{"id":214307,"date":"2020-12-09T06:07:17","date_gmt":"2020-12-08T22:07:17","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=214307"},"modified":"2020-12-08T21:07:53","modified_gmt":"2020-12-08T13:07:53","slug":"%e8%83%a1%e8%89%af%e5%85%b5%e5%9b%a2%e9%98%9fadv-energy-mater-%ef%bc%9a%e9%ab%98%e7%86%b5%e9%87%91%e5%b1%9e%e7%a1%ab%e5%8c%96%e7%89%a9%e7%ba%b3%e7%b1%b3%e7%b2%92%e5%ad%90%e5%ae%9e%e7%8e%b0%e9%ab%98","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=214307","title":{"rendered":"\u80e1\u826f\u5175\u56e2\u961fAdv. Energy Mater.\uff1a\u9ad8\u71b5\u91d1\u5c5e\u786b\u5316\u7269\u7eb3\u7c73\u7c92\u5b50\u5b9e\u73b0\u9ad8\u6548\u7535\u50ac\u5316\u6790\u6c27\u53cd\u5e94"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u901a\u8fc7\u7535\u5316\u5b66\u65b9\u6cd5\u8fdb\u884c\u6c34\u5206\u89e3\u5df2\u88ab\u8bc1\u660e\u662f\u4e00\u79cd\u5177\u6709\u6210\u672c\u6548\u76ca\uff0c\u6e05\u6d01\u4e14\u9ad8\u6548\u7684\u80fd\u91cf\u8f6c\u6362\u6280\u672f\uff0c\u5728\u8fc7\u53bb\u7684\u51e0\u5341\u5e74\u4e2d\u53d7\u5230\u4e86\u5e7f\u6cdb\u7684\u5173\u6ce8\u3002\u7531\u4e8e\u5176\u590d\u6742\u7684\u56db\u7535\u5b50\u8f6c\u79fb\u8fc7\u7a0b\uff0c\u6790\u6c27\u53cd\u5e94(OER)\u52a8\u529b\u5b66\u7f13\u6162\u963b\u788d\u4e86\u8be5\u6280\u672f\u7684\u8fdb\u4e00\u6b65\u53d1\u5c55\u3002\u56e0\u6b64\uff0c\u5f00\u53d1\u9ad8\u6548\uff0c\u8010\u7528\u4e14\u4f4e\u6210\u672c\u7684\u7535\u50ac\u5316\u5242\u5bf9\u4e8e\u51cf\u5c0f\u8fc7\u7535\u4f4d\u548c\u6539\u5584\u6574\u4f53OER\u6027\u80fd\u81f3\u5173\u91cd\u8981\u3002\u8fc7\u6e21\u91d1\u5c5e\u786b\u5316\u7269(Mx<\/sub>Sy<\/sub>)\u50ac\u5316\u5242\u5176\u5177\u6709\u826f\u597d\u7684\u5bfc\u7535\u6027\u548c\u50ac\u5316\u6d3b\u6027\u3002\u7136\u800c\uff0cMx<\/sub>Sy<\/sub>\u7684\u7a33\u5b9a\u6027\u8f83\u5dee\uff0c\u5305\u62ec\u70ed\u529b\u5b66\u4e0d\u7a33\u5b9a\uff0c\u7ed3\u6784\u4e0d\u7a33\u5b9a\u4ee5\u53ca\u5728\u9ad8\u6c27\u5316\u7535\u5316\u5b66\u6761\u4ef6\u4e0b\u50ac\u5316\u5242\u4ece\u57fa\u6750\u4e0a\u8131\u843d\u7b49\u95ee\u9898\u3002\u53e6\u5916\uff0c\u4ec5\u5177\u6709\u5c11\u91cf\u91d1\u5c5e\u5143\u7d20\u7684\u4e00\u5143\uff0c\u4e8c\u5143\u548c\u4e09\u5143Mx<\/sub>Sy<\/sub>\u50ac\u5316\u5242\u7f3a\u4e4f\u6210\u5206\u7684\u53ef\u8c03\u6027\u3002\u76f8\u6bd4\u4e4b\u4e0b\uff0c\u5177\u6709\u591a\u79cd\u91d1\u5c5e\u5143\u7d20\u7684\u9ad8\u71b5\u91d1\u5c5e\u786b\u5316\u7269(HEMS)\u53ef\u4ee5\u6839\u636eSabatier\u539f\u7406\u5b9e\u73b0\u6700\u4f73\u53cd\u5e94\u4e2d\u95f4\u4f53\u5438\u9644\uff0c\u4ece\u800c\u8fdb\u4e00\u6b65\u63d0\u9ad8OER\u6d3b\u6027\u3002HEMS\u5177\u6709\u591a\u79cd\u91d1\u5c5e\u5143\u7d20(\u22655)\u3002\u53d7\u76ca\u4e8e\u9ad8\u6df7\u5408\u71b5\u56fa\u6eb6\u4f53\u7684\u7a33\u5b9a\u6027\uff0c\u9884\u8ba1HEMS\u5177\u6709\u826f\u597d\u7684\u7ed3\u6784\u7a33\u5b9a\u6027\uff0c\u8fd9\u80fd\u591f\u6781\u5927\u7684\u6539\u5584OER\u8fc