{"id":215345,"date":"2021-01-07T06:00:53","date_gmt":"2021-01-06T22:00:53","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=215345"},"modified":"2021-01-06T22:06:22","modified_gmt":"2021-01-06T14:06:22","slug":"mof%e6%9c%80%e6%96%b0nat-chem-%e3%80%81nat-mater-%e3%80%81nat-energy%e3%80%81nat-nanotech-nat-commun","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=215345","title":{"rendered":"MOF\u6700\u65b0Nat. Chem.\u3001Nat. Mater.\u3001Nat. Energy\u3001Nat. Nanotech.\u2026"},"content":{"rendered":"<p><strong><b>Nat. Chem.\uff1a\u8868\u73b0\u51fa\u4e8c\u6c27\u5316\u78b3\u8bf1\u5bfc\u7684\u987a\u78c1\u6027\u548c\u4e9a\u78c1\u6027\u4e4b\u95f4\u7684\u8f6c\u53d8MOF<\/b><\/strong><\/p>\n<p>\u5982\u679c\u6709\u8db3\u591f\u7684\u6784\u9020\u5757\uff0c\u91d1\u5c5e\u6709\u673a\u6846\u67b6(MOFs)\u53ef\u4ee5\u7ed3\u5408\u78c1\u6027\u6392\u5e8f\u548c\u5b54\u9699\u7387\u3002\u8fd9\u4f7f\u5f97MOFs\u662f\u4e00\u79cd\u5f88\u6709\u524d\u9014\u7684\u5f00\u53d1\u523a\u6fc0\u54cd\u5e94\u6750\u6599\u7684\u5e73\u53f0\uff0c\u5176\u8868\u73b0\u51fa\u622a\u7136\u4e0d\u540c\u7684\u78c1\u6027\u80fd\u53d6\u51b3\u4e8e\u5176\u5b54\u6d1e\u4e2d\u662f\u5426\u5b58\u5728\u5ba2\u4f53\u5206\u5b50\u3002\u65e5\u672c\u4e1c\u5317\u5927\u5b66Hitoshi Miyasaka\u6559\u6388\u7b49\u4eba\u62a5\u9053\u4e86\u4e00\u79cdCO<sub>2<\/sub>\u54cd\u5e94\u578b\u78c1\u6027MOF\uff0c\u5b83\u5728CO<sub>2<\/sub>\u5438\u9644\u65f6\u7531\u94c1\u78c1\u8f6c\u53d8\u4e3a\u987a\u78c1\uff0c\u5728CO<sub>2<\/sub>\u89e3\u5438\u65f6\u53c8\u6062\u590d\u5230\u94c1\u78c1\u72b6\u6001\u3002\u7814\u7a76\u53d1\u73b0\uff0c\u8be5\u4e9a\u94c1\u78c1\u6027\u6750\u6599\u662f\u5177\u6709[D<sup>+<\/sup>\u2013A<sup>&#8211;<\/sup>\u2013D]\u5206\u5b50\u5f0f\u7684\u5c42\u72b6MOF\uff0c\u5b83\u662f\u7531\u4e09\u6c1f\u82ef\u7532\u9178\u916f\u6865\u8054\u7684\u6868\u8f6e\u578b\u4e8c\u948c\uff08II\uff09\u7c07\u4f5c\u4e3a\u7535\u5b50\u4f9b\u4f53\uff08D\uff09\u4e0e\u4e8c\u4e59\u6c27\u57fa\u56db\u6c30\u57fa\u55b9\u4e8c\u7532\u70f7\u4f5c\u4e3a\u7535\u5b50\u53d7\u4f53\uff08A \uff09\u3002\u5728\u5438\u9644CO<sub>2<\/sub>\u65f6\uff0cMOF\u4f1a\u7ecf\u5386\u9762\u5185\u7535\u5b50\u8f6c\u79fb\u548c\u7ed3\u6784\u8f6c\u53d8\uff0c\u4ece\u800c\u5f62\u6210[D\u2013A\u2013D]\u987a\u78c1\u6027\u5f62\u5f0f\u3002\u5728CO<sub>2<\/sub>\u5438\u6536\u65f6\uff0c\u5b83\u7ecf\u5386\u4e86\u5e73\u9762\u5185\u7684\u7535\u5b50\u8f6c\u79fb\u548c\u7ed3\u6784\u8dc3\u8fc1\uff0c\u91c7\u7528[D-A-D]\u987a\u78c1\u5f62\u5f0f\u3002\u8fd9\u79cd\u78c1\u6027\u76f8\u53d8\uff0c\u4ee5\u53ca\u968f\u4e4b\u5bf9MOF\u7684\u7535\u5b50\u5bfc\u7535\u6027\u548c\u4ecb\u7535\u5e38\u6570\u7684\u6539\u53d8\uff0c\u90fd\u662f\u7531\u6846\u67b6\u5185\u7684\u5ba2\u4f53\u4e8c\u6c27\u5316\u78b3\u5206\u5b50\u7535\u5b50\u7a33\u5b9a\u7684\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cA metal\u2013organic framework that exhibits\u00a0CO<sub>2<\/sub>-induced transitions between paramagnetism\u00a0and ferrimagnetism\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nat. Chem.