{"id":224669,"date":"2021-07-16T12:00:41","date_gmt":"2021-07-16T04:00:41","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=224669"},"modified":"2021-07-16T10:51:55","modified_gmt":"2021-07-16T02:51:55","slug":"%e7%a6%8f%e5%bb%ba%e5%b8%88%e5%a4%a7%e5%be%b7%e5%85%8b%e8%90%a8%e6%96%af%e5%a4%a7%e5%ad%a6%e5%9c%a3%e5%ae%89%e4%b8%9c%e5%b0%bc%e5%a5%a5%e5%88%86%e6%a0%a1nature-chemistry%ef%bc%9a%e7%a8%b3%e5%ae%9a","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=224669","title":{"rendered":"\u798f\u5efa\u5e08\u5927&#038;\u5fb7\u514b\u8428\u65af\u5927\u5b66\u5723\u5b89\u4e1c\u5c3c\u5965\u5206\u6821Nature Chemistry\uff1a\u7a33\u5b9a\u6c22\u952e\u6709\u673a\u9aa8\u67b6\u4e2d\u4e59\u70ef\/\u4e59\u70f7\u7684\u5206\u79bb"},"content":{"rendered":"<p>\u7b2c\u4e00\u4f5c\u8005\uff1aYisi Yang\uff0cLibo Li, Rui-Biao Lin<\/p>\n<p>\u901a\u8baf\u4f5c\u8005\uff1aZhangjing Zhang\uff0cShengchang Xiang\uff0cBanglin Chen<\/p>\n<p>\u901a\u8baf\u5355\u4f4d\uff1a\u798f\u5efa\u5e08\u8303\u5927\u5b66\uff0c\u5fb7\u514b\u8428\u65af\u5927\u5b66\u5723\u5b89\u4e1c\u5c3c\u5965\u5206\u6821<\/p>\n<p>DOI\uff1ahttps:\/\/doi.org\/10.1038\/s41557-021-00740-z<\/p>\n<p><strong>\u80cc\u666f<\/strong><\/p>\n<p>\u5206\u79bb\u662f\u5316\u5de5\u5206\u79bb\u548c\u63d0\u7eaf\u5de5\u4e1a\u5546\u54c1\u7684\u5173\u952e\u5de5\u5e8f\uff0c\u5982\u6c14\u4f53\u548c\u6c34\u7684\u84b8\u998f\uff0c\u5360\u5168\u7403\u80fd\u6e90\u6d88\u8017\u768410-15%\u3002\u56e0\u6b64\uff0c\u5bf9\u66ff\u4ee3\u548c\u8282\u80fd\u5206\u79bb\u6280\u672f\u7684\u5f00\u53d1\uff0c\u6ee1\u8db3\u73b0\u4ee3\u5316\u5de5\u7684\u5206\u79bb\u662f\u5341\u5206\u91cd\u8981\u7684\u3002\u591a\u5b54\u6750\u6599\u5728\u5f00\u53d1\u4f4e\u6210\u672c\u3001\u9ad8\u80fd\u6548\u7684\u5206\u79bb\u5de5\u827a\u65b9\u9762\u975e\u5e38\u6709\u524d\u9014\uff0c\u4f8b\u5982\u4ece\u4e59\u70ef\/\u4e59\u70f7\u6df7\u5408\u7269\u4e2d\u63d0\u7eaf\u4e59\u70ef\uff0c\u8fd9\u662f\u4e00\u4e2a\u91cd\u8981\u4f46\u76ee\u524d\u5177\u6709\u6311\u6218\u6027\u7684\u5de5\u4e1a\u8fc7\u7a0b\u3002<\/p>\n<p><strong>\u672c\u6587\u7814\u7a76\u7684\u95ee\u9898<\/strong><\/p>\n<p>\u5728\u8fd9\u91cc\uff0c\u672c\u6587\u62a5\u544a\u4e86\u4e00\u79cd\u7531\u56db\u6c30\u57fa-\u8054\u5494\u5511\u7ec4\u6210\u7684\u5fae\u5b54\u6c22\u952e\u6709\u673a\u9aa8\u67b6\uff0c\u901a\u8fc7\u5206\u5b50\u95f4CN\u00b7\u00b7\u00b7H-C\u6c22\u952e\u4f5c\u7528\u7ed3\u5408\u5728\u4e00\u8d77\uff0c\u5f62\u6210\u4e00\u4e2a\u4e09\u91cd\u4e92\u7a7f\u7684\u9aa8\u67b6\uff0c\u5177\u6709\u5408\u9002\u5927\u5c0f\u7684\u5b54\uff0c\u53