOSMs\u4f5c\u4e3aHTL\u7684\u8bbe\u5907\u7684J<\/em>–V<\/em>\u66f2\u7ebf\u548cEQE\u5149\u8c31\uff1b<\/p>\n

\uff08e\uff09\u4e0e\u4e0d\u540cBHJ\u8584\u819c\u96c6\u6210\u7684CsPbIBr2<\/sub>\u7684\u80fd\u7ea7\u56fe\u3002<\/p>\n

\u56fe\u4e8c\u3001\u4e0d\u540c\u5668\u4ef6\u914d\u7f6e\u6d4b\u91cfISCs\u7684J<\/em>–V<\/em>\u66f2\u7ebf<\/strong>
\n \"\"\uff08a\uff09ITO\/Cl-TiO2<\/sub>\/CsPbIBr2<\/sub>\/PBDB-T\/MoO3<\/sub>\/Al\uff1b<\/p>\n

\uff08b\uff09ITO\/Cl-TiO2<\/sub>\/CsPbIBr2<\/sub>\/PBDB-T\/BT2b\/MoO3<\/sub>\/Al\uff1b<\/p>\n

\uff08c\uff09\u76f8\u5e94\u7684EQE\u5149\u8c31\u3002<\/p>\n

\u56fe\u4e09\u3001\u4e0d\u540c\u7ec4\u6210\u8584\u819c\u7684\u6027\u80fd<\/strong>
\n \"\"\uff08a\uff09PBDB-T\u548cBT2b\u5728MeOH\/THF\u6df7\u5408\u6eb6\u5242\u4e2d\u7684\u6eb6\u89e3\u5ea6\uff1b<\/p>\n

\uff08b\uff09CsPbIBr2<\/sub>\u3001CsPbIBr2<\/sub>\/BHJ-2\u548cCsPbIBr2<\/sub>\/BHJ-2-RC\u8584\u819c\u7684\u5438\u6536\u5149\u8c31\uff1b<\/p>\n

\uff08c\uff09\u88f8PBDB-T\u3001\u88f8BT2b\u548cBHJ-2-RC\u8584\u819c\u7684\u8868\u9762\u7535\u52bf\uff08SP\uff09\uff1b<\/p>\n

\uff08d\uff09\u5bf9BHJ-2\u548cBHJ-2-RC\u8584\u819c\u7684N\u5143\u7d20\u8fdb\u884cEDS\u6620\u5c04\uff1b<\/p>\n

\uff08e\uff09\u6d82\u6709BHJ-2\u6216BHJ-2-RC\u7684CsPbIBr2<\/sub>\u9499\u949b\u77ff\u819c\u7684XRD\u56fe\u8c31\u3002<\/p>\n

\u56fe\u56db\u3001BHJ-2\u548cBHJ-2-RC\u8584\u819c\u7684\u8868\u5f81<\/strong>
\n \"\"\uff08a\uff09CsPbIBr2<\/sub>\/BHJ-2\u548cCsPbIBr2<\/sub>\/BHJ-2-RC\u8584\u819c\u7684AFM\u9ad8\u5ea6\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09BHJ-2\u548cBHJ-2-RC\u8584\u819c\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09\u7528\u4e8eBHJ-2\u548cBHJ-2-RC\u8584\u819c\u76842D GIWAXS\u6a21\u5f0f\uff1b<\/p>\n

\uff08d\uff09BHJ-2\u548cBHJ-2-RC\u8584\u819c\u7684\u9762\u5916\u548c\u9762\u5185GIWAXS\u8f6e\u5ed3\uff1b<\/p>\n

\uff08e\uff09BHJ-2\u548cBHJ-2-RC\u8584\u819c\uff08100\uff09\u5c42\u72b6\u884d\u5c04\u7684\u7535\u6781\u56fe\u3002<\/p>\n

\u56fe\u4e94\u3001\u4e0d\u540c\u8584\u819c\u7684\u7a33\u6001PL\u5149\u8c31\u548cXPS\u5149\u8c31<\/strong>
\n \"\"\uff08a-b\uff09\u5728\u73bb\u7483\u57fa\u5e95\u4e0a\u5236\u4f5c\u4e0d\u540c\u8584\u819c\u7684\u7a33\u6001PL\u5149\u8c31\u548cTRPL\u56fe\uff1b<\/p>\n

\uff08c-d\uff09CsPbIBr2<\/sub>\u3001CsPbIBr2<\/sub>\/BHJ-2\u548cCsPbIBr2\/BHJ-2-RC\u8584\u819c\u7684Cs 3d\u548cPb 4f\u7684XPS\u5149\u8c31\u3002<\/p>\n

\u56fe\u516d\u3001BHJ-2\u8584\u819c\u91cd\u94f8\u8fc7\u7a0b\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u4e03\u3001BHJ-2-RC\u57faISCs\u7684\u6027\u80fd\u6d4b\u8bd5<\/strong>
\n \"\"\uff08a\uff09BHJ-2-RC\u57faISCs\u7684\u622a\u9762SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09\u5728AM 1.5G\u3001100 mW\/cm2<\/sup>\u5149\u7167\u4e0b\uff0cBHJ-2-RC\u57faISCs\u7684J<\/em>–V<\/em>\u66f2\u7ebf\uff1b<\/p>\n