\u4e0a\u3002DOI:\u00a010.1038\/s41557-020-00577-y<\/p>\n<p>\u56fe1\u00a0\u5316\u5408\u72691\u7684CO<sub>2<\/sub>\u5438\u9644\u3001\u6676\u4f53\u7ed3\u6784\u53d8\u5316\u548c\u7ea2\u5916\u5149\u8c31<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215346 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-1-22.png\" alt=\"\" width=\"600\" height=\"767\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-1-22.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-1-22-235x300.png 235w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Nat. Energy\uff1a<\/b><\/strong><strong><b>\u9ad8\u6d3b\u6027\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6\u7535\u50ac\u5316\u5242\u5728OER\u4e2d\u7684\u7ed3\u6784\u8f6c\u53d8<\/b><\/strong><\/p>\n<p>\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6(MOFs)\u4f5c\u4e3a\u6790\u6c27\u53cd\u5e94(OER)\u7684\u7535\u50ac\u5316\u5242\u5f97\u5230\u4e86\u8d8a\u6765\u8d8a\u591a\u7684\u7814\u7a76\u3002\u5c3d\u7ba1\u5b83\u4eec\u6709\u5f88\u597d\u7684\u50ac\u5316\u6d3b\u6027\uff0c\u4f46\u5173\u4e8e\u5b83\u4eec\u7684\u7ed3\u6784-\u6027\u80fd\u5173\u7cfb\u7684\u8bb8\u591a\u57fa\u672c\u95ee\u9898\uff0c\u7279\u522b\u662f\u90a3\u4e9b\u4e0e\u6d3b\u6027\u7269\u8d28\u7684\u4f5c\u7528\u6709\u5173\u7684\u95ee\u9898\uff0c\u4ecd\u6709\u5f85\u56de\u7b54\u3002\u56fd\u5bb6\u7eb3\u7c73\u79d1\u5b66\u4e2d\u5fc3\u5510\u667a\u52c7\u6559\u6388\u8054\u5408\u4e2d\u56fd\u79d1\u5b66\u9662\u9ad8\u80fd\u7269\u7406\u7814\u7a76\u6240\u8463\u4fca\u624d\u7814\u7a76\u5458\u3001\u54c8\u5de5\u5927<a href=\"http:\/\/www.baidu.com\/link?url=k0cO2uGKtK5OMsZ9IH-xT2ZlcGS5EgmZOlu8S-qPUcqsnRmXMfFUhrK5fPzIndae7-Wl3iU-Vqkoycv_gOAkkK\">\u5218\u7ecd\u7434<\/a>\u6559\u6388\u901a\u8fc7\u539f\u4f4dX\u5c04\u7ebf\u5438\u6536\u5149\u8c31\u5206\u6790\u548c\u9ad8\u5206\u8fa8\u7387\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u6210\u50cf\uff0c\u7814\u7a76\u5c55\u793a\u4e86Ni<sub>0.5<\/sub>Co<sub>0.5<\/sub>-MOF-74\u5728OER\u8fc7\u7a0b\u4e2d\u7684\u7ed3\u6784\u8f6c\u53d8\u3002\u7814\u7a76\u8ba4\u4e3aNi<sub>0.5<\/sub>Co<sub>0.5<\/sub>OOH<sub>0.75<\/sub>\u5177\u6709\u4e30\u5bcc\u7684\u6c27\u7a7a\u4f4d\u548c\u9ad8\u6c27\u5316\u6001\uff0c\u5728\u539f\u4f4d\u5f62\u6210\uff0c\u662f\u89c2\u5bdf\u5230\u7684\u9ad8OER\u6d3b\u6027\u7684\u539f\u56e0\u3002\u53cc\u91d1\u5c5e\u4e2d\u5fc3\u4e2dNi\u4e0eCo\u7684\u6bd4\u4f8b\u6539\u53d8\u4e86\u5f62\u6210\u6d3b\u6027\u7269\u8d28\u7684\u51e0\u4f55\u7ed3\u6784\u548c\u7535\u5b50\u7ed3\u6784\uff0c\u8fdb\u800c\u6539\u53d8\u4e86\u50ac\u5316\u6d3b\u6027\u3002\u57fa\u4e8e\u5bf9\u8be5\u7cfb\u7edf\u7684\u7406\u89e3\uff0c\u5236\u4f5c\u4e86Ni<sub>0.9<\/sub>Fe<sub>0.1<\/sub>-MOF\uff0c\u572810 mA cm<sup>\u22122<\/sup>\u548c20 mA cm<sup>\u22122<\/sup>\u7684\u4f4e\u8fc7\u7535\u538b\u5206\u522b\u4e3a198 mV\u548c231 mV\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cStructural transformation of highly active metal\u2013organic framework electrocatalysts during the\u00a0oxygen evolution reaction\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nat. Energy\u4e0a\u3002DOI:\u00a010.1038\/s41560-020-00709-1<\/p>\n<p>\u56fe2\u00a0\u7ed3\u6784\u8868\u5f81\u548c\u7535\u5316\u5b66\u8bc4\u4ef7<\/p>\n<p><strong><b><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215347 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-2-21.png\" alt=\"\" width=\"600\" height=\"504\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-2-21.