{"id":225181,"date":"2021-07-30T06:35:34","date_gmt":"2021-07-29T22:35:34","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=225181"},"modified":"2021-07-29T18:35:48","modified_gmt":"2021-07-29T10:35:48","slug":"%e7%8e%8b%e8%bf%9e%e6%b4%b2%e5%bd%ad%e7%94%9f%e6%9d%b0nano-micro-lett-%e5%ae%bd%e6%b8%a9%e5%ba%a6%e8%8c%83%e5%9b%b4%e5%ba%94%e7%94%a8%e7%9a%84%e9%93%9d%e7%a6%bb%e5%ad%90%e7%94%b5%e6%b1%a0%e6%ad%a3","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=225181","title":{"rendered":"\u738b\u8fde\u6d32&\u5f6d\u751f\u6770Nano-Micro Lett.:\u5bbd\u6e29\u5ea6\u8303\u56f4\u5e94\u7528\u7684\u94dd\u79bb\u5b50\u7535\u6c60\u6b63\u6781\u6750\u6599\u8bbe\u8ba1"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u53ef\u5145\u7535\u94dd\u79bb\u5b50\u7535\u6c60 (AIBs) \u56e0\u5176\u5177\u6709\u5730\u58f3\u4e0a\u6700\u4e30\u5bcc\u7684\u91d1\u5c5e\u8d44\u6e90\u3001\u6210\u672c\u4f4e\u3001\u8fd0\u884c\u5b89\u5168\u3001\u4f53\u79ef\u5bb9\u91cf\u6700\u9ad8\u7b49\u4f18\u70b9\uff0c\u662f\u4e0b\u4e00\u4ee3\u6700\u5177\u4ee3\u8868\u6027\u7684\u7535\u6c60\u4e4b\u4e00\u3002\u4ee5\u524d\uff0cAl\u8d1f\u6781\u4e0a\u7684\u5185\u5728\u7684\u52a0\u6c22\u4f5c\u7528\u548c\u6c34\u7cfb\u4f53\u7cfb\u4e2d\u949d\u5316\u6c27\u5316\u5c42\u7684\u5f62\u6210\u663e\u8457\u964d\u4f4e\u4e86\u7535\u6c60\u7535\u538b\u548c\u5faa\u73af\u6548\u7387\u3002\u4f46\u81ea\u4ece\u4f7f\u7528\u79bb\u5b50\u6db2\u4f53 (IL) \u7535\u89e3\u8d28\u6765\u907f\u514d\u8fd9\u4e9b\u95ee\u9898\uff0c\u5728IL\u57faAIB\u4e2d\u63d0\u51fa\u4e86\u5404\u79cd\u6b63\u6781\u6750\u6599\uff0c\u5305\u62ec\u77f3\u58a8\u57fa\u6750\u6599\u3001\u91d1\u5c5e\u6c27\u5316\u7269\/\u786b\u5316\u7269\/\u7852\u3001MXene\u548c\u805a\u5408\u7269\u57fa\u6750\u6599\uff0c\u4ee5\u8fdb\u4e00\u6b65\u6539\u5584\u975e\u6c34\u7cfbAIBs\u3002\u7136\u800c\uff0c\u5728\u5b9e\u9645\u5e94\u7528\u4e2d\uff0c\u57fa\u4e8eIL\u7684AIBs\u4ecd\u7136\u9047\u5230\u4e86\u4e00\u4e9b\u5173\u952e\u95ee\u9898\uff0c\u5373\u7535\u6781\u6750\u6599\u7684\u8870\u89e3\u3001\u77ed\u671f\u7a33\u5b9a\u6027\u548c\u4f4e\u901f\u7387\u5bb9\u91cf\uff08\u4f8b\u5982\u5927\u591a\u6570\u91d1\u5c5e\u786b\u9178\u76d0\u6b63\u6781\u5177\u6709\u4f4e\u500d\u7387\u5bb9\u91cf\uff09\u7b49\u95ee\u9898\u3002\u56e0\u6b64\uff0c\u975e\u5e38\u9700\u8981\u5728\u53ef\u5145\u7535AIBs \u4e2d\u6784\u5efa\u5177\u6709\u9ad8\u5bb9\u91cf\u3001\u957f\u5faa\u73af\u7a33\u5b9a\u6027\u548c\u500d\u7387\u6027\u80fd\u589e\u5f3a\u7684\u65b0\u578b\u7ed3\u6784\u7535\u6781\u6750\u6599\u3002\u540c\u65f6\uff0c\u65b0\u5f00\u53d1\u7684ILs\u5177\u6709\u8f83\u5bbd\u7684\u5de5\u4f5c\u6e29\u5ea6\u7a97\u53e3\uff0c\u4f46\u7531\u4e8e\u5176\u56fa\u6709\u7684\u4f4e\u5bb9\u91cf\uff0c\u65b0\u5174\u7684\u9ad8\u5bb9\u91cf\u91d1\u5c5e\u786b\u9178\u76d0\u7535\u6781\u662f\u5f88\u6709\u524d\u9014\u7684\u5168\u6c14\u5019\u5019\u9009\u7269\uff0c\u800c\u5b83\u4eec\u7684\u4f4e\u79bb\u5b50\/\u7535\u5b50\u7535\u5bfc\u7387\u548c\u4f4e\u5faa\u73af\u7a33\u5b9a\u6027\u9700\u8981\u88ab\u4f18\u5316\uff0c\u4ee5\u7528\u4e8e\u5168\u6c14\u5019\u7684AIBs\u3002FeS2<\/sub>\u4f5c\u4e3a\u4e00\u79cd\u5730\u7403\u4e30\u5bcc\u548c\u4f4e\u6210\u672c\u77ff\u7269\uff0c\u5177\u6709\u9ad8\u7406\u8bba\u5bb9\u91cf\u548c\u826f\u597d\u7684\u79bb\u5b50\/\u7535\u5b50\u4f20\u5bfc\u6027\uff0c\u662f\u5168\u6c14\u5019\u4e0b\u7684\u5546\u4e1a\u6b63\u6781\u6750\u6599\uff0c\u7279\u522b\u662f\u5728\u4f4e\u6e29\u4e0b\u3002\u4f46\u76f8\u5173\u7684\u6587\u732e\u8fd8\u672a\u62a5\u9053\u4f7f\u7528FeS2<\/sub>\u4f5c\u4e3aAIBs\u7684\u5168\u6c14\u5019\u7535\u6781\u3002<\/p>\n

