{"id":210140,"date":"2020-09-28T12:00:41","date_gmt":"2020-09-28T04:00:41","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=210140"},"modified":"2020-09-28T10:10:30","modified_gmt":"2020-09-28T02:10:30","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e5%b8%ad%e8%81%98%e8%b4%a4%e9%bb%84%e5%8b%83%e9%be%99jacs%ef%bc%9a%e9%93%b1%e5%8d%95%e5%8e%9f%e5%ad%90%e4%b8%8e%e6%b0%a7%e7%a9%ba%e4%bd%8d%e8%80%a6","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=210140","title":{"rendered":"\u5e2d\u8058\u8d24&\u9ec4\u52c3\u9f99JACS\uff1a\u94f1\u5355\u539f\u5b50\u4e0e\u6c27\u7a7a\u4f4d\u8026\u5408\u4fc3\u8fdb\u9178\u6027\u4ecb\u8d28\u4e2d\u7684\u6790\u6c27\u53cd\u5e94"},"content":{"rendered":"

\u3010\u7814\u7a76\u80cc\u666f\u3011<\/strong><\/p>\n

\u6790\u6c27\u53cd\u5e94\uff08OER\uff09\u5728\u53ef\u6301\u7eed\u53d1\u5c55\u548c\u80fd\u91cf\u8f6c\u6362\u88c5\u7f6e\u4e2d\u5177\u6709\u91cd\u8981\u4f5c\u7528\u3002\u9057\u61be\u7684\u662f\uff0c\u7531\u4e8e\u56db\u7535\u5b50\/\u56db\u8d28\u5b50\u8dc3\u8fc1\uff0cOER\u52a8\u529b\u5b66\u8f83\u6162\u3002\u56e0\u6b64\uff0c\u8bbe\u8ba1\u7ecf\u6d4e\u3001\u7a33\u5b9a\u7684\u9178\u6027OER\u7535\u50ac\u5316\u5242\u6210\u4e3a\u4eca\u540e\u7814\u7a76\u7684\u91cd\u70b9\u3002\u8fd1\u5e74\u6765\uff0c\u5355\u539f\u5b50\u50ac\u5316\u5242\uff08SACs\uff09\u5728\u8bb8\u591a\u53cd\u5e94\u4e2d\u8868\u73b0\u51fa\u60ca\u4eba\u7684\u7535\u50ac\u5316\u6027\u80fd\uff0c\u5c24\u5176\u662f\u5bf9\u6c27\u8fd8\u539f\u53cd\u5e94\uff08ORR\uff09\u548cCO2<\/sub>\u8fd8\u539f\u53cd\u5e94\uff08CO2<\/sub>RR\uff09\u8868\u73b0\u51fa\u4e86\u60ca\u4eba\u7684\u7535\u50ac\u5316\u6027\u80fd\u3002\u7136\u800c\uff0cSACs\u7684\u5236\u5907\u4ecd\u662f\u4e00\u5927\u96be\u9898\uff0c\u56e0\u6b64\u8bbe\u8ba1\u7b80\u5355\u6613\u884c\u7684SACs\u5236\u5907\u65b9\u6cd5\u662f\u91cd\u4e2d\u4e4b\u91cd\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

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\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001<\/strong>NiCo2<\/sub>O4<\/strong>\u548c<\/strong>Ir\u2212NiCo2<\/sub>O4 NSs<\/strong>\u7684\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09NiCo2<\/sub>O4<\/sub>\u548cIr\u2212NiCo2<\/sub>O4<\/sub> NSs\u7684XRD\u8868\u5f81\u3002<\/p>\n

\uff08b-c\uff09NiCo2<\/sub>O4<\/sub> NSs\u7684SEM\uff0cTEM\u548cHRTEM\u8868\u5f81\u3002<\/p>\n

\uff08d-f\uff09Ir-NiCo2<\/sub>O4<\/sub> NSs\u7684SEM\uff0cTEM\u548cHRTEM\u8868\u5f81\u3002<\/p>\n

\uff08g\uff09NiCo2<\/sub>O4<\/sub>\u548cIr-NiCo2<\/sub>O4<\/sub> NSs\u7684O 1s\u5149\u8c31\u3002<\/p>\n

