{"id":220660,"date":"2021-04-18T06:39:39","date_gmt":"2021-04-17T22:39:39","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=220660"},"modified":"2021-04-17T20:39:51","modified_gmt":"2021-04-17T12:39:51","slug":"nature-energy%ef%bc%9a%e5%ae%89%e6%97%b6%ef%bc%88ah%ef%bc%89%e7%ba%a7%e5%88%ab%e7%9a%84%e7%9a%84%e9%94%8c%e7%a9%ba%e6%b0%94%e8%bd%af%e5%8c%85%e7%94%b5%e6%b1%a0","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=220660","title":{"rendered":"Nature Energy\uff1a\u5b89\u65f6\uff08Ah\uff09\u7ea7\u522b\u7684\u7684\u950c\u7a7a\u6c14\u8f6f\u5305\u7535\u6c60"},"content":{"rendered":"<p>\u7b2c\u4e00\u4f5c\u8005\uff1aSambhaji S. Shinde<\/p>\n<p>\u901a\u8baf\u4f5c\u8005\uff1aSang Uck Lee\uff0cand Jung-Ho Lee<\/p>\n<p>\u901a\u8baf\u5355\u4f4d\uff1a\u97e9\u56fd\u6c49\u9633\u5927\u5b66<\/p>\n<p>DOI\uff1ahttps:\/\/doi.org\/10.1038\/s41560-021-00807-8<\/p>\n<p><strong>\u80cc\u666f<\/strong><\/p>\n<p>\u76ee\u524d\uff0c\u5168\u56fa\u6001\u950c\u7a7a\u6c14\u8f6f\u5305\u7535\u6c60\u53ef\u4ee5\u4fdd\u8bc1\u9ad8\u7684\u80fd\u91cf\u6210\u672c\u6bd4\u548c\u5185\u5728\u5b89\u5168\u6027\u3002\u7136\u800c\uff0c\u5bfb\u627e\u81ea\u7136\u754c\u5bcc\u542b\u7684\u9ad8\u529f\u7387\/\u80fd\u91cf\u6bd4\u8d1f\u6781\u6750\u6599\u548c\u8d85\u79bb\u5b50\u7535\u89e3\u8d28\u4ecd\u7136\u662f\u4e00\u4e2a\u6781\u5927\u7684\u6311\u6218\u3002<\/p>\n<p><strong>\u7814\u7a76\u7684\u95ee\u9898<\/strong><\/p>\n<p>\u672c\u6587\u4ecb\u7ecd\u4e86\u7531(101)\u9762\u78f7\u786b\u5316\u94dc[CPS(101)]\u4f5c\u4e3a\u8d1f\u6781\u7684\u950c\u7a7a\u6c14\u8f6f\u5305\u7535\u6c60\uff0c\u4ee5\u53ca\u4f5c\u4e3a\u8d85\u79bb\u5b50\u5bfc\u4f53\u7535\u89e3\u8d28\u7684\u9632\u51bb\u58f3\u805a\u7cd6-\u751f\u7269\u7ea4\u7ef4\u7d20\u3002\u672c\u6587\u6240\u63d0\u51fa\u7684\u6c2f\u5316\u77f3\u8721(101)\u5bf9\u53ef\u9006\u6c27\u53cd\u5e94\u548c\u6790\u6c22\u53cd\u5e94\u8868\u73b0\u51fa\u4e09\u5143\u6d3b\u6027\u548c\u7a33\u5b9a\u6027(&gt; 30000\u4e2a\u5faa\u73af)\uff0c\u8fd9\u660e\u663e\u4f18\u4e8e\u5546\u4e1a\u7528\u7684\u94c2\u78b3\u548c\u6c27\u5316\u948c\u3002\u6b64\u5916\uff0c\u5229\u7528\u805a\u5408\u58f3\u805a\u7cd6-\u751f\u7269\u7ea4\u7ef4\u7d20\u7684\u6c22\u6c27\u5316\u7269\u8d85\u79bb\u5b50\u5bfc\u4f53\u663e\u793a\u51fa\u4f18\u5f02\u7684\u5bfc\u7535\u6027(25\u00b0C\u65f6\u4e3a86.7 mS\/cm)\uff0c\u8fd9\u8bf4\u660e\u5176\u5177\u6709\u5f88\u9ad8\u7684\u673a\u68b0\/\u5316\u5b66\u7a33\u5b9a\u6027\u3002460 Wh kg<sub>cell<\/sub><sup>\u20131<\/sup>\/1389 Wh l<sup>-1<\/sup>\u7684\u9ad8\u7535\u6c60\u80fd\u91cf\u5bc6\u5ea6\u901a\u5e38\u572820\/70%\u653e\u7535\u6df1\u5ea6\u4e0b\u5faa\u73af\u5bff\u547d\u4e3a6000\/1100\u6b21\u3002\u672c\u6587\u6240\u63d0\u51fa\u7684\u7535\u6c60\u80fd\u8fbe\u5230\u7684\u6700\u9ad8\u5bc6\u5ea6\u4e3a523 Wh kg<sub>cell<\/sub><sup>\u20131<\/sup>\/1609 Wh l<sup>-1<\/sup>\u3002\u8f6f\u5305\u7535\u6c60\u572820\u81f380\u2103\u7684\u5bbd\u6e29\u5ea6\u8303\u56f4\u5185\u80fd\u591f\u4ee55\u2013200\u6beb\u5b89\u6bcf\u5e73\u65b9\u5398\u7c73\u7684\u901f\u7387\u826f\u597d\u8fd0\u884c\u3002<\/p>\n<p><strong>\u56fe\u6587\u5206\u6790<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-220674 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-1-3.png\" alt=\"\" width=\"600\" height=\"412\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-1-3.