\uff08c\uff09\u57281 V\u7684V<\/em>bias<\/sub>\u4e0b\uff0c\u6d4b\u91cfBHJ-2-RC\u57faISCs\u7684\u7a33\u6001PCE\uff1b<\/p>\n

\uff08d\uff09BHJ-2-RC\u57faISCs\u7684EQE\u9891\u8c31\uff1b<\/p>\n

\uff08e\uff09BHJ-2-\u548cBHJ-2-RC\u57faISCs\u7684\u5149\u7535\u573a\u5206\u5e03\uff1b<\/p>\n

\uff08f\uff09\u6700\u8fd1\u62a5\u9053\u768420\u79cd\u5168\u65e0\u673aCsPbIBr2<\/sub>\u57fapero-SCs\u6216ISCs\u7684J<\/em>sc<\/sub>\u548cPCE\u7684\u7edf\u8ba1\u56fe\uff1b<\/p>\n

\uff08g\uff09\u5728\u70ed\u9000\u706b\u6e29\u5ea6\u4e3a85\u2103\u3001N2<\/sub>\u6c14\u6c1b\u4e0b\uff0c\u4e0d\u540c\u8584\u819c\u7684\u5f52\u4e00\u5316PCE\uff1b<\/p>\n

\uff08h\uff09\u5728100 mW\/cm2<\/sup>\u7d2b\u5916\u7ebf\u7167\u5c04\u3001N2<\/sub>\u6c14\u6c1b\u4e0b\uff0c\u4e0d\u540c\u8584\u819c\u7684\u5f52\u4e00\u5316PCE\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u62a5\u9053\u4e86\u4e00\u79cd\u6709\u673aBHJ\u8584\u819c\u7684\u91cd\u94f8\u7b56\u7565\uff0c\u5e76\u6210\u529f\u5730\u5236\u5907\u4e86\u5168\u65e0\u673a\u9499\u949b\u77ff\/\u6709\u673aBHJ ISCs\u3002\u57fa\u4e8eCsPbIBr2<\/sub>\/BHJ-2-RC\u8584\u819c\u7684ISCs\u5177\u6709\u6700\u4e30\u5bcc\u7684PBDB-T\u7a7a\u95f4\u5206\u5e03\uff0c\u53ef\u4ee5\u663e\u7740\u6291\u5236\u754c\u9762\u7535\u8377\u8f7d\u6d41\u5b50\u7684\u590d\u5408\uff0c\u5e76\u6539\u5584\u96c6\u6210\u7684\u4e24\u4e2a\u5149\u654f\u5c42\u4e2d\u7684\u53cc\u6781\u6027\u7535\u8377\u4f20\u8f93\u884c\u4e3a\u3002\u5177\u6709CsPbIBr2<\/sub>\/BHJ-2-RC\u8584\u819c\u7684ISCs\u7684\u5149\u54cd\u5e94\u4ece600 nm\u6269\u5c55\u5230730 nm\uff0c\u4ece\u800c\u8d21\u732e20\uff05\u7684J<\/em>sc<\/sub>\u3002\u540c\u65f6\uff0cV<\/em>oc<\/sub>\u4e3a1.22 V\u3001FF\u4e3a72.66\uff05\u3001PCE\u4e3a11.08\uff05\u3002\u5176\u4e2d\uff0cPCE\u662f\u5df2\u62a5\u9053\u7684CsPbIBr2<\/sub>\u57fapero-SCs\u4e2d\u6700\u9ad8\u7684\u3002\u6b64\u5916\uff0c\u5229\u7528\u91cd\u94f8\u7b56\u7565\u7684ISCs\u5728\u9ad8\u6e29\u548c\u5f3a\u7d2b\u5916\u7ebf\u7167\u5c04\u4e0b\u4e5f\u5177\u6709\u5f88\u597d\u7684\u957f\u671f\u7a33\u5b9a\u6027\u3002\u603b\u4e4b\uff0c\u8be5\u65b9\u6cd5\u4e3a\u5236\u5907\u9ad8\u6027\u80fdISCs\u5f00\u8f9f\u4e86\u4e00\u6761\u65b0\u9014\u5f84\uff0c\u5e76\u4e14\u5fc5\u5c06\u52a0\u901fISCs\u5728\u5b9e\u9645\u5e94\u7528\u4e2d\u7684\u5f00\u53d1\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aSpatial Distribution Recast for Organic Bulk Heterojunctions for High-Performance All-Inorganic Perovskite\/Organic Integrated Solar Cells<\/strong>\uff08Adv. Energy Mater.<\/em>, 2020<\/strong>, DOI: 10.1002\/aenm.202000851\uff09<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

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