\uff08h\uff09IrO2<\/sub>\u548cIr-NiCo2<\/sub>O4<\/sub> NSs\u7684Ir 4f\u5149\u8c31\u3002<\/p>\n

\uff08i\uff09NiCo2<\/sub>O4<\/sub>\u548cIr-NiCo2<\/sub>O4<\/sub> NSs\u7684O-K\u8fb9XANES\u8868\u5f81\u3002<\/p>\n

\u56fe\u4e8c\u3001<\/strong>Ir-NiCo2<\/sub>O4<\/sub> NSs<\/strong>\u7684\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09Ir-NiCo2<\/sub>O4<\/sub> NSs\u7684\u7ed3\u6784\u793a\u610f\u56fe\u3002<\/p>\n

\uff08b\uff09Ir-NiCo2<\/sub>O4<\/sub> NSs\u7684HAADF-STEM\u56fe\u50cf\u3002<\/p>\n

\uff08c\uff09\u6807\u6ce8\u6709Ir\u2212SAs\u7684Ir-NiCo2<\/sub>O4<\/sub> NSs\u7684HAADF-STEM\u56fe\u50cf\u3002<\/p>\n

\uff08d\uff09IrO2<\/sub>\u548cIr-NiCo2<\/sub>O4<\/sub> NSs\u7684XANES\u8868\u5f81\u3002<\/p>\n

\uff08e\uff09IrO2<\/sub>\u548cIr-NiCo2<\/sub>O4<\/sub> NSs\u7684EXAFS\u8868\u5f81\u3002<\/p>\n

\uff08f\uff09\u5bf9Ir-NiCo2<\/sub>O4<\/sub> NSs\u548c\u5546\u7528IrO2<\/sub>\u7684k3\u52a0\u6743Ir L3\u2212edge EXAFS\u4fe1\u53f7\u8fdb\u884c\u4e86\u76f8\u5e94\u7684\u5c0f\u6ce2\u53d8\u6362\u3002<\/p>\n

\uff08g-h\uff09k\uff08g\uff09\u548cR\uff08h\uff09\u7a7a\u95f4\u4e2dIr-NiCo2<\/sub>O4<\/sub> NSs\u7684Ir L3\u2212edge EXAFS\uff0c\u66f2\u7ebf\u662f\u62df\u5408\uff08\u7ea2\u7ebf\uff09\u548c\u5b9e\u9a8c\u4fe1\u53f7\uff08\u9ed1\u7ebf\uff09\u4e2d\u5305\u542b\u7684Ir\u2013O\u540e\u5411\u6563\u5c04\u4fe1\u53f7\uff08\u03c72<\/sub>\uff09\u3002<\/p>\n

\u56fe\u4e09\u3001\u9178\u6027<\/strong>OER<\/strong>\u7535\u5b50\u6d3b\u52a8\u7684\u7406\u8bba\u89e3\u91ca<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u542bVO<\/sub>\u7684NiCo2<\/sub>O4<\/sub>\u8868\u9762\u4fef\u89c6\u56fe\uff1b\u542bVO<\/sub>\u7684NiCo2<\/sub>O4<\/sub>\u8868\u9762\u7535\u5b50\u8f68\u9053\u7b49\u9ad8\u7ebf\u56fe\u4fa7\u89c6\u56fe\uff1bNiCo2<\/sub>O4<\/sub>\u8868\u9762VO<\/sub>\u4f4d\u9644\u8fd1\u951a\u5b9a\u7684\u539f\u5b50Ir\uff1b\u4ee5\u53caIr-NiCo2<\/sub>O4<\/sub>\u2212VO<\/sub>\u7684\u4fee\u6b63\u8f68\u9053\u7b49\u9ad8\u7ebf\u56fe\u4fa7\u89c6\u56fe\u3002<\/p>\n

\uff08b\uff09\u4ece\u4f53\u6676\u683c\u5230\u8868\u9762\u533a\u57dfCo\u22123d\u5e26\u7684PDOSs\u3002<\/p>\n

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\uff08e\uff09Ir-NiCo2<\/sub>O4<\/sub>\u2212VO<\/sub>\u8868\u9762Ni\u3001Co\u548cIr\u4f4d\u7684p\u2212d\u8f68\u9053\u6392\u5217\u3002<\/p>\n

