{"id":219262,"date":"2021-03-18T12:00:50","date_gmt":"2021-03-18T04:00:50","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=219262"},"modified":"2021-03-18T11:27:00","modified_gmt":"2021-03-18T03:27:00","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e4%b8%ad%e7%a7%91%e9%99%a2%e5%8c%96%e5%ad%a6%e6%89%80%e5%ae%8b%e5%bb%b6%e6%9e%97%e6%9d%8e%e6%98%8e%e7%8f%a0%e6%b5%99%e6%b1%9f%e5%a4%a7%e5%ad%a6","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=219262","title":{"rendered":"\u4e2d\u79d1\u9662\u5316\u5b66\u6240\u5b8b\u5ef6\u6797&\u674e\u660e\u73e0&\u6d59\u6c5f\u5927\u5b66\u6c99\u5a01\u56e2\u961fAdv. Mater.\uff1a\u5f69\u8272\u7684\u9ad8\u6548\u83ab\u5c14\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u6709\u673a-\u65e0\u673a\u6742\u5316\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\uff08PSCs\uff09\u7531\u4e8e\u5177\u6709\u5927\u5438\u6536\u7cfb\u6570\u3001\u957f\u8f7d\u6d41\u5b50\u6269\u6563\u957f\u5ea6\u3001\u8f83\u5c11\u6676\u754c\u548c\u7f3a\u9677\u7684\u5927\u6676\u7c92\u5c3a\u5bf8\u7b49\u4f18\u826f\u7684\u5149\u7535\u7279\u6027\uff0c\u4ee5\u53ca\u4e0e\u7845\u592a\u9633\u80fd\u7535\u6c60\u76f8\u6bd4\u751f\u4ea7\u6210\u672c\u4f4e\u7b49\u7279\u70b9\uff0c\u53ef\u53d1\u5c55\u6210\u4e3a\u6027\u80fd\u4f18\u8d8a\u7684\u8584\u819c\u5149\u4f0f\u5668\u4ef6\u3002\u6700\u8fd1\uff0cPSCs\u7684\u529f\u7387\u8f6c\u6362\u6548\u7387\uff08PCE\uff09\u5df2\u63d0\u9ad8\u5230\u8ba4\u8bc1\u6548\u7387\u768425.5%\u3002\u5728\u5f00\u53d1\u66f4\u8f7b\u3001\u66f4\u8584\u3001\u66f4\u9ad8\u6548\u7684PSCs\u7684\u540c\u65f6\uff0c\u4e3a\u4e86\u5c06\u6765\u7684\u91cf\u4ea7\uff0c\u4eba\u4eec\u8fd8\u5728\u51cf\u5c11\u6750\u6599\u7528\u91cf\uff08\u5c24\u5176\u662f\u51cf\u5c11\u94c5\u7684\u7528\u91cf\uff09\u548c\u751f\u4ea7\u6210\u672c\u65b9\u9762\u505a\u4e86\u8bb8\u591a\u52aa\u529b\u3002\u867d\u7136\u9499\u949b\u77ff\u662f\u4e00\u79cd\u4f18\u826f\u7684\u5149\u7535\u6750\u6599\uff0c\u4f46\u5176PCE\u4ecd\u4f4e\u4e8e\u5176\u7406\u8bba\u6781\u9650\u503c\u3002\u7279\u522b\u662f\u670935%\u7684\u5149\u635f\u5931\uff0c\u5305\u62ec14%\u88ab\u5bfc\u7535\u57fa\u677f\uff08FTO\u3001ITO\uff09\u5438\u6536\uff0c4%\u88ab\u73bb\u7483\u57fa\u677f\u8868\u9762\u53cd\u5c04\uff0c2%\u5728\u529f\u80fd\u5c42\uff08\u7535\u5b50\u4f20\u8f93\u5c42\u3001\u7a7a\u7a74\u4f20\u8f93\u5c42\u548c\u7535\u6781\u5c42\uff09\u635f\u5931\uff0c15%\u4ecePSCs\u9038\u51fa\u3002\u6709\u6548\u7684\u5149\u5b50\u7ba1\u7406\u6709