{"id":227449,"date":"2021-09-18T12:00:38","date_gmt":"2021-09-18T04:00:38","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=227449"},"modified":"2021-09-20T15:23:29","modified_gmt":"2021-09-20T07:23:29","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e8%92%99%e7%ba%b3%e5%a3%ab%e5%a4%a7%e5%ad%a6nat-commun-%ef%bc%9a%e5%8f%af%e7%94%a8%e4%ba%8e%e6%9c%89%e6%95%88%e8%b0%83%e8%8a%82li-s%e7%94%b5%e6%b1%a0","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=227449","title":{"rendered":"\u8499\u7eb3\u58eb\u5927\u5b66Nat. Commun.\uff1a\u53ef\u7528\u4e8e\u6709\u6548\u8c03\u8282Li-S\u7535\u6c60\u4e2d\u591a\u786b\u5316\u7269\u7684\u7cd6\u57fa\u7c98\u5408\u5242"},"content":{"rendered":"

\u3010\u7814\u7a76\u80cc\u666f\u3011<\/strong><\/p>\n

\u9502\u79bb\u5b50\u7535\u6c60\u7684\u51fa\u73b0\u5f15\u8d77\u4e86\u65b0\u80fd\u6e90\u9886\u57df\u7684\u5de8\u5927\u53d8\u9769\u3002\u4f46\u968f\u7740\u793e\u4f1a\u5927\u89c4\u6a21\u8fdc\u79bb\u5316\u77f3\u71c3\u6599\uff0c\u5177\u6709\u66f4\u9ad8\u5b58\u50a8\u5bb9\u91cf\u548c\u66f4\u4f4e\u5173\u952e\u77ff\u7269\u9700\u6c42\u7684\u65b0\u578b\u7535\u6c60\u662f\u53d1\u5c55\u7684\u65b9\u5411\u3002\u4e0e\u6b64\u540c\u65f6\uff0c\u8bb8\u591a\u65b0\u5174\u6280\u672f\u7684\u53ef\u884c\u6027\uff0c\u4f8b\u5982\u822a\u7a7a\u6280\u672f\uff0c\u9700\u8981\u66f4\u8f7b\u7684\u7535\u6c60\u3002Li-S\u7535\u6c60\u5b8c\u5168\u6ee1\u8db3\u8fd9\u4e9b\u9700\u6c42\uff0c\u7406\u8bba\u4e0a\u5b83\u53ef\u4ee5\u5b58\u50a8\u591a\u8fbe\u9502\u79bb\u5b50\u80fd\u91cf\u7684\u4e94\u500d\uff0c\u5e76\u4e14\u5177\u6709400-600 Wh kg-1<\/sup>\u7684\u53ef\u5b9e\u73b0\u6bd4\u80fd\u91cf\u3002\u4f46\u662f\u5b83\u4f5c\u4e3a\u4e00\u79cd\u50a8\u80fd\u6280\u672f\u7684\u53ef\u884c\u6027\u53d6\u51b3\u4e8e\u5176\u957f\u671f\u5faa\u73af\u7a33\u5b9a\u6027\uff0c\u800c\u5927\u591a\u6570\u4e0d\u7a33\u5b9a\u6027\u6e90\u4e8e\u591a\u786b\u5316\u7269\u4ece\u9634\u6781\u7684\u91ca\u653e\u548c\u8fd0\u8f93\uff0c\u5bfc\u81f4\u9502\u8d1f\u6781\u4e0a\u957f\u6ee1\u679d\u6676\uff0c\u5bfc\u81f4\u7535\u89e3\u8d28\u7684\u6301\u7eed\u6d88\u8017\u3002\u56e0\u6b64\uff0c\u5f00\u53d1\u5177\u6709\u6700\u5c0f\u591a\u786b\u5316\u7269\u9003\u9038\u7684\u8010\u7528\u9634\u6781\u81f3\u5173\u91cd\u8981\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u6fb3\u5927\u5229\u4e9a\u8499\u7eb3\u58eb\u5927\u5b66<\/strong>Mainak Majumder<\/strong>\u6559\u6388\u3001<\/strong>Matthew R. Hill<\/strong>\u6559\u6388\u548c<\/strong>Mahdokht Shaibani<\/strong>\u6559\u6388<\/strong>\u5171\u540c\u63d0\u51fa\u4e86\u4e00\u79cd\u57fa\u4e8e\u7cd6\u7684\u7c98\u5408\u5242\u7cfb\u7edf\uff0c\u7531\u4e8e\u5176\u8fd8\u539f\u7279\u6027\uff0c\u8be5\u7cfb\u7edf\u5177\u6709\u8c03\u8282\u591a\u786b\u5316\u7269\u7684\u80fd\u529b\u3002\u6b64\u5916\uff0c\u7c98\u5408\u5242\u5728\u94f8\u9020\u8fc7\u7a0b\u4e2d\u4fc3\u8fdb\u7c98\u5f39\u6027\u7ea4\u7ef4\u7684\u5f62\u6210\uff0c\u4ece\u800c\u8d4b\u4e88\u786b\u9634\u6781\u7406\u60f3\u7684\u7f51\u72b6\u5fae\u89c2\u7ed3\u6784\u3002\u7efc\u5408\u5b9e\u9a8c\u8868\u660e\uff0c\u786b\u5229\u7528\u7387\u9ad8\u8fbe97%\uff0c\u5faa\u73af\u5bff\u547d\u4e3a1000\u6b21\u5faa\u73af\uff089\u4e2a\u6708\uff09\uff0c\u6700\u540e\u7684\u5bb9\u91cf\u4fdd\u6301\u7387\u4e3a700 mAh g-1<\/sup>\u3002\u636e\u6b64\u4f5c\u8005\u8fd8\u751f\u4ea7\u51fa\u6bd4\u80fd\u91cf\u9ad8\u8fbe206 Wh kg-1<\/sup>\u7684\u8f6f\u5305\u7535\u6c60\u539f\u578b\uff0c\u5c55\u793a\u4e86\u5b9e\u9645\u5e94\u7528\u7684\u6f5c\u529b\u3002\u8be5\u6587\u7ae0\u8fd1\u65e5\u4ee5\u9898\u4e3a\u201cA saccharide-based binder for efficient polysulfide regulations in Li-S batteries<\/strong>\u201d\u53d1\u8868\u5728\u77e5\u540d\u9876\u520aNature Communications<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001<\/strong>LiPS<\/strong>\u5438\u9644\u6a21\u62df<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09Li2<\/sub>S4<\/sub>\u3001Li2<\/sub>S6<\/sub>\u548cLi2<\/sub>S8<\/sub>\u5728\u8461\u8404\u7cd6\u4e0a\u7684\u5438\u9644\u6784\u8c61\u548c\u7ed3\u5408\u80fd\u3002<\/p>\n

