{"id":209027,"date":"2020-09-08T12:00:05","date_gmt":"2020-09-08T04:00:05","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=209027"},"modified":"2020-09-08T11:05:17","modified_gmt":"2020-09-08T03:05:17","slug":"%e5%b7%b2%e6%a0%a1%e7%a8%bf%e4%bb%b6-nano-energy%ef%bc%9a%e9%93%9c%e6%8e%ba%e6%9d%82%e9%92%99%e9%92%9b%e7%9f%bf%e7%ba%b3%e7%b1%b3%e5%a4%8d%e5%90%88%e6%9d%90%e6%96%99%e5%ae%9e%e7%8e%b0%e9%ab%98","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=209027","title":{"rendered":"Nano Energy\uff1a\u94dc\u63ba\u6742\u9499\u949b\u77ff\u7eb3\u7c73\u590d\u5408\u6750\u6599\u5b9e\u73b0\u9ad8\u6548\u8fd8\u539f\u542b\u6c27\u6c14\u7684\u4e8c\u6c27\u5316\u78b3"},"content":{"rendered":"

\u3010\u6587\u7ae0\u4eae\u70b9\u3011<\/strong><\/p>\n

1\u3001\u62a5\u9053\u4e86\u4e00\u79cd\u57fa\u4e8eCO2<\/sub>\/O2<\/sub>\u6df7\u5408\u7269\u5230\u7eafCO\u7684\u9ad8\u6548\u6c27\u5316\u8fd8\u539f\u7b56\u7565\uff0c\u7528\u4e8e\u751f\u4ea7\u9ad8\u4ef7\u503c\u5316\u5b66\u54c1\u3002<\/p>\n

2\u3001\u5728CO2<\/sub>\u53cd\u5e94\u5668\u4e2d\u4ee5\u6c27\u8f7d\u4f53\u9ad8\u6d3b\u6027\u548c\u9ad8\u7a33\u5b9a\u6027\u5b9e\u73b0\u4e86\u9ad8\u7684CO\u6536\u7387\u3002<\/p>\n

3\u3001\u8be5\u5de5\u4f5c\u901a\u8fc7\u5229\u7528\u78b3\u6355\u83b7\u8fc7\u7a0b\u4e2d\u4ea7\u751f\u7684\u4f4e\u6210\u672cCO2<\/sub>\/O2<\/sub>\u6df7\u5408\u7269\u4e3a\u539f\u6599\uff0c\u4e3aCO2<\/sub>\u5316\u5b66\u5de5\u4e1a\u5f00\u8f9f\u4e86\u65b0\u65b9\u5411\u3002<\/p>\n

