{"id":228544,"date":"2021-10-22T06:30:46","date_gmt":"2021-10-21T22:30:46","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=228544"},"modified":"2021-10-21T18:43:50","modified_gmt":"2021-10-21T10:43:50","slug":"%ef%bc%88%e5%b7%b2%e6%a0%a1%e7%a8%bf%e4%bb%b6%ef%bc%89%e4%b8%9c%e4%ba%ac%e5%a4%a7%e5%ad%a6riken-nature-materials%ef%bc%9a%e6%97%a0%e6%ba%b6%e5%89%82%e8%87%aa%e5%82%ac%e5%8c%96%e8%b6%85%e5%88%86","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=228544","title":{"rendered":"\u4e1c\u4eac\u5927\u5b66&RIKEN Nature Materials\uff1a\u65e0\u6eb6\u5242\u81ea\u50ac\u5316\u8d85\u5206\u5b50\u805a\u5408"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u8d85\u5206\u5b50\u805a\u5408\u7269\u662f\u4e0b\u4e00\u4ee3\u6750\u6599\u7684\u6709\u5e0c\u671b\u7684\u5019\u9009\u8005\uff0c\u56e0\u4e3a\u5176\u56fa\u6709\u7684\u52a8\u6001\u6027\u8d28\u800c\u6709\u6781\u597d\u7684\u53ef\u56de\u6536\u6027\u548c\u518d\u5229\u7528\u529f\u80fd\u3002\u7136\u800c\uff0c\u4ece\u5b9e\u9645\u5e94\u7528\u4e0a\u770b\uff0c\u65e0\u6eb6\u5242\u6761\u4ef6\u4e0b\u7684\u8d85\u5206\u5b50\u805a\u5408\u7b56\u7565\u66f4\u4e3a\u6709\u5229\uff0c\u56e0\u4e3a\u5176\u751f\u6210\u7684\u8d85\u7ed3\u6784\u53ef\u4ee5\u76f4\u63a5\u4f7f\u7528\uff0c\u800c\u4e0d\u4f1a\u5931\u53bb\u5176\u7ed3\u6784\u5b8c\u6574\u6027\u3002\u9700\u6ce8\u610f\u7684\u662f\uff0c\u5728\u8d85\u5206\u5b50\u805a\u5408\u7814\u7a76\u7684\u65e9\u671f\uff0c\u975e\u5171\u4ef7\u805a\u5408\u7269\u7ed3\u6784\u662f\u7531\u7ed3\u6676\u548c\u6db2\u6676\u7ec4\u88c5\u4f53\u4e2d\u7684\u6c22\u952e\uff08H\u952e\uff09\u5206\u5b50\u5f62\u6210\u7684\u3002\u4f46\u662f\uff0c\u5206\u5b50\u7ec4\u88c5\u5728\u65e0\u6eb6\u5242\u6761\u4ef6\u4e0b\u5f88\u96be\u63a7\u5236\u3002\u5982\u679c\u4e00\u4e2a\u5316\u5b66\u53cd\u5e94\u7684\u4ea7\u7269\u80fd\u50ac\u5316\u5176\u81ea\u8eab\u7684\u5f62\u6210\uff0c\u5219\u8be5\u53cd\u5e94\u88ab\u79f0\u4e3a\u81ea\u50ac\u5316\u53cd\u5e94\u3002\u5728\u7406\u60f3\u60c5\u51b5\u4e0b\uff0c\u81ea\u50ac\u5316\u5316\u5b66\u53cd\u5e94\u5e94\u663e\u793a\u4ea7\u54c1\u6d53\u5ea6\u53d8\u5316\u7684S-\u578b\u65f6\u7a0b\u66f2\u7ebf\u3002\u81ea\u50ac\u5316\u4e0e\u751f\u547d\u7684\u51fa\u73b0\u6709\u5173\uff0c\u5e76\u4e14\u662f\u8bb8\u591a\u751f\u7269\u8fc7\u7a0b\u7684\u56fa\u6709\u8fc7\u7a0b\uff0c\u4f8b\u5982\u751f\u7269\u5206\u5b50\u7684\u81ea\u6211\u590d\u5236\u3002\u5982\u4f55\u5b9e\u73b0\u65e0\u6291\u5236\u7684\u6709\u673a\u81ea\u50ac\u5316\uff1f\u81ea\u50ac\u5316\u901a\u5e38\u9700\u8981\u9ad8\u7a00\u91ca\u5ea6\uff0c\u4ee5\u907f\u514d\u7ec4\u88c5\u4f5c\u4e3a\u6a21\u677f\u7684\u4ea7\u54c1\uff0c\u56e0\u800c\u5176\u5728\u5927\u89c4\u6a21\u5316\u5b66\u54c1\u5236\u9020\u4e2d\u7684\u5b9e\u9645\u5e94\u7528\u9762\u4e34\u5de8\u5927\u7684\u969c\u788d\u3002
\n \"\"
