{"id":222362,"date":"2021-05-25T12:00:16","date_gmt":"2021-05-25T04:00:16","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=222362"},"modified":"2021-11-27T11:40:59","modified_gmt":"2021-11-27T03:40:59","slug":"%ef%bc%88%e5%b7%b2%e6%a0%a1%e7%a8%bf%e4%bb%b6%ef%bc%89%e5%8c%97%e8%88%aa-sci-adv-%ef%bc%9a%e6%9c%80%e9%ab%98%e5%80%bc%ef%bc%81%e7%ba%b3%e7%b1%b3%e9%80%9a%e9%81%93%e9%98%b5%e5%88%97%e8%96%84%e8%86%9c","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=222362","title":{"rendered":"\u5317\u822a Sci. Adv.\uff1a\u6700\u9ad8\u503c\uff01\u7eb3\u7c73\u901a\u9053\u9635\u5217\u8584\u819c\u5b9e\u73b0\u8d85\u9ad8\u6e17\u900f\u80fd\u8f6c\u6362"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u6d77\u6c34\u548c\u6cb3\u6c34\u4e4b\u95f4\u5b58\u5728\u7684\u6e17\u900f\u80fd\u662f\u4e00\u79cd\u5927\u89c4\u6a21\u3001\u53ef\u518d\u751f\u3001\u53ef\u6301\u7eed\u7684\u80fd\u6e90\uff0c\u901a\u8fc7\u53cd\u7535\u6e17\u6790\uff08RED\uff09\u53ef\u4ee5\u76f4\u63a5\u8f6c\u6362\u4e3a\u7535\u80fd\u3002\u5728RED\u7cfb\u7edf\u4e2d\uff0c\u79bb\u5b50\u9009\u62e9\u6027\u8f6c\u8fd0\u8584\u819c\u662f\u6700\u91cd\u8981\u7684\u90e8\u5206\u4e4b\u4e00\u3002\u7136\u800c\uff0c\u4f20\u7edf\u7684\u8584\u819c\u7531\u4e8e\u5176\u9ad8\u7535\u963b\u800c\u8868\u73b0\u51fa\u8f83\u5dee\u7684\u529f\u7387\u5bc6\u5ea6\u3002\u76ee\u524d\uff0c\u6709\u4e24\u79cd\u4f20\u7edf\u7684\u65b9\u6cd5\u63d0\u9ad8\u80fd\u91cf\u8f6c\u6362\u6027\u80fd\uff1a\u4e00\u662f\u7eb3\u7c73\u5b54\uff0c\u5355\u4e2a\u7eb3\u7c73\u5b54\u901a\u8fc7\u51cf\u5c0f\u8584\u819c\u539a\u5ea6\u800c\u663e\u793a\u51fa\u8d85\u9ad8\u529f\u7387\u5bc6\u5ea6\uff0c\u4f46\u662f\u5173\u952e\u7684\u529b\u5b66\u6027\u80fd\u4ecd\u9700\u8981\u63d0\u9ad8\u3002\u4e8c\u662f\u4eff\u751f\u7684\u7eb3\u7c73\u901a\u9053\u8584\u819c\uff08BNM\uff09\uff0c\u901a\u8fc7\u589e\u52a0\u6709\u6548\u5b54\u5bc6\u5ea6\u548c\u51cf\u5c0f\u8584\u819c\u539a\u5ea6\u6765\u5b9e\u73b0\u9ad8\u8f93\u51fa\u529f\u7387\u5bc6\u5ea6\uff0c\u4f46\u8584\u819c\u539a\u5ea6\u6700\u5c0f\u5316\u53d7\u5230\u529b\u5b66\u95ee\u9898\u7684\u9650\u5236\u3002\u6b64\u5916\uff0c\u4e0d\u540c\u76f4\u5f84\u548c\u5468\u671f\u6027\u5c3a\u5bf8\uff08\u901a\u5e38\u5728106<\/sup>-1010<\/sup> cm-2<\/sup>\u5185\uff09\u7684\u7eb3\u7c73\u901a\u9053\u4e4b\u95f4\u7684\u4e0d\u5339\u914d\u9650\u5236\u4e86\u7eb3\u7c73\u901a\u9053\u5bc6\u5ea6\u7684\u6700\u5927\u5316\u3002\u4f17\u6240\u5468\u77e5\uff0c\u77ed\u4e8c\u6781\u7ba1\u5177\u6709\u6bd4\u957f\u4e8c\u6781\u7ba1\u66f4\u9ad8\u7684\u6269\u6563\u7535\u6d41\u3002\u540c\u65f6\uff0cCl–<\/sup>\u901a\u9053\u4e2d\u6781\u8584\u7684\u9009\u62e9\u6027\u6ee4\u6ce2\u5668\u6709\u52a9\u4e8e\u79bb\u5b50\u5feb\u901f\u6269\u6563\uff0c\u662f\u9ad8\u529f\u7387\u5bc6\