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u5c06\u4e8c\u6c27\u5316\u78b3\uff08CO2<\/sub>\uff09\u8fd8\u539f\u4e3a\u4e00\u6c27\u5316\u78b3\uff08CO\uff09\u7528\u4f5c\u6c14\u6001\u71c3\u6599\u6216\u751f\u4ea7\u9ad8\u4ef7\u503c\u5316\u5b66\u54c1\u7684\u4e2d\u95f4\u4f53\uff0c\u6709\u5229\u4e8e\u5b9e\u73b0\u78b3\u5faa\u73af\u548c\u5316\u5de5\u5e94\u7528\u3002\u5176\u4e2d\uff0c\u5229\u7528\u592a\u9633\u80fd\u5149\u50ac\u5316\u53ef\u5c06CO2<\/sub>\u8fd8\u539f\u4e3aCO\uff0c\u4f46\u662f\u5176\u50ac\u5316\u6548\u7387\u4f4e\u4e8e0.2\uff05\u3002\u867d\u7136\u7535\u50ac\u5316\u8fd8\u539f\u662f\u7528\u4e8eCO2<\/sub>\u5faa\u73af\u7684\u6709\u6548\u6280\u672f\uff0c\u4f46\u662f\u5176\u6d3b\u6027\u548cCO2<\/sub>\u8fd8\u539f\u7684\u9009\u62e9\u6027\u53d7\u5230\u6c14\u6001\u6742\u8d28\uff08\u5982O2<\/sub>\u7b49\uff09\u7684\u5e72\u6270\u4e25\u91cd\uff0c\u65e0\u6cd5\u5e94\u7528\u4e8e\u542b\u5927\u91cfO2<\/sub>\u7684CO2<\/sub>\u6c14\u4f53\u8f6c\u5316\u3002\u800c\u5728\u57fa\u4e8e\u7a7a\u6c14\u6216\u5de5\u4e1a\u70df\u6c14\u7684CO2<\/sub>\u5206\u79bb\u6355\u96c6\u8fc7\u7a0b\u4e2d\uff0cCO2<\/sub>\u63d0\u7eaf\u6210\u672c\u968f\u7740CO2<\/sub>\u7684\u6d53\u5ea6\u663e\u8457\u589e\u52a0\u3002\u56e0\u6b64\uff0c\u6709O2<\/sub>\u6761\u4ef6\u4e0b\uff0c\u5f00\u53d1\u9ad8\u9009\u62e9\u6027\u548c\u8f6c\u5316\u7387\u7684CO2<\/sub>\u8fd8\u539f\u6280\u672f\u81f3\u5173\u91cd\u8981\u3002\u5316\u5b66\u94fe\u6280\u672f\u901a\u8fc7\u4e24\u6b65\u53cd\u5e94\u53ef\u5c06CO2<\/sub>\u4e0eCH4<\/sub>\u5206\u522b\u8f6c\u5316\u4e3a\u7eafCO\u548c\u5408\u6210\u6c14\uff0c\u5229\u4e8e\u4e0b\u6e38\u7684\u5316\u5de5\u54c1\u6216\u71c3\u6599\u751f\u4ea7\u3002\u5229\u7528\u542bO2<\/sub>\u7684CO2<\/sub>\u6df7\u5408\u6c14\u4f5c\u4e3a\u539f\u6599\uff0c\u53ef\u4ee5\u5927\u5927\u964d\u4f4eCO2<\/sub>\u6355\u96c6\u7684\u6210\u672c\uff0c\u8fdb\u800c\u4f7f\u6574\u4f53CO2<\/sub>\u8f6c\u5316\u7cfb\u7edf\u66f4\u5177\u7ade\u4e89\u4f18\u52bf\uff0c\u4f46\u662f\u7531\u4e8eO2<\/sub>\u7684\u6c27\u5316\u6d3b\u6027\u8fdc\u9ad8\u4e8eCO2<\/sub>\uff0c\u9700\u8bbe\u8ba1\u65b0\u578b\u6c27\u8f7d\u4f53\u5e73\u8861CO2<\/sub>\u4e0eO2<\/sub>\u7684\u7ade\u4e89\u53cd\u5e94\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6606\u660e\u7406\u5de5\u5927\u5b66\u674e\u5b54\u658b\u535a\u58eb\u3001\u7f8e\u56fd\u54e5\u4f26\u6bd4\u4e9a\u5927\u5b66\u9648\u66e6\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u5229\u7528\u9499\u949b\u77ff\u590d\u5408\u6750\u6599\u5c06\u542bO2<\/sub>\u7684CO2<\/sub>\u8fd8\u539f\u4e3aCO\u7684\u7b56\u7565\u3002\u8be5\u7b56\u7565\u662f\u901a\u8fc7\u4ee5Cu\uff085 at\uff05\uff09\u63ba\u6742\u7684LaFeO3<\/sub>\u9499\u949b\u77ff\u4f5c\u4e3a\u6709\u6548\u6c27\u8f7d\u4f53\u6765\u5b9e\u65bd\u5316\u5b66\u94fe\u5faa\u73af\u3002\u5728O2<\/sub>\u5b58\u5728\u7684\u60c5\u51b5\u4e0b\u7684CO2<\/sub>-CH4<\/sub>\u5316\u5b66\u94fe\u91cd\u6574\u5faa\u73af\u4e2d\uff0c\u8be5\u9499\u949b\u77ff\u590d\u5408\u6750\u6599\u53ef\u5b9e\u73b0\u6700\u9ad8\u53ef\u8fbe2.28 mol\/kg\u7684CO\u6536\u7387\uff0c\u800c\u539f\u59cb\u7684LaFeO3<\/sub>\u9499\u949b\u77ff\u4ec5\u8868\u73b0\u51fa\u6709\u6548\u7684\u7eafCO2<\/sub>\u8fd8\u539f\u80fd\u529b\u3002\u6b64\u5916\uff0c\u901a\u8fc7Cu\u6539\u6027\u540e\uff0c\u5408\u6210\u6c14\u751f\u4ea7\u7387\u63d0\u9ad8\u4e86\u4e00\u500d\u3002\u901a\u8fc7\u5b9e\u9a8c\u8868\u5f81\u548cDFT\u8ba1\u7b97\uff0c\u4f5c\u8005\u53d1\u73b0\u4e86\u5728\u8fd8\u539f\u578b\u9499\u949b\u77ff\u8868\u9762\u4e0a\u6790\u51fa\u7684\u91d1\u5c5eCu\u80fd\u591f\u51cf\u7f13CO2<\/sub>\u4e0eO2<\/sub>\u4e4b\u95f4\u5728\u6c27\u5316\u6b65\u9aa4\u4e2d\u7684\u7ade\u4e89\u53cd\u5e94\u3002\u57fa\u4e8e\u6b64\uff0c\u4f5c\u8005\u63d0\u51fa\u4e86\u57fa\u4e8e\u5316\u5b66\u94fe\u6280\u672f\uff0c\u5b9e\u73b0\u65e0\u9700\u9ad8\u5ea6\u63d0\u7eafCO2<\/sub>\u7684\u78b3\u5229\u7528\u7cfb\u7edf\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cHighly efficient reduction of O2<\/sub>-containing CO2<\/sub> via chemical looping based on perovskite nanocomposites\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNano Energy\u4e0a<\/strong>\u3002<\/p>\n

