{"id":222292,"date":"2021-05-26T12:00:07","date_gmt":"2021-05-26T04:00:07","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=222292"},"modified":"2021-05-26T11:28:29","modified_gmt":"2021-05-26T03:28:29","slug":"%ef%bc%88%e5%b7%b2%e6%a0%a1%e7%a8%bf%e4%bb%b6%ef%bc%89%e6%b1%aa%e5%9b%bd%e7%a7%80%e7%8e%8b%e6%98%a5%e7%94%9f%e7%ad%89-nat-commun-%ef%bc%9a%e5%88%b6%e5%a4%87%e9%ab%98%e6%af%94%e8%83%bd%e9%87%8f","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=222292","title":{"rendered":"\u6c6a\u56fd\u79c0&\u738b\u6625\u751f\u7b49 Nat. Commun.\uff1a\u5236\u5907\u9ad8\u6bd4\u80fd\u91cf\u6c34\u7cfb\u591a\u4ef7\u79bb\u5b50\u7535\u6c60\u7684\u901a\u7528\u7b56\u7565"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u53ef\u9760\u7684\u5927\u89c4\u6a21\u50a8\u80fd\u5bf9\u4e8e\u5c06\u592a\u9633\u80fd\u3001\u98ce\u80fd\u7b49\u53ef\u518d\u751f\u80fd\u6e90\u6574\u5408\u5230\u7535\u7f51\u4e2d\u5fc5\u4e0d\u53ef\u5c11\u3002\u4f5c\u4e3a\u9502\uff08Li\uff09\u79bb\u5b50\u7535\u6c60\u7684\u7ecf\u6d4e\u9ad8\u6548\u66ff\u4ee3\u54c1\uff0c\u53ef\u518d\u5145\u7535\u591a\u4ef7\u79bb\u5b50\u7535\u6c60\uff08MIBs\uff09\u662f\u7535\u7f51\u89c4\u6a21\u5e94\u7528\u7684\u7406\u60f3\u50a8\u80fd\u6280\u672f\u3002\u5176\u4e2d\uff0cCa2+<\/sup>\u3001Mg2+<\/sup>\u548cAl3+<\/sup>\u9633\u79bb\u5b50\u4e0d\u4ec5\u5177\u6709\u65e0\u6bd2\u3001\u7a33\u5b9a\u7684\u5316\u5408\u4ef7\u6001\u3001\u4f4e\u7684\u6c27\u5316\u8fd8\u539f\u7535\u4f4d\u7b49\u4f18\u70b9\u3001\u800c\u4e14\u5b83\u4eec\u53ef\u4ee5\u8f6c\u79fb\u4e00\u4e2a\u4ee5\u4e0a\u7684\u7535\u5b50\uff0c\u8fdb\u800c\u589e\u52a0\u6bd4\u80fd\u91cf\u3002\u4f46\u662f\uff0cMIBs\u7684\u53d1\u5c55\u8fd8\u5b58\u5728\u4ee5\u4e0b\u6311\u6218\uff1a1\uff09\u591a\u4ef7\u9633\u79bb\u5b50\u5728\u6709\u673a\u7535\u89e3\u8d28\u91d1\u5c5e\u6c27\u5316\u7269\u6b63\u6781\u4e2d\u6c89\u79ef\/\u6eb6\u89e3\u7684\u7f13\u6162\u52a8\u529b\u5b66\uff1b2\uff09\u5bf9\u4e8e\u8d1f\u6781\uff0c\u591a\u4ef7\u9633\u79bb\u5b50\u96be\u4ee5\u7a7f\u900fCa\u3001Mg\u548cAl\u91d1\u5c5e\u8d1f\u6781\u8868\u9762\u5bcc\u542b\u6709\u673a\u6210\u5206\u7684\u949d\u5316\u754c\u9762\u5c42\uff0c\u5176\u4e2d\u6709\u673a\u6210\u5206\u4e3b\u8981\u662f\u7535\u89e3\u8d28\u4e2d\u6709\u673a\u6eb6\u5242\u7684\u8fd8\u539f\u800c\u5f62\u6210\u3002\u56e0\u6b64\uff0c\u91cd\u65b0\u8bbe\u8ba1\u7535\u6c60\u5316\u5b66\u6280\u672f\u5bf9\u4e8e\u5f00\u53d1MIBs\u81f3\u5173\u91cd\u8981\u3002\u901a\u8fc7\u5408\u7406\u8bbe\u8ba1\u9ad8\u7535\u538b\u6c34\u7cfb\u7535\u6c60\uff0c\u5b9e\u73b0MIBs\u5316\u5b66\u7684\u518d\u521b\u65b0\uff0c\u5e94\u91c7\u7528\u4f4e\u6bd2\u3001\u4e0d\u71c3\u7684\u9ad8\u6d53\u5ea6\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u66ff\u4ee3\u6613\u71c3\u7684\u6709\u673a\u919a\u57fa\u7535\u89e3\u8d28\u3002\u5728\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u4e2d\uff0c\u7531\u4e8e\u6c34\/\u8d28\u5b50\u7684\u5171\u6c89\u79ef\uff0c\u591a\u4ef7\u9633\u79bb\u5b50\u5728\u91d1\u5c5e\u6c27\u5316\u7269\u6b63\u6781\u4e2d\u7684\u6c89\u79ef\/\u6eb6\u89e3\u52a8\u529b\u5b66\u5f88\u5feb\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6fb3\u5927\u5229\u4e9a\u6089\u5c3c\u79d1\u6280\u5927\u5b66\u6c6a\u56fd\u79c0\u6559\u6388\u548c<\/strong>Dong