ef\u4ee5\u9009\u62e9\u6027\u5730\u6355\u83b7\u4e59\u70ef\u3002\u7279\u522b\u7684\u662f\uff0c\u6c22\u952e\u6709\u673a\u9aa8\u67b6\u8868\u73b0\u201c\u521a\u67d4\u5e76\u6d4e\u201d\u7684\u7ed3\u6784\u7279\u70b9\uff0c\u5e76\u901a\u8fc7\u201c\u95e8\u63a7\u673a\u5236\u201d\u5b9e\u73b0\u9ad8\u6548\u4e59\u70ef\uff0f\u4e59\u70f7\u5206\u79bb\u3002\u901a\u8fc7\u7814\u7a76\u8868\u660e\uff0c\u76f8\u6bd4\u8f83\u4e8e\u4e59\u70ef\uff0c\u4e59\u70f7\u4ec5\u5728\u8f83\u4f4e\u6e29\u5ea6\u4e0b\u5177\u6709\u5438\u9644\uff0c\u800c\u4e14\u5176\u9608\u503c\u538b\u529b\u968f\u6e29\u5ea6\u5347\u9ad8\u800c\u663e\u8457\u589e\u52a0\uff08\u5438\u9644\u91cf\u964d\u4f4e\uff09\u3002\u4e59\u70ef\/\u4e59\u70f7\u7684\u5206\u79bb\u901a\u8fc7\u7a7f\u900f\u5b9e\u9a8c\u5f97\u5230\u9a8c\u8bc1\uff0c\u5728333 K\u4e0b\u53ef\u83b7\u5f97\u9ad8\u7eaf\u5ea6\u7684\u4e59\u70ef(99.1%)\u3002\u6b64\u5916\uff0c\u901a\u5e38\u6c22\u952e\u6709\u673a\u9aa8\u67b6\u5b58\u5728\u7a33\u5b9a\u6027\u95ee\u9898\uff0c\u4f46\u672c\u6587\u7684\u6750\u6599\u5728\u6781\u7aef\u6761\u4ef6\u4e0b(\u5305\u62ec\u66b4\u9732\u5728\u5f3a\u9178\u6027\u3001\u78b1\u6027\u548c\u5404\u79cd\u9ad8\u6781\u6027\u6eb6\u5242\u4e2d)\u90fd\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u7a33\u5b9a\u6027\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-224670\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-1-19.png\" alt=\"\" width=\"593\" height=\"476\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-1-19.png 593w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-1-19-300x241.png 300w\" sizes=\"(max-width: 593px) 100vw, 593px\" \/> \u56fe1|\u8c03\u63a7\u201c\u95e8\u63a7\u673a\u5236\u201d\u7528\u4e8e\u6c14\u4f53\u7684\u9ad8\u6548\u9009\u62e9\u6027\u5206\u79bb<\/p>\n<ul>\n<li>\u201c\u95e8\u63a7\u201d\u73b0\u8c61\u5728\u591a\u5b54\u6750\u6599\u4e2d\u5f97\u5230\u4e86\u5f88\u597d\u7684\u8bc1\u5b9e\u3002\u4e00\u822c\u6765\u8bf4\uff0c\u5438\u9644\/\u89e3\u5438\u662f\u4e00\u4e2a\u5e73\u8861\u7684\u7269\u7406\u548c\u653e\u70ed\u8fc7\u7a0b(\u56fe1)\uff0c\u8fd9\u610f\u5473\u7740\u63d0\u9ad8\u5438\u9644\u6e29\u5ea6\u5c06\u6709\u5229\u4e8e\u5e73\u8861\u5411\u5de6(\u8f83\u5c11\u7684\u6c14\u4f53\u5438\u6536)\uff0c\u800c\u589e\u52a0\u6c14\u4f53\u538b\u529b(\u6c14\u4f53\u6d53\u5ea6)\u5c06\u6709\u5229\u4e8e\u5411\u53f3(\u66f4\u591a\u7684\u6c14\u4f53\u5438\u6536)\u5e73\u8861\u3002<img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-224671\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-2-20.png\" alt=\"\" width=\"600\" height=\"651\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-2-20.