{"id":226554,"date":"2021-08-31T06:25:12","date_gmt":"2021-08-30T22:25:12","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=226554"},"modified":"2021-08-30T21:25:32","modified_gmt":"2021-08-30T13:25:32","slug":"nature-reviews-materials%e4%bb%8e%e9%87%91%e5%b1%9e%e8%85%90%e8%9a%80%e7%a7%91%e5%ad%a6%e8%a7%92%e5%ba%a6%e8%a7%a3%e8%af%bb%e9%94%82%e9%87%91%e5%b1%9e%e8%b4%9f%e6%9e%81%e9%92%9d%e5%8c%96%e5%b1%82","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=226554","title":{"rendered":"Nature Reviews Materials:\u4ece\u91d1\u5c5e\u8150\u8680\u79d1\u5b66\u89d2\u5ea6\u89e3\u8bfb\u9502\u91d1\u5c5e\u8d1f\u6781\u949d\u5316\u5c42"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u9502\u79bb\u5b50\u7535\u6c60 (LIBs) \u56e0\u5176\u5177\u6709\u9ad8\u6bd4\u80fd\u91cf\uff08\u76ee\u524d~250 Wh kg-1<\/sup>\uff09\u548c\u529f\u7387\uff08\u76ee\u524d~500 W kg-1<\/sup>\uff09\uff0c\u5728\u4fbf\u643a\u5f0f\u7535\u5b50\u8bbe\u5907\u4e2d\u5f97\u5230\u4e86\u5e7f\u6cdb\u7684\u5e94\u7528\u3002\u7136\u800c\uff0c\u5546\u7528LIBs\u7684\u6027\u80fd\u6b63\u5728\u63a5\u8fd1\u5176\u7406\u8bba\u6781\u9650\uff0c\u800c\u5bf9\u9ad8\u6027\u80fd\uff0c\u4f4e\u6210\u672c\u50a8\u80fd\u6280\u672f\u7684\u9700\u6c42\u4e5f\u5728\u4e0d\u65ad\u589e\u957f\uff0c\u4ece\u800c\u91cd\u65b0\u6fc0\u53d1\u4e86\u5bf9\u9502\u79bb\u5b50\u9ad8\u80fd\u7535\u6c60\u7cfb\u7edf\u66ff\u4ee3\u7cfb\u7edf\u7684\u7814\u7a76\u3002\u7814\u7a76\u8868\u660e\uff0c\u5177\u6709\u66f4\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7684\u9502\u91d1\u5c5e\u7535\u6c60\uff08LMBs\uff09\u6709\u671b\u66ff\u4ee3LIBs\u3002\u5176\u4e2d\uff0c\u5728\u9502\u91d1\u5c5e\u8868\u9762\u4e0e\u7535\u89e3\u6db2\u63a5\u89e6\u65f6\u81ea\u53d1\u5f62\u6210\u7684\u949d\u5316\u819c\u7684\u7ec4\u6210\u548c\u7ed3\u6784\uff0c\u5bf9\u4e8e\u9502\u91d1\u5c5e\u53ef\u9006\u6c89\u79ef\/\u5265\u79bb\u548c\u5747\u5300\u6027\u8d77\u7740\u81f3\u5173\u91cd\u8981\u7684\u4f5c\u7528\u3002\u5c3d\u7ba1\u9502\u5728\u6db2\u6001\u7535\u89e3\u8d28\u4e2d\u5177\u6709\u6781\u5f3a\u7684\u53cd\u5e94\u6027\uff0c\u4f46\u7531\u4e8e\u8868\u9762\u819c\u7684\u5feb\u901f\u751f\u957f\uff0c\u5b83\u4ecd\u4fdd\u6301\u76f8\u5bf9\u7a33\u5b9a\u3002\u7406\u60f3\u7684\u949d\u5316\u819c\u5fc5\u987b\u6ee1\u8db3\u4ee5\u4e0b\u5148\u51b3\u6761\u4ef6\uff1a\uff081\uff09<\/strong>\u4fdd\u62a4\u9502\u91d1\u5c5e\u8868\u9762\u4e0d\u4e0e\u7535\u89e3\u6db2\u63a5\u89e6\uff1b\uff082\uff09<\/strong>\u5141\u8bb8\u5feb\u901f\u7684\u9502\u79bb\u5b50\uff08Li+<\/sup>\uff09\u7a7f\u8fc7\u8584\u819c\uff1b\uff083\uff09<\/strong>\u6291\u5236Li+<\/sup>\u4e0e\u7535\u89e3\u8d28\u4e4b\u95f4\u7684\u7535\u5b50\u8f6c\u79fb\uff1b\uff084\uff09<\/strong>\u9632\u6b62\u9502\u679d\u6676\u7684\u6210\u6838\u548c\u751f\u957f\uff1b\uff085\uff09<\/strong>\u9002\u5e94\u9502\u6c89\u79ef\/\u5265\u79bb\u8fc7\u7a0b\u4e2d\u9502\u8868\u9762\u5f62\u8c8c\u7684\u53d8\u5316\u3002\u521b\u9020\u8fd9\u6837\u4e00\u79cd\u7406\u60f3\u5316\u7684\u949d\u5316\u819c\uff0c\u9700\u8981\u6df1\u5165\u4e86\u89e3\u949d\u5316\u819c\u7684\u6210\u5206\uff0c\u7ed3\u6784\uff0c\u5f62\u8c8c\u548c\u62d3\u6251\u7ed3\u6784\u3002<\/p>\n