\u671b\u901a\u8fc7\u6784\u7b51\u6355\u5149\u7eb3\u7c73\u7ed3\u6784\u5c06\u5149\u5bcc\u96c6\u5230\u5438\u6536\u5c42\uff0c\u5e76\u5ef6\u957f\u5149\u8def\uff0c\u4ece\u800c\u589e\u52a0\u5149\u8f7d\u6d41\u5b50\u7684\u6570\u91cf\uff0c\u4f7f\u5149\u7535\u6d41\u548cPCE\u5f97\u5230\u63d0\u5347\uff0c\u5e76\u6709\u671b\u5b9e\u73b0\u4f4e\u6210\u672c\u7684\u9ad8\u6548\u8584\u578bPSCs\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5728\u4e2d\u56fd\u79d1\u5b66\u9662\u5316\u5b66\u7814\u7a76\u6240\u5b8b\u5ef6\u6797\u7814\u7a76\u5458<\/b><\/strong>\u548c\u674e\u660e\u73e0\u7814\u7a76\u5458\u3001\u6d59\u6c5f\u5927\u5b66\u6c99\u5a01\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005<\/b><\/strong>\uff09\u56e2\u961f\u7b49\u4eba\u5e26\u9886\u4e0b\uff0c\u6c6a\u6d0b\u535a\u58eb\u00a0\u7b49\u901a\u8fc7\u538b\u5370\u65b9\u6cd5\uff0c\u501f\u52a9\u5546\u7528DVD\u5149\u76d8\uff0c\u8bbe\u8ba1\u5e76\u5236\u9020\u51fa\u5177\u6709\u83ab\u5c14\u5e72\u6d89\u7ed3\u6784\u7684\u5f69\u8272\u9ad8\u6548\u83ab\u5c14PSCs\u3002\u4ece\u5b9e\u9a8c\u548c\u7406\u8bba\u8bc1\u660e\uff0c\u901a\u8fc7\u6539\u53d8\u65cb\u8f6c\u89d2\u5ea6\uff080\u00b0\u201390\u00b0\uff09\uff0c\u53ef\u4ee5\u6709\u6548\u5730\u63a7\u5236\u83ab\u5c14\u5e72\u6d89\u7ed3\u6784\u7684\u5149\u5bcc\u96c6\u80fd\u529b\u3002\u589e\u5f3a\u7684\u77ed\u8def\u7535\u6d41\u5f52\u56e0\u4e8e\u589e\u52a0\u4e86\u5149\u884d\u5c04\u901a\u9053\uff0c\u5ef6\u957f\u5165\u5c04\u5149\u5149\u8def\uff0c\u5e76\u5c06\u5165\u5c04\u5149\u5bcc\u96c6\u5230\u9499\u949b\u77ff\u5c42\u4e2d\u3002\u6b64\u5916\uff0c\u538b\u5370\u8fc7\u7a0b\u6291\u5236\u4e86\u6d3b\u6027\u5c42\u754c\u9762\u7684\u7f3a\u9677\u548c\u7a7a\u6d1e\uff0c\u6d88\u9664\u4e86\u6ede\u540e\u3002\u83ab\u5c14PSCs\u5177\u6709\u4f18\u5316\u768430\u00b0\u65cb\u8f6c\u89d2\u5ea6\uff0c\u53ef\u5b9e\u73b0\u6700\u4f73\u7684\u5149\u6536\u96c6\u589e\u5f3a\u6548\u679c\uff08\u6bd4\u539f\u59cb\u9ad828.5\uff05\uff09\uff0c\u4f7f\u6548\u7387\u8d85\u8fc720.17\uff05\uff08MAPbI3<\/sub>\uff09\u548c21.76\uff05\uff08(FAPbI3<\/sub>)1\u2010x<\/sub>\u00a0(MAPbBr3<\/sub>)x<\/sub>\uff09\u3002\u8be5\u6210\u679c\u4ee5\u9898\u4e3a\u201cColorful Efficient Moir\u00e9-Perovskite Solar Cells<\/b><\/strong>\u201d\u53d1\u8868\u5728\u4e86Adv. Mater.<\/b><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe1 \u5546\u7528DVD\u5149\u76d8<\/b><\/strong>\u538b\u5370<\/b><\/strong>\u6469\u5c14PSCs\u7684\u793a\u610f\u56fe<\/b><\/strong>\"\"<\/p>\n