\n \u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u65e5\u672c\u4e1c\u4eac\u5927\u5b66Takuzo Aida\u548c\u65e5\u672c\u7406\u5316\u5b66\u7814\u7a76\u6240\uff08RIKEN\uff09Daigo Miyajima\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u65e0\u6eb6\u5242\u81ea\u50ac\u5316\u8d85\u5206\u5b50\u805a\u5408\uff08SF-ASP\uff09\uff0c\u5176\u63d0\u4f9b\u4e86\u4e00\u79cd\u65e0\u6291\u5236\u7684\u6a21\u677f\u53bb\u8f85\u52a9\u50ac\u5316\u6709\u673a\u8f6c\u5316\uff0c\u5145\u5206\u5229\u7528\u4e86\u4ea7\u7269\uff08\u6a21\u677f\uff09\u5728\u65e0\u6eb6\u5242\u6761\u4ef6\u4e0b\u7ecf\u5386\u65e0\u7ec8\u6b62\u6210\u6838-\u5ef6\u4f38\u7ec4\u88c5\uff08\u6d3b\u6027\u8d85\u5206\u5b50\u805a\u5408\uff09\u7684\u8fc7\u7a0b\u3002SF-ASP\u5b9e\u73b0\u4e86\u6c22\u952e\u90bb\u82ef\u4e8c\u7532\u8148\u4ee5\u6781\u9ad8\u7684\u4ea7\u7387\uff08>80%\uff09\u8fd8\u539f\u6210\u76f8\u5e94\u7684\u915e\u83c1\u3002\u6b64\u5916\uff0cSF-ASP\u4f1a\u4f7f\u751f\u957f\u4e2d\u7684\u805a\u5408\u7269\u5f62\u6210\u516d\u8fb9\u5f62\u5806\u79ef\u7684\u7ed3\u6676\u7ea4\u7ef4\uff0c\u53ef\u80fd\u5728\u5176\u6a2a\u622a\u9762\u8fb9\u7f18\u9884\u7ec4\u7ec7\u90bb\u82ef\u4e8c\u7532\u8148\u4ee5\u5b9e\u73b0\u6709\u6548\u8f6c\u5316\u3002\u4f5c\u8005\u4f7f\u7528\u91d1\u5c5e\u6cb9\u9178\u916f\uff0cSF-ASP\u518d\u6b21\u4ee5\u6781\u9ad8\u7684\u4ea7\u7387\u751f\u4ea7\u91d1\u5c5e\u915e\u83c1\u7684\u5355\u6676\u7ea4\u7ef4\uff0c\u8fd9\u4e9b\u7ea4\u7ef4\u5728\u6ca1\u6709\u672b\u7aef\u8026\u5408\u4e0b\u5b9e\u73b0\u53cc\u5411\u751f\u957f\uff0c\u76f4\u5230\u90bb\u82ef\u4e8c\u7532\u8148\u524d\u4f53\u5b8c\u5168\u6d88\u8017\u3002\u901a\u8fc7\u5229\u7528\u805a\u5408\u7684\u8fd9\u79cd\u6d3b\u6027\u6027\u8d28\uff0c\u5229\u7528\u4e0d\u542b\/\u542b\u91d1\u5c5e\u6cb9\u9178\u916f\u7684\u591a\u6b65SF-ASP\u53ef\u4ee5\u7cbe\u786e\u5408\u6210\u591a\u5d4c\u6bb5\u8d85\u5206\u5b50\u5171\u805a\u7269\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cSolvent-free autocatalytic supramolecular polymerization\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNature Materials<\/strong>\u4e0a\u3002\u672c\u6587\u7b2c\u4e00\u4f5c\u8005\u4e3a\u6e05\u534e\u5927\u5b66\u6df1\u5733\u56fd\u9645\u7814\u7a76\u9662\u9648\u632f\u52a9\u7406\u6559\u6388<\/strong>\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u65e0\u6eb6\u5242\u8d85\u5206\u5b50\u805a\u5408\u9a71\u52a8\u7684\u81ea\u50ac\u5316<\/strong>
\n \"\"\uff08a\uff09SF-ASP\u6982\u5ff5\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u4f7f\u7528PNC4<\/sub>\u901a\u8fc7SF-ASP\u83b7\u5f97\u7684\u915e\u83c1\uff08H<\/sup><\/em>PCCn<\/sub>\uff09\u884d\u751f\u7269\u53ca\u5176\u4e0eZn\u3001Fe\u3001Co\u548cCu\u7684\u91d1\u5c5e\u7edc\u5408\u7269\uff08M<\/sup><\/em>PCC4<\/sub>\uff09\u7684\u5316\u5b66\u7ed3\u6784\uff1b<\/p>\n