7\u7a0b\u7a33\u5b9a\u6027\u3002\u901a\u8fc7\u591a\u5143\u7d20\u7535\u5b50\u534f\u540c\u4f5c\u7528\u6765\u8c03\u8282\u50ac\u5316\u5242\u4e0e\u4e2d\u95f4\u4f53\u7684\u76f8\u4e92\u4f5c\u7528\uff0c\u4ee5\u8c03\u8282\u91d1\u5c5e\u786b\u5316\u7269\u4e2d\u7684\u7535\u8377\u72b6\u6001\uff0c\u5bf9\u4e8e\u63d0\u9ad8\u50ac\u5316\u6d3b\u6027\u5177\u6709\u826f\u597d\u7684\u524d\u666f\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c<\/strong>\u9a6c\u91cc\u5170\u5927\u5b66\u80e1\u826f\u5175\u6559\u6388\u56e2\u961f<\/strong>\u9996\u6b21\u901a\u8fc7\u8109\u51b2\u70ed\u5206\u89e3\u65b9\u6cd5\u5408\u6210\u4e86Mx<\/sub>Sy<\/sub>\u7eb3\u7c73\u9897\u7c92\uff0c\u4ee5\u514b\u670d\u591a\u79cd\u91d1\u5c5e\u6210\u5206\u7684\u4e0d\u6df7\u6eb6\u6027\u3002\u6240\u5236\u5907(CrMnFeCoNi)Sx<\/sub>\u7eb3\u7c73\u7c92\u5b50\u57281 M KOH\u6eb6\u6db2\u4e2d\u7528\u4f5cOER\u7684\u7535\u50ac\u5316\u5242\uff0c\u5728100 mA cm-2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5176\u8fc7\u7535\u4f4d\u4e3a295 mV\uff0c\u572810 h\u5185\u5177\u6709\u51fa\u8272\u7684\u7a33\u5b9a\u6027\u3002HEMS\u7eb3\u7c73\u9897\u7c92\u7684\u6027\u80fd\u4f18\u4e8e\u6587\u732e\u4e2d\u62a5\u9053\u7684\u5927\u591a\u6570Mx<\/sub>Sy<\/sub>\u6750\u6599\uff0c\u4ee5\u53ca\u4e00\u5143\uff0c\u4e8c\u5143\uff0c\u4e09\u5143\u548c\u56db\u5143Mx<\/sub>Sy<\/sub>\u5bf9\u5e94\u7269\u3002\u4e00\u5143\u81f3\u56db\u5143Mx<\/sub>Sy<\/sub>\u7eb3\u7c73\u7c92\u5b50\u7684\u8fc7\u7535\u4f4d\u4e0e\u91d1\u5c5e\u5143\u7d20\u7684\u6570\u91cf\u5448\u53cd\u6bd4\u5173\u7cfb\uff0c\u8868\u660e\u91d1\u5c5e\u5143\u7d20\u4e4b\u95f4\u5177\u6709\u534f\u540c\u6548\u5e94\uff0c\u901a\u8fc7DFT\u8ba1\u7b97\u5206\u6790\u8bc1\u5b9e\u4e86\u8fd9\u4e00\u70b9\u3002HEMS\u51fa\u8272\u7684OER\u6d3b\u6027\u548c\u826f\u597d\u7684\u8010\u4e45\u6027\u8bc1\u660e\u4e86\u5176\u4f5c\u4e3a\u9ad8\u6548\u6c34\u5206\u89e3\u7535\u50ac\u5316\u5242\u7684\u826f\u597d\u6f5c\u529b\uff0c\u540c\u65f6\u4f5c\u8005\u63d0\u51fa\u7684\u8109\u51b2\u70ed\u5206\u89e3\u65b9\u6cd5\u4e3a\u5176\u4ed6\u5e94\u7528\u63d0\u4f9b\u4e86\u4e00\u79cd\u5408\u6210\u591a\u5143\u7d20\u786b\u5316\u7269\u7684\u901a\u7528\u65b9\u6cd5\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u201cHigh-Entropy Metal Sulfide Nanoparticles Promise High-Performance Oxygen Evolution Reaction<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Advanced Energy Materials<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00<\/strong>HEMS(CrMnFeCoNi)Sx<\/sub><\/strong>\u7eb3\u7c73\u9897\u7c92\u7684\u7ed3\u6784\u53ca\u5176\u5728<\/strong>OER<\/strong>\u50ac\u5316\u5242\u4e2d\u7684\u5e94\u7528<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5c06\u4e0d\u6df7\u6eb6\u7684\u91d1\u5c5e\u5143\u7d20\uff08\u5373Cr\uff0cMn\uff0cFe\uff0cCo\u548cNi\uff09\u6df7\u5408\u6210\u9ad8\u71b5\u786b\u5316\u7269\u7eb3\u7c73\u9897\u7c92\u793a\u610f\u56fe\u3002<\/p>\n