u5ea6\u7684\u5173\u952e\u56e0\u7d20\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5317\u4eac\u822a\u7a7a\u822a\u5929\u5927\u5b66\u9ad8\u9f99\u6210\u526f\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u3001\u6c5f\u96f7\u9662\u58eb\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u53ef\u5927\u9762\u79ef\u5236\u5907\u3001\u5177\u6709\u8d85\u8584\u79bb\u5b50\u9009\u62e9\u5c42\u7684\u8d85\u9ad8\u5bc6\u5ea6\u8611\u83c7\u72b6\u7684\u7eb3\u7c73\u901a\u9053\u9635\u5217\u8584\u819c\u3002\u8be5\u7eb3\u7c73\u901a\u9053\u7531\u4ee5\u4e0b\u4e24\u90e8\u5206\u7ec4\u6210\uff1a\u830e\u90e8\u5206\u662f\u7531\u5d4c\u6bb5\u5171\u805a\u7269\uff08BCP\uff09\u81ea\u7ec4\u88c5\u800c\u6210\u7684\u4e00\u7ef4\uff081D\uff09\u5e26\u8d1f\u7535\u8377\u7684\u7eb3\u7c73\u901a\u9053\u9635\u5217\uff0c\u5bc6\u5ea6\u7ea6\u4e3a1011<\/sup> cm-2<\/sup>\uff1b\u5e3d\u72b6\u90e8\u5206\u662f\u7531\u5355\u5206\u5b50\u5c42\u8d85\u652f\u5316\u805a\u4e59\u70ef\u4e9a\u80fa\uff08h-PEI\uff09\u7ec4\u6210\u7684\u5e26\u6b63\u7535\u8377\u7684\u4e09\u7ef4\uff083D\uff09\u901a\u9053\u7f51\u7edc\uff0c\u76f8\u5f53\u4e8e\u6bcf\u6839\u830e\u4e0a\u6709\u6570\u5341\u4e2a1D\u7eb3\u7c73\u901a\u9053\uff0c\u56e0\u6b64\u8be5\u8584\u819c\u7eb3\u7c73\u5b54\u7684\u603b\u9762\u79ef\u5bc6\u5ea6\u9ad8\u8fbe\u7ea61012<\/sup> cm-2<\/sup>\u3002\u5177\u6709\u8d85\u9ad8\u5bc6\u5ea6\u7684\u79bb\u5b50\u901a\u9053\u8868\u73b0\u51fa\u5355\u5411\u79bb\u5b50\u4f20\u8f93\u548c\u826f\u597d\u7684\u79bb\u5b50\u9009\u62e9\u6027\uff0c\u5b9e\u73b0\u4e86\u9ad8\u6027\u80fd\u7684\u80fd\u91cf\u8f6c\u6362\u3002\u5728500\u500d\u7684\u76d0\u68af\u5ea6\u4e0b\uff0c\u5176\u8f93\u51fa\u529f\u7387\u5bc6\u5ea6\u6700\u9ad8\u53ef\u8fbe22.4 W m-2<\/sup>\uff0c\u662f\u9ad8\u6027\u80fd\u8584\u819c\u4e2d\u7684\u6700\u9ad8\u503c\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u8be5\u8584\u819c\u7684\u5236\u5907\u53ef\u4ee5\u5f88\u597d\u7684\u63a7\u5236\uff0c\u540c\u65f6\u53c8\u4e0d\u727a\u7272\u5176\u9ad8\u8f93\u51fa\u529f\u7387\u5bc6\u5ea6\u548c\u529b\u5b66\u7a33\u5b9a\u6027\u3002\u603b\u4e4b\uff0c\u8be5\u8584\u819c\u8bbe\u8ba1\u7b56\u7565\u4e3a\u5927\u89c4\u6a21\u6e17\u900f\u80fd\u91cf\u8f6c\u6362\u63d0\u4f9b\u4e86\u4e00\u79cd\u5f88\u6709\u524d\u9014\u7684\u65b9\u6cd5\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cLarge-scale, robust mushroom-shaped nanochannel array membrane for ultrahigh osmotic energy conversion\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520a\u00a0Sci. Adv.<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u7eb3\u7c73\u901a\u9053\u9635\u5217\u8584\u819c\u7528\u4e8e\u6e17\u900f\u53d1\u7535<\/strong>
\n \"\"\uff08A\uff09BCP\u5206\u5b50\u7ed3\u6784\u548cSA\u7eb3\u7c73\u7ed3\u6784\uff1b<\/p>\n