\uff08b\uff09\u6bd4\u8f83\u8461\u8404\u7cd6\u548c\u5e38\u7528PVDF\u7c98\u5408\u5242\u4e0e\u5404\u79cdLiPS\u7269\u8d28\u7684\u7ed3\u5408\u80fd\uff0c\u8bc1\u660e\u8461\u8404\u7cd6\u5438\u9644\u591a\u786b\u5316\u7269\u7684\u80fd\u529b\u3002<\/p>\n

\u56fe\u4e8c\u3001\u591a\u786b\u5316\u7269\u7684\u5438\u9644\u7814\u7a76<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u591a\u786b\u5316\u7269\u4e0e\u8461\u8404\u7cd6\u5728DOL\/DME\u7535\u89e3\u8d28\u6eb6\u6db2\u4e2d\u7684\u65f6\u95f4\u53d8\u5316\u3002<\/p>\n

\uff08b\uff09\u7279\u5b9a\u65f6\u95f4\u540e\uff0c\u5728DOL\/DME\u7535\u89e3\u8d28\u6eb6\u6db2\u4e2dLi2<\/sub>S6<\/sub>\u4e0e\u8461\u8404\u7cd6\u7684\u7d2b\u5916-\u53ef\u89c1\u5149\u8c31\u3002<\/p>\n

\uff08c\uff09CMC\u548c\u8461\u8404\u7cd6\u5bf9LiPS\u5438\u9644\u7684\u6bd4\u8f83\u3002<\/p>\n

\uff08d-e\uff09\u5728\u9ad8\u6d53\u5ea6\u591a\u786b\u5316\u9502\u5b58\u5728\u4e0b\u591a\u786b\u5316\u7269\u7684\u6f14\u53d8\u56fe\u793a\u3002<\/p>\n

\uff08f\uff09\u60ac\u6d6e\u6db2\u7684\u62c9\u66fc\u5149\u8c31\u3002<\/p>\n

\uff08g\uff09\u6d17\u6da4\u540e\u56fa\u4f53\u6b8b\u7559\u7269\u7684FTIR\u5149\u8c31\u3002<\/p>\n

