{"id":226411,"date":"2021-09-02T06:30:42","date_gmt":"2021-09-01T22:30:42","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=226411"},"modified":"2021-09-01T17:20:23","modified_gmt":"2021-09-01T09:20:23","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e7%8e%8b%e6%b5%b7%e6%a2%81acc-chem-res-%e7%bb%bc%e8%bf%b0%e7%94%a8%e4%ba%8eco2%e8%bf%98%e5%8e%9f%e5%8f%8d%e5%ba%94%e7%9a%84%e9%87%91%e5%b1%9e%e9%85%9e","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=226411","title":{"rendered":"\u738b\u6d77\u6881Acc. Chem. Res.\u7efc\u8ff0:\u7528\u4e8eCO2\u8fd8\u539f\u53cd\u5e94\u7684\u91d1\u5c5e\u915e\u83c1\u5f02\u76f8\u5206\u5b50\u50ac\u5316\u5242"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

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\u8fd1\u65e5\uff0c\u7f8e\u56fd<\/strong>\u8036\u9c81\u5927\u5b66\u738b\u6d77\u6881\u6559\u6388<\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u6df1\u5165\u7406\u89e3\u4e86\u7528\u4e8e\u7535\u5316\u5b66\u8fd8\u539f CO2<\/sub>\u7684\u5f02\u76f8\u91d1\u5c5e\u915e\u83c1\u5206\u5b50\u50ac\u5316\u5242\u3002\u4ece\u5bf9CO2<\/sub>\u8fd8\u539f\u4e3aCO\u7684\u7535\u50ac\u5316\u6d3b\u6027\u7684\u5236\u5907\u65b9\u6cd5\u548c\u6750\u6599\u7ed3\u6784\u7684\u4f18\u5316\uff0c\u53d1\u73b0\u6d3b\u6027\u6750\u6599\u7684\u5206\u5b50\u7ea7\u5206\u6563\u548c\u8f7d\u4f53\u7684\u9ad8\u7535\u5bfc\u7387\u662f\u63a7\u5236\u6d3b\u6027\u7684\u6700\u91cd\u8981\u56e0\u7d20\u4e4b\u4e00\u3002\u50ac\u5316\u5242\u6d3b\u6027\u4f4d\u70b9\u7684\u5206\u5b50\u6027\u8d28\u662f\u8fdb\u884c\u50ac\u5316\u5242\u4f18\u5316\u7684\u91cd\u8981\u4fdd\u969c\u3002<\/p>\n

\u540c\u65f6\uff0c\u4f5c\u8005\u5c55\u793a\u4e86\u5982\u4f55\u5229\u7528\u5438\u7535\u5b50\u548c\u4f9b\u7535\u5b50\u914d\u4f53\u53d6\u4ee3\u6765\u6539\u53d8\u5206\u5b50\u7684\u6c27\u5316\u8fd8\u539f\u6027\u80fd\uff0c\u5e76\u63d0\u9ad8\u5176\u50ac\u5316\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\u3002\u8fdb\u4e00\u6b65\u8c03\u6574\u8fd9\u4e9b\u56e0\u7d20\uff0c\u80fd\u591f\u5b9e\u73b0CO2<\/sub>\u7684\u7535\u5316\u5b66\u8fd8\u539f\u7532\u9187\u7684\u4f18\u5f02\u6027\u80fd\uff0c\u8fd9\u4e5f\u662f\u4f20\u7edf\u5206\u5b50\u50ac\u5316\u5242\u65e0\u6cd5\u5b9e\u73b0\u7684\u3002\u5176\u4e2d\uff0c\u516d\u7535\u5b50\u8fd8\u539f\u8fc7\u7a0b\u4ee5CO\u4e3a\u5173\u952e\u4e2d\u95f4\u4f53\uff0c\u5411\u6d3b\u6027\u4f4d\u70b9\u7684\u5feb\u901f\u8fde\u7eed\u7535\u5b50\u4f20\u9012\u6709\u5229\u4e8e\u5c06CO\u8fdb\u4e00\u6b65\u8fd8\u539f\u4e3a\u7532\u9187\u3002\u6b64\u5916\uff0c\u4f5c\u8005\u8fd8\u6307\u51fa\uff0c\u5728\u50ac\u5316\u5242\u5206\u5b50\u6eb6\u89e3\u5728\u7535\u89e3\u8d28\u6eb6\u6db2\u4e2d\u7684\u5747\u76f8\u7535\u50ac\u5316\u4e2d\uff0c\u5373\u4f7f\u5206\u5b50\u7ed3\u6784\u4fdd\u6301\u5b8c\u6574\uff0c\u5b9e\u9645\u7684\u50ac\u5316\u4f5c\u7528\u4e5f\u53ef\u80fd\u7531\u6c38\u4e45\u5438\u9644\u5728\u7535\u6781\u8868\u9762\u7684\u5206\u5b50\u4e3b\u5bfc\uff0c\u56e0\u6b64\u672c\u8d28\u4e0a\u662f\u975e\u5747\u76f8\u7684\u3002\u672c\u7814\u7a76\u4f5c\u8005\u5bf9\u91d1\u5c5e\u915e\u83c1\u5206\u5b50\u50ac\u5316CO2<\/sub>\u7535\u8fd8\u539f\u53cd\u5e94\u7684\u7814\u7a76\uff0c\u6765\u4ee5\u6b64\u8bf4\u660e\u5bf9\u5f02\u76f8\u5206\u5b50\u7535\u50ac\u5316\u7684\u7406\u89e3\uff0c\u8fd9\u4e5f\u9002\u7528\u4e8e\u5176\u4ed6\u7535\u5316\u5b66\u7cfb\u7edf\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cHeterogeneous Molecular Catalysts of Metal Phthalocyanines for Electrochemical CO<\/strong>2<\/sub><\/strong>\u00a0Reduction Reactions<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Acc. Chem. Res.<\/i><\/em><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe<\/b><\/strong>\u4e00<\/b><\/strong>\u3001\u4fc3\u8fdbCO<\/b><\/strong>2<\/b><\/sub><\/strong>\u5230CO\u7684\u8f6c\u5316<\/b><\/strong>\"\"<\/b><\/strong>\uff08a\uff09CoPc\/CNT\u548c\u88f8CoPc\u6676\u4f53\u7684\u7535\u5b50\u663e\u5fae\u955c\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09\u57280.1 M KHCO3<\/sub>\u4e2d\uff0c\u4e0d\u540c\u9634\u6781\u7535\u4f4d\u4e0bCoPc\/CNT\u548c\u88f8CoPc\u7684CO\u504f\u7535\u6d41\u5bc6\u5ea6\u7684\u5bf9\u6bd4\uff1b<\/p>\n

