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ACS Catalysis\uff1a\u90bb\u8fd1\u91d1\u5c5e\u8fc1\u79fb\u5bf9\u53cc\u529f\u80fd\u590d\u5408\u6750\u6599\u50ac\u5316\u5408\u6210\u6c14\u5236\u70ef\u70c3\u7684\u5f71\u54cd\uff08\u901a\u8baf\u4f5c\u8005\uff1a\u5305\u4fe1\u548c\uff09[2]<\/b><\/strong><\/p>\n

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\"\"<\/p>\n

Catalysis Science & Technology\uff1a\u7532\u82ef\u5b58\u5728\u4e0bCO<\/b><\/strong>2<\/b><\/sub><\/strong>\/H<\/b><\/strong>2<\/b><\/sub><\/strong>\u9009\u62e9\u6027\u5408\u6210\u5bf9\u4e8c\u7532\u82ef\u548c\u8f7b\u70ef\u70c3\uff08\u901a\u8baf\u4f5c\u8005\uff1a\u6f58\u79c0\u83b2\uff0c\u5305\u4fe1\u548c\uff09[3]<\/b><\/strong><\/p>\n

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\"\"<\/p>\n

Nature Communications\uff1a\u7535\u5b50\u7a7f\u900f\u89e6\u53d1Pt-\u77f3\u58a8\u70ef\u7684\u754c\u9762\u6d3b\u6027\u7528\u4e8e\u5ba4\u6e29CO\u6c27\u5316<\/b><\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff1a\u9093\u5fb7\u4f1a\uff09[4]<\/b><\/strong><\/p>\n

\"\"<\/p>\n

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\u5728\u8fd9\u91cc\uff0c\u5f00\u53d1\u4e86\u4e00\u79cd\u72ec\u7279\u7684\u6765\u81eaCoNi\u7eb3\u7c73\u9897\u7c92\u7684\u77f3\u58a8\u70ef\u5b64\u7acb\u7684Pt\u7eb3\u7c73\u9897\u7c92\uff08Pt\u01c0CoNi\uff09\uff0c\u7528\u4e8e\u5728\u5bcc\u6c27\u6c14\u6c1b\u4e2d\u9ad8\u6548\u50ac\u5316CO\u6c27\u5316\u3002\u954d\u5408\u91d1\u88ab\u8d85\u8584\u77f3\u58a8\u70ef\u5916\u58f3\u4fdd\u62a4\u800c\u4e0d\u88ab\u6c27\u5316\uff0c\u4ece\u800c\u901a\u8fc7\u7535\u5b50\u7a7f\u900f\u6548\u5e94\u8c03\u8282pt -\u77f3\u58a8\u70ef\u754c\u9762\u7684\u7535\u5b50\u6027\u80fd\u3002\u8be5\u50ac\u5316\u5242\u5728\u5ba4\u6e29\u4e0b\u53ef\u4ee5\u8fbe\u5230\u63a5\u8fd1100%\u7684CO\u8f6c\u5316\u7387\uff0c\u800cPt\/C\u548cPt\/CoNiOx\u50ac\u5316\u5242\u7684\u8f6c\u5316\u7387\u6709\u9650\u3002\u5b9e\u9a8c\u548c\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0cCO\u4f1a\u4f7fPt\u4f4d\u9971\u548c\uff0c\u800cO2<\/sub>\u53ef\u4ee5\u5438\u9644\u5728Pt-\u77f3\u58a8\u70ef\u754c\u9762\u800c\u4e0d\u4e0eCO\u7ade\u4e89\uff0c\u8fd9\u6709\u5229\u4e8eO2<\/sub>\u7684\u6d3b\u5316\u548c\u968f\u540e\u7684\u8868\u9762\u53cd\u5e94\u3002\u8fd9\u79cd\u77f3\u58a8\u70ef\u5206\u79bb\u4f53\u7cfb\u4e0d\u540c\u4e8e\u4f20\u7edf\u7684\u91d1\u5c5e-\u91d1\u5c5e\u6c27\u5316\u7269\u50ac\u5316\u754c\u9762\uff0c\u4e3a\u591a\u76f8\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u63d0\u4f9b\u4e86\u65b0\u7684\u601d\u8def\u3002<\/p>\n