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-2-21-300x252.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/b><\/strong><\/p>\n<p><strong><b>Nat<\/b><\/strong><strong><b>. Mater<\/b><\/strong><strong><b>.\uff1a<\/b><\/strong><strong><b>\u76f4\u63a5X\u5c04\u7ebf\u548c\u7535\u5b50\u675f\u5149\u523b\u5364\u5316\u54aa\u5511\u6cb8\u77f3\u9aa8\u67b6<\/b><\/strong><\/p>\n<p>\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6\u6750\u6599\u7531\u4e8e\u5176\u72ec\u7279\u7684\u5fae\u5b54\u7279\u6027\uff0c\u5728\u5fae\u7535\u5b50\u548c\u5149\u7535\u5b50\u5b66\u9886\u57df\u5177\u6709\u98a0\u8986\u6027\u7684\u6f5c\u529b\u3002\u5728\u5fae\u578b\u5316\u7684\u56fa\u6001\u5668\u4ef6\u4e2d\uff0c\u7eb3\u7c73\u5c3a\u5ea6\u7684\u56fe\u5f62\u5316\u662f\u5b9e\u73b0MOFs\u7684\u4e00\u4e2a\u57fa\u672c\u6b65\u9aa4\u3002\u4f20\u7edf\u7684MOF\u6210\u50cf\u65b9\u6cd5\u5206\u8fa8\u7387\u4f4e\uff0c\u56fe\u50cf\u8fb9\u7f18\u6a21\u7cca\u3002\u5728\u8fd9\u91cc\uff0c\u6bd4\u5229\u65f6\u9c81\u6c76\u5927\u5b66\u7684Rob Ameloot\u6559\u6388\u56e2\u961f\u5c55\u793a\u65e0\u7535\u963b\u3001\u76f4\u63a5X\u5c04\u7ebf\u548c\u7535\u5b50\u675f\u5149\u523b\u7684MOFs\u3002\u8fd9\u4e00\u8fc7\u7a0b\u907f\u514d\u4e86\u8680\u523b\u635f\u4f24\u548c\u6c61\u67d3\uff0c\u5e76\u4f7f\u56fe\u6848MOFs\u7684\u5b54\u9699\u548c\u7ed3\u6676\u5ea6\u4fdd\u6301\u5b8c\u6574\u3002\u5f97\u5230\u7684\u9ad8\u8d28\u91cf\u56fe\u6848\u5177\u6709\u4f18\u5f02\u7684\u4e9a50nm\u5206\u8fa8\u7387\uff0c\u5e76\u63a5\u8fd1\u4e2d\u5b54\u72b6\u6001\u3002X\u5c04\u7ebf\u548c\u7535\u5b50\u675f\u5149\u523b\u6280\u672f\u4e0e\u73b0\u6709\u7684\u5fae\u3001\u7eb3\u7c73\u52a0\u5de5\u5de5\u827a\u7684\u517c\u5bb9\u5c06\u6709\u52a9\u4e8eMOFs\u5728\u5c0f\u578b\u5316\u8bbe\u5907\u4e2d\u7684\u96c6\u6210\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cDirect X-ray and electron-beam lithography of\u00a0halogenated zeolitic imidazolate frameworks\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nat. Mater.\u4e0a\u3002DOI: 10.1038\/s41563-020-00827-x<\/p>\n<p>\u56fe3\u00a0XRL\u548cEBL\u5bf9MOF\u8584\u819c\u7684\u76f4\u63a5\u6a21\u5f0f\u5316\u7814\u7a76<\/p>\n<p><strong><b><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215349 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-3-20.png\" alt=\"\" width=\"600\" height=\"809\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-3-20.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-3-20-222x300.png 222w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/b><\/strong><\/p>\n<p><strong><b>Nat<\/b><\/strong><strong><b>. Mater<\/b><\/strong><strong><b>.