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-2-20-276x300.png 276w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/li>\n<\/ul>\n<p>\u56fe2| HOF-FJU-1\u7684\u6676\u4f53\u7ed3\u6784<\/p>\n<ul>\n<li>\u901a\u8fc73\uff0c6-\u4e8c\u6eb4\u5494\u5511(\u56fe2a)\u7684\u6c27\u5316\u5076\u8054\u53cd\u5e94\uff0c\u75313\uff0c3\u2032\uff0c6\uff0c6\u2032-\u56db\u6eb4-9\uff0c9\u2032-\u8054\u5494\u5511(2)\u7684\u6c30\u57fa\u5316\u53cd\u5e94\u5f97\u5230\u56db\u6c30\u57fa-\u8054\u5494\u5511\u6709\u673a\u7ed3\u6784\u5355\u5143(<strong><b>3<\/b><\/strong>)\uff0c\u7ea2\u5916\u5149\u8c31\u3001<sup>1<\/sup>H\u6838\u78c1\u5171\u632f\u3001<sup>13<\/sup>C\u6838\u78c1\u5171\u632f\u3001\u5143\u7d20\u5206\u6790\u548c\u70ed\u91cd\u5206\u6790(TGA)\u8bc1\u5b9e\u4e86\u8fd9\u4e00\u70b9\u3002<\/li>\n<li>\u53e6\u4e00\u65b9\u9762\uff0c\u672c\u6587\u4ece\u70ed\u7684\u4e8c\u7532\u57fa\u7532\u9170\u80fa\u9971\u548c\u6eb6\u6db2\u4e2d\u91cd\u7ed3\u6676\u51fa\u9ad8\u8d28\u91cf\u7684\u5355\u6676\u3002\u5355\u6676X\u5c04\u7ebf\u884d\u5c04\u7814\u7a76\u8868\u660e\uff0cHOF-FJU-1\u5728\u6b63\u4ea4\u7a7a\u95f4\u7fa4Pnn2\u4e2d\u7ed3\u6676\u3002\u5728\u8fd9\u4e2aHOF\u4e2d\uff0c\u5176\u4e0d\u5bf9\u79f0\u5355\u5143\u4e2d\u6709\u4e09\u4e2a\u6676\u4f53\u5b66\u4e0a\u72ec\u7acb\u7684\u56db\u6c30\u57fa-\u8054\u5494\u5511\u5206\u5b50\uff0c\u6bcf\u4e2a\u8054\u5494\u5511\u5355\u5143\u901a\u8fc7\u56db\u5bf9\u6cbfac\u5e73\u9762\u8ddd\u79bb\u4e3a431-3.536\u57c3\u7684CN\u2026H\u2013C\u6c22\u952e\u8fde\u63a5\u5230\u56db\u4e2a\u76f8\u90bb\u7684\u8054\u5494\u5511\uff0c\u5f62\u6210\u5355diamond\u7f51\u683c (\u56fe2b\uff0cc)<\/li>\n<\/ul>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-224672\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-3-19.png\" alt=\"\" width=\"600\" height=\"588\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-3-19.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-3-19-300x294.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe3| C<sub>2<\/sub>H<sub>4<\/sub>\u548cC<sub>2<\/sub>H<sub>6<\/sub>\u5728HOF-FJU-1a\u4e2d\u7684\u5438\u9644\u548c\u5206\u79bb\u3002\u4e0d\u540c\u6e29\u5ea6\u4e0bHOF-FJU-1a\u5bf9C<sub>2<\/sub>H<sub>4<\/sub>\u548cC<sub>2<\/sub>H<sub>6<\/sub>\u7684\u6c14\u4f53\u5438\u9644\u66f2\u7ebf\u4e0eC<sub>2<\/sub>H<sub>4<\/sub>\/C<sub>2<\/sub>H<sub>6<\/sub>\u6df7\u5408\u6c14\u5728\u4e0d\u540c\u6e29\u5ea6\u4e0b\u7684\u7a7f\u900f\u5b9e\u9a8c\u548c\u7a7f\u900f\u5faa\u73af\u5b9e\u9a8c\u3002<\/p>\n<ul>\n<li>\u901a\u8fc7\u6536