\uff08f\uff09\u6676\u683cO\u22122p\u5e26\u4ece\u4f53\u6676\u683c\u5230\u8868\u9762\u533a\u57df\u7684PDOSs\u3002<\/p>\n

\uff08g\uff09\u4e2d\u95f4\u6c27\u7269\u79cdO\u22122p\u5e26\u7684PDOS\u3002<\/p>\n

\u56fe\u56db\u3001\u50ac\u5316\u6027\u80fd\u8bc4\u4f30<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5546\u7528IrO2<\/sub>\uff0cNiCo2<\/sub>O4<\/sub>\u4ee5\u53caIr-NiCo2<\/sub>O4<\/sub> NSs\u57280.5 M H2<\/sub>SO4<\/sub>\u7684LSV\u66f2\u7ebf\u3002<\/p>\n

\uff08b\uff09\u7528\u4e8eOER\u7684Ir-NiCo2<\/sub>O4<\/sub> NSs\u7684TOF\u66f2\u7ebf\u3002<\/p>\n

\uff08c\uff09\u7528\u4e8eOER\u7684NiCo2<\/sub>O4<\/sub>\u548cIr-NiCo2<\/sub>O4<\/sub> NSs\u57280.5 M H2<\/sub>SO4<\/sub>\u4e2d10 mA cm\u22122<\/sup>\u7684\u8ba1\u65f6\u7535\u6d41\u54cd\u5e94\u3002<\/p>\n

\uff08d\uff09NiCo2<\/sub>O4<\/sub>\u548cIr-NiCo2<\/sub>O4<\/sub> NSs\u57280.5 M H2<\/sub>SO4<\/sub>\u4e2d\u7684EIS\u66f2\u7ebf\u3002<\/p>\n

\uff08e\uff09\u6bd4\u8f83\u4e86j<\/em>=10 mA cm\u22122<\/sup>\u65f6\u7684\u8fc7\u7535\u4f4d\u548cIr-NiCo2<\/sub>O4<\/sub> NSs\u4e0e\u5148\u524d\u62a5\u9053\u7684OER\u50ac\u5316\u5242\u5728\u9178\u6027\u4ecb\u8d28\u4e2d\u7684\u7a33\u5b9a\u6027\u3002<\/p>\n

\uff08f\uff09\u6839\u636eNiCo2<\/sub>O4<\/sub>\u548cIr-NiCo2<\/sub>O4<\/sub> NSs\u7684\u626b\u63cf\u901f\u7387\u7ed8\u5236\u4e86\u53d8\u5316\u7684\u7535\u6d41\u5bc6\u5ea6\u5dee\uff08\u0394j<\/em>\uff09\u3002<\/p>\n

\uff08g\uff09\u4e0d\u540c\u6e29\u5ea6\u4e0b\u7528\u4e8eOER\u7684Ir-NiCo2<\/sub>O4<\/sub>-NSs\u7684LSV\u66f2\u7ebf\u3002<\/p>\n

\uff08h\uff09\u5728\u4e0d\u540c\u6e29\u5ea6\u4e0b\uff0c\u7528\u4e8eOER\u76840.5 M H2<\/sub>SO4<\/sub>\u4e2d10 mA cm\u22122<\/sup>\u4e0bIr-NiCo2<\/sub>O4<\/sub> NSs\u7684\u8ba1\u65f6\u7535\u6d41\u54cd\u5e94\u3002<\/p>\n

\uff08i\uff09\u57280.5 M H2<\/sub>SO4<\/sub>\u4e2d\uff0c\u7528\u4e8eOER\u7684\u4e0d\u540c\u6c27\u5316\u7269\u886c\u5e95\u4e0a\u7684LSV\u66f2\u7ebf\u3002<\/p>\n

\u56fe\u4e94\u3001\u9178\u6027\u6761\u4ef6\u4e0b<\/strong>OER<\/strong>\u9014\u5f84<\/strong><\/p>\n

\"\"<\/p>\n

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\uff08b\uff09\u5728U=1.23V\u65f6\uff0cOER\u9014\u5f84\u603b\u7ed3\u3002<\/p>\n