\uff1a<\/b><\/strong><strong><b>\u5bfc\u7535\u4e8c\u7ef4MOF\u7684\u539f\u5b50\u7ea7\u7cbe\u786e\u5355\u6676\u7ed3\u6784<\/b><\/strong><\/p>\n<p>\u5bfc\u7535\u4e8c\u7ef4\u91d1\u5c5e\u6709\u673a\u6846\u67b6(MOFs)\u7531\u4e8e\u5176\u516d\u8fb9\u5f62\u4e8c\u7ef4\u6676\u683c\u6a21\u62df\u77f3\u58a8\u548c\u5176\u4ed6\u4e8c\u7ef4\u8303\u5fb7\u534e\u5806\u79ef\u6750\u6599\u800c\u5f15\u8d77\u4e86\u5e7f\u6cdb\u7684\u5173\u6ce8\u3002\u7136\u800c\uff0c\u4e86\u89e3\u5b83\u4eec\u7684\u5185\u5728\u6027\u8d28\u4ecd\u7136\u662f\u4e00\u4e2a\u6311\u6218\uff0c\u56e0\u4e3a\u5b83\u4eec\u7684\u6676\u4f53\u592a\u5c0f\u6216\u8d28\u91cf\u592a\u5dee\uff0c\u65e0\u6cd5\u786e\u5b9a\u6676\u4f53\u7ed3\u6784\u3002\u5728\u8fd9\u91cc\uff0c\u7f8e\u56fd\u9ebb\u7701\u7406\u5de5\u5b66\u9662\u7684Mircea Dinc\u0103\u4ee5\u53ca\u5317\u4eac\u5927\u5b66\u7684\u5b59\u4fca\u826f\u6559\u6388\u7b49\u4eba\u62a5\u9053\u4e86\u4e00\u7c7b\u4e8c\u7ef4\u03c0\u5171\u8f6dMOF\u7684\u539f\u5b50\u7ea7\u7cbe\u786e\u7ed3\u6784\u3002\u8fd9\u7c7bMOF\u6750\u6599\u7531\u5c3a\u5bf8\u8fbe200\u5fae\u7c73\u7684\u5355\u6676\u884d\u751f\u800c\u6765\uff0c\u53ef\u901a\u8fc7\u9ad8\u5206\u8fa8\u884d\u5c04\u6280\u672f\u8fdb\u884c\u539f\u5b50\u7ea7\u5206\u8fa8\u7387\u7684\u5206\u6790\u3002\u7814\u7a76\u62a5\u9053\u4e24\u79cd\u5177\u6709\u7c7b\u4f3c\u4e8c\u7ef4\u8702\u7a9d\u72b6\u7247\u72b6\u7ed3\u6784\u7684\u6676\u4f53\u7ed3\u6784\u7c7b\u578b\uff0c\u4f46\u5177\u6709\u4e0d\u540c\u7684\u5145\u586b\u65b9\u5f0f\u548c\u5b54\u9699\u542b\u91cf\u3002\u5355\u6676\u7535\u8f93\u8fd0\u6d4b\u91cf\u660e\u663e\u5730\u663e\u793a\u4e86\u5782\u76f4\u4e8e\u548c\u5e73\u884c\u4e8e\u03c0\u5171\u8f6d\u8584\u7247\u7684\u5404\u5411\u5f02\u6027\u8f93\u8fd0\uff0c\u63ed\u793a\u4e86\u7edd\u5bf9\u7535\u5bfc\u7387\u548c\u91d1\u5c5e\u9633\u79bb\u5b50\u7684\u6027\u8d28\u4ee5\u53ca\u4e8c\u7ef4\u8584\u7247\u586b\u5145\u56fe\u6848\u4e4b\u95f4\u7684\u660e\u786e\u76f8\u5173\u6027\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cAtomically precise single-crystal structures\u00a0of electrically conducting 2D metal\u2013organic\u00a0frameworks\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nat.\u00a0Mater.\u4e0a\u3002DOI:\u00a010.1038\/s41563-020-00847-7<\/p>\n<p>\u56fe4\u00a0\u4e8c\u7ef4MOFs\u5355\u6676\u751f\u957f\u7684\u8bbe\u8ba1\u3001\u5408\u6210<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215350 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-4-20.png\" alt=\"\" width=\"600\" height=\"532\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-4-20.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-4-20-300x266.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Nat. Nanotech.\uff1a\u4e8c\u7ef4MOF\u89e3\u51b3\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u7a33\u5b9a\u6027\u548c\u94c5\u6cc4\u9732<\/b><\/strong><\/p>\n<p>\u5c3d\u7ba1\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u53d6\u5f97\u4e86\u663e\u8457\u7684\u8fdb\u5c55\uff0c\u4f46\u4fdd\u6301\u957f\u671f\u8fd0\u884c\u7684\u7a33\u5b9a\u6027\u548c\u6700\u5927\u9650\u5ea6\u5730\u51cf\u5c11\u6f5c\u5728\u7684\u94c5(Pb<sup>2+<\/sup>)\u79bb\u5b50\u6cc4\u6f0f\u4ecd\u662f\u4e24\u4e2a\u6709\u5f85\u89e3\u51b3\u7684\u6311\u6218\u3002\u5728\u8fd9\u91cc\uff0c\u9999\u6e2f\u57ce\u5e02\u5927\u5b66Alex K.