a\uff09\u5177\u6709\u6709\u6548\u5149\u5438\u6536\u7684PSCs\u7684\u793a\u610f\u56fe\u3002\u56e0\u7f3a\u4e4f\u6709\u6548\u7684\u5149\u6355\u83b7\u7ed3\u6784, \u5927\u91cf\u7684\u5149\u5728\u9499\u949b\u77ff\u5149\u7535\u5668\u4ef6\u4e2d\u88ab\u6d6a\u8d39\u3002<\/p>\n

b\uff09\u5177\u6709\u53cc\u884d\u5c04\u5149\u6805\u7684PSCs\u7684\u793a\u610f\u56fe\u3002<\/p>\n

c\uff09\u83ab\u5c14PSCs\u5177\u6709\u4e0d\u540c\u76f8\u4ea4\u89d2\u5ea6\uff0c\u4ee5\u63d0\u9ad8\u5149\u6536\u96c6\u6548\u7387\u3002<\/p>\n

d\uff09\u5468\u671f\u22480.75\u00b5m\uff0c\u5bbd\u5ea6\u22480.25\u00b5m\uff0c\u9ad8\u5ea6\u22480.1\u00b5m\u7684PVK\u5149\u6805\u7ed3\u6784\u9499\u949b\u77ff\u8584\u819c\u7684AFM\u56fe\u50cf\u3002<\/p>\n

e\uff0cf\uff09\u4f7f\u7528\u53cc\u884d\u5c04\u5149\u6805\u7684\u83ab\u5c14\u9499\u949b\u77ff\u8584\u819c\u7684\u5149\u675f\u56fe\u50cf\uff0c\u5728532nm\u5904\u89c2\u5bdf\u5230\u884d\u5c04\uff08e\uff1a\u4fa7\u89c6\u56fe\uff0cf\uff1a\u6b63\u89c6\u56fe\uff09\u3002\u5b83\u6709\u4e09\u7ec4\u884d\u5c04\u5149\u675f\u548c\u884d\u5c04\u70b9\u3002<\/p>\n

\u56fe2 \u83ab\u5c14\u9499\u949b\u77ff\u8584\u819c\u7684\u5149\u5b66\u8868\u5f81<\/b><\/strong>\"\"<\/p>\n

a\uff09\u4e24\u4e2a\u5468\u671f\u6027\u7ed3\u6784\u76f8\u4e92\u5e72\u6270\u9020\u6210\u7684\u83ab\u5c14\u56fe\u50cf\u3002<\/p>\n

b\uff09\u901a\u8fc7\u5c06\u4e24\u4e2a\u884d\u5c04\u5149\u6805\u4ece0\u00b0\u65cb\u8f6c\u523090\u00b0\u6765\u5236\u5907\u83ab\u5c14PSCs\u3002\u83ab\u5c14\u5468\u671f\u53d6\u51b3\u4e8e\u4e24\u4e2a\u5149\u6805\u4e4b\u95f4\u7684\u65cb\u8f6c\u89d2\u5ea6\u3002<\/p>\n

c\uff09\u83ab\u5c14\u5468\u671f\u4e0e\u65cb\u8f6c\u89d2\u5ea6\u7684\u76f8\u56fe\uff08\u4ece0\u00b0\u523090\u00b0\uff09\u548c\u83ab\u5c14\u56fe\u6848\u5f62\u6210\u7684\u793a\u610f\u56fe\uff08\u63d2\u56fe\uff08c\uff09\uff09\u3002\u83ab\u5c14\u5468\u671f\u968f\u7740\u65cb\u8f6c\u89d2\u7684\u589e\u52a0\u800c\u51cf\u5c0f\u3002<\/p>\n