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-1-3-300x206.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe1 |\u9ad8\u80fdZPCs\u7684\u8bbe\u8ba1\u7b56\u7565\u53ca\u4e0e\u5546\u7528\u50a8\u80fd\u7535\u6c60\u7684\u6bd4\u8f83\u3002<\/p>\n<p>\u8981\u70b9\uff1a<\/p>\n<ul>\n<li>\u5b89\u65f6\u89c4\u6a21\u7684\u96f6\u7535\u6d41\u7535\u5bb9\u5668\u662f\u4f7f\u7528\u5bf9\u79f0\u7ed3\u6784\u5236\u9020\u7684\uff0c\u5176\u4e2d\u5728\u7ea610\u78c5\/\u5e73\u65b9\u82f1\u5bf8\u7684\u5f31\u5916\u90e8\u538b\u529b\u4e0b\uff0c\u8d1f\u6781\u4fdd\u62a4\u7cfb\u7edf(101)\u548c\u7535\u89e3\u8d28(CBCs)\u4f4d\u4e8e\u56fe\u6848\u5316\u950c\u6b63\u6781\u7684\u4e24\u4fa7(\u56fe1a-d)\u3002\u8fd9\u79cd\u7535\u6c60\u7ed3\u6784\u6709\u5229\u4e8e\u6784\u5efa\u575a\u56fa\u7684\u56fa\u4f53\u7535\u89e3\u8d28\u754c\u9762(SEI)\u3002\u8fd9\u79cdSEI\u662f\u57fa\u4e8e\u6cbfCBC\u4e3b\u94fe\u7684\u5e26\u8d1f\u7535\u7684\u6709\u673a\u7269\u8d28\u3001\u950c\u79bb\u5b50\u7684\u9759\u7535\u76f8\u4e92\u4f5c\u7528\u548cCPS17\u7684\u5f3a\u7ed3\u6676\u53d6\u5411\u4e4b\u95f4\u7684\u534f\u540c\u4f5c\u7528\u7684\u7ed3\u679c\u3002<\/li>\n<\/ul>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-220675 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-2-3.png\" alt=\"\" width=\"600\" height=\"315\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-2-3.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-2-3-300x158.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe2 |\u53cc\u529f\u80fd\u7535\u5316\u5b66\uff08ORR\u548cOER\uff09\u6027\u80fd\u548c\u57fa\u4e8e\u94dc\u8d1f\u6781\u7684\u52a8\u529b\u5b66\u3002<\/p>\n<p>\u8981\u70b9\uff1a<\/p>\n<ul>\n<li>\u672c\u6587\u8bc4\u4f30\u4e86\u6c2f\u5316\u77f3\u8721(101)\u4e0e\u5546\u4e1a\u94c2\/\u78b3(20 wt%)\u548c\u5176\u4ed6\u6c2f\u5316\u77f3\u8721\u57fa\u50ac\u5316\u5242\u57280.1 M\u6c22\u6c27\u5316\u94be\u7535\u89e3\u6db2\u4e2d\u7684\u6c27\u5316\u8fd8\u539f\u80fd\u529b\u3002CPS(101)\u7684\u5faa\u73af\u4f0f\u5b89\u6cd5\u663e\u793a\u51fa\u660e\u663e\u7684\u6c27\u8fd8\u539f\u7535\u4f4d(~0.9 V\u5bf9RHE)\uff0c\u5e76\u4e14\u8868\u73b0\u51fa\u663e\u8457\u7684\u56fa\u6709ORR\u6d3b\u6027\u3002\u4f5c\u4e3a\u7535\u5316\u5b66\u6027\u80fd\u7684\u57fa\u51c6\uff0c\u7ebf\u6027\u626b\u63cf\u4f0f\u5b89\u6cd5\u663e\u793a\u51faCPS(101)\u7684\u534a\u6ce2\u7535\u4f4d(E1\/2= 0.90\u4f0f)\u6709\u6240\u6539\u5584\uff0c\u5176\u6570\u91cf\u7ea7\u4e3aCF &lt; CP&lt; CS &lt;\u672c\u4f53CPS &lt;\u94c2\/\u78b3&lt; CPS(101)(\u56fe2a)\u3002<\/li>\n<li>CPS(101)\u572830000\u6b21\u5faa\u73af\u540e\u8868\u73b0\u51fa\u6781\u5927\u7684\u8010\u4e45\u6027\uff0c\u534a\u6ce2\u7535\u4f4d\u635f\u5931\u53ef\u5ffd\u7565\u4e0d\u8ba1(&lt; 11\u6beb\u4f0f)\uff0c\u8fd9\u4f18\u4e8e\u7f8e\u56fd\u80fd\u6e90\u90e8\u52a0\u901f\u8010\u4e45\u6027\u534f\u8bae(\u5373&lt; 30\u6beb\u4f0f\u7684\u534a\u6ce2\u7535\u4f4d\u635f\u5931)\u4ee5\u53ca\u5546\u7528\u94c2\u78b3(\u56fe2b)\u3002<\/li>\n<\/ul>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-220676 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-3-3.png\" alt=\"\" width=\"600\" height=\"359\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-3-3.