\uff08c\uff09\u4f5c\u4e3aSF-ASP\u5355\u4f53\u524d\u4f53\u7684\u6247\u5f62\u4e8c\u786b\u4ee3\u70f7\u57fa\u90bb\u82ef\u4e8c\u7532\u8148\uff08PNCn<\/sub>\uff09\u884d\u751f\u7269\u7684\u5316\u5b66\u7ed3\u6784\u3002<\/p>\n

\u56fe\u4e8c\u3001SF-ASP\u7684\u8868\u5f81<\/strong>
\n \"\"
\n \uff08a\uff09PNC3<\/sub>\u3001PNC4<\/sub>\u3001PNC5<\/sub>\u3001PNC6<\/sub>\u548cPNC4<\/sub>N-Me<\/sup>\u52a0\u70ed\u65f6\u5939\u5728\u73bb\u7483\u677f\u4e4b\u95f4\uff0c\u5176\u4e2dSF-ASP \u663e\u793a\u51fasigmoidal\u65f6\u7a0b\u7279\u5f81\uff1b
\n \uff08b\uff09H<\/sup><\/em>PCC4<\/sub>\u548cPNC4<\/sub>\u4ee5\u53caSF-ASP\u4f7f\u7528PNC4<\/sub>\u5728\u4e0d\u540c\u6e29\u5ea6\u4e0b\u52a0\u70ed24 h\u5f62\u6210\u7684\u526f\u4ea7\u7269\u7684\u91cd\u91cf\u5206\u6570\uff1b
\n \uff08c\uff09SF-ASP\u4f7f\u7528PNC4<\/sub>\u5728160 \u00b0C\u52a0\u70ed\u65f6\u83b7\u5f97\u7684\u53cd\u5e94\u6df7\u5408\u7269\u7684\u5149\u5b66\u56fe\u50cf\uff1b
\n \uff08d\uff09\u4f7f\u7528PNC3<\/sub>\u3001PNC4<\/sub>\u3001PNC5<\/sub>\u3001PNC6<\/sub>\u548cPNC4<\/sub>N-Me<\/sup>\u52a0\u70ed24 h\u540e\u901a\u8fc7SF-ASP\u83b7\u5f97\u7684\u53cd\u5e94\u6df7\u5408\u7269\u7684MALDI-TOF\u8d28\u8c31\u56fe\uff1b
\n \uff08e\uff09\u4f7f\u7528PNC3<\/sub>\u3001PNC5<\/sub>\u3001PNC6<\/sub>\u548cPNC4<\/sub>N-Me<\/sup>\u52a0\u70ed24 h\u540e\u7684SF-ASP\u53cd\u5e94\u6df7\u5408\u7269\u7684\u5149\u5b66\u56fe\u50cf\u3002<\/p>\n

