{"id":214697,"date":"2020-12-18T06:51:45","date_gmt":"2020-12-17T22:51:45","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=214697"},"modified":"2020-12-17T19:51:57","modified_gmt":"2020-12-17T11:51:57","slug":"angew%ef%bc%9a%e9%a2%9c%e8%89%b2%e5%92%8c%e7%bb%b4%e5%ba%a6%e5%8f%af%e8%b0%83%e7%9a%84%e5%85%89%e6%8d%95%e8%8e%b7%e6%9c%89%e6%9c%ba%e7%94%b5%e8%8d%b7%e8%bd%ac%e7%a7%bb%e5%90%88%e9%87%91","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=214697","title":{"rendered":"Angew\uff1a\u989c\u8272\u548c\u7ef4\u5ea6\u53ef\u8c03\u7684\u5149\u6355\u83b7\u6709\u673a\u7535\u8377\u8f6c\u79fb\u5408\u91d1"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5929\u6d25\u5927\u5b66\u96f7\u4e49\u9f99\u6559\u6388\u548c\u9996\u90fd\u5e08\u8303\u5927\u5b66\u4ed8\u7ea2\u5175\u6559\u6388\u3001<\/strong>\u5ed6\u6e05<\/strong>\u6559\u6388\u7814\u7a76\u56e2\u961f<\/strong>\u7406\u6027\u9009\u62e9\u4e86\u5206\u5b50\u7ed3\u6784\u53ca\u5c3a\u5bf8\u5339\u914d\u7684\u4e8c\u8418\u5d4c\u82ef\uff08Pe\uff09\u548c9,10-\u4e8c\u6c30\u57fa\u84bd\uff08DCA\uff09\u7535\u5b50\u7ed9\/\u53d7\u4f53\u5bf9\uff0c\u5e76\u57fa\u4e8e\u8be5\u4e24\u8005\u5206\u5b50\u95f4\u7684\u5f31CT\u76f8\u4e92\u4f5c\u7528\uff0c\u5229\u7528\u6db2\u76f8\u5171\u7ec4\u88c5\u8def\u7ebf\u6210\u529f\u6784\u5efa\u4e24\u7c7b\u6709\u673a\u7535\u8377\u8f6c\u79fb\uff08CT\uff09\u5408\u91d1\u7ec4\u88c5\u4f53\u3002\u901a\u8fc7\u8c03\u5236Pe\u548cDCA\u4e4b\u95f4\u7684\u6469\u5c14\u6bd4\uff0c\u80fd\u91cf\u53ef\u4eceDCA\u6216\u03b1-Pe\u4f20\u9012\u5230Pe-DCA CT\u4e8c\u5143\u590d\u5408\u7269\uff0c\u83b7\u5f97\u4e86\u989c\u8272\u548c\u7ef4\u5ea6\u53ef\u8c03\u7684CT\u5408\u91d1\uff0c\u5305\u62ec\u4e00\u7ef4\uff081D\uff09\uff08DCA)1-x<\/em><\/sub>\uff08Pe\uff09x<\/sub><\/em>\uff080 \u2264 x<\/em> \u2264 10%\uff09\u5fae\u7c73\u5e26\u548c\u4e8c\u7ef4 \uff082D\uff09\uff08Pe\uff091-y<\/em><\/sub>\uff08DCA\uff09y<\/sub><\/em>\uff080 \u2264 y<\/em> \u2264 5\uff05\uff09\u7eb3\u7c73\u7247\u3002\u91cd\u8981\u7684\u662f\uff0c\u8be5\u4e24\u7c7b\u6709\u673a\u5408\u91d1\u7ec4\u88c5\u4f53\u663e\u793a\u51fa\u7ef4\u5ea6\u76f8\u5173\u7684\u5149\u6ce2\u5bfc\u6027\u80fd\uff1a\u4e00\u7ef4\uff08DCA\uff091-x<\/em><\/sub>\uff08Pe\uff09x<\/sub><\/em>\u5fae\u7c73\u5e26\u4e2d\u5149\u6ce2\u5bfc\u635f\u8017\u8fde\u7eed\u53ef\u8c03\uff0c\u4ee5\u53ca\u4e8c\u7ef4\uff08Pe\uff091-y<\/em><\/sub>\uff08DCA\uff09y<\/sub><\/em>\u7eb3\u7c73\u7247\u4e2d\u6ce2\u5bfc\u4ece\u5404\u5411\u540c\u6027\u5230\u5404\u5411\u5f02\u6027\u8fde\u7eed\u8f6c\u6362\u3002\u8be5\u6210\u679c\u8fd1\u65e5\u4ee5\u9898\u4e3a\u201cColor\u2010and Dimension\u2010Tunable Light\u2010Harvesting Organic Charge\u2010Transfer Alloys for Controllable Photon\u2010Transport Photonics<\/strong>\u201d\u53d1\u8868\u5728\u8457\u540d\u671f\u520aAngew. Chem. Int. Ed.<\/strong>\u4e0a\uff0c\u8bba\u6587\u7b2c\u4e00\u4f5c\u8005\u4e3a\u5929\u6d25\u5927\u5b66\u7855\u58eb\u7814\u7a76\u751f\u97e9\u5e0c\u5e0c\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\uff1a<\/strong>Pe<\/strong>\u548c<\/strong> DCA<\/strong>\u7684\u5206\u5b50\u6784\u578b\u3001\u5c3a\u5bf8\u53ca\u5f62\u6210\u7684\u4e24\u79cd\u7c7b\u578b\u7684\u6709\u673a\u5408\u91d1\u7ed3\u6784<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a-b\uff09Pe\u548cDCA\u7684\u5206\u5b50\u7ed3\u6784\u548c\u5c3a\u5bf8\u3002<\/p>\n