\u8fd1\u65e5\uff0c\u7f8e\u56fd\u52b3\u4f26\u65af\u4f2f\u514b\u5229\u56fd\u5bb6\u5b9e\u9a8c\u5ba4Robert Kostecki\u6559\u6388\uff0c\u5fb7\u56fd\u4e4c\u5c14\u59c6\u4ea5\u59c6\u970d\u5179\u7814\u7a76\u6240Stefano\u00a0Passerini\u6559\u6388\u548cArnulf\u00a0Latz\u6559\u6388<\/strong>\uff08<\/strong>\u5171\u540c<\/strong>\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u57fa\u4e8e\u91d1\u5c5e\u8150\u8680\u548c\u949d\u5316\u73b0\u8c61\u7684\u4e00\u822c\u6027\u6982\u5ff5\uff0c\u4ece\u4e0d\u540c\u7684\u89d2\u5ea6\u6df1\u5165\u7406\u89e3\u9502\u7535\u6781-\u6db2\u6001\u7535\u89e3\u8d28\u754c\u9762\u4e0a\u53d1\u751f\u7684\u53cd\u5e94\uff0c\u5e76\u91cd\u65b0\u603b\u7ed3\u548c\u5f52\u7eb3\u4e86\u57fa\u672c\u7684\u7535\u5316\u5b66\u7406\u8bba\u548c\u6a21\u578b<\/strong>\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u8fc4\u4eca\u4e3a\u6b62\u9502\u91d1\u5c5e\u8d1f\u6781\u5c1a\u672a\u4ece\u8150\u8680\u79d1\u5b66\u7684\u89d2\u5ea6\u8fdb\u884c\u5f7b\u5e95\u7814\u7a76\u3002\u901a\u8fc7\u8ba8\u8bbaLi+<\/sup>\u5728\u77ac\u65f6\u5f62\u6210\u7684\u949d\u5316\u5c42\uff08\u56fa\u4f53\u7535\u89e3\u8d28\u754c\u9762-SEI\uff09\u4e0a\u7684\u8f6c\u79fb\uff0c\u5728\u8150\u8680\u79d1\u5b66\u548c\u7535\u6c60\u7535\u5316\u5b66\u4e4b\u95f4\u67b6\u8d77\u4e86\u4e00\u5ea7\u6865\u6881\u3002\u5c06\u8fd9\u4e9b\u8003\u8651\u4e0e\u4ee5\u6750\u6599\u79d1\u5b66\u4e3a\u5bfc\u5411\u7684\u65b9\u6cd5\u76f8\u7ed3\u5408\uff0c\u901a\u8fc7\u539f\u4f4d\u548c\u975e\u539f\u4f4d\u5b9e\u73b0\u7cbe\u5fc3\u8bbe\u8ba1\u7684\u949d\u5316\u5c42\u6216\u4eba\u5de5\u4fdd\u62a4\u5c42\uff0c\u4ece\u800c\u8fbe\u5230\u6291\u5236\u7535\u89e3\u8d28\u8fde\u7eed\u5206\u89e3\u548c\u9502\u6d88\u8017\u3002\u6700\u540e\uff0c\u4f5c\u8005\u63d0\u51fa\u4e86\u7406\u60f3\u949d\u5316\u5c42\u7684\u8bbe\u8ba1\u6784\u60f3\uff0c\u5e76\u786e\u5b9a\u4e86\u53ef\u80fd\u5bfc\u81f4\u9502\u91d1\u5c5e\u7535\u6c60\u5728\u5546\u4e1a\u5316\u8fdb\u7a0b\u4e2d\u6240\u9047\u5230\u7684\u6311\u6218\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cThe passivity of lithium electrodes in liquid electrolytes for secondary batteries<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nature Reviews Materials<\/i><\/em><\/strong><\/a>\u4e0a\u3002\u4f55\u6b23\u548cDominic Bresser\u4e3a\u672c\u6587\u7b2c\u5171\u540c\u4e00\u4f5c\u8005\uff0c\u4f55\u6b23\u73b0\u5c31\u804c\u4e8e\u56db\u5ddd\u5927\u5b66\u5316\u5b66\u5de5\u7a0b\u5b66\u9662\uff0c\u4efb\u7279\u8058\u7814\u7a76\u5458\u3002\"\"<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe<\/b><\/strong>\u4e00<\/b><\/strong>\u3001\u91d1\u5c5e\u7535\u6781\u7684\u80fd\u91cf\u5bc6\u5ea6\u53ca\u76f8\u5e94\u7684\u8150\u8680\u53cd\u5e94<\/b><\/strong>\"\"<\/b><\/strong>\uff08a\uff09\u5404\u79cd\u7535\u6c60\u6280\u672f\u7684\u6bd4\u80fd\u91cf\u5bc6\u5ea6\u548c\u7535\u52bf\u56fe\uff1b<\/p>\n