\uff08c\uff09\u57280.1 M KHCO3<\/sub>\u4e2d\uff0c\u4e0d\u540c\u9634\u6781\u7535\u4f4d\u4e0b\u88f8NiPc\u548cNiPc\/CNT\u5728GDE\u4e0a\u7684CO\u504f\u7535\u6d41\u5bc6\u5ea6\u7684\u5bf9\u6bd4\uff1b<\/p>\n

\u56fe<\/b><\/strong>\u4e8c\u3001\u5b9e\u73b0CO<\/b><\/strong>2<\/b><\/sub><\/strong>\u5230\u7532\u9187\u7684\u8f6c\u5316<\/b><\/strong>\"\"<\/b><\/strong>\uff08a\uff09CoPc\/CNT\u901a\u8fc7CO\u4f5c\u4e3a\u4e2d\u95f4\u4f53\u50ac\u5316\u7684CO2<\/sub>\u5230MeOH\u7684\u8f6c\u5316\uff1b<\/p>\n

\uff08b\uff09\u57280.1 M KHCO3<\/sub>\u4e2d\uff0c\u4e0d\u540c\u9634\u6781\u7535\u4f4d\u7531CoPc\/CNT\u50ac\u5316\u7684CO2<\/sub>\u8fd8\u539f\u7684\u4ea7\u7269\u9009\u62e9\u6027\u3002<\/p>\n

\u56fe<\/b><\/strong>\u4e09<\/b><\/strong>\u3001\u5747\u76f8<\/b><\/strong>\u8fd8\u662f\u5f02\u76f8<\/b><\/strong>\u7535\u50ac\u5316<\/b><\/strong>\uff1f<\/b><\/strong>\"\"\uff08a\uff09\u53ef\u6eb6\u6027CoPc\u5206\u5b50\u7684\u7ed3\u6784\uff1b<\/p>\n

\uff08b\uff09\u5bf9\u7167\u5b9e\u9a8c\u4ee5\u9a8c\u8bc1\u6240\u89c2\u5bdf\u5230\u7684\u53ef\u6eb6\u6027CoPc\u5206\u5b50\u50ac\u5316\u7684\u6027\u8d28\uff1b<\/p>\n

\uff08c\uff09\u5728\u7b2c\u4e00\u6b21\u548c\u7b2c\u4e8c\u6b21\u7535\u89e3\u8fc7\u7a0b\u4e2d\u5bf9CO2<\/sub>\u548cCO\u8fd8\u539f\u7684\u50ac\u5316\u6027\u80fd\u3002<\/p>\n

\u56fe<\/b><\/strong>\u56db<\/b><\/strong>\u3001\u5438\u7535\u5b50\u57fa\u56e2<\/b><\/strong>\"\"\uff08a\uff09\u5c06\u6c30\u57fa\u53d6\u4ee3\u57fa\u4f5c\u4e3a\u5438\u7535\u5b50\u57fa\u56e2\u6dfb\u52a0\u5230MPc\u5206\u5b50\uff1b<\/p>\n

\uff08b\uff09CoPc\/CNT\u548cCoPc-CN\/CNT\u5728CO2<\/sub>\u9971\u548c\u76840.1 M KHCO3<\/sub>\u4e2d\u7684\u5faa\u73af\u4f0f\u5b89\u56fe\uff1b<\/p>\n