-Y. Jen\uff0c\u6731\u5b97\u9f99\uff0c\u5f90\u653f\u6d9b\u6559\u6388\u7b49\u4f7f\u7528\u786b\u9187\u529f\u80fd\u5316\u6765\u89e3\u51b3\u8fd9\u4e9b\u95ee\u9898\uff0c\u4e8c\u7ef4\u5171\u8f6d\u91d1\u5c5e-\u6709\u673a\u6846\u67b6\u4f5c\u4e3a\u7535\u5b50\u63d0\u53d6\u5c42\u5728\u9499\u949b\u77ff\/\u9634\u6781\u754c\u9762\u3002\u8be5\u5668\u4ef6\u8868\u73b0\u51fa\u9ad8\u529f\u7387\u8f6c\u6362\u6548\u7387(22.02%)\u4ee5\u53ca\u663e\u8457\u6539\u5584\u7684\u957f\u671f\u8fd0\u884c\u7a33\u5b9a\u6027\u3002\u540c\u65f6\u663e\u8457\u6539\u5584\u4e86\u5176\u957f\u671f\u8fd0\u884c\u7a33\u5b9a\u6027\u3002\u572885\u00b0C\u4e0b\u6700\u5927\u529f\u7387\u70b9\u8ddf\u8e2a1000h\u7684\u8fde\u7eed\u5149\u7167\u7684\u52a0\u901f\u6d4b\u8bd5\u6761\u4ef6\u4e0b\uff0c\u4ecd\u80fd\u4fdd\u6301\u5176\u521d\u59cb\u6548\u7387\u768490%\u4ee5\u4e0a\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0c\u529f\u80fd\u5316\u7684\u91d1\u5c5e\u6709\u673a\u6846\u67b6\u53ef\u4ee5\u901a\u8fc7\u5f62\u6210\u4e0d\u6eb6\u4e8e\u6c34\u7684\u56fa\u4f53\u6765\u6355\u83b7\u5927\u90e8\u5206\u4ece\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u964d\u89e3\u6cc4\u6f0f\u7684Pb<sup>2+<\/sup>\u3002\u56e0\u6b64\uff0c\u8fd9\u79cd\u540c\u65f6\u89e3\u51b3\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u8fd0\u884c\u7a33\u5b9a\u6027\u548c\u94c5\u6c61\u67d3\u95ee\u9898\u7684\u65b9\u6cd5\uff0c\u53ef\u4ee5\u5927\u5927\u63d0\u9ad8\u9499\u949b\u77ff\u5149\u4f0f\u6280\u672f\u5927\u89c4\u6a21\u90e8\u7f72\u7684\u53ef\u884c\u6027\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201c2D metal\u2013organic framework for stable perovskite\u00a0solar cells with minimized lead leakage\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nat. Nanotech.\u4e0a\u3002DOI: 10.1038\/s41565-020-0765-7<\/p>\n<p>\u56fe5\u00a0ZrL3:bis-C60EELs\u00a0\u57faPVSCs\u7684\u5668\u4ef6\u7ed3\u6784\u4e0e\u6027\u80fd<\/p>\n<p><strong><b><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215351 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-5-23.png\" alt=\"\" width=\"600\" height=\"327\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-5-23.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-5-23-300x164.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/b><\/strong><\/p>\n<p><strong><b>Nat. Nanotech.\uff1a\u53ef\u9009\u62e9\u6e17\u900f<\/b><\/strong><strong><b>M<\/b><\/strong><strong><b>OF\u51dd\u80f6\u819c\u7528\u4e8e\u5b9e\u73b0\u53ef\u5145\u7535\u6709\u673a\u7535\u6c60\u7684\u957f\u5bff\u547d\u5faa\u73af<\/b><\/strong><\/p>\n<p>\u53ef\u5145\u7535\u6709\u673a\u7535\u6c60\u663e\u793a\u51fa\u5de8\u5927\u7684\u6f5c\u529b\uff0c\u4f5c\u4e3a\u4e00\u79cd\u4f4e\u6210\u672c\u3001\u53ef\u6301\u7eed\u548c\u53ef\u5927\u89c4\u6a21\u751f\u4ea7\u7684\u66ff\u4ee3\u73b0\u6709\u7684\u8fc7\u6e21\u91d1\u5c5e\u7535\u6c60;\u7136\u800c\uff0c\u4e25\u91cd\u7684\u7535\u6781\u6eb6\u89e3\u95ee\u9898\u548c\u6709\u673a\u6c27\u5316\u8fd8\u539f\u4e2d\u95f4\u4f53\u7684\u6eb6\u89e3(\u7a7f\u68ad\u6548\u5e94)\u5df2\u7ecf\u56f0\u6270\u8fd9\u4e9b\u7ec6\u80de\u7684\u5bb9\u91cf\u4fdd\u7559\u548c\u5faa\u73af\u80fd\u529b\u3002\u5728\u8fd9\u91cc\uff0c\u97e9\u56fd\u9996\u5c14\u5927\u5b66Kisuk