\uff08B\uff09\u901a\u8fc7\u7d2b\u5916\u5149\u5904\u7406\u5f62\u6210\u7eb3\u7c73\u901a\u9053\uff1b<\/p>\n

\uff08C\uff09\u901a\u8fc7\u9170\u80fa\u5316\u53cd\u5e94\u5f62\u6210\u575a\u56fa\u7684h-PEI\u5c01\u7aef\u7684\u7eb3\u7c73\u901a\u9053\uff1b<\/p>\n

\uff08D\uff09BCP SA\u8584\u819c\u7684TEM\u56fe\u50cf\uff0c\u663e\u793a\u516d\u65b9\u5806\u79ef\u7684\u5706\u67f1\u7ed3\u6784\uff1b<\/p>\n

\uff08E\uff09\u7eb3\u7c73\u901a\u9053\u9635\u5217\u8584\u819c\u7684TEM\u56fe\u50cf\uff0c\u663e\u793a\u516d\u65b9\u5806\u79ef\u7684\u7eb3\u7c73\u901a\u9053\u7ed3\u6784\uff1b<\/p>\n

\uff08F\uff09h-PEI\u8986\u76d6\u7684\u8584\u819c\u7684TEM\u56fe\u50cf\uff0c\u8868\u660e\u6210\u529f\u4fee\u9970\uff1b<\/p>\n

\uff08G\uff09\u5927\u578b\u81ea\u652f\u6491\u8584\u819c\uff08>50 cm-2<\/sup>\uff09\u7684\u7167\u7247\uff0c\u8868\u660e\u53ef\u7f29\u653e\u7684\u5236\u9020\u5de5\u827a\u548c\u51fa\u8272\u7684\u529b\u5b66\u6027\u80fd\uff1b<\/p>\n

\uff08H\uff09\u7d2b\u5916\u5149\u5904\u7406\u524d\u540e\uff0cSA\u8584\u819c\u4ee5\u53cah-PEI\u5c01\u7aef\u7684\u8584\u819c\u7684\u5e94\u529b-\u5e94\u53d8\u66f2\u7ebf\uff0c\u5728\u7d2b\u5916\u7ebf\u4ea4\u8054\u540e\u8868\u73b0\u51fa\u9ad8\u5ea6\u589e\u5f3a\u7684\u529b\u5b66\u5f3a\u5ea6\uff1b<\/p>\n

\uff08I\uff09\u57fa\u4e8eh-PEI\u5c01\u7aef\u7684\u7eb3\u7c73\u901a\u9053\u8584\u819c\u7684\u6e17\u900f\u80fd\u8f6c\u6362\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u4e8c\u3001\u8d85\u9ad8\u5bc6\u5ea6\u3001\u8611\u83c7\u72b6\u7684\u7eb3\u7c73\u901a\u9053\u9635\u5217\u8584\u819c<\/strong>
\n \"\"\uff08A\uff09\u7a7a\u6c14\u4e2dh-PEI\u8986\u76d6\u7684\u7eb3\u7c73\u901a\u9053\u8584\u819c\u8868\u9762\u7684AFM\u9ad8\u5ea6\u56fe\u50cf\uff1b<\/p>\n

\uff08B\uff09\u6c34\u6eb6\u6db2\u4e2dh-PEI\u5c01\u7aef\u7684\u7eb3\u7c73\u901a\u9053\u819c\u8868\u9762\u7684AFM\u9ad8\u5ea6\u56fe\u50cf\uff1b<\/p>\n

\uff08C\uff09\u8611\u83c7\u72b6\u7eb3\u7c73\u901a\u9053\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08D\uff09\u5728h-PEI\u4fee\u9970\u524d\u540e\uff0c\u7eb3\u7c73\u901a\u9053\u8584\u819c\uff08\u57280.1 M\u6eb6\u6db2\u4e2d\uff09\u7684I-V\u66f2\u7ebf\uff1b<\/p>\n