\uff08c\uff09NiPc\/CNT\u548cNiPc-CN\/CNT\u5728Ar\u9971\u548c\u76840.1 M\u78f7\u9178\u76d0\u7f13\u51b2\u6db2\u4e2d\u7684\u5faa\u73af\u4f0f\u5b89\u56fe\uff1b<\/p>\n

\uff08d\uff09CoPc\/CNT\u548cCoPc-CN\/CNT\u5728H\u578b\u7535\u89e3\u6c60\u53cd\u5e94\u5668\u4e2d\uff0c\u4e0d\u540c\u9634\u6781\u7535\u4f4d\u4e0bCO2<\/sub>\u9971\u548c\u76840.1 M KHCO3<\/sub>\u6eb6\u6db2\u4e2d\u7684\u50ac\u5316\u6027\u80fd\u7684\u6bd4\u8f83\uff1b<\/p>\n

\uff08e\uff09\u57281.0 M KHCO3<\/sub>\u4e0d\u540c\u9634\u6781\u7535\u4f4d\u4e0b\uff0cGDE\u914d\u7f6e\u4e2dNiPc\/CNT\u548cNiPc-CN\/CNT \u7684CO\u504f\u7535\u6d41\u5bc6\u5ea6\u7684\u5bf9\u6bd4\u3002<\/p>\n

\u56fe<\/b><\/strong>\u4e94<\/b><\/strong>\u3001\u6c28\u57fa<\/b><\/strong>\u4f5c\u4e3a\u4f9b<\/b><\/strong>\u7535\u5b50\u57fa\u56e2<\/b><\/strong>\"\"<\/p>\n

\uff08a\uff09\u5c06\u6c28\u57fa\u53d6\u4ee3\u57fa\u4f5c\u4e3a\u4f9b\u7535\u5b50\u57fa\u56e2\u9644\u52a0\u5230CoPc\u5206\u5b50\u4e0a\uff1b<\/p>\n

\uff08b\uff09CO2<\/sub>\u9971\u548c\u76840.1 M KHCO3<\/sub>\u6eb6\u6db2\u4e2dCoPc\/CNT\u548cCoPc-NH2\/CNT\u7684\u5faa\u73af\u4f0f\u5b89\u56fe\uff1b<\/p>\n

\uff08c\uff09CoPc\/CNT\u4e0eCoPc-NH2<\/sub>\/CNT\u50ac\u5316\u7684\u957f\u5faa\u73afCO2<\/sub>\u4ea7\u7269\u7684\u5bf9\u6bd4\u3002<\/p>\n

\u56fe<\/b><\/strong>\u516d<\/b><\/strong>\u3001\u7532\u6c27\u57fa<\/b><\/strong>\u4f5c\u4e3a\u4f9b\u7535\u5b50\u57fa\u56e2<\/b><\/strong>\"\"\uff08a\uff09\u5c06\u7532\u6c27\u57fa\u53d6\u4ee3\u57fa\u4f5c\u4e3a\u7ed9\u7535\u5b50\u57fa\u56e2\u9644\u52a0\u5230NiPc\u5206\u5b50\u4e0a\uff1b<\/p>\n

\uff08b\uff09NiPc\/CNT\uff0cNiPc-CN\/CNT\u548cNiPc-OMe\/CNT\u4e4b\u95f4\u50ac\u5316\u8010\u4e45\u6027\u7684\u5bf9\u6bd4\uff1b<\/p>\n

\uff08c\uff09\u5728\u542b\u6216\u4e0d\u542bCO\u7684\u4e09\u79cdNiPc\u914d\u5408\u7269\u4e2d\uff0c\u901a\u8fc7DFT\u8ba1\u7b97\u7684Ni\u548cN\u4e4b\u95f4\u7684\u952e\u7ea7\uff1b<\/p>\n

\uff08d\uff09\u5728-150 mA cm-2<\/sup>\u603b\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0cNiPc-OMe\/CNT\u57281.0 M KHCO3<\/sub>\u4e2d\u7684\u957f\u5faa\u73afCO2<\/sub>\u7535\u89e3\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a\u201c<\/strong>Heterogeneous Molecular Catalysts of Metal Phthalocyanines for Electrochemical CO<\/u><\/strong>2<\/sub><\/u><\/strong>\u00a0Reduction Reactions<\/u><\/strong><\/a>\u201d(<\/strong>Acc. Chem. Res.<\/i><\/em><\/strong>\uff0c<\/b><\/strong>202<\/strong>1<\/strong>\uff0c10.1021\/acs.accounts.1c00200)<\/strong><\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4ebaCYM\u7f16\u8bd1\u4f9b\u7a3f\u3002\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

\u6750\u6599\u4eba\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaokefu \u3002<\/p>\n

\u3010<\/b><\/strong>\u56e2\u961f\u4ecb\u7ecd<\/b><\/strong>\u3011<\/b><\/strong><\/p>\n

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