\u56fe\u4e09\u3001\u6838\u78c1\u6c22\u8c31\u5206\u6790\u6a21\u62df\u7535\u6c60\u73af\u5883\u4e2d\u8461\u8404\u7cd6\u4e0e<\/strong>Li2<\/sub>S6<\/sub><\/strong>\u7684\u76f8\u4e92\u4f5c\u7528<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u8461\u8404\u7cd6\/Li2<\/sub>S6<\/sub>\u590d\u5408\u7269\u76841<\/sup>H NMR\u5168\u8c31\u3002<\/p>\n

\uff08b\uff098\u5929\u5185H1\u03b1<\/sub>\u548cH1\u03b1<\/sub>\u030d\u6bd4\u4f8b\u7684\u53d8\u5316\u3002<\/p>\n

\uff08c\uff098\u5929\u51851<\/sup>H NMR\u8c31\u56fe\u7684\u53d8\u5316\u3002<\/p>\n

\u56fe\u56db\u3001\u4e0d\u540c\u7c98\u7ed3\u5242\u4f53\u7cfb\u786b\u7535\u6781\u7684\u5fae\u89c2\u7ed3\u6784\u7814\u7a76\u3001\u5143\u7d20\u56fe\u548c\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a-c\uff09\u5c06\u7eafCMC\u7528\u4f5c\u7c98\u5408\u5242\uff0c\u8868\u660e\u51dd\u805a\u9897\u7c92\u7684\u5185\u805a\u7f51\u7edc\u88ab\u56f0\u5728\u7c98\u5408\u5242\u7f51\u7edc\u4e2d\u3002<\/p>\n

\uff08d-f\uff09CMC\/G\u4f5c\u4e3a\u7c98\u5408\u5242\uff0c\u8bf4\u660e\u4e86\u4e00\u79cd\u5206\u79bb\u7ed3\u6784\uff0c\u8be5\u7ed3\u6784\u5206\u79bb\u7531\u7f51\u72b6\u7c98\u5408\u5242\u8fde\u63a5\u7684\u9897\u7c92\u3002<\/p>\n

\uff08g-i\uff09\u7eafCMC\u4f5c\u4e3a\u7c98\u5408\u5242\uff0c\u5728\u9897\u7c92\u8868\u9762\u5f62\u6210\u8fde\u7eed\u7684\u7c98\u5408\u5242\u819c\u3002<\/p>\n

\uff08j-l\uff09CMC\/G\u4f5c\u4e3a\u7c98\u5408\u5242\uff0c\u8bf4\u660e\u7535\u6781\u4e0a\u5b58\u5728\u6865\u63a5\u952e\uff0c\u4e14\u786b\u66b4\u9732\u826f\u597d\u3002<\/p>\n

\u56fe\u4e94\u3001\u7269\u7406\u3001\u6d41\u53d8\u548c\u7ea4\u7ef4\u7a00\u91ca\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u7c89\u672b\u6df7\u5408\u7269\u7684\u5bc6\u5ea6\uff0c\u5305\u62ec\u786b\u3001\u78b3\u548c\u7c98\u5408\u5242\uff0c\u4ee5\u53ca\u56db\u79cd\u4e0d\u540c\u60c5\u51b5\u4e0b\u6700\u7ec8\u7535\u6781\u7684\u5b54\u9699\u7387\u3002<\/p>\n

\uff08b\uff09\u4ee5CMC\/G\u548c\u7eafCMC\u4e3a\u7c98\u5408\u5242\u7684\u9634\u6781\u62c9\u4f38\u8bd5\u9a8c\u548c\u538b\u75d5\u8bd5\u9a8c\u3002<\/p>\n

\uff08c\uff09\u7a33\u6001\u526a\u5207\u6d41\u53d8\u884c\u4e3a\u3002<\/p>\n

\uff08d\uff09\u56db\u4e2a\u6837\u54c1\u4e4b\u95f4\u5265\u79bb\u8bd5\u9a8c\u7684\u529b-\u4f4d\u79fb\u56fe\u3002<\/p>\n

\uff08e-f\uff09\u5265\u79bb\u8bd5\u9a8c\u88c5\u7f6e\u7684\u7167\u7247\u3002<\/p>\n

\uff08i-l\uff09\u76f8\u5e94\u6837\u54c1\u7684\u7c98\u7ed3\u5242\u5fae\u89c2\u7ed3\u6784\u3002<\/p>\n

\u56fe\u516d\u3001<\/strong>CMC<\/strong>\u6b63\u6781\u548c<\/strong>CMC\/G<\/strong>\u6b63\u6781\u5faa\u73af\u6027\u80fd\u6bd4\u8f83<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a-b\uff09\u914d\u7f6e\u67093 mg\/cm2<\/sup>\u786b\u8d1f\u8f7d\u6b63\u6781\u30016.5 mg\/cm2<\/sup>\u786b\u8d1f\u8f7d\u6b63\u6781\u548c10.5 mg\/cm2<\/sup>\u786b\u8d1f\u8f7d\u6b63\u6781\u7684\u7ebd\u6263\u7535\u6c60\uff0c\u5982\u63d2\u5165\u56fe\u4e2d\u6240\u793a\u3002<\/p>\n