\uff08c\uff09\u521d\u59cb\u53cd\u5e94\u7269\u3001\u4e2d\u95f4\u4ea7\u7269\u6216\u6700\u7ec8\u4ea7\u7269\u5728Ir-NiCo2<\/sub>O4<\/sub>\u2212VO<\/sub>\u4e0a\u7684\u5c40\u90e8\u7ed3\u6784\u6784\u578b\u3002<\/p>\n

\u3010\u7ed3\u8bba\u5c55\u671b\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aIridium Single Atoms Coupling with Oxygen Vacancies Boosts Oxygen Evolution Reaction in Acid Media<\/a> ( J. Am. Chem. Soc.<\/em>, 2020<\/strong>, DOI: 10.1021\/jacs.0c05050)<\/p>\n

\u56e2\u961f\u7b80\u4ecb\uff1a<\/strong><\/p>\n

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\u5b66\u57fa\u91d1\u9762\u4e0a\u9879\u76ee\u4e00\u9879\uff0c\u7518\u8083\u7701\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u4e00\u9879,\u5b8c\u6210\u9752\u5e74\u57fa\u91d1\u4e00\u9879\uff0c\u6559\u80b2\u90e8\u535a\u58eb\u70b9\u57fa\u91d1\u4e00\u9879;\u5728J. Am. Chem. Soc.<\/em>, Adv. Mater.<\/em>, ACS Nano<\/em>, Inorg. Chem.<\/em>, Adv. Funct. Mater.<\/em>, Chem. Commun.<\/em>, J. Phys. Chem. C<\/em>\u7b49\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u658750\u591a\u7bc7\u3002<\/p>\n

\u9ec4\u52c3\u9f99<\/strong>\uff0c\u5251\u6865\u5927\u5b66\u535a\u58eb\uff0c\u9999\u6e2f\u7406\u5de5\u5927\u5b66\u5e94\u7528\u751f\u7269\u53ca\u5316\u5b66\u79d1\u6280\u5b66\u7cfb\u52a9\u7406\u6559\u6388\u3001\u535a\u58eb\u751f\u5bfc\u5e08\uff0c\u7814\u7a76\u65b9\u5411\u4e3a\u5148\u8fdb\u7406\u8bba\u8ba1\u7b97\u7b97\u6cd5\u5f00\u53d1\u7814\u7a76\u548c\u7a00\u571f\u65e0\u673a\u529f\u80fd\u6750\u6599\u5e94\u7528\u4e0e\u6027\u8d28\u8c03\u63a7\u3002\u9ec4\u52c3\u9f99\u6559\u6388\u957f\u671f\u5728\u56fa\u4f53\u529f\u80fd\u6750\u6599\u7535\u5b50\u7f3a\u9677\u6001\u7684\u7814\u7a76\u7406\u8bba\u548c\u8ba1\u7b97\u6280\u672f\u9886\u57df\u53d6\u5f97\u4e86\u7a81\u51fa\u7684\u7814\u7a76\u6210\u679c\u3002\u8fd1 5 \u5e74\u6765\uff0c\u5df2\u5728\u76f8\u5173\u9886\u57df\u53d1\u8868\u8bba\u658780\u4f59\u7bc7\uff0c\u5305\u62ec\u4ee5\u901a\u8baf\u4f5c\u8005\u6216\u7b2c\u4e00\u4f5c\u8005\u53d1\u8868\u4e86\u591a\u7bc7Adv. Mater.\uff0cAdv. Energy Mater., Nano Energy, Chem, ACS Catal. \u7b49\u3002\u540c\u65f6\uff0c\u9ec4\u52c3\u9f99\u8001\u5e08\u4e0e\u56fd\u5185\u5916\u524d\u6cbf\u8bfe\u9898\u7ec4(\u5317\u4eac\u5927\u5b66\uff0c\u65b0\u52a0\u5761\u56fd\u7acb\u5927\u5b66\u7b49)\u5747\u4fdd\u6301\u5bc6\u5207\u5408\u4f5c\uff0c\u5171\u540c\u53d1\u8868\u591a\u7bc7\u9ad8\u6c34\u5e73\u5408\u4f5c\u6587\u7ae0\u5305\u62ecNature, Science, Energy Environment. Science\u548cNature Communication\u3002<\/p>\n

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