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\u56fe<\/b><\/strong>\u4e8c\u3001\u9502\u91d1\u5c5e\u7535\u6781\u7684\u8150\u8680\u53cd\u5e94<\/b><\/strong>\"\"<\/b><\/strong>\u56fe<\/b><\/strong>\u4e09<\/b><\/strong>\u3001\u975e\u6c34<\/b><\/strong>\u7cfb<\/b><\/strong>\u7535\u89e3\u8d28\u4e2d\u7684\u9502\u8150\u8680<\/b><\/strong>\"\"\u56fe<\/b><\/strong>\u56db<\/b><\/strong>\u3001\u9502\u91d1\u5c5e-\u6db2<\/b><\/strong>\u6001<\/b><\/strong>\u7535\u89e3\u8d28\u754c\u9762\u548c<\/b><\/strong>\u754c\u9762<\/b><\/strong>\u76f8\u7684\u53c2\u6570<\/b><\/strong>\"\"<\/p>\n

\uff08a\uff09\u9502\u91d1\u5c5e\u7684\u751f\u4ea7\uff0c\u9502\u7b94\u7684\u5236\u5907\u548c\u968f\u540e\u5728\u53ef\u63a7\u6c14\u4f53\u6c14\u6c1b\u4e0b\u7684\u949d\u5316\uff1b<\/p>\n

\uff08b\uff09\u901a\u5e38\u7528\u4f5c\u7535\u89e3\u8d28\u7684\u6709\u673a\u6eb6\u5242\u5305\u62ecDME\uff0cDOL\uff0cEC\uff0cDEC\uff0cPC\uff0c\u7528\u4e8e\u6784\u5efa\u539f\u4f4dSEI\u4fdd\u62a4\u5c42\uff1b<\/p>\n

\uff08c\uff09\u57fa\u4e8e\u65e0\u673a\u7ec4\u5206\uff08\u91d1\u5c5e\u6c2f\u5316\u7269\uff09\uff0c\u805a\u5408\u7269\uff08\u805a\u4e19\u70ef\u9178\uff09\u6216\u6df7\u5408\u4f53\u7cfb\uff08Cu3<\/sub>N\u7eb3\u7c73\u9897\u7c92\u4e0e\u82ef\u4e59\u70ef-\u4e01\u4e8c\u70ef\u6a61\u80f6\uff09\u7684\u4eba\u5de5\u4fdd\u62a4\u5c42\u3002<\/p>\n

\u56fe<\/b><\/strong>\u4e94<\/b><\/strong>\u3001<\/b><\/strong>\u539f\u4f4d<\/b><\/strong>\u548c<\/b><\/strong>\u975e\u539f\u4f4d\u4fdd\u62a4\u5c42<\/b><\/strong>\"\"<\/p>\n