\u56fe\u4e09\u3001SF-ASP\u83b7\u5f97\u7684[H<\/em><\/sup>PCC4<\/sub>]CF<\/sup>\u7684\u8868\u5f81<\/strong>
\n \"\"\uff08a\uff09\u572825 \u00b0C\u4e0b\u7528\u7532\u9187\u6d17\u6da4\u540e\uff0cSF-ASP\u5f62\u6210\u7684[H<\/sup><\/em>PCC4<\/sub>]CF<\/sup>\u7684POM\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff09\u572825 \u00b0C\u4e0b\u7528\u7532\u9187\u6d17\u6da4\u540e\uff0cSF-ASP\u5f62\u6210\u7684[H<\/sup><\/em>PCC4<\/sub>]CF<\/sup>\u7684PXRD\u56fe\u6848\u53ca\u5176\u5177\u6709\u4e8c\u7ef4\u516d\u8fb9\u5f62\u51e0\u4f55\u5f62\u72b6\u7684\u67f1\u72b6\u6392\u5217\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08c\uff09\u572825 \u00b0C\u4e0b\u7528\u7532\u9187\u6d17\u6da4\u540e\uff0c\u901a\u8fc7SF-ASP\u83b7\u5f97\u7684[H<\/sup><\/em>PCC4<\/sub>]CF<\/sup>\u5355\u7ea4\u7ef4\u7684\u900f\u89c6\u4e8c\u7ef4SAXS\u56fe\u6848\uff1b<\/p>\n

\uff08d\uff09\u572825 \u00b0C\u4e0b\u7528\u7532\u9187\u6d17\u6da4\u540e\uff0c\u901a\u8fc7SF-ASP\u83b7\u5f97\u7684[H<\/em><\/sup>PCC4<\/sub>]CF<\/sup>\u5355\u7ea4\u7ef4\u7684SAED\u56fe\u6848\uff1b<\/p>\n

\uff08e\uff09[H<\/sup><\/em>PCC4<\/sub>]CF<\/sup>\u53ef\u80fd\u7ed3\u6784\u7684\u7ebf\u6846\u8868\u793a\uff0c\u5176\u4e2d\u7701\u7565\u4e86\u6c22\u539f\u5b50\u548c\u4fa7\u94fe\uff1b<\/p>\n

\uff08f\uff09\u572825 \u00b0C\u4e0b\u7528\u7532\u9187\u6d17\u6da4\u540e\uff0c\u901a\u8fc7SF-ASP\u83b7\u5f97\u7684[H<\/sup><\/em>PCC4<\/sub>]CF<\/sup>\u5355\u7ea4\u7ef4\u57280\u00b0\u81f390\u00b0\u7684\u4e0d\u540c\u65b9\u4f4d\u89d2\uff08\u03b8\uff09\u4e0b\u7684\u504f\u632fFT-IR\u5149\u8c31\u3002<\/p>\n

\u56fe\u56db\u3001SF-ASP\u83b7\u5f97\u7684\u7ed3\u6676\u7ea4\u7ef4\u7684\u5e8f\u5217\u548c\u53d6\u5411\u63a7\u5236<\/strong>
\n \"\"\uff08a\uff09\u4f7f\u7528PNC4<\/sub>\u4e0eZn(oleate)2<\/sub>\u3001Fe(oleate)3<\/sub>\u3001Co(oleate)2<\/sub>\u548cCu(oleate)2<\/sub>\u5939\u5728\u73bb\u7483\u677f\u4e4b\u95f4\u7684\u53cd\u5e94\u6df7\u5408\u7269\uff0c\u5728160 \u00b0C\u52a0\u70ed\u540e\uff0c\u901a\u8fc7SF-ASP\u83b7\u5f97\u7684700 nm\u5904\u7684\u65f6\u95f4\u4f9d\u8d56\u6027\u5438\u6536\u5149\u8c31\u53d8\u5316\uff1b<\/p>\n

\uff08b\uff09\u4f7f\u7528PNC4<\/sub>\u4e0eZn(oleate)2<\/sub>\u3001Fe(oleate)3<\/sub>\u3001Co(oleate)2<\/sub>\u548cCu(oleate)2<\/sub>\u5728160 \u00b0C\u4e0b\u52a0\u70ed12 h\u5f97\u5230\u7684SF-ASP\u53cd\u5e94\u6df7\u5408\u7269\u7684\u5149\u5b66\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09\u4f7f\u7528PNC4<\/sub>\u52a0\/\u4e0d\u52a0Zn(oleate)2<\/sub>\u3001Fe(oleate)3<\/sub>\u3001Co(oleate)2<\/sub>\u548cCu(oleate)2<\/sub>\u5939\u5728\u88abCYTOP\u8584\u819c\u8986\u76d6\u7684\u73bb\u7483\u677f\u4e4b\u95f4\uff0c\u5728180 \u00b0C\u4e0b\u52a0\u70ed2-4 h\u540e\uff0c\u901a\u8fc7\u591a\u6b65SF-ASP\u83b7\u5f97\u7684\u53cd\u5e94\u6df7\u5408\u7269\u7684\u5149\u5b66\u56fe\u50cf\uff1b<\/p>\n