Kang\u6559\u6388\u7b49\u4eba\u62a5\u9053\u4e86\u4f7f\u7528\u91d1\u5c5e\u6709\u673a\u6846\u67b6(MOF)\u51dd\u80f6\u819c\u4f5c\u4e3a\u6709\u673a\u7535\u6c60\u7684\u9694\u819c\u3002\u5747\u8d28\u5fae\u5b54\uff0cMOF-\u51dd\u80f6\u5206\u79bb\u5668\u7684\u56fa\u6709\u7279\u6027\uff0c\u4f5c\u4e3a\u9776\u5411\u6709\u673a\u4e2d\u95f4\u4f53\u7684\u6e17\u900f\u9009\u62e9\u6027\u901a\u9053\uff0c\u4ece\u800c\u5728\u4e0d\u727a\u7272\u529f\u7387\u7684\u60c5\u51b5\u4e0b\u7f13\u89e3\u4e86\u7a7f\u68ad\u95ee\u9898\u3002\u7814\u7a76\u7ed3\u679c\u663e\u793a\uff0c\u91c7\u7528MOF\u51dd\u80f6\u9694\u819c\u548c5\uff0c5\u2019-\u4e8c\u7532\u57fa-2\uff0c2\u2019-\u53cc\u5bf9\u82ef\u918c\uff08Me2BBQ\uff09\u4f5c\u4e3a\u7535\u6781\u7684\u7535\u6c60\u5177\u6709\u6781\u9ad8\u7684\u5faa\u73af\u7a33\u5b9a\u6027\uff0c2000\u6b21\u5faa\u73af\u540e\u5bb9\u91cf\u4fdd\u6301\u7387\u4e3a82.9%\uff0c\u5bb9\u91cf\u8870\u51cf\u7387\u4e3a0.008%\uff0c\u653e\u7535\u5bb9\u91cf\u4e3a171 mA\u00a0h\u00a0g<sup>\u2212<\/sup><sup>1<\/sup>\uff0c\u7535\u6d41\u5bc6\u5ea6\u4e3a300\u2009mA\u2009g<sup>\u2212<\/sup><sup>1<\/sup>\u3002MOF-\u51dd\u80f6\u5206\u79bb\u5668\u7684\u5206\u5b50\u548c\u79bb\u5b50\u7b5b\u5206\u80fd\u529b\u5177\u6709\u901a\u7528\u6027\uff0c\u56e0\u4e3a\u5176\u5b54\u5f84\u53ef\u4ee5\u8c03\u6574\u5230\u7279\u5b9a\u7684\u6709\u673a\u7535\u6781\u6750\u6599\u3002\u5229\u7528MOF-\u51dd\u80f6\u9694\u677f\u9632\u6b62\u53ef\u6eb6\u6709\u673a\u6c27\u5316\u8fd8\u539f\u4e2d\u95f4\u4f53\u7684\u526f\u53cd\u5e94\uff0c\u53ef\u5f00\u53d1\u51fa\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u548c\u957f\u5faa\u73af\u5bff\u547d\u7684\u53ef\u5145\u7535\u6709\u673a\u7535\u6c60\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cPermselective metal\u2013organic framework gel\u00a0membrane enables long-life cycling of\u00a0rechargeable organic batteries\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nat. Nanotech.\u4e0a\u300210.1038\/s41565-020-00788-x<\/p>\n<p>\u56fe6\u00a0\u53ef\u5145\u7535\u6709\u673a\u7535\u6c60\u4e2dMOF-\u51dd\u80f6\u9694\u677f\u7684\u793a\u610f\u56fe<\/p>\n<p><strong><b><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215352 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-6-18.png\" alt=\"\" width=\"600\" height=\"382\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-6-18.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-6-18-300x191.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/b><\/strong><\/p>\n<p><strong><b>Nat<\/b><\/strong><strong><b>. Commun<\/b><\/strong><strong><b>.\uff1a<\/b><\/strong><strong><b>\u7528\u4e8e\u4e59\u7094\/\u4e59\u70ef\u5206\u79bb<\/b><\/strong><strong><b>\u7684<\/b><\/strong><strong><b>\u53ef\u8c03\u8282\u5c42\u95f4\u548c\u5c42\u5185\u7a7a\u95f4\u7684\u4e8c\u7ef4MOFs<\/b><\/strong><\/p>\n<p>\u4e09\u7ef4\u91d1\u5c5e-\u6709\u673a\u6846\u67b6(MOFs)\u662f\u5438\u9644\u53bb\u9664\u5fae\u91cf\u6c14\u4f53\u7684\u5c16\u7aef\u6750\u6599\uff0c\u7531\u4e8e\u5176\u4e30\u5bcc\u7684\u5b54\u9699\u5177\u6709\u7279\u5b9a\u7684\u5316\u5b66\u6027\u8d28\u3002\u7136\u800c\uff0c\u5f00\u53d1\u9ad8\u5438\u9644\u5bb9\u91cf\u3001\u9ad8\u9009\u62e9\u6027\u3001\u9ad8\u7a33\u5b9a\u6027\u7684\u7406\u60f3\u5438\u9644\u5242\u4ecd\u662f\u4e00\u4e2a\u6311\u6218\u3002\u5728\u8fd9\u91cc\uff0c\u6d59\u6c5f\u5927\u5b66\u6768\u542f\u709c\u56e2\u961f\u5c55\u793a\u4e86\u4e00\u79cd\u8bbe\u8ba1\u5438\u9644\u5242\u7684\u7b56