\u8bba\u6587\u4f5c\u8005\u8fd8\u5305\u62ec\u5317\u5361\u7f57\u62c9\u7eb3\u5dde\u7acb\u5927\u5b66\u674e\u51e1\u661f\u6559\u6388\u548c\u4e2d\u79d1\u9662\u5e7f\u5dde\u80fd\u6e90\u6240\u9ec4\u632f\u526f\u7814\u7a76\u5458\u7b49<\/strong>\u3002<\/p>\n

\"\"<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u8bbe\u8ba1\u7528\u4e8e\u8fd8\u539fO2<\/sub>\/CO2<\/sub>\u6df7\u5408\u7269\u7684\u6c27\u5316\u8fd8\u539f\u6750\u6599<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u4e8c\u3001Cu\u63ba\u6742\u7684LaFeO3<\/sub>\u7684\u7ed3\u6784\u8868\u5f81\u548c\u6027\u80fd<\/strong>
\n \"\"\uff08a-f\uff09La0.95<\/sub>Cu0.05<\/sub>FeO3-\u03b4<\/sub>\u6837\u54c1\u7684STEM\u56fe\u3001HRTEM\u56fe\u3001\u76f8\u5e94\u7684\u5feb\u901f\u5085\u7acb\u53f6\u53d8\u6362\u56fe\u548cEDS\u56fe\uff1b<\/p>\n

\uff08g\uff09\u9499\u949b\u77ff\u7ed3\u6784LaFeO3<\/sub>\u548cLa0.95<\/sub>Cu0.05<\/sub>FeO3-\u03b4<\/sub>\u7684XRD\u56fe\u8c31\u548cRietveld\u7cbe\u4fee\u7ed3\u679c\uff1b<\/p>\n

\uff08h-i\uff09CO2<\/sub>\u8fd8\u539f\u8fc7\u7a0b\u4e2dLaFeO3<\/sub>\u548cLa0.95<\/sub>Cu0.05<\/sub>FeO3-\u03b4<\/sub>\u5bf9\u5e94\u7684CO\u548cCO2<\/sub>\u77ac\u65f6\u6469\u5c14\u6d53\u5ea6\uff0c\u7528\u4e8e\u5206\u79bb\u7eafCO2<\/sub>\u548c\u542bO2<\/sub>\u7684CO2<\/sub>\uff1b<\/p>\n

\uff08j-k\uff09\u4e0d\u540cCu\u542b\u91cf\u7684LaFeO3<\/sub>\u9499\u949b\u77ff\u5728CO2<\/sub>\u5206\u89e3\u6b65\u9aa4\u4e2dCO2<\/sub>\u8f6c\u5316\u7387\u548cCO\u4ea7\u7387\uff0c\u4ee5\u53ca\u7532\u70f7\u90e8\u5206\u6c27\u5316\u6b65\u9aa4\u4e2d\u7684\u7532\u70f7\u8f6c\u5316\u7387\u548c\u5408\u6210\u6c14\u4ea7\u7387\u3002<\/p>\n

\u56fe\u4e09\u3001La0.95<\/sub>Cu0.05<\/sub>FeO3-\u03b4<\/sub>\u7684\u6c27\u5316\u8fd8\u539f\u7279\u5f81\u4e0e\u673a\u7406<\/strong>
\n \"\"\uff08a\uff09\u7532\u70f7\u8fd8\u539f7 min\u621614 min\u7684\u6837\u54c1\uff0c\u5e76\u901a\u8fc7\u542bO2<\/sub>\u7684CO2<\/sub>\u5206\u89e3\u6b65\u9aa4\u5c06\u8fd8\u539f\u6837\u54c1\u91cd\u65b0\u6c27\u5316\u540e\u7684XRD\u56fe\u8c31\uff1b<\/p>\n

\uff08b\uff09X\u5c04\u7ebf\u884d\u5c04\u56fe\u7684\u653e\u5927\u533a\u57df\uff0c\u4ee5\u8bf4\u660e\u91d1\u5c5eCu\u7684\u5b58\u5728\uff1b<\/p>\n