\u96c6\u5e38\u6e29\u4e0bC<sub>2<\/sub>H<sub>4<\/sub>\u548cC<sub>2<\/sub>H<sub>6<\/sub>\u7684\u5355\u7ec4\u5206\u5438\u9644\u7b49\u6e29\u7ebf\uff0c\u8fdb\u4e00\u6b65\u8003\u5bdf\u4e86HOF-FJU-1a\u5206\u79bbC<sub>2<\/sub>H<sub>4<\/sub>\/C<sub>2<\/sub>H<sub>6<\/sub>\u7684\u6f5c\u529b\u3002\u5728298K\u65f6\uff0cHOF-FJU-1a\u7684C<sub>2<\/sub>H<sub>4<\/sub>\u5438\u9644\u7b49\u6e29\u7ebf\u5728\u76f8\u5bf9\u8f83\u4f4e\u7684\u538b\u529b\u4e0b\u8868\u73b0\u51fa\u660e\u663e\u7684\u9661\u5ced\u53f0\u9636(\u56fe3a)\uff0c\u8fd9\u8868\u660e\u5b83\u5728HOF\u7684\u81f4\u5bc6\u5b54\u9699\u7a7a\u95f4\u4e2d\u88ab\u5f88\u597d\u5730\u5bb9\u7eb3\uff0c\u5373\u4f7f\u5728\u4f4e\u538b\u529b\u548c\u6c14\u4f53\u6d53\u5ea6\u4e0b\u4e5f\u53ef\u4ee5\u8fdb\u884c\u5e73\u8861\u5438\u9644\u3002\u57281bar\u548c298K\u4e0b\u7684\u603bC<sub>2<\/sub>H<sub>4<\/sub>\u5438\u6536\u91cf\u4e3a47cm<sup>3<\/sup>g<sup>\u2212<\/sup><sup>1<\/sup>(2.1 mmolg<sup>\u2212<\/sup><sup>1<\/sup>)\u3002\u5f53\u4f9b\u7ed9\u538b\u529b\u4f4e\u4e8e58bar\u65f6\uff0cHOF-FJU-1a\u5bf9C<sub>2<\/sub>H<sub>6<\/sub>\u7684\u5438\u6536\u53ef\u5ffd\u7565\u4e0d\u8ba1\uff0c\u968f\u540e\u538b\u529b\u589e\u52a0\uff0c\u5b54\u9053\u6253\u5f00\u540e\u5438\u9644\u91cf\u6025\u5267\u4e0a\u5347\uff0c\u603b\u5438\u6536\u91cf\u4e3a38cm<sup>3<\/sup>\u00a0g<sup>\u2212<\/sup><sup>1<\/sup>(1bar)\u3002<\/li>\n<li>\u8fd9\u4e9b\u7ed3\u679c\u8868\u660e\uff0cHOF-FJU-1a\u5728\u76f8\u5bf9\u8f83\u4f4e\u7684\u538b\u529b\u4e0b\u5bf9C<sub>2<\/sub>H<sub>4<\/sub>\/C<sub>2<\/sub>H<sub>6<\/sub>\u5177\u6709\u8f83\u9ad8\u7684\u5206\u79bb\u6f5c\u529b\u3002\u8003\u8651\u5230\u95e8\u63a7\u538b\u529b\u5728\u9ad8\u6e29\u4e0b\u4f1a\u589e\u52a0\uff0c\u672c\u6587\u8fdb\u4e00\u6b65\u7814\u7a76\u4e86HOF-FJU-1a\u5728318K\u548c333K\u4e0b\u5bf9C<sub>2<\/sub>H<sub>4<\/sub>\u548cC<sub>2<\/sub>H<sub>6<\/sub>\u7684\u5438\u9644\u884c\u4e3a(\u56fe3b\uff0cc)\u3002\u4e8b\u5b9e\u4e0a\uff0c\u7531\u4e8e333K\u548c1bar\u4e0b\u7684\u95e8\u63a7\u538b\u529b\u589e\u52a0\uff0cHOF-FJU-1a\u5bf9C<sub>2<\/sub>H<sub>6<\/sub>\u7684\u5438\u6536\u53ef\u5ffd\u7565\u4e0d\u8ba1\uff0c\u4e3a1cm<sup>3<\/sup>g<sup>\u2212<\/sup><sup>1<\/sup>(0.04mmolg<sup>\u2212<\/sup><sup>1<\/sup>)\uff0c\u4f4e\u4e8eUTSA-280(0.1mmolg<sup>\u2212<\/sup><sup>1<\/sup>)\uff0c\u5e76\u4e14C<sub>2<\/sub>H<sub>4<\/sub>\u5438\u9644\u51e0\u4e4e\u4e0d\u53d8\uff0c\u5438\u9644\u91cf\u4e3a36cm<sup>3<\/sup>\u00a0g<sup>\u2212<\/sup><sup>1<\/sup>(1.6mmolg<sup>\u2212<\/sup><sup>1<\/sup>)\u3002<img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-224673\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-4-17.png\" alt=\"\" width=\"600\" height=\"438\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-4-17.