Zhou<\/strong>\u3001\u7f8e\u56fd\u9a6c\u91cc\u5170\u5927\u5b66\u738b\u6625\u751f\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u7cfb\u5217\u7684\u6c34\u7cfb\u591a\u4ef7\u79bb\u5b50\u7535\u6c60\uff0c\u6709\u6548\u7684\u89e3\u51b3\u4e86\u6709\u673a\u7535\u89e3\u8d28\u4e2d\u52a8\u529b\u5b66\u7f13\u6162\u7684\u95ee\u9898\uff0c\u540c\u65f6\u8fd8\u63d0\u5347\u4e86\u7535\u6c60\u7684\u5b89\u5168\u6027\u80fd\u3002\u8be5\u6c34\u7cfb\u79bb\u5b50\u7535\u6c60\u7531\u6d53\u7f29\u7684\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u3001\u542b\u786b\u8d1f\u6781\u548c\u9ad8\u7535\u538b\u91d1\u5c5e\u6c27\u5316\u7269\u6b63\u6781\u7ec4\u6210\uff0c\u5176\u5177\u6709\u9ad8\u6bd4\u80fd\u91cf\u3001\u826f\u597d\u7684\u53ef\u9006\u6027\u548c\u66f4\u9ad8\u7684\u5b89\u5168\u6027\u3002\u4f5c\u4e3a\u6f14\u793a\u6a21\u578b\uff0c\u4f5c\u8005\u62a5\u9053\u4e86\u5728\u5ba4\u6e29\u4e0b\u7684\u6c34\u7cfb\u9499\u79bb\u5b50\/\u786b\u5168\u7535\u6c60\uff08ACSB\uff09\u662f\u7531\u786b\/\u78b3\uff08S\/C\uff09\u8d1f\u6781\u3001\u5c42\u72b6Ca0.4<\/sub>MnO2<\/sub>\u6b63\u6781\u548c\u57fa\u4e8e8.37 m\uff08mol kg-1<\/sup>solvent<\/sub>\uff09\u9971\u548cCa(NO3<\/sub>)2<\/sub>\u6c34\u6eb6\u6db2\u7684\u51dd\u80f6\u7535\u89e3\u8d28\u7ec4\u6210\u3002\u51dd\u80f6\u7535\u89e3\u8d28\u7684\u4f4e\u6c34\u6d3b\u5ea6\u6709\u6548\u5730\u6291\u5236\u4e86\u591a\u786b\u5316\u9499\u5728\u8d1f\u6781\u4e2d\u6eb6\u89e3\u800c\u5f15\u8d77\u7684\u5bb9\u91cf\u635f\u5931\uff0c\u540c\u65f6\u6709\u5229\u4e8e\u9499\u79bb\u5b50\u5728\u6b63\u6781\u4e2d\u5feb\u901f\u7a33\u5b9a\u7684\u6c89\u79ef\/\u6eb6\u89e3\u3002\u6240\u5236\u5907\u7684ACSBs\u6bd4\u80fd\u91cf\u9ad8\u8fbe110 Wh kg-1<\/sup>\uff0c\u57280.2 \u2103\u4e0b\u5faa\u73af150\u6b21\u540e\u5bb9\u91cf\u4fdd\u6301\u7387\u4ecd\u4e3a83%\uff0c\u5728\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u4e2d\u5177\u6709\u4f18\u5f02\u7684\u5b89\u5168\u6027\u3002\u6b64\u5916\uff0c\u4f5c\u8005\u8fd8\u8bc1\u660e\u4e86\u8fd9\u79cd\u7b56\u7565\u4e5f\u53ef\u4ee5\u63a8\u5e7f\u5230\u5236\u9020\u9ad8\u6bd4\u80fd\u91cf\u6c34\u7cfb\u9541\u79bb\u5b50\/\u786b||\u91d1\u5c5e\u6c27\u5316\u7269\u548c\u94dd\u79bb\u5b50\/\u786b||\u91d1\u5c5e\u6c27\u5316\u7269\u7535\u6c60\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cA universal strategy towards high-energy aqueous multivalent-ion batteries\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNature Communications<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u7535\u89e3\u8d28\u7684\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u7a97\u53e3<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff091 m\u30012 m\u30015 m\u3001\u9971\u548c\uff088.37 m\uff09Ca(NO3<\/sub>)2<\/sub>\u7535\u89e3\u8d28\u548c\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u7684\u7ebf\u6027\u4f0f\u5b89\u66f2\u7ebf\uff0c\u626b\u63cf\u901f\u7387\u4e3a1 mV s-1<\/sup>\uff0c\u5176\u4e2dm\u4e3amol kg-1<\/sup>solvent<\/sub>\uff1b<\/p>\n