\uff08d-e\uff09\u5728PNC4<\/sub>\u548cPNC3<\/sub>\u70ed\u7194\u4f53\u4e2d180 \u00b0C\u4e0b\u4fdd\u63014 h\u540e\uff0c\u901a\u8fc7SF-ASP\u83b7\u5f97\u7684[H<\/sup><\/em>PCC3<\/sub>]CF<\/sup>\u548c[H<\/em><\/sup>PCC4<\/sub>]CF<\/sup>\u6676\u79cd\u7684\u53d8\u5316\uff1b<\/p>\n

\uff08f\uff09\u4f7f\u7528PNC4\u548c1-\u5341\u4e8c\u70f7\u786b\u9187\uff08DCTH\uff09\u901a\u8fc7SF-ASP\u83b7\u5f97\u7684\u53cd\u5e94\u6df7\u5408\u7269\u7684\u5149\u5b66\u56fe\u50cf\uff1b<\/p>\n

\uff08g\uff09\u572810 T\u78c1\u573a\u4e2d\uff0c\u4f7f\u7528PNC4<\/sub>\u4e0eFe(oleate)3<\/sub>\u548cCo(oleate)2<\/sub>\u6216\u4e0d\u542b\u91d1\u5c5e\u6cb9\u9178\u76d0\u5728160 \u2103\u52a0\u70ed6 h\u540e\uff0c\u901a\u8fc7SF-ASP\u83b7\u5f97\u7684\u53cd\u5e94\u6df7\u5408\u7269\u7684\u5149\u5b66\u56fe\u50cf\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u901a\u8fc7\u5bf9\u5076\u7136\u53d1\u73b0\u7684\u8be6\u7ec6\u7814\u7a76\uff0c\u66f4\u65b0\u4e86\u89c2\u5ff5\uff0c\u5373\u7eff\u8272\u7684\u8584\u7ea4\u7ef4\u5728\u70ed\u53f0\u4e0a\u52a0\u70ed\u6db2\u6676PN\u65f6\u5f62\u6210\u5e76\u62c9\u957f\u3002\u672c\u6587\u5f00\u53d1\u7684SF-ASP\u63d0\u4f9b\u4e86\u4e00\u79cd\u65e0\u6291\u5236\u6a21\u677f\u8f85\u52a9\u7684\u50ac\u5316\u6709\u673a\u8f6c\u5316\u7b56\u7565\uff0c\u5145\u5206\u5730\u5229\u7528\u4e86\u5176\u4ea7\u54c1\uff08\u6a21\u677f\uff09\u5728\u65e0\u6eb6\u5242\u6761\u4ef6\u4e0b\u7684\u65e0\u7ec8\u6b62\u6210\u6838-\u5ef6\u4f38\u7ec4\u88c5\uff08\u6d3b\u6027\u8d85\u5206\u5b50\u805a\u5408\uff09\u3002\u8003\u8651\u5230\u5176\u5bf9\u5176\u4ed6\u03c0-\u7535\u5b50\u548c\u5927\u73af\u5355\u4f53\u5408\u6210\u7684\u6f5c\u5728\u9002\u7528\u6027\uff0cSF-ASP\u53ef\u4ee5\u5728\u65e0\u6eb6\u5242\u6761\u4ef6\u4e0b\u4f7f\u7528\u539f\u4f4d\u751f\u4ea7\u7684\u5355\u4f53\u8fdb\u884c\u7cbe\u786e\u7684\u5927\u5206\u5b50\u5de5\u7a0b\uff0c\u53ef\u80fd\u662f\u53ef\u6301\u7eed\u672a\u6765\u805a\u5408\u7269\u5236\u9020\u7684\u7406\u60f3\u5f62\u5f0f\u4e4b\u4e00\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aSolvent-free autocatalytic supramolecular polymerization<\/a><\/strong>. Nature Materials<\/em>, 2021<\/strong>, DOI: 10.1038\/s41563-021-01122-z.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1\uff1atougao@cailiaoren.com.<\/p>\n

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