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-3-3-300x180.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe3 |\u7535\u50ac\u5316CPS\u6d3b\u6027\u7684\u7406\u8bba\u8ba1\u7b97\u3002<\/p>\n<p>\u8981\u70b9\uff1a<\/p>\n<ul>\n<li>\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u63ed\u793a\u4e86\u6c2f\u5316\u77f3\u8721(101)\u8868\u73b0\u51fa\u4f18\u5f02\u7684HER\/OER\/ORR\u50ac\u5316\u6027\u80fd\u7684\u539f\u56e0\uff0c\u5176\u4e2d\u78f7\u548c\u786b\u4e4b\u95f4\u7684\u7a7a\u95f4\u5206\u79bb\u4e3aHER\u63d0\u4f9b\u4e86\u8d28\u5b50\u548c\u6c27\u5316\u7269\u53d7\u4f53\u4f4d\u70b9\uff0c\u540c\u65f6\u4e3aOER\/ORR\u63d0\u4f9b\u4e86\u786b\u79bb\u5b50\u5e76\u4e14\u6ca1\u6709\u53d1\u751f\u4e25\u91cd\u7684\u7535\u5b50\u8026\u5408(\u56fe3a)\u3002<\/li>\n<\/ul>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-220677 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-4-2.png\" alt=\"\" width=\"600\" height=\"281\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-4-2.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-4-2-300x141.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe4 | CPS\uff08101\uff09\u8d1f\u6781\u7684\u7535\u8377\u8865\u507f\u673a\u5236\u3002<\/p>\n<p>\u8981\u70b9\uff1a<\/p>\n<ul>\n<li>\u7528XRD\u548cXANES\u5206\u6790\u8bc4\u4ef7\u4e86\u6c2f\u5316\u77f3\u8721(101)\u7535\u5316\u5b66\u6027\u80fd\u7684\u6765\u6e90\u3002\u5728\u5145\u653e\u7535\u8fc7\u7a0b\u4e2d\uff0c\u6c2f\u5316\u77f3\u8721(101)\u901a\u8fc7(101)\u9762\u95f4\u6676\u683c\u95f4\u8ddd\u7684\u53ef\u9006\u53d8\u5316\u53d1\u751f\u56fa\u6eb6\u53cd\u5e94\uff0c\u8fd9\u5bf9\u5e94\u4e8e\u6b63\u4ea4\u76f8\u4e2d\u6676\u683c\u95f4\u8ddd\u5206\u522b\u4e3a0.466-0.478\u7eb3\u7c73\u65f6\u7684287.2-294.6\u57c3\u7684\u7acb\u65b9\u6676\u80de\u4f53\u79ef(\u56fe4a\uff0cb)\u3002<\/li>\n<\/ul>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-220678 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-5-2.png\" alt=\"\" width=\"600\" height=\"419\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-5-2.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-5-2-300x210.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe5 |\u8d85\u79bb\u5b50CBC\u5bfc\u4f53\u7684\u5408\u6210\u4e0e\u8868\u5f81\u3002<\/p>\n<p>\u8981\u70b9\uff1a<\/p>\n<ul>\n<li>\u901a\u8fc7\u90e8\u5206\u6c27\u5316\u76842\uff0c2\uff0c6\uff0c6-\u56db\u7532\u57fa\u54cc\u5576-1-\u6c27\u57fa(TEMPO) CBCs (oCBCs)\u548c1\uff0c4-\u4e8c\u6c2e\u6742\u53cc\u73af[2 . 2 . 