\u7565\uff0c\u5229\u7528\u4e8c\u7ef4\u6c1f\u5316MOFs\u5c42\u95f4\u548c\u5c42\u5185\u7a7a\u95f4\u7684\u53ef\u8c03\u6027\u6765\u6355\u83b7\u4e59\u70ef\u4e2d\u7684\u4e59\u7094\u3002\u901a\u8fc7X\u5c04\u7ebf\u884d\u5c04\u548c\u6a21\u578b\u9a8c\u8bc1\uff0c\u8fde\u63a5\u5242\u539f\u5b50\u6c27\u5316\u6001\u7684\u7cfb\u7edf\u53d8\u5316\u80fd\u591f\u5bf9\u5c42\u5806\u79ef\u6a21\u5f0f\u548c\u8fde\u63a5\u5242\u6784\u8c61\u8fdb\u884c\u7cbe\u7ec6\u8c03\u63a7\uff0c\u4ece\u800c\u5b9e\u73b0\u5206\u5b50\u7684\u5c42\u95f4\u6355\u83b7\u548c\u5c42\u5185\u534f\u540c\u7ed3\u5408\u3002\u5728\u5de5\u4e1a\u4e0a\u5e38\u7528\u76840.001\u20130.05 bar\u538b\u529b\u8303\u56f4\u5185\uff0cZUL-100\u548cZUL-200\u8868\u73b0\u51fa\u9ad8\u9009\u62e9\u6027\u3002\u7a81\u7834\u6027\u7684\u5b9e\u9a8c\u8bc1\u5b9e\u4e86\u5b83\u4eec\u5728\u4e59\u7094\/\u4e59\u70ef\u5206\u79bb\u65b9\u9762\u7684\u6548\u7387\uff0c\u5373\u4f7f\u5728\u6f6e\u6e7f\u7684\u6761\u4ef6\u4e0b\u5faa\u73af\uff0c\u4e59\u70ef\u4ea7\u7387\u4e5f\u975e\u5e38\u9ad8(\u4ece1\/99\u7684\u6df7\u5408\u7269\u4e2d\u5f97\u5230121mmol\/g, 99.9999%)\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cSimultaneous interlayer and intralayer space control in two-dimensional metal\u2212organic frameworks for acetylene\/ethylene separation\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nat. Commun.\u4e0a\u3002DOI:\u00a010.1038\/s41467-020-20101-7<\/p>\n<p>\u56fe7\u00a0MOFs\u7684\u8868\u9762\u9759\u7535\u52bf\u548cC<sub>2<\/sub>H<sub>2<\/sub>\u5438\u9644\u7b49\u6e29\u7ebf<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215353 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-7-13.png\" alt=\"\" width=\"600\" height=\"334\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-7-13.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-7-13-300x167.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong><b>Nat<\/b><\/strong><strong><b>. Commun<\/b><\/strong><strong><b>.\uff1aM<\/b><\/strong><strong><b>OF\u5bbf\u4e3b\u52a8\u529b\u5b66\u7684\u5dee\u5f02\u5ba2\u4f53\u4f4d\u7f6e\u589e\u5f3a\u4e19\u70ef\/\u4e19\u70f7\u7684\u5206\u79bb<\/b><\/strong><\/p>\n<p>\u8282\u80fd\u7684\u65b9\u6cd5\u6765\u5206\u79bb\u4e19\u70ef\/\u4e19\u70f7\uff0c\u5982\u5206\u5b50\u7b5b\u5206\u662f\u76f8\u5f53\u91cd\u8981\u5728\u77f3\u5316\u5de5\u4e1a\u3002\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6NbOFFIVE-1-Ni\u5728\u5ba4\u6e29\u548c\u5e38\u538b\u4e0b\u5438\u9644\u4e19\u70ef\uff0c\u800c\u4e0d\u5438\u9644\u4e19\u70f7\uff0c\u800c\u540c\u7ed3\u6784\u7684SIFSIX -3-Ni\u5728\u76f8\u540c\u6761\u4ef6\u4e0b\u4e0d\u6392\u9664\u4e19\u70f7\u3002\u4e24\u79cd\u6750\u6599\u7684\u5b54\u9699\u5f00\u53e3\u7684\u9759\u6001\u5c3a\u5bf8\u90fd\u592a\u5c0f\uff0c\u4e0d\u80fd\u5bb9\u7eb3\u4efb\u4f55\u4e00\u4e2a\u5ba2\u4f53\uff0c\u8fd9\u8868\u660e\u4e86\u4e3b\u4f53\u52a8\u529b\u5bf9\u4e8e\u5ba2\u4f53\u8fdb\u5165\u548c\u901a\u8fc7\u901a\u9053\u8fd0\u8f93\u7684\u91cd\u8981\u6027\u3002\u82f1\u56fd\u5229\u7269\u6d66\u5927\u5b66Matthew