d\uff09\u83ab\u5c14\u884d\u5c04\u7684\u65cb\u8f6c\u89d2\u5ea6\u4e0e\u5165\u5c04\u6ce2\u957f\u7684\u5173\u7cfb\u56fe\u3002\u4ece5\u00b0\u523055\u00b0\u7684\u65cb\u8f6c\u89d2\u5ea6\u786e\u4fdd\u83ab\u5c14\u5149\u884d\u5c04\u8986\u76d6\u5bbd\u7684\u5165\u5c04\u6ce2\u957f\uff08400-800 nm\uff09\u3002<\/p>\n

e\uff09\u8ba1\u7b97\u4e86\u4e24\u4e2a\u5165\u5c04\u6ce2\u957f\uff08500\u548c700 nm\uff09\u4e0b\uff0c\u4ece0\u00b0\u523070\u00b0\u7684\u5149\u5438\u6536\u4e0e\u65cb\u8f6c\u89d2\u5ea6\u7684\u5173\u7cfb\u3002<\/p>\n

f\uff09\u6d4b\u91cf\u83ab\u5c14\u9499\u949b\u77ff\u8584\u819c\u7684\u53cd\u5c04\u7387\u548cLHE\u3002\u83ab\u5c14\u9499\u949b\u77ff\u8584\u819c\u63d0\u9ad8\u4e86\u957f\u6ce2\u957f\u8303\u56f4\uff08\u03bb> 700 nm\uff09\u7684\u5149\u6355\u83b7\u6548\u7387\u548c\u5149\u6355\u83b7\u80fd\u529b\u3002\u00a0<\/p>\n

g\uff09\u76f8\u5bf9\u4e8e\u975e\u504f\u632f\u5165\u5c04\u5149\u675f\uff08532 nm\uff09\u7684\u5149\u529f\u7387\uff08dB\uff09\uff0c\u572830\u00b0\u65cb\u8f6c\u89d2\u4e0b\u8fdb\u5165\u83ab\u5c14PSC\u3002<\/p>\n

h\uff09\u8003\u8651\u5230PSCs\u7684\u53cd\u5c04\u635f\u8017\u3001EQE\u3001Yablonovitch 4n2<\/sup>\u6781\u9650\u548c4n2<\/sup>\u6781\u9650\u3002\u7531\u4e8e\u83ab\u5c14\u884d\u5c04\u5149\u6805\u8026\u5408\u6548\u5e94\u63d0\u9ad8LHE\uff0c\u5728\u957f\u6ce2\u957f\uff08\u03bb> 700 nm\uff09\u8303\u56f4\u5185\uff0c\u83ab\u5c14PSCs\u7684EQE\u5f97\u5230\u4e86\u589e\u5f3a\u3002<\/p>\n

\u56fe3 \u91c7\u7528\u4e0d\u540c\u5149\u6355\u83b7\u7ed3\u6784\u7684PSCs\u5149\u5438\u6536\u76843D FDTD\u6a21\u62df<\/b><\/strong>\"\"<\/p>\n