\uff08a\uff0cb\uff09\u5728\u4f20\u7edf\u7535\u89e3\u6db2\u4e2d\u5f62\u6210\u82d4\u85d3\u72b6\u679d\u6676\u72b6\uff0c\u6539\u6027\u540e\u6c89\u79ef\u5f62\u8c8c\u5f97\u5230\u6539\u5584\uff0c\u5f62\u6210\u7684\u949d\u5316\u5c42\u66f4\u52a0\u5747\u5300\uff1b<\/p>\n

\uff08c\uff09\u57fa\u4e8epoly(vinylsulfonyl fluoride-ran-2-vinyl-1,3-dioxolane)\u548c\u6c27\u5316\u77f3\u58a8\u70ef\u7eb3\u7c73\u7247\u7684\u6df7\u5408\u805a\u5408\u7269-\u65e0\u673a\u4eba\u5de5\u4fdd\u62a4\u5c42\uff1b<\/p>\n

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\uff08e\uff09\u78b3\u5316\u6728\u6750\u4f5c\u4e3a\u8bf1\u5bfc\u9502\u5747\u5300\u6c89\u79ef\u7684\u9aa8\u67b6\u3002<\/p>\n

\u56fe<\/b><\/strong>\u516d<\/b><\/strong>\u3001\u5f71\u54cd\u754c\u9762<\/b><\/strong>\u76f8<\/b><\/strong>\u6f14\u5316\u7684\u56e0\u7d20<\/b><\/strong>\"\"<\/p>\n

\uff08a\uff09Li+<\/sup>\u4f9d\u6b21\u901a\u8fc7\u7535\u89e3\u8d28\u3001\u56fa\u4f53\u754c\u9762\u76f8\u548c\u9502\u91d1\u5c5e\u8d1f\u6781\uff08Lislab<\/sub>\uff09\uff0c\u5176\u4e2d\u0394Edes<\/sub>\u662fLi+<\/sup>\u53bb\u6eb6\u5242\u7684\u80fd\u5792\uff1b\u0394Ediff<\/sub>\u662fLi+<\/sup>\u4ece\u56fa\u4f53\u7535\u89e3\u8d28\u754c\u9762\u76f8\u8f6c\u79fb\u5230\u9502\u91d1\u5c5e\u8d1f\u6781\u7684\u80fd\u5792\uff1b<\/p>\n

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\u56fe<\/b><\/strong>\u4e03<\/b><\/strong>\u3001\u9502\u91d1\u5c5e\u7535\u6c60\u5546\u4e1a<\/b><\/strong>\u5316<\/b><\/strong>\u7684\u76f8\u5173\u53c2\u6570<\/b><\/strong>\"\"\uff08a\uff09\u9502\u91d1\u5c5e\u7535\u6c60\u4f9d\u636e\u4e0d\u540c\u9502\u542b\u91cf\u800c\u4e0d\u540c\u7684\u6210\u672c\u4f30\u8ba1\uff1b<\/p>\n

\uff08b\uff09\u7535\u6c60\u6c34\u5e73\u4e0a\u7684\u521d\u59cb\u80fd\u91cf\u5bc6\u5ea6\uff1b<\/p>\n

\uff08c\uff09\u4ece\u7ec4\u88c5\u5230\u7535\u6c60\u5931\u6548\uff0c\u7d2f\u8ba1\u8150\u8680\u7684\u9502\u91d1\u5c5e\u542b\u91cf\u7684\u767e\u5206\u6bd4\uff1b<\/p>\n

\uff08d\uff09\u4e0d\u540c\u7684\u5faa\u73af\u5708\u6570\u4e0b\uff0c\u9502\u91d1\u5c5e\u7535\u6c60\u80fd\u91cf\u5bc6\u5ea6\u7684\u6f14\u5316\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a\u201c<\/strong>The passivity of lithium electrodes in liquid electrolytes for secondary batteries<\/u><\/strong><\/a>\u201d(<\/strong>Nature Reviews Materials<\/i><\/em><\/strong><\/a>\uff0c<\/b><\/strong>202<\/strong>1<\/strong>\uff0c<\/strong>10.1038\/s41578-021-00345-5<\/strong>)<\/strong><\/p>\n

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