\uff08c-d\uff09Pe\u548cDCA\u5206\u522b\u6cbfa<\/em>\u548cc<\/em>\u8f74\u89c2\u5bdf\u5230\u7684\u5206\u5b50\u5806\u79ef\u6784\u578b\u3002<\/p>\n

\uff08e\uff09\uff08DCA\uff091-\u00a0x<\/em><\/sub>\uff08Pe\uff09x<\/sub><\/em>\u548c\uff08Pe\uff091-\u00a0y<\/em><\/sub>\uff08DCA\uff09y<\/sub><\/em>\u4e24\u79cd\u7c7b\u578b\u6709\u673a\u5408\u91d1\u7684\u7ed3\u6784\u53ca\u5f62\u6210\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u4e8c\uff1a<\/strong>(DCA)1-x<\/em><\/sub>(Pe)<\/strong>x<\/sub>\u5fae\u7c73\u5e26\u7684\u5fae\u89c2\u5f62\u8c8c\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a-d\uff09(DCA) 1-x<\/em><\/sub> (Pe)x<\/sub><\/em>\uff08x<\/em> = (a,e) 0, (b,f) 0.1%, (c,g) 1%\u548c(d,h) 10\u2009%\uff09\u5408\u91d1\u5fae\u7c73\u5e26\u7684SEM\u56fe\uff0c\u6807\u5c3a\u4e3a25 \u03bcm\u3002<\/p>\n

\uff08e-h\uff09(DCA) 1-x<\/em><\/sub> (Pe)x<\/sub><\/em>\uff08x<\/em> = (a,e) 0, (b,f) 0.1%, (c,g) 1%\u548c(d,h) 10\u2009%\uff09\u5408\u91d1\u5fae\u7c73\u5e26\u7684TEM\u56fe\uff0c\u6807\u5c3a\u4e3a500 nm\u3002<\/p>\n