\uff08b\uff09\u4e00\u5143\uff0c\u4e8c\u5143\uff0c\u4e09\u5143\uff0c\u56db\u5143\u6750\u6599\u548c\u4e94\u5143HEMS\u4e4b\u95f4\u7684\u8fc7\u7535\u4f4d\u548c\u91d1\u5c5e\u5143\u7d20\u6570\u91cf\u7684\u5173\u7cfb\u56fe\u3002<\/p>\n

\u56fe\u4e8c<\/strong>HEMS(CrMnFeCoNi)Sx<\/sub><\/strong>\u7eb3\u7c73\u9897\u7c92\u7684\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09(CrMnFeCoNi)Sx<\/sub>\u7eb3\u7c73\u9897\u7c92\u5728\u78b3\u886c\u5e95\u4e0a\u7684TEM\u56fe\u50cf\u3002<\/p>\n

\uff08b\uff09(CrMnFeCoNi)Sx<\/sub>\u7684\u7c92\u5ea6\u5206\u6790\u3002<\/p>\n

\uff08c\uff09(CrMnFeCoNi)Sx<\/sub>\u7eb3\u7c73\u9897\u7c92\u7684\u9ad8\u5206\u8fa8\u7387TEM\u56fe\u50cf\u3002<\/p>\n

\uff08d\uff09(CrMnFeCoNi)Sx<\/sub>\u7eb3\u7c73\u9897\u7c92\u7684HAADF-STEM\u56fe\u50cf\u548c\u76f8\u5e94\u7684EDS\u5143\u7d20\u5206\u6790\u3002<\/p>\n

\u56fe\u4e09<\/strong>(CrMnFeCoNi)Sx<\/sub><\/strong>\u7684\u7269\u76f8\u548c<\/strong>DFT<\/strong>\u8ba1\u7b97\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09(CrMnFeCoNi)Sx<\/sub>\u7684XRD\u56fe\u8c31\u3002<\/p>\n

\uff08b\uff0cc\uff09(CrMnFeCoNi)Sx<\/sub>\uff0c\u4e8c\u5143(NiFe)9<\/sub>S8<\/sub>\u548c\u4e09\u5143(FeCoNi)9<\/sub>S8<\/sub>\u7684Fe 2p\u548cCo 2p\u7684\u9ad8\u5206\u8fa8\u7387XPS\u5149\u8c31\u3002<\/p>\n

\uff08d\uff09\u901a\u8fc7\u5c06\u9633\u79bb\u5b50Co\u4e2d\u5fc3\u89c6\u4e3a\u6d3b\u6027\u4f4d\u70b9\u6765\u6784\u5efa(Cr2<\/sub>MnFe2<\/sub>Co2<\/sub>Ni2<\/sub>)S8<\/sub>\u6a21\u578b\u7684\u793a\u610f\u56fe\u3002<\/p>\n

\uff08e\uff09OER\u53cd\u5e94\u673a\u5236\u4e2d\u7684\u81ea\u7531\u80fd\u6f14\u5316\u3002<\/p>\n