\u8fd1\u65e5\uff0c\u6fb3\u5927\u5229\u4e9a<\/strong>\u6606\u58eb\u5170\u5927\u5b66\u738b\u8fde\u6d32\u6559\u6388<\/strong>\u8054\u5408\u5357\u4eac\u822a\u7a7a\u822a\u5929\u5927\u5b66\u5f6d\u751f\u6770\u6559\u6388<\/strong>\uff08<\/strong>\u5171\u540c<\/strong>\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u8bbe\u8ba1\u4e00\u79cd\u81ea\u652f\u6491\u4e14\u65e0\u7c98\u5408\u5242\u7684\u78b3\u7eb3\u7c73\u7ba1 (CNT) \u5305\u88f9\u91d1\u5c5e\u6709\u673a\u6846\u67b6 (MOF) \u884d\u751f\u7684\u78b3\u5305\u8986FeS2<\/sub>\u00a0(FeS2<\/sub>@C\/CNT) \u4f5c\u4e3a\u9ad8\u5bb9\u91cf\u5168\u6c14\u5019AIBs\uff0c\u5176\u4e2d\u7684\u91d1\u5c5e\u786b\u5316\u7269\u6b63\u6781\u5177\u6709\u51fa\u8272\u7684\u67d4\u6027\u3002\u7814\u7a76\u8868\u660e\uff0c\u65e0\u7c98\u5408\u5242\u548c\u81ea\u652f\u6491\u86cb\u9ec4-\u58f3\u7ed3\u6784\u6d88\u9664\u4e86\u4e0eIL\u7535\u89e3\u8d28\u7c98\u5408\u5242\/\u96c6\u6d41\u4f53\u4e4b\u95f4\u7684\u526f\u53cd\u5e94\uff0c\u548c\u62b5\u6297\u4e86\u5faa\u73af\u8fc7\u7a0b\u4e2d\u7684\u4f53\u79ef\u81a8\u80c0\u3002\u540c\u65f6\uff0c\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba (DFT) \u6a21\u62df\u8fd8\u9a8c\u8bc1\u4e86\u7cbe\u5fc3\u8bbe\u8ba1\u7684N\u63ba\u6742\u78b3\u58f3\u4e0d\u4ec5\u9650\u5236\u4e86FeS2<\/sub>\u7c89\u788e\uff0c\u800c\u4e14\u4e5f\u6709\u5229\u4e8e\u6d3b\u6027\u79bb\u5b50\u671d\u5411FeS2<\/sub>@C\/CNT\u7684\u52a8\u529b\u5b66\u8fc7\u7a0b\u3002\u6b64\u5916\uff0c\u9ad8\u5bfc\u7535\u6027\u78b3\u57fa\u5e95\u548c\u591a\u5b54\u7ed3\u6784\u663e\u8457\u6539\u5584\u4e86\u7535\u5b50\/\u79bb\u5b50\u6269\u6563\u9014\u5f84\u548c\u7535\u89e3\u8d28\u6e17\u900f\uff0c\u5177\u6709\u51fa\u8272\u7684\u5168\u6c14\u5019\u6027\u80fd\uff08-25\u81f350\u2103\uff09\uff0c\u6709\u52a9\u4e8e\u63d0\u9ad8\u5bb9\u91cf\u4fdd\u6301\u7387\uff08\u9ad8\u4e8e117 mAh g-1<\/sup>\uff09\u3002\u5373\u4f7f\u5728-25\u2103\u7684\u4f4e\u6e29\u6761\u4ef6\u4e0b\u4e5f\u5177\u6709\u4f18\u5f02\u7684\u500d\u7387\u5bb9\u91cf\u3002\u8fd9\u79cdFeS2<\/sub>@C\/CNT\u7684\u65b0\u9896\u8bbe\u8ba1\u4e3a\u9ad8\u6027\u80fd\u3001\u5168\u6c14\u5019\u548c\u67d4\u6027\u7684AIBs\u94fa\u5e73\u4e86\u53d1\u5c55\u9053\u8def\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cAllClimate AluminumIon Batteries Based on BinderFree MOFDerived FeS<\/strong>2<\/sub><\/strong>@C\/CNT Cathode<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nano-Micro Lett.<\/i><\/em><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe<\/b><\/strong>\u4e00<\/b><\/strong>\u3001FeS<\/b><\/strong>2<\/b><\/sub><\/strong>@C\/CNT\u7684\u5408\u6210\u548c\u8868\u5f81<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