2]\u8f9b\u70f7\u5b63\u94f5\u5316CBCs (qCBCs)\u4e4b\u95f4\u7684\u4ea4\u8054\uff0c\u6784\u5efa\u6279\u91cf\u89c4\u6a21(\u5c3a\u5bf8\u7ea6900 cm<sup>2<\/sup>)\u7684CBC\u8d85\u79bb\u5b50\u5bfc\u4f53(\u56fe5a)\u3002\u5728\u76f8\u4e92\u4ea4\u8054\u4e4b\u524d\uff0c\u8fd9\u4e24\u4e2a\u5173\u952e\u8fc7\u7a0b(\u6c27\u5316\u548c\u5b63\u94f5\u5316)\u663e\u8457\u63d0\u9ad8\u4e86\u5206\u5b50\u91cf\u3001\u8d1f\u7535\u8377\u5bc6\u5ea6\u3001\u6297\u6eb6\u80c0\u6027\u3001\u4ea4\u8054\u76f8\u5bb9\u6027\u548c\u4e0e\u4e0d\u540c\u6709\u673a\u6eb6\u5242\u7684\u79bb\u5b50\u8bc6\u522b\u7279\u6027\u3002\u672c\u6587\u4f7f\u7528<sup>1<\/sup>H\u6838\u78c1\u5171\u632f(\u56fe5a\uff0cb)\u5206\u6790\u9a8c\u8bc1\u4e86\u6bcf\u4e2a\u5316\u5b66\u6b65\u9aa4\uff0c\u5e76\u4e14\u5728\u4ea4\u8054\u4e4b\u540e\u6700\u7ec8\u83b7\u5f97\u4e86CBC\u5bfc\u4f53\u3002<\/li>\n<\/ul>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-220679 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-6-3.png\" alt=\"\" width=\"600\" height=\"466\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-6-3.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-6-3-300x233.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe6 |\u5728\u5e02\u552e\u6761\u4ef6\u4e0b\u67d4\u6027ZPC\u7684\u7535\u5316\u5b66\u6027\u80fd\u3002<\/p>\n<p>\u8981\u70b9\uff1a<\/p>\n<ul>\n<li>\u7531\u4e8e\u8d85\u79bb\u5b50\u5bfc\u7535\u6027\uff0c\u91c7\u7528CBCs\u5bfc\u4f53\u7684\u7535\u6c60\u57285\u201320 mA\u00b7cm<sup>-2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u8868\u73b0\u51fa\u22651000\u6b21\u5faa\u73af\u7684\u9ad8\u5ea6\u7a33\u5b9a\u6027\uff0c\u5e76\u4e14\u6ca1\u6709\u4efb\u4f55\u5316\u5b66\u964d\u89e3(\u56fe6a)\uff0c\u800c\u5546\u7528A201\u8868\u73b0\u51fa23\u6b21\u5faa\u73af\u7684\u77ed\u5bff\u547d\u3002<\/li>\n<\/ul>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter wp-image-220680 size-full\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-7-3.png\" alt=\"\" width=\"600\" height=\"653\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-7-3.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/04\/\u56fe\u7247-7-3-276x300.png 276w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe7 | CPS\uff08101\uff09|| CBC || CBC || CBCS || CBC || CPS\uff08101\uff09\u8f6f\u5305\u7535\u6c60\u5728\u6076\u52a3\u6761\u4ef6\u4e0b\u7684\u6027\u80fd\u3002<\/p>\n<p><strong>\u7ed3\u8bed<\/strong><\/p>\n<p>\u672c\u6587\u63d0\u51fa\u5e76\u8bbe\u8ba1\u7684CPS(101)\u8d1f\u6781\u3001CBC\u7535\u89e3\u8d28\u548c\u56fe\u6848\u5316\u950c\u6b63\u6781\u96c6\u6210\u7684\u5168\u56fa\u6001ZPCs\uff0c\u5176\u8868\u73b0\u51fa\u7a33\u5b9a\u7684\u52a8\u529b\u5b66\u7279\u6027\u3001\u8d85\u79bb\u5b50\u5bfc\u7535\u6027\u548c\u7535\u5316\u5b66\u8010\u4e45\u6027\u3002\u5bf9\u4e8e\u5546\u4e1a\u4e0a\u7684\u5e94\u7528\u6765\u8bf4\uff0c1-Ah\u7ea7ZPCs\u5728\u5b9e\u9645\u5de5\u4f5c\u6761\u4ef6\u4e0b\u8868\u73b0\u51fa\u51fa\u8272\u7684\u7535\u6c60\u7ea7\u80fd\u91cf\u5bc6\u5ea6(\u7ea6460\u2013523 Wh kg<sub>cell<\/sub><sup>\u20131<\/sup>\u548c\u7ea61389\u20131609 Wh l<sup>-1<\/sup>)\u3001\u5faa\u73af\u5bff\u547d(&gt; 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