\uff08E\uff09\u975e\u5bf9\u79f0\u7eb3\u7c73\u901a\u9053\u79bb\u5b50\u6d53\u5ea6\u5206\u5e03\u7684\u6570\u503c\u6a21\u62df\u7ed3\u679c\u3002<\/p>\n

\u56fe\u4e09\u3001\u7eb3\u7c73\u901a\u9053\u9635\u5217\u8584\u819c\u7684\u79bb\u5b50\u4f20\u8f93\u8c03\u8282\u6027\u80fd<\/strong>
\n \"\"\uff08A\uff09\u5728\u5bbd\u76d0\u5ea6\u8303\u56f4\u5185\u83b7\u5f97\u7684I-V\u66f2\u7ebf\uff1b<\/p>\n

\uff08B\uff09\u5728\u4e0d\u540c\u6d53\u5ea6\u4e0b\u7684\u76f8\u5e94\u7684\u6574\u6d41\u6bd4\uff0c\u8868\u660e\u5728\u5bbd\u6d53\u5ea6\u8303\u56f4\u4e0b\u5747\u5177\u6709\u51fa\u8272\u7684\u79bb\u5b50\u8fc1\u79fb\u8c03\u8282\u80fd\u529b\u3002<\/p>\n

\uff08C\uff09\u5728\u6781\u9ad8\u76d0\u5ea6\u68af\u5ea6\uff081 \u03bcM\/0.1 M\uff09\u4e0b\u7684I-V\u66f2\u7ebf\uff0c\u5177\u6709\u6781\u9ad8\u7684Cl-\u79bb\u5b50\u9009\u62e9\u6027\uff1b<\/p>\n

\uff08D\uff09\u5f53\u4f7f\u7528[Fe(CN)6<\/sub>]3-<\/sup>\u4f5c\u4e3a\u9633\u79bb\u5b50\u7535\u6d3b\u6027\u63a2\u9488\u548c[Ru(NH3<\/sub>)6<\/sub>]3+<\/sup>\u4f5c\u4e3a\u9634\u79bb\u5b50\u7535\u6d3b\u6027\u63a2\u9488\u65f6\uff0c\u8584\u819c\u7684CV\u66f2\uff1b<\/p>\n

\uff08E\uff09\u5f53\u4f7f\u7528[Fe(CN)6<\/sub>]3-<\/sup>\u548c[Ru(NH3<\/sub>)6<\/sub>]3+<\/sup>\u4e3a\u63a2\u9488\u65f6\uff0cCV\u66f2\u7ebf\u7684\u5cf0\u503c\u7535\u6d41\uff1b<\/p>\n

\uff08F\uff09\u8584\u819c\u57281 mM\/0.5 M\u68af\u5ea6\u4e0b\u7684I-V\u66f2\u7ebf\uff0c\u9ad8\u6d53\u5ea6\u6eb6\u6db2\u5728\u5e3d\u4fa7\u3002<\/p>\n

\u56fe\u56db\u3001\u8d85\u9ad8\u6e17\u900f\u80fd\u8f6c\u6362\u6027\u80fd<\/strong>
\n \"\"\uff08A\uff09\u5728\u4e0d\u540c\u6d53\u5ea6\u4e0b\uff0c\u7535\u6d41\u5bc6\u5ea6\u968f\u7740\u5916\u7535\u963b\u7684\u6539\u53d8\u800c\u53d8\u5316\uff1b<\/p>\n

\uff08B\uff09\u4e0d\u540c\u6d53\u5ea6\u4e0b\uff0c\u529f\u7387\u5bc6\u5ea6\u968f\u7740\u5916\u7535\u963b\u7684\u6539\u53d8\u800c\u53d8\u5316\uff1b<\/p>\n

\uff08C\uff09\u4e0d\u540c\u6d53\u5ea6\u4e0b\uff0c\u6700\u5927\u8f93\u51fa\u529f\u7387\u5bc6\u5ea6\u6210\u500d\u53d8\u5316\uff1b<\/p>\n

\uff08D\uff09\u4f7f\u7528\u9ad8\u76d0\u5ea6\u6eb6\u6db2\u7684\u6700\u5927\u8f93\u51fa\u529f\u7387\u5bc6\u5ea6\uff1b<\/p>\n