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/07\/\u56fe\u7247-4-17-300x219.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/li>\n<\/ul>\n<p>\u56fe4| HOF-FJU-1\u22190.94 C<sub>2<\/sub>H<sub>4<\/sub>\u7684\u5355\u6676\u7ed3\u6784<\/p>\n<ul>\n<li>\u672c\u6587\u5bf9\u8d1f\u8f7dC<sub>2<\/sub>H<sub>4<\/sub>\u7684HOF-FJU-1a\u6837\u54c1\u8fdb\u884c\u4e86\u5355\u6676X\u5c04\u7ebf\u884d\u5c04\u6d4b\u91cf\uff0c\u4ee5\u786e\u5b9aC<sub>2<\/sub>H<sub>4<\/sub>\u7684\u7ed3\u5408\u6784\u8c61\u3002\u5728100K\u4e0b\u6536\u96c6\u4e86HOF-FJU-1\u221994 C<sub>2<\/sub>H<sub>4<\/sub>\u7684\u6570\u636e\uff0c\u786e\u5b9a\u4e86\u4e09\u4e2a\u7ed3\u6676\u5b66\u4e0a\u72ec\u7acb\u7684C<sub>2<\/sub>H<sub>4<\/sub>\u5206\u5b50\u7684\u4f4d\u7f6e(\u56fe4a)\u3002<\/li>\n<li>C<sub>2<\/sub>H<sub>4<\/sub>\u5206\u5b50\u6cbf\u4e00\u7ef4\u5b54\u9053\u5206\u6563\u826f\u597d\uff0c\u901a\u8fc7C-H\u00b7\u00b7\u00b7\u03c0\u4e0e\u9aa8\u67b6(3.701-4.124 \u57c3) \u5f62\u6210\u4e3b-\u5ba2\u4f53\u95f4\u6c22\u952e\u4f5c\u7528(\u56fe4b\uff0cc)\u3002<\/li>\n<\/ul>\n<p><strong>\u7ed3\u8bed<\/strong><\/p>\n<p>\u7efc\u4e0a\u6240\u8ff0\uff0c\u672c\u6587\u901a\u8fc7\u8c03\u8282\u4e0d\u540c\u6e29\u5ea6\u4e0b\u7684\u5438\u9644\u95e8\u63a7\u538b\u529b\uff0c\u6210\u529f\u5730\u5b9e\u73b0\u4e86\u4e00\u79cd \u201c\u521a\u67d4\u5e76\u6d4e\u201d\u7684\u6c22\u952e\u6709\u673a\u9aa8\u67b6\uff08HOF-FJU-1\uff09\uff0c\u6700\u7ec8\u5b9e\u73b0\u4e86\u4e59\u70ef\u548c\u4e59\u70f7\u7684\u9ad8\u6548\u5206\u79bb\u3002\u8fd9\u79cd\u65b0\u65b9\u6cd5\u6210\u529f\u5730\u51cf\u5c11\u4e86\u4e59\u70f7\u7684\u5171\u5438\u9644\uff0c\u540c\u65f6\u6700\u5927\u91cf\u7684\u4fdd\u7559\u4e59\u70ef\u5438\u9644\uff0c\u4ece\u800c\u5927\u5927\u63d0\u9ad8\u4e86\u4e59\u70ef\/\u4e59\u70f7\u5728\u9ad8\u6e29\u4e0b\u7684\u5206\u79bb\u6027\u80fd\u3002\u5728333 K\u7684\u56fa\u5b9a\u5e8a\u67f1\u4e2d\uff0c\u8fd9\u79cdHOF\u6750\u6599\u53ef\u4ee5\u5f88\u5bb9\u6613\u5730\u4eceC<sub>2<\/sub>H<sub>4<\/sub>\/C<sub>2<\/sub>H<sub>6<\/sub>\u6df7\u5408\u7269\u4e2d\u751f\u4ea7\u51fa\u9ad8\u7eaf\u5ea6\u7684C<sub>2<\/sub>H<sub>4<\/sub>\uff08&gt;99%\u7eaf\u5ea6\uff09\uff0c\u8fd9\u4e00\u6e29\u5ea6\u63a5\u8fd1\u5b9e\u9645\u5206\u79bb\u4e59\u70ef\u4e59\u70f7\u6df7\u5408\u6c14\u7684\u5206\u79bb\u6e29\u5ea6\uff0c\u8868\u660e\u8fd9\u79cd\u201c\u521a\u67d4\u5e76\u6d4e\u201d\u7684\u591a\u5b54\u6750\u6599\u5728\u5de5\u4e