\uff08f\uff09\u4e00\u5143Mx<\/sub>Sy<\/sub>\u548cHEMS(Cr2<\/sub>MnFe2<\/sub>Co2<\/sub>Ni2<\/sub>)S8<\/sub>\u7684\u50ac\u5316\u6d3b\u6027\u56fe\u3002<\/p>\n

\uff08g\uff09\u9760\u8fd1Co\u4e2d\u5fc3\u7684(Cr2<\/sub>MnFe2<\/sub>Co2<\/sub>Ni2<\/sub>)S8<\/sub>\u548cCo9<\/sub>S8<\/sub>\u4e4b\u95f4\u7684\u7535\u8377\u5bc6\u5ea6\u5dee\u3002<\/p>\n

\uff08h\uff09(Cr2<\/sub>MnFe2<\/sub>Co2<\/sub>Ni2<\/sub>)S8<\/sub>\u4e2dCr\uff0cMn\uff0cFe\uff0cCo\u548cNi\u7684\u76f8\u5bf9\u7535\u8377\u6001\u3002<\/p>\n

\uff08i\uff09(Cr2<\/sub>MnFe2<\/sub>Co2<\/sub>Ni2<\/sub>)S8<\/sub>\u548c\u4e00\u5143Mx<\/sub>Sy<\/sub>\u50ac\u5316\u5242\u7684d\u5e26\u4e2d\u5fc3\u80fd\u91cf\u968f\u5438\u9644\u80fd\uff08\u0394E<\/em>o<\/sub>\u2217<\/sub>\uff09\u7684\u53d8\u5316\u6bd4\u8f83\u3002<\/p>\n

\u56fe\u56db<\/strong> \u5404\u79cd<\/strong>Mx<\/sub>Sy<\/sub><\/strong>\u7684<\/strong>OER<\/strong>\u7535\u50ac\u5316\u6027\u80fd\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09(CrMnFeCoNi)Sx<\/sub>\uff0c(MnFeCoNi)9<\/sub>S8<\/sub>\uff0c(FeCoNi)9<\/sub>S8<\/sub>\u548c(NiFe)9<\/sub>S8<\/sub>\u7684LSV\u66f2\u7ebf\u3002<\/p>\n

\uff08b\uff09\u4ece\u76f8\u5e94\u7684LSV\u66f2\u7ebf\u5f97\u51fa\u7684Tafel\u56fe\u3002<\/p>\n

\uff08c\uff09\u4f7f\u7528100 mA cm-2<\/sup>\u7684\u6052\u5b9a\u7535\u6d41\u5bc6\u5ea6\u5bf9(CrMnFeCoNi)Sx<\/sub> \u8fdb\u884c10\u4e2a\u5c0f\u65f6\u7684\u8ba1\u65f6\u7535\u4f4d\u6d4b\u8bd5\u3002<\/p>\n

\uff08d\uff09(CrMnFeCoNi)Sx<\/sub>\u572820\u300150\u3001100\u3001150\u548c200 mA cm-2<\/sup>\u7684\u591a\u6b65\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u8ba1\u65f6\u7535\u4f4d\u6cd5\u3002<\/p>\n

\uff08e\uff09\u4e94\u5143(CrMnFeCoNi)Sx<\/sub>\uff0c\u56db\u5143(MnFeCoNi)9<\/sub>S8<\/sub>\uff0c\u4e09\u5143(FeCoNi)9<\/sub>S8<\/sub>\uff0c\u4e8c\u5143(NiFe)9<\/sub>S8<\/sub>\u548c\u4e00\u5143Mn9<\/sub>S8<\/sub>\uff0cCo9<\/sub>S8<\/sub>\uff0cNi9<\/sub>S8<\/sub>\u548cFe9<\/sub>S8<\/sub>\u7684\u8fc7\u7535\u52bf\u548cTafel\u659c\u7387\u6bd4\u8f83\u3002<\/p>\n