\uff08b\uff09\u4ece\u5b9e\u9a8c\u6570\u636e\u83b7\u5f97\u7535\u89e3\u8d28\u7684\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u7a97\u53e3\uff0c\u4ee5\u53caCa0.4<\/sub>MnO2<\/sub>\u6b63\u6781\u548c\u786b\u8d1f\u6781\u7684\u6c27\u5316\u8fd8\u539f\u7535\u538b\u3002<\/p>\n

\u56fe\u4e8c\u3001\u7535\u89e3\u8d28\u7684\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df\u548c\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a-c\uff09\u57fa\u4e8e10 ns\u5206\u5b50\u52a8\u529b\u5b66\uff08MD\uff09\u6a21\u62df\u83b7\u5f971 m Ca(NO3<\/sub>)2<\/sub>\u7535\u89e3\u8d28\u3001\u9971\u548cCa(NO3<\/sub>)2<\/sub>\u7535\u89e3\u8d28\u548c\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u7684\u5c40\u90e8\u7ed3\u6784\u6f14\u5316\u7167\u7247\uff1b<\/p>\n

\uff08d\uff09\u57fa\u4e8e10 ns\u5206\u5b50\u52a8\u529b\u5b66\uff08MD\uff09\u6a21\u62df\uff0c\u4e09\u4e2a\u7535\u89e3\u8d28\u6837\u54c1\u7684\u6c22\u952e\u548c\u4e0eCa2+<\/sup>\u914d\u4f4d\u7684\u6c34\u5206\u5b50\u767e\u5206\u6bd4\u3002<\/p>\n

\uff08e\uff091 m\u30012 m\u30015 m\u548c\u9971\u548c\uff088.37 m\uff09Ca(NO3<\/sub>)2<\/sub>\u6c34\u7cfb\u7535\u89e3\u8d28\u548c\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u7684\u62c9\u66fc\u5149\u8c31\uff0c\u5176\u4e2dm\u4e3amol kg-1<\/sup>solvent<\/sub>\u3002<\/p>\n

\u56fe\u4e09\u3001\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u4e2d\u5143\u7d20\u786b\u7684\u53cd\u5e94\u673a\u7406<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u57fa\u4e8e\u5206\u5b50\u52a8\u529b\u5b66\uff08MD\uff09\u6a21\u62df\uff0cCaS4<\/sub>\u57281 m\u30018.37 m Ca(NO3<\/sub>)2<\/sub>\u7535\u89e3\u8d28\u548c\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u4e2d\u7684\u6269\u6563\u7684\u5c40\u90e8\u7ed3\u6784\u6f14\u53d8\uff0c\u5176\u4e2dm\u4e3amol kg-1<\/sup>solvent<\/sub>\uff1b<\/p>\n

\uff08b\uff09\u76ee\u89c6\u89c2\u5bdf\u591a\u786b\u5316\u9499\u57281 m\u30018.37 m Ca(NO3<\/sub>)2<\/sub>\u7535\u89e3\u8d28\u548c\u51dd\u80f6\u7535\u89e3\u8d28\u4e2d\u7684\u6269\u6563\uff1b<\/p>\n

\uff08c\uff09\u5728\u542b\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u4e2d\uff0cS\/C\u7535\u6781\u7684\u521d\u59cbCV\u66f2\u7ebf\uff0c\u626b\u63cf\u901f\u7387\u4e3a0.21 mV s-1<\/sup>\uff1b<\/p>\n