\u56fe\u4e09\uff1a<\/strong>\uff08<\/strong>DCA<\/strong>\uff09<\/strong>1-\u00a0x<\/em><\/sub><\/strong>\uff08<\/strong>Pe<\/strong>\uff09<\/strong>x<\/sub><\/em><\/strong>\u5fae\u7c73\u5e26\u7684\u7ed3\u6784\u5206\u6790\u53ca\u751f\u957f\u6a21\u62df\u5f62\u8c8c<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5728x<\/em> = 0\u30010.1\uff05\uff0c1\uff05\u548c10\uff05\u65f6\u5f62\u6210\u7684\uff08DCA\uff091- x<\/em>\uff08Pe\uff09x<\/em>\u5408\u91d1\u5fae\u7c73\u5e26\u7684\u7c89\u672bXRD\u56fe\u548c\u4f9d\u636e\u5176\u7ed3\u6676\u5b66\u6570\u636e\u6a21\u62df\u7684DCA\u7684\u5355\u6676XRD\u56fe\u3002<\/p>\n

\uff08b\uff09\u4f7f\u7528Material Studio\u8f6f\u4ef6\u6a21\u62df\u7684DCA\u7684\u7406\u8bba\u751f\u957f\u5f62\u8c8c\u3002\u5185\u63d2\u56fe\u663e\u793a\u4e86\u6cbf[100]\u65b9\u5411\u751f\u957f\u7684DCA\u5fae\u7c73\u5e26\u7684\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u56db\uff1a\uff08<\/strong>DCA<\/strong>\uff09<\/strong>1- x<\/strong>\uff08<\/strong>Pe<\/strong>\uff09<\/strong>x<\/strong>\u7684\u8367\u5149\u7279\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\u2013d\uff09\u7d2b\u5916\u5149\u6fc0\u53d1\u4e0b\uff0c\uff08DCA\uff091-x<\/em><\/sub>\uff08Pe\uff09x<\/sub><\/em>\u5fae\u7c73\u5e26\u5728x<\/em> = 0\u30010.1\uff05\uff0c1\uff05\u548c10\uff05\u65f6\u7684\u8367\u5149\u663e\u5fae\u56fe\u3002<\/p>\n

\uff08e\uff09\u5bf9\u5e94\u7684\u56fa\u6001\u5438\u6536\u548cPL\u5149\u8c31\u3002\u6fc0\u53d1\u6ce2\u957f\u4e3a420 nm\u3002<\/p>\n

\uff08f\uff09\u5728375 nm\u6fc0\u5149\u6fc0\u53d1\u65f6\u7684\uff08DCA\uff091-\u00a0x<\/em><\/sub>\uff08Pe\uff09x<\/sub><\/em>\u5728540\u548c620 nm\u5904\u7684\u65f6\u95f4\u5206\u8fa8\u8367\u5149\u8870\u51cf\u66f2\u7ebf\u3002<\/p>\n

\uff08g\uff09\uff08DCA\uff091-\u00a0x<\/em><\/sub>\uff08Pe\uff09x<\/sub><\/em>\u5408\u91d1\u4e2d\u7684\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u4e94\uff1a\uff08<\/strong>Pe<\/strong>\uff09<\/strong>1-\u00a0y<\/em><\/sub><\/strong>\uff08<\/strong>DCA<\/strong>\uff09<\/strong>y<\/sub><\/em><\/strong>\u7eb3\u7c73\u7247\u7684\u7ed3\u6784\u53ca\u5149\u5b66\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\u2013d\uff09\uff08Pe\uff091-\u00a0y<\/em><\/sub>\uff08DCA\uff09y<\/sub><\/em>\uff08y<\/em>\u00a0=\uff08a,e\uff090,\uff08b,f\uff090.25\uff05,\uff08c,g\uff091\uff05,\uff08d,h\uff095\uff05\uff09\u7eb3\u7c73\u7247\u7684TEM\u3002<\/p>\n

\uff08e\u2013h\uff09\uff08Pe\uff091-\u00a0y<\/em><\/sub>\uff08DCA\uff09y<\/sub><\/em>\uff08y<\/em>\u00a0=\uff08a,e\uff090,\uff08b,f\uff090.25\uff05,\uff08c,g\uff091\uff05,(d,h\uff095\uff05\uff09\u7eb3\u7c73\u7247\u7684\u8367\u5149\u663e\u5fae\u56fe\u3002<\/p>\n