1aC<sub>2<\/sub>H<sub>4<\/sub>\/C<sub>2<\/sub>H<sub>6<\/sub>\u5206\u79bb\u4e2d\u5177\u6709\u5149\u660e\u524d\u666f\u3002\u6b64\u5916\uff0cHOF-FJU-1\u4e0d\u4ec5\u5177\u6709\u4f18\u5f02\u7684\u70ed\u7a33\u5b9a\u6027\uff0c\u800c\u4e14\u5728\u5e38\u89c1\u6709\u673a\u6eb6\u5242\u548cpH\u503c\u8303\u56f4\u4e3a1\u523014\u7684\u6eb6\u6db2\u4e2d\u4e5f\u7a33\u5b9a\uff0c\u5373\u4f7f\u572812 M HCl\u548c10 M NaOH\u7684\u6eb6\u6db2\u4e2d\u4e5f\u662f\u5982\u6b64\u3002\u8fd9\u4e9b\u7ed3\u679c\u63ed\u793a\u4e86HOF\u57fa\u6750\u6599\u5728\u5b9e\u73b0\u91cd\u8981\u6c14\u4f53\u5206\u79bb\u65b9\u9762\u7684\u5de8\u5927\u5e94\u7528\u6f5c\u529b\uff0c\u5e76\u5c06\u8fdb\u4e00\u6b65\u63a8\u52a8HOF\u6750\u6599\u7684\u53d1\u5c55\u3002<\/p>\n<p><strong>\u4f5c\u8005\u4ecb\u7ecd<\/strong><\/p>\n<p>\u5f20\u7ae0\u9759\uff0c\u5973\uff0c1979\u5e74\u751f\uff0c\u535a\u58eb\uff0c\u7814\u7a76\u5458\uff0c\u535a\u58eb\u751f\u5bfc\u5e08\u3002\u5165\u9009\u798f\u5efa\u7701\u767e\u5343\u4e07\u4eba\u624d\u5de5\u7a0b\u3001\u798f\u5efa\u7701\u6770\u9752\u3001\u798f\u5efa\u7701\u65b0\u4e16\u7eaa\u4f18\u79c0\u4eba\u624d\u3001\u798f\u5efa\u7701\u9ad8\u6821\u6770\u51fa\u9752\u5e74\u4eba\u624d\uff0c\u8363\u83b7\u798f\u5efa\u7701\u8fd0\u76db\u9752\u5e74\u79d1\u6280\u5956\u3001\u798f\u5efa\u7701\u9752\u5e74\u79d1\u6280\u5956\u3002\u4ece\u4e8b\u6676\u6001\u591a\u5b54\u6750\u6599\u7684\u8bbe\u8ba1\u4e0e\u5408\u6210\uff0c\u7528\u4e8e\u6c14\u4f53\u5438\u9644\u5206\u79bb\u3001\u79bb\u5b50\u5bfc\u4f53\u7b49\u65b9\u9762\u7814\u7a76\u3002\u72ec\u7acb\u5f00\u5c55\u5de5\u4f5c\u540e\uff0c\u4ee5\u901a\u8baf\u4f5c\u8005\u5728Nature Chemistry., Science Advance., JACS (7\u7bc7), Angew. Chem. Int. Ed., Adv Mater.,\u7b49\u671f\u520a\u53d1\u8868\u8bba\u658760\u4f59\u7bc7\u3002\u5355\u7bc7\u6700\u9ad8\u5f15\u7528500\u4f59\u6b21\u3002ESI 1%\u9ad8\u88ab\u5f15\u8bba\u65878\u7bc7\uff0cH-index 39\u3002\u4e3b\u6301\u56fd\u5bb6\u53ca\u7701\u90e8\u7ea7\u9879\u76ee15\u9879\u3002<\/p>\n<p>\u76f8\u5173\u4f18\u8d28\u6587\u732e\u63a8\u8350\uff1a<\/p>\n<p>1\uff1aLizhen Liu,<sup>+<\/sup>\u00a0Zizhu Yao,<sup>+<\/sup>\u00a0Yingxiang Ye, Yike Yang, Quanjie Lin,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>,* Michael O\u2019Keeffe, Shengchang Xiang,* Integrating pillared-layer strategy and pore-space partition method to construct multicomponent MOFs for C<sub>2<\/sub>H<sub>2<\/sub>\/CO<sub>2<\/sub>\u00a0separation, <strong><em><b><i>Journal of the American Chemical Society<\/i><\/b><\/em><\/strong><em><i>\u00a0<\/i><\/em><strong><b>2020<\/b><\/strong>,\u00a0<em><i>142<\/i><\/em>(20), 9258-9266.