\uff08c-d\uff09\u901a\u8fc7\u4e0d\u540c\u6c14\u4f53\u8fd8\u539f\/\u6c27\u5316\u7684La0.95<\/sub>Cu0.05<\/sub>FeO3<\/sub>\u6837\u54c1\u4e0a\u7684Cu 2p XPS\u56fe\u8c31\u548c\u8868\u9762\u5143\u7d20\u7684\u6d53\u5ea6\uff1b<\/p>\n

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\u56fe\u56db\u3001DFT\u8ba1\u7b97\u7ed3\u679c<\/strong>
\n \"\"\uff08a\uff09\u6709\u3001\u65e0Cu\u539f\u5b50\u7684\u8fd8\u539fLaFeO3<\/sub>(110)\u8868\u9762\u4e0aCO2<\/sub>\u548cO2<\/sub>\u7684\u5438\u9644\u80fd\u5bf9\u6bd4\u56fe\uff1b<\/p>\n

\uff08b\uff09\u6709\u3001\u65e0Cu\u539f\u5b50\u7684\u60c5\u51b5\u4e0b\uff0c\u8fd8\u539f\u7684LaFeO3<\/sub>(110)\u8868\u9762\u4e0a\u7684O2<\/sub>\u5206\u89e3\u548cCO2<\/sub>\u5206\u89e3\u6210\u6c27\u539f\u5b50\u548c\u4e00\u6c27\u5316\u78b3\u5206\u5b50\u7684\u53cd\u5e94\u8def\u5f84\u3002<\/p>\n

\u56fe\u4e94\u3001\u6c27\u5316\u8fd8\u539f\u7a33\u5b9a\u6027<\/strong>
\n \"\"\uff08a\uff09\u542bO2<\/sub>\u7684CO2<\/sub>\u4e0e\u7532\u70f7\u8fde\u7eed\u5316\u5b66\u94fe\u5faa\u73af\u4e2dCO2<\/sub>\u8f6c\u5316\u7387\u548cCO\u4ea7\u7387\u53d8\u5316\u56fe\uff1b<\/p>\n

\uff08b\uff0950\u6b21\u5316\u5b66\u94fe\u5faa\u73af\u4e2d\u7532\u70f7\u8f6c\u5316\u7387\u3001\u5408\u6210\u6c14\u4ea7\u7387\u548cH2<\/sub>\/CO\u6469\u5c14\u6bd4\u53d8\u5316\u56fe\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u63d0\u51fa\u4e86\u4e00\u79cd\u65b0\u578b\u7684Cu\u63ba\u6742\u9499\u949b\u77ff\u4f5c\u4e3a\u6c27\u8f7d\u4f53\uff0c\u53ef\u901a\u8fc7\u5316\u5b66\u94fe\u6982\u5ff5\u5c06\u542bO2<\/sub>\u7684CO2<\/sub>\u6709\u6548\u5730\u8fd8\u539f\u4e3aCO\u3002\u5c06CO2<\/sub>\/O2<\/sub>\u7684\u6df7\u5408\u7269\uff08\u6469\u5c14\u6bd4\u4e3a5\uff1a1\uff09\u8fdb\u884c\u8f6c\u5316\uff0c\u53ef\u4ee5\u83b7\u5f97\u8f83\u9ad8\u7684CO\u4ea7\u7387\uff082.28 mol\/kg\uff09\uff0c\u901a\u8fc7\u5b9e\u884c\u6781\u9ad8\u7684\u5408\u6210\u6c14\u751f\u4ea7\u7387\uff0811.0 mol\/kg\uff09\uff0c\u4f7f\u5f97Cu\u63ba\u6742\u7684\u9499\u949b\u77ff\u5341\u5206\u5177\u6709\u5438\u5f15\u529b\u3002\u901a\u8fc7\u5b9e\u9a8c\u548c\u7406\u8bba\u7814\u7a76\uff0c\u9610\u660e\u4e86\u5728\u6c27\u5316\u8fd8\u539f\u8fc7\u7a0b\u4e2d\u9499\u949b\u77ff\u8868\u9762\u91d1\u5c5eCu\u7684\u6790\u51fa\u548c\u81ea\u518d\u751f\uff0cCu\u7684\u7279\u6b8a\u4f5c\u7528\u4f7f\u8be5\u6c27\u8f7d\u4f53\u5373\u4fbf\u5728\u5b58\u5728O2<\/sub>\u7684\u60c5\u51b5\u4e0b\uff0c\u4e5f\u80fd\u8fdb\u884c\u9ad8\u6548\u7684CO2<\/sub>\u8fd8\u539f\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aHighly efficient reduction of O2<\/sub>-containing CO2<\/sub> via chemical looping based on perovskite nanocomposites<\/a><\/strong> \uff08Nano Energy<\/em>, 2020<\/strong>, DOI: 10.1016\/j.nanoen.2020.105320\uff09<\/p>\n

\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb<\/strong><\/p>\n

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