\u56fe\u516d\uff1a\uff08<\/strong>DCA<\/strong>\uff09<\/strong>1-\u00a0x<\/em><\/sub><\/strong>\uff08<\/strong>Pe<\/strong>\uff09<\/strong>x<\/sub><\/em><\/strong>\u5fae\u7c73\u5e26\u7684\u5149\u6ce2\u5bfc\u884c\u4e3a<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a,c,e\uff09\uff08DCA\uff091-\u00a0x<\/em><\/sub>\uff08Pe\uff09x<\/sub><\/em>\u5408\u91d1\u5fae\u7c73\u5e26\u5728x<\/em>\u00a0=\uff08a\uff090\uff0c\uff08c\uff090.1\uff05\u548c\uff08e\uff091\uff05\u65f6\u5f62\u6210\u7684\u4eae\u573a\u548cPL\u56fe\uff0c\u8be5\u7cfb\u5217\u56fe\u50cf\u901a\u8fc7\u5728\u4e00\u7ef4\u5fae\u7c73\u5e26\u4e2d\u6fc0\u53d1\u4e94\u5904\u4e0d\u540c\u7684\u4f4d\u7f6e\u83b7\u53d6\u3002\u56fe\u4e2d\u6807\u5c3a\uff0c25 \u03bcm\u3002<\/p>\n

\uff08b,d,f\uff09\u5bf9\u5e94\u7684\u7a7a\u95f4\u5206\u8fa8PL\u5149\u8c31\uff0c\u8be5\u7cfb\u5217\u5149\u8c31\u901a\u8fc7\u91c7\u96c6\u968f\u4e0d\u540c\u4f20\u64ad\u8ddd\u79bbd<\/em>\u6539\u53d8\u7684\u5355\u6839\u5fae\u7c73\u5e26\u7aef\u90e8\u7684PL\u6240\u83b7\u5f97\u3002<\/p>\n

\u56fe\u4e03\uff1a\uff08<\/strong>Pe<\/strong>\uff09<\/strong>1-\u00a0y<\/em><\/sub><\/strong>\uff08<\/strong>DCA<\/strong>\uff09<\/strong>y<\/sub><\/em><\/strong> \u7eb3\u7c73\u7247\u7684\u5149\u6ce2\u5bfc\u884c\u4e3a<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\u2013e\uff09\uff08Pe\uff091-y<\/em><\/sub>\uff08DCA\uff09y<\/sub><\/em>\u5408\u91d1\u7eb3\u7c73\u7247\u5728y<\/em> = 0\u30010.25\uff05\uff0c0.5\uff05\uff0c1\uff05\u548c5\uff05\u5904\u7684PL\u56fe\uff0c\u8be5\u7cfb\u5217PL\u56fe\u901a\u8fc7\u5ef6\u65b9\u54111\u548c2\u6fc0\u53d1\u5355\u4e2a\u7eb3\u7c73\u7247\u4e2d\u4e94\u5904\u4e0d\u540c\u4f4d\u7f6e\u83b7\u5f97\u3002\u6807\u5c3a\u4e3a25 \u03bcm\u3002<\/p>\n

\uff08f\u2013j\uff09\u5728f\uff09560\u548cg\u2013j\uff09610 nm\u5904\uff0cI<\/em>tip<\/sub>\/I<\/em>ex<\/sub>\u4e0ed<\/em>\u7684\u5bf9\u6570\u5173\u7cfb\uff0c\u5176\u4e2dI<\/em>tip<\/sub>\u548cI<\/em>ex<\/sub>\u5206\u522b\u662f\u8f93\u51fa\u8fb9\u7f18\u548c\u6fc0\u53d1\u70b9\u5904\u7684\u53d1\u5c04\u5f3a\u5ea6\u3002<\/p>\n

\uff08k\u2013o\uff09\u968f\u504f\u632f\u89d2\u5ea6\u53d8\u5316\u7684PL\u5f3a\u5ea6\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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