\u8d75\u4e1c\u5143<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u7269\u7406\u5316\u5b66\u5bb6\uff0c\u4e3b\u8981\u4ece\u4e8b\u6cb8\u77f3\u5206\u5b50\u7b5b\u3001\u7eb3\u7c73\u4ecb\u5b54\u6750\u6599\u5408\u6210\u3001\u7ed3\u6784\u548c\u5728\u50ac\u5316\u3001\u7535\u6c60\u3001\u6c34\u5904\u7406\u7b49\u80fd\u6e90\u65b9\u5411\u5e94\u7528\u9886\u57df\u7814\u7a76\u30022007\u5e74\u5f53\u9009\u4e3a\u4e2d\u56fd\u79d1\u5b66\u9662\u9662\u58eb\u3002<\/p>\n

\u8d75\u4e1c\u5143\u5f15\u9886\u56e2\u961f\u5b8c\u6210\u7684\u9879\u76ee\u201c\u6709\u5e8f\u4ecb\u5b54\u9ad8\u5206\u5b50\u548c\u78b3\u6750\u6599\u7684\u521b\u5236\u548c\u5e94\u7528\u201d\uff0c\u5728\u56fd\u9645\u4e0a\u7387\u5148\u63d0\u51fa\u4e86\u6709\u673a-\u6709\u673a\u81ea\u7ec4\u88c5\u65b0\u601d\u60f3\uff0c\u521b\u5236\u4e86\u5168\u65b0\u6709\u5e8f\u4ecb\u5b54\u9ad8\u5206\u5b50\u548c\u78b3\u6750\u6599,\u9996\u6b21\u5c06\u4ecb\u5b54\u6750\u6599\u4ece\u65e0\u673a\u7ec4\u6210\u6269\u5c55\u5230\u6709\u673a\u9ad8\u5206\u5b50\u548c\u78b3,\u4e3a\u72ec\u7279\u7684\u65b0\u4e00\u4ee3\u836f\u7269\u5408\u6210\u50ac\u5316\u5242\u3001\u4eff\u751f\u79bb\u5b50\u901a\u9053\u3001\u67d4\u6027\u5fae\u6d41\u63a7\u5668\u4ef6\u7b49\u7684\u6784\u7b51\u5960\u5b9a\u4e86\u57fa\u7840\uff0c\u521b\u9020\u4e86\u5de8\u5927\u7684\u7ecf\u6d4e\u6548\u76ca\u3002\u7814\u7a76\u6210\u679c\u88ab\u56fd\u9645\u540c\u884c\u8ba4\u4e3a\u662f\u201c\u9996\u6b21\u201d\u53d1\u73b0\u3001\u4ecb\u5b54\u6750\u6599\u9886\u57df\u201c\u91cc\u7a0b\u7891\u5f0f\u201d\u548c\u201c\u5148\u9a71\u201d\u7684\u8fdb\u5c55\u3002[5]<\/p>\n

Journal of the American Chemical Society\uff1a\u7528\u4e8e\u9ad8\u4f53\u79ef\u5bc6\u5ea6\u8d5d\u7535\u5bb9\u7684\u7cbe\u786e\u8bbe\u8ba1\u7684\u4ecb<\/b><\/strong>\u5b54<\/b><\/strong>\u4e8c\u6c27\u5316\u949b<\/b><\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff1a\u9b4f\u6e6b\u9f99\uff0c\u8d75\u4e1c\u5143\uff09[6]<\/b><\/strong><\/p>\n

\u7531\u4e8e\u5176\u5e94\u7528\u9886\u57df\u4ece\u4fbf\u643a\u5f0f\u7535\u5b50\u8bbe\u5907\u5230\u7535\u52a8\u6c7d\u8f66\uff0c\u7535\u5316\u5b66\u50a8\u80fd\u5177\u6709\u5e7f\u9614\u7684\u524d\u666f\u548c\u91cd\u5927\u610f\u4e49\u3002\u968f\u7740\u5bf9\u66f4\u5feb\u901f\u50a8\u80fd\u7684\u6280\u672f\u9700\u6c42\u4e0d\u65ad\u589e\u957f\uff0c\u80fd\u591f\u5728\u51e0\u79d2\u949f\u5185\u5145\u7535\u5e76\u63d0\u4f9b\u6bd4\u4f20\u7edf\u7535\u6c60\u66f4\u591a\u529f\u7387\u7684\u7535\u5bb9\u6750\u6599\u5728\u4e00\u7cfb\u5217\u5e94\u7528\uff08\u4f8b\u5982\u7535\u7f51\u4e2d\u7684\u80fd\u91cf\u6536\u96c6\u548c\u529f\u7387\u7f13\u51b2\uff09\u4e2d\u5177\u6709\u5438\u5f15\u529b\u3002\u5bf9\u4e8e\u8d5d\u7535\u5bb9\uff0c\u5b83\u53ef\u4ee5\u901a\u8fc7\u7eb3\u7c73\u7ed3\u6784\u5316\u7535\u5316\u5b66\u6d3b\u6027\u6750\u6599\u6765\u5b9e\u73b0\uff0c\u4ee5\u6700\u5927\u5316\u8fd1\u8868\u9762\u53ef\u9006\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u7684\u8868\u9762\u901a\u8def\u3002\u7136\u800c\uff0c\u7eb3\u7c73\u5c3a\u5bf8\u7684\u6d3b\u6027\u6750\u6599\u4ecd\u7136\u5b58\u5728\u6839\u672c\u6027\u7684\u6311\u6218\u3002\u7531\u4e8e\u7eb3\u7c73\u6750\u6599\u7684\u632f\u5b9e\u5bc6\u5ea6\u4f4e\uff0c\u7535\u5bb9\u6750\u6599\u7684\u4e00\u4e2a\u5173\u952e\u9650\u5236\u662f\u5b83\u4eec\u7684\u4f53\u79ef\u5bb9\u91cf\u4f4e\u3002<\/p>\n