<\/p>\n<p>2\uff1aYingxiang Ye, Lingshan Gong, Shengchang Xiang,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>,* Banglin Chen*, Metal-organic frameworks as a versatile platform for proton conductors,\u00a0<strong><em><b><i>Advanced Materials <\/i><\/b><\/em><\/strong><strong><b>2020<\/b><\/strong>, 1907090.<\/p>\n<p>3\uff1aBin Wang, Rui-Biao Lin,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>,* Shengchang Xiang, Banglin Chen,* Hydrogen-bonded organic frameworks as a tunable platform for functional materials,\u00a0<strong><em><b><i>Journal of the American Chemical Society <\/i><\/b><\/em><\/strong><strong><b>2020<\/b><\/strong>, 142(34): 14399-14416.<\/p>\n<p>4: Bin Wang, Ru He, Lin-Hua Xie, Zu-Jin Lin, Xin Zhang, Jing Wang, Hongliang Huang,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>*, Kirk S. Schanze, Jian Zhang, Shengchang Xiang, Banglin Chen*, Microporous hydrogen-bonded organic framework for highly efficient turn-up fluorescent sensing of aniline,\u00a0<strong><em><b><i>Journal of the American Chemical Society <\/i><\/b><\/em><\/strong><strong><b>2020<\/b><\/strong>,142(28): 12478-12485.<\/p>\n<p>5\uff1a\u00a0Zizhu Yao,<sup>+<\/sup>\u00a0Liang Pan,<sup>+<\/sup>\u00a0Lizhen Liu, Jindan Zhang, Quanjie Lin, Yingxiang Ye,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>,* Shengchang Xiang,* Banglin Chen,* Simultaneous implementation of resistive switching and rectifying effects in a metal-organic framework with switched hydrogen bond pathway,\u00a0<strong><em><b><i>Science Advances <\/i><\/b><\/em><\/strong><strong><b>2019<\/b><\/strong>, 5(8): eaaw4515.<\/p>\n<p>6\uff1aYingxiang Ye, Zhenlin Ma, Rui-Biao Lin, Rajamani Krishna, Wei Zhou, Quanjie Lin,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>,* Shengchang Xiang,* Banglin Chen,* Pore space partition within a metal-organic framework for highly efficient C<sub>2<\/sub>H<sub>2<\/sub>\/CO<sub>2<\/sub>\u00a0separation.\u00a0<strong><em><b><i>Journal of the American Chemical Society<\/i><\/b><\/em><\/strong>\u00a02019,\u00a0<strong><b>141<\/b><\/strong>, 4130-4136.<\/p>\n<p>7: \u00a0Yuanchao Lv*, Zhile Xiong, Zizhu Yao, Yisi Yang, Shengchang Xiang,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>*, Yong Sheng Zhao*, Steric-hindrance-controlled laser switch based on pure metal\u2013organic framework microcrystals,\u00a0<strong><em><b><i>Journal of the American Chemical Society <\/i><\/b><\/em><\/strong>2019, <strong><b>141<\/b><\/strong>, 51, 19959-19963.