\uff08d\uff09\u57281 m Ca(NO3<\/sub>)2<\/sub>\u548c\u6c34\u51dd\u80f6\u7535\u89e3\u8d28\u4e2d\u6d4b\u8bd5\u7684S\/C\u8d1f\u6781\u7684\u6768\u6c0f\u6a21\u91cf\uff1b<\/p>\n

\uff08e\uff09DFT\u8ba1\u7b97\u51cf\u5c11Ca2+<\/sup>(NO3<\/sub>–<\/sup>)3<\/sub>(H2<\/sub>O)x<\/sub>\u96c6\u5408\u4f53\u7684\u8fd8\u539f\uff1b<\/p>\n

\uff08f\uff09\u5728\u6b63\u6781CV\u626b\u63cf\u540e\uff0cS\/C\u7535\u6781\u7684\u6df1\u5ea6Ca 2p XPS\u3002<\/p>\n

\u56fe\u56db\u3001<\/strong>Ca0.4<\/sub>MnO2<\/sub><\/strong>\u6b63\u6781\u7684\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5728\u539f\u4f4d\u7535\u5316\u5b66\u8f6c\u5316\u8fc7\u7a0b\u4e2d\uff0c\u539f\u5b50\u7ed3\u6784\u53d8\u5316\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b-c\uff09Mn3<\/sub>O4<\/sub>\u524d\u4f53\u548cCa0.4<\/sub>MnO2<\/sub>\u6b63\u6781\u6750\u6599\u7684HADDF-STEM\u56fe\u50cf\uff1b<\/p>\n

\uff08d\uff09Mn3<\/sub>O4<\/sub>\u3001\u6c34\u94a0\u9530\u77ffMnO2<\/sub>\u548cCa0.4<\/sub>MnO2<\/sub>\u7684\u540c\u6b65\u52a0\u901f\u5668\u7c89\u672b\u884d\u5c04\u56fe\uff1b<\/p>\n

\uff08e\uff09Ca0.4<\/sub>MnO2<\/sub>\u6b63\u6781\u7684CV\u66f2\u7ebf\uff0c\u626b\u63cf\u901f\u7387\u4e3a0.3 mV s-1<\/sup>\u3002<\/p>\n

\u56fe\u4e94\u3001\u7ec4\u88c5\u540e<\/strong>ACSBs<\/strong>\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09S\/C|\u6c34\u51dd\u80f6\u7535\u89e3\u8d28|Ca0.4<\/sub>MnO2<\/sub>\u5168\u7535\u6c60\u7684CV\u66f2\u7ebf\uff0c\u626b\u63cf\u901f\u7387\u4e3a0.2 mV s-1\uff1b<\/p>\n

\uff08b\uff09\u5177\u6709\u4e0d\u540c\u7535\u89e3\u8d28\u7684\u5168\u7535\u6c60\u7684\u500d\u7387\u6027\u80fd\uff1b<\/p>\n

\uff08c\uff09\u5728\u4e0d\u540c\u7684\u6bd4\u7535\u6d41\u4e0b\uff0c\u6c34\u6027\u51dd\u80f6\u7535\u89e3\u8d28\u7ec4\u88c5\u7684\u5168\u7535\u6c60\u7684\u7535\u538b\u66f2\u7ebf\uff1b<\/p>\n

\uff08d\uff09\u57fa\u4e8e\u7535\u6781\u6d3b\u6027\u6750\u6599\u7684\u603b\u8d28\u91cf\uff0c\u6bd4\u8f83\u5404\u79cd\u6c34\u7cfb\u50a8\u80fd\u88c5\u7f6e\u7684\u6bd4\u80fd\u91cf\uff1b<\/p>\n

\uff08e\uff09S\/C||Ca0.4<\/sub>MnO2<\/sub>\u5168\u7535\u6c60\u57280.2 C\u65f6\u7684\u5faa\u73af\u6027\u80fd\u548c\u76f8\u5e94\u7684\u5e93\u4ed1\u6548\u7387\uff1b<\/p>\n

\uff08f\uff09\u5207\u89d2\u540e\uff0c\u5e26\u7535\u7684S\/C|\u6c34\u51dd\u80f6\u7535\u89e3\u8d28|Ca0.4<\/sub>MnO2<\/sub>\u888b\u5f0f\u7535\u6c60\u7684\u6d78\u6c34\u5b9e\u9a8c\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a<\/strong>A universal strategy towards high-energy aqueous multivalent-ion batteries<\/a><\/strong>. Nat. Commun., 2021<\/strong>, DOI: 10.1038\/s41467-021-23209-6.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1\uff1a<\/strong>tougao@cailiaoren.com.<\/p>\n

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