\u5149\u6805\u5468\u671f\u662f750nm\u3002\u6ce2\u957f\u4e3a500\u3001600\u3001700\u548c750 nm\u7684xz\u9762\u7535\u78c1\u80fd\u91cf\u5bc6\u5ea6\u7684\u7a7a\u95f4\u5206\u5e03\uff1aa\uff09\u53c2\u7167\u6837\u53c2\u7167\u6837\uff0cb\uff09D-TiO2<\/sub>\uff0cc\uff09D-\u9499\u949b\u77ff\uff0cd\uff09\u83ab\u5c14\u9499\u949b\u77ff\u8584\u819c\u3002\u83ab\u5c14\u9499\u949b\u77ff\u8584\u819c\u7684\u8be6\u7ec6\u53c2\u6570\u5305\u62ec\u572825 nm\u81f4\u5bc6TiO2<\/sub>\u5c42\uff0c\u00a0180 nm\u7684\u4ecb\u5b54TiO2<\/sub>\u3002\u5728meso-TiO2<\/sub>\/PVK\u754c\u9762\u5904\u6709\u6df1\u5ea680 nm\u7684\u5149\u6805\uff0c\u00a0330 nm\u7684PVK\u3002\u00a0Spiro-OMeTAD\u539a\u5ea6\u4e3a300 nm\u7684\u6ce2\u7eb9\uff0c\u5305\u62ecPVK\/Spiro\u754c\u9762\u7684\u5149\u6805\u6df1\u5ea6100 nm\u3002\u4e0e\u5176\u4ed6\u6837\u54c1\uff08\u539f\u59cb\u3001D-TiO2<\/sub>\u3001D-\u9499\u949b\u77ff\u8584\u819c\uff09\u76f8\u6bd4\uff0c\u83ab\u5c14\u9499\u949b\u77ff\u8584\u819c\u83b7\u5f97\u4e86\u6700\u5f3a\u7684\u5438\u6536\uff0c\u8fd9\u662f\u7531\u4e8e\u83ab\u5c14\u884d\u5c04\u5149\u6805\u7684\u8026\u5408\u6548\u5e94\u6240\u81f4\u3002<\/p>\n

\u56fe4 \u83ab\u5c14\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u5149\u7535\u6027\u80fd<\/b><\/strong>\"\"<\/p>\n

a\uff09\u5f69\u8272PSCs\u7684\u89c6\u89c9\u6548\u679c\u3002<\/p>\n

b\uff09\u83ab\u5c14PSCs\u4e0eMAPbI3<\/sub>\u548c(FAPbI3<\/sub>)1\u2010x<\/sub>(MAPbBr3<\/sub>)x<\/sub>\u9499\u949b\u77ff\u6d3b\u6027\u5c42\u7684\u7684J-V\u7279\u6027\u3002\u5bf9\u4e8eMAPbI3<\/sub>\uff0c\u83ab\u5c14PSCs\u7684PCE\uff0820.17\uff05\uff09\u9ad8\u4e8e\u53c2\u7167\u6837\uff0817.42\uff05\uff09\u3002\u5bf9\u4e8e(FAPbI3<\/sub>)1\u2010x<\/sub>(MAPbBr3<\/sub>)x<\/sub>\uff0c\u83ab\u5c14PSCs\u7684PCE\uff0821.76\uff05\uff09\u9ad8\u4e8e\u53c2\u7167\u6837\uff0819.11\uff05\uff09\u3002<\/p>\n

c\uff09PSCs\u7684J-V\u78c1\u6ede\u3002\u83ab\u5c14PSCs\u663e\u793a\u51fa\u53ef\u5ffd\u7565\u7684\u5149\u7535\u6d41\u6ede\u540e\u3002<\/p>\n

d\uff0ce\uff09\u5229\u7528MAPbI3<\/sub>\u5bf9PSCs\u7684J-V\u7279\u6027\u8fdb\u884c\u5b9e\u9a8c\u6d4b\u91cf\u548c\u7406\u8bba\u62df\u5408\u3002<\/p>\n

f\uff09PSCs\u7684Voc<\/sub>\u4e0e\u5149\u5f3a\u5ea6\u7684\u5173\u7cfb\u3002<\/p>\n

g\uff0ch\uff09\u5728\u5149\u5f3a\u5ea6\u4e3a100 mW cm-2<\/sup>\u7684480\u00a0nm\u548c650\u00a0nm\u7167\u5c04\u4e0b\uff0cPSCs\u7684J-V\u78c1\u6ede\u6d4b\u91cf\u3002<\/p>\n

i\uff09\u6700\u5927\u8f93\u51fa\u529f\u7387\u70b9\u7684\u7535\u6d41\u5bc6\u5ea6\u548c\u76f8\u5e94\u7684PCE\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>Colorful Efficient Moir\u00e9-Perovskite Solar Cells<\/u><\/a>\uff08Adv. Mater.\uff0c2021\uff0cDOI:10.1002\/adma.202008091\uff09<\/p>\n

\u672c\u6587\u7531\u6728\u6587\u97ec<\/b><\/strong>\u7ffb\u8bd1\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

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