\uff08f\uff09\u4e0e\u5176\u4ed6\u540c\u7c7b\u578b\u5de5\u4f5c\u7684\u5bf9\u6bd4\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u603b\u4e4b\uff0c\u5728\u8fd9\u9879\u7814\u7a76\u4e2d\uff0c\u4f5c\u8005\u901a\u8fc7\u8109\u51b2\u70ed\u5206\u89e3\u65b9\u6cd5\u5408\u6210\u4e86\u5747\u5300\u6df7\u5408\u548c\u71b5\u7a33\u5b9a\u7684HEMS(CrMnFeCoNi)Sx<\/sub>\u7eb3\u7c73\u7c92\u5b50\uff0c\u4ee5\u514b\u670d\u591a\u79cd\u91d1\u5c5e\u5143\u7d20\u4e0d\u6df7\u6eb6\u6027\u7684\u9650\u5236\u3002\u76f8\u5173\u8ba1\u7b97\u5de5\u4f5c\u8868\u660e\uff0c\u7535\u8377\u72b6\u6001\u5728\u591a\u4e2a\u91d1\u5c5e\u4f4d\u70b9\u4e4b\u95f4\u8fc1\u79fb\uff0c\u4ece\u800c\u8c03\u8282\u7535\u5b50\u7ed3\u6784\u4ee5\u5f71\u54cdOER\u6027\u80fd\u3002\u5f53\u4f5c\u4e3aOER\u50ac\u5316\u5242\u8fdb\u884c\u6d4b\u8bd5\u65f6\uff0c(CrMnFeCoNi)Sx<\/sub>\u7eb3\u7c73\u50ac\u5316\u5242\u5c31\u534f\u540c\u6548\u5e94\u800c\u8a00\u5177\u6709\u826f\u597d\u7684\u50ac\u5316\u6d3b\u6027\u548c\u8f83\u957f\u7684\u8010\u4e45\u6027\uff0c\u4ece\u800c\u9a8c\u8bc1\u4e86\u8ba1\u7b97\u9884\u6d4b\u3002\u8fd9\u9879\u7814\u7a76\u4e3a\u5408\u6210\u7528\u4e8e\u5404\u79cd\u80fd\u91cf\u548c\u50ac\u5316\u5e94\u7528\u7684\u5404\u79cd\u9ad8\u71b5\u5316\u5408\u7269\u7eb3\u7c73\u9897\u7c92\uff08\u6c27\u5316\u7269\uff0c\u786b\u5316\u7269\uff0c\u78f7\u5316\u7269\u548c\u7852\u5316\u7269\u7b49\uff09\u6253\u5f00\u4e86\u65b0\u7684\u5927\u95e8\u3002<\/p>\n

\u00a0<\/strong>\u6587\u732e\u94fe\u63a5\uff1a<\/strong>\u201c<\/strong>High-Entropy Metal Sulfide Nanoparticles Promise High-Performance Oxygen Evolution Reaction<\/strong><\/a>\u201d(Adv. Energy Mater.<\/strong> DOI: 10.1002\/aenm.202002887)<\/strong><\/p>\n

\u00a0<\/strong>\u3010\u901a\u8baf\u4f5c\u8005\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u80e1\u826f\u5175\u6559\u6388\uff0c\u7f8e\u56fd\u9a6c\u91cc\u5170\u5927\u5b66\u7ec8\u8eab\u6559\u6388\uff08<\/strong>Herbert Rabin Distinguished Professor<\/strong>\uff09\uff0c<\/strong> \u6750\u6599\u521b\u65b0\u4e2d\u5fc3\u4e3b\u4efb\uff08<\/strong>Center for Materials Innovation<\/strong>\uff09\u3002\u5df2\u5728<\/strong>Science<\/strong>\u53ca\u5176\u5b50\u520a<\/strong>, Nature<\/strong>\u53ca\u5176\u5b50\u520a<\/strong>, JACS<\/strong>\uff0c<\/strong> Angewandte Chemie International Edition<\/strong>\uff0c<\/strong> Energy & Environmental Science, Advanced Materials, Advanced Energy Materials, Chemical Reviews, Nano Letters, ACS Nano <\/strong>\u7b49\u9876\u7ea7\u671f\u520a\u4e0a\u53d1\u8868\u5b66\u672f\u8bba\u6587<\/strong>300<\/strong>\u4f59\u7bc7\uff0c\u88ab\u5f15\u7528\u8d85\u8fc7<\/strong>54,000<\/strong>\u6b21\uff0c<\/strong>H-Index<\/strong>\u4e3a<\/strong>113<\/strong>\u3002<\/strong><\/p>\n

\u00a0<\/strong>\u672c\u6587\u7531\u5fae\u89c2\u4e16\u754c\u7f16\u8bd1\u4f9b\u7a3f\u3002<\/p>\n

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