\uff08E\uff09\u4f7f\u7528\u5929\u7136\u6d77\u6c34\u548c\u6cb3\u6c34\u548c10 mM\/0.5 M NaCl\u6eb6\u6db2\u5f97\u7684\u529f\u7387\u5bc6\u5ea6\uff1b<\/p>\n

\uff08F\uff09\u5728500\u500d\u65f6\uff0c\u6700\u5927\u8f93\u51fa\u529f\u7387\u5bc6\u5ea6\u968f\u8584\u819c\u539a\u5ea6\u7684\u53d8\u5316\uff0c\u8868\u660e\u529f\u7387\u5bc6\u5ea6\u968f\u8584\u819c\u539a\u5ea6\u7684\u51cf\u5c0f\u800c\u589e\u5927\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u62a5\u9053\u4e86\u4e00\u79cd\u8d85\u9ad8\u5bc6\u5ea6\u7684\u8611\u83c7\u72b6\u7eb3\u7c73\u901a\u9053\u9635\u5217\u8584\u819c\u3002\u5728500\u500d\u7684\u76d0\u5ea6\u68af\u5ea6\u4e0b\uff0c\u8be5\u8584\u819c\u7684\u529f\u7387\u5bc6\u5ea6\u8fbe\u523022.4 W m-2<\/sup>\uff0c\u800c\u57281000\u500d\u7684\u76d0\u5ea6\u68af\u5ea6\u4e0b\uff0c\u5176\u529f\u7387\u5bc6\u5ea6\u751a\u81f3\u9ad8\u8fbe33.2 W m-2<\/sup>\uff0c\u662f\u9ad8\u6027\u80fd\u8584\u819c\u4e2d\u7684\u6700\u9ad8\u503c\u3002\u901a\u8fc7\u8986\u76d6BCP\u884d\u751f\u7684\u7eb3\u7c73\u901a\u9053\u7684\u5355\u5206\u5b50\u5c42h-PEI\u5f62\u6210\u4e86\u8611\u83c7\u72b6\u7eb3\u7c73\u901a\u9053\uff0c\u5176\u4e2d\u5e26\u8d1f\u7535\u8377\u7684\u830e\u90e8\u5206\u7684\u5bc6\u5ea6\u7ea6\u4e3a1011<\/sup> cm-2<\/sup>\uff0c\u5e26\u6b63\u7535\u8377\u7684\u5e3d\u90e8\u5206\u662f3D\u901a\u9053\u7f51\u7edc\uff0c\u76f8\u5f53\u4e8e\u6bcf\u6839\u830e\u6709\u6570\u5341\u4e2a1D\u7eb3\u7c73\u901a\u9053\uff0c\u56e0\u6b64\u4e0d\u5bf9\u79f0\u7eb3\u7c73\u901a\u9053\u7684\u603b\u5bc6\u5ea6\u8fbe\u5230\u7ea61012<\/sup> cm-2<\/sup>\u3002\u6781\u9ad8\u5bc6\u5ea6\u7684\u79bb\u5b50\u901a\u9053\u663e\u793a\u51fa\u5355\u5411\u79bb\u5b50\u4f20\u8f93\u548c\u51fa\u8272\u7684\u79bb\u5b50\u9009\u62e9\u6027\uff0c\u4ece\u800c\u5b9e\u73b0\u4e86\u9ad8\u6027\u80fd\u7684\u80fd\u91cf\u8f6c\u6362\u3002\u6b64\u5916\uff0c\u53ef\u63a7\u7684\u8584\u819c\u5236\u9020\u5de5\u827a\u4e3a\u5de5\u4e1a\u751f\u4ea7\u63d0\u4f9b\u4e86\u4e00\u79cd\u6709\u524d\u9014\u7684\u65b9\u6cd5\u3002\u8be5\u5de5\u4f5c\u4e3a\u5f00\u53d1\u4e0b\u4e00\u4ee3\u4e0d\u5bf9\u79f0\u7eb3\u7c73\u5b54\u8584\u819c\u8fc8\u51fa\u4e86\u91cd\u8981\u4e00\u6b65\uff0c\u5e76\u4e3a\u5927\u89c4\u6a21\u6e17\u900f\u80fd\u8f6c\u5316\u6253\u5f00\u4e86\u5e7f\u9614\u7684\u524d\u666f\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aLarge-scale, robust mushroom-shaped nanochannel array membrane for ultrahigh osmotic energy conversion<\/a><\/strong>. Sci. Adv.<\/em>, 2021<\/strong>, DOI: 10.1126\/sciadv.abg2183.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

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