\uff08a\uff0cb\uff09Fe-MOF\u3001FeS2<\/sub>@C\u6838\u58f3\u7eb3\u7c73\u7403\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c-e\uff09FeS2<\/sub>@C\u6838\u58f3\u7eb3\u7c73\u7403\u7684TEM\u548cHR-TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08f\uff09FeS2<\/sub>@C\u7684\u5143\u7d20\u6620\u5c04\uff1b<\/p>\n

\uff08g\uff0ch\uff09FeS2<\/sub>@C\/CNT\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08i\uff09\u5e26\u6709\u6298\u53e0\u7535\u6781\u63d2\u56fe\u7684\u67d4\u6027FeS2<\/sub>@C\/CNT\u7535\u6781\u7684\u5e94\u529b-\u5e94\u53d8\u66f2\u7ebf\u3002<\/p>\n

\u56fe<\/b><\/strong>\u4e8c<\/b><\/strong>FeS<\/b><\/strong>2<\/b><\/sub><\/strong>@C\/CNT<\/b><\/strong>\u7684\u7535\u5316\u5b66\u6027\u80fd<\/b><\/strong>\"\"<\/p>\n

\u00a0<\/b><\/strong>\uff08a\uff09FeS2<\/sub>@C\/CNT\u7684\u5faa\u73af\u4f0f\u5b89\u66f2\u7ebf\uff1b<\/p>\n

\uff08b\uff09FeS2<\/sub>@C\/CNT\u548cFeS2<\/sub>\/C\u7684\u6052\u7535\u6d41\u5145\u653e\u7535\u66f2\u7ebf\uff1b<\/p>\n