\uff08c\uff09\u4e24\u4e2a\u7ebd\u6263\u7535\u6c60\u4e4b\u95f4\u7684\u500d\u7387\u80fd\u529b\u6570\u636e\u6bd4\u8f83\uff082 mg\/cm2<\/sup>\u786b\u8d1f\u8f7d\uff09\u3002<\/p>\n

\uff08d-e\uff09\u5355\u9762\u6b63\u6781\u7684\u8f6f\u5305\u7535\u6c60\u914d\u7f6e\u548c\u8d2b\u7535\u89e3\u8d28\u6761\u4ef6\u4e0b\u7684\u53cc\u9762\u9634\u6781\uff08E\/S = 6 \u03bcL mg-1<\/sup>\uff09\uff0c\u4f18\u5316\u6bd4\u80fd\u91cf\u3002<\/p>\n

\u56fe\u4e03\u3001\u5177\u6709\u4e24\u79cd\u4e0d\u540c\u7c98\u5408\u5242\u4f53\u7cfb\u7684\u786b\u6b63\u6781\u7684\u7535\u5316\u5b66\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09CV\u66f2\u7ebf\u5bf9\u6bd4\u3002<\/p>\n

\uff08b-c\uff09\u91c7\u7528CMC\/G\u6b63\u6781\u548cCMC\u6b63\u6781\u7684Li-S\u7535\u6c60\u5728\u4e0d\u540c\u626b\u63cf\u901f\u7387\u4e0b\u7684CV\u66f2\u7ebf\u3002<\/p>\n

\uff08d\uff09\u91c7\u7528CMC\/G\u6b63\u6781\uff08A1\u3001B1\u3001C1\uff09\u548cCMC\u6b63\u6781\uff08A2\u3001B2\u3001C2\uff09\u7684Li-S\u7535\u6c60\u7684CV\u5cf0\u503c\u7535\u6d41\u7684\u7ebf\u6027\u62df\u5408\uff08R2<\/sup>=0.99\uff09\u3002<\/p>\n

\uff08e-f\uff09\u91c7\u7528CMC\/G\u6b63\u6781\u548cCMC\u6b63\u6781\u7684Li-S\u7535\u6c60\u7684\u5145\u7535\/\u653e\u7535\u66f2\u7ebf\u3002<\/p>\n

\uff08g\uff09\u572880\u6b21\u5faa\u73af\u524d\u540e\uff0c\u4f7f\u7528CMC\/G\u548cCMC\u6b63\u6781\u7684Li-S\u7535\u6c60\u7684\u7535\u5316\u5b66\u963b\u6297\u8c31\u5948\u594e\u65af\u7279\u56fe\u3002<\/p>\n

\uff08h\uff09\u5faa\u73af\u540e\u7535\u6c60\u7684\u5948\u594e\u65af\u7279\u56fe\u548c\u7b49\u6548\u7535\u8def\u62df\u5408\u3002<\/p>\n

\u56fe\u516b\u3001\u5267\u70c8\u5faa\u73af\u540e\u9502\u91d1\u5c5e\u8d1f\u6781\u548c\u786b\u6b63\u6781\u7684\u539f\u4f4d\u9a8c\u6536<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a-b\uff09\u9502\u91d1\u5c5e\u4e0eCMC\u6b63\u6781\u548cCMC\/G\u6b63\u6781\u5076\u8054\u7684\u4fef\u89c6SEM\u56fe\u50cf\u3002<\/p>\n

\uff08c-h\uff09CMC\u6b63\u6781\u548cCMC\/G\u6b63\u6781\u5728\u5b8c\u5168\u5145\u7535\u72b6\u6001\u4e0b\u7684\u6a2a\u622a\u9762\u89c2\u5bdf\u548c\u5143\u7d20\u5206\u5e03\u56fe\u3002<\/p>\n

\u3010\u5168\u6587\u603b\u7ed3\u3011<\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aA saccharide-based binder for efficient polysulfide regulations in Li-S batteries<\/a> (Nat. Commun.<\/em> 2021<\/strong>, 12<\/em>, 5375)<\/p>\n

\u672c\u6587\u7531\u5927\u5175\u54e5\u4f9b\u7a3f\u3002<\/p>\n

\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n

\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

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 <\/p>\n","protected":false},"excerpt":{"rendered":"

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