S. Dyer\u6559\u6388\u7b49\u4eba\u4f7f\u7528\u4ece\u5934\u8ba1\u7b97\u7ed3\u5408\u6676\u4f53\u5b66\u548c\u5438\u9644\u5b66\u6570\u636e\u6765\u8868\u660e\u4e24\u4e2a\u6846\u67b6\u5f62\u6210\u5355\u5143\uff0c\u591a\u539f\u5b50\u9634\u79bb\u5b50\u548c\u5421\u55ea\uff0c\u63a7\u5236\u6269\u6563\u548c\u5206\u79bb\u7684\u52a8\u529b\u5b66\u3002\u5ba2\u4f53\u6269\u6563\u662f\u901a\u8fc7\u6253\u5f00\u7531\u56db\u79cd\u5421\u55ea\u5f62\u6210\u7684\u67d4\u6027\u7a97\u53e3\u53d1\u751f\u7684\u3002\u5728NbOFFIVE-1-Ni\u4e2d\uff0c(NbOF<sub>5<\/sub>) <sup>2-<\/sup>\u8d1f\u79bb\u5b50\u5b9a\u4f4d\u4f7f\u4e19\u70f7\u8fdc\u79bb\u7a97\u53e3\uff0c\u4ece\u800c\u589e\u5f3a\u4e86\u4e19\u70ef\/\u4e19\u70f7\u7684\u5206\u79bb\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cDifferential guest location by host dynamics\u00a0enhances propylene\/propane separation\u00a0in a metal-organic framework\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Nat. Commun.\u4e0a\u3002DOI:\u00a010.1038\/s41467-020-19207-9<\/p>\n<p>\u56fe8\u00a0[Ni(NbOF<sub>5<\/sub>)(C<sub>4<\/sub>H<sub>4<\/sub>N<sub>2<\/sub>)<sub>2<\/sub>]\u7ed3\u6784<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-215354 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-8-13.png\" alt=\"\" width=\"600\" height=\"345\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-8-13.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2020\/12\/\u56fe\u7247-8-13-300x173.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u6587\u4e2d\u6240\u8ff0\u5982\u6709\u4e0d\u59a5\u4e4b\u5904\uff0c\u6b22\u8fce\u8bc4\u8bba\u533a\u7559\u8a00~<\/p>\n<p>\u672c\u6587\u7531Junas\u4f9b\u7a3f\u3002<\/p>\n<p>\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n<p>\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n<p>\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n<p>\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaorenVIP\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"<p>Nat. Chem.\uff1a\u8868\u73b0\u51fa\u4e8c\u6c27\u5316\u78b3\u8bf1\u5bfc\u7684\u987a\u78c1\u6027\u548c\u4e9a\u78c1\u6027\u4e4b\u95f4\u7684\u8f6c\u53d8MOF \u5982\u679c\u6709\u8db3\u591f\u7684\u6784\u9020\u5757\uff0c\u91d1\u5c5e\u6709\u673a\u6846\u67b6(MOFs)\u53ef\u4ee5\u7ed3\u5408\u78c1\u6027\u6392\u5e8f\u548c\u5b54\u9699\u7387\u3002\u8fd9\u4f7f\u5f97MOFs\u662f&#8230;<\/p>\n","protected":false},"author":11454,"featured_media":215360,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[1187],"tags":[],"class_list":["post-215345","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-zhuanlan"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/215345"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/11454"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=215345"}],"version-history":[{"count":2,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/215345\/revisions"}],"predecessor-version":[{"id":215740,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/215345\/revisions\/215740"}],"wp:featuredmedia":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/media\/215360"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=215345"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=215345"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=215345"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}