\u5728\u8fd9\u91cc\uff0c\u63d0\u51fa\u4e86\u4e00\u79cd\u5177\u6709\u7cbe\u786e\u63a7\u5236\u7684\u4ecb\u5b54\u6846\u67b6\u7684\u6709\u524d\u9014\u7684\u4e2d\u5c3a\u5ea6 TiO2<\/sub>\u7ed3\u6784\u4f5c\u4e3a\u9ad8\u5bc6\u5ea6\u8d5d\u7535\u5bb9\u6a21\u578b\u7cfb\u7edf\u3002\u5fae\u7c73\u5c3a\u5bf8\u7684\u81f4\u5bc6\u4ecb\u5b54TiO2<\/sub>\u63d0\u4f9b\u4e86\u9ad8\u53ef\u53ca\u8868\u9762\u79ef(124 m2<\/sup>g\u20131<\/sup>\u00a0)\u548c\u5f84\u5411\u6392\u5217\u7684\u4ecb\u5b54\u901a\u9053\uff0c\u4f46\u632f\u5b9e\u5bc6\u5ea6\u9ad8(1.7 g cm\u20133<\/sup>)\u8fdc\u9ad8\u4e8eTiO2<\/sub>\u7eb3\u7c73\u9897\u7c92(0.47g cm\u20133<\/sup>\u00a0)\u3002\u4f5c\u4e3a\u8d5d\u7535\u5bb9\u94a0\u79bb\u5b50\u5b58\u50a8\u9633\u6781\uff0c\u7cbe\u786e\u8bbe\u8ba1\u7684\u4ecb\u5b54TiO2<\/sub>\u6a21\u578b\u57280.025 A g\u20131<\/sup>\u65f6\u5b9e\u73b0\u4e86\u6700\u5927\u7684\u91cd\u91cf\u5bb9\u91cf\uff08240 mAh g\u20131<\/sup>\uff09\u548c\u4f53\u79ef\u5bb9\u91cf\uff08350 mAh cm\u20133<\/sup>\uff09\u3002\u8fd9\u79cd\u8bbe\u8ba1\u7684\u8d5d\u7535\u5bb9\u4ecb\u5b54\u7ed3\u6784\u57289.47 mg cm\u20132<\/sup>\u7684\u9ad8\u8d28\u91cf\u8d1f\u8f7d\u4e0b\u8fdb\u4e00\u6b65\u5b9e\u73b0\u4e86\u5546\u4e1a\u4e0a\u53ef\u6bd4\u7684\u9762\u79ef\u5bb9\u91cf(2.1 mAh cm\u20132 <\/sup>)\u3002\u8fd9\u79cd\u80fd\u591f\u5728\u81f4\u5bc6\u7eb3\u7c73\u7ed3\u6784\u4e2d\u5b9e\u73b0\u5feb\u901f\u94a0\u5316\u7684\u4ecb\u5b54\u7ed3\u6784\u7535\u6781\u5bf9\u9ad8\u529f\u7387\u5e94\u7528\u3001\u5feb\u901f\u5145\u7535\u8bbe\u5907\u548c\u8d5d\u7535\u5bb9\u7535\u6781\u8bbe\u8ba1\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002<\/p>\n

\"\"<\/p>\n

Nano Letters\uff1a\u57fa\u4e8e\u754c\u9762\u52a8\u6001\u8fc1\u79fb\u7b56\u7565\u7684\u5177\u6709\u53ef\u8c03\u8c10\u66f2\u7387\u7684\u6d41\u7ebf\u578b\u4ecb\u5b54\u7845\u7eb3\u7c73\u9897\u7c92\uff08\u901a\u8baf\u4f5c\u8005\uff1a\u674e\u6653\u6c11\uff0c\u8d75\u4e1c\u5143\uff09[7]<\/b><\/strong><\/p>\n