\uff08c\uff09FeS2<\/sub>@C\/CNT\u548cFeS2<\/sub>\/C\u4e0eAIBs \u4e2d\u4ee3\u8868\u6027\u6b63\u6781\u500d\u7387\u5bb9\u91cf\u7684\u5bf9\u6bd4\uff1b<\/p>\n

\uff08d\uff09FeS2<\/sub>@C\/CNT\u5728100 mA g-1<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u5faa\u73af\u6027\u80fd\uff1b<\/p>\n

\uff08e\uff09\u57281 A g-1<\/sup>\u7684\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0cFeS2<\/sub>@C\/CNT\u7535\u6781\u7684\u653e\u7535\u5bb9\u91cf\u548c\u5e93\u4ed1\u6548\u7387\u3002<\/p>\n

\u56fe<\/b><\/strong>\u4e09<\/b><\/strong>\u3001<\/b><\/strong>\u673a\u7406\u7814\u7a76<\/b><\/strong>\u548cDFT<\/b><\/strong>\u8ba1\u7b97<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

\uff08a\uff09AIBs\u5145\u653e\u7535\u8fc7\u7a0b\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u6676\u80de\u4e2dFeS2<\/sub>\u4f53\u79ef\u81a8\u80c0\u7684\u6a21\u62df\uff1b<\/p>\n

\uff08c\uff0cd\uff09FeS2<\/sub>\u5728N-C\u4e0a\u7684\u6700\u4f73FeS2<\/sub>\u548c\u5438\u9644\u4f4d\u70b9\u7684\u53ef\u884c\u6027\u6a21\u578b\uff1b<\/p>\n

\uff08e-f\uff09Al\u79bb\u5b50\u5728FeS2<\/sub>\u4e0a\u4ee5\u53caN-C\u548cFeS2<\/sub>\u4e4b\u95f4\u7684\u6700\u4f73\u5438\u9644\u4f4d\u70b9\u7684\u53ef\u884c\u6a21\u578b\uff1b<\/p>\n

\uff08g\uff09N-C\u548cFeS2<\/sub>\u4e4b\u95f4 Al \u79bb\u5b50\u7684\u4e0d\u540c\u7535\u8377\u5bc6\u5ea6\u3002<\/p>\n

\u56fe<\/b><\/strong>\u56db<\/b><\/strong>\u3001<\/b><\/strong>FeS<\/b><\/strong>2<\/b><\/sub><\/strong>@C\/CNT<\/b><\/strong>\u5728AIB<\/b><\/strong>s<\/b><\/strong>\u4e2d\u7684\u5168\u6c14\u5019\u6027\u80fd<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

\uff08a\uff09\u7535\u6d41\u5bc6\u5ea6\u4e3a100 mA g-1<\/sup>\u4e0b\uff0cFeS2<\/sub>@C\/CNT\u5728\u4e00\u5b9a\u6e29\u5ea6\u8303\u56f4\u5185\u7684\u5145\u653e\u7535\u66f2\u7ebf\uff1b<\/p>\n

\uff08b\uff09FeS2<\/sub>@C\/CNT\u548cFeS2<\/sub>\/C\u7535\u6781\u5728-25\u81f350\u2103\u7684\u6e29\u5ea6\u4e0b\uff0c\u7535\u6d41\u5bc6\u5ea6\u4e3a 100 mA g-1<\/sup>\u00a0\u65f6\u7684\u5bb9\u91cf\u4fdd\u6301\u7387\uff1b<\/p>\n

\uff08c\uff09\u5728-25\u2103\u3001100 mA g-1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0cFeS2<\/sub>@C\/CNT\u7684\u7b2c5\u6b21\u3001\u7b2c50\u6b21\u548c\u7b2c100\u6b21\u5145\u653e\u7535\u66f2\u7ebf\uff1b<\/p>\n