<\/p>\n<p>8: \u00a0Yingxiang Ye, Weigang Guo, Lihua Wang, Ziyin Li, Zhengju Song, Jun Chen,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>*, Shengchang Xiang, Banglin Chen,* Straightforward loading of imidazole molecules into metal\u2013organic framework for high proton conduction,\u00a0<strong><em><b><i>Journal of the American Chemical Society <\/i><\/b><\/em><\/strong><strong><b>2017<\/b><\/strong>,\u00a0<em><i>139<\/i><\/em>, 15604\u221215607.<\/p>\n<p>9: \u00a0Yingxiang Ye, Liuqin Zhang, Qinfang Peng, Guan-E Wang, Yangcan Shen, Ziyin Li, Lihua Wang, Xiuling Ma, Qian-Huo Chen,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>,* Shengchang Xiang,*\u00a0High anhydrous proton conductivity of imidazole-loaded mesoporous polyimides over a wide range from subzero to moderate temperature,\u00a0<strong><em><b><i>Journal of the American Chemical Society <\/i><\/b><\/em><\/strong><strong><b>2015<\/b><\/strong>,\u00a0<em><i>137<\/i><\/em>(2), 913\u2013918.<\/p>\n<p>10: Xi Fan, Furong Yuan, Dejing Li, Shuai Chen, Zhibin Cheng,\u00a0<strong><b>Zhangjing Zhang<\/b><\/strong>,* Shengchang Xiang, Shuang-Quan Zang, Jian Zhang, Lei Zhang,* Threefold collaborative stabilization of Ag<sub>14<\/sub>-nanorods by hydrophobic Ti<sub>16<\/sub>-oxo clusters and alkynes: Designable assembly and solid-state optical-limiting application,\u00a0<strong><em><b><i>Angewandte Chemie International Edition <\/i><\/b><\/em><\/strong><strong><b>2021<\/b><\/strong>, 60,12949\u201312954.<\/p>\n<p>\u672c\u6587\u7531SSC\u4f9b\u7a3f\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u7b2c\u4e00\u4f5c\u8005\uff1aYisi Yang\uff0cLibo Li, Rui-Biao Lin \u901a\u8baf\u4f5c\u8005\uff1aZhangjing Zhang\uff0cShengchang Xiang\uff0cBangl&#8230;<\/p>\n","protected":false},"author":11454,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-224669","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/224669"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/11454"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=224669"}],"version-history":[{"count":2,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/224669\/revisions"}],"predecessor-version":[{"id":224675,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/224669\/revisions\/224675"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=224669"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=224669"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=224669"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}