\u5f15\u4eba\u5165\u80dc\u7684\u81ea\u7136\u7269\u79cd\u5e7f\u6cdb\u6fc0\u53d1\u4e86\u8bbe\u8ba1\u5404\u79cd\u529f\u80fd\u6750\u6599\u7684\u7075\u611f\uff0c\u8fd9\u4e9b\u529f\u80fd\u6750\u6599\u5177\u6709\u72ec\u7279\u7684\u51e0\u4f55\u6784\u578b\uff0c\u9002\u7528\u4e8e\u591a\u79cd\u6280\u672f\uff0c\u5c24\u5176\u662f\u6d41\u7ebf\u578b\u7684\u5916\u5f62\u589e\u5f3a\u4e86\u8fd0\u52a8\u6027\u3002\u540c\u6837\uff0c\u5177\u6709\u4f4e\u6d41\u4f53\u963b\u529b\u7cfb\u6570\u7684\u7eb3\u7c73\u6d41\u7ebf\u578b\u7ed3\u6784\u7684\u6784\u5efa\u53ef\u80fd\u4f1a\u5728\u836f\u7269\u8f93\u9001\u3001\u4e34\u5e8a\u8bca\u65ad\u548c\u7eb3\u7c73\u9a6c\u8fbe\u65b9\u9762\u5f00\u8f9f\u5de8\u5927\u7684\u5e94\u7528\u524d\u666f\u3002\u4e0d\u5e78\u7684\u662f\uff0c\u5c3d\u7ba1\u5728\u7eb3\u7c73\u9a6c\u8fbe\u7684\u7ed3\u6784\u526a\u88c1\u65b9\u9762\u5df2\u7ecf\u505a\u51fa\u4e86\u76f8\u5f53\u5927\u7684\u52aa\u529b\uff0c\u5236\u9020\u5177\u6709\u7cbe\u786e\u53ef\u63a7\u6d41\u7ebf\u51e0\u4f55\u5f62\u72b6\u7684\u7eb3\u7c73\u7c92\u5b50\u4ecd\u7136\u662f\u4e00\u4e2a\u5de8\u5927\u7684\u6311\u6218\u3002<\/p>\n

\u5728\u6b64\uff0c\u62a5\u9053\u4e86\u4e00\u79cd\u7b80\u5355\u7684\u754c\u9762\u52a8\u6001\u8fc1\u79fb\u7b56\u7565\uff0c\u4ee5\u5408\u6210\u5177\u6709\u4e0d\u540c\u7ed3\u6784\u7684\u6d41\u7ebf\u578b\u4ecb\u5b54\u7eb3\u7c73\u874c\u86aa\u3002\u8fd9\u4e9b\u874c\u86aa\u72b6\u7684\u7eb3\u7c73\u9897\u7c92\u5177\u6709\u5927\u7684\u6d41\u7ebf\u578b\u5934\u90e8\u548c\u7ec6\u957f\u7684\u5c3e\u5df4\uff0c\u5177\u6709\u5927\u7684\u5185\u8154(75-170 nm)\uff0c\u9ad8\u7684\u8868\u9762\u79ef(424-488m2<\/sup>g–<\/sup>1<\/sup>)\u548c\u5747\u5300\u7684\u4e2d\u5b54\u5c3a\u5bf8(2.4-3.2 nm)\u3002\u6d41\u7ebf\u578b\u4ecb\u5b54\u7eb3\u7c73\u9897\u7c92\u7684\u5934\u90e8\u66f2\u7387\u53ef\u57282.96\u00d710–<\/sup>2<\/sup>\u00a0~ 5.56\u00d710–<\/sup>2<\/sup>\u00a0nm–<\/sup>1<\/sup>\u8303\u56f4\u5185\u8c03\u8282\uff0c\u5c3e\u957f\u53ef\u572830 ~ 650 nm\u8303\u56f4\u5185\u8c03\u8282\u3002\u901a\u8fc7\u5c06Fe3<\/sub>O4<\/sub>\u50ac\u5316\u5242\u9009\u62e9\u6027\u8d1f\u8f7d\u5728\u6d41\u7ebf\u578b\u4e8c\u6c27\u5316\u7845\u7eb3\u7c73\u6781\u7684\u7a7a\u8154\u4e2d\uff0c\u8bbe\u8ba1\u4e86H2<\/sub>O2<\/sub>\u9a71\u52a8\u7684\u4ecb\u5b54\u7eb3\u7c73\u9a6c\u8fbe\u3002\u5177\u6709\u4f18\u5316\u7ed3\u6784\u53c2\u6570\u7684\u4ecb\u5b54\u7eb3\u7c73\u9a6c\u8fbe\u8868\u73b0\u51fa\u51fa\u8272\u7684\u65b9\u5411\u6027\u548c8.15 \u03bcm2<\/sup>s\u20131<\/sup>\u7684\u6269\u6563\u7cfb\u6570\u3002\u5177\u6709\u53ef\u8c03\u7ed3\u6784\u53c2\u6570\u7684\u6d41\u7ebf\u578b\u4e2d\u7a7a\u4ecb\u5b54\u7eb3\u7c73\u7c92\u5b50\u4e3a\u64cd\u7eb5\u7eb3\u7c73\u9a6c\u8fbe\u7684\u8fd0\u52a8\u884c\u4e3a\u8bbe\u7f6e\u4e86\u5e73\u53f0\uff0c\u4f7f\u6d41\u7ebf\u578b\u4ecb\u5b54\u7eb3\u7c73\u9a6c\u8fbe\u6210\u4e3a\u672a\u6765\u5728\u6709\u9488\u5bf9\u6027\u7684\u4e3b\u52a8\u8d27\u7269\u8fd0\u8f93\u3001\u4e34\u5e8a\u751f\u7269\u533b\u5b66\u5e94\u7528\u4e2d\u5e94\u7528\u7684\u6709\u524d\u9014\u7684\u5de5\u5177\u3002<\/p>\n