\uff08d\uff09\u5728-25\u2103\u4e0b\uff0cFeS2<\/sub>@C\/CNT\u5728AIBs\u4e2d\u7684\u500d\u7387\u6027\u80fd\uff0c\u4ee5\u53ca\u5176\u4ed6\u4f4e\u6e29\u7535\u6781\u5728\u4e0d\u540c\u7684\u7535\u6c60\u7cfb\u7edf\u4e2d\u7684\u6027\u80fd\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u672c\u6587\u5236\u5907\u4e86\u4e00\u79cd\u81ea\u652f\u6491\u548c\u65e0\u7c98\u7ed3\u5242\u7684FeS2<\/sub>@C\/CNT\uff0c\u5e76\u9996\u6b21\u5e94\u7528\u4e8e\u5168\u6c14\u5019\u7684\u94dd\u79bb\u5b50\u7535\u6c60\u3002\u4f18\u5316\u540e\u7684\u7535\u6781\u8868\u73b0\u51fa\u9ad8\u5bb9\u91cf\u548c\u4f18\u5f02\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0c\u4f18\u5f02\u7684\u5168\u6c14\u5019\u5faa\u73af\u80fd\u529b\uff0c\u5927\u5927\u4fc3\u8fdb\u4e86\u94dd\u79bb\u5b50\u7535\u6c60\u7684\u53d1\u5c55\u3002\u57fa\u4e8e\u8be6\u7ec6\u7684\u8868\u5f81\u548cDFT\u6a21\u62df\uff0c\u8868\u660e\u63d0\u5347\u7535\u5316\u5b66\u6027\u80fd\u4e3b\u8981\u6709\u4e24\u4e2a\u539f\u56e0\uff1a\u4f18\u8d8a\u7684\u6838\u58f3\u7ed3\u6784\u9650\u5236\u4e86\u4f53\u79ef\u81a8\u80c0\u548c\u7535\u6781\u7c89\u788e\uff0c\u5177\u6709\u826f\u597d\u7684\u7535\u6781\u5faa\u73af\u7a33\u5b9a\u6027\uff1b\u7cbe\u5fc3\u8bbe\u8ba1\u7684\u5206\u5c42\u7ed3\u6784\u548c\u5177\u6709CNT\u77e9\u9635\u7684N-C\u6d82\u5c42\u4e0d\u4ec5\u5141\u8bb8\u6d3b\u6027\u4f4d\u70b9\u5927\u91cf\u66b4\u9732\uff0c\u800c\u4e14\u5373\u4f7f\u5728\u8f83\u5bbd\u7684\u6e29\u5ea6\u7a97\u53e3\u4e0b\uff0c\u4e5f\u6709\u5229\u4e8e\u6539\u5584\u79bb\u5b50\/\u7535\u5b50\u7535\u5bfc\u7387\u7684\u52a8\u529b\u5b66\u8fc7\u7a0b\u3002\u6b64\u5916\uff0c\u65e0\u7c98\u7ed3\u5242\u548c\u81ea\u652f\u6491\u7684\u7279\u5f81\u51cf\u5c11\u4e86\u6d3b\u6027\u7269\u8d28\u7684\u5d29\u89e3\u548c\u8d1f\u53cd\u5e94\u3002\u5e76\u663e\u8457\u63d0\u9ad8\u4e86\u5728\u73af\u5883\u6e29\u5ea6\u4e0b\u7684\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u3002\u672c\u6587\u4e5f\u4e3a\u5728\u5404\u79cd\u6c14\u5019\u5e94\u7528\u4e2d\u53ef\u6269\u5c55\u548c\u53ef\u5b58\u5728\u7684\u9ad8\u6027\u80fd\u590d\u5408\u7535\u6781\u7684\u5408\u7406\u8bbe\u8ba1\u63d0\u4f9b\u4e86\u65b0\u7684\u89c1\u89e3\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a\u201c<\/strong>All-Climate Aluminum-Ion Batteries Based on Binder-Free MOF-Derived FeS<\/u><\/strong>2<\/sub><\/u><\/strong>@C\/CNT Cathode<\/u><\/strong><\/a>\u201d(<\/strong>Nano-Micro Lett.<\/i><\/em><\/strong>\uff0c<\/b><\/strong>202<\/strong>1<\/strong>\uff0c<\/strong>10.1007\/s40820-021-00682-8<\/strong>)<\/strong><\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4ebaCYM\u7f16\u8bd1\u4f9b\u7a3f\u3002\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

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