\"\"<\/p>\n

Nature Communications\uff1a<\/b><\/strong>\u91c7\u7528\u65e0\u673a-\u6709\u673a\u7ade\u4e89\u5305\u8986\u7b56\u7565\uff0c\u5236\u5907\u4e86\u7528\u4e8e\u8d85\u9ad8\u901f\u548c\u957f\u671f\u9502\u79bb\u5b50\u7535\u6c60\u7684\u5747\u5300\u7a7a\u5fc3\u68af\u5ea6\u7ed3\u6784\u7684\u6c27\u5316\u94c1-\u78b3\u7eb3\u7c73\u7403<\/b><\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff1a\u674e\u4f1f\uff0c\u8d75\u4e1c\u5143\uff09[8]<\/b><\/strong><\/p>\n

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\"\"<\/p>\n

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[1] \u4e2d\u56fd\u79d1\u5b66\u9662\u5316\u5b66\u7269\u7406\u7814\u7a76\u6240\u5b98\u7f51\uff0chttp:\/\/www.dicp.ac.cn\/xwdt\/ttxw\/202111\/t20211103_6241179.html<\/p>\n

[2] Ding Y, Jiao F, Pan X, et al. Effects of Proximity-Dependent Metal Migration on Bifunctional Composites Catalyzed Syngas to Olefins. ACS Catalysis. 2021;11(15):9729-9737.<\/p>\n

[3] Miao D, Pan X, Jiao F, et al. Selective synthesis of para-xylene and light olefins from CO2\/H2 in the presence of toluene. Catalysis Science & Technology. 2021;11(13):4521-4528.<\/p>\n

[4] Wang Y, Ren P, Hu J, et al. Electron penetration triggering interface activity of Pt-graphene for CO oxidation at room temperature. Nat Commun. Oct 4 2021;12(1):5814.<\/p>\n

[5]\u590d\u65e6\u5927\u5b66\u5b98\u7f51\uff0chttps:\/\/news.fudan.edu.cn\/2021\/1103\/c1268a110469\/page.htm<\/p>\n

[6] Lan K, Liu L, Zhang JY, et al. Precisely Designed Mesoscopic Titania for High-Volumetric-Density Pseudocapacitance. J Am Chem Soc. Sep 8 2021;143(35):14097-14105.<\/p>\n

[7] Ma Y, Lan K, Xu B, et al. Streamlined Mesoporous Silica Nanoparticles with Tunable Curvature from Interfacial Dynamic-Migration Strategy for Nanomotors. Nano Lett. Jul 28 2021;21(14):6071-6079.<\/p>\n

[8] Xia Y, Zhao T, Zhu X, et al. Inorganic-organic competitive coating strategy derived uniform hollow gradient-structured ferroferric oxide-carbon nanospheres for ultra-fast and long-term lithium-ion battery. Nat Commun. May 20 2021;12(1):2973.<\/p>\n

\u672c\u6587\u7531\u6625\u56